期刊文献+

交指状流场质子交换膜燃料电池的数值分析 被引量:1

Numerical analysis of proton exchange membrane fuel cell with interdigitated flow fields
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摘要 为研究流场结构设计对电池内的流动、组分传递和电池性能等的影响,建立了一个稳态的三维非等温质子交换膜燃料电池数学模型,应用此模型对一个交指状流场设计的电池单体(电极面积为6.4 cm×6.5 cm)进行了数值研究.数值计算得到了电池的温度、组分质量浓度和局部电流密度等的空间分布,分析了不同电池反应物湿度等对电池特性的影响.结果表明,受传质的影响,沟道下方阴极催化层的温度大于相应沟脊下方的区域;与饱和气流进气的基本工况相比,降低阴极的进气湿度能提高电池的性能,而降低阳极的进气湿度则会导致电池性能的下降. In order to investigate the effects of the flow field structure design on the flow characteristics, species transport and cell performance, a steady-state three-dimensional non-isothermal mathematical mod- el based on computation fluid dynamics was presented. The developed mathematical model was employed to numerically study a single proton exchange membrane fuel cell with interdigitated flow fields (with the electrode area of 6.4 cm ×6.5 cm), and the spatial distributions of temperature, species concentration and local current density were obtained. Furthermore, the effect of different reactant humidity on the cell performance was discussed. The results indicate that the temperature in the cathode catalyst layer under the channel is higher than that under the shoulder; compared with the case of saturated inlet reactants, the decrease of cathode gas relative humidity will enhance the cell performance, while the decrease of anode gas relative humidity will reduce the cell performance.
出处 《浙江大学学报(工学版)》 EI CAS CSCD 北大核心 2009年第6期1147-1151,共5页 Journal of Zhejiang University:Engineering Science
基金 国家自然科学基金资助项目(50806068 50706045) 教育部科学技术研究重点资助项目(207043) 浙江省自然科学基金资助项目(Y106161) 能源清洁利用国家重点实验室开放课题资助项目(ZJUCEU2008001)
关键词 质子交换 膜燃料电池 交指状流场 两相流 组分传递 proton exchange membrane fuel cell interdigitated flow field two-phase flow species transport
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参考文献12

  • 1BERNARDI D M,VERBRUGGE M W.A mathematical model of the solid-polymer-electrolyte fuel cell[J].Journal Electrochem Soc,1992,139:2477-2491.
  • 2NGUYEN T V,WHITE R E.A water and heat management model for proton-exchange-membrane fuel cells[J].Journal Electrochem Soc,1993,140(8):2178-2186.
  • 3GURAU V,LIU H T,SADIK K.Two-dimensional model for proton exchange membrane fuel cells[J].AICHE Journal,1998,44(11):2410-2422.
  • 4BERNING T,LU D M,DJILALIN.Three-dimensional computational analysis of transport phenomena in a PEM fuel cell[J].Journal Power Sources,2002,106(1):284-294.
  • 5DUTTA S,SHIMPALEE S,VAN ZEE J W.Three-dimensional numerical simulation of straight channel PEM fuel cells[J].Journal Appl Electrochem,2000,30:135-146.
  • 6MENG H.Numerical investigation of transient responses of a PEM fuel cell using a two-phase non-isothermal mixed-domain model[J].Journal of Power Sources,2007,171(2):738-46.
  • 7WANG Z H,WANG C Y,CHEN K S.Two-phase flow and transport in the air cathode of proton exchange membrane fuel cell[J].Journal Power Sources,2001,94(1):40-50.
  • 8NATARAJAN D,NGUYEN V T.A two-dimensional,two-phase,multicomponent,transient model for the cathode of a proton exchange membrane fuel cell using conventional gas distributors[J].Journal Electrochem Soc,2001,148(12):A1324-1335.
  • 9胡桂林,樊建人,岑可法.复杂流道质子交换膜燃料电池的三维数值分析[J].浙江大学学报(工学版),2005,39(7):1019-1024. 被引量:9
  • 10KAZIM A,LIU H T,FORGES P.Modeling of performance of PEM fuel cells with conventional and interdigitated flow fields[J].Journal Appl Electrochem,1999,29(12):1409-1416.

二级参考文献25

  • 1胡桂林,樊建人,岑可法.复杂流道质子交换膜燃料电池的三维数值分析[J].浙江大学学报(工学版),2005,39(7):1019-1024. 被引量:9
  • 2胡桂林,樊建人.质子交换膜燃料电池内电荷传递的数值模拟[J].能源工程,2007,27(4):9-14. 被引量:1
  • 3BERNARDI D M, VERBRUGGE M W. A mathematical model of the solid-polymer-electrolyte fuel cell[J]. Journal of Electrochemical Society, 1992,139: 2477 - 2491.
  • 4SPRINGER T E, WILSON M S, GOTTESFELD S. Modeling and experimental diagnostics in polymer electrolyte fuel cells[J]. Journal of Electrochemical Society, 1993, 140(12): 513 - 3526.
  • 5ROWE A, LI X. Mathematical modeling of proton exchange membrane fuel cells[J]. Journal of Power Sources, 2001, 102: 82 - 96.
  • 6FULLER T F, NEWMAN J. Water and thermal management in solid-polymer-electrolyte fuel cells[J]. Journal of Electrochemical Society, 1993,140:1218 - 1225.
  • 7NGUYEN T V, WHITE R E. A water and heat management model for proton-exchange-membrane fuel cells[J]. Journal of Electrochemical Society, 1993, 140(8): 2178 - 2186.
  • 8YI J S, NGUYEN T V. An along-the-channel model for proton exchange membrane fuel cells[J]. Journal of Electrochemical Society, 1998, 145(4): 1149 - 1159.
  • 9GURAU V, LIU H, KAKAC S. Two-dimensional model for proton exchange membrane fuel cells[J]. AICHE Journal, 1998, 44: 2410 - 2422.
  • 10DUTTA S, SHIMPALEE S, VAN ZEE J W. Three-dimensional numerical simulation of straight channel PEM fuel cells[J]. Journal of Applicated Electrochemistry, 2000, 30: 135 - 146.

共引文献8

同被引文献20

  • 1刘朝玮,王保国,何小荣.质子交换膜燃料电池研究及应用现状[J].现代化工,2004,24(9):10-13. 被引量:5
  • 2谢晋,黄允千.温度、湿度对质子交换膜燃料电池性能的影响[J].上海海事大学学报,2005,26(3):60-63. 被引量:12
  • 3丁刚强,罗志平,潘牧.温度、流量和湿度对单蛇形流场PEMFC的影响[J].电池,2006,36(3):178-180. 被引量:4
  • 4WANG Y, CHEN K S, MISHLER J, et al. A review of polymer electrolyte membrane fuel cells: technology, applications, and needs on fundamental research [J]. Applied Energy, 2011, 88(4): 981-1007.
  • 5YOUSFI STEINER N, MOOTGUY P, CANDUSSO D, et al. A review on PEM voltage degradation associated with water management: Impacts, influent factors and characterization [J]. Journal of Power Sources, 2008, 183(1): 260-274.
  • 6WONG K H, LOO K H, LAI Y M, et al. A theoretical study of inlet relative humidity control in PEM fuel cell [J]. International Journal of Hydrogen Energy, 2011, 36(18): 11871-11885.
  • 7WANG L, HUSAR A, ZHOU T, et al. A parametric study of PEM fuel cell performances [J]. International Journal of Hydrogen Energy, 2003, 28(11): 1263-1272.
  • 8HYUN D, KIM J. Study of external humidification method in proton exchange membrane fuel cell [J]. Journal of Power Sources, 2004, 126(1): 98-103.
  • 9AMIRINEJAD M, ROWSHANZAMIR S, EIKANI M H. Effects of operating parameters on performance of a proton exchange membrane fuel cell [J]. Journal of Power Sources, 2006, 161(2): 872-875.
  • 10LIN R, CAO C, MA J, et al. Optimizing the relative humidity to improve the stability of a proton exchange membrane by segmented fuel cell technology [J]. International Journal of Hydrogen Energy, 2012, 37(4): 3373-3381.

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