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Hydroxyl,hydroperoxyl free radicals determination methods in atmosphere and troposphere 被引量:4
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作者 Guoying Wang Yves Iradukunda +3 位作者 Gaofeng Shi Pascaline Sanga Xiuli Niu Zhijun Wu 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2021年第1期324-335,共12页
The hydroxyl radical(·OH)has a crucial function in the oxidation and removal of many atmospheric compounds that are harmful to health.Nevertheless,high reactivity,low atmospheric abundance,determination of hydrox... The hydroxyl radical(·OH)has a crucial function in the oxidation and removal of many atmospheric compounds that are harmful to health.Nevertheless,high reactivity,low atmospheric abundance,determination of hydroxyl,and hydroperoxyl radical’s quantity is very difficult.In the atmosphere and troposphere,hydroperoxyl radicals(HO_(2))are closely demanded in the chemical oxidation of the troposphere.But advances in technology have allowed researchers to improve the determination methods on the research of free radicals through some spectroscopic techniques.So far,several methods such as laser-induced fluorescence(LIF),high-performance liquid chromatography(HPLC),and chemical ionization mass spectroscopy have been identified and mostly used in determining the quantity of hydroxyl and hydroperoxyl radicals.In this systematic review,we have advised the use of scavenger as an advance for further researchers to circumvent some of these problems caused by free radicals.The primary goal of this review is to deepen our understanding of the functions of the most critical free radical(·OH,HO_(2))and also understand the currently used methods to quantify them in the atmosphere and troposphere. 展开更多
关键词 atmosphere Determination method Hydroxyl radical Hydroperoxyl radical Troposphere
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A comprehensive evaluation of RNA secondary structures prediction methods
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作者 Xinlong Chen En Lou +2 位作者 Zouchenyu Zhou Ya-Lan Tan Zhi-Jie Tan 《Chinese Physics B》 2025年第8期115-127,共13页
RNAs have important biological functions and the functions of RNAs are generally coupled to their structures, especiallytheir secondary structures. In this work, we have made a comprehensive evaluation of the performa... RNAs have important biological functions and the functions of RNAs are generally coupled to their structures, especiallytheir secondary structures. In this work, we have made a comprehensive evaluation of the performances of existingtop RNA secondary structure prediction methods, including five deep-learning (DL) based methods and five minimum freeenergy (MFE) based methods. First, we made a brief overview of these RNA secondary structure prediction methods.Afterwards, we built two rigorous test datasets consisting of RNAs with non-redundant sequences and comprehensivelyexamined the performances of the RNA secondary structure prediction methods through classifying the RNAs into differentlength ranges and different types. Our examination shows that the DL-based methods generally perform better thanthe MFE-based methods for RNAs with long lengths and complex structures, while the MFE-based methods can achievegood performance for small RNAs and some specialized MFE-based methods can achieve good prediction accuracy forpseudoknots. Finally, we provided some insights and perspectives in modeling RNA secondary structures. 展开更多
关键词 RNA secondary structure prediction computational methods comprehensive evaluation traditional methods deep-learning-based methods
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Estimation and comparison of night-time OH levels in the UK urban atmosphere using two different analysis methods 被引量:1
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作者 M.Anwar H.Khan M.M.Nazmul Hoque +3 位作者 S.Shamsul Alam M.J.Ashfold Graham Nickless Dudley E.Shallcross 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2011年第1期60-64,共5页
Night-time OH levels have been determined for UK urban surface environments using two methods, the decay and steady state approximation methods. Measurement data from the UK National Environmental Technology Centre ar... Night-time OH levels have been determined for UK urban surface environments using two methods, the decay and steady state approximation methods. Measurement data from the UK National Environmental Technology Centre archive for four urban sites (Bristol, Harwell, London Eltham and Edinburgh) over the time period of 1996 to 2000 have been used in this study. Three reactive alkenes, namely isoprene, 1,3-butadiene and trans-2-pentene were chosen for the calculation of OH levels by the decay method. Hourly measurements of NO, NO〉 03, CO and 20 VOCs were used to determine night-time OH level using the steady state approximation method. Our results showed that the night-time OH levels were in the range of 1 × 10^3-1× 10^6 molecules/cm3 at these four urbap sites in the UK. The application of a t-test of these analyses indicated that except Bristol, there was no significant difference between the OH levels found from the decay and steady state approximation methods. Night-time levels of the OH radical appeared to peak in summer and spring time tracking the night-time 03 levels which also passed through a maximum at this time. 展开更多
关键词 night-time urban National Environmental Technology Center steady state approximation hydrocarbon decay method
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Mechanism analysis of effect of MgO on reduction swelling behaviour of iron pellets in CO/H_(2)atmosphere based on first-principles calculations
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作者 Hong-ming Long Jing-shu An +3 位作者 Xing-wang Li Ting Wu Sheng-ping He Jie Lei 《Journal of Iron and Steel Research International》 2025年第1期73-84,共12页
To explain the influence mechanism of MgO on the consolidation and reduction characteristics of roasted iron pellets,the properties and structure of pellets were investigated from multi-dimensions.It indicated that th... To explain the influence mechanism of MgO on the consolidation and reduction characteristics of roasted iron pellets,the properties and structure of pellets were investigated from multi-dimensions.It indicated that the MgO addition decreased the reduction swelling index(RSI)and reduction degree of pellets in both CO and H_(2)atmospheres.During the stepwise reduction process of Fe2O3→Fe3O4→FeO,the reduction behaviour of pellets in CO and H_(2)was similar,while the reduction rate of pellets in H_(2)atmosphere was almost twice as high as that in CO atmosphere.During the stepwise reduction process of FeO→Fe,the RSI of pellets showed a logarithmic increase in CO atmosphere and a linear decrease in H_(2)atmosphere.As investigated by first-principles calculations,C and Fe mainly formed chemical bonds,and the CO reduction process released energy,promoting the formation of iron whiskers.However,H and Fe produced weak physical adsorption,and the H_(2)reduction process was endothermic,inhibiting the generation of iron whiskers.With Mg2+doping in FexO,the nucleation region of iron whiskers expanded in CO reduction process,and the morphology of iron whiskers transformed from“slender”to“stocky,”reducing RSI of the pellets. 展开更多
关键词 MGO CO atmosphere H_(2)atmosphere Reduction degree Reduction swelling index First-principles calculation
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Novel adaptive IMEX two-step Runge-Kutta temporal discretization methods for unsteady flows
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作者 Xueyu QIN Jian YU +2 位作者 Xin ZHANG Zhenhua JIANG Chao YAN 《Chinese Journal of Aeronautics》 2025年第8期142-153,共12页
Efficient and accurate simulation of unsteady flow presents a significant challenge that needs to be overcome in computational fluid dynamics.Temporal discretization method plays a crucial role in the simulation of un... Efficient and accurate simulation of unsteady flow presents a significant challenge that needs to be overcome in computational fluid dynamics.Temporal discretization method plays a crucial role in the simulation of unsteady flows.To enhance computational efficiency,we propose the Implicit-Explicit Two-Step Runge-Kutta(IMEX-TSRK)time-stepping discretization methods for unsteady flows,and develop a novel adaptive algorithm that correctly partitions spatial regions to apply implicit or explicit methods.The novel adaptive IMEX-TSRK schemes effectively handle the numerical stiffness of the small grid size and improve computational efficiency.Compared to implicit and explicit Runge-Kutta(RK)schemes,the IMEX-TSRK methods achieve the same order of accuracy with fewer first derivative calculations.Numerical case tests demonstrate that the IMEX-TSRK methods maintain numerical stability while enhancing computational efficiency.Specifically,in high Reynolds number flows,the computational efficiency of the IMEX-TSRK methods surpasses that of explicit RK schemes by more than one order of magnitude,and that of implicit RK schemes several times over. 展开更多
关键词 Implicit-explicit temporal methods Two-step Runge-Kutta methods Adaptive algorithm Unsteady flows Navier-Stokes equations
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Development prospects of residual stress detection methods
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作者 Xin LI Hanjun GAO Qiong WU 《Chinese Journal of Aeronautics》 2025年第7期601-603,共3页
In the aerospace field, residual stress directly affects the strength, fatigue life and dimensional stability of thin-walled structural components, and is a key factor to ensure flight safety and reliability. At prese... In the aerospace field, residual stress directly affects the strength, fatigue life and dimensional stability of thin-walled structural components, and is a key factor to ensure flight safety and reliability. At present, research on residual stress at home and abroad mainly focuses on the optimization of traditional detection technology, stress control of manufacturing process and service performance evaluation, among which research on residual stress detection methods mainly focuses on the improvement of the accuracy, sensitivity, reliability and other performance of existing detection methods, but it still faces many challenges such as extremely small detection range, low efficiency, large error and limited application range. 展开更多
关键词 residual stress flight safety reliability detection methods optimization traditional detection technology residual stress detection methods service performance evaluation IMPROVEMENT stress control
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Oxygen atmosphere enhances ball milling remediation of petroleum-contaminated soil and reuse as adsorptive/catalytic materials for wastewater treatment 被引量:1
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作者 Pingting Gao Simin Song +2 位作者 Mingxin Wang Meng Yao Jinjuan Xue 《Journal of Environmental Sciences》 2025年第1期652-664,共13页
Ball milling is an environmentally friendly technology for the remediation of petroleumcontaminated soil(PCS),but the cleanup of organic pollutants requires a long time,and the post-remediation soil needs an economica... Ball milling is an environmentally friendly technology for the remediation of petroleumcontaminated soil(PCS),but the cleanup of organic pollutants requires a long time,and the post-remediation soil needs an economically viable disposal/reuse strategy due to its vast volume.The present paper develops a ball milling process under oxygen atmosphere to enhance PCS remediation and reuse the obtained carbonized soil(BCS-O)as wastewater treatment materials.The total petroleum hydrocarbon removal rates by ball milling under vacuum,air,and oxygen atmospheres are 39.83%,55.21%,and 93.84%,respectively.The Langmuir and pseudo second-order models satisfactorily describe the adsorption capacity and behavior of BCS-O for transition metals.The Cu^(2+),Ni^(2+),and Mn^(2+)adsorbed onto BCS-O were mainly bound to metal carbonates and metal oxides.Furthermore,BCS-O can effectively activate persulfate(PDS)oxidation to degrade aniline,while BCS-O loaded with transition metal(BCS-O-Me)shows better activation efficiency and reusability.BCS-O and BCS-O-Me activated PDS oxidation systems are dominated by^(1)O_(2)oxidation and electron transfer.The main active sites are oxygen-containing functional groups,vacancy defects,and graphitized carbon.The oxygen-containing functional groups and vacancy defects primarily activate PDS to generate^(1)O_(2)and attack aniline.Graphitized carbon promotes aniline degradation by accelerating electron transfer.The paper develops an innovative strategy to simultaneously realize efficient remediation of PCS and sequential reuse of the postremediation soil. 展开更多
关键词 Petroleum-contaminated soil Ball milling Oxygen atmosphere PYROLYSIS Resource utilization
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Improved methods,properties,applications and prospects of microbial induced carbonate precipitation(MICP)treated soil:A review 被引量:2
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作者 Xuanshuo Zhang Hongyu Wang +3 位作者 Ya Wang Jinghui Wang Jing Cao Gang Zhang 《Biogeotechnics》 2025年第1期34-54,共21页
Soil improvement is one of the most important issues in geotechnical engineering practice.The wide application of traditional improvement techniques(cement/chemical materials)are limited due to damage ecological en-vi... Soil improvement is one of the most important issues in geotechnical engineering practice.The wide application of traditional improvement techniques(cement/chemical materials)are limited due to damage ecological en-vironment and intensify carbon emissions.However,the use of microbially induced calcium carbonate pre-cipitation(MICP)to obtain bio-cement is a novel technique with the potential to induce soil stability,providing a low-carbon,environment-friendly,and sustainable integrated solution for some geotechnical engineering pro-blems in the environment.This paper presents a comprehensive review of the latest progress in soil improvement based on the MICP strategy.It systematically summarizes and overviews the mineralization mechanism,influ-encing factors,improved methods,engineering characteristics,and current field application status of the MICP.Additionally,it also explores the limitations and correspondingly proposes prospective applications via the MICP approach for soil improvement.This review indicates that the utilization of different environmental calcium-based wastes in MICP and combination of materials and MICP are conducive to meeting engineering and market demand.Furthermore,we recommend and encourage global collaborative study and practice with a view to commercializing MICP technique in the future.The current review purports to provide insights for engineers and interdisciplinary researchers,and guidance for future engineering applications. 展开更多
关键词 Soil improvement Bio-cement MICP Improved methods Field application cases
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Flash Calcination of Kaolinite Clay in a Pilot Reactor: Evaluation of Clay Color Change in Oxidizing, Inert and Reducing Atmospheres
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作者 Gabriel Henrique Wienhage Vinícius Henrique de Freitas +4 位作者 Julio Zeppone Carlos Luis Filipe von Rainer Fabiani Luiz Felipe de Pinho Rodrigo de Souza Borges Vinicyus Rodolfo Wiggers 《Journal of Building Material Science》 2025年第1期73-82,共10页
Cement production,while essential for global infrastructure,contributes significantly to carbon dioxide emissions,accounting for approximately 7%of total emissions.To mitigate these environmental impacts,flash calcina... Cement production,while essential for global infrastructure,contributes significantly to carbon dioxide emissions,accounting for approximately 7%of total emissions.To mitigate these environmental impacts,flash calcination of kaolinitic clays has been investigated as a sustainable alternative.This technique involves the rapid heating of clays,enabling their use as supplementary cementitious materials.The primary objective of this study was to modify the color of calcined clay in various atmospheres(oxidizing,inert,and reducing)to achieve a grayish tone similar to commercial cement while preserving its reactive properties.The experimental procedure employed a tubular reactor with precise control of gas flows(atmospheric air,nitrogen,and a carbon monoxide–nitrogen mixture).Physicochemical characterization of the raw clay was conducted before calcination,with analyses repeated on the calcined clays following experimentation.Results indicated that clay calcined in an oxidizing atmosphere acquired a reddish hue,attributed to the oxidation of iron in hematite.The Clay exhibited a pinkish tone in an inert atmosphere,while calcination in a reducing atmosphere yielded the desired grayish color.Regarding pozzolanic activity,clays calcined in oxidizing and inert atmospheres displayed robust strength,ranging from 82%to 87%.Calcination in a reducing atmosphere resulted in slightly lower strength,around 74%,likely due to the clay’s chemical composition and the calcination process,which affects compound formation and material reactivity. 展开更多
关键词 Flash Calcination Kaolinite Clay Reducing atmosphere Reduction of Hematite
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Inter-hemispheric couplings in the middle atmosphere exhibited by principal component analysis of the SD-WACCM-X simulations
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作者 Sheng-Yang Gu YuBo Zeng +3 位作者 Jin Hu YuSong Qin Liang Tang YuXuan Liu 《Earth and Planetary Physics》 2025年第4期925-937,共13页
This study employs Principal Component Analysis(PCA)and 13 years of SD-WACCM-X model data(2007-2019)to investigate the characteristics and mechanisms of Inter-hemispheric Coupling(IHC)triggered by sudden stratospheric... This study employs Principal Component Analysis(PCA)and 13 years of SD-WACCM-X model data(2007-2019)to investigate the characteristics and mechanisms of Inter-hemispheric Coupling(IHC)triggered by sudden stratospheric warming(SSW)events.IHC in both hemispheres leads to a cold anomaly in the equatorial stratosphere,a warm anomaly in the equatorial mesosphere,and increased temperatures in the mesosphere and lower thermosphere(MLT)region of the summer hemisphere.However,the IHC features during boreal winter period are significantly weaker than during the austral winter period,primarily due to weaker stationary planetary wave activity in the Southern Hemisphere(SH).During the austral winter period,IHC results in a warm anomaly in the polar mesosphere of the SH,which does not occur in the NH during boreal winter period.This study also examines the possible influence of quasi-two-day waves(QTDWs)on IHC.We found that the largest temperature anomaly in the summer polar MLT region is associated with a large wind instability area,and a well-developed critical layer structure of QTDW in January.In contrast,during July,despite favorable conditions for QTDW propagation in the Northern Hemisphere,weaker IHC response is observed,suggesting that IHC features and the relationship with QTDWs during July would be more complex than during January. 展开更多
关键词 inter-hemispheric coupling principal component analysis middle atmosphere quasi-two-day waves
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Iron carbide-catalyzed deoxygenative coupling of benzyl alcohols toward bibenzyls under hydrogen atmosphere
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作者 Yichao Wang Leilei Zhang +2 位作者 Xiaoli Pan Aiqin Wang Tao Zhang 《Chinese Journal of Catalysis》 2025年第4期179-186,共8页
The direct deoxygenative homo-coupling of benzyl alcohols holds great promise to build up bibenzyl motifs in organic synthesis,yet it remains a grand challenge in selectivity and activity control.Herein,we first disco... The direct deoxygenative homo-coupling of benzyl alcohols holds great promise to build up bibenzyl motifs in organic synthesis,yet it remains a grand challenge in selectivity and activity control.Herein,we first discovered that iron carbide catalysts displayed high efficiency and selectivity in the catalytic deoxygenative homo-coupling of benzyl alcohols into bibenzyls using H_(2)as the reductant.Ir-promoted Fe0@Fe_(5)C_(2)gave the best performance among the investigated catalysts,and a broad scope of substrates with diverse functional groups could be smoothly converted into bibenzyls,with the yield up to 85%.In addition,in the presence of alkenes,three-component coupling reactions between alcohols and alkenes were also for the first time achieved to construct more complex multi-ring molecules.The radical-trapping experiment and FTIR measurements revealed the radical nature of the reaction and the significantly promoted C–O bond activation after carbonization,respectively.This work will provide guidelines for the rational design of efficient and selective catalysts for the alcohol-involved carbon-carbon coupling reactions. 展开更多
关键词 Deoxygenative coupling reaction Benzyl alcohols BIBENZYLS Iron carbide Hydrogen atmosphere
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Subseasonal impact of extreme Tibetan Plateau snow cover on the local atmosphere in summer
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作者 Yuanyan Xu Wenkai Li 《Atmospheric and Oceanic Science Letters》 2025年第5期36-40,共5页
Due to the high elevation and cold climate of the Tibetan Plateau,the western region retains extensive snow cover during the summer,which can exhibit rapid variability over the course of just a few days.This study uti... Due to the high elevation and cold climate of the Tibetan Plateau,the western region retains extensive snow cover during the summer,which can exhibit rapid variability over the course of just a few days.This study utilizes numerical experiments to investigate the atmospheric response to extreme Tibetan Plateau snow cover(TPSC)events on a subseasonal timescale during summer.The results indicate that the subseasonal variations in TPSC exert limited impact on nonlocal atmospheric circulation and temperature during this period.Nevertheless,local surface energy and atmospheric temperature exhibit rapid cooling responses to increased snow cover.Specifically,an increase in snow cover over the western Tibetan Plateau leads to a sharp rise in surface albedo,resulting in a reduction in land surface energy and a negative response in the diabatic heating rate from the surface to 350 hPa locally.This negative diabatic heating response subsequently causes a decline in both surface and overlying atmospheric temperatures.The temperature response is confined to the western Tibetan Plateau and extends vertically from the surface to approximately 350 hPa.These extreme TPSC events and their associated atmospheric impacts occur within a two-week timescale. 展开更多
关键词 Land-atmosphere interaction Snow cover Extreme events Atmospheric temperature Tibetan Plateau
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Enhancing External Combustion Efficiency in Stirling Engine Combustors: Influence of Oxygen Atmosphere, Ejection Ratio, and Pressure
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作者 Yelin Li Jian Lan +5 位作者 Tian Lyu Jiefei Zhou Xin Yang Gangtao Lin Genxiang Gu Dong Han 《哈尔滨工程大学学报(英文版)》 2025年第3期634-645,共12页
Knowing the optimal operating parameters of Stirling engines is important for efficient combustion through adaptability to changed pressures and oxygen atmospheres. In this study, the optimum operating conditions for ... Knowing the optimal operating parameters of Stirling engines is important for efficient combustion through adaptability to changed pressures and oxygen atmospheres. In this study, the optimum operating conditions for efficient combustion in a singular Stirling engine combustor at different oxygen atmospheres were investigated and determined. Numerical simulations were performed to investigate the effects of ejection ratio and pressure on combustion performance. In an oxygen/carbon dioxide atmosphere, the results show that increasing the ejection ratio substantially alters the flame distribution in the Stirling engine combustor, increasing heat transfer and external combustion efficiency. In contrast, increasing the ejection ratio reduces the average and maximum temperatures of the Stirling engine combustor. Increased pressure affects the flame distribution in the Stirling engine combustor and impedes the flow and convective heat transfer in the combustor, reducing the overall external combustion efficiency at pressures above 6.5 MPa. In an air/carbon dioxide atmosphere, an increased ejection ratio reduces the average and maximum temperatures in the Stirling engine combustor. However, the overall flame distribution does not change substantially. The external combustion efficiency tends to increase and then decrease because of two opposing factors: the increase in the convective heat transfer coefficient and the decrease in the temperature difference. Increasing pressure inhibits forced convection heat transfer in the Stirling engine combustor, reducing external combustion efficiency, which drops from 78% to 65% when pressure increases from 0.2 MPa to 0.5 MPa. 展开更多
关键词 Stirling engine combustor Oxygen atmosphere Ejection ratio PRESSURE External combustion efficiency
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Influence of cooling atmosphere on the structure,magnetization,and dielectric properties of CaBaCo_(4)O_(7)
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作者 Gaoshang Gong Minghao Wang +4 位作者 Ruoshui Liu Yang Wu Lichen Wang Yongqiang Wang Baogen Shen 《Chinese Physics B》 2025年第4期585-589,共5页
CaBaCo_(4)O_(7)has been widely studied because of its distinctive structure and magnetic properties.This study examined the influence of different cooling atmospheres on the structure,magnetic properties,and dielectri... CaBaCo_(4)O_(7)has been widely studied because of its distinctive structure and magnetic properties.This study examined the influence of different cooling atmospheres on the structure,magnetic properties,and dielectric behavior of CaBaCo_(4)O_(7).Samples were cooled under different atmospheric conditions to assess these influences.Our findings indicate that reduced oxygen content leads to increased lattice distortion.Since oxygen atoms play a crucial role in mediating magnetic exchange,oxygen deficiency disrupts long-range magnetic order and promotes short-range antiferromagnetic interactions.Additionally,the cooling atmosphere significantly impacts grain size,thereby affecting the dielectric constant and dielectric loss.In the argon-cooled CaBaCo_(4)O_(7)(Ar)sample,oxygen deficiency reduced dielectric permittivity and increased dielectric loss. 展开更多
关键词 CaBaCo_(4)O_(7) cooling atmosphere MAGNETIZATION DIELECTRIC
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Overview of the studies on the interactions between atmosphere,sea ice,and ocean in the Arctic Ocean and its climatic effects:Contributions from Chinese scientists
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作者 Ruibo Lei Fanyi Zhang +6 位作者 Qinghua Yang Ruonan Zhang Wenli Zhong Qi Shu Minghu Ding Fengming Hui Chao Min 《Acta Oceanologica Sinica》 2025年第3期3-34,共32页
The year,2024,marks the 40th anniversary of Chinese research expeditions in the polar regions and the 25th anniversary of its Arctic research expeditions.China has conducted 14 national Arctic research expeditions.Wit... The year,2024,marks the 40th anniversary of Chinese research expeditions in the polar regions and the 25th anniversary of its Arctic research expeditions.China has conducted 14 national Arctic research expeditions.With the increase of understandings on the global impacts of the changes of Arctic climate system,especially on China’s weather and climate,and demands for commercial utilization of the Arctic sea routes,Chinese scientists have made great progresses on in site and remote sensing observation technologies for Arctic Ocean,interaction mechanisms between atmosphere,sea ice,and ocean,the connection mechanism between the Arctic Ocean and other regions,and have achieved a series of research results.This study summarizes the research achievements by Chinese scientists in the above-mentioned aspects or beyond,identifies knowledge gaps,and based on this,discusses prospects and provides suggestions.From a perspective of observation,improving the observation capabilities of the Arctic Ocean in winter and the ocean under the ice,as well as floe-scale processes of sea ice and mesoscale and submesoscale processes of the ocean,is an urgent task to be addressed.Strengthening international cooperation is necessary for building a monitoring network for the Arctic marine environment.From a perspective of numerical simulation,the descriptive ability and parameterization scheme of sub-grid processes based on observational evidence need to be developed.From a perspective of cross-sphere interactions,in addition to the multi-media coupling within the Arctic Ocean that this review focuses on,the interaction between the Arctic Ocean and land or ice sheet(Greenland),especially the water cycle process,is also a scientific domain that needs to be considered,in the context of Arctic warming and humidification.From a perspective of climate effects,the physical mechanisms that affect the robustness of teleconnection need to be clarified. 展开更多
关键词 Chinese National Arctic Research Expedition(CHINARE) Arctic Ocean atmosphere sea ice climate
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Effects of combined soluble gas stabilization,modified atmosphere packaging and cold plasma on controlling chilled chicken breasts spoilage
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作者 Jing Li Chen Xu +6 位作者 Yifeng Lu Xiaoming Wang Shuangshuang Jin Yun Bai Xia Wang Xinglian Xu Minyi Han 《Food Science and Human Wellness》 2025年第7期2860-2871,共12页
The hurdle technology for food preservation effectively addresses the limitations of individual antimicrobial technologies by integrating their strengths.It can not only prolong the storage time of food but also maint... The hurdle technology for food preservation effectively addresses the limitations of individual antimicrobial technologies by integrating their strengths.It can not only prolong the storage time of food but also maintains its high quality.In this study,three antimicrobial and bactericidal technologies,namely soluble gas stabilization(SGS),modified atmosphere packaging(MAP),and cold plasma(CP),were applied to chilled chicken breasts.The packaging,total viable count(TVC),and physicochemical properties of chilled chicken breasts after treatments and storage at 4℃were monitored.The microbial diversity at the initial and end points of the storage time of each group was also analyzed.The results indicated that a 3−5 h SGS treatment can effectively increase the proportion of carbon dioxide in the MAP during the storage process of chilled chicken breasts,thereby alleviating the packaging collapse problem.Simultaneously,the effect of SGS,MAP,and CP combinational treatments significantly extended the storage time of chilled chicken breasts while maintaining the physicochemical qualities of samples.Compared to the control group,the TVC of chicken breast treated with SGS,MAP,and CP treatments decreased by 0.58(lg(CFU/g))at 0 day.The shelf life was extended by 5 days.After 8 days,the total volatile basic nitrogen(TVB-N)was 26.67 vs.19.50 mg/100 g,thiobarbituric acid reactive substances(TBARS)was 0.99 vs.0.72 mg MDA/kg,and TVC was 8.22 vs.6.52(lg(CFU/g)).High-throughput sequencing results showed that SGS and MAP treatments significantly reduce the proportion of Pseudomonas and Psychrobacter,which are sensitive to carbon dioxide,in the total bacterial genera.This study underscores the potential of integrating multiple antimicrobial technologies for effective food preservation. 展开更多
关键词 Soluble gas stabilization Modified atmosphere packaging Cold plasma Chilled chicken breasts Storage time Microbial diversity
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A Comprehensive Study on Application and Prospect of Hydrogel Detection Methods
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作者 Caixia Chen Pengyu Liu +3 位作者 Changhua Wang Yanyan Xie Wei Wang Xiaomin Kang 《Journal of Polymer Materials》 2025年第3期621-660,共40页
Due to their high water content,stimulus responsiveness,and biocompatibility,hydrogels,which are functional materials with a three-dimensional network structure,are widely applied in fields such as biomedicine,environ... Due to their high water content,stimulus responsiveness,and biocompatibility,hydrogels,which are functional materials with a three-dimensional network structure,are widely applied in fields such as biomedicine,environmental monitoring,and flexible electronics.This paper provides a systematic review of hydrogel charac-terization methods and their applications,focusing on primary evaluation techniques for physical properties(e.g.,mechanical strength,swelling behavior,and pore structure),chemical properties(e.g.,composition,crosslink density,and degradation behavior),biocompatibility,and functional properties(e.g.,drug release,environmental stimulus response,and conductivity).It analyzes the challenges currently faced by characterization methods,such as a lack of standardization,difficulties in dynamic monitoring,an insufficient micro-macro correlation,and poor adaptability to complex environments.It proposes solutions,such as a hierarchical standardization system,in situ imaging technology,cross-scale characterization,and biomimetic testing platforms.Looking ahead,hydrogel characterization techniques will evolve toward intelligent,real-time,multimodal coupling and standardized approaches.These techniques will provide superior technical support for precision medicine,environmental restoration,and flexible electronics.They will also offer systematic methodological guidance for the performance optimization and practical application of hydrogel materials. 展开更多
关键词 HYDROGEL characterization methods PROPERTIES STANDARDIZATION APPLICATION
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Prediction of specific spoilage organisms in smoked chicken legs with modified atmosphere packaging at 4℃ using multivariate statistical analysis
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作者 Qiang Wang Yubo Zhao +5 位作者 Yumeng Sui Qian Chen Zhiming Dong Qian Liu Baohua Kong Ligang Qin 《Food Science and Human Wellness》 2025年第1期271-281,共11页
The present study monitored bacterial succession,physicochemical properties,and volatile organic compounds(VOCs)changes in smoked chicken legs with modified atmosphere packaging(MAP,60% CO_(2) and 40%N_(2))during a 25... The present study monitored bacterial succession,physicochemical properties,and volatile organic compounds(VOCs)changes in smoked chicken legs with modified atmosphere packaging(MAP,60% CO_(2) and 40%N_(2))during a 25-day storage period at 4℃.After 15 days of storage,S erratia proteamaculans and Pseudomonas fragi became the predominant bacteria.Furthermore,physicochemical properties changed significantly,as evidenced by an increase in thiobarbituric acid reactive substances and b*(yellowness)value,and a decrease in hardness.A total of 65 VOCs were identified during storage.Correlation between bacterial succession and quality indicators(including VOCs and physicochemical properties)allowed the identification of 26 core dominant bacteria,including S.proteamaculans,Psychrobacter alimentarius,Pseudomonas putida,and Pseudomonas poae,which were positively related to spoilage VOCs(e.g.,1-octen-3-ol,1-pentanol,and 3-methyl-1-butanol)and could be defined as specific spoilage organisms(SSOs).The results of this study provide a systematic approach to predict SSOs in smoked chicken legs during storage,which can also provide a basis for product safety. 展开更多
关键词 Smoked chicken legs Modified atmosphere packaging Bacterial community Volatile organic compounds Specific spoilage organisms
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Martian atmosphere sputtering escape generated by penetrating hydrogen energetic neutral atoms
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作者 JiJie Ma LingGao Kong +13 位作者 Hao Gu WenYa Li YuMing Wang YuTian Chi BinBin Tang XiaoPeng Liu YiFan Song BaiQu Pu FuHao Qiao LiMin Wang Jun Cui Yong Wei AiBing Zhang Chi Wang 《Earth and Planetary Physics》 2025年第6期1147-1156,共10页
Atmospheric escape plays a critical role in shaping the long-term climate evolution of Mars.Among the various escape mechanisms,energetic neutral atoms(ENAs)generated through charge exchange between solar wind ions an... Atmospheric escape plays a critical role in shaping the long-term climate evolution of Mars.Among the various escape mechanisms,energetic neutral atoms(ENAs)generated through charge exchange between solar wind ions and exospheric neutrals serve as an important diagnostic for ion-neutral interactions and upper atmospheric loss.This study presents direct observations of hydrogen ENAs(H-ENAs)on the dayside of Mars by using the Mars Ion and Neutral Particle Analyzer(MINPA)onboard China’s Tianwen-1 orbiter.By analyzing H-ENA data during a coronal mass ejection and a stream interaction region from December 29,2021,to January 1,2022,and comparing these data with MAVEN/SWIA(Mars Atmosphere and Volatile EvolutioN/Solar Wind Ion Analyzer)solar wind measurements,we examine the temporal evolution of H-ENA flux and the associated sputtered escape of atmospheric constituents.The observed H-ENA velocity is consistent with upstream solar wind ions,and the H-ENA-to-ion intensity ratio is used to infer variations in exospheric density,revealing a delayed response to enhanced solar wind activity.Penetrating H-ENA intensities reach up to 5.3×10^(6)s^(−1) cm^(−2),with energy fluxes on the order of(0.5-8.1)×10^(−3) mW/m^(2).The estimated oxygen sputtered escape rate driven by penetrating H-ENAs ranges from 5.5×10^(23)s^(−1) to 5.2×10^(24)s^(−1),comparable to or exceeding previous estimates based on penetrating ions.The findings highlight the need for low-altitude H-ENA observations to better quantify their atmospheric interactions and refine our understanding of nonthermal escape processes at Mars. 展开更多
关键词 penetrating energetic neutral atoms sputtered escape Mars atmosphere loss Tianwen-1 future energetic neutral atom observations
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Advances in Research of Characteristics, Environmental Impact and Treatment Methods of Dairy Wastewater
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作者 Jiping XIE Ming QIAO +1 位作者 Ying BAI Li SONG 《Asian Agricultural Research》 2025年第3期18-21,39,共5页
Dairy wastewater,a kind of high concentration organic wastewater,is produced in large quantities and difficult to treat,and has a negative impact on the ecological environment.In this study,the source,composition,wate... Dairy wastewater,a kind of high concentration organic wastewater,is produced in large quantities and difficult to treat,and has a negative impact on the ecological environment.In this study,the source,composition,water quality characteristics of dairy wastewater and its impact on the ecological environment were analyzed,and the treatment methods of dairy wastewater at home and abroad in recent years were summarized,in order to provide a reference for the treatment of dairy wastewater. 展开更多
关键词 Dairy products WASTEWATER Treatment methods Advances in research
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