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Ultrasonic Study on Charge Ordering in Nd0.5Ca0.5Mn1-xAlxO3(x=0,0.03)

Ultrasonic Study on Charge Ordering in Nd_(0.5)Ca_(0.5)Mn_(1-x)Al_xO_3(x=0,0.03)
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摘要 The ultrasonic, magnetic and transport properties of Nd0.5Ca0.5Mn1-xAlxO3 (x=0, 0.03) were studied from 15 to 300 K. The temperature dependencies of resistivity and magnetization show that Nd0.5Ca0.5MnO3 undergoes a charge ordering transition at TCO-257 K. An obvious softening of the longitudinal sound velocity above TCO and a dramatic stiffening below Too accompanied by an attenuation peak were observed. These features imply a strong electron phonom interaction via the Jahn-Teller effect iu the sample, Another broad attenuation peak was observed at around Tp-80 K. This anomaly is attributed to the phase separtion between the antiferromagnetic (AFM) and paramagnetic (PM) phases and gives a direct evidence for spin-phonon coupling in the compound. For the x=0.03 sample, both the minimum of sound velocity and attenuation peaks shift to a lower temperature. The results indicate that the charge ordering and CE-type AFM state in Nd0.5Ca0.5MnO3 are both partially suppressed by replacing Mn with A1.
出处 《Chinese Journal of Chemical Physics》 SCIE CAS CSCD 北大核心 2006年第6期535-538,共4页 化学物理学报(英文)
基金 supported by the National Natural Science Foundation of China(No.10274075) the Specialized Research Fund for the Doctoral Program of Higher Education(No.20030358056).
关键词 MANGANITE Charge ordering Phase separation Ultrasonic velocity and attenuation 锰氧化物 电荷有序 相分离 超声声速与衰减
分类号 O [理学]
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