Soil microbial communities are key factors in maintaining ecosystem multifunctionality(EMF).However,the distribution patterns of bacterial diversity and how the different bacterial taxa and their diversity dimensions ...Soil microbial communities are key factors in maintaining ecosystem multifunctionality(EMF).However,the distribution patterns of bacterial diversity and how the different bacterial taxa and their diversity dimensions affect EMF remain largely unknown.Here,we investigated variation in three measures of diversity(alpha diversity,community composition and network complexity)among rare,intermediate,and abundant taxa across a latitudinal gradient spanning five forest plots in Yunnan Province,China and examined their contributions on EMF.We aimed to characterize the diversity distributions of bacterial groups across latitudes and to assess the differences in the mechanisms underlying their contributions to EMF.We found that multifaceted diversity(i.e.,diversity assessed by the three different metrics)of rare,intermediate,and abundant bacteria generally decreased with increasing latitude.More importantly,we found that rare bacterial taxa tended to be more diverse,but they contributed less to EMF than intermediate or abundant bacteria.Among the three dimensions of diversity we assessed,only community composition significantly affected EMF across all locations,while alpha diversity had a negative effect,and network complexity showed no significant impact.Our study further emphasizes the importance of intermediate and abundant bacterial taxa as well as community composition to EMF and provides a theoretical basis for investigating the mechanisms by which belowground microorganisms drive EMF along a latitudinal gradient.展开更多
All-solid-state lithium batteries(ASSLBs)are strongly considered as the next-generation energy storage devices for their high energy density and intrinsic safety.The solid-solid contact between lithium metal and solid...All-solid-state lithium batteries(ASSLBs)are strongly considered as the next-generation energy storage devices for their high energy density and intrinsic safety.The solid-solid contact between lithium metal and solid electrolyte plays a vital role in the performance of working ASSLBs,which is challenging to investigate quantitatively by experimental approach.This work proposed a quantitative model based on the finite element method for electrochemical impedance spectroscopy simulation of different solid-solid contact states in ASSLBs.With the assistance of an equivalent circuit model and distribution of relaxation times,it is discovered that as the number of voids and the sharpness of cracks increase,the contact resistance Rcgrows and ultimately dominates the battery impedance.Through accurate fitting,inverse proportional relations between contact resistance Rcand(1-porosity)as well as crack angle was disclosed.This contribution affords a fresh insight into clarifying solid-solid contact states in ASSLBs.展开更多
ZnO-containing slags are common in pyrometallurgical processing of the base metals and steel.This caused the interest to the thermodynamics of the ZnO-SiO2 system.A complete literature survey,critical evaluation of th...ZnO-containing slags are common in pyrometallurgical processing of the base metals and steel.This caused the interest to the thermodynamics of the ZnO-SiO2 system.A complete literature survey,critical evaluation of the available experimental data and a thermodynamic optimization of the phase equilibria and thermodynamic properties of the system ZnO-SiO2 at 1.013×105 Pa are presented.The molten oxide was described as an associate solution.The properties of liquid were reassessed and enthalpy term of the Gibbs energy of solid Zn2SiO4 was re-fitted to be compatible with the new data in the willemite primary phase field.The thermodynamic data set agrees well with the recent experimental observations.It can be used for predicting,e.g.,the thermodynamic properties and the domains of the phase diagram,like critical point of the liquid miscibility gap,with a better accuracy than using the previous assessments.A set of optimized model parameters were obtained,reproducing the reliable thermodynamic and phase equilibrium data within their experimental errors from 298 K to liquidus temperatures,over the entire composition range.The created database can be used in a Gibbs energy minimization software to calculate the thermodynamic properties and the phase diagram sections of interest.展开更多
The development of stretchable conductors with high deformation,conductivity,and thermal conductivity using liquid metal(LM)has sparked widespread interest in the fields of flexible electronics,electromagnetic interfe...The development of stretchable conductors with high deformation,conductivity,and thermal conductivity using liquid metal(LM)has sparked widespread interest in the fields of flexible electronics,electromagnetic interference(EMI),and multifunctional materi-als.However,fabricating desirable shielding materials by directly coating LMs on soft polymer substrates remains a challenge because of the huge surface tension and weak wettability of LMs.In this study,Ga-based composite paste is prepared from a mixture of Ga and dia-mond nonmetallic particles through ultrasonic fragmentation.At various temperatures,the resulting LM composite putty(LMP)exhibits soft and hard properties and can thus be molded into specific shapes according to application needs.In addition,the composite can be eas-ily coated onto polymer substrates,such as thermoplastic polyurethane(TPU)elastomer.The fabricated LMP–TPU exhibits an impress-ive shape deformation capacity of 1100%,demonstrating exceptional tensile properties and achieving electromagnetic interference–shielding effectiveness of up to 52 dB.Furthermore,it retains an ultrahigh conductivity of 20000 S/m,even under a strain of 600%.This feature further makes it a highly competitive multifunctional material.展开更多
Childhood neuroblastoma,a leading cause of cancer-related mortality in young children,accounts for approximately 8%-10%of pediatric cancers1.Originating from neural crest cells of the sympathetic nervous system,these ...Childhood neuroblastoma,a leading cause of cancer-related mortality in young children,accounts for approximately 8%-10%of pediatric cancers1.Originating from neural crest cells of the sympathetic nervous system,these tumors affect primarily children younger than 5 years of age and are often diagnosed in advanced stages,because of their aggressive nature and vague early symptoms2-4.展开更多
1.About CASEE The Chinese Academy of Science and Education Evaluation(CASEE),also known as the Chinese Academy of Evaluation Sciences(CAES),is a key evaluation and research institute established by Hangzhou Dianzi Uni...1.About CASEE The Chinese Academy of Science and Education Evaluation(CASEE),also known as the Chinese Academy of Evaluation Sciences(CAES),is a key evaluation and research institute established by Hangzhou Dianzi University in 2017.Prof.Junping Qiu,a well-known Chinese bibliometrican who has expertise in evaluation management and subsidized by the State Council of China,is the founder and the first president of CASEE.Under the leadership of Prof.Qiu,the CASEE attempts to achieve the following objectives.展开更多
基金supported by the Fundamental Research Funds of Chinese Academy of Forestry(Nos.CAFYBB2022SY037,CAFYBB2021ZA002 and CAFYBB2022QC002)the Basic Research Foundation of Yunnan Province(Grant No.202201AT070264).
文摘Soil microbial communities are key factors in maintaining ecosystem multifunctionality(EMF).However,the distribution patterns of bacterial diversity and how the different bacterial taxa and their diversity dimensions affect EMF remain largely unknown.Here,we investigated variation in three measures of diversity(alpha diversity,community composition and network complexity)among rare,intermediate,and abundant taxa across a latitudinal gradient spanning five forest plots in Yunnan Province,China and examined their contributions on EMF.We aimed to characterize the diversity distributions of bacterial groups across latitudes and to assess the differences in the mechanisms underlying their contributions to EMF.We found that multifaceted diversity(i.e.,diversity assessed by the three different metrics)of rare,intermediate,and abundant bacteria generally decreased with increasing latitude.More importantly,we found that rare bacterial taxa tended to be more diverse,but they contributed less to EMF than intermediate or abundant bacteria.Among the three dimensions of diversity we assessed,only community composition significantly affected EMF across all locations,while alpha diversity had a negative effect,and network complexity showed no significant impact.Our study further emphasizes the importance of intermediate and abundant bacterial taxa as well as community composition to EMF and provides a theoretical basis for investigating the mechanisms by which belowground microorganisms drive EMF along a latitudinal gradient.
基金supported by the Beijing Natural Science Foundation(Z200011,L233004)the National Key Research and Development Program(2021YFB2500300)+3 种基金the National Natural Science Foundation of China(52394170,52394171,22109011,22393900,and 22108151)the Tsinghua-Jiangyin Innovation Special Fund(TJISF)(2022JYTH0101)the S&T Program of Hebei(22344402D)the Tsinghua University Initiative Scientific Research Program.
文摘All-solid-state lithium batteries(ASSLBs)are strongly considered as the next-generation energy storage devices for their high energy density and intrinsic safety.The solid-solid contact between lithium metal and solid electrolyte plays a vital role in the performance of working ASSLBs,which is challenging to investigate quantitatively by experimental approach.This work proposed a quantitative model based on the finite element method for electrochemical impedance spectroscopy simulation of different solid-solid contact states in ASSLBs.With the assistance of an equivalent circuit model and distribution of relaxation times,it is discovered that as the number of voids and the sharpness of cracks increase,the contact resistance Rcgrows and ultimately dominates the battery impedance.Through accurate fitting,inverse proportional relations between contact resistance Rcand(1-porosity)as well as crack angle was disclosed.This contribution affords a fresh insight into clarifying solid-solid contact states in ASSLBs.
基金the financial support of Tekes, Fimecc Oy (SIMP program),Finnish, Metals Producers FundCIMO (Centre for International Movement, an agency of Finnish Ministry of Education and Culture)
文摘ZnO-containing slags are common in pyrometallurgical processing of the base metals and steel.This caused the interest to the thermodynamics of the ZnO-SiO2 system.A complete literature survey,critical evaluation of the available experimental data and a thermodynamic optimization of the phase equilibria and thermodynamic properties of the system ZnO-SiO2 at 1.013×105 Pa are presented.The molten oxide was described as an associate solution.The properties of liquid were reassessed and enthalpy term of the Gibbs energy of solid Zn2SiO4 was re-fitted to be compatible with the new data in the willemite primary phase field.The thermodynamic data set agrees well with the recent experimental observations.It can be used for predicting,e.g.,the thermodynamic properties and the domains of the phase diagram,like critical point of the liquid miscibility gap,with a better accuracy than using the previous assessments.A set of optimized model parameters were obtained,reproducing the reliable thermodynamic and phase equilibrium data within their experimental errors from 298 K to liquidus temperatures,over the entire composition range.The created database can be used in a Gibbs energy minimization software to calculate the thermodynamic properties and the phase diagram sections of interest.
基金supported by the National Natural Science Foundation of China(Nos.52271167 and U21A2064)the Key Program of Natural Science Foundation of Henan Province,China(No.242300421188)+1 种基金ZUA Innovation Fund for Graduate Education,China(No.2024CX134)Henan Key Laboratory of Aeronautical Material and Technology Open Foundation,China(No.ZHKF-240103).
文摘The development of stretchable conductors with high deformation,conductivity,and thermal conductivity using liquid metal(LM)has sparked widespread interest in the fields of flexible electronics,electromagnetic interference(EMI),and multifunctional materi-als.However,fabricating desirable shielding materials by directly coating LMs on soft polymer substrates remains a challenge because of the huge surface tension and weak wettability of LMs.In this study,Ga-based composite paste is prepared from a mixture of Ga and dia-mond nonmetallic particles through ultrasonic fragmentation.At various temperatures,the resulting LM composite putty(LMP)exhibits soft and hard properties and can thus be molded into specific shapes according to application needs.In addition,the composite can be eas-ily coated onto polymer substrates,such as thermoplastic polyurethane(TPU)elastomer.The fabricated LMP–TPU exhibits an impress-ive shape deformation capacity of 1100%,demonstrating exceptional tensile properties and achieving electromagnetic interference–shielding effectiveness of up to 52 dB.Furthermore,it retains an ultrahigh conductivity of 20000 S/m,even under a strain of 600%.This feature further makes it a highly competitive multifunctional material.
基金supported by grants from the National Natural Science Foundation of China(Grant No.82470544)the Fundamental Research Funds for the Central Universities(Grant No.226-2024-00153).
文摘Childhood neuroblastoma,a leading cause of cancer-related mortality in young children,accounts for approximately 8%-10%of pediatric cancers1.Originating from neural crest cells of the sympathetic nervous system,these tumors affect primarily children younger than 5 years of age and are often diagnosed in advanced stages,because of their aggressive nature and vague early symptoms2-4.
文摘1.About CASEE The Chinese Academy of Science and Education Evaluation(CASEE),also known as the Chinese Academy of Evaluation Sciences(CAES),is a key evaluation and research institute established by Hangzhou Dianzi University in 2017.Prof.Junping Qiu,a well-known Chinese bibliometrican who has expertise in evaluation management and subsidized by the State Council of China,is the founder and the first president of CASEE.Under the leadership of Prof.Qiu,the CASEE attempts to achieve the following objectives.
