The incidence of large bone defects caused by traumatic injury is increasing worldwide,and the tissue regeneration process requires a long recovery time due to limited self-healing capability.Endogenous bioelectrical ...The incidence of large bone defects caused by traumatic injury is increasing worldwide,and the tissue regeneration process requires a long recovery time due to limited self-healing capability.Endogenous bioelectrical phenomena have been well recognized as critical biophysical factors in bone remodeling and regeneration.Inspired by bioelectricity,electrical stimulation has been widely considered an external intervention to induce the osteogenic lineage of cells and enhance the synthesis of the extracellular matrix,thereby accelerating bone regeneration.With ongoing advances in biomaterials and energy-harvesting techniques,electroactive biomaterials and self-powered systems have been considered biomimetic approaches to ensure functional recovery by recapitulating the natural electrophysiological microenvironment of healthy bone tissue.In this review,we first introduce the role of bioelectricity and the endogenous electric field in bone tissue and summarize different techniques to electrically stimulate cells and tissue.Next,we highlight the latest progress in exploring electroactive hybrid biomaterials as well as self-powered systems such as triboelectric and piezoelectric-based nanogenerators and photovoltaic cell-based devices and their implementation in bone tissue engineering.Finally,we emphasize the significance of simulating the target tissue’s electrophysiological microenvironment and propose the opportunities and challenges faced by electroactive hybrid biomaterials and self-powered bioelectronics for bone repair strategies.展开更多
Finely tuning spectral characteristics of the epsilon-negative(ε'<0,EN) response is full of challenges when its regulatory mechanism in metacomposites is not yet clear.Herein,we have meticulously designed Cu/C...Finely tuning spectral characteristics of the epsilon-negative(ε'<0,EN) response is full of challenges when its regulatory mechanism in metacomposites is not yet clear.Herein,we have meticulously designed Cu/CaCu_(3)Ti_(4)O_(12)(Cu/CCTO) percolative metacomposites,successfully achieved both epsilon-negative and ε'-near-zero(ENZ)responses in the radio-frequency band.Before percolation,a large number of electric dipoles in the metacomposites achieved resonance characteristics near the ENZ point under the excitation of radio frequency electromagnetic fields,and as the Cu content increased,the ENZ frequency varied from 942,858,862 to 632 MHz.展开更多
The total nitrogen(TN)is a major factor contributing to eutrophication and is a crucial parameter in assessing surface water quality.Accurate and rapid methods are crucial for determining the TN content in water.Herei...The total nitrogen(TN)is a major factor contributing to eutrophication and is a crucial parameter in assessing surface water quality.Accurate and rapid methods are crucial for determining the TN content in water.Herein,a fast,highly sensitive,and pollution-free approach is proposed,which combines ultraviolet(UV)absorption spectroscopy with Bayesian optimized least squares support vector machine(LSSVM)for detecting TN content in water.Water samples collected from sampling points near the Yangtze River basin in Chongqing of China were analyzed using national standard methods to measure TN content as reference values.The prediction of TN content in water was achieved by integrating the UV absorption spectra of water samples with LSSVM.To make the model quickly and accurately select the optimal parameters to improve the accuracy of the prediction model,the Bayesian optimization(BO)algorithm was used to optimize the parameters of the LSSVM.Results show that the prediction model performs well in predicting TN concentration,with a high coefficient of prediction determination(R^(2)=0.9413)and a low root mean square error of prediction(RMSE=0.0779 mg/L).Comparative analysis with previous studies indicates that the model used in this paper achieves lower prediction errors and superior predictive performance.展开更多
The design and development of high-performance anodes pose significant challenges in the construction of next-generation rechargeable lithium-ion batteries(LIBs).Sodium molybdate dihydrate(Na_(2)MoO_(4)·2H_(2)O)h...The design and development of high-performance anodes pose significant challenges in the construction of next-generation rechargeable lithium-ion batteries(LIBs).Sodium molybdate dihydrate(Na_(2)MoO_(4)·2H_(2)O)has garnered increasing attention due to its cost-effectiveness,non-toxicity and earth abundance.To enhance the Li storage performance of Na_(2)MoO_(4)·2H_(2)O,a crystallographic orientation regulation strategy is proposed in this work.Initially,density functional theory calculations are carried out to demonstrate that the(020)crystal plane of Na_(2)MoO_(4)·2H_(2)O offers the lowest energy barrier for Li^(+)migration.Subsequently,the preferred crystallographic orientation of Na_(2)MoO_(4)·2H_(2)O crystal is tuned through a low-temperature recrystallization method.Furthermore,the microstructure and phase changes of Na_(2)MoO_(4)·2H_(2)O during the lithiation/de-lithiation process are studied using in situ and ex situ XRD tests,ex situ XPS and cyclic voltammetry to unravel its Li^(+)storage mechanism.Upon application as LIBs anode,the Na_(2)MoO_(4)·2H_(2)O single-crystal particles with a preferred(020)surface exhibit superior reversible capacity,high-capacity retention and high cycling stability.The enhanced Li storage performance should be attributed to the regulated crystallographic orientation and small changes in the crystal microstructure during the charge/discharge process,which facilitates Li^(+)migration and bolsters structural stability.Notably,this study introduces a novel concept and a simple synthesis method for the advancement of electrodes in rechargeable batteries.展开更多
Controlling the construction of physical colors on the surfaces of transparent dielectric crystals is crucial for surface coloration and anti-counterfeiting applications.In this study,we present a novel approach to cr...Controlling the construction of physical colors on the surfaces of transparent dielectric crystals is crucial for surface coloration and anti-counterfeiting applications.In this study,we present a novel approach to creating stable physical colors on the surface of lithium niobate crystals by combining gold ion implantation with laser direct writing technologies.The interaction between the laser,the implanted gold nanoparticles,and the crystal lattice induces permanent,localized modifications on the crystal surface.By fine-tuning the laser direct writing parameters,we reshaped the gold nanoparticles into spheres of varying sizes on the crystal surface,resulting in the display of red,green,blue,and pale-yellow colors.We investigated the influence of the implanted Au nanoparticles-particularly their localized surface plasmon resonances-on the modifications of the lithium niobate crystal lattice during the laser writing process using confocal Raman spectroscopy and high-resolution transmission electron microscopy.Our findings reveal that the embedded Au nanoparticles play a pivotal role in altering the conventional light-matter interaction between the crystal lattice and the laser,thereby facilitating the generation of surface colors.This work opens new avenues for the development of vibrant surface colors on transparent dielectric crystals.展开更多
CaCu_(3)Ti_(4)O_(12)(CCTO)ceramic nanocomposites incorporating graphene–carbon black(GRCB)fillers were fabricated by spark plasma sintering process.The percolative effects of conductive GRCB fillers on dielectric res...CaCu_(3)Ti_(4)O_(12)(CCTO)ceramic nanocomposites incorporating graphene–carbon black(GRCB)fillers were fabricated by spark plasma sintering process.The percolative effects of conductive GRCB fillers on dielectric response of GRCB/CCTO ternary metacomposites were systematically investigated.The weakly real permittivity(ε′)-negative response(ε′~−1×10^(2))was achieved which originated from weakly low-frequency plasmonic state of free carriers within constructed GRCB networks.With enhancing three-dimensional GRCB network,the plasma frequency of metacomposites increased while the damping factor decreased.Herein,theε′-negative values of metacomposites were tuned from−10^(2) to−10^(4) orders of magnitude andε′-near-zero(ENZ)frequencies from~142 to~340 MHz which substantially benefited from the moderate carrier concentration of GRCB dual fillers.The Drude model and equivalent circuit models were adopted to demonstrate dielectric and electrical characteristics.The obtained metacomposites show strong EM shielding effect along with enhanced plasmonic oscillation and even better achieving perfect EM shielding effect in ENZ media.This work achieves the tunableε′-negative andε′-near-zero response and more importantly clarifies its regulation mechanism in ceramic-based ternary metacomposites,which opens up the possibility of designing high-performance EM shielding materials based on metacomposites.展开更多
Lithium-sulfur batteries(LSBs)have already developed into one of the most promising new-generation high-energy density electrochemical energy storage systems with outstanding features including high-energy density,low...Lithium-sulfur batteries(LSBs)have already developed into one of the most promising new-generation high-energy density electrochemical energy storage systems with outstanding features including high-energy density,low cost,and environmental friendliness.However,the development and commercialization path of LSBs still presents significant limitations and challenges,particularly the notorious shuttle effect triggered by soluble longchain lithium polysulfides(LiPSs),which inevitably leads to low utilization of cathode active sulfur and high battery capacity degradation,short cycle life,etc.Substantial research efforts have been conducted to develop various sulfur host materials capable of effectively restricting the shuttle effect.This review firstly introduces the fundamental electrochemical aspects of LSBs,followed by a comprehensive analysis of the mechanism underlying the shuttle effect in Li–S batteries and its profound influence on various battery components as well as the overall battery performance.Subsequently,recent advances and strategies are systematically reviewed,including physical confinement,chemisorption,and catalytic conversion of sulfur hosts for restricting LiPSs shuttle effects.The interplay mechanisms of sulfur hosts and LiPSs are discussed in detail and the structural advantages of different host materials are highlighted.Furthermore,key insights for the rational design of advanced host materials for LSBs are provided,and the upcoming challenges and the prospects for sulfur host materials in lithium-sulfur batteries are also explored.展开更多
In this paper,a liquid-solid origami composite design is proposed for the improvement of impact resistance.Employing this design strategy,Kresling origami composite structures with different fillings were designed and...In this paper,a liquid-solid origami composite design is proposed for the improvement of impact resistance.Employing this design strategy,Kresling origami composite structures with different fillings were designed and fabricated,namely air,water,and shear thickening fluid(STF).Quasi-static compression and drop-weight impact experiments were carried out to compare and reveal the static and dynamic mechanical behavior of these structures.The results from drop-weight impact experiments demonstrated that the solid-liquid Kresling origami composite structures exhibited superior yield strength and reduced peak force when compared to their empty counterparts.Notably,the Kresling origami structures filled with STF exhibited significantly heightened yield strength and reduced peak force.For example,at an impact velocity of 3 m/s,the yield strength of single-layer STF-filled Kresling origami structures increased by 772.7%and the peak force decreased by 68.6%.This liquid-solid origami composite design holds the potential to advance the application of origami structures in critical areas such as aerospace,intelligent protection and other important fields.The demonstrated improvements in impact resistance underscore the practical viability of this approach in enhancing structural performance for a range of applications.展开更多
Permanent magnet synchronous motor based electro-mechanical actuation servo drives have widespread applications in the aviation field,such as unmanned aerial vehicle electric servos,electric cabin doors,and mechanical...Permanent magnet synchronous motor based electro-mechanical actuation servo drives have widespread applications in the aviation field,such as unmanned aerial vehicle electric servos,electric cabin doors,and mechanical arms.The performance of the servo drive,which encompasses the response to the torque,efficiency,control bandwidth and the steady-state positioning accuracy,significantly influences the performance of the aviation actuation.Consequently,enhancing the control bandwidth and refining the positioning accuracy of aviation electro-mechanical actuation servo drives have emerged as a focal point of research.This paper investigates the multi-source disturbances present in aviation electro-mechanical actuation servo systems and summarizes recent research on high-performance servo control methods based on active disturbance rejection control(ADRC).We present a comprehensive overview of the research status pertaining to servo control architecture,strategies for suppressing disturbances in the current loop,and ADRC-based strategies for the position loop.We delineate the research challenges and difficulties encountered by aviation electro-mechanical actuation servo drive control technology.展开更多
The combination of advanced photoelectric detectors has rendered single-band camouflage materials ineffective,necessitating the development of infrared multispectral camouflage.However,the design and fabrication of ex...The combination of advanced photoelectric detectors has rendered single-band camouflage materials ineffective,necessitating the development of infrared multispectral camouflage.However,the design and fabrication of existing works remain complex as they usually require the integration of multiscale structures.Here,we introduce phase modulation into the infrared camouflage metasurfaces with metal-dielectric-metal configuration,enabling them to achieve camouflage across more bands.Based on this strategy,a simple but effective single-layer cascaded metasurface is demonstrated for the first time to achieve low reflection at multi-wavelength lasers,low infrared radiation in atmospheric windows,and broadband thermal management.As a proof-of-concept,a 4-inch sample with a minimum linewidth of 1.8μm is fabricated using photolithography.The excellent infrared multispectral camouflage performance is verified in experiments,showing low reflectance in 0.9–1.6μm,low infrared emissivity in mid-wavelength infrared(MWIR)and long-wavelength infrared(LWIR)bands,and high absorptance at the wavelength of 10.6μm.Meanwhile,broadband high emissivity in 5–8μm can provide high-performance radiative heat dissipation.When the input power is 1.57 W·cm^(-2),the surface/radiation temperature of the metasurface decreases by 5.3℃/18.7℃ compared to the reference.The proposed metasurface may trigger further innovation in the design and application of compact multispectral optical devices.展开更多
As an essential field of multimedia and computer vision,3D shape recognition has attracted much research attention in recent years.Multiview-based approaches have demonstrated their superiority in generating effective...As an essential field of multimedia and computer vision,3D shape recognition has attracted much research attention in recent years.Multiview-based approaches have demonstrated their superiority in generating effective 3D shape representations.Typical methods usually extract the multiview global features and aggregate them together to generate 3D shape descriptors.However,there exist two disadvantages:First,the mainstream methods ignore the comprehensive exploration of local information in each view.Second,many approaches roughly aggregate multiview features by adding or concatenating them together.The information loss for some discriminative characteristics limits the representation effectiveness.To address these problems,a novel architecture named region-based joint attention network(RJAN)was proposed.Specifically,the authors first design a hierarchical local information exploration module for view descriptor extraction.The region-to-region and channel-to-channel relationships from different granularities can be comprehensively explored and utilised to provide more discriminative characteristics for view feature learning.Subsequently,a novel relation-aware view aggregation module is designed to aggregate the multiview features for shape descriptor generation,considering the view-to-view relationships.Extensive experiments were conducted on three public databases:ModelNet40,ModelNet10,and ShapeNetCore55.RJAN achieves state-of-the-art performance in the tasks of 3D shape classification and 3D shape retrieval,which demonstrates the effectiveness of RJAN.The code has been released on https://github.com/slurrpp/RJAN.展开更多
This study presents a breakthrough in flexible strain sensor technology with the development of an ultrahigh sensitivity and wide-range sensor,addressing the critical challenge of reconciling sensitivity with measurem...This study presents a breakthrough in flexible strain sensor technology with the development of an ultrahigh sensitivity and wide-range sensor,addressing the critical challenge of reconciling sensitivity with measurement range.Inspired by the structure of bamboo slips,we introduce a novel approach that utilises liquid metal to modulate the electrical pathways within a cracked platinum fabric electrode.The resulting sensor demonstrates a gauge factor greater than 108 and a strain measurement capability exceeding 100%.The integration of patterned liquid metal enables customisable tuning of the sensor’s response,while the porous fabric structure ensures superior comfort and air permeability for the wearer.Our design not only optimises the sensor’s performance but also enhances the electrical stability that is essential for practical applications.Through systematic investigation,we reveal the intrinsic mechanisms governing the sensor’s response,offering valuable insights for the design of wearable strain sensors.The sensor’s exceptional performance across a spectrum of applications,from micro-strain to large-strain detection,highlights its potential for a wide range of real-world uses,demonstrating a significant advancement in the field of flexible electronics.展开更多
Fourier Ptychographic Microscopy(FPM)is a high-throughput computational optical imaging technology reported in 2013.It effectively breaks through the trade-off between high-resolution imaging and wide-field imaging.In...Fourier Ptychographic Microscopy(FPM)is a high-throughput computational optical imaging technology reported in 2013.It effectively breaks through the trade-off between high-resolution imaging and wide-field imaging.In recent years,it has been found that FPM is not only a tool to break through the trade-off between field of view and spatial resolution,but also a paradigm to break through those trade-off problems,thus attracting extensive attention.Compared with previous reviews,this review does not introduce its concept,basic principles,optical system and series of applications once again,but focuses on elaborating the three major difficulties faced by FPM technology in the process from“looking good”in the laboratory to“working well”in practical applications:mismatch between numerical model and physical reality,long reconstruction time and high computing power demand,and lack of multi-modal expansion.It introduces how to achieve key technological innovations in FPM through the dual drive of Artificial Intelligence(AI)and physics,including intelligent reconstruction algorithms introducing machine learning concepts,optical-algorithm co-design,fusion of frequency domain extrapolation methods and generative adversarial networks,multi-modal imaging schemes and data fusion enhancement,etc.,gradually solving the difficulties of FPM technology.Conversely,this review deeply considers the unique value of FPM technology in potentially feeding back to the development of“AI+optics”,such as providing AI benchmark tests under physical constraints,inspirations for the balance of computing power and bandwidth in miniaturized intelligent microscopes,and photoelectric hybrid architectures.Finally,it introduces the industrialization path and frontier directions of FPM technology,pointing out that with the promotion of the dual drive of AI and physics,it will generate a large number of industrial application case,and looks forward to the possibilities of future application scenarios and expansions,for instance,body fluid biopsy and point-of-care testing at the grassroots level represent the expansion of the growth market.展开更多
1.Opportunities for electric motor drives in the low-altitude economy The implementation plan for the innovative application of general aviation equipment(2024–2030)outlines that by 2027,new general aviation equipmen...1.Opportunities for electric motor drives in the low-altitude economy The implementation plan for the innovative application of general aviation equipment(2024–2030)outlines that by 2027,new general aviation equipment will achieve commercial applications in urban air transport,logistics distribution and emergency rescue.展开更多
Cross-domain routing in Integrated Heterogeneous Networks(Inte-HetNet)should ensure efficient and secure data transmission across different network domains by satisfying diverse routing requirements.However,current so...Cross-domain routing in Integrated Heterogeneous Networks(Inte-HetNet)should ensure efficient and secure data transmission across different network domains by satisfying diverse routing requirements.However,current solutions face numerous challenges in continuously ensuring trustworthy routing,fulfilling diverse requirements,achieving reasonable resource allocation,and safeguarding against malicious behaviors of network operators.We propose CrowdRouting,a novel cross-domain routing scheme based on crowdsourcing,dedicated to establishing sustained trust in cross-domain routing,comprehensively considering and fulfilling various customized routing requirements,while ensuring reasonable resource allocation and effectively curbing malicious behavior of network operators.Concretely,CrowdRouting employs blockchain technology to verify the trustworthiness of border routers in different network domains,thereby establishing sustainable and trustworthy crossdomain routing based on sustained trust in these routers.In addition,CrowdRouting ingeniously integrates a crowdsourcing mechanism into the auction for routing,achieving fair and impartial allocation of routing rights by flexibly embedding various customized routing requirements into each auction phase.Moreover,CrowdRouting leverages incentive mechanisms and routing settlement to encourage network domains to actively participate in cross-domain routing,thereby promoting optimal resource allocation and efficient utilization.Furthermore,CrowdRouting introduces a supervisory agency(e.g.,undercover agent)to effectively suppress the malicious behavior of network operators through the game and interaction between the agent and the network operators.Through comprehensive experimental evaluations and comparisons with existing works,we demonstrate that CrowdRouting excels in providing trustworthy and fine-grained customized routing services,stimulating active participation in cross-domain routing,inhibiting malicious operator behavior,and maintaining reasonable resource allocation,all of which outperform baseline schemes.展开更多
The advent of 6G wireless networks promises unprecedented connectivity,supporting ultra-high data rates,low latency,and massive device connectivity.However,these ambitious goals introduce significant challenges,partic...The advent of 6G wireless networks promises unprecedented connectivity,supporting ultra-high data rates,low latency,and massive device connectivity.However,these ambitious goals introduce significant challenges,particularly in channel estimation due to complex and dynamic propagation environments.This paper explores the concept of channel knowledge maps(CKMs)as a solution to these challenges.CKMs enable environment-aware communications by providing location-specific channel information,reducing reliance on real-time pilot measurements.We categorize CKM construction techniques into measurement-based,model-based,and hybrid methods,and examine their key applications in integrated sensing and communication(ISAC)systems,beamforming,trajectory optimization of unmanned aerial vehicles(UAVs),base station(BS)placement,and resource allocation.Furthermore,we discuss open challenges and propose future research directions to enhance the robustness,accuracy,and scalability of CKM-based systems in the evolving 6G landscape.展开更多
Developing fast-charging lithium-ion batteries(LIBs)that feature high energy density is critical for the scalable application of electric vehicles.Iron vanadate(FVO)holds great potential as anode material in fast-char...Developing fast-charging lithium-ion batteries(LIBs)that feature high energy density is critical for the scalable application of electric vehicles.Iron vanadate(FVO)holds great potential as anode material in fast-charging LIBs because of its high theoretical specific capacity and the high natural abundance of its constituents.However,the capacity of FVO rapidly decays due to its low electrical conductivity.Herein,uniform FVO nanoparticles are grown in situ on ordered mesoporous carbon(CMK-3)support,forming a highly electrically conductive porous network,FVO/CMK-3.The structure of CMK-3 helps prevent agglomeration of FVO particles.The electrically conductive nature of CMK-3 can further enhance the electrical conductivity of FVO/CMK-3 and buffer the volume expansion of FVO particles during cycling processes.As a result,the FVO/CMK-3 displays excellent fast-charging performance of 364.6 mAh·g^(-1)capacity for 2500 cycles at 10 A·g^(-1)(with an ultralow average capacity loss per cycle of 0.003%)through a pseudocapacitive-dominant process.Moreover,the LiCoO_(2)//FVO/CMK-3 full cell achieves a high capacity of 100.2 mAh·g^(-1)and a high capacity retention(96.2%)after 200 cycles.The superior electrochemical performance demonstrates that FVO/CMK-3 is an ideal anode material candidate for fast-charging,stable LIBs with high energy density.展开更多
The expansive spectral coverage and superior optical properties of lithium niobate(LN)offer a comprehensive suite of tools for exploring novel functionalities.Achieving high-quality(Q)photonic resonator cavities is cr...The expansive spectral coverage and superior optical properties of lithium niobate(LN)offer a comprehensive suite of tools for exploring novel functionalities.Achieving high-quality(Q)photonic resonator cavities is crucial for enhancing light-matter interactions.However,this task is challenging as the device performance is heavily dependent on the fabrication quality of the LN.In this paper,we present experimental validation of an etchless approach to fabricating high-Q photonic crystal nanobeam cavities(PCNBCs).We successfully fabricate PCNBCs with Q factors exceeding 105 while maintaining high transmittance by capitalizing on the low waveguide loss and high fabrication tolerance of TE-polarized mode.Remarkably,the Q factor achieved here exceeds previous reports on etchless LN PCNBCs by over an order of magnitude.Benefiting from this advancement,we further explore a variety of optical functions,including thermo-optic tuning,optically induced bistability,and Fano line shapes generation.These findings present promising prospects for a versatile platform technique,facilitating the development of high-performance electro-optic or acousto-optic modulators,optical logic devices,and quantum photonics,highlighting its significant impact in the field of photonic integration.展开更多
Low energy-storage density and inferior thermal stability are a long-term obstacle to the advancement of pulse power devices.Herein,these concerns are addressed by improving bandgap and fabricating polar nanoregions,a...Low energy-storage density and inferior thermal stability are a long-term obstacle to the advancement of pulse power devices.Herein,these concerns are addressed by improving bandgap and fabricating polar nanoregions,and the superior high efficiency of~86.7%,excellent thermal stability of~2%(31-160℃)and energy density of~6.8 J·cm^(-3)are achieved in Bi_(0.5)Na_(0.5)TiO_(3)-La_(0.1)Sr_(0.8)TiO_(3)-δ-NaNbO_(3)ceramics.The high breakdown strength(460 kV·cm^(-1))is ascribed to the broadened bandgap and refined grain.Slim ferroelectric loops originate from the construction of polar nanoregions(PNRs)in a pseudocubic matrix,and transmission electron microscope and piezoelectric force microscope measurements reveal the occurrence of PNRs.The phase-field stimulation and UV-Vis spectrophotometer measurement reveal that the increased grain boundary density and bandgap are beneficial for promoting breakdown strength.The strategy provides an efficient path to prepare Bi_(0.5)Na_(0.5)TiO_(3)La_(0.1)Sr_(0.8)TiO_(3)-δ-based ceramics with superior efficiency,high energy density and outstanding thermal stability.展开更多
Aerogels with excellent properties combination of ultralow density and great thermal insulation are drawing attention to applications in harsh conditions.Common aerogels,however,are usually constructed with nanopartic...Aerogels with excellent properties combination of ultralow density and great thermal insulation are drawing attention to applications in harsh conditions.Common aerogels,however,are usually constructed with nanoparticles with a weakness in physical combination.The silicon carbide nano wire(SiC_(NW)) is a kind of one-dimensional(1D) nano wire possessing the promising properties of flexibility,great thermal insulation,and stability at high temperatures.An aerogel constructed by the SiC_(NW) will produce a great material with a promising material,the amazing SiC_(NW) aerogel.Here,a novel SiC_(NW) aerogel was fabricated consisting of quantities of β-SiC_(NW) of15-40 nm in diameter and tens to hundreds of micrometers in length.This SiC_(NW) aerogel possessed an ultralow density of 5.82 mg·cm^(-3),high-temperature resistance,and great thermal insulation with its thermal conductivities of0.063 W·m^(-1)·K^(-1) at 100℃ and 0.243 W·m^(-1)·K^(-1) at900℃ in He.Furthermore,the thermal insulation applicability of this aerogel was simulated.This study provides a promising way for designing and fabricating other multifunctional nanowire aerogels for high-temperature thermal insulation.展开更多
基金support of the National Natural Science Foundation of China(Grant No.52205593)Shaanxi Natural Science Foundation Project(2024JC-YBMS-711).
文摘The incidence of large bone defects caused by traumatic injury is increasing worldwide,and the tissue regeneration process requires a long recovery time due to limited self-healing capability.Endogenous bioelectrical phenomena have been well recognized as critical biophysical factors in bone remodeling and regeneration.Inspired by bioelectricity,electrical stimulation has been widely considered an external intervention to induce the osteogenic lineage of cells and enhance the synthesis of the extracellular matrix,thereby accelerating bone regeneration.With ongoing advances in biomaterials and energy-harvesting techniques,electroactive biomaterials and self-powered systems have been considered biomimetic approaches to ensure functional recovery by recapitulating the natural electrophysiological microenvironment of healthy bone tissue.In this review,we first introduce the role of bioelectricity and the endogenous electric field in bone tissue and summarize different techniques to electrically stimulate cells and tissue.Next,we highlight the latest progress in exploring electroactive hybrid biomaterials as well as self-powered systems such as triboelectric and piezoelectric-based nanogenerators and photovoltaic cell-based devices and their implementation in bone tissue engineering.Finally,we emphasize the significance of simulating the target tissue’s electrophysiological microenvironment and propose the opportunities and challenges faced by electroactive hybrid biomaterials and self-powered bioelectronics for bone repair strategies.
基金supported by the National Natural Science Foundation of China(No.52461002)
文摘Finely tuning spectral characteristics of the epsilon-negative(ε'<0,EN) response is full of challenges when its regulatory mechanism in metacomposites is not yet clear.Herein,we have meticulously designed Cu/CaCu_(3)Ti_(4)O_(12)(Cu/CCTO) percolative metacomposites,successfully achieved both epsilon-negative and ε'-near-zero(ENZ)responses in the radio-frequency band.Before percolation,a large number of electric dipoles in the metacomposites achieved resonance characteristics near the ENZ point under the excitation of radio frequency electromagnetic fields,and as the Cu content increased,the ENZ frequency varied from 942,858,862 to 632 MHz.
基金supported by the National Natural Science Foundation of China(Nos.32171627 and 62105252)the Science and Technology Research Program of Chongqing Municipal Education Commission(No.KJZD-M202200602)the Hangzhou Science and Technology Development Project(No.202204T04).
文摘The total nitrogen(TN)is a major factor contributing to eutrophication and is a crucial parameter in assessing surface water quality.Accurate and rapid methods are crucial for determining the TN content in water.Herein,a fast,highly sensitive,and pollution-free approach is proposed,which combines ultraviolet(UV)absorption spectroscopy with Bayesian optimized least squares support vector machine(LSSVM)for detecting TN content in water.Water samples collected from sampling points near the Yangtze River basin in Chongqing of China were analyzed using national standard methods to measure TN content as reference values.The prediction of TN content in water was achieved by integrating the UV absorption spectra of water samples with LSSVM.To make the model quickly and accurately select the optimal parameters to improve the accuracy of the prediction model,the Bayesian optimization(BO)algorithm was used to optimize the parameters of the LSSVM.Results show that the prediction model performs well in predicting TN concentration,with a high coefficient of prediction determination(R^(2)=0.9413)and a low root mean square error of prediction(RMSE=0.0779 mg/L).Comparative analysis with previous studies indicates that the model used in this paper achieves lower prediction errors and superior predictive performance.
基金supported by the Natural Science Foundation of Guizhou Province(No.ZK 2022-044)the Platform of Science and Technology and Talent Team Plan of Guizhou Province(No.GCC[2023]007)+1 种基金the National Science Foundation of China(Nos.52101010 and 11964006)the Fund of Natural Science Special(Special Post)Research Foundation of Guizhou University(No.2021-018).
文摘The design and development of high-performance anodes pose significant challenges in the construction of next-generation rechargeable lithium-ion batteries(LIBs).Sodium molybdate dihydrate(Na_(2)MoO_(4)·2H_(2)O)has garnered increasing attention due to its cost-effectiveness,non-toxicity and earth abundance.To enhance the Li storage performance of Na_(2)MoO_(4)·2H_(2)O,a crystallographic orientation regulation strategy is proposed in this work.Initially,density functional theory calculations are carried out to demonstrate that the(020)crystal plane of Na_(2)MoO_(4)·2H_(2)O offers the lowest energy barrier for Li^(+)migration.Subsequently,the preferred crystallographic orientation of Na_(2)MoO_(4)·2H_(2)O crystal is tuned through a low-temperature recrystallization method.Furthermore,the microstructure and phase changes of Na_(2)MoO_(4)·2H_(2)O during the lithiation/de-lithiation process are studied using in situ and ex situ XRD tests,ex situ XPS and cyclic voltammetry to unravel its Li^(+)storage mechanism.Upon application as LIBs anode,the Na_(2)MoO_(4)·2H_(2)O single-crystal particles with a preferred(020)surface exhibit superior reversible capacity,high-capacity retention and high cycling stability.The enhanced Li storage performance should be attributed to the regulated crystallographic orientation and small changes in the crystal microstructure during the charge/discharge process,which facilitates Li^(+)migration and bolsters structural stability.Notably,this study introduces a novel concept and a simple synthesis method for the advancement of electrodes in rechargeable batteries.
基金supported by the National Natural Science Foundation of China (NSFC) (Grants No. 12274236, 12134009, 12074223)Shandong Provincial Natural Science Foundation (Grants No. 2022HWYQ-047, ZR2024MA041)+3 种基金Taishan Scholars Program of Shandong Province (Grants No. tsqn201909041)“Qilu Young Scholar Program” of Shandong UniversityCore Facility Sharing Platform of Shandong UniversityOpen Foundation of the State Key Laboratory of Fluid Power and Mechatronic Systems
文摘Controlling the construction of physical colors on the surfaces of transparent dielectric crystals is crucial for surface coloration and anti-counterfeiting applications.In this study,we present a novel approach to creating stable physical colors on the surface of lithium niobate crystals by combining gold ion implantation with laser direct writing technologies.The interaction between the laser,the implanted gold nanoparticles,and the crystal lattice induces permanent,localized modifications on the crystal surface.By fine-tuning the laser direct writing parameters,we reshaped the gold nanoparticles into spheres of varying sizes on the crystal surface,resulting in the display of red,green,blue,and pale-yellow colors.We investigated the influence of the implanted Au nanoparticles-particularly their localized surface plasmon resonances-on the modifications of the lithium niobate crystal lattice during the laser writing process using confocal Raman spectroscopy and high-resolution transmission electron microscopy.Our findings reveal that the embedded Au nanoparticles play a pivotal role in altering the conventional light-matter interaction between the crystal lattice and the laser,thereby facilitating the generation of surface colors.This work opens new avenues for the development of vibrant surface colors on transparent dielectric crystals.
基金This work was financially supported by the National Natural Science Foundation of China(No.52205593)the Fund of Natural Science Special(Special Post)Research Foundation of Guizhou University(No.2023-032)the Platform of Science and Technology and Talent Team Plan of Guizhou Province(No.GCC[2023]007).
文摘CaCu_(3)Ti_(4)O_(12)(CCTO)ceramic nanocomposites incorporating graphene–carbon black(GRCB)fillers were fabricated by spark plasma sintering process.The percolative effects of conductive GRCB fillers on dielectric response of GRCB/CCTO ternary metacomposites were systematically investigated.The weakly real permittivity(ε′)-negative response(ε′~−1×10^(2))was achieved which originated from weakly low-frequency plasmonic state of free carriers within constructed GRCB networks.With enhancing three-dimensional GRCB network,the plasma frequency of metacomposites increased while the damping factor decreased.Herein,theε′-negative values of metacomposites were tuned from−10^(2) to−10^(4) orders of magnitude andε′-near-zero(ENZ)frequencies from~142 to~340 MHz which substantially benefited from the moderate carrier concentration of GRCB dual fillers.The Drude model and equivalent circuit models were adopted to demonstrate dielectric and electrical characteristics.The obtained metacomposites show strong EM shielding effect along with enhanced plasmonic oscillation and even better achieving perfect EM shielding effect in ENZ media.This work achieves the tunableε′-negative andε′-near-zero response and more importantly clarifies its regulation mechanism in ceramic-based ternary metacomposites,which opens up the possibility of designing high-performance EM shielding materials based on metacomposites.
基金supported by the National Natural Science Foundation of China(Nos.52105575&52205593)the Fundamental Research Funds for the Central Universities(No.QTZX23063)+1 种基金the Proof of Concept Foundation of Xidian University Hangzhou Institute of Technology(Nos.GNYZ2023YL0302&GNYZ2023QC0401)the Aeronautical Science Foundation of China(No.2022Z073081001)。
文摘Lithium-sulfur batteries(LSBs)have already developed into one of the most promising new-generation high-energy density electrochemical energy storage systems with outstanding features including high-energy density,low cost,and environmental friendliness.However,the development and commercialization path of LSBs still presents significant limitations and challenges,particularly the notorious shuttle effect triggered by soluble longchain lithium polysulfides(LiPSs),which inevitably leads to low utilization of cathode active sulfur and high battery capacity degradation,short cycle life,etc.Substantial research efforts have been conducted to develop various sulfur host materials capable of effectively restricting the shuttle effect.This review firstly introduces the fundamental electrochemical aspects of LSBs,followed by a comprehensive analysis of the mechanism underlying the shuttle effect in Li–S batteries and its profound influence on various battery components as well as the overall battery performance.Subsequently,recent advances and strategies are systematically reviewed,including physical confinement,chemisorption,and catalytic conversion of sulfur hosts for restricting LiPSs shuttle effects.The interplay mechanisms of sulfur hosts and LiPSs are discussed in detail and the structural advantages of different host materials are highlighted.Furthermore,key insights for the rational design of advanced host materials for LSBs are provided,and the upcoming challenges and the prospects for sulfur host materials in lithium-sulfur batteries are also explored.
基金supported by the National Natural Science Foundation of China(Grant Nos.12302151 and 52105575)the BIT Research and Innovation Promoting Project(Grant No.2023YCXY049)+2 种基金the Fundamental Research Funds for the Central Universities(Grant No.QTZX23063)the Aeronautical Science Foundation of China(Grant No.2022Z073081001)the Open Research Funds of State Key Laboratory of Intelligent Manufacturing Equipment and Technology(Grant No.IMETKF2024008).
文摘In this paper,a liquid-solid origami composite design is proposed for the improvement of impact resistance.Employing this design strategy,Kresling origami composite structures with different fillings were designed and fabricated,namely air,water,and shear thickening fluid(STF).Quasi-static compression and drop-weight impact experiments were carried out to compare and reveal the static and dynamic mechanical behavior of these structures.The results from drop-weight impact experiments demonstrated that the solid-liquid Kresling origami composite structures exhibited superior yield strength and reduced peak force when compared to their empty counterparts.Notably,the Kresling origami structures filled with STF exhibited significantly heightened yield strength and reduced peak force.For example,at an impact velocity of 3 m/s,the yield strength of single-layer STF-filled Kresling origami structures increased by 772.7%and the peak force decreased by 68.6%.This liquid-solid origami composite design holds the potential to advance the application of origami structures in critical areas such as aerospace,intelligent protection and other important fields.The demonstrated improvements in impact resistance underscore the practical viability of this approach in enhancing structural performance for a range of applications.
基金supported by the National Natural Science Foundation of China(Nos.52177059 and 52407064).
文摘Permanent magnet synchronous motor based electro-mechanical actuation servo drives have widespread applications in the aviation field,such as unmanned aerial vehicle electric servos,electric cabin doors,and mechanical arms.The performance of the servo drive,which encompasses the response to the torque,efficiency,control bandwidth and the steady-state positioning accuracy,significantly influences the performance of the aviation actuation.Consequently,enhancing the control bandwidth and refining the positioning accuracy of aviation electro-mechanical actuation servo drives have emerged as a focal point of research.This paper investigates the multi-source disturbances present in aviation electro-mechanical actuation servo systems and summarizes recent research on high-performance servo control methods based on active disturbance rejection control(ADRC).We present a comprehensive overview of the research status pertaining to servo control architecture,strategies for suppressing disturbances in the current loop,and ADRC-based strategies for the position loop.We delineate the research challenges and difficulties encountered by aviation electro-mechanical actuation servo drive control technology.
基金financial supports from the National Natural Science Foundation of China(Grant Nos.51925503&52105575)the Fundamental Research Funds for the Central Universities(Grant No.QTZX23063)+2 种基金the Aeronautical Science Foundation of China(Grant No.2022Z073081001)the Postdoctoral Fellowship Program of CPSF(Grant No.GZC20232028)the Open Research Funds of State Key Laboratory of Intelligent Manufacturing Equipment and Technology(Grant No.IMETKF2024008).
文摘The combination of advanced photoelectric detectors has rendered single-band camouflage materials ineffective,necessitating the development of infrared multispectral camouflage.However,the design and fabrication of existing works remain complex as they usually require the integration of multiscale structures.Here,we introduce phase modulation into the infrared camouflage metasurfaces with metal-dielectric-metal configuration,enabling them to achieve camouflage across more bands.Based on this strategy,a simple but effective single-layer cascaded metasurface is demonstrated for the first time to achieve low reflection at multi-wavelength lasers,low infrared radiation in atmospheric windows,and broadband thermal management.As a proof-of-concept,a 4-inch sample with a minimum linewidth of 1.8μm is fabricated using photolithography.The excellent infrared multispectral camouflage performance is verified in experiments,showing low reflectance in 0.9–1.6μm,low infrared emissivity in mid-wavelength infrared(MWIR)and long-wavelength infrared(LWIR)bands,and high absorptance at the wavelength of 10.6μm.Meanwhile,broadband high emissivity in 5–8μm can provide high-performance radiative heat dissipation.When the input power is 1.57 W·cm^(-2),the surface/radiation temperature of the metasurface decreases by 5.3℃/18.7℃ compared to the reference.The proposed metasurface may trigger further innovation in the design and application of compact multispectral optical devices.
基金the National Key Research and Development Program of China,Grant/Award Number:2020YFB1711704the National Natural Science Foundation of China,Grant/Award Number:62272337。
文摘As an essential field of multimedia and computer vision,3D shape recognition has attracted much research attention in recent years.Multiview-based approaches have demonstrated their superiority in generating effective 3D shape representations.Typical methods usually extract the multiview global features and aggregate them together to generate 3D shape descriptors.However,there exist two disadvantages:First,the mainstream methods ignore the comprehensive exploration of local information in each view.Second,many approaches roughly aggregate multiview features by adding or concatenating them together.The information loss for some discriminative characteristics limits the representation effectiveness.To address these problems,a novel architecture named region-based joint attention network(RJAN)was proposed.Specifically,the authors first design a hierarchical local information exploration module for view descriptor extraction.The region-to-region and channel-to-channel relationships from different granularities can be comprehensively explored and utilised to provide more discriminative characteristics for view feature learning.Subsequently,a novel relation-aware view aggregation module is designed to aggregate the multiview features for shape descriptor generation,considering the view-to-view relationships.Extensive experiments were conducted on three public databases:ModelNet40,ModelNet10,and ShapeNetCore55.RJAN achieves state-of-the-art performance in the tasks of 3D shape classification and 3D shape retrieval,which demonstrates the effectiveness of RJAN.The code has been released on https://github.com/slurrpp/RJAN.
基金support from the National Key R&D Program of China(2021YFB3200700)the National Natural Science Foundation of China(Grant No.0214100221,51925503).
文摘This study presents a breakthrough in flexible strain sensor technology with the development of an ultrahigh sensitivity and wide-range sensor,addressing the critical challenge of reconciling sensitivity with measurement range.Inspired by the structure of bamboo slips,we introduce a novel approach that utilises liquid metal to modulate the electrical pathways within a cracked platinum fabric electrode.The resulting sensor demonstrates a gauge factor greater than 108 and a strain measurement capability exceeding 100%.The integration of patterned liquid metal enables customisable tuning of the sensor’s response,while the porous fabric structure ensures superior comfort and air permeability for the wearer.Our design not only optimises the sensor’s performance but also enhances the electrical stability that is essential for practical applications.Through systematic investigation,we reveal the intrinsic mechanisms governing the sensor’s response,offering valuable insights for the design of wearable strain sensors.The sensor’s exceptional performance across a spectrum of applications,from micro-strain to large-strain detection,highlights its potential for a wide range of real-world uses,demonstrating a significant advancement in the field of flexible electronics.
基金National Natural Science Foundation of China(No.12574332)the Space Optoelectronic Measurement and Perception Lab.,Beijing Institute of Control Engineering(No.LabSOMP-2023-10)Major Science and Technology Innovation Program of Xianyang City(No.L2024-ZDKJ-ZDCGZH-0021)。
文摘Fourier Ptychographic Microscopy(FPM)is a high-throughput computational optical imaging technology reported in 2013.It effectively breaks through the trade-off between high-resolution imaging and wide-field imaging.In recent years,it has been found that FPM is not only a tool to break through the trade-off between field of view and spatial resolution,but also a paradigm to break through those trade-off problems,thus attracting extensive attention.Compared with previous reviews,this review does not introduce its concept,basic principles,optical system and series of applications once again,but focuses on elaborating the three major difficulties faced by FPM technology in the process from“looking good”in the laboratory to“working well”in practical applications:mismatch between numerical model and physical reality,long reconstruction time and high computing power demand,and lack of multi-modal expansion.It introduces how to achieve key technological innovations in FPM through the dual drive of Artificial Intelligence(AI)and physics,including intelligent reconstruction algorithms introducing machine learning concepts,optical-algorithm co-design,fusion of frequency domain extrapolation methods and generative adversarial networks,multi-modal imaging schemes and data fusion enhancement,etc.,gradually solving the difficulties of FPM technology.Conversely,this review deeply considers the unique value of FPM technology in potentially feeding back to the development of“AI+optics”,such as providing AI benchmark tests under physical constraints,inspirations for the balance of computing power and bandwidth in miniaturized intelligent microscopes,and photoelectric hybrid architectures.Finally,it introduces the industrialization path and frontier directions of FPM technology,pointing out that with the promotion of the dual drive of AI and physics,it will generate a large number of industrial application case,and looks forward to the possibilities of future application scenarios and expansions,for instance,body fluid biopsy and point-of-care testing at the grassroots level represent the expansion of the growth market.
基金supported by the National Natural Science Foundation of China(No.52407064)。
文摘1.Opportunities for electric motor drives in the low-altitude economy The implementation plan for the innovative application of general aviation equipment(2024–2030)outlines that by 2027,new general aviation equipment will achieve commercial applications in urban air transport,logistics distribution and emergency rescue.
基金supported in part by the National Natural Science Foundation of China under Grant U23A20300 and 62072351in part by the Key Research Project of Shaanxi Natural Science Foundation under Grant 2023-JC-ZD-35+1 种基金in part by the Concept Verification Funding of Hangzhou Institute of Technology of Xidian University under Grant GNYZ2024XX007in part by the 111 Project under Grant B16037.
文摘Cross-domain routing in Integrated Heterogeneous Networks(Inte-HetNet)should ensure efficient and secure data transmission across different network domains by satisfying diverse routing requirements.However,current solutions face numerous challenges in continuously ensuring trustworthy routing,fulfilling diverse requirements,achieving reasonable resource allocation,and safeguarding against malicious behaviors of network operators.We propose CrowdRouting,a novel cross-domain routing scheme based on crowdsourcing,dedicated to establishing sustained trust in cross-domain routing,comprehensively considering and fulfilling various customized routing requirements,while ensuring reasonable resource allocation and effectively curbing malicious behavior of network operators.Concretely,CrowdRouting employs blockchain technology to verify the trustworthiness of border routers in different network domains,thereby establishing sustainable and trustworthy crossdomain routing based on sustained trust in these routers.In addition,CrowdRouting ingeniously integrates a crowdsourcing mechanism into the auction for routing,achieving fair and impartial allocation of routing rights by flexibly embedding various customized routing requirements into each auction phase.Moreover,CrowdRouting leverages incentive mechanisms and routing settlement to encourage network domains to actively participate in cross-domain routing,thereby promoting optimal resource allocation and efficient utilization.Furthermore,CrowdRouting introduces a supervisory agency(e.g.,undercover agent)to effectively suppress the malicious behavior of network operators through the game and interaction between the agent and the network operators.Through comprehensive experimental evaluations and comparisons with existing works,we demonstrate that CrowdRouting excels in providing trustworthy and fine-grained customized routing services,stimulating active participation in cross-domain routing,inhibiting malicious operator behavior,and maintaining reasonable resource allocation,all of which outperform baseline schemes.
基金supported by the National Natural Science Foundation of China under Grants Nos.62431014 and 62271310the Fundamental Research Funds for the Central Universities of China。
文摘The advent of 6G wireless networks promises unprecedented connectivity,supporting ultra-high data rates,low latency,and massive device connectivity.However,these ambitious goals introduce significant challenges,particularly in channel estimation due to complex and dynamic propagation environments.This paper explores the concept of channel knowledge maps(CKMs)as a solution to these challenges.CKMs enable environment-aware communications by providing location-specific channel information,reducing reliance on real-time pilot measurements.We categorize CKM construction techniques into measurement-based,model-based,and hybrid methods,and examine their key applications in integrated sensing and communication(ISAC)systems,beamforming,trajectory optimization of unmanned aerial vehicles(UAVs),base station(BS)placement,and resource allocation.Furthermore,we discuss open challenges and propose future research directions to enhance the robustness,accuracy,and scalability of CKM-based systems in the evolving 6G landscape.
基金supported by the National Natural Science Foundation of China(No.52002170)the Central Guidance Fund Project for Local Scientific and Technological Development in Qinghai Province(No.2024ZY013)+1 种基金the Foundation of Key Laboratory of Flexible Electronics of Zhejiang Province(No.2023FE011)the Postgraduate Research&Practice Innovation Program of Jiangsu Province(No.KYCX24_1635).
文摘Developing fast-charging lithium-ion batteries(LIBs)that feature high energy density is critical for the scalable application of electric vehicles.Iron vanadate(FVO)holds great potential as anode material in fast-charging LIBs because of its high theoretical specific capacity and the high natural abundance of its constituents.However,the capacity of FVO rapidly decays due to its low electrical conductivity.Herein,uniform FVO nanoparticles are grown in situ on ordered mesoporous carbon(CMK-3)support,forming a highly electrically conductive porous network,FVO/CMK-3.The structure of CMK-3 helps prevent agglomeration of FVO particles.The electrically conductive nature of CMK-3 can further enhance the electrical conductivity of FVO/CMK-3 and buffer the volume expansion of FVO particles during cycling processes.As a result,the FVO/CMK-3 displays excellent fast-charging performance of 364.6 mAh·g^(-1)capacity for 2500 cycles at 10 A·g^(-1)(with an ultralow average capacity loss per cycle of 0.003%)through a pseudocapacitive-dominant process.Moreover,the LiCoO_(2)//FVO/CMK-3 full cell achieves a high capacity of 100.2 mAh·g^(-1)and a high capacity retention(96.2%)after 200 cycles.The superior electrochemical performance demonstrates that FVO/CMK-3 is an ideal anode material candidate for fast-charging,stable LIBs with high energy density.
基金the National Key R&D Program of China(No.2022ZD0119002)the National Natural Science Foundation of China(Grant No.62025402,62090033,92364204,92264202 and 62293522)Major Program of Zhejiang Natural Science Foundation(Grant No.LDT23F04024F04)。
文摘The expansive spectral coverage and superior optical properties of lithium niobate(LN)offer a comprehensive suite of tools for exploring novel functionalities.Achieving high-quality(Q)photonic resonator cavities is crucial for enhancing light-matter interactions.However,this task is challenging as the device performance is heavily dependent on the fabrication quality of the LN.In this paper,we present experimental validation of an etchless approach to fabricating high-Q photonic crystal nanobeam cavities(PCNBCs).We successfully fabricate PCNBCs with Q factors exceeding 105 while maintaining high transmittance by capitalizing on the low waveguide loss and high fabrication tolerance of TE-polarized mode.Remarkably,the Q factor achieved here exceeds previous reports on etchless LN PCNBCs by over an order of magnitude.Benefiting from this advancement,we further explore a variety of optical functions,including thermo-optic tuning,optically induced bistability,and Fano line shapes generation.These findings present promising prospects for a versatile platform technique,facilitating the development of high-performance electro-optic or acousto-optic modulators,optical logic devices,and quantum photonics,highlighting its significant impact in the field of photonic integration.
基金supported by the National Natural Science Foundation of China(Nos.12364015 and 52176072)the Five-Year Action Plan for Shccig-Qinling Program and Key Project of Hubei Province Key Research and Development Plan(No.2021BCA140)+4 种基金the Industry and Education Combination Innovation Platform of Intelligent Manufacturing and Graduate Joint Training Base at Guizhou University(No.2020-520000-83-01-324061)the National Key Research and Development Plan(No.2022YFF0706500)Guizhou University Natural Science Special(special post)Research Fund(No.(2023)17)Guizhou Engineering Research Center for Smart Services(No.2203-520102-04-04-298868)the Construction of Science and Technology Platform of Guiyang(No.[2023]7-3).
文摘Low energy-storage density and inferior thermal stability are a long-term obstacle to the advancement of pulse power devices.Herein,these concerns are addressed by improving bandgap and fabricating polar nanoregions,and the superior high efficiency of~86.7%,excellent thermal stability of~2%(31-160℃)and energy density of~6.8 J·cm^(-3)are achieved in Bi_(0.5)Na_(0.5)TiO_(3)-La_(0.1)Sr_(0.8)TiO_(3)-δ-NaNbO_(3)ceramics.The high breakdown strength(460 kV·cm^(-1))is ascribed to the broadened bandgap and refined grain.Slim ferroelectric loops originate from the construction of polar nanoregions(PNRs)in a pseudocubic matrix,and transmission electron microscope and piezoelectric force microscope measurements reveal the occurrence of PNRs.The phase-field stimulation and UV-Vis spectrophotometer measurement reveal that the increased grain boundary density and bandgap are beneficial for promoting breakdown strength.The strategy provides an efficient path to prepare Bi_(0.5)Na_(0.5)TiO_(3)La_(0.1)Sr_(0.8)TiO_(3)-δ-based ceramics with superior efficiency,high energy density and outstanding thermal stability.
基金financially supported by the Talent Introduction Project Foundation of Nantong University (No. 135421615077)the Large Instruments Open Foundation of Nantong University (No. KFJN2237)+5 种基金the Fundamental Research Funds for the Central Universities (No. D5000210522)China Postdoctoral Science Foundation (No. 2021M702665)the Natural Science Foundation of Shaanxi Province (No. 2022JQ-482)Jiangsu Planned Projects for Postdoctoral Research FundBasic Research Programs of Taicang (No. TC2021JC01)2022 Suzhou Association for Science and Technology Youth Science and Technology Talent Support Project Fund。
文摘Aerogels with excellent properties combination of ultralow density and great thermal insulation are drawing attention to applications in harsh conditions.Common aerogels,however,are usually constructed with nanoparticles with a weakness in physical combination.The silicon carbide nano wire(SiC_(NW)) is a kind of one-dimensional(1D) nano wire possessing the promising properties of flexibility,great thermal insulation,and stability at high temperatures.An aerogel constructed by the SiC_(NW) will produce a great material with a promising material,the amazing SiC_(NW) aerogel.Here,a novel SiC_(NW) aerogel was fabricated consisting of quantities of β-SiC_(NW) of15-40 nm in diameter and tens to hundreds of micrometers in length.This SiC_(NW) aerogel possessed an ultralow density of 5.82 mg·cm^(-3),high-temperature resistance,and great thermal insulation with its thermal conductivities of0.063 W·m^(-1)·K^(-1) at 100℃ and 0.243 W·m^(-1)·K^(-1) at900℃ in He.Furthermore,the thermal insulation applicability of this aerogel was simulated.This study provides a promising way for designing and fabricating other multifunctional nanowire aerogels for high-temperature thermal insulation.
