In this paper, some indices of sulfide, organic carbon, oil and heavy metals （copper, lead, zinc, cadmium, mercury, arsenic and chromium） in the sediments from Dagu Dainage Canal at the Bohai Bay during four seasons...In this paper, some indices of sulfide, organic carbon, oil and heavy metals （copper, lead, zinc, cadmium, mercury, arsenic and chromium） in the sediments from Dagu Dainage Canal at the Bohai Bay during four seasons in 2012 - 2013 are selected, and Water Quality Pollution Index （API） is applied to evaluate water quality indices, aiming for the systematic evaluation of the water quality of Dagu Dainage Canal. The results showed that four stations of D3, D6, D7and D9 for S2 had the type Ⅱand Ⅲ of water; others had the type Ⅰ ; the total level of TOC, TPH, Cu, Pb, Zn, Cd, Hg, As and Cr were type Ⅰ, Ⅳ, Ⅱ, Ⅴ, Ⅱ, Ⅴ, Ⅲ, Vand Ⅴ. Water Quality Pollution Index （API） was 3.28, which illustrated Dagu Dainage Canal was in the state of contamination and the degree of pollution exceeded the standard functional areas.展开更多
Persistent organochlorine compounds were analyzed by means of GC-ECD in surface sediment samples from two selected rivers in Tianjin, Haihe River and Dagu Drainage River. A total of 16 surface sediment sites were sele...Persistent organochlorine compounds were analyzed by means of GC-ECD in surface sediment samples from two selected rivers in Tianjin, Haihe River and Dagu Drainage River. A total of 16 surface sediment sites were selected along the both rivers. The frequency of detection of T-HCH and T-DDT in sediment samples both was up to 100%, which illustrated that the contamination of HCH and DDT was widespread in Haihe and Dagu Drainage Rivers. Results indicated that the concentrations of various pesticides in sediments from Haihe River were in the range of 3.30-75.96 ng/g dw for T-HCH and 1.57-211.57 ng/g dw for T-DDT. Compared with Haihe River, Dagu Drainage River was contaminated by HCHs and DDTs along the all locations and the values of T-HCH and T-DDT residues in sediments ranged from 2.30 to 124.61 ng/g dw and from 11.28 to 237.30 ng/g dw, respectively, The possible pollution sources were analyzed through monitoring results of organochlorine pesticides（OCPs） residues in sediments from the two rivers. The investigation also indicated that HCH was still used as pesticide in Tianjin partial area.展开更多
To understand the pollution characteristics and distributions of microplastics in the Dagu River,an important inland river that flows to Jiaozhou Bay,the abundance,particle size,shape,color,and polymer type of micropl...To understand the pollution characteristics and distributions of microplastics in the Dagu River,an important inland river that flows to Jiaozhou Bay,the abundance,particle size,shape,color,and polymer type of microplastics in the surface waters and floodplain sediments were investigated.The results showed that the abundance of microplastics in the surface waters varied between 0.68 and 3.96 items L^(−1).The abundance of microplastics in the floodplain sediments varied between 115.5 and 495 items kg^(−1).The distribution of microplastics in the river has obvious characteristics:1)The abundance of microplastics downstream was significantly higher than that upstream.2)The abundance of microplastics decreased significantly in the estuary.3)The abundance of microplastics was higher in densely populated areas.4)Factors such as effluent discharge from sewage treatment plants and inflow of tributaries affect the abundance of microplastics in rivers.The main polymer types of microplastics were polypropylene(PP),polyethylene(PE),and polyvinyl chloride(PVC).Both the abundance and polymer types of microplastics show a positive correlation between the surface waters and floodplain sediment samples,indicating that the microplastics in surface waters and floodplain sediments come from the same source.The present study demonstrates that the abundance,distribution,and sources of microplastics might be affected by geology,hydrogeology,land use types,and anthropogenic activities.This study provides basic data for the study of microplastics in rivers and provides a reference for the establishment of microplastic control measures.展开更多
Based on the 39 surface sediment samples collected in the flood season and the dry season in 2012 respectively and the measured hydrological data in October 2012, the sediment grain size characteristics has been analy...Based on the 39 surface sediment samples collected in the flood season and the dry season in 2012 respectively and the measured hydrological data in October 2012, the sediment grain size characteristics has been analyzed and the response mechanism of surface sediments to estuarine hydrodynamics was revealed by calculating the range of waves and tidal currents. The results show that:(1) The grain size of the surface sediment samples decreased gradually from land to sea in the flood season. The fine sediment was redistributed under marine hydrodynamics in the dry season and the sediments showed coarser tendency ingeneral;(2) tidal current stirring sediment was very obvious in Dagu River estuary area, and wave stirring sediments mainly occurred in the tidal flat area and estuary sand bar area;(3) in the flood season, surface sediment sat the estuary were transported towards south and southeast. In the dry season, surface sediments were transported towards southwest at the north area of Jiaozhou Bay Bridge, and sediments were transported towards northeast area at the south of Jiaozhou Bay Bridge.展开更多
Sediment samples were collected in the intertidal zone of the Dagu River Estuary, Jiaozhou Bay, China in April,July and October 2010 and February 2011 for examining seasonal dynamics of meiofaunal distribution and the...Sediment samples were collected in the intertidal zone of the Dagu River Estuary, Jiaozhou Bay, China in April,July and October 2010 and February 2011 for examining seasonal dynamics of meiofaunal distribution and their relationship with environmental variables. A total of ten meiofaunal taxa were identified, including free-living marine nematodes, benthic copepods, polychaetes, oligochaetes, bivalves, ostracods, cnidarians, turbellarians,tardigrades and other animals. Free-living marine nematodes were the most dominant group in both abundance and biomass. The abundances of marine nematodes were higher in winter and spring than those in summer and autumn. Most of the meiofauna distributed in the 0–2 cm sediment layer. The abundance of meiofauna in hightidal zone was lower than those in low-tidal and mid-tidal zones. Results of correlation analysis showed that Chlorophyll a was the most important factor to influence the seasonal dynamics of the abundance, biomass of meiofauna and abundances of nematodes and copepods. CLUSTER analysis divided the meiofaunal assemblages into three groups and BIOENV results indicated that salinity, concentration of organic matter, sediment sorting coefficient and sediment median diameter were the main environmental factors influencing the meiofaunal assemblages.展开更多
Dissolved organic carbon （DOC） is an important component for both carbon cycle and energy balance. The concentration, UV absorbance, and export flux of DOC in the natural environment dominate many important transpor...Dissolved organic carbon （DOC） is an important component for both carbon cycle and energy balance. The concentration, UV absorbance, and export flux of DOC in the natural environment dominate many important transport processes. To better understand the temporal and spatial variation of DOC, 7 sites along the Lower Dagu River were chosen to conduct a comprehensive measure- ment from March 2013 to February 2014. Specifically, water samples were collected from the Lower Dagu River between the 26th and 29th of every month during the experimental period. The DOC concentration （Cooc） and UV absorbance were analyzed using a total organic carbon analyzer and the ultraviolet-visible absorption spectrum, and the DOC export flux was estimated with a simple empirical model. The results showed that the CDoc of the Lower Dagu River varied from 1.32 to 12.56 mg/L, consistent with global rivers. The CDoc and UV absorbance showed significant spatial variation in the Dagu River during the experiential period because of the upstream natural processes and human activities in the watershed. The spatial variation is mainly due to dam or reservoir constructions, riverside ecological environment changes, and non-point source or wastewater discharge. The seasonal variation of CDoc was mainly related to the source of water DOC, river runoff, and temperature, and the UV absorbance and humification degree of DOC had no obvious differences among months （P〈 0.05）. UV absorbance was applied to test the CDOC in Lower Dagu River using wave lengths of 254 and 280 nm. The results revealed that the annual DOC export flux varied from 1.6 to 3.76x 105 g C^rn2/yr in a complete hydrological year, significantly lower than the global average. It is worth mentioning that the DOC export flux was mainly concentrated in summer （-90% of all-year flux in July and August）, since the runoff in the Dagu River took place frequently in summer. These observations implied environment change could bring the temporal-spatial variation of DOC and the exports, which would further affect the land-ocean interactions in the Lower Dagu River and the global carbon cycle.展开更多
Concentrations of polybrominated diphenyl ethers (PBDEs), organochlorine pesticides (OCPs) and heavy metals in two sediment cores, taken from the Dagu Drainage River, were determined. The contamination trends of these...Concentrations of polybrominated diphenyl ethers (PBDEs), organochlorine pesticides (OCPs) and heavy metals in two sediment cores, taken from the Dagu Drainage River, were determined. The contamination trends of these three kinds of compounds were obtained. The results showed that concentrations of PBDEs increased in recent years; there were new contamination sources for OCPs in this area; contamination levels of heavy metals had no significant change in the last several years. Comparing the results of these two cores, erosion and dilution of seawater had different effects on the transportation of these compounds.展开更多
基金financially supported by Key Laboratory of Marine Oil Spill Identification and Damage Assessment Technology, State Oceanic Administration (201214)Key Laboratory of Pollution Processes and Environmental Criteria (Nankai University),Ministry of Education (KL-PPEC-2013-09)
文摘In this paper, some indices of sulfide, organic carbon, oil and heavy metals （copper, lead, zinc, cadmium, mercury, arsenic and chromium） in the sediments from Dagu Dainage Canal at the Bohai Bay during four seasons in 2012 - 2013 are selected, and Water Quality Pollution Index （API） is applied to evaluate water quality indices, aiming for the systematic evaluation of the water quality of Dagu Dainage Canal. The results showed that four stations of D3, D6, D7and D9 for S2 had the type Ⅱand Ⅲ of water; others had the type Ⅰ ; the total level of TOC, TPH, Cu, Pb, Zn, Cd, Hg, As and Cr were type Ⅰ, Ⅳ, Ⅱ, Ⅴ, Ⅱ, Ⅴ, Ⅲ, Vand Ⅴ. Water Quality Pollution Index （API） was 3.28, which illustrated Dagu Dainage Canal was in the state of contamination and the degree of pollution exceeded the standard functional areas.
基金The Hi-Tech Research and Development Program(863) of China(No.2002AA648010)
文摘Persistent organochlorine compounds were analyzed by means of GC-ECD in surface sediment samples from two selected rivers in Tianjin, Haihe River and Dagu Drainage River. A total of 16 surface sediment sites were selected along the both rivers. The frequency of detection of T-HCH and T-DDT in sediment samples both was up to 100%, which illustrated that the contamination of HCH and DDT was widespread in Haihe and Dagu Drainage Rivers. Results indicated that the concentrations of various pesticides in sediments from Haihe River were in the range of 3.30-75.96 ng/g dw for T-HCH and 1.57-211.57 ng/g dw for T-DDT. Compared with Haihe River, Dagu Drainage River was contaminated by HCHs and DDTs along the all locations and the values of T-HCH and T-DDT residues in sediments ranged from 2.30 to 124.61 ng/g dw and from 11.28 to 237.30 ng/g dw, respectively, The possible pollution sources were analyzed through monitoring results of organochlorine pesticides（OCPs） residues in sediments from the two rivers. The investigation also indicated that HCH was still used as pesticide in Tianjin partial area.
基金financially supported by the National Major Special Project for Water Pollution Treatment and Control ‘Technology Integration of Watershed Ecological Function Zoning Management’ Project (No. 2017ZX073 01-001)the National Key Research and Development Program of China (No. 2018YFC1407601)。
文摘To understand the pollution characteristics and distributions of microplastics in the Dagu River,an important inland river that flows to Jiaozhou Bay,the abundance,particle size,shape,color,and polymer type of microplastics in the surface waters and floodplain sediments were investigated.The results showed that the abundance of microplastics in the surface waters varied between 0.68 and 3.96 items L^(−1).The abundance of microplastics in the floodplain sediments varied between 115.5 and 495 items kg^(−1).The distribution of microplastics in the river has obvious characteristics:1)The abundance of microplastics downstream was significantly higher than that upstream.2)The abundance of microplastics decreased significantly in the estuary.3)The abundance of microplastics was higher in densely populated areas.4)Factors such as effluent discharge from sewage treatment plants and inflow of tributaries affect the abundance of microplastics in rivers.The main polymer types of microplastics were polypropylene(PP),polyethylene(PE),and polyvinyl chloride(PVC).Both the abundance and polymer types of microplastics show a positive correlation between the surface waters and floodplain sediment samples,indicating that the microplastics in surface waters and floodplain sediments come from the same source.The present study demonstrates that the abundance,distribution,and sources of microplastics might be affected by geology,hydrogeology,land use types,and anthropogenic activities.This study provides basic data for the study of microplastics in rivers and provides a reference for the establishment of microplastic control measures.
基金The authors are grateful to Lei Guo ,Xiao-lei Liu ,Yonggang Jia,Lu-lu Qiao,Bin Chen and others for discussions and help in this study. The authors are grateful to the anonymous reviewers and Dr. Yan Yang for their comments and suggestions,which significantly improved the quality of the manuscript. This study is supported financially by National Natural Science Foundation of China (41506107)Special Program for Basic Research of the Ministry of Science and Technology,China (2013FY112200),"China- ASEAN Marine Geoscience Research and Disaster Reduction and Prevention initiatives Project" Ministry of Foreign Affairs of China.
文摘Based on the 39 surface sediment samples collected in the flood season and the dry season in 2012 respectively and the measured hydrological data in October 2012, the sediment grain size characteristics has been analyzed and the response mechanism of surface sediments to estuarine hydrodynamics was revealed by calculating the range of waves and tidal currents. The results show that:(1) The grain size of the surface sediment samples decreased gradually from land to sea in the flood season. The fine sediment was redistributed under marine hydrodynamics in the dry season and the sediments showed coarser tendency ingeneral;(2) tidal current stirring sediment was very obvious in Dagu River estuary area, and wave stirring sediments mainly occurred in the tidal flat area and estuary sand bar area;(3) in the flood season, surface sediment sat the estuary were transported towards south and southeast. In the dry season, surface sediments were transported towards southwest at the north area of Jiaozhou Bay Bridge, and sediments were transported towards northeast area at the south of Jiaozhou Bay Bridge.
基金The National Natural Science Foundation of China under contract No.41576135the Student Research Development Program of Ocean University of China(OUC-SRDP)under contract No.101201051
文摘Sediment samples were collected in the intertidal zone of the Dagu River Estuary, Jiaozhou Bay, China in April,July and October 2010 and February 2011 for examining seasonal dynamics of meiofaunal distribution and their relationship with environmental variables. A total of ten meiofaunal taxa were identified, including free-living marine nematodes, benthic copepods, polychaetes, oligochaetes, bivalves, ostracods, cnidarians, turbellarians,tardigrades and other animals. Free-living marine nematodes were the most dominant group in both abundance and biomass. The abundances of marine nematodes were higher in winter and spring than those in summer and autumn. Most of the meiofauna distributed in the 0–2 cm sediment layer. The abundance of meiofauna in hightidal zone was lower than those in low-tidal and mid-tidal zones. Results of correlation analysis showed that Chlorophyll a was the most important factor to influence the seasonal dynamics of the abundance, biomass of meiofauna and abundances of nematodes and copepods. CLUSTER analysis divided the meiofaunal assemblages into three groups and BIOENV results indicated that salinity, concentration of organic matter, sediment sorting coefficient and sediment median diameter were the main environmental factors influencing the meiofaunal assemblages.
文摘Dissolved organic carbon （DOC） is an important component for both carbon cycle and energy balance. The concentration, UV absorbance, and export flux of DOC in the natural environment dominate many important transport processes. To better understand the temporal and spatial variation of DOC, 7 sites along the Lower Dagu River were chosen to conduct a comprehensive measure- ment from March 2013 to February 2014. Specifically, water samples were collected from the Lower Dagu River between the 26th and 29th of every month during the experimental period. The DOC concentration （Cooc） and UV absorbance were analyzed using a total organic carbon analyzer and the ultraviolet-visible absorption spectrum, and the DOC export flux was estimated with a simple empirical model. The results showed that the CDoc of the Lower Dagu River varied from 1.32 to 12.56 mg/L, consistent with global rivers. The CDoc and UV absorbance showed significant spatial variation in the Dagu River during the experiential period because of the upstream natural processes and human activities in the watershed. The spatial variation is mainly due to dam or reservoir constructions, riverside ecological environment changes, and non-point source or wastewater discharge. The seasonal variation of CDoc was mainly related to the source of water DOC, river runoff, and temperature, and the UV absorbance and humification degree of DOC had no obvious differences among months （P〈 0.05）. UV absorbance was applied to test the CDOC in Lower Dagu River using wave lengths of 254 and 280 nm. The results revealed that the annual DOC export flux varied from 1.6 to 3.76x 105 g C^rn2/yr in a complete hydrological year, significantly lower than the global average. It is worth mentioning that the DOC export flux was mainly concentrated in summer （-90% of all-year flux in July and August）, since the runoff in the Dagu River took place frequently in summer. These observations implied environment change could bring the temporal-spatial variation of DOC and the exports, which would further affect the land-ocean interactions in the Lower Dagu River and the global carbon cycle.
基金Supported by the National Basic Research Program of China (Grant No. 2003CB415001)Chinese Academy of Sciences (Grant No. KZCX3-SW-431)
文摘Concentrations of polybrominated diphenyl ethers (PBDEs), organochlorine pesticides (OCPs) and heavy metals in two sediment cores, taken from the Dagu Drainage River, were determined. The contamination trends of these three kinds of compounds were obtained. The results showed that concentrations of PBDEs increased in recent years; there were new contamination sources for OCPs in this area; contamination levels of heavy metals had no significant change in the last several years. Comparing the results of these two cores, erosion and dilution of seawater had different effects on the transportation of these compounds.
