Ambient PM2.5 samples were collected at four sites in Xiamen, including Gulangyu （GLY）. Hongwen （HW）, Huli （HL） and Jimei （JM） during January, April, July and October 2013. Local source samples were obtained f...Ambient PM2.5 samples were collected at four sites in Xiamen, including Gulangyu （GLY）. Hongwen （HW）, Huli （HL） and Jimei （JM） during January, April, July and October 2013. Local source samples were obtained from coal burning power plants, industries, motor vehicles, biomass burning, fugitive dust, and sea salt for the source apportionment studies. The highest value of PM2.5 mass concentration and species related to human activities （SO42- , NO3 , Pb, Ni, V, Cu, Cd, organic carbon （OC） andelemental carbon （EC）） were found in the ambient-samples from HL, and t-he highest and lowest loadings of PM2.5 and its components occurred in winter and summer, respectively. The reconstructed mass balance indicated that ambient PM2.5 consisted of 24% OM （organic matter）, 23% sulfate, 14% nitrate, 9% ammonium, 9% geological material, 6% sea salt, 5% EC and 10% others. For the source profiles, the dominant components were OC for coal burning, motor vehicle, biomass burning and sea salt; SO42 for industry; and crustal elements for fugitive dust. Source contributions were calculatedusing a chemical mass＇balance （CMB） model basedon ambient PM2.5 concentrations and the source profiles. GLY was characterized by high contributions from secondary sulfate and cooking, while HL and JM were most strongly affected by motor vehicle emissions, and biomass burning and fugitivedust, respectively. The CMB results-indicated that PM2.5 from Xiamen is composed of 27.4% secondary inorganic components, 20.8% motor vehicle emissions, 11.7% fugitive dust, 9.9% sea salt, 9.3% coal burning, 5.0% biomass burning, 3.1% industry and 6.8% others.展开更多
基金This work was supported by the Xiamen Environ- mental Protection Special Project （No. 19 （10）, 2013）, Science and Technology Project of Fujian Provincial Environmental Protection Depart- ment （2014）, and also supported by a project from Ministry of Science and Technology （2013FY 112700） and the Natural Science Foundation of China （Grant No. 41673125）.
文摘Ambient PM2.5 samples were collected at four sites in Xiamen, including Gulangyu （GLY）. Hongwen （HW）, Huli （HL） and Jimei （JM） during January, April, July and October 2013. Local source samples were obtained from coal burning power plants, industries, motor vehicles, biomass burning, fugitive dust, and sea salt for the source apportionment studies. The highest value of PM2.5 mass concentration and species related to human activities （SO42- , NO3 , Pb, Ni, V, Cu, Cd, organic carbon （OC） andelemental carbon （EC）） were found in the ambient-samples from HL, and t-he highest and lowest loadings of PM2.5 and its components occurred in winter and summer, respectively. The reconstructed mass balance indicated that ambient PM2.5 consisted of 24% OM （organic matter）, 23% sulfate, 14% nitrate, 9% ammonium, 9% geological material, 6% sea salt, 5% EC and 10% others. For the source profiles, the dominant components were OC for coal burning, motor vehicle, biomass burning and sea salt; SO42 for industry; and crustal elements for fugitive dust. Source contributions were calculatedusing a chemical mass＇balance （CMB） model basedon ambient PM2.5 concentrations and the source profiles. GLY was characterized by high contributions from secondary sulfate and cooking, while HL and JM were most strongly affected by motor vehicle emissions, and biomass burning and fugitivedust, respectively. The CMB results-indicated that PM2.5 from Xiamen is composed of 27.4% secondary inorganic components, 20.8% motor vehicle emissions, 11.7% fugitive dust, 9.9% sea salt, 9.3% coal burning, 5.0% biomass burning, 3.1% industry and 6.8% others.
