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Low-Temperature Plasma-Catalytic Reduction of NO_x by C_2H_2 in the Presence of Excess Oxygen 被引量:1

Low-Temperature Plasma-Catalytic Reduction of NO_x by C_2H_2 in the Presence of Excess Oxygen
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摘要 Synergistic effects of pulsed DC dielectric barrier discharge (DBD) plasma and Indium modified HZSM-5 (In/HZSM-5) catalyst for C2H2 selective reduction of NOx at 200℃, in the presence of enriched oxygen by using a one-stage plasma-over-catalyst (POC) reactor, are reported. With a reactant gas mixture of 480 ppm NO, 500 ppm C2H2, 13.0% O2 in N2 and gas hourly space velocity (GHSV) = 10000 h^-1, pure catalytic, pure plasma-induced (discharges over fused silica pellets) and plasma-catalytic NOx conversion percentages are 45.0%, 4.0% and 92.2%, respectively. NOx conversion rates and energy costs were also compared for pulsed DC DBD and AC DBD reactors. Synergistic effects of pulsed DC dielectric barrier discharge (DBD) plasma and Indium modified HZSM-5 (In/HZSM-5) catalyst for C2H2 selective reduction of NOx at 200℃, in the presence of enriched oxygen by using a one-stage plasma-over-catalyst (POC) reactor, are reported. With a reactant gas mixture of 480 ppm NO, 500 ppm C2H2, 13.0% O2 in N2 and gas hourly space velocity (GHSV) = 10000 h^-1, pure catalytic, pure plasma-induced (discharges over fused silica pellets) and plasma-catalytic NOx conversion percentages are 45.0%, 4.0% and 92.2%, respectively. NOx conversion rates and energy costs were also compared for pulsed DC DBD and AC DBD reactors.
出处 《Plasma Science and Technology》 SCIE EI CAS CSCD 2008年第4期466-470,共5页 等离子体科学和技术(英文版)
基金 National Natural Science Foundation of China(No.20077005) Natural Science Foundation of Dalian Nationalities University of China(No.20076205)
关键词 pulsed DC DBD AC DBD plasma-catalytic reduction synergistic effect In/HZSM-5 catalyst pulsed DC DBD, AC DBD, plasma-catalytic reduction, synergistic effect In/HZSM-5 catalyst
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