Synergistic carbon emission reduction at the urban scale is an inherent requirement for China to realize its carbon emission reduction commitments and promote sustainable and regional synergistic development.Using 16 ...Synergistic carbon emission reduction at the urban scale is an inherent requirement for China to realize its carbon emission reduction commitments and promote sustainable and regional synergistic development.Using 16 prefectural cities in Shandong Province as an example,this study defines and quantifies the regional carbon emission reduction capacity(CERC)based on the synergistic development of carbon emission reduction,environmental protection,and economic growth objectives.The spatial network characteristics of the(CERC)and its drivers were analyzed using social network analysis and quadratic assignment procedure regression methods.The results revealed that the spatial correlation of the CERC among prefectural cities has been increasing over the years.Jinan−Zibo−Qingdao is the center of the network,while the spatial linkage strength in the southwest and northeast of Shandong Province is weak.Geospatial distance and scientific development differences have a significant negative effect on the intensity of spatial association,while differences in economic and informatization developments have a considerable positive impact.Environmental regulatory differences and transportation differences are not significant.This study offers a methodological reference for similar studies in other countries or regions.At the same time,the findings provide a scientific basis for the government to rationally allocate urban resources and promote regional synergistic carbon emission reduction.展开更多
Conductive inks based on graphene materials have received significant attention for the fabrication of a wide range of printed and flexible devices.However,the application of graphene fillers is limited by their restr...Conductive inks based on graphene materials have received significant attention for the fabrication of a wide range of printed and flexible devices.However,the application of graphene fillers is limited by their restricted mass production and the low concentration of their suspensions.In this study,a highly concentrated and conductive ink based on defect-free graphene was developed by a scalable fluid dynamics process.A high shear exfoliation and mixing process enabled the production of graphene at a high concentration of 47.5 mg mL^(−1)for graphene ink.The screen-printed graphene conductor exhibits a high electrical conductivity of 1.49×10^(4)S m^(−1)and maintains high conductivity under mechanical bending,compressing,and fatigue tests.Based on the as-prepared graphene ink,a printed electrochemical sodium ion(Na^(+))sensor that shows high potentiometric sensing performance was fabricated.Further,by integrating a wireless electronic module,a prototype Na^(+)-sensing watch is demonstrated for the real-time monitoring of the sodium ion concentration in human sweat during the indoor exercise of a volunteer.The scalable and efficient procedure for the preparation of graphene ink presented in this work is very promising for the low-cost,reproducible,and large-scale printing of flexible and wearable electronic devices.展开更多
One-dimensional alkali metal titanates containing potassium,sodium,and lithium are of great concern owing to their high ion mobility and high specific surface area.When those titanates are combined with conductive mat...One-dimensional alkali metal titanates containing potassium,sodium,and lithium are of great concern owing to their high ion mobility and high specific surface area.When those titanates are combined with conductive materials such as graphene,carbon nanotube,and carbon nanofiber,they are able to be employed as efficient electrode materials for supercapacitors.Potassium hexa-titanate(K2Ti6O13,KTO),in particular,has shown superior electrochemical properties compared to other alkali metal titanates because of their large lattice parameters induced by the large radius of potassium ions.Here,we present porous rGO crumples(PGC)decorated with KTO nanoparticles(NPs)for application to supercapacitors.The KTO NP/PGC composites were synthesized by aerosol spray pyrolysis and post-heat treatment.KTO NPs less than 10 nm in diameter were loaded onto PGCs ranging from 3 to 5μm.Enhanced porous structure of the composites was obtained by the activation of rGO by adding an excessive amount of KOH to the composites.The KTO NP/PGC composite electrodes fabricated at the GO/KOH/TiO2 ratio of 1:3:0.25 showed the highest performance(275 F g−1)in capacitance with different KOH concentrations and cycling stability(83%)after 2000 cycles at a current density of 1 A g−1.展开更多
It is urgent to significantly reduce greenhouse gas emissions to actively deal with global warming.This paper investigates Shandong Province,a typical province of energy consumption,as the research object,aiming to op...It is urgent to significantly reduce greenhouse gas emissions to actively deal with global warming.This paper investigates Shandong Province,a typical province of energy consumption,as the research object,aiming to optimize total energy consumption and consumption structure in the future planning year.This paper constructs a methodological system to optimize energy consumption structure in Shandong Province,using a scenario combination of system dynamics(SD)prediction and analysis based on the coupling of key scenario elements affecting different energy consumption from different perspectives.Structural equation modeling and SD sensitivity analysis indicate an overlap between key factors restricting energy consumption.Pairing the key scenario factors can better reflect the internal mechanism of energy consumption development.Based on this,21 scenarios based on different combinations of the key elements are constructed.Through SD prediction and analysis,the most suitable scenario mode for optimizing energy consumption structure in Shandong Province is selected.This paper provides a suitable development range for the average gross domestic product growth rate,the proportion of secondary industry,energy consumption intensity of secondary industry,and the urbanization rate for Shandong Province.This paper can provide a reference for similar research and the government in formulating the optimization scheme of energy consumption structure.展开更多
Construction and demolition(C&D)waste has seriously affected the ecological environment.The utilization of C&D waste resources can greatly alleviate this problem,and it is an important way to help achieve the ...Construction and demolition(C&D)waste has seriously affected the ecological environment.The utilization of C&D waste resources can greatly alleviate this problem,and it is an important way to help achieve the goal of zero carbon in 2050.In this study,insulation concrete blocks were developed with recycled aggregates,cement,fly ash as main raw materials,expanded polystyrene(EPS)insulation boards as block insulation filling material,and selfdeveloped construction waste composite activator,interface enhancer,surface modifier and other additives.Through experimental research and performance test analysis,the best mix ratio of the product and the mechanism of each additive were proved.The experimental results showed that the insulation concrete block prepared under the conditions of recycled aggregates sand ratio of 45%,active activator Na_(2)SO_(4)content of 0.15%and fly ash content of 30%has the best performance and meets the relevant standards.展开更多
Although the tobacco industry is a significant contributor to energy consumption and carbon emissions its negative environmental impact has received inadequate attention globally.Cigarette factories are a key link in ...Although the tobacco industry is a significant contributor to energy consumption and carbon emissions its negative environmental impact has received inadequate attention globally.Cigarette factories are a key link in the tobacco industry’s production chain,and using data provided by a cigarette factory in China we conduct a life cycle assessment to account for the carbon footprint of cigar production in cigarette factories.The results of the assessment show that factory air conditioning is the most important contributor to the environmental load of the cigar manufacturing process,while electricity is the key factor that contributes the greatest envi‐ronmental load across all of the processes in the product life cycle.In addition,packaging,including small boxes and cigarette cartons,has a significant impact on the industry’s environmental footprint due to its use of raw materials.We find the carbon footprint of the entire production process for cigar products to be 383.59 kg CO_(2) eq.Based on our findings,we suggest ways to optimize cigar/cigarette factory processes to re‐duce carbon emissions that can help to promote sustainable development in related industries.展开更多
The rapid development of urbanization has led to a rapid increase in total energy consumption.The proportion of domestic energy consumption to total energy consumption has gradually increased and has become the major ...The rapid development of urbanization has led to a rapid increase in total energy consumption.The proportion of domestic energy consumption to total energy consumption has gradually increased and has become the major driving force for energy consumption.With the pressure from urbanization and domestic energy consumption,it is necessary to study the impact of urbanization on domestic energy consumption of the regional level and to explore the function paths of these two factors.The findings are helpful to realize sustainable development based on the actual situation analysis,horizontal survey data and statistical yearbook panel data.The current situation and changing trends in domestic energy consumption of Shandong Province are systematically examined through field investigation and survey questionnaire.The time-series econometric model is applied to analyze the relationship between urbanization rate and total domestic energy consumption.The research results show that the total domestic energy consumption and urbanization rate of Shandong are generally increasing.The urbanization rate development and domestic energy consumption have a long-term stable and balanced relationship.An increase in urbanization rate can cause an increase in domestic energy consumption.There is a slight difference between the average total energy consumption levels of urban and rural residents,but their energy consumption structures differ a lot.These findings provide basic data support and reference for local governments to formulate energy-conservation and emission-reduction policies.展开更多
基金supported by the Department of Science and Technology of Shandong Province [Grant No.2021SFGC0904-05]Shandong Natural Science Foundation [Grant No.ZR2023MD079]+3 种基金Shandong Province Social Science Planning Research Project [Grant No.22CKRJ04]Taishan Scholar Project [Grant No.tsqn202103010]Zaozhuang Science and Technology Bureau [Grant No.2021GH22]the Key R&D Program of Shandong Province,China [Grant No.2023SFGC0101].
文摘Synergistic carbon emission reduction at the urban scale is an inherent requirement for China to realize its carbon emission reduction commitments and promote sustainable and regional synergistic development.Using 16 prefectural cities in Shandong Province as an example,this study defines and quantifies the regional carbon emission reduction capacity(CERC)based on the synergistic development of carbon emission reduction,environmental protection,and economic growth objectives.The spatial network characteristics of the(CERC)and its drivers were analyzed using social network analysis and quadratic assignment procedure regression methods.The results revealed that the spatial correlation of the CERC among prefectural cities has been increasing over the years.Jinan−Zibo−Qingdao is the center of the network,while the spatial linkage strength in the southwest and northeast of Shandong Province is weak.Geospatial distance and scientific development differences have a significant negative effect on the intensity of spatial association,while differences in economic and informatization developments have a considerable positive impact.Environmental regulatory differences and transportation differences are not significant.This study offers a methodological reference for similar studies in other countries or regions.At the same time,the findings provide a scientific basis for the government to rationally allocate urban resources and promote regional synergistic carbon emission reduction.
基金the National Research Foundation of Korea(NRF)Grant funded by the Ministry of Science and ICT(No.2021R1A2C1009926)“Basic project(referring to projects performed with the budget directly contributed by the Government to achieve the purposes of establishment of Government-funded research Institutes)”+3 种基金supported by the KOREA RESEARCH INSTITUTE of CHEMICAL TECHNOLOGY(KRICT)(SS2042-10)Basic research project(Project:21-3212-1)of the Korea institute of GeoscienceMineral resources funded by the Ministry of Science and ICT of Koreaby Nanomedical Devices Development Project of NNFC in 2021.
文摘Conductive inks based on graphene materials have received significant attention for the fabrication of a wide range of printed and flexible devices.However,the application of graphene fillers is limited by their restricted mass production and the low concentration of their suspensions.In this study,a highly concentrated and conductive ink based on defect-free graphene was developed by a scalable fluid dynamics process.A high shear exfoliation and mixing process enabled the production of graphene at a high concentration of 47.5 mg mL^(−1)for graphene ink.The screen-printed graphene conductor exhibits a high electrical conductivity of 1.49×10^(4)S m^(−1)and maintains high conductivity under mechanical bending,compressing,and fatigue tests.Based on the as-prepared graphene ink,a printed electrochemical sodium ion(Na^(+))sensor that shows high potentiometric sensing performance was fabricated.Further,by integrating a wireless electronic module,a prototype Na^(+)-sensing watch is demonstrated for the real-time monitoring of the sodium ion concentration in human sweat during the indoor exercise of a volunteer.The scalable and efficient procedure for the preparation of graphene ink presented in this work is very promising for the low-cost,reproducible,and large-scale printing of flexible and wearable electronic devices.
基金supported as a Basic Research Project of the Korea Institute of Geoscience and Mineral Resources (KIGAM)funded by the Ministry of Science and ICT
文摘One-dimensional alkali metal titanates containing potassium,sodium,and lithium are of great concern owing to their high ion mobility and high specific surface area.When those titanates are combined with conductive materials such as graphene,carbon nanotube,and carbon nanofiber,they are able to be employed as efficient electrode materials for supercapacitors.Potassium hexa-titanate(K2Ti6O13,KTO),in particular,has shown superior electrochemical properties compared to other alkali metal titanates because of their large lattice parameters induced by the large radius of potassium ions.Here,we present porous rGO crumples(PGC)decorated with KTO nanoparticles(NPs)for application to supercapacitors.The KTO NP/PGC composites were synthesized by aerosol spray pyrolysis and post-heat treatment.KTO NPs less than 10 nm in diameter were loaded onto PGCs ranging from 3 to 5μm.Enhanced porous structure of the composites was obtained by the activation of rGO by adding an excessive amount of KOH to the composites.The KTO NP/PGC composite electrodes fabricated at the GO/KOH/TiO2 ratio of 1:3:0.25 showed the highest performance(275 F g−1)in capacitance with different KOH concentrations and cycling stability(83%)after 2000 cycles at a current density of 1 A g−1.
文摘It is urgent to significantly reduce greenhouse gas emissions to actively deal with global warming.This paper investigates Shandong Province,a typical province of energy consumption,as the research object,aiming to optimize total energy consumption and consumption structure in the future planning year.This paper constructs a methodological system to optimize energy consumption structure in Shandong Province,using a scenario combination of system dynamics(SD)prediction and analysis based on the coupling of key scenario elements affecting different energy consumption from different perspectives.Structural equation modeling and SD sensitivity analysis indicate an overlap between key factors restricting energy consumption.Pairing the key scenario factors can better reflect the internal mechanism of energy consumption development.Based on this,21 scenarios based on different combinations of the key elements are constructed.Through SD prediction and analysis,the most suitable scenario mode for optimizing energy consumption structure in Shandong Province is selected.This paper provides a suitable development range for the average gross domestic product growth rate,the proportion of secondary industry,energy consumption intensity of secondary industry,and the urbanization rate for Shandong Province.This paper can provide a reference for similar research and the government in formulating the optimization scheme of energy consumption structure.
基金This work was supported by Science and technology project of housing and urban-rural Development Department of Shandong Province(2018)and Shandong Provincial Social Science Planning Research Project(20CGLJ13).
文摘Construction and demolition(C&D)waste has seriously affected the ecological environment.The utilization of C&D waste resources can greatly alleviate this problem,and it is an important way to help achieve the goal of zero carbon in 2050.In this study,insulation concrete blocks were developed with recycled aggregates,cement,fly ash as main raw materials,expanded polystyrene(EPS)insulation boards as block insulation filling material,and selfdeveloped construction waste composite activator,interface enhancer,surface modifier and other additives.Through experimental research and performance test analysis,the best mix ratio of the product and the mechanism of each additive were proved.The experimental results showed that the insulation concrete block prepared under the conditions of recycled aggregates sand ratio of 45%,active activator Na_(2)SO_(4)content of 0.15%and fly ash content of 30%has the best performance and meets the relevant standards.
基金supported by Shandong Natural Science Founda‐tion[Grant No.ZR2023MD079]Shandong Province Social Science Planning Research Project[Grant No.22CKRJ04]+2 种基金Taishan Scholar Project[Grant No.tsqn202103010]Department of Science and Tech‐nology of Shandong Province[Grant No.2021SFGC0904-05]Zaozhuang Science and Technology Bureau[Grant No.2021GH22].
文摘Although the tobacco industry is a significant contributor to energy consumption and carbon emissions its negative environmental impact has received inadequate attention globally.Cigarette factories are a key link in the tobacco industry’s production chain,and using data provided by a cigarette factory in China we conduct a life cycle assessment to account for the carbon footprint of cigar production in cigarette factories.The results of the assessment show that factory air conditioning is the most important contributor to the environmental load of the cigar manufacturing process,while electricity is the key factor that contributes the greatest envi‐ronmental load across all of the processes in the product life cycle.In addition,packaging,including small boxes and cigarette cartons,has a significant impact on the industry’s environmental footprint due to its use of raw materials.We find the carbon footprint of the entire production process for cigar products to be 383.59 kg CO_(2) eq.Based on our findings,we suggest ways to optimize cigar/cigarette factory processes to re‐duce carbon emissions that can help to promote sustainable development in related industries.
基金funded by Natural Science Foundation of China(71974116)Shandong Natural Science Foundation(2019MG009)Shandong Provincial Social Science Planning Research Project(20CGLJ13).
文摘The rapid development of urbanization has led to a rapid increase in total energy consumption.The proportion of domestic energy consumption to total energy consumption has gradually increased and has become the major driving force for energy consumption.With the pressure from urbanization and domestic energy consumption,it is necessary to study the impact of urbanization on domestic energy consumption of the regional level and to explore the function paths of these two factors.The findings are helpful to realize sustainable development based on the actual situation analysis,horizontal survey data and statistical yearbook panel data.The current situation and changing trends in domestic energy consumption of Shandong Province are systematically examined through field investigation and survey questionnaire.The time-series econometric model is applied to analyze the relationship between urbanization rate and total domestic energy consumption.The research results show that the total domestic energy consumption and urbanization rate of Shandong are generally increasing.The urbanization rate development and domestic energy consumption have a long-term stable and balanced relationship.An increase in urbanization rate can cause an increase in domestic energy consumption.There is a slight difference between the average total energy consumption levels of urban and rural residents,but their energy consumption structures differ a lot.These findings provide basic data support and reference for local governments to formulate energy-conservation and emission-reduction policies.
