摘要
A thorough understanding of the oxygen evolution reaction(OER)in Mo-based materials is crucial for the advancement of water-splitting technologies.However,the identification of the active phase in Mo-based systems remains a subject of debate,largely due to the dissolution of molybdenum oxides in alkaline electrolytes.In this review,we provide a comprehensive overview of recent advances in the application of Mo-based materials for OER in alkaline media,with an emphasis on their diverse roles in catalysis.Various design strategies employed to optimize Mo-based materials are discussed,focusing on how these approaches influence their physicochemical properties and the specific effects of different design perspectives on their OER performance.Additionally,the structure-performance relationship underlying these materials is explored,offering insights into how structural modifications impact catalytic efficiency.Lastly,key challenges for Mo-based materials in OER applications are provided,and future research directions for further improving the efficacy of sustainable water-splitting technologies in alkaline environments are proposed.
基金
financially supported by the National Natural Science Foundation of China(52162036 and 22378342)
the Key Project of Nature Science Foundation of Xinjiang(2021D01D08)
the Major Projects of Xinjiang(2022A01005-4 and 2021A01001-1)
the Key Research and Development Project of Xinjiang(2023B01025-1)。
