In the paper we use detrended cross-correlation analysis （DCCA） to study the electroencephalograms of healthy young subjects and healthy old subjects. It is found that the cross-correlation between different leads o...In the paper we use detrended cross-correlation analysis （DCCA） to study the electroencephalograms of healthy young subjects and healthy old subjects. It is found that the cross-correlation between different leads of a healthy young subject is larger than that of a healthy old subject. It was shown that the cross-correlation relationship decreases with the aging process and the phenomenon can help to diagnose whether the subject＇s brain function is healthy or not.展开更多
Multifractal detrended fluctuation analysis （MF-DFA） is a relatively new method of multifractal analysis. It is extended from detrended fluctuation analysis （DFA）, which was developed for detecting the long-range ...Multifractal detrended fluctuation analysis （MF-DFA） is a relatively new method of multifractal analysis. It is extended from detrended fluctuation analysis （DFA）, which was developed for detecting the long-range correlation and the fractal properties in stationary and non-stationary time series. Although MF-DFA has become a widely used method, some relationships among the exponents established in the original paper seem to be incorrect under the general situation. In this paper, we theoretically and experimentally demonstrate the invalidity of the expression r（q） = qh（q） - 1 stipulating the relationship between the multifractal exponent T（q） and the generalized Hurst exponent h（q）. As a replacement, a general relationship is established on the basis of the universal multifractal formalism for the stationary series as .t-（q） = qh（q） - qH - 1, where H is the nonconservation parameter in the universal multifractal formalism. The singular spectra, a and f（a）, are also derived according to this new relationship.展开更多
We present a multifractal detrended fluctuation analysis （MFDFA） of the time series of return generated by our recently-proposed Ising financial market model with underlying small world topology. The result of the M...We present a multifractal detrended fluctuation analysis （MFDFA） of the time series of return generated by our recently-proposed Ising financial market model with underlying small world topology. The result of the MFDFA shows that there exists obvious multifractal scaling behavior in produced time series. We compare the MFDFA results for original time series with those for shuffled series, and find that its multifractal nature is due to two factors： broadness of probability density function of the series and different correlations in small- and large-scale fluctuations. This may provide new insight to the problem of the origin of multifractality in financial time series.展开更多
We use multifractal detrended fluctuation analysis （MF-DFA） method to investigate the multifractal behavior of the interevent time series in a modified Olami-Feder-Christensen （OFC） earthquake model on assortative...We use multifractal detrended fluctuation analysis （MF-DFA） method to investigate the multifractal behavior of the interevent time series in a modified Olami-Feder-Christensen （OFC） earthquake model on assortative scale-free networks. We determine generalized Hurst exponent and singularity spectrum and find that these fluctuations have multifraetal nature. Comparing the MF-DFA results for the original interevent time series with those for shuffled and surrogate series, we conclude that the origin of multifractality is due to both the broadness of probability density function and long-range correlation.展开更多
Temporal-spatial cross-correlation analysis of non-stationary wind speed time series plays a crucial role in wind field reconstruction as well as in wind pattern recognition.Firstly,the near-surface wind speed time se...Temporal-spatial cross-correlation analysis of non-stationary wind speed time series plays a crucial role in wind field reconstruction as well as in wind pattern recognition.Firstly,the near-surface wind speed time series recorded at different locations are studied using the detrended fluctuation analysis(DFA),and the corresponding scaling exponents are larger than 1.This indicates that all these wind speed time series have non-stationary characteristics.Secondly,concerning this special feature( i.e.,non-stationarity)of wind signals,a cross-correlation analysis method,namely detrended cross-correlation analysis(DCCA) coefficient,is employed to evaluate the temporal-spatial cross-correlations between non-stationary time series of different anemometer pairs.Finally,experiments on ten wind speed data synchronously collected by the ten anemometers with equidistant arrangement illustrate that the method of DCCA cross-correlation coefficient can accurately analyze full-scale temporal-spatial cross-correlation between non-stationary time series and also can easily identify the seasonal component,while three traditional cross-correlation techniques(i.e.,Pearson coefficient,cross-correlation function,and DCCA method) cannot give us these information directly.展开更多
Taking the return series of the EU carbon allowance price, WTI crude oil price, the European renewable energy index and Shenzhen carbon emission price, Daqing crude oil price, the China securities new energy index as ...Taking the return series of the EU carbon allowance price, WTI crude oil price, the European renewable energy index and Shenzhen carbon emission price, Daqing crude oil price, the China securities new energy index as sample data, the multifractal detrend cross-correlation analysis method(MF-DCCA)is used to research the dynamic cross-correlation relationships among the carbon emission market, crude oil market and the new energy market in Europe and China and the source of the multifractality. The empirical analysis shows that the cross-correlations among the carbon emission market, crude oil market and new energy market in Europe and China have all significant multifractal characteristics. Moreover, the multifractal strength of cross-correlation between the carbon emission market and crude oil market is less than that between the carbon emission market and new energy market in Europe. The Chinese market is the opposite. In addition, the multifractal strength of cross-correlation between the crude oil market and new energy market in Europe is more than that between the crude oil market and new energy market in China. It is also found that the long-range correlation of the sequences themselves and the fat-tailed distribution in fluctuations are the common causes of the multifractality, and the fat-tailed in fluctuations distribution contributes more to the multifractals of the series.展开更多
When exploring the temporal and spatial change law of ocean environment, the most common method used is using smaller-scale observed data to derive the change law for a larger-scale system. For instance, using 30-year...When exploring the temporal and spatial change law of ocean environment, the most common method used is using smaller-scale observed data to derive the change law for a larger-scale system. For instance, using 30-year observation data to derive 100-year return period design wave height. Therefore, the study of inherent self-similarity in ocean hydrological elements becomes increasingly important to the study of multi-year return period design wave height derivation. In this paper, we introduced multifractal to analyze the statistical characteristics of wave height series data observed from oceanic hydrological station. An improvement is made to address the existing problems of the multifractal detrended fluctuation analysis (MF-DFA) method, where trend function showed a discontinuity between intervals. The improved MFDFA method is based on signal mode decomposition, replacing piecewise polynomial fitting used in the original method. We applied the proposed method to the wave height data collected at Chaolian Island, Shandong, China, from 1963 to 1989 and was able to conclude the wave height sequence presented weak multi-fractality. This result provided strong support to the past research on the derivation of multi-year return period design wave height with observed data. Moreover, the new method proposed in this paper also provides a new perspective to explore the intrinsic characteristic of data.展开更多
Massive seamounts have been surveyed and documented in the last decades.However,the morphologies of seamounts are usually described in qualitative manners,yet few quantitative detections have been carried out.Here,bas...Massive seamounts have been surveyed and documented in the last decades.However,the morphologies of seamounts are usually described in qualitative manners,yet few quantitative detections have been carried out.Here,based on the high-re solution multi-beam bathymetric data,we report a recentlysurveyed guy ot on the Caroline Ridge in the West Pacific,and the large-scale volcanic structures and smallscale erosive-depositional landforms in the guyot area have been identified.The multifractal features of the guyot are characterized for the first time by applying multifractal detrended fluctuation analysis on the surveyed bathymetric data.The results indicate that the multifractal spectrum parameters of the seafloor have strong spatial dependency on the fluctuations of local landforms.Both small-and large-scale components contribute to the degree of asymmetry of the multifractal spectrum(B),while the fluctuations of B are mostly attributed to the changes in small-scale roughness.The maximum singularity strength(α0)correlates well with the roughness of large-scale landforms and likely reflects the large-scale topographic irregularity.Comparing to traditional roughness parameters or monofractal exponents,multifractal spectra are able to depict not only the multiscale characteristics of submarine landforms,but also the spatial variations of scaling behaviors.Although more comparative works are required for various seamounts,we hope this study,as a case of quantifying geomorphological characters and multiscale behaviors of seamounts,can encourage further studies on seamounts concerning geomorphological processes,ocean bottom circulations,and seamount ecosystems.展开更多
The shrinkage of the Aral Sea,which is closely related to the Amu Darya River,strongly affects the sustainability of the local natural ecosystem,agricultural production,and human well-being.In this study,we used the B...The shrinkage of the Aral Sea,which is closely related to the Amu Darya River,strongly affects the sustainability of the local natural ecosystem,agricultural production,and human well-being.In this study,we used the Bayesian Estimator of Abrupt change,Seasonal change,and Trend(BEAST)model to detect the historical change points in the variation of the Aral Sea and the Amu Darya River and analyse the causes of the Aral Sea shrinkage during the 1950–2016 period.Further,we applied multifractal detrend cross-correlation analysis(MF-DCCA)and quantitative analysis to investigate the responses of the Aral Sea to the runoff in the Amu Darya River,which is the main source of recharge to the Aral Sea.Our results showed that two significant trend change points in the water volume change of the Aral Sea occurred,in 1961 and 1974.Before 1961,the water volume in the Aral Sea was stable,after which it began to shrink,with a shrinkage rate fluctuating around 15.21 km3/a.After 1974,the water volume of the Aral Sea decreased substantially at a rate of up to 48.97 km3/a,which was the highest value recorded in this study.In addition,although the response of the Aral Sea's water volume to its recharge runoff demonstrated a complex non-linear relationship,the replenishment of the Aral Sea by the runoff in the lower reaches of the Amu Darya River was identified as the dominant factor affecting the Aral Sea shrinkage.Based on the scenario analyses,we concluded that it is possible to slow down the retreat of the Aral Sea and restore its ecosystem by increasing the efficiency of agricultural water use,decreasing agricultural water use in the middle and lower reaches,reducing ineffective evaporation from reservoirs and wetlands,and increasing the water coming from the lower reaches of the Amu Darya River to the 1961–1973 level.These measures would maintain and stabilise the water area and water volume of the Aral Sea in a state of ecological restoration.Therefore,this study focuses on how human consumption of recharge runoff affects the Aral Sea and provides scientific perspective on its ecological conservation and sustainable development.展开更多
This paper presents fault detection,classification,and location for a PV-Wind-based DC ring microgrid in the MATLAB/SIMULINK platform.Initially,DC fault signals are collected from local measurements to examine the out...This paper presents fault detection,classification,and location for a PV-Wind-based DC ring microgrid in the MATLAB/SIMULINK platform.Initially,DC fault signals are collected from local measurements to examine the outcomes of the proposed system.Accurate detection is carried out for all faults,(i.e.,cable and arc faults)under two cases of fault resistance and distance variation,with the assistance of primary and secondary detection techniques,i.e.second-order differential current derivatived2I3 dt2and sliding mode window-based Pearson’s correlation coefficient.For fault classification a novel approach using modified multifractal detrended fluctuation analysis(M-MFDFA)is presented.The advantage of this method is its ability to estimate the local trends of any order polynomial function with the help of polynomial and trigonometric functions.It also doesn’t require any signal processing algorithm for decomposition resulting and this results in a reduction of computational burden.The detected fault signals are directly passed through the M-MFDFA classifier for fault type classification.To enhance the performance of the proposed classifier,statistical data is obtained from the M-MFDFA feature vectors,and the obtained data is plotted in 2-D and 3-D scatter plots for better visualization.Accurate fault distance estimation is carried out for all types of faults in the DC ring bus microgrid with the assistance of recursive least squares with a forgetting factor(FF-RLS).To verify the performance and superiority of the proposed classifier,it is compared with existing classifiers in terms of features,classification accuracy(CA),and relative computational time(RCT).展开更多
As an important component of secondary aerosols,sulfate plays a crucial role in regulating atmospheric radiative balance and influencing the secondary formation of ozone(O_(3)).In real atmosphere,atmospheric oxidants ...As an important component of secondary aerosols,sulfate plays a crucial role in regulating atmospheric radiative balance and influencing the secondary formation of ozone(O_(3)).In real atmosphere,atmospheric oxidants NO_(2)and O_(3)can promote the oxidation of SO_(2)to form sulfate(SO_(4)^(2−))through multiphase chemistry that occur at different time scales.Due to the combined impact of meteorology,pollution sources,atmospheric chemistry,etc.,time-scale dependence of SO_(2)-SO_(4)^(2−)conversion makes the impact of NO_(2)/O_(3)on it more complex.In this study,based on long-term time series(2013-2020)of air pollution variables from seven stations in Hong Kong,the Multifractal Detrended Cross-Correlation Analysis(MFDCCA)method has been employed to quantify the cross-correlations between SO_(2)and SO_(4)^(2−)in real atmosphere at different time scales,for examining the time-scale dependence of SO_(2)-SO_(4)^(2−)conversion efficiency.Furthermore,the Pearson correlation analysis has been used to study the influence of NO_(2)/O_(3)on SO_(2)-SO_(4)^(2−)conversion,and the regional and seasonal differences have been analyzed by considering factors such as meteorology,pollution sources,and regional transport.Changes in the main components of secondary aerosols are closely linked with the co-control of regional PM_(2.5)and O_(3).Therefore,the exploration of the impact of co-existing NO_(2)/O_(3)gases on the secondary formation of sulfates in real atmosphere is significant.展开更多
基金supported by the Science Foundation of Jiangsu Province of China (Grant No.BK2011759)
文摘In the paper we use detrended cross-correlation analysis （DCCA） to study the electroencephalograms of healthy young subjects and healthy old subjects. It is found that the cross-correlation between different leads of a healthy young subject is larger than that of a healthy old subject. It was shown that the cross-correlation relationship decreases with the aging process and the phenomenon can help to diagnose whether the subject＇s brain function is healthy or not.
基金Project supported by the National Natural Science Foundation of China (Grant No.11071282)the Chinese Program for New Century Excellent Talents in University (Grant No.NCET-08-06867)
文摘Multifractal detrended fluctuation analysis （MF-DFA） is a relatively new method of multifractal analysis. It is extended from detrended fluctuation analysis （DFA）, which was developed for detecting the long-range correlation and the fractal properties in stationary and non-stationary time series. Although MF-DFA has become a widely used method, some relationships among the exponents established in the original paper seem to be incorrect under the general situation. In this paper, we theoretically and experimentally demonstrate the invalidity of the expression r（q） = qh（q） - 1 stipulating the relationship between the multifractal exponent T（q） and the generalized Hurst exponent h（q）. As a replacement, a general relationship is established on the basis of the universal multifractal formalism for the stationary series as .t-（q） = qh（q） - qH - 1, where H is the nonconservation parameter in the universal multifractal formalism. The singular spectra, a and f（a）, are also derived according to this new relationship.
基金Supported by the Scientific Research Foundation for the Returned Overseas Chinese Scholars of State Education Ministry
文摘We present a multifractal detrended fluctuation analysis （MFDFA） of the time series of return generated by our recently-proposed Ising financial market model with underlying small world topology. The result of the MFDFA shows that there exists obvious multifractal scaling behavior in produced time series. We compare the MFDFA results for original time series with those for shuffled series, and find that its multifractal nature is due to two factors： broadness of probability density function of the series and different correlations in small- and large-scale fluctuations. This may provide new insight to the problem of the origin of multifractality in financial time series.
基金Supported by Foundation for Outstanding Young and Middle-aged Scientists in Shandong Province under Grant No.BS2011HZ019State Key Laboratory of Data Analysis and Applications,State Oceanic Administration under Grant No.LDAA-2011-02the Fundamental Research Funds for the Central Universities under Grant No.201113006
文摘We use multifractal detrended fluctuation analysis （MF-DFA） method to investigate the multifractal behavior of the interevent time series in a modified Olami-Feder-Christensen （OFC） earthquake model on assortative scale-free networks. We determine generalized Hurst exponent and singularity spectrum and find that these fluctuations have multifraetal nature. Comparing the MF-DFA results for the original interevent time series with those for shuffled and surrogate series, we conclude that the origin of multifractality is due to both the broadness of probability density function and long-range correlation.
基金Projects(61271321,61573253,61401303)supported by the National Natural Science Foundation of ChinaProject(14ZCZDSF00025)supported by Tianjin Key Technology Research and Development Program,China+1 种基金Project(13JCYBJC17500)supported by Tianjin Natural Science Foundation,ChinaProject(20120032110068)supported by Doctoral Fund of Ministry of Education of China
文摘Temporal-spatial cross-correlation analysis of non-stationary wind speed time series plays a crucial role in wind field reconstruction as well as in wind pattern recognition.Firstly,the near-surface wind speed time series recorded at different locations are studied using the detrended fluctuation analysis(DFA),and the corresponding scaling exponents are larger than 1.This indicates that all these wind speed time series have non-stationary characteristics.Secondly,concerning this special feature( i.e.,non-stationarity)of wind signals,a cross-correlation analysis method,namely detrended cross-correlation analysis(DCCA) coefficient,is employed to evaluate the temporal-spatial cross-correlations between non-stationary time series of different anemometer pairs.Finally,experiments on ten wind speed data synchronously collected by the ten anemometers with equidistant arrangement illustrate that the method of DCCA cross-correlation coefficient can accurately analyze full-scale temporal-spatial cross-correlation between non-stationary time series and also can easily identify the seasonal component,while three traditional cross-correlation techniques(i.e.,Pearson coefficient,cross-correlation function,and DCCA method) cannot give us these information directly.
基金supported by the Jiangsu postgraduate research and practice innovation program (Grant No. KYCX18_1386)
文摘Taking the return series of the EU carbon allowance price, WTI crude oil price, the European renewable energy index and Shenzhen carbon emission price, Daqing crude oil price, the China securities new energy index as sample data, the multifractal detrend cross-correlation analysis method(MF-DCCA)is used to research the dynamic cross-correlation relationships among the carbon emission market, crude oil market and the new energy market in Europe and China and the source of the multifractality. The empirical analysis shows that the cross-correlations among the carbon emission market, crude oil market and new energy market in Europe and China have all significant multifractal characteristics. Moreover, the multifractal strength of cross-correlation between the carbon emission market and crude oil market is less than that between the carbon emission market and new energy market in Europe. The Chinese market is the opposite. In addition, the multifractal strength of cross-correlation between the crude oil market and new energy market in Europe is more than that between the crude oil market and new energy market in China. It is also found that the long-range correlation of the sequences themselves and the fat-tailed distribution in fluctuations are the common causes of the multifractality, and the fat-tailed in fluctuations distribution contributes more to the multifractals of the series.
基金Supported by the NSFC-Shandong Joint Fund “Study on the DisasterCausing Mechanism and Disaster Prevention Countermeasures of MultiSource Storm Surges”(No.U1706226)the National Natural Science Foundation of China “Coastal Engineering and Risk Assessment Based on a Four-Layer Nested Multi-Objective Probability Model”(No.51379195)+1 种基金the Natural Science Foundation of Shandong Province “Three-Layer Nested Multi-Objective Probability Prediction and Risk Assessment in Coastal Engineering”(No.ZR2013EEM034)the Program of Promotion Plan for Postgraduates’ Educational Quality “Paying More Attention to the Study on the Cultivation Mode of Mathematical Modeling for Engineering Postgraduates”(No.861801232417)
文摘When exploring the temporal and spatial change law of ocean environment, the most common method used is using smaller-scale observed data to derive the change law for a larger-scale system. For instance, using 30-year observation data to derive 100-year return period design wave height. Therefore, the study of inherent self-similarity in ocean hydrological elements becomes increasingly important to the study of multi-year return period design wave height derivation. In this paper, we introduced multifractal to analyze the statistical characteristics of wave height series data observed from oceanic hydrological station. An improvement is made to address the existing problems of the multifractal detrended fluctuation analysis (MF-DFA) method, where trend function showed a discontinuity between intervals. The improved MFDFA method is based on signal mode decomposition, replacing piecewise polynomial fitting used in the original method. We applied the proposed method to the wave height data collected at Chaolian Island, Shandong, China, from 1963 to 1989 and was able to conclude the wave height sequence presented weak multi-fractality. This result provided strong support to the past research on the derivation of multi-year return period design wave height with observed data. Moreover, the new method proposed in this paper also provides a new perspective to explore the intrinsic characteristic of data.
基金the Senior User Project of R/V Kexue(No.KEXUE2018G11)the Science and Technology Basic Resources Investigation Program ofChina(No.2017FY100801)the Open Fund of the Key Laboratoryof Marine Geology and Environment,Chinese Academy of Sciences(No.MGE2018KG02)。
文摘Massive seamounts have been surveyed and documented in the last decades.However,the morphologies of seamounts are usually described in qualitative manners,yet few quantitative detections have been carried out.Here,based on the high-re solution multi-beam bathymetric data,we report a recentlysurveyed guy ot on the Caroline Ridge in the West Pacific,and the large-scale volcanic structures and smallscale erosive-depositional landforms in the guyot area have been identified.The multifractal features of the guyot are characterized for the first time by applying multifractal detrended fluctuation analysis on the surveyed bathymetric data.The results indicate that the multifractal spectrum parameters of the seafloor have strong spatial dependency on the fluctuations of local landforms.Both small-and large-scale components contribute to the degree of asymmetry of the multifractal spectrum(B),while the fluctuations of B are mostly attributed to the changes in small-scale roughness.The maximum singularity strength(α0)correlates well with the roughness of large-scale landforms and likely reflects the large-scale topographic irregularity.Comparing to traditional roughness parameters or monofractal exponents,multifractal spectra are able to depict not only the multiscale characteristics of submarine landforms,but also the spatial variations of scaling behaviors.Although more comparative works are required for various seamounts,we hope this study,as a case of quantifying geomorphological characters and multiscale behaviors of seamounts,can encourage further studies on seamounts concerning geomorphological processes,ocean bottom circulations,and seamount ecosystems.
基金supported by the National Natural Science Foundation of China (42230708)the Joint CAS (Chinese Academy of Sciences) & MPG (Max-Planck-Gesellschaft) Research Project (HZXM20225001MI)the Tianshan Talent Project of Xinjiang Uygur Autonomous Region, China (2022TSYCLJ0056)。
文摘The shrinkage of the Aral Sea,which is closely related to the Amu Darya River,strongly affects the sustainability of the local natural ecosystem,agricultural production,and human well-being.In this study,we used the Bayesian Estimator of Abrupt change,Seasonal change,and Trend(BEAST)model to detect the historical change points in the variation of the Aral Sea and the Amu Darya River and analyse the causes of the Aral Sea shrinkage during the 1950–2016 period.Further,we applied multifractal detrend cross-correlation analysis(MF-DCCA)and quantitative analysis to investigate the responses of the Aral Sea to the runoff in the Amu Darya River,which is the main source of recharge to the Aral Sea.Our results showed that two significant trend change points in the water volume change of the Aral Sea occurred,in 1961 and 1974.Before 1961,the water volume in the Aral Sea was stable,after which it began to shrink,with a shrinkage rate fluctuating around 15.21 km3/a.After 1974,the water volume of the Aral Sea decreased substantially at a rate of up to 48.97 km3/a,which was the highest value recorded in this study.In addition,although the response of the Aral Sea's water volume to its recharge runoff demonstrated a complex non-linear relationship,the replenishment of the Aral Sea by the runoff in the lower reaches of the Amu Darya River was identified as the dominant factor affecting the Aral Sea shrinkage.Based on the scenario analyses,we concluded that it is possible to slow down the retreat of the Aral Sea and restore its ecosystem by increasing the efficiency of agricultural water use,decreasing agricultural water use in the middle and lower reaches,reducing ineffective evaporation from reservoirs and wetlands,and increasing the water coming from the lower reaches of the Amu Darya River to the 1961–1973 level.These measures would maintain and stabilise the water area and water volume of the Aral Sea in a state of ecological restoration.Therefore,this study focuses on how human consumption of recharge runoff affects the Aral Sea and provides scientific perspective on its ecological conservation and sustainable development.
文摘This paper presents fault detection,classification,and location for a PV-Wind-based DC ring microgrid in the MATLAB/SIMULINK platform.Initially,DC fault signals are collected from local measurements to examine the outcomes of the proposed system.Accurate detection is carried out for all faults,(i.e.,cable and arc faults)under two cases of fault resistance and distance variation,with the assistance of primary and secondary detection techniques,i.e.second-order differential current derivatived2I3 dt2and sliding mode window-based Pearson’s correlation coefficient.For fault classification a novel approach using modified multifractal detrended fluctuation analysis(M-MFDFA)is presented.The advantage of this method is its ability to estimate the local trends of any order polynomial function with the help of polynomial and trigonometric functions.It also doesn’t require any signal processing algorithm for decomposition resulting and this results in a reduction of computational burden.The detected fault signals are directly passed through the M-MFDFA classifier for fault type classification.To enhance the performance of the proposed classifier,statistical data is obtained from the M-MFDFA feature vectors,and the obtained data is plotted in 2-D and 3-D scatter plots for better visualization.Accurate fault distance estimation is carried out for all types of faults in the DC ring bus microgrid with the assistance of recursive least squares with a forgetting factor(FF-RLS).To verify the performance and superiority of the proposed classifier,it is compared with existing classifiers in terms of features,classification accuracy(CA),and relative computational time(RCT).
基金supported by the National Natural Science Foundation of China(No.52160024)the Natural Science Foundation of Hunan Province,China(No.2022JJ30475)+2 种基金the Innovation Team Funds of China West Normal University(No.KCXTD2023-4)the Natural Science Foundation of Sichuan,China(No.24NSFSC0537)the Fundamental Research Funds of China West Normal University(Nos.22kE015 and 22kE016).
文摘As an important component of secondary aerosols,sulfate plays a crucial role in regulating atmospheric radiative balance and influencing the secondary formation of ozone(O_(3)).In real atmosphere,atmospheric oxidants NO_(2)and O_(3)can promote the oxidation of SO_(2)to form sulfate(SO_(4)^(2−))through multiphase chemistry that occur at different time scales.Due to the combined impact of meteorology,pollution sources,atmospheric chemistry,etc.,time-scale dependence of SO_(2)-SO_(4)^(2−)conversion makes the impact of NO_(2)/O_(3)on it more complex.In this study,based on long-term time series(2013-2020)of air pollution variables from seven stations in Hong Kong,the Multifractal Detrended Cross-Correlation Analysis(MFDCCA)method has been employed to quantify the cross-correlations between SO_(2)and SO_(4)^(2−)in real atmosphere at different time scales,for examining the time-scale dependence of SO_(2)-SO_(4)^(2−)conversion efficiency.Furthermore,the Pearson correlation analysis has been used to study the influence of NO_(2)/O_(3)on SO_(2)-SO_(4)^(2−)conversion,and the regional and seasonal differences have been analyzed by considering factors such as meteorology,pollution sources,and regional transport.Changes in the main components of secondary aerosols are closely linked with the co-control of regional PM_(2.5)and O_(3).Therefore,the exploration of the impact of co-existing NO_(2)/O_(3)gases on the secondary formation of sulfates in real atmosphere is significant.
