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Lattice Anchoring Stabilizesα-FAPbI_(3) Perovskite for High-Performance X-Ray Detectors
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作者 Yu-Hua Huang Su-Yan Zou +5 位作者 Cong-Yi Sheng Yu-Chuang Fang Xu-Dong Wang Wei Wei Wen-Guang Li Dai-Bin Kuang 《Nano-Micro Letters》 2026年第1期337-354,共18页
Formamidinium lead iodide(FAPbI_(3))perovskite exhibits an impressive X-ray absorption coefficient and a large carrier mobility-lifetime product(μτ),making it as a highly promising candidate for X-ray detection appl... Formamidinium lead iodide(FAPbI_(3))perovskite exhibits an impressive X-ray absorption coefficient and a large carrier mobility-lifetime product(μτ),making it as a highly promising candidate for X-ray detection application.However,the presence of larger FA^(+)cation induces to an expansion of the Pb-I octahedral framework,which unfortunately affects both the stability and charge carrier mobility of the corresponding devices.To address this challenge,we develop a novel low-dimensional(HtrzT)PbI_(3) perovskite featuring a conjugated organic cation(1H-1,2,4-Triazole-3-thiol,HtrzT^(+))which matches well with theα-FAPbI_(3) lattices in two-dimensional plane.Benefiting from the matched lattice between(HtrzT)PbI_(3) andα-FAPbI_(3),the anchored lattice enhances the Pb-I bond strength and effectively mitigates the inherent tensile strain of theα-FAPbI_(3) crystal lattice.The X-ray detector based on(HtrzT)PbI_(3)(1.0)/FAPbI_(3) device achieves a remarkable sensitivity up to 1.83×10^(5)μC Gy_(air)^(−1) cm^(−2),along with a low detection limit of 27.6 nGy_(air) s^(−1),attributed to the release of residual stress,and the enhancement in carrier mobility-lifetime product.Furthermore,the detector exhibits outstanding stability under X-ray irradiation with tolerating doses equivalent to nearly 1.17×10^(6) chest imaging doses. 展开更多
关键词 α-FAPbI_(3)perovskite Conjugated organic cation Lattice anchoring Phase stability x-ray detectors
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Ultralow dark current soft X-ray detectors based on lead-free double perovskite Cs_(2)AgBiBr_(6)
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作者 Long Cheng Lijuan Huang +15 位作者 Mulin Sun Ying Meng Yuan Li Tianyu Liu Pengju Tan Mingzhu Hu Huaqing Yang Xiaolan Ma Shunjie Yu Xiaohu Hou Yong Guan Junfa Zhu Xiaosong Liu Yu Li Shibing Long Qin Hu 《Journal of Semiconductors》 2026年第1期109-116,共8页
Soft X-ray detectors play a vital role in materials science,high-energy physics and medical imaging.Cs_(2)AgBiBr_(6),a lead-free double perovskite,has gained attention for its excellent optoelectronic properties,stabi... Soft X-ray detectors play a vital role in materials science,high-energy physics and medical imaging.Cs_(2)AgBiBr_(6),a lead-free double perovskite,has gained attention for its excellent optoelectronic properties,stability,and nontoxicity.However,its fast crystallization and requirement for high-temperature annealing(>250℃)often lead to inferior film quality,limiting its application in flexible devices.This study introduces an alloying strategy that significantly improves the quality of Cs_(2)AgBiBr_(6)thin films annealed at a reduced temperature of 150℃.Devices based on the alloyed thin films exhibit an ultra-low dark current of 0.32 nA·cm^(-2)and a quantum efficiency of 725%.Furthermore,the first successful integration of Cs_(2)AgBiBr_(6)with a thinfilm transistor backplane demonstrates its superior imaging performance,indicating that Cs_(2)AgBiBr_(6)is a promising material for next-generation soft X-ray sensors. 展开更多
关键词 soft x-ray detector lead-free double perovskite Cs_(2)AgBiBr_(6) ALLOYING IMAGING
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Response estimation and evaluation of direct-conversion dual-layer perovskite X-ray detectors:a numerical study with a cascaded signal model
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作者 Han Cui Yu-Hang Tan +7 位作者 Xin Zhang Hao-Di Wu Ting Su Jiong-Tao Zhu Hai-Rong Zheng Dong Liang Xiang-Ming Sun Yong-Shuai Ge 《Nuclear Science and Techniques》 2026年第2期156-168,共13页
This study aims to investigate the responses of a perovskite-based direct-conversion dual-layer flat-panel detector(DL-FPD)numerically.To this end,the X-ray sensitivity,spatial resolution quantified by the modulation ... This study aims to investigate the responses of a perovskite-based direct-conversion dual-layer flat-panel detector(DL-FPD)numerically.To this end,the X-ray sensitivity,spatial resolution quantified by the modulation transfer function(MTF),and detective quantum efficiency(DQE)of the DL-FPD are evaluated numerically using a linear cascade model.In addition,both the single-crystal(SC)and polycrystalline(PC)structures of MAPbI_(3)are investigated,along with various other key parameters such as the material thickness,electric field strength,X-ray beam spectrum,and electronic readout noise.The results demonstrate that SC perovskite consistently exhibits better performance than PC perovskite owing to fewer material defects.Increasing the layer thickness may decrease the MTF,but can also enhance the sensitivity and DQE.Moreover,appropriately increasing the external electric field within the material can improve the sensitivity,MTF,and DQE.Finally,reducing the electronic readout noise can significantly enhance the DQE for low-dose imaging.This study demonstrates the potential of high-quality dual-energy X-ray imaging using direct-conversion perovskite DL-FPDs. 展开更多
关键词 x-ray imaging Dual-layer flat-panel detector Perovskite x-ray detector
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CMOS direct conversion X-ray detector coupled with fluorinated liquid 被引量:1
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作者 Shi-Hua Liu Chao-Song Gao +5 位作者 Xin Zhang Xiang-Ming Sun Meng Wu Zhi-Hui Han Tong Wan Yong-Shuai Ge 《Nuclear Science and Techniques》 2025年第1期59-68,共10页
X-ray detectors show potential applications in medical imaging,materials science,and nuclear energy.To achieve high detection efficiency and spatial resolution,many conventional semiconductor materials,such as amorpho... X-ray detectors show potential applications in medical imaging,materials science,and nuclear energy.To achieve high detection efficiency and spatial resolution,many conventional semiconductor materials,such as amorphous selenium,cadmium telluride zinc,and perovskites,have been utilized in direct conversion X-ray detectors.However,these semiconductor materials are susceptible to temperature-induced performance degradation,crystallization,delamination,uneven lattice growth,radiation damage,and high dark current.This study explores a new approach by coupling an FC40 electronic fluorinated liquid with a specialized high-resolution and high-readout-speed complementary metal-oxide-semiconductor(CMOS)pixel array,specifically the Topmetal II−chip,to fabricate a direct conversion X-ray detector.The fluorinated liquid FC40(molecular formula:C_(21)F_(48)N_(2))is an electronic medium that is minimally affected by temperature and displays no issues with uniform conductivity.It exhibits a low dark current and minimal radiation damage and enables customizable thickness in X-ray absorption.This addresses the limitations inherent in conventional semiconductor-based detectors.In this study,simple X-ray detector imaging tests were conducted,demonstrating the excellent coupling capability between FC40 electronic fluorinated liquid and CMOS chips by the X-ray detector.A spatial resolution of 4.0 lp/mm was measured using a striped line par card,and a relatively clear image of a cockroach was displayed in the digital radiography imaging results.Preliminary test results indicated the feasibility of fabricating an X-ray detector by combining FC40 electronic fluorinated liquid and CMOS chips.Owing to the absence of issues related to chip-material coupling,a high spatial resolution could be achieved by reducing the chip pixel size.This method presents a new avenue for studies on novel liquid-based direct conversion X-ray detectors. 展开更多
关键词 FC40 electronic fluorinated liquid CMOS pixel chip x-ray detector Spatial resolution
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Face-/Edge-Shared 3D Perovskitoid Single Crystals with Suppressed Ion Migration for Stable X-Ray Detector
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作者 Zimin Zhang Xiaoli Wang +10 位作者 Huayang Li Dong Li Yang Zhang Nan Shen Xue-Feng Yu Yucheng Liu Shengzhong Liu Haomin Song Yanliang Liu Xingzhu Wang Shi Chen 《Nano-Micro Letters》 2025年第12期336-348,共13页
Although three-dimensional metal halide perovskites are promising candidates for direct X-ray detection,the ion migration of perovskites seriously affects the detector stability.Herein,face-/edge-shared 3D heterometal... Although three-dimensional metal halide perovskites are promising candidates for direct X-ray detection,the ion migration of perovskites seriously affects the detector stability.Herein,face-/edge-shared 3D heterometallic glycinate hybrid perovskitoid Pb_(2)CuGly_(2)X_(4)(Gly=-O_(2)C-CH_(2)-NH_(2);X=Cl,Br)single crystals(SCs),in which the adjacent lead halide layers are linked by large-sized Cu(Gly)_(2)pillars,are synthesized in water.The Cu(Gly)_(2)pillars in combination with face-/edge-shared inorganic skeleton are found able to synergistically suppress the ion migration,delivering a high ion migration activation energy(Ea)of 1.06 eV.The Pb_(2)CuGly_(2)Cl_(4)SC X-ray detector displays extremely low dark current drift of 1.20×10^(-9)nA mm^(-1)s^(-1)V^(-1)under high electric field(120 V mm^(-1))and continuous X-ray irradiation(2.86 Gy),and a high sensitivity of 9,250μC Gy^(-1)cm^(-2)is also achieved.More excitingly,the Pb_(2)CuGly_(2)Cl_(4)nanocrystal can be easily dispersed in water and directly blade-coated on thin-film transistor(TFT)array substrate,and the obtained Pb_(2)CuGly_(2)Cl_(4)-based TFT array detector offers an X-ray imaging capability with spatial resolution of 2.2 lp mm^(-1). 展开更多
关键词 3D perovskitoid Single crystals Suppressed ion migration High operating stability x-ray detector
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Design of the solar X-ray detector for the Macao Science Satellite-1B 被引量:4
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作者 YongQiang Shi LianSheng Li +5 位作者 JianWu Chen FuChang Zuo XiaoPing Zhang ZhiWu Mei Li Wang Keke Zhang 《Earth and Planetary Physics》 EI CSCD 2023年第1期125-130,共6页
The solar X-ray detector(SXD)onboard the Macao Science Satellite-1B was designed to monitor solar flare bursts and to study the solar activity in the 25th solar cycle.The SXD includes two parts:a soft X-ray detection ... The solar X-ray detector(SXD)onboard the Macao Science Satellite-1B was designed to monitor solar flare bursts and to study the solar activity in the 25th solar cycle.The SXD includes two parts:a soft X-ray detection unit and a hard X-ray detection unit.Both the soft X-ray detection unit and the hard X-ray detection unit include two collimators,two X-ray detectors(a silicon drift detector and a cadmium-zinc-telluride detector),and a processing circuit.Compared with similar instruments,the energy range of the SXD is wider(1–600 ke V)and the energy resolution is better(150 e V at 5.9 ke V,12%at 59.5 ke V,and 3%at 662 keV). 展开更多
关键词 Macao Science Satellite-1B(MSS-1B) solar x-ray detector solar x-ray SPECTROMETER
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Metal-Halide Perovskite Submicrometer-Thick Films for Ultra-Stable Self-Powered Direct X-Ray Detectors 被引量:1
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作者 Marco Girolami Fabio Matteocci +7 位作者 Sara Pettinato Valerio Serpente Eleonora Bolli Barbara Paci Amanda Generosi Stefano Salvatori Aldo Di Carlo Daniele M.Trucchi 《Nano-Micro Letters》 SCIE EI CAS CSCD 2024年第9期410-431,共22页
Metal-halide perovskites are revolutionizing the world of X-ray detectors,due to the development of sensitive,fast,and cost-effective devices.Self-powered operation,ensuring portability and low power consumption,has a... Metal-halide perovskites are revolutionizing the world of X-ray detectors,due to the development of sensitive,fast,and cost-effective devices.Self-powered operation,ensuring portability and low power consumption,has also been recently demonstrated in both bulk materials and thin films.However,the signal stability and repeatability under continuous X-ray exposure has only been tested up to a few hours,often reporting degradation of the detection performance.Here it is shown that self-powered direct X-ray detectors,fabricated starting from a FAPbBr_(3)submicrometer-thick film deposition onto a mesoporous TiO_(2)scaffold,can withstand a 26-day uninterrupted X-ray exposure with negligible signal loss,demonstrating ultra-high operational stability and excellent repeatability.No structural modification is observed after irradiation with a total ionizing dose of almost 200 Gy,revealing an unexpectedly high radiation hardness for a metal-halide perovskite thin film.In addition,trap-assisted photoconductive gain enabled the device to achieve a record bulk sensitivity of 7.28 C Gy^(−1)cm^(−3)at 0 V,an unprecedented value in the field of thin-film-based photoconductors and photodiodes for“hard”X-rays.Finally,prototypal validation under the X-ray beam produced by a medical linear accelerator for cancer treatment is also introduced. 展开更多
关键词 Metal-halide perovskite thin films Direct x-ray detectors Self-powered devices Operational stability Medical linear accelerator
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Orientation and mobility control of 4HCB organic film for flexible X-ray detectors with high performance
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作者 Meng Xu Menghua Zhu +8 位作者 Dou Zhao Sixin Chen Shilin Liu Quanchao Zhang Pei Yuan Binbin Zhang Paul Sellin Wanqi Jie Yadong Xu 《Journal of Materials Science & Technology》 SCIE EI CAS CSCD 2023年第4期46-53,共8页
In comparison to inorganic counterparts,organic semiconducting(OSC)crystalline films are promising for building large-area and flexible ionizing radiation detectors for X-ray imaging or dosimetry due to their tissue e... In comparison to inorganic counterparts,organic semiconducting(OSC)crystalline films are promising for building large-area and flexible ionizing radiation detectors for X-ray imaging or dosimetry due to their tissue equivalence,simple processing and large-scale production accessibility.Fabrication processes,how-ever,hinder the ability to generate aligned and large-area films with high carrier mobility.In this work,the space-confined melt process is used to produce highly orientated 4HCB(4-hydroxycyanobenzene)OSC films with a large area of 15×18 mm^(2).The out-of-plane direction of the 4HCB film is<001>,and the benzene rings are found to be extensively overlapped inside the in-plane direction,according to the XRD patterns.The film exhibits a high resistivity up to 1012cm,and high hole mobility of 10.62 cm^(2)V^(−1)s^(−1).Furthermore,the 4HCB(80μm-thick film)based X-ray detectors can achieve a sensitivity of 93μC Gy air^(−1) cm^(−2)and on/offratio of 157.The device also shows steady flexibility,with no degradation in detecting function after 100 cycles of bending.Finally,the proposed 4HCB film detectors demonstrated a high-resolution X-ray imaging capability.The imaging of several materials with sharp edges(copper and polytetrafluoroethylene)has been obtained.This work has developed a fast but efficient approach for producing large-area,highly oriented OSC films for high-performance X-ray detectors. 展开更多
关键词 Organic semiconducting films Highly oriented x-ray detector x-ray imaging Wearable detector
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A characterization study on perovskite X-ray detector performance based on a digital radiography system
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作者 Yang Wang Qiong Zhang 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2023年第5期56-66,共11页
X-ray imaging technologies such as digital radiography(DR),is an important aspect of modern non-destructive testing and medical diagnosis.Innovative flexible X-ray detector technologies have recently been proposed and... X-ray imaging technologies such as digital radiography(DR),is an important aspect of modern non-destructive testing and medical diagnosis.Innovative flexible X-ray detector technologies have recently been proposed and are now receiving increasing attention owing to their superior material flexibility compared with traditional flat-panel detectors.This work aims to study these innovative flexible X-ray detectors in terms of their effectiveness in DR imaging,such as detection efficiency and spatial resolution.To achieve this goal,first,a Monte Carlo model was developed and calibrated to an in-lab 150 kV DR imaging system containing a flat-panel X-ray detector.Second,the validated model was updated with various types of flexible X-ray detectors to assess their performance in nearly realistic conditions.Key parameters such as the detection efficiency pertaining to the crystal material and thickness were studied and analyzed across a broader energy range up to 662 keV.Finally,the imaging performance of the different detectors was evaluated and compared to that of the flat-panel detector in the 150 kV DR imaging system.The results show that the flexible detectors such as the CsPbBr3crystal detector deliver promising performance in X-ray imaging and can be applied to a wider range of application scenarios,especially those requiring accurate detection at challenging angles. 展开更多
关键词 Flexible x-ray detector DR imaging system Monte Carlo simulation
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Calibration of Soft X-Ray Detector for Astronomic Observation
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作者 ZHAO Yi-Dong CUI Ming-Qi +9 位作者 ZHU Pei-Ping LI Gang TANG He-Sen ZHANG Ren-Jian GU Zheng-Hai GU Fu-Yuan GONG Yi-Zhong LIU Shan-Zhao SHI Xi-Zhao ZHANG Nan 《Beijing Synchrotron Radiation Facility》 2001年第2期205-212,共8页
A flowing gas proportional counter(FGPC)as the detector for astronomical observationin soft X-ray(0.2-3.5keV)range is calibrated on the 3WIB beamline at Beijing Synchrotron Ra-diation Facility(BSRF).The dead time,coun... A flowing gas proportional counter(FGPC)as the detector for astronomical observationin soft X-ray(0.2-3.5keV)range is calibrated on the 3WIB beamline at Beijing Synchrotron Ra-diation Facility(BSRF).The dead time,counting rate plateau curves,X-ray energy linearity,en-ergy resolution and window transparency of the FGPC have been measured.By means of a calibratedphotodiode(AXUV 100G IRD USA,calihrated in NIST)as a standard detector,the efficiency ofthe FGPC as function of photons energy has been obtained with an uncertainty between10%-18%. 展开更多
关键词 soft x-ray proportional counter detector calibration synchrotron radiation
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Direct Conversion X-Ray Detectors with High Sensitivity at Low Dose Rate Based on All-Inorganic Lead-Free Perovskite Wafers
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作者 Cuixian Zhang 《Detection》 2022年第2期13-27,共15页
Just as lead-based perovskites that are hot in solar cell preparation, Bi-based perovskites have demonstrated excellent performance in direct X-ray detection, especially the Cs<sub>3</sub>Bi<sub>2<... Just as lead-based perovskites that are hot in solar cell preparation, Bi-based perovskites have demonstrated excellent performance in direct X-ray detection, especially the Cs<sub>3</sub>Bi<sub>2</sub>I<sub>9</sub> single crystals (SCs). However, compared with lead-halide perovskites, one challenge for the Cs<sub>3</sub>Bi<sub>2</sub>I<sub>9</sub> SCs for X-ray detection application is that it is difficult to prepare large-sized and high-quality SCs. Therefore, how to get a large area with a high-quality wafer is also as important as Cs<sub>3</sub>Bi<sub>2</sub>I<sub>9</sub> growth method research. Here, different anti-solvents are used for the preparation of poly-crystalline powder with the Antisolvents precipitation (A) method, as a control, High-energy ball milling (B) was also used to prepare poly-crystalline powders. The resultant two types of Cs<sub>3</sub>Bi<sub>2</sub>I<sub>9</sub> wafer exhibit a micro-strain of 1.21 × 10<sup>-3</sup>, a resistivity of 5.13 × 10<sup>8</sup> Ω cm and a microstrain of 1.21 × 10<sup>-3</sup>, a resistivity of 2.21 × 10<sup>9</sup> Ω cm. As a result, an X-ray detector based on the high-quality Cs<sub>3</sub>Bi<sub>2</sub>I<sub>9</sub> wafer exhibits excellent dose rate linearity, a sensitivity of 588 μC·Gyairs<sup>-1</sup>·cm<sup>-2</sup> and a limit of detection (LoD) of 76 nGyair·s<sup>-1</sup>. 展开更多
关键词 x-ray Detection Sensitivity Cs3Bi2I9
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Calibration of the Solar X-ray Detector on-board the Macao Science Satellite-1B for Soft X-ray Detection
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作者 Man-Hei NG Xiaoping ZHANG +13 位作者 Jianwu CHEN Yongqiang SHI Fuchang ZUO Wenxi PENG Weichun FU Liansheng LI Pengwei LUO Chi-Long TANG Guozheng ZHANG Zhiwu MEI Li WANG Cunhui LI Jiaming OU Yanyan Xu 《Science China Earth Sciences》 2025年第1期11-26,共16页
The Solar X-ray Detector(SXD)on-board the Macao Science Satellite-1B(MSS-1B)was successfully launched via the Chinese Long March-2C rocket on 21 May 2023,and commenced operations in early June of the same year.The MSS... The Solar X-ray Detector(SXD)on-board the Macao Science Satellite-1B(MSS-1B)was successfully launched via the Chinese Long March-2C rocket on 21 May 2023,and commenced operations in early June of the same year.The MSS-1B/Soft X-ray Detection Units(SXDUs)employ two silicon drift detectors(SDDs),providing a wide range of energy spectra spanning from 0.7 to 24 keV.Notably,the SXDUs deliver a high-resolution capability of 0.14 keV@5.9 keV and operate with a time cadence of 1 second.Here,we perform thorough calibrations of the MSS-1B/SXDUs,employing a combination of ground experiments and simulations.In addition,quantitative analysis comparing the flux measurements obtained by the MSS-1B/SXDUs to the data collected by the Geostationary Operational Environmental Satellite(GOES),provides compelling evidence of their consistency.Furthermore,the preliminary spectral analysis results showcase the robustness and expected performance of the MSS-1B/SXDUs,unlocking their potential for facilitating the study of dynamic evolution of solar flares.Moreover,the innovative MSS-1B/Solar X-ray Detector facilitates concurrent observations of solar soft and hard X-rays,thereby making valuable contributions to the advancements in solar research. 展开更多
关键词 Macao Science Satellite-1B(MSS-1B) CALIBRATION Solar x-ray detector Spectrometer Soft x-rays Solar flares Solar abundances
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High-temperature stable and sensitive X-ray detector based on two-dimensional lead-free perovskite Cs_(4)MnBi_(2)Cl_(12) single crystal
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作者 Conghui Dun Jingli Ma +10 位作者 Mengyao Zhang Huifang Ji Meng Su Xiaoyang Xing Xinzhen Ji Meng Wang Qicong Zhou Weihong Chu Jinglu Zhang Junmin Xu Zhifeng Shi 《Nano Research》 2025年第8期1088-1096,共9页
Lead-halide perovskites have made great advances in direct X-ray detection due to their large mobility-lifetime(μτ),strong X-ray absorption,and ease of synthesis,but the presence of toxic lead and high ionic migrati... Lead-halide perovskites have made great advances in direct X-ray detection due to their large mobility-lifetime(μτ),strong X-ray absorption,and ease of synthesis,but the presence of toxic lead and high ionic migration severely limit their commercial applicability and operational stability.In this study,we substituted toxic Pb^(2+)with Bi^(3+)and Mn^(2+)for preparing eco-friendly two-dimensional lead-free perovskite Cs_(4)MnBi_(2)Cl_(12)single crystal(SC)by a hydrothermal method.The SC possesses smooth surface,good crystallinity,highμτ(1.8×10^(-3)cm^(2)·V^(-1)),and excellent stability.Therefore,the X-ray detector prepared with the Cs_(4)MnBi_(2)Cl_(12)SC achieved an extraordinary sensitivity of 2.1×10^(3)μC·Gyair^(-1)·cm^(-2)and a low limit-of-detection of 1.05 nGyair·s-1.Notably,the detector demonstrates remarkable operational stability,maintaining its original X-ray response even after 6 months of unsealed storage in air,and can function effectively at elevated temperatures up to 100℃,making it highly suitable for application in harsh environments.Moreover,the SC detector achieves high-resolution X-ray imaging because of its outstanding X-ray detection performance.This study not only verifies the feasibility of Cs_(4)MnBi_(2)Cl_(12)SC for high-performance X-ray detection and imaging but also provides new design for preparation of eco-friendly X-ray detectors with both high sensitivity and stability. 展开更多
关键词 two-dimensional perovskite Cs_(4)MnBi_(2)Cl_(12) single crystal x-ray detectors x-ray imaging
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Lead-free perovskite Cs_(2)AgBiBr_(6)/Cs_(3)Bi_(2)Br_(9) single-crystalline heterojunction X-ray detector with enhanced sensitivity and ultra-low detection limit 被引量:2
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作者 Hongjie Liu Xue Sun +10 位作者 Jiaxin Liu Xiang Li Yunqiu Hua Zhongjie Yue Jian Song Xilong Wang Yujie Yang Qianqian Lin Zhongjun Zhai Xutang Tao Guodong Zhang 《Science China Materials》 2025年第2期561-570,共10页
Lead-halide perovskite single crystal(SC)heterojunctions have attracted significant attention for X-raydetection owing to their unique combination of high sensitivity,resolution,stability and low detection limit.Howev... Lead-halide perovskite single crystal(SC)heterojunctions have attracted significant attention for X-raydetection owing to their unique combination of high sensitivity,resolution,stability and low detection limit.However,the toxicity of lead in those perovskite heterojunctions limitstheir practical applications.Herein,we report the constructionof the first all-inorganic lead-free Cs_(2)AgBiBr_(6)/Cs_(3)Bi_(2)Br_(9)SCheterojunctions with an area of 20×20 mm^(2)via a facile liquidphase epitaxial method through temperature-lowering crystallization.The epitaxial crystallization of the three-dimensional(3D)Cs_(2)AgBiBr_(6)SC film on a 2D Cs_(3)Bi_(2)Br_(9)SCsubstrate requires a large driving force for transitioning fromthe Volmer–Weber mode to the layer-by-layer growth modeunder a rapid cooling rate.The Cs_(2)AgBiBr_(6)/Cs_(3)Bi_(2)Br_(9)SCheterojunction detector achieves a high sensitivity of1390μC Gy_(air)^(−1)cm^(−2)for 100 keV hard X-ray detection atroom temperature,which is enhanced to 2075μC Gy_(air)^(−1)cm^(−2)at 75℃,demonstrating impressive high-temperature stability.Moreover,the detector achieves a detection limit of37.48 nG_(yair)s^(−1)and excellent stability for 90 days without anyencapsulation.This work demonstrates the feasibility of usingthe epitaxial mechanism of perovskite formation on a highsurface-energy substrate for the controllable construction of a3D/2D heterojunction that significantly enhances X-ray detection performance. 展开更多
关键词 lead-free halide perovskite single-crystal heterojunctions epitaxial crystallization x-ray detection low detection limit
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Substance discrimination imaging derived from switchable soft and hard x-ray sensing in direct x-ray detector 被引量:1
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作者 Jingda Zhao Xin Wang +7 位作者 Yuwei Li Qi Cheng Damian Chinedu Onwudiwe Byung Seong Bae Mehmet Ertugrul Ying Zhu Wei Lei Xiaobao Xu 《InfoMat》 2025年第2期142-152,共11页
Substance discrimination beyond the shape feature is urgently desired for x-ray imaging for enhancing target identification.With two x-ray sources or stacked two detectors,the two-energy-channel x-ray detection can di... Substance discrimination beyond the shape feature is urgently desired for x-ray imaging for enhancing target identification.With two x-ray sources or stacked two detectors,the two-energy-channel x-ray detection can discriminate substance density by normalizing the target thickness.Nevertheless,the artifacts,high radiation dose and difficulty in image alignment due to two sources or two detectors impede their widespread application.In this work,we report a single direct x-ray detector with MAPbI_(3)/MAPbBr_(3)heterojunction for switchable soft x-ray(<20 keV)and hard x-ray(>20 keV)detection under one x-ray source.Systematic characterizations confirm soft and hard x-ray deposit their energy in MAPbI_(3)and MAPbBr_(3)layer,respectively,while working voltages can control the collection of generated charge carriers in each layer for selective soft/hard x-ray detection.The switching rate between soft and hard x-ray detection mode reaches 100 Hz.Moreover,the detector possesses a moderate performance with~50 nGy s^(-1)in limit-of-detection,~8000μC Gy^(-1)cm^(-2)in sensitivity and ~7 lp/mm in imaging resolution.By defining the attenuation coefficient ratio(μL/μH)as substance label,we effectively mitigate the influence of target thickness and successfully discriminate substances in the acquired x-ray images. 展开更多
关键词 PEROVSKITE PHOTOdetector single crystal substance discrimination x-ray imaging
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Impacts of X-ray energy and beam size on CD-SAXS measurement precision
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作者 Xu-Yang Qin Bing Guo +7 位作者 Nan Pan Xin-Hao Gao Shu-Min Yang Chun-Xia Hong Ying Wang Xiu-Hong Li Chun-Ming Yang Feng-Gang Bian 《Nuclear Science and Techniques》 2026年第4期65-78,共14页
With the development of the semiconductor industry below the 7 nm scale,critical dimension small-angle X-ray scattering(CD-SAXS)has emerged as a powerful tool for quantitatively measuring nanoscale deviations.In this ... With the development of the semiconductor industry below the 7 nm scale,critical dimension small-angle X-ray scattering(CD-SAXS)has emerged as a powerful tool for quantitatively measuring nanoscale deviations.In this study,the effects of X-ray beam size and photon energy on the accuracy of critical dimension measurements were investigated.Critical dimensions measured using beams with different spot sizes showed different deviations from the expected values.Beam sizes that were either too large or too small did not improve confidence intervals.As the incident energy increased,the X-ray transmission rate increased,while the scattering cross section decreased,resulting in a gradual decrease in the signal-to-noise ratio of the diffraction peaks,which reduced the accuracy of the CD-SAXS measurements.An optimal accuracy was obtained at 12 keV with a smaller beam size.Using an effective trapezoid model,the results yielded an average pitch of 100.4±0.2 nm,width of 49.8±0.2 nm,height of 130.0±0.2 nm,and a sidewall angle below 1.1°±0.1°.These results provide crucial guidance for the future development of CD-SAXS laboratories and the construction of X-ray machines as well as robust support for research in related fields. 展开更多
关键词 Critical dimension small-angle x-ray scattering Nonlinear fitting Beam size x-ray energy Chip
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Prototype of front-end electronics based on FPGA-ADC for TOF PET detector applications
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作者 Song-Qing Liu Bo Wang +2 位作者 Wei-Wei Xu Xin-Sheng Wang Kun Hu 《Nuclear Science and Techniques》 2026年第2期134-142,共9页
Traditional digitizers for signal readout of PET detectors are based on commercial analog-to-digital converters(ADC).However,the cost and power consumption of an entire electronic readout system based on digitizers fo... Traditional digitizers for signal readout of PET detectors are based on commercial analog-to-digital converters(ADC).However,the cost and power consumption of an entire electronic readout system based on digitizers for a PET scanner are high.To address this problem,a soft-core ADC based on a field-programmable gate array(FPGA)was proposed.An FPGA-based ADC(FPGA-ADC)combines low loss and high performance.To achieve good performance,the FPGA-ADC requires three calibrations:time-to-digital converter(TDC)length calibration,TDC alignment calibration,and TDC-to-ADC calibration.A prototype front-end electronics based on FPGA-ADC was built to evaluate the performance of time-of-flight positron emission tomography(TOF PET)detectors.Each PET detector consists of a LYSO crystal single-ended coupled to a silicon photomultiplier(SiPM).The experimental results show that the full-width at half-maximum(FWHM)energy resolution for 511 keV gamma photons after saturation correction of the SiPM was 12.3%.The FWHM coincidence timing resolution(CTR)of the TOF PET detector with the readout of the front-end electronic prototype is 385.2 ps.FPGA-ADCbased front-end electronics are very promising for multichannel,low-cost,highly integrated,and power-efficient readout electronic systems for radiation detector applications. 展开更多
关键词 Front-end electronics Analog-to-digital converter Radiation detector PET FPGA
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Unity-based virtual reality for detector and event visualization in JUNO experiment
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作者 Kai-Xuan Huang Tian-Zi Song +4 位作者 Yu-Ning Su Cheng-Xin Wu Xue-Sen Wang Yu-Mei Zhang Zheng-Yun You 《Nuclear Science and Techniques》 2026年第4期127-138,共12页
Detector and event visualization are crucial components of high-energy physics(HEP)experimental software.Virtual reality(VR)technologies and multimedia development platforms,such as Unity,offer enhanced display effect... Detector and event visualization are crucial components of high-energy physics(HEP)experimental software.Virtual reality(VR)technologies and multimedia development platforms,such as Unity,offer enhanced display effects and flexible extensibility for visualization in HEP experiments.In this study,we present a VR-based method for detector and event displays in the Jiangmen Underground Neutrino Observatory(JUNO)experiment.This method shares the same detector geometry descriptions and event data model as those in the offline software and provides the necessary data conversion interfaces.The VR methodology facilitates an immersive exploration of the virtual environment in JUNO,enabling users to investigate the detector geometry,visualize event data,and tune the detector simulation and event reconstruction algorithms.Additionally,this approach supports applications in data monitoring,physics data analysis,and public outreach initiatives. 展开更多
关键词 Virtual reality Event display UNITY detector geometry JUNO
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Tracing equatorward and poleward boundaries of the magnetospheric cusp from a simulated X-ray image
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作者 Xue Wang TianRan Sun +4 位作者 C.Philippe Escoubet Andy Read YiHong Guo Steve Sembay Chi Wang 《Earth and Planetary Physics》 2026年第1期144-155,共12页
A large-scale view of the magnetospheric cusp is expected to be obtained by the Soft X-ray Imager(SXI)onboard the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE).However,it is challenging to trace the three-d... A large-scale view of the magnetospheric cusp is expected to be obtained by the Soft X-ray Imager(SXI)onboard the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE).However,it is challenging to trace the three-dimensional cusp boundary from a two-dimensional X-ray image because the detected X-ray signals will be integrated along the line of sight.In this work,a global magnetohydrodynamic code was used to simulate the X-ray images and photon count images,assuming an interplanetary magnetic field with a pure Bz component.The assumption of an elliptic cusp boundary at a given altitude was used to trace the equatorward and poleward boundaries of the cusp from a simulated X-ray image.The average discrepancy was less than 0.1 RE.To reduce the influence of instrument effects and cosmic X-ray backgrounds,image denoising was considered before applying the method above to SXI photon count images.The cusp boundaries were reasonably reconstructed from the noisy X-ray image. 展开更多
关键词 SMILE mission x-ray image cusp boundary
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Three-dimensional characterization of intermetallic compound formation in magnesium alloys with micro X-ray computed tomography
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作者 SUN Wei HU Xiao-juan +5 位作者 DENG Yang-chao YANG Yang YAO Hu ZHANG Yong-hong ZHANG Rui-feng ZENG Guang 《Journal of Central South University》 2026年第1期160-174,共15页
This comprehensive study investigates the formation and evolution of intermetallic compounds during the solidification process of magnesium alloys using advanced micro X-ray computed tomography.By analyzing both commo... This comprehensive study investigates the formation and evolution of intermetallic compounds during the solidification process of magnesium alloys using advanced micro X-ray computed tomography.By analyzing both common industrial Mg-Al-Zn alloys and a novel rare earth-containing Mg-Ni-Gd-Y alloy,we aim to characterize the nucleation,growth,and distribution of Al-Mn and eutectic intermetallics across various stages of solidification.The non destructive imaging technique employed in this research provides high-resolution,three-dimensional insights into the microstructural development,allowing for a detailed examination of the morphology,spatial arrangement,and interconnectivity of intermetallic phases.This approach overcomes limitations of traditional two-dimensional metallographic methods,offering a more comprehensive understanding of the complex three-dimensional structures formed during solidification. 展开更多
关键词 magnesium alloy x-ray computed tomography SOLIDIFICATION INTERMETALLICS DEFECTS
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