In this paper, we study the homotopy category of unbounded complexes of strongly copure projective modules with bounded relative homologies K;(SCP).We show that the existence of a right recollement of K;(SCP) with...In this paper, we study the homotopy category of unbounded complexes of strongly copure projective modules with bounded relative homologies K;(SCP).We show that the existence of a right recollement of K;(SCP) with respect to K;(SCP), K;(SCP) and K;(SCP) has the homotopy category of strongly copure projective acyclic complexes as a triangulated subcategory in some case.展开更多
The properties of electrolytes are critical for fast-charging and stable-cycling applications in lithium metal batteries(LMBs).However,the slow kinetics of Li^(+)transport and desolvation in commercial carbonate elect...The properties of electrolytes are critical for fast-charging and stable-cycling applications in lithium metal batteries(LMBs).However,the slow kinetics of Li^(+)transport and desolvation in commercial carbonate electrolytes,cou pled with the formation of unstable solid electrolyte interphases(SEI),exacerbate the degradation of LMB performance at high current densities.Herein,we propose a versatile electrolyte design strategy that incorporates cyclohexyl methyl ether(CME)as a co-solvent to reshape the Li^(+)solvation environment by the steric-hindrance effect of bulky molecules and their competitive coordination with other solvent molecules.Simulation calculations and spectral analysis demonstrate that the addition of CME molecules reduces the involvement of other solvent molecules in the Li solvation sheath and promotes the formation of Li^(+)-PF_(6)^(-)coordination,thereby accelerating Li^(+)transport kinetics.Additionally,this electrolyte composition improves Li^(+)desolvation kinetics and fosters the formation of inorganic-rich SEI,ensuring cycle stability under fast charging.Consequently,the Li‖LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)battery with the modified electrolyte retains 82% of its initial capacity after 463 cycles at 1 C.Even under the extreme fast-charging condition of 5 C,the battery can maintain 80% capacity retention after 173 cycles.This work provides a promising approach for the development of highperformance LMBs by modulating solvation environment of electrolytes.展开更多
Despite the promising progress in conductive hydrogels made with pure conducting polymer,great challenges remain in the interface adhesion and robustness in longterm monitoring.To address these challenges,Prof.Seung H...Despite the promising progress in conductive hydrogels made with pure conducting polymer,great challenges remain in the interface adhesion and robustness in longterm monitoring.To address these challenges,Prof.Seung Hwan Ko and Taek-Soo Kim’s team introduced a laserinduced phase separation and adhesion method for fabricating conductive hydrogels consisting of pure poly(3,4-ethylenedioxythiophene):polystyrene sulfonate on polymer substrates.The laser-induced phase separation and adhesion treated conducting polymers can be selectively transformed into conductive hydrogels that exhibit wet conductivities of 101.4 S cm^(−1) with a spatial resolution down to 5μm.Moreover,they maintain impedance and charge-storage capacity even after 1 h of sonication.The micropatterned electrode arrays demonstrate their potential in long-term in vivo signal recordings,highlighting their promising role in the field of bioelectronics.展开更多
Biomarker and stable carbon isotope analyses are presented for the Garau Formation of the Cretaceous Age,an important source rock in western Iran,to reveal its potential as an oilprone source rock.The C_(28)/C_(29)ste...Biomarker and stable carbon isotope analyses are presented for the Garau Formation of the Cretaceous Age,an important source rock in western Iran,to reveal its potential as an oilprone source rock.The C_(28)/C_(29)sterane ratio value range(0.72 to 0.83)of bitumen samples from the formation suggests that they were likely formed during phytoplankton blooms.Sterane,hopane,and isoprenoid/n-alkane ratios indicate that the formation's organic matter predominantly consists of algae,and bacteria,accompanied by some reworked material derived from higher plants.Due to the predominance of anoxic conditions and the actions of sulfate-reducing bacteria,the bitumen present is enriched with sulfur compounds.The percentages of saturates,aromatics,and nitrogen-sulfuroxygen(NSO)fractions in the bitumen samples classify them as naphthenic oils.Isotope analysis reveals that biodegradation and water-washing have reduced the concentrations of some volatile saturates and low molecular weight aromatics in the bitumen samples.These actions have resulted in distinctiveδ^(13)C values for the formation's kerogen and bitumen fractions.The formation's organic matter has been subjected to high-temperature thermal regimes and has entered the oil-generation window at the sampled localities,with vitrinite reflectance(%R_(C))varying between 0.7%and 0.75%.展开更多
In this paper,we study the Bowen entropy of stable sets in positive entropy G-system of amenable group actions.The lower bound of the Bowen entropy of these sets are estimated.
针对现有无数据模型窃取攻击技术在有限的查询预算下难以拟合原始训练集分布,进而影响对目标模型决策边界拟合效果问题,提出了一种基于Stable Diffusion的模型窃取攻击方法(Model Extraction Attack Based on Stable Diffusion,MEASD)....针对现有无数据模型窃取攻击技术在有限的查询预算下难以拟合原始训练集分布,进而影响对目标模型决策边界拟合效果问题,提出了一种基于Stable Diffusion的模型窃取攻击方法(Model Extraction Attack Based on Stable Diffusion,MEASD).利用预训练的Stable Diffusion生成训练数据可能涵盖多个域,并包含大量非判别性样本,设计了ILAF方法以优化Stable Diffusion生成的数据品质.将高质量合成数据的原始样本与由对抗样本生成器生成的对抗样本组成替代训练集.由DPA模块组合的替代模型基于替代训练集拟合目标模型的决策边界.实验结果表明,在四个主流的基准数据集上与EBFA和DMEAE方法相比,所提的MEASD方法能够将目标模型决策边界的拟合程度提高至84%,对目标模型的黑盒对抗攻击成功率超过68%,并且查询预算较低.MEASD方法能够有效地提升目标模型决策边界拟合效果及攻击成功率.展开更多
University courses should have both breadth and depth.However,most courses in universities only focus on the breadth construction,while neglecting the depth construction,resulting in students being unable to apply the...University courses should have both breadth and depth.However,most courses in universities only focus on the breadth construction,while neglecting the depth construction,resulting in students being unable to apply the knowledge they have learned to conduct research or solve real-world application problems.The students’high-level abilities are insufficient and not well-trained.Therefore,in this paper,we propose a T-structured course design method to ensure both breadth and depth of a course.The proposed T-structured course design method includes four aspects:T-structured course contents,T-structured teaching activities,T-structured examination formats,and T-structured homework difficulty.By applying our proposed T-structured course design strategy to the course Optimization Algorithms and Intelligent Computing,good results are achieved,demonstrating the applicability of our proposed strategy.展开更多
文摘In this paper, we study the homotopy category of unbounded complexes of strongly copure projective modules with bounded relative homologies K;(SCP).We show that the existence of a right recollement of K;(SCP) with respect to K;(SCP), K;(SCP) and K;(SCP) has the homotopy category of strongly copure projective acyclic complexes as a triangulated subcategory in some case.
基金supported by the Lithium Resources and Lithium Materials Key Laboratory of Sichuan Province(LRMKF202405)the National Natural Science Foundation of China(52402226)+3 种基金the Natural Science Foundation of Sichuan Province(2024NSFSC1016)the Scientific Research Startup Foundation of Chengdu University of Technology(10912-KYQD2023-10240)the opening funding from Key Laboratory of Engineering Dielectrics and Its Application(Harbin University of Science and Technology)(KFM202507,Ministry of Education)the funding provided by the Alexander von Humboldt Foundation。
文摘The properties of electrolytes are critical for fast-charging and stable-cycling applications in lithium metal batteries(LMBs).However,the slow kinetics of Li^(+)transport and desolvation in commercial carbonate electrolytes,cou pled with the formation of unstable solid electrolyte interphases(SEI),exacerbate the degradation of LMB performance at high current densities.Herein,we propose a versatile electrolyte design strategy that incorporates cyclohexyl methyl ether(CME)as a co-solvent to reshape the Li^(+)solvation environment by the steric-hindrance effect of bulky molecules and their competitive coordination with other solvent molecules.Simulation calculations and spectral analysis demonstrate that the addition of CME molecules reduces the involvement of other solvent molecules in the Li solvation sheath and promotes the formation of Li^(+)-PF_(6)^(-)coordination,thereby accelerating Li^(+)transport kinetics.Additionally,this electrolyte composition improves Li^(+)desolvation kinetics and fosters the formation of inorganic-rich SEI,ensuring cycle stability under fast charging.Consequently,the Li‖LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)battery with the modified electrolyte retains 82% of its initial capacity after 463 cycles at 1 C.Even under the extreme fast-charging condition of 5 C,the battery can maintain 80% capacity retention after 173 cycles.This work provides a promising approach for the development of highperformance LMBs by modulating solvation environment of electrolytes.
基金supported by the National Natural Science Foundation of China(52475610)Zhejiang Provincial Natural Science Foundation of China(LDQ24E050001).
文摘Despite the promising progress in conductive hydrogels made with pure conducting polymer,great challenges remain in the interface adhesion and robustness in longterm monitoring.To address these challenges,Prof.Seung Hwan Ko and Taek-Soo Kim’s team introduced a laserinduced phase separation and adhesion method for fabricating conductive hydrogels consisting of pure poly(3,4-ethylenedioxythiophene):polystyrene sulfonate on polymer substrates.The laser-induced phase separation and adhesion treated conducting polymers can be selectively transformed into conductive hydrogels that exhibit wet conductivities of 101.4 S cm^(−1) with a spatial resolution down to 5μm.Moreover,they maintain impedance and charge-storage capacity even after 1 h of sonication.The micropatterned electrode arrays demonstrate their potential in long-term in vivo signal recordings,highlighting their promising role in the field of bioelectronics.
文摘Biomarker and stable carbon isotope analyses are presented for the Garau Formation of the Cretaceous Age,an important source rock in western Iran,to reveal its potential as an oilprone source rock.The C_(28)/C_(29)sterane ratio value range(0.72 to 0.83)of bitumen samples from the formation suggests that they were likely formed during phytoplankton blooms.Sterane,hopane,and isoprenoid/n-alkane ratios indicate that the formation's organic matter predominantly consists of algae,and bacteria,accompanied by some reworked material derived from higher plants.Due to the predominance of anoxic conditions and the actions of sulfate-reducing bacteria,the bitumen present is enriched with sulfur compounds.The percentages of saturates,aromatics,and nitrogen-sulfuroxygen(NSO)fractions in the bitumen samples classify them as naphthenic oils.Isotope analysis reveals that biodegradation and water-washing have reduced the concentrations of some volatile saturates and low molecular weight aromatics in the bitumen samples.These actions have resulted in distinctiveδ^(13)C values for the formation's kerogen and bitumen fractions.The formation's organic matter has been subjected to high-temperature thermal regimes and has entered the oil-generation window at the sampled localities,with vitrinite reflectance(%R_(C))varying between 0.7%and 0.75%.
基金Supported by NSFC(No.11861010),also supported by NSFC(No.12171175),also supported by NSFC(No.12261006)NSF of Guangxi Province(No.2018GXNSFFA281008)Project of Guangxi First Class Disciplines of Statistics(No.GJKY-2022-01)。
文摘In this paper,we study the Bowen entropy of stable sets in positive entropy G-system of amenable group actions.The lower bound of the Bowen entropy of these sets are estimated.
文摘针对现有无数据模型窃取攻击技术在有限的查询预算下难以拟合原始训练集分布,进而影响对目标模型决策边界拟合效果问题,提出了一种基于Stable Diffusion的模型窃取攻击方法(Model Extraction Attack Based on Stable Diffusion,MEASD).利用预训练的Stable Diffusion生成训练数据可能涵盖多个域,并包含大量非判别性样本,设计了ILAF方法以优化Stable Diffusion生成的数据品质.将高质量合成数据的原始样本与由对抗样本生成器生成的对抗样本组成替代训练集.由DPA模块组合的替代模型基于替代训练集拟合目标模型的决策边界.实验结果表明,在四个主流的基准数据集上与EBFA和DMEAE方法相比,所提的MEASD方法能够将目标模型决策边界的拟合程度提高至84%,对目标模型的黑盒对抗攻击成功率超过68%,并且查询预算较低.MEASD方法能够有效地提升目标模型决策边界拟合效果及攻击成功率.
基金supported in part by the fund of 2023 Guangdong Province Science and Technology Innovation Strategy Special Project“Construction of Industrial Data and Intelligent Application Innovation Platform”(2023A011),2024 Shanwei New Generation Electronic Information Industry Talent Revitalization Plan,and the project“Research on the Impact and Countermeasures of Large Scale Charging Facility Access on Guangdong Power Grid Planning and Construction.”。
文摘University courses should have both breadth and depth.However,most courses in universities only focus on the breadth construction,while neglecting the depth construction,resulting in students being unable to apply the knowledge they have learned to conduct research or solve real-world application problems.The students’high-level abilities are insufficient and not well-trained.Therefore,in this paper,we propose a T-structured course design method to ensure both breadth and depth of a course.The proposed T-structured course design method includes four aspects:T-structured course contents,T-structured teaching activities,T-structured examination formats,and T-structured homework difficulty.By applying our proposed T-structured course design strategy to the course Optimization Algorithms and Intelligent Computing,good results are achieved,demonstrating the applicability of our proposed strategy.