Plasmon induced hot electrons have attracted a great deal of interest as a novel route for photodetection and lightenergy harvesting. Herein, we report a hot electron photodetector in which a large array of nanocones ...Plasmon induced hot electrons have attracted a great deal of interest as a novel route for photodetection and lightenergy harvesting. Herein, we report a hot electron photodetector in which a large array of nanocones deposited sequentially with aluminum, titanium dioxide, and gold films can be integrated functionally with nanophotonics and microelectronics. The device exhibits a strong photoelectric response at around 620 nm with a responsivity of 180 μA/W under short-circuit conditions with a significant increase under 1 V reverse bias to 360 μA/W. The increase in responsivity and a red shift in the peak value with increasing bias voltage indicate that the bias causes an increase in the hot electron tunneling effect. Our approach will be advantageous for the implementation of the proposed architecture on a vast variety of integrated optoelectronic devices.展开更多
A polarization-insensitive plasmonic absorber is designed consisting of Au fishnet structures on a TiO2 spacer/Ag mirror. The fishnet structures excite localized surface plasmon and generate hot electrons from the abs...A polarization-insensitive plasmonic absorber is designed consisting of Au fishnet structures on a TiO2 spacer/Ag mirror. The fishnet structures excite localized surface plasmon and generate hot electrons from the absorbed photons, while the TiO2 layer induces Fabry–Perot resonance, and the Ag mirror acts as a back reflector.Through optimizing the TiO2 layer thickness, numerical simulation shows that 97% of the incident light is absorbed in the Au layer. The maximum responsivity and external quantum efficiency of the device can approach 5 mA/W and ~1%, respectively, at the wavelength of 700 nm.展开更多
Transparent conductive oxides exhibit attractive optical nonlinearity with ultrafast response and giant refractive index change near the epsilon-near-zero(ENZ) wavelength, originating from the intraband dynamics of co...Transparent conductive oxides exhibit attractive optical nonlinearity with ultrafast response and giant refractive index change near the epsilon-near-zero(ENZ) wavelength, originating from the intraband dynamics of conduction electrons. The optical nonlinearity of ENZ materials has been explained by using the overall-effective-mass and the overall-scattering-time of electrons in the extended Drude model. However, their response to optical excitation is yet the last building block to complete the theory. In this paper, the concept of thermal energy is theoretically proposed to account for the total energy of conduction electrons exceeding their thermal equilibrium value. The time-varying thermal energy is adopted to describe the transient optical response of indium-tin-oxide(ITO), a typical ENZ material. A spectrally-resolved femtosecond pump-probe experiment was conducted to verify our theory. By correlating the thermal energy with the pumping density, both the giant change and the transient response of the permittivity of ITO can be predicted. The results in this work provide a new methodology to describe the transient permittivities of ENZ materials, which will benefit the design of ENZ-based nonlinear photonic devices.展开更多
基金National Natural Science Foundation of China(NSFC)(61675171,61675169,61522507)Fundamental Research Funds for the Central Universities of China(3102017HQZZ022,3102017zy021)Shaanxi Provincical Key R&D Program(2018KW-009)
文摘Plasmon induced hot electrons have attracted a great deal of interest as a novel route for photodetection and lightenergy harvesting. Herein, we report a hot electron photodetector in which a large array of nanocones deposited sequentially with aluminum, titanium dioxide, and gold films can be integrated functionally with nanophotonics and microelectronics. The device exhibits a strong photoelectric response at around 620 nm with a responsivity of 180 μA/W under short-circuit conditions with a significant increase under 1 V reverse bias to 360 μA/W. The increase in responsivity and a red shift in the peak value with increasing bias voltage indicate that the bias causes an increase in the hot electron tunneling effect. Our approach will be advantageous for the implementation of the proposed architecture on a vast variety of integrated optoelectronic devices.
基金the National Natural Science Foundation of China (NSFC)(Nos. 91950207,61675171,and 61675169)Fundamental Research Funds for the Central Universities of China (Nos. 3102017-HQZZ022 and 3102017zy021)。
文摘A polarization-insensitive plasmonic absorber is designed consisting of Au fishnet structures on a TiO2 spacer/Ag mirror. The fishnet structures excite localized surface plasmon and generate hot electrons from the absorbed photons, while the TiO2 layer induces Fabry–Perot resonance, and the Ag mirror acts as a back reflector.Through optimizing the TiO2 layer thickness, numerical simulation shows that 97% of the incident light is absorbed in the Au layer. The maximum responsivity and external quantum efficiency of the device can approach 5 mA/W and ~1%, respectively, at the wavelength of 700 nm.
基金supported by the National Natural Science Foundation of China(Grant Nos.91950207,12174310,61805157,and 11974282)。
文摘Transparent conductive oxides exhibit attractive optical nonlinearity with ultrafast response and giant refractive index change near the epsilon-near-zero(ENZ) wavelength, originating from the intraband dynamics of conduction electrons. The optical nonlinearity of ENZ materials has been explained by using the overall-effective-mass and the overall-scattering-time of electrons in the extended Drude model. However, their response to optical excitation is yet the last building block to complete the theory. In this paper, the concept of thermal energy is theoretically proposed to account for the total energy of conduction electrons exceeding their thermal equilibrium value. The time-varying thermal energy is adopted to describe the transient optical response of indium-tin-oxide(ITO), a typical ENZ material. A spectrally-resolved femtosecond pump-probe experiment was conducted to verify our theory. By correlating the thermal energy with the pumping density, both the giant change and the transient response of the permittivity of ITO can be predicted. The results in this work provide a new methodology to describe the transient permittivities of ENZ materials, which will benefit the design of ENZ-based nonlinear photonic devices.
