期刊文献+

长江口溶解无机碳循环的地球化学研究 被引量:6

A Geochemical Study on Carbon Cycling in the Changjiang Estuary
原文传递
导出
摘要 于2005年6月对长江口23个站点的溶解性无机碳及其同位素组成进行了采样调查。结果发现长江河流区水体的pCO2均处于过饱和状态,但在进入河口区后发生大幅度的下降;δ13CDIC为-10.0‰~-0.9‰,且随盐度发生梯度性变化;DIC和δ13CDIC值偏离河水、海水混合线,显示了长江河口碳的复杂生物地球化学过程,包括内部碳酸盐岩体系及外部生物的作用:河流区主要受水-气界面CO2逸散的影响;河口区主要受光合作用的影响;海岸区则主要受碳酸盐类矿物沉淀作用的影响。 Water samples collected along the Changjiang River estuary in June 2005 were studied for their dissolved inorganic carbon (DIC) contents and their isotopic composition. We found that CO2 super-saturation significantly occurred in the riverine zone and decreased sharply in the coastal zone. The δ13CDIC values are within the range of -10.0‰ and -0.9‰, and vary along the salinity gradient. The deviation of observed DIC concentrations and δ13 CDIC from the mixing equation between riverine and marine water indicates multiple processes controlling the carbon cycling in different zones. Degassing of CO2 mainly occurred in the riverine zone, photosynthesis in the estuary zone and carbonate mineral precipitation in the coastal zone.
出处 《地球与环境》 CAS CSCD 北大核心 2010年第4期409-413,共5页 Earth and Environment
基金 国家自然科学基金重点项目(90610037) 国家自然科学基金创新群体项目(40721002)
关键词 长江 河口 溶解无机碳 同位素 CO2 the Changjiang River estuary dissolved inorganic carbon isotope CO2
  • 相关文献

参考文献15

  • 1Meybeek M. Carbon, nitrogen and phosphorus transport by world rivers[J]. Am J Sci, 1982, 82(4): 401-450.
  • 2Degens E T, Kempe S, Richey J E. SCOPE 42 : Biogeochemistry of major world rivers[M]. Wiley, UK. 1991.
  • 3Ludwig W, Probst J L, Kempe S. Predicting the oceanic input of organic carbon by continental erosion[J].Global Biogeochemistry Cycle, 1996, 10 (1) : 23-41.
  • 4Meybeck M. Riverine transport of atmospheric carbon[J].Water, Air, & Soil Pollution, 1993, 70: 443-463.
  • 5高全洲,沈承德.河流碳通量与陆地侵蚀研究[J].地球科学进展,1998,13(4):369-375. 被引量:43
  • 6Zhai W, Dai M, Guo X. Carbonate system and CO2 degassing fluxes in the inner estuary of Changjiang(Yangtze) River, China[J]. Mar Chem, 2007, 107: 342-356.
  • 7高学鲁,宋金明,李学刚,李宁,袁华茂.长江口及杭州湾邻近海域夏季表层海水中的溶解无机碳[J].海洋科学,2008,32(4):61-67. 被引量:12
  • 8Weiss R F. Carbon dioxide in water and sea water: the solubility of a non-ideal gas[S]. Mar Chem, 1974, 2: 203-215.
  • 9Millero F J. Chemical Oceanography, 2nd edition[M]. CRC Press, Boca Raton, 1996.
  • 10Mucci A. The solubility of caIcite and aragonite in sea water at various salinities, temperatures,and one atmosphere total pressure[J]. Am J Sci, 1983, 283: 780-799.

二级参考文献35

  • 1刘子琳,宁修仁.杭州湾锋区浮游植物现存量和初级生产力[J].东海海洋,1994,12(4):58-66. 被引量:15
  • 2Zhang S,Mar Chem,1992年,38卷,53页
  • 3纪明侯(译),海洋有机化学,1992年,89页
  • 4Can W B,Transport of Carbon and Minerals in Major World Rievers.2,1983年
  • 5Lee K, Millero F J, Wanninkhof R. The carbon dioxide system in the Atlantic Oeean[J]. Journal of Geophysical Research, 1997,102(C7) : 15 693-15 708.
  • 6Tipping E, Lofts S, Lawlor A. Modelling the chemical speciation of trace metals in the surface waters of the Humber system[J]. The Science of the Total Environment, 1998,210/211 : 63-77.
  • 7Abril G, Frankignoulle M. Nitrogen-alkalinity interaction in the highly polluted Scheldt basin (Belgium) [J]. Water Research, 2001,35: 844-850.
  • 8Mook W G, Koene B K S. Chemistry of dissolved inorganic carbon in estuarine and coastal brackish waters [J]. Estuarine Coastal Marine Science, 1975,3. 325- 336.
  • 9Meybeck M. Riverine transport of atmospheric carbon: sources, global typology and budget[J]. Water Air and Soil Pollution, 1993,70 : 443-463.
  • 10Amiotte Suchet P, Probst J L. A global model for present-day atmospheric/soil CO2 consumption by chemical erosion of continental rocks (GEM-CO2) [J]. Tellus, 1995,47B(2) : 273-280.

共引文献53

同被引文献114

引证文献6

二级引证文献58

相关作者

内容加载中请稍等...

相关机构

内容加载中请稍等...

相关主题

内容加载中请稍等...

浏览历史

内容加载中请稍等...
;
使用帮助 返回顶部