To fully utilize the resources provided by optical fiber networks,a cross-band quantum light source generating photon pairs,where one photon in a pair is at C band and the other is at O band,is proposed in this work.T...To fully utilize the resources provided by optical fiber networks,a cross-band quantum light source generating photon pairs,where one photon in a pair is at C band and the other is at O band,is proposed in this work.This source is based on spontaneous four-wave mixing(SFWM)in a piece of shallow-ridge silicon waveguide.Theoretical analysis shows that the waveguide dispersion could be tailored by adjusting the ridge width,enabling broadband photon pair generation by SFWM across C band and O band.The spontaneous Raman scattering(SpRS)in silicon waveguides is also investigated experimentally.It shows that there are two regions in the spectrum of generated photons from SpRS,which could be used to achieve cross-band photon pair generation.A chip of shallow-ridge silicon waveguide samples with different ridge widths has been fabricated,through which cross-band photon pair generation is demonstrated experimentally.The experimental results show that the source can be achieved using dispersion-optimized shallow-ridge silicon waveguides.This cross-band quantum light source provides a way to develop new fiber-based quantum communication functions utilizing both C band and O band and extends applications of quantum networks.展开更多
Scalability remains a major challenge in building practical fault-tolerant quantum computers.Currently,the largest number of qubits achieved across leading quantum platforms ranges from hundreds to thousands.In atom a...Scalability remains a major challenge in building practical fault-tolerant quantum computers.Currently,the largest number of qubits achieved across leading quantum platforms ranges from hundreds to thousands.In atom arrays,scalability is primarily constrained by the capacity to generate large numbers of optical tweezers,and conventional techniques using acousto-optic deflectors or spatial light modulators struggle to produce arrays much beyond∼10,000 tweezers.Moreover,these methods require additional microscope objectives to focus the light into micrometer-sized spots,which further complicates system integration and scalability.Here,we demonstrate the experimental generation of an optical tweezer array containing 280×280 spots using a metasurface,nearly an order of magnitude more than most existing systems.The metasurface leverages a large number of subwavelength phase-control pixels to engineer the wavefront of the incident light,enabling both large-scale tweezer generation and direct focusing into micron-scale spots without the need for a microscope.This result shifts the scalability bottleneck for atom arrays from the tweezer generation hardware to the available laser power.Furthermore,the array shows excellent intensity uniformity exceeding 90%,making it suitable for homogeneous single-atom loading and paving the way for trapping arrays of more than 10,000 atoms in the near future.展开更多
Quantum information processing based on Rydberg atoms emerged as a promising direction two decades ago.Recent experimental and theoretical progresses have shined exciting light on this avenue.In this concise review,we...Quantum information processing based on Rydberg atoms emerged as a promising direction two decades ago.Recent experimental and theoretical progresses have shined exciting light on this avenue.In this concise review,we will briefly introduce the basics of Rydberg atoms and their recent applications in associated areas of neutral atom quantum computation and simulation.We shall also include related discussions on quantum optics with Rydberg atomic ensembles,which are increasingly used to explore quantum computation and quantum simulation with photons.展开更多
Artificially constructed van der Waals heterostructures(vdWHs)provide an ideal platform for realizing emerging quantum phenomena in condensed matter physics.Two methods for building vdWHs have been developed:stacking ...Artificially constructed van der Waals heterostructures(vdWHs)provide an ideal platform for realizing emerging quantum phenomena in condensed matter physics.Two methods for building vdWHs have been developed:stacking two-dimensional(2D)materials into a bilayer structure with different lattice constants,or with different orientations.The interlayer coupling stemming from commensurate or incommensurate superlattice pattern plays an important role in vdWHs for modulating the band structures and generating new electronic states.In this article,we review a series of novel quantum states discovered in two model vdWH systems—graphene/hexagonal boron nitride(hBN)hetero-bilayer and twisted bilayer graphene(tBLG),and discuss how the electronic structures are modified by such stacking and twisting.We also provide perspectives for future studies on hetero-bilayer materials,from which an expansion of 2D material phase library is expected.展开更多
We demonstrate the in situ growth of ultra-thin InA s nanowires with an epitaxial Al film by molecular-beam epitaxy.Our InAs nanowire diameter(~30 nm)is much thinner than before(~100 nm).The ultra-thin InAs nanowires ...We demonstrate the in situ growth of ultra-thin InA s nanowires with an epitaxial Al film by molecular-beam epitaxy.Our InAs nanowire diameter(~30 nm)is much thinner than before(~100 nm).The ultra-thin InAs nanowires are pure phase crystals for various different growth directions.Transmission electron microscopy confirms an atomically abrupt and uniform interface between the Al shell and the InAs wire.Quantum transport study on these devices resolves a hard induced superconducting gap and 2 e-periodic Coulomb blockade at zero magnetic field,a necessary step for future Majorana experiments.By reducing wire diameter,our work presents a promising route for reaching fewer sub-band regime in Major ana nanowire devices.展开更多
Topological superconductors(TSCs)have been widely investigated in recent years due to their novel physics and ability to host Majorana fermions(MFs)which are key to topological quantum computation.Despite the great in...Topological superconductors(TSCs)have been widely investigated in recent years due to their novel physics and ability to host Majorana fermions(MFs)which are key to topological quantum computation.Despite the great interest,only a few compounds have been proposed as candidates of intrinsic TSCs,such as iron-based superconductor FeSe_(0.55)Te_(0.45) and 2M-WS_(2).Among them,quasi-one-dimensional superconductor TaSe_(3) possesses fascinating properties such as its simple stoichiometry,layered nature and chemical stability.Here,using scanning tunneling microscope/spectroscopy(STM/STS),we systematically investigate the topography and electronic structure of TaSe_(3).Our STM/STS measurement reveals large atomically flat,defect-free surfaces suitable for the search of MF;electronic density of states consistent with our angle-resolved photoemission result and band-structure calculations,and a uniform superconducting gap with a typical size of∼0.25 meV.Remarkably,additional edge states are observed in the vicinity of the terrace edge,suggesting they may have a topological origin.Our result proves the coexistence of superconductivity and topological electronic structure in TaSe_(3),making it an intriguing platform to investigate topological superconductivity.展开更多
We have developed a low-damage photolithography method for magnetically doped(Bi,Sb)_(2)Te_(3)quantum anomalous Hall(QAH) thin films incorporating an additional resist layer of poly(methyl methacrylate)(PMMA). By perf...We have developed a low-damage photolithography method for magnetically doped(Bi,Sb)_(2)Te_(3)quantum anomalous Hall(QAH) thin films incorporating an additional resist layer of poly(methyl methacrylate)(PMMA). By performing control experiments on the transport properties of five devices at varied gate voltages(V_(g)s), we revealed that the modified photolithography method enables fabricating QAH devices with the transport and magnetic properties unaffected by fabrication process. Our experiment represents a step towards the production of novel micro-structured electronic devices based on the dissipationless QAH chiral edge states.展开更多
Angle-resolved photoemission spectroscopy(ARPES)and torque magnetometry(TM)measurements have been carried out to study the electronic structures of a correlated topological insulator(TI)candidate Yb B6.We observed cle...Angle-resolved photoemission spectroscopy(ARPES)and torque magnetometry(TM)measurements have been carried out to study the electronic structures of a correlated topological insulator(TI)candidate Yb B6.We observed clear surface states on the[001]surface centered at theГ^- and М^- points of the surface Brillouin zone.Interestingly,the fermiology revealed by the quantum oscillation of TM measurements agrees excellently with ARPES measurements.Moreover,the band structures we observed suggest that the band inversion in Yb B6 happens between the Yb5 dand B2bands,instead of the Yb5dand Yb4fbands as suggested by previous theoretical investigation,which will help settle the heavy debate regarding the topological nature of samarium/ytterbium hexaborides.展开更多
The thickness dependence of linearly polarized light-induced momentum anisotropy and the inverse spin Hall effect(PISHE)in topological insulator(TI)Bi_(2)Te_(3)films has been investigated.A significant enhancement of ...The thickness dependence of linearly polarized light-induced momentum anisotropy and the inverse spin Hall effect(PISHE)in topological insulator(TI)Bi_(2)Te_(3)films has been investigated.A significant enhancement of the PISHE signal is observed in the 12-quintuple-layer(QL)Bi_(2)Te_(3)film compared with that of the 3-and 5-QL samples,whereas a minimal value of photoinduced momentum anisotropy is found in the 12-QL sample.The photoinduced momentum anisotropy and the PISHE in Bi_(2)Te_(3)films are more than three and two orders of magnitude larger than those in Bi2Se3 films grown on SrTiO_(3)substrates,respectively.The 3-QL sample exhibits a sinusoidal dependence of the PISHE current on the light spot position,while the 5-QL and 12-QL samples show aW-shaped dependence,which arises from the different angles between the coordinate axis x and the in-plane crystallographic axis of the Bi_(2)Te_(3)films.Our findings demonstrate the critical role of film thickness in modulating both the photoinduced momentum anisotropy and the PISHE current,thereby suggesting a thickness-engineering strategy for designing novel optoelectronic devices based on TIs.展开更多
Recent experimental evidence of the charge-6e condensed phase in Kagome superconductors has generated significant interest.This study investigates the unconventional superconductivity in the Kagome superconductor CsV_...Recent experimental evidence of the charge-6e condensed phase in Kagome superconductors has generated significant interest.This study investigates the unconventional superconductivity in the Kagome superconductor CsV_(3)Sb_(5),focusing on the emergence of charge-6e superconductivity(SC)at temperatures higher than the conventional charge-2e SC state.By modeling the phase coherence of the SC order parameter using a frustrated antiferromagnetic XY model on an emergent Kagome lattice,the condensation of fractional vortices with 1/3 vorticity stabilizes the phase coherence in exp(i3θ),resulting in a charge-6e SC state.Using a tensor network approach tailored for frustrated spin systems,a Berezinskii-Kosterlitz-Thouless transition is identified at T_(c)/J≃0.075,where the unbinding of 1/3 fractional vortex-antivortex pairs transforms the system from the charge-6e SC phase to the normal phase.Below T_(c),the 1/3 fractional vortex correlations exhibit a power-law decay,whereas the integer vortex correlations decay exponentially,reflecting the dominance of charge-6e SC in the absence of charge-2e SC.The results provide a theoretical understanding of charge-6e SC in two-dimensional Kagome superconductors,emphasizing the interaction between fractional vortices,frustration,and topology in stabilizing the exotic SC phase.展开更多
An intrinsic magnetic topological insulator(TI) is a stoichiometric magnetic compound possessing both inherent magnetic order and topological electronic states. Such a material can provide a shortcut to various novel ...An intrinsic magnetic topological insulator(TI) is a stoichiometric magnetic compound possessing both inherent magnetic order and topological electronic states. Such a material can provide a shortcut to various novel topological quantum effects but remained elusive experimentally for a long time. Here we report the experimental realization of thin films of an intrinsic magnetic TI, MnBi2Te4, by alternate growth of a Bi2Te3 quintuple layer and a MnTe bilayer with molecular beam epitaxy. The material shows the archetypical Dirac surface states in angle-resolved photoemission spectroscopy and is demonstrated to be an antiferromagnetic topological insulator with ferromagnetic surfaces by magnetic and transport measurements as well as first-principles calculations. The unique magnetic and topological electronic structures and their interplays enable the material to embody rich quantum phases such as quantum anomalous Hall insulators and axion insulators at higher temperature and in a well-controlled way.展开更多
The dimensionality of quantum materials strongly affects their physical properties.Although many emergent phenomena,such as charge-density wave and Luttinger liquid behavior,are well understood in one-dimensional(1D)s...The dimensionality of quantum materials strongly affects their physical properties.Although many emergent phenomena,such as charge-density wave and Luttinger liquid behavior,are well understood in one-dimensional(1D)systems,the generalization to explore them in higher dimensional systems is still a challenging task.In this study,we aim to bridge this gap by systematically investigating the crystal and electronic structures of molybdenum-oxide family compounds,where the contexture of 1D chains facilitates rich emergent properties.While the quasi-1D chains in these materials share general similarities,such as the motifs made up of MoO_(6)octahedrons,they exhibit vast complexity and remarkable tunability.We disassemble the 1D chains in molybdenum oxides with different dimensions and construct effective models to excellently fit their low-energy electronic structures obtained by ab initio calculations.Furthermore,we discuss the implications of such chains on other physical properties of the materials and the practical significance of the effective models.Our work establishes the molybdenum oxides as simple and tunable model systems for studying and manipulating the dimensionality in quantum systems.展开更多
We train a neural network to identify impurities in the experimental images obtained by the scanning tunneling microscope(STM)measurements.The neural network is first trained with a large number of simulated data and ...We train a neural network to identify impurities in the experimental images obtained by the scanning tunneling microscope(STM)measurements.The neural network is first trained with a large number of simulated data and then the trained neural network is applied to identify a set of experimental images taken at different voltages.We use the convolutional neural network to extract features from the images and also implement the attention mechanism to capture the correlations between images taken at different voltages.We note that the simulated data can capture the universal Friedel oscillation but cannot properly describe the non-universal physics short-range physics nearby an impurity,as well as noises in the experimental data.And we emphasize that the key of this approach is to properly deal with these differences between simulated data and experimental data.Here we show that even by including uncorrelated white noises in the simulated data,the performance of the neural network on experimental data can be significantly improved.To prevent the neural network from learning unphysical short-range physics,we also develop another method to evaluate the confidence of the neural network prediction on experimental data and to add this confidence measure into the loss function.We show that adding such an extra loss function can also improve the performance on experimental data.Our research can inspire future similar applications of machine learning on experimental data analysis.展开更多
Monolayer group VI transition metal dichalcogenides(TMDs)have recently emerged as promising candidates for photonic and opto-valleytronic applications.The optoelectronic properties of these atomically-thin semiconduct...Monolayer group VI transition metal dichalcogenides(TMDs)have recently emerged as promising candidates for photonic and opto-valleytronic applications.The optoelectronic properties of these atomically-thin semiconducting crystals are strongly governed by the tightly bound electron-hole pairs such as excitons and trions(charged excitons).The anomalous spin and valley configurations at the conduction band edges in monolayer WS_(2)give rise to even more fascinating valley many-body complexes.Here we find that the indirect Q valley in the first Brillouin zone of monolayer WS_(2)plays a critical role in the formation of a new excitonic state,which has not been well studied.By employing a high-quality h-BN encapsulated WS_(2)field-effect transistor,we are able to switch the electron concentration within K-Q valleys at conduction band edges.Consequently,a distinct emission feature could be excited at the high electron doping region.Such feature has a competing population with the K valley trion,and experiences nonlinear power-law response and lifetime dynamics under doping.Our findings open up a new avenue for the study of valley many-body physics and quantum optics in semiconducting 2D materials,as well as provide a promising way of valley manipulation for next-generation entangled photonic devices.展开更多
Iron-based superconductor family FeX(X=S,Se,Te)has been one of the research foci in physics and material science due to their record-breaking superconducting temperature(FeSe film)and rich physical phenomena.Recently,...Iron-based superconductor family FeX(X=S,Se,Te)has been one of the research foci in physics and material science due to their record-breaking superconducting temperature(FeSe film)and rich physical phenomena.Recently,FeS,the least studied Fe X compound(due to the difficulty in synthesizing high quality macroscopic crystals)attracted much attention because of its puzzling superconducting pairing symmetry.In this work,combining scanning tunneling microscopy and angle resolved photoemission spectroscopy(ARPES)with sub-micron spatial resolution,we investigate the intrinsic electronic structures of superconducting FeS from individual single crystalline domains.Unlike FeTe or FeSe,FeS remains identical tetragonal structure from room temperature down to 5 K,and the band structures observed can be well reproduced by our ab-initio calculations.Remarkably,mixed with the 1×1 tetragonal metallic phase,we also observe the coexistence of √5×√5 reconstructed insulating phase in the crystal,which not only helps explain the unusual properties of FeS,but also demonstrates the importance of using spatially resolved experimental tools in the study of this compound.展开更多
We introduce Quafu-Qcover,an open-source cloud-based software package developed for solving combinatorial optimization problems using quantum simulators and hardware backends.Quafu-Qcover provides a standardized and c...We introduce Quafu-Qcover,an open-source cloud-based software package developed for solving combinatorial optimization problems using quantum simulators and hardware backends.Quafu-Qcover provides a standardized and comprehensive workflow that utilizes the quantum approximate optimization algorithm(QAOA).It facilitates the automatic conversion of the original problem into a quadratic unconstrained binary optimization(QUBO)model and its corresponding Ising model,which can be subsequently transformed into a weight graph.The core of Qcover relies on a graph decomposition-based classical algorithm,which efficiently derives the optimal parameters for the shallow QAOA circuit.Quafu-Qcover incorporates a dedicated compiler capable of translating QAOA circuits into physical quantum circuits that can be executed on Quafu cloud quantum computers.Compared to a general-purpose compiler,our compiler demonstrates the ability to generate shorter circuit depths,while also exhibiting superior speed performance.Additionally,the Qcover compiler has the capability to dynamically create a library of qubits coupling substructures in real-time,utilizing the most recent calibration data from the superconducting quantum devices.This ensures that computational tasks can be assigned to connected physical qubits with the highest fidelity.The Quafu-Qcover allows us to retrieve quantum computing sampling results using a task ID at any time,enabling asynchronous processing.Moreover,it incorporates modules for results preprocessing and visualization,facilitating an intuitive display of solutions for combinatorial optimization problems.We hope that Quafu-Qcover can serve as an instructive illustration for how to explore application problems on the Quafu cloud quantum computers.展开更多
With the rapid advancement of quantum computing,hybrid quantum–classical machine learning has shown numerous potential applications at the current stage,with expectations of being achievable in the noisy intermediate...With the rapid advancement of quantum computing,hybrid quantum–classical machine learning has shown numerous potential applications at the current stage,with expectations of being achievable in the noisy intermediate-scale quantum(NISQ)era.Quantum reinforcement learning,as an indispensable study,has recently demonstrated its ability to solve standard benchmark environments with formally provable theoretical advantages over classical counterparts.However,despite the progress of quantum processors and the emergence of quantum computing clouds,implementing quantum reinforcement learning algorithms utilizing parameterized quantum circuits(PQCs)on NISQ devices remains infrequent.In this work,we take the first step towards executing benchmark quantum reinforcement problems on real devices equipped with at most 136 qubits on the BAQIS Quafu quantum computing cloud.The experimental results demonstrate that the policy agents can successfully accomplish objectives under modified conditions in both the training and inference phases.Moreover,we design hardware-efficient PQC architectures in the quantum model using a multi-objective evolutionary algorithm and develop a learning algorithm that is adaptable to quantum devices.We hope that the Quafu-RL can be a guiding example to show how to realize machine learning tasks by taking advantage of quantum computers on the quantum cloud platform.展开更多
Large superconducting Fe Se crystals of（001） orientation have been prepared via a hydrothermal ion release/introduction route for the first time. The hydrothermally derived Fe Se crystals are up to 10 mm×5 mm&#...Large superconducting Fe Se crystals of（001） orientation have been prepared via a hydrothermal ion release/introduction route for the first time. The hydrothermally derived Fe Se crystals are up to 10 mm×5 mm×0.3 mm in dimension. The pure tetragonal FeSe phase has been confirmed by x-ray diffraction（XRD） and the composition determined by both inductively coupled plasma atomic emission spectroscopy（ICP-AES） and energy dispersive x-ray spectroscopy（EDX）. The superconducting transition of the Fe Se samples has been characterized by magnetic and transport measurements. The zero-temperature upper critical field H（c2） is calculated to be 13.2–16.7 T from a two-band model. The normal-state cooperative paramagnetism is found to be predominated by strong spin frustrations below the characteristic temperature T（sn）, where the Ising spin nematicity has been discerned in the FeSe superconductor crystals as reported elsewhere.展开更多
Atomically thin transition metal dichalcogenide films with distorted trigonal(1T') phase have been predicted to be candidates for realizing quantum spin Hall effect. Growth of 1T' film and experimental investi...Atomically thin transition metal dichalcogenide films with distorted trigonal(1T') phase have been predicted to be candidates for realizing quantum spin Hall effect. Growth of 1T' film and experimental investigation of its electronic structure are critical. Here we report the electronic structure of 1T'-MoTe2 films grown by molecular beam epitaxy(MBE).Growth of the 1T'-MoTe2 film depends critically on the substrate temperature, and successful growth of the film is indicated by streaky stripes in the reflection high energy electron diffraction(RHEED) and sharp diffraction spots in the low energy electron diffraction(LEED). Angle-resolved photoemission spectroscopy(ARPES) measurements reveal a metallic behavior in the as-grown film with an overlap between the conduction and valence bands. First principles calculation suggests that a suitable tensile strain along the a-axis direction is needed to induce a gap to make it an insulator. Our work not only reports the electronic structure of MBE grown 1T'-MoTe2 films, but also provides insights for strain engineering to make it possible for quantum spin Hall effect.展开更多
Our recent scanning tunneling microscopy （STM） studies of the NaFelxCoxAs phase diagram over a wide range of dopings and temperatures are reviewed. Similar to the high-Tc cuprates, the iron-based superconductors lie...Our recent scanning tunneling microscopy （STM） studies of the NaFelxCoxAs phase diagram over a wide range of dopings and temperatures are reviewed. Similar to the high-Tc cuprates, the iron-based superconductors lie in close proximity to a magnetically ordered phase. Therefore, it is widely believed that magnetic interactions or fluctuations play an important role in triggering their Cooper pairings. Among the key issues regarding the electronic phase diagram are the properties of the parent spin density wave （SDW） phase and the superconducting （SC） phase, as well as the interplay between them. The NaFe l-xCoxAs is an ideal system for resolving these issues due to its rich electronic phases and the charge-neutral cleaved surface. In our recent work, we directly observed the SDW gap in the parent state, and it exhibits unconventional features that are incompatible with the simple Fermi surface nesting picture. The optimally doped sample has a single SC gap, but in the underdoped regime we directly viewed the microscopic coexistence of the SDW and SC orders, which compete with each other. In the overdoped regime we observed a novel pseudogap-like feature that coexists with supercon- ductivity in the ground state, persists well into the normal state, and shows great spatial variations. The rich electronic structures across the phase diagram of NaFel_xCoxAs revealed here shed important new light for defining microscopic models of the iron-based superconductors. In particular, we argue that both the itinerant electrons and local moments should be considered on an equal footing in a realistic model.展开更多
基金supported by the Quantum Science and Technology-National Science and Technology Major Project (Grant No.2024ZD0302502 for WZ)the National Natural Science Foundation of China(Grant No.92365210 for WZ)+1 种基金Tsinghua Initiative Scientific Research Program (for WZ)the project of Tsinghua University-Zhuhai Huafa Industrial Share Company Joint Institute for Architecture Optoelectronic Technologies (JIAOT,for YH)。
文摘To fully utilize the resources provided by optical fiber networks,a cross-band quantum light source generating photon pairs,where one photon in a pair is at C band and the other is at O band,is proposed in this work.This source is based on spontaneous four-wave mixing(SFWM)in a piece of shallow-ridge silicon waveguide.Theoretical analysis shows that the waveguide dispersion could be tailored by adjusting the ridge width,enabling broadband photon pair generation by SFWM across C band and O band.The spontaneous Raman scattering(SpRS)in silicon waveguides is also investigated experimentally.It shows that there are two regions in the spectrum of generated photons from SpRS,which could be used to achieve cross-band photon pair generation.A chip of shallow-ridge silicon waveguide samples with different ridge widths has been fabricated,through which cross-band photon pair generation is demonstrated experimentally.The experimental results show that the source can be achieved using dispersion-optimized shallow-ridge silicon waveguides.This cross-band quantum light source provides a way to develop new fiber-based quantum communication functions utilizing both C band and O band and extends applications of quantum networks.
基金supported by the National Natural Science Foundation of China (Grant No.92576208)Tsinghua University Initiative Scientific Research Program+1 种基金Beijing Science and Technology Planning ProjectTsinghua University Dushi Program。
文摘Scalability remains a major challenge in building practical fault-tolerant quantum computers.Currently,the largest number of qubits achieved across leading quantum platforms ranges from hundreds to thousands.In atom arrays,scalability is primarily constrained by the capacity to generate large numbers of optical tweezers,and conventional techniques using acousto-optic deflectors or spatial light modulators struggle to produce arrays much beyond∼10,000 tweezers.Moreover,these methods require additional microscope objectives to focus the light into micrometer-sized spots,which further complicates system integration and scalability.Here,we demonstrate the experimental generation of an optical tweezer array containing 280×280 spots using a metasurface,nearly an order of magnitude more than most existing systems.The metasurface leverages a large number of subwavelength phase-control pixels to engineer the wavefront of the incident light,enabling both large-scale tweezer generation and direct focusing into micron-scale spots without the need for a microscope.This result shifts the scalability bottleneck for atom arrays from the tweezer generation hardware to the available laser power.Furthermore,the array shows excellent intensity uniformity exceeding 90%,making it suitable for homogeneous single-atom loading and paving the way for trapping arrays of more than 10,000 atoms in the near future.
基金Project supported by the National Key R&D Program of China(Grant Nos.2018YFA0306504 and 2018YFA0306503)the Key-Area Research and Development Program of Guang Dong Province,China(Grant No.2019B030330001)+1 种基金the National Natural Science Foundation of China(Grant Nos.91636213,11654001,91736311,91836302,and U1930201)support from Beijing Academy of Quantum Information Sciences(BAQIS)Research Program(Grant No.Y18G24)。
文摘Quantum information processing based on Rydberg atoms emerged as a promising direction two decades ago.Recent experimental and theoretical progresses have shined exciting light on this avenue.In this concise review,we will briefly introduce the basics of Rydberg atoms and their recent applications in associated areas of neutral atom quantum computation and simulation.We shall also include related discussions on quantum optics with Rydberg atomic ensembles,which are increasingly used to explore quantum computation and quantum simulation with photons.
基金support from the National Natural Science Foundation of China(Grant No.11725418)the National Key Research and Development Program of China(Grant No.2016YFA0301004)+3 种基金Science Challenge Project,China(Grant No.TZ2016004)Beijing Advanced Innovation Center for Future Chip(ICFC)Tsinghua University Initiative Scientific Research Programfunded by the Deutsche Forschungsgemeinschaft(DFG,German Research Foundation)–TRR 173–268565370(projects A02)。
文摘Artificially constructed van der Waals heterostructures(vdWHs)provide an ideal platform for realizing emerging quantum phenomena in condensed matter physics.Two methods for building vdWHs have been developed:stacking two-dimensional(2D)materials into a bilayer structure with different lattice constants,or with different orientations.The interlayer coupling stemming from commensurate or incommensurate superlattice pattern plays an important role in vdWHs for modulating the band structures and generating new electronic states.In this article,we review a series of novel quantum states discovered in two model vdWH systems—graphene/hexagonal boron nitride(hBN)hetero-bilayer and twisted bilayer graphene(tBLG),and discuss how the electronic structures are modified by such stacking and twisting.We also provide perspectives for future studies on hetero-bilayer materials,from which an expansion of 2D material phase library is expected.
基金supported by the National Natural Science Foundation of China(Grant Nos.92065106,61974138,12104053,and 11704364)the Beijing Natural Science Foundation(Grant No.1192017)+2 种基金Tsinghua University Initiative Scientifc Research Programthe support from Youth Innovation Promotion Association,Chinese Academy of Sciences(Grant No.Y2021043)China Postdoctoral Science Foundation(Grant Nos.2020M670173 and 2020T130058)。
文摘We demonstrate the in situ growth of ultra-thin InA s nanowires with an epitaxial Al film by molecular-beam epitaxy.Our InAs nanowire diameter(~30 nm)is much thinner than before(~100 nm).The ultra-thin InAs nanowires are pure phase crystals for various different growth directions.Transmission electron microscopy confirms an atomically abrupt and uniform interface between the Al shell and the InAs wire.Quantum transport study on these devices resolves a hard induced superconducting gap and 2 e-periodic Coulomb blockade at zero magnetic field,a necessary step for future Majorana experiments.By reducing wire diameter,our work presents a promising route for reaching fewer sub-band regime in Major ana nanowire devices.
基金Supported by the National Key R&D Program of China(Grant No.2017YFA0305400)the Shanghai Technology Innovation Action Plan 2020-Integrated Circuit Technology Support Program(Grant No.20DZ1100605)+2 种基金the National Natural Science Foundation of China(Grant Nos.52072168,21733001,51861145201,U1932217,and 11974246)the National Key Basic Research Program of China(Grant No.2018YFA0306200)the Science and Technology Commission of Shanghai Municipality(Grant No.19JC1413900).
文摘Topological superconductors(TSCs)have been widely investigated in recent years due to their novel physics and ability to host Majorana fermions(MFs)which are key to topological quantum computation.Despite the great interest,only a few compounds have been proposed as candidates of intrinsic TSCs,such as iron-based superconductor FeSe_(0.55)Te_(0.45) and 2M-WS_(2).Among them,quasi-one-dimensional superconductor TaSe_(3) possesses fascinating properties such as its simple stoichiometry,layered nature and chemical stability.Here,using scanning tunneling microscope/spectroscopy(STM/STS),we systematically investigate the topography and electronic structure of TaSe_(3).Our STM/STS measurement reveals large atomically flat,defect-free surfaces suitable for the search of MF;electronic density of states consistent with our angle-resolved photoemission result and band-structure calculations,and a uniform superconducting gap with a typical size of∼0.25 meV.Remarkably,additional edge states are observed in the vicinity of the terrace edge,suggesting they may have a topological origin.Our result proves the coexistence of superconductivity and topological electronic structure in TaSe_(3),making it an intriguing platform to investigate topological superconductivity.
基金supported by the National Key Research and Development Program of China (Grant No. 2018YFA0307100)the Basic Science Center Project of the National Natural Science Foundation of China (Grant No. 52388201)+4 种基金the National Natural Science Foundation of China (Grant Nos. 12274453 and 92065206)the Innovation Program for Quantum Science and Technology (Grant No. 2021ZD0302502)supported by Open Research Fund Program of the State Key Laboratory of Low-Dimensional Quantum Physics (Grant No. KF202204)supported by the New Cornerstone Science Foundation through the New Cornerstone Investigator Programthe XPLORER PRIZE。
文摘We have developed a low-damage photolithography method for magnetically doped(Bi,Sb)_(2)Te_(3)quantum anomalous Hall(QAH) thin films incorporating an additional resist layer of poly(methyl methacrylate)(PMMA). By performing control experiments on the transport properties of five devices at varied gate voltages(V_(g)s), we revealed that the modified photolithography method enables fabricating QAH devices with the transport and magnetic properties unaffected by fabrication process. Our experiment represents a step towards the production of novel micro-structured electronic devices based on the dissipationless QAH chiral edge states.
基金supported by the National Natural Science Foundation of China (Grant Nos. 11774190, 11674229, 11634009, and 11774427)the National Key R&D Program of China (Grant Nos. 2017YFA0304600 and 2017YFA0305400)+5 种基金support from the EPSRC (UK) grant EP/K04074X/1 and a DARPA (US) MESO project (No. N66001-11-1-4105)supported by the Office of Naval Research through the National Science Foundation under Award No. DMR-1707620 (magnetization measurement)supported by the Office of Basic Energy Sciences of the U.S. Department of Energy (DE-AC0205CH11231)SIMES and SLAC National Accelerator Laboratory is supported by the Office of Basic Energy Sciences of the U.S. Department of Energy (DE-AC0276SF00515)Nanjing University is supported by the National Basic Research Program of China (Grant No. 51002074)the National Basic Research of China (Grant Nos. 2012CB921503 and 2012CB632702)
文摘Angle-resolved photoemission spectroscopy(ARPES)and torque magnetometry(TM)measurements have been carried out to study the electronic structures of a correlated topological insulator(TI)candidate Yb B6.We observed clear surface states on the[001]surface centered at theГ^- and М^- points of the surface Brillouin zone.Interestingly,the fermiology revealed by the quantum oscillation of TM measurements agrees excellently with ARPES measurements.Moreover,the band structures we observed suggest that the band inversion in Yb B6 happens between the Yb5 dand B2bands,instead of the Yb5dand Yb4fbands as suggested by previous theoretical investigation,which will help settle the heavy debate regarding the topological nature of samarium/ytterbium hexaborides.
基金supported by the National Natural Science Foundation of China(Grant Nos.62074036,61674038,and 11574302)the Foreign Cooperation Project of Fujian Province,China(Grant No.2023I0005)+2 种基金the Open Research Fund Program of the State Key Laboratory of Low Dimensional Quantum Physics(Grant No.KF202108)the National Key Research and Development Program of China(Grant No.2016YFB0402303)the Foundation of the Fujian Provincial Department of Industry and Information Technology of China(Grant No.82318075).
文摘The thickness dependence of linearly polarized light-induced momentum anisotropy and the inverse spin Hall effect(PISHE)in topological insulator(TI)Bi_(2)Te_(3)films has been investigated.A significant enhancement of the PISHE signal is observed in the 12-quintuple-layer(QL)Bi_(2)Te_(3)film compared with that of the 3-and 5-QL samples,whereas a minimal value of photoinduced momentum anisotropy is found in the 12-QL sample.The photoinduced momentum anisotropy and the PISHE in Bi_(2)Te_(3)films are more than three and two orders of magnitude larger than those in Bi2Se3 films grown on SrTiO_(3)substrates,respectively.The 3-QL sample exhibits a sinusoidal dependence of the PISHE current on the light spot position,while the 5-QL and 12-QL samples show aW-shaped dependence,which arises from the different angles between the coordinate axis x and the in-plane crystallographic axis of the Bi_(2)Te_(3)films.Our findings demonstrate the critical role of film thickness in modulating both the photoinduced momentum anisotropy and the PISHE current,thereby suggesting a thickness-engineering strategy for designing novel optoelectronic devices based on TIs.
基金supported by the National Key Research and Development Program of China(Grant No.2023YFA1406400)。
文摘Recent experimental evidence of the charge-6e condensed phase in Kagome superconductors has generated significant interest.This study investigates the unconventional superconductivity in the Kagome superconductor CsV_(3)Sb_(5),focusing on the emergence of charge-6e superconductivity(SC)at temperatures higher than the conventional charge-2e SC state.By modeling the phase coherence of the SC order parameter using a frustrated antiferromagnetic XY model on an emergent Kagome lattice,the condensation of fractional vortices with 1/3 vorticity stabilizes the phase coherence in exp(i3θ),resulting in a charge-6e SC state.Using a tensor network approach tailored for frustrated spin systems,a Berezinskii-Kosterlitz-Thouless transition is identified at T_(c)/J≃0.075,where the unbinding of 1/3 fractional vortex-antivortex pairs transforms the system from the charge-6e SC phase to the normal phase.Below T_(c),the 1/3 fractional vortex correlations exhibit a power-law decay,whereas the integer vortex correlations decay exponentially,reflecting the dominance of charge-6e SC in the absence of charge-2e SC.The results provide a theoretical understanding of charge-6e SC in two-dimensional Kagome superconductors,emphasizing the interaction between fractional vortices,frustration,and topology in stabilizing the exotic SC phase.
基金Supported by the Ministry of Science and Technology of Chinathe National Science Foundation of Chinathe Beijing Advanced Innovation Center for Future Chip(ICFC)
文摘An intrinsic magnetic topological insulator(TI) is a stoichiometric magnetic compound possessing both inherent magnetic order and topological electronic states. Such a material can provide a shortcut to various novel topological quantum effects but remained elusive experimentally for a long time. Here we report the experimental realization of thin films of an intrinsic magnetic TI, MnBi2Te4, by alternate growth of a Bi2Te3 quintuple layer and a MnTe bilayer with molecular beam epitaxy. The material shows the archetypical Dirac surface states in angle-resolved photoemission spectroscopy and is demonstrated to be an antiferromagnetic topological insulator with ferromagnetic surfaces by magnetic and transport measurements as well as first-principles calculations. The unique magnetic and topological electronic structures and their interplays enable the material to embody rich quantum phases such as quantum anomalous Hall insulators and axion insulators at higher temperature and in a well-controlled way.
文摘The dimensionality of quantum materials strongly affects their physical properties.Although many emergent phenomena,such as charge-density wave and Luttinger liquid behavior,are well understood in one-dimensional(1D)systems,the generalization to explore them in higher dimensional systems is still a challenging task.In this study,we aim to bridge this gap by systematically investigating the crystal and electronic structures of molybdenum-oxide family compounds,where the contexture of 1D chains facilitates rich emergent properties.While the quasi-1D chains in these materials share general similarities,such as the motifs made up of MoO_(6)octahedrons,they exhibit vast complexity and remarkable tunability.We disassemble the 1D chains in molybdenum oxides with different dimensions and construct effective models to excellently fit their low-energy electronic structures obtained by ab initio calculations.Furthermore,we discuss the implications of such chains on other physical properties of the materials and the practical significance of the effective models.Our work establishes the molybdenum oxides as simple and tunable model systems for studying and manipulating the dimensionality in quantum systems.
基金supported by Beijing Outstanding Scholar Programthe National Key Research and Development Program of China(Grant No. 2016YFA0301600)+3 种基金the National Natural Science Foundation of China(Grant No. 11734010)supported by a startup fund from UCSDsupported by the Fundamental Research Funds for the Central Universitiesthe Research Funds of Renmin University of China
文摘We train a neural network to identify impurities in the experimental images obtained by the scanning tunneling microscope(STM)measurements.The neural network is first trained with a large number of simulated data and then the trained neural network is applied to identify a set of experimental images taken at different voltages.We use the convolutional neural network to extract features from the images and also implement the attention mechanism to capture the correlations between images taken at different voltages.We note that the simulated data can capture the universal Friedel oscillation but cannot properly describe the non-universal physics short-range physics nearby an impurity,as well as noises in the experimental data.And we emphasize that the key of this approach is to properly deal with these differences between simulated data and experimental data.Here we show that even by including uncorrelated white noises in the simulated data,the performance of the neural network on experimental data can be significantly improved.To prevent the neural network from learning unphysical short-range physics,we also develop another method to evaluate the confidence of the neural network prediction on experimental data and to add this confidence measure into the loss function.We show that adding such an extra loss function can also improve the performance on experimental data.Our research can inspire future similar applications of machine learning on experimental data analysis.
基金the strong support from Singapore Ministry of Education via AcRF Tier 3 Programme “Geometrical Quantum Materials” (MOE2018-T3-1-002)AcRF Tier 2 grants (MOE2017-T2-1040)+7 种基金the National Natural Science Foundation of China (Grant No. 61435010)the National Natural Science Foundation of China (Grant No. 61905156)the National Natural Science Foundation of China (Grant No. 61575010)the China Postdoctoral Science Foundation (Grant No. 2017M622764)the Natural Science Foundation of Fujian Province (Grant No. 2022J01555)the Beijing Municipal Natural Science Foundation (Grant No. 4162016)the financial support of the Presidential Postdoctoral Fellowship program of the Nanyang Technological Universitysupport from the Elemental Strategy Initiative conducted by the MEXT, Japan and the CREST (JPMJCR15F3), JST
文摘Monolayer group VI transition metal dichalcogenides(TMDs)have recently emerged as promising candidates for photonic and opto-valleytronic applications.The optoelectronic properties of these atomically-thin semiconducting crystals are strongly governed by the tightly bound electron-hole pairs such as excitons and trions(charged excitons).The anomalous spin and valley configurations at the conduction band edges in monolayer WS_(2)give rise to even more fascinating valley many-body complexes.Here we find that the indirect Q valley in the first Brillouin zone of monolayer WS_(2)plays a critical role in the formation of a new excitonic state,which has not been well studied.By employing a high-quality h-BN encapsulated WS_(2)field-effect transistor,we are able to switch the electron concentration within K-Q valleys at conduction band edges.Consequently,a distinct emission feature could be excited at the high electron doping region.Such feature has a competing population with the K valley trion,and experiences nonlinear power-law response and lifetime dynamics under doping.Our findings open up a new avenue for the study of valley many-body physics and quantum optics in semiconducting 2D materials,as well as provide a promising way of valley manipulation for next-generation entangled photonic devices.
基金Project supported by CAS-Shanghai Science Research Center,China(Grant No.CAS-SSRC-YH-2015-01)the National Key R&D Program of China(Grant No.2017YFA0305400)+4 种基金the National Natural Science Foundation of China(Grant Nos.11674229,11227902,and 11604207)the EPSRC Platform Grant(Grant No.EP/M020517/1)Hefei Science Center,Chinese Academy of Sciences(Grant No.2015HSC-UE013)Science and Technology Commission of Shanghai Municipality,China(Grant No.14520722100)the Strategic Priority Research Program(B)of the Chinese Academy of Sciences(Grant No.XDB04040200)。
文摘Iron-based superconductor family FeX(X=S,Se,Te)has been one of the research foci in physics and material science due to their record-breaking superconducting temperature(FeSe film)and rich physical phenomena.Recently,FeS,the least studied Fe X compound(due to the difficulty in synthesizing high quality macroscopic crystals)attracted much attention because of its puzzling superconducting pairing symmetry.In this work,combining scanning tunneling microscopy and angle resolved photoemission spectroscopy(ARPES)with sub-micron spatial resolution,we investigate the intrinsic electronic structures of superconducting FeS from individual single crystalline domains.Unlike FeTe or FeSe,FeS remains identical tetragonal structure from room temperature down to 5 K,and the band structures observed can be well reproduced by our ab-initio calculations.Remarkably,mixed with the 1×1 tetragonal metallic phase,we also observe the coexistence of √5×√5 reconstructed insulating phase in the crystal,which not only helps explain the unusual properties of FeS,but also demonstrates the importance of using spatially resolved experimental tools in the study of this compound.
基金supported by the National Natural Science Foundation of China(Grant No.92365206)the support of the China Postdoctoral Science Foundation(Certificate Number:2023M740272)+1 种基金supported by the National Natural Science Foundation of China(Grant No.12247168)China Postdoctoral Science Foundation(Certificate Number:2022TQ0036)。
文摘We introduce Quafu-Qcover,an open-source cloud-based software package developed for solving combinatorial optimization problems using quantum simulators and hardware backends.Quafu-Qcover provides a standardized and comprehensive workflow that utilizes the quantum approximate optimization algorithm(QAOA).It facilitates the automatic conversion of the original problem into a quadratic unconstrained binary optimization(QUBO)model and its corresponding Ising model,which can be subsequently transformed into a weight graph.The core of Qcover relies on a graph decomposition-based classical algorithm,which efficiently derives the optimal parameters for the shallow QAOA circuit.Quafu-Qcover incorporates a dedicated compiler capable of translating QAOA circuits into physical quantum circuits that can be executed on Quafu cloud quantum computers.Compared to a general-purpose compiler,our compiler demonstrates the ability to generate shorter circuit depths,while also exhibiting superior speed performance.Additionally,the Qcover compiler has the capability to dynamically create a library of qubits coupling substructures in real-time,utilizing the most recent calibration data from the superconducting quantum devices.This ensures that computational tasks can be assigned to connected physical qubits with the highest fidelity.The Quafu-Qcover allows us to retrieve quantum computing sampling results using a task ID at any time,enabling asynchronous processing.Moreover,it incorporates modules for results preprocessing and visualization,facilitating an intuitive display of solutions for combinatorial optimization problems.We hope that Quafu-Qcover can serve as an instructive illustration for how to explore application problems on the Quafu cloud quantum computers.
基金supported by the Beijing Academy of Quantum Information Sciencessupported by the National Natural Science Foundation of China(Grant No.92365206)+2 种基金the support of the China Postdoctoral Science Foundation(Certificate Number:2023M740272)supported by the National Natural Science Foundation of China(Grant No.12247168)China Postdoctoral Science Foundation(Certificate Number:2022TQ0036)。
文摘With the rapid advancement of quantum computing,hybrid quantum–classical machine learning has shown numerous potential applications at the current stage,with expectations of being achievable in the noisy intermediate-scale quantum(NISQ)era.Quantum reinforcement learning,as an indispensable study,has recently demonstrated its ability to solve standard benchmark environments with formally provable theoretical advantages over classical counterparts.However,despite the progress of quantum processors and the emergence of quantum computing clouds,implementing quantum reinforcement learning algorithms utilizing parameterized quantum circuits(PQCs)on NISQ devices remains infrequent.In this work,we take the first step towards executing benchmark quantum reinforcement problems on real devices equipped with at most 136 qubits on the BAQIS Quafu quantum computing cloud.The experimental results demonstrate that the policy agents can successfully accomplish objectives under modified conditions in both the training and inference phases.Moreover,we design hardware-efficient PQC architectures in the quantum model using a multi-objective evolutionary algorithm and develop a learning algorithm that is adaptable to quantum devices.We hope that the Quafu-RL can be a guiding example to show how to realize machine learning tasks by taking advantage of quantum computers on the quantum cloud platform.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11574370,11274358,and 11190020)the National Basic Research Program of China(Grant No.2013CB921700)the Strategic Priority Research Program(B)of the Chinese Academy of Sciences(Grant No.XDB07020100)
文摘Large superconducting Fe Se crystals of（001） orientation have been prepared via a hydrothermal ion release/introduction route for the first time. The hydrothermally derived Fe Se crystals are up to 10 mm×5 mm×0.3 mm in dimension. The pure tetragonal FeSe phase has been confirmed by x-ray diffraction（XRD） and the composition determined by both inductively coupled plasma atomic emission spectroscopy（ICP-AES） and energy dispersive x-ray spectroscopy（EDX）. The superconducting transition of the Fe Se samples has been characterized by magnetic and transport measurements. The zero-temperature upper critical field H（c2） is calculated to be 13.2–16.7 T from a two-band model. The normal-state cooperative paramagnetism is found to be predominated by strong spin frustrations below the characteristic temperature T（sn）, where the Ising spin nematicity has been discerned in the FeSe superconductor crystals as reported elsewhere.
基金Project supported by the National Basic Research Program of China(Grant Nos.2016YFA0301004 and 2015CB921001)the National Natural Science Foundation of China(Grant Nos.11334006,11725418,and 11674188)
文摘Atomically thin transition metal dichalcogenide films with distorted trigonal(1T') phase have been predicted to be candidates for realizing quantum spin Hall effect. Growth of 1T' film and experimental investigation of its electronic structure are critical. Here we report the electronic structure of 1T'-MoTe2 films grown by molecular beam epitaxy(MBE).Growth of the 1T'-MoTe2 film depends critically on the substrate temperature, and successful growth of the film is indicated by streaky stripes in the reflection high energy electron diffraction(RHEED) and sharp diffraction spots in the low energy electron diffraction(LEED). Angle-resolved photoemission spectroscopy(ARPES) measurements reveal a metallic behavior in the as-grown film with an overlap between the conduction and valence bands. First principles calculation suggests that a suitable tensile strain along the a-axis direction is needed to induce a gap to make it an insulator. Our work not only reports the electronic structure of MBE grown 1T'-MoTe2 films, but also provides insights for strain engineering to make it possible for quantum spin Hall effect.
基金supported by the National Basic Research Program of China(Grant Nos.2009CB929400 and 2010CB923003)
文摘Our recent scanning tunneling microscopy （STM） studies of the NaFelxCoxAs phase diagram over a wide range of dopings and temperatures are reviewed. Similar to the high-Tc cuprates, the iron-based superconductors lie in close proximity to a magnetically ordered phase. Therefore, it is widely believed that magnetic interactions or fluctuations play an important role in triggering their Cooper pairings. Among the key issues regarding the electronic phase diagram are the properties of the parent spin density wave （SDW） phase and the superconducting （SC） phase, as well as the interplay between them. The NaFe l-xCoxAs is an ideal system for resolving these issues due to its rich electronic phases and the charge-neutral cleaved surface. In our recent work, we directly observed the SDW gap in the parent state, and it exhibits unconventional features that are incompatible with the simple Fermi surface nesting picture. The optimally doped sample has a single SC gap, but in the underdoped regime we directly viewed the microscopic coexistence of the SDW and SC orders, which compete with each other. In the overdoped regime we observed a novel pseudogap-like feature that coexists with supercon- ductivity in the ground state, persists well into the normal state, and shows great spatial variations. The rich electronic structures across the phase diagram of NaFel_xCoxAs revealed here shed important new light for defining microscopic models of the iron-based superconductors. In particular, we argue that both the itinerant electrons and local moments should be considered on an equal footing in a realistic model.
