Emerging bio-inspired computing systems simulate the cognitive functions of the brain for the realiza-tion of future computing systems.For the development of such efficient neuromorphic electronics,the emulation of sh...Emerging bio-inspired computing systems simulate the cognitive functions of the brain for the realiza-tion of future computing systems.For the development of such efficient neuromorphic electronics,the emulation of short-term and long-term synaptic plasticity behaviors of the biological synapses is an es-sential step.However,the electronic synaptic devices suffer from higher variability issues which hinder the application of such devices to build neuromorphic systems.For practical applications,it is essen-tial to minimize the cycle-to-cycle and device-to-device variations in the synaptic functions of artifi-cial electronic synapses.This study involves the fabrication of diffusive memristor devices using WTe_(2) chalcogenide as the main switching material.The choice of the switching material provides a facile so-lution to the variability problem.The greater uniformity in the switching characteristics of the WTe_(2)-based memristor offers higher uniformity for the synaptic emulation.These devices exhibit both volatile and nonvolatile switching properties,allowing them to emulate both short-term and long-term synaptic functions.The WTe_(2)-based electronic synaptic devices present a high degree of uniformity for the emula-tion of various essential biological synaptic functions including short-term potentiation(STP),long-term potentiation(LTP),long-term depression(LTD),spike-rate-dependent plasticity(SRDP),and spike-timing-dependent plasticity(STDP).A higher recognition accuracy of∼92%is attained for pattern recognition using the modified National Institute of Standards and Technology(MNIST)handwritten digits,which is attributed to the enhanced linearity and higher uniformity of LTP/LTD characteristics.展开更多
An experimental study of the diffusive mass transfer between a droplet and an oscillating immiscible liquid in a horizontal axisymmetricHele-Shaw cell is carried out.Theliquid oscillates radially in the cell.Thetransv...An experimental study of the diffusive mass transfer between a droplet and an oscillating immiscible liquid in a horizontal axisymmetricHele-Shaw cell is carried out.Theliquid oscillates radially in the cell.Thetransverse size of the droplet exceeds the cell thickness.The viscosities of the droplet and the surrounding liquid are comparable.Relevant effort is provided to design and test an experimental setup and validate a protocol for determining the mass transfer rate of a solute in a two-liquid system.In particular,fluorescent dye Rhodamine B is considered as the solute.A critical comparison of the situations with and without oscillation is implemented.A procedure is introduced and validated to determine the molecular and effective diffusion coefficients through evaluation of the growth of the diffusion zone width over time.It is shown that,in the presence of the liquid oscillations,there is a significant increase in the width of the zone in which Rhodamine B is present compared to the reference case with no oscillations.The oscillatory flow leads to an intensification of the solute diffusion due to intense time-averaged flows inside the droplet and the surrounding liquid and oscillations of the drop itself.Thestudy is of significant practical interest with particular relevance to typical processes for liquid-liquid extraction.展开更多
The effects of long-term moisture changes on the migration,release,and bioavailability of selenium in soil are complex.Due to the lack of effective monitoring methods for precise quantification,its dynamic behavior is...The effects of long-term moisture changes on the migration,release,and bioavailability of selenium in soil are complex.Due to the lack of effective monitoring methods for precise quantification,its dynamic behavior is still unclear.Based on the DGT(Diffusive Gradients in Thin-films)technology,this study sets up three moisture control scenarios:continuous wet,wet-dry alternating,and continuous dry,and carries out a 6-month soil moisture control experiment.In the experiment,the DGT device collected the diffusion gradient data of soil selenium under different scenarios,and analyzed the migration characteristics of selenium in combination with the adsorption isotherm.Meanwhile,the release rate,migration coefficient,and bioavailability parameters of selenium are calculated by fitting the first-order kinetic model,further verifying the reliability and applicability of the DGT data.The experimental results demonstrate that under continuous wet conditions,the release rate of soil selenium reaches 1.85µg·cm^(-2)·h^(-1),with a migration coefficient of 0.012 cm^(2)·h^(-1)and a bioavailability parameter of 0.74;under wet-dry alternating conditions,they are 1.42µg·cm^(-2)·h^(-1),0.01 cm^(2)·h^(-1),and 0.68,respectively;under continuous dry conditions,the release rate of soil selenium is the smallest,at 0.88µg·cm^(-2)·h^(-1),with a migration coefficient of 0.004 cm^(-2)·h^(-1)and a bioavailability parameter of 0.5.The results of this experiment reveal the dynamic behavior of soil selenium under different moisture conditions and reflect the high efficiency of DGT technology in dynamic monitoring and quantitative analysis of soil selenium behavior,providing a scientific basis for the optimal management of rhizosphere soil selenium.展开更多
To investigate the potential use of two Japanese regional clayey soils, named Ariake clay and Akaboku soil, as soil barrier materials, a series of laboratory diffusion tests are presented. Using an available computer ...To investigate the potential use of two Japanese regional clayey soils, named Ariake clay and Akaboku soil, as soil barrier materials, a series of laboratory diffusion tests are presented. Using an available computer program Pollute V6.3, the effective diffusion coefficients of K^＋ of the soils were back-calculated from the diffusion tests. It is found that the Ariake clay has a larger effective diffusion coefficient than the Akaboku soil, indicating that the Ariake clay may provide a better diffusion barrier. A comparison of the effective diffusion coefficients between the single-salt solution condition and the multi-salt solution condition indicates that soils have higher effective diffusion coefficients under the former condition. It is suggested to use miscible solution close to landfill leachates for determining effective diffusion coefficients of specified chemical species for a practical design.展开更多
基金supported by the Singapore Ministry of Educa-tion under Research(Grant no.MOE-T2EP50120-0003).
文摘Emerging bio-inspired computing systems simulate the cognitive functions of the brain for the realiza-tion of future computing systems.For the development of such efficient neuromorphic electronics,the emulation of short-term and long-term synaptic plasticity behaviors of the biological synapses is an es-sential step.However,the electronic synaptic devices suffer from higher variability issues which hinder the application of such devices to build neuromorphic systems.For practical applications,it is essen-tial to minimize the cycle-to-cycle and device-to-device variations in the synaptic functions of artifi-cial electronic synapses.This study involves the fabrication of diffusive memristor devices using WTe_(2) chalcogenide as the main switching material.The choice of the switching material provides a facile so-lution to the variability problem.The greater uniformity in the switching characteristics of the WTe_(2)-based memristor offers higher uniformity for the synaptic emulation.These devices exhibit both volatile and nonvolatile switching properties,allowing them to emulate both short-term and long-term synaptic functions.The WTe_(2)-based electronic synaptic devices present a high degree of uniformity for the emula-tion of various essential biological synaptic functions including short-term potentiation(STP),long-term potentiation(LTP),long-term depression(LTD),spike-rate-dependent plasticity(SRDP),and spike-timing-dependent plasticity(STDP).A higher recognition accuracy of∼92%is attained for pattern recognition using the modified National Institute of Standards and Technology(MNIST)handwritten digits,which is attributed to the enhanced linearity and higher uniformity of LTP/LTD characteristics.
基金supported by the Russian Science Foundation(Grant No.23-11-00242).
文摘An experimental study of the diffusive mass transfer between a droplet and an oscillating immiscible liquid in a horizontal axisymmetricHele-Shaw cell is carried out.Theliquid oscillates radially in the cell.Thetransverse size of the droplet exceeds the cell thickness.The viscosities of the droplet and the surrounding liquid are comparable.Relevant effort is provided to design and test an experimental setup and validate a protocol for determining the mass transfer rate of a solute in a two-liquid system.In particular,fluorescent dye Rhodamine B is considered as the solute.A critical comparison of the situations with and without oscillation is implemented.A procedure is introduced and validated to determine the molecular and effective diffusion coefficients through evaluation of the growth of the diffusion zone width over time.It is shown that,in the presence of the liquid oscillations,there is a significant increase in the width of the zone in which Rhodamine B is present compared to the reference case with no oscillations.The oscillatory flow leads to an intensification of the solute diffusion due to intense time-averaged flows inside the droplet and the surrounding liquid and oscillations of the drop itself.Thestudy is of significant practical interest with particular relevance to typical processes for liquid-liquid extraction.
文摘The effects of long-term moisture changes on the migration,release,and bioavailability of selenium in soil are complex.Due to the lack of effective monitoring methods for precise quantification,its dynamic behavior is still unclear.Based on the DGT(Diffusive Gradients in Thin-films)technology,this study sets up three moisture control scenarios:continuous wet,wet-dry alternating,and continuous dry,and carries out a 6-month soil moisture control experiment.In the experiment,the DGT device collected the diffusion gradient data of soil selenium under different scenarios,and analyzed the migration characteristics of selenium in combination with the adsorption isotherm.Meanwhile,the release rate,migration coefficient,and bioavailability parameters of selenium are calculated by fitting the first-order kinetic model,further verifying the reliability and applicability of the DGT data.The experimental results demonstrate that under continuous wet conditions,the release rate of soil selenium reaches 1.85µg·cm^(-2)·h^(-1),with a migration coefficient of 0.012 cm^(2)·h^(-1)and a bioavailability parameter of 0.74;under wet-dry alternating conditions,they are 1.42µg·cm^(-2)·h^(-1),0.01 cm^(2)·h^(-1),and 0.68,respectively;under continuous dry conditions,the release rate of soil selenium is the smallest,at 0.88µg·cm^(-2)·h^(-1),with a migration coefficient of 0.004 cm^(-2)·h^(-1)and a bioavailability parameter of 0.5.The results of this experiment reveal the dynamic behavior of soil selenium under different moisture conditions and reflect the high efficiency of DGT technology in dynamic monitoring and quantitative analysis of soil selenium behavior,providing a scientific basis for the optimal management of rhizosphere soil selenium.
文摘To investigate the potential use of two Japanese regional clayey soils, named Ariake clay and Akaboku soil, as soil barrier materials, a series of laboratory diffusion tests are presented. Using an available computer program Pollute V6.3, the effective diffusion coefficients of K^＋ of the soils were back-calculated from the diffusion tests. It is found that the Ariake clay has a larger effective diffusion coefficient than the Akaboku soil, indicating that the Ariake clay may provide a better diffusion barrier. A comparison of the effective diffusion coefficients between the single-salt solution condition and the multi-salt solution condition indicates that soils have higher effective diffusion coefficients under the former condition. It is suggested to use miscible solution close to landfill leachates for determining effective diffusion coefficients of specified chemical species for a practical design.
