Persistent toxic substances(PTS)represent a paramount environmental issue in the 21st century.Understanding the concentrations and forms of PTS in the environment is crucial for accurately assessing their environmenta...Persistent toxic substances(PTS)represent a paramount environmental issue in the 21st century.Understanding the concentrations and forms of PTS in the environment is crucial for accurately assessing their environmental health impacts.This article presents a concise overview of the components of PTS,pertinent environmental regulations,and conventional detection methodologies.Additionally,we offer an in-depth review of the principles,development,and practical applications of surface-enhanced Raman scattering(SERS)in environmental monitoring,emphasizing the advancements in detecting trace amounts of PTS in complex environmental matrices.Recent progress in enhancing SERS sensitivity,improving selectivity,and practical implementations are detailed,showcasing innovative materials and methods.Integrating SERS with advanced algorithms are highlighted as pivotal areas for future research.展开更多
The authors regret that in 1.2.Instruments section of the article,when describing the principle of TiH300,the original content of“Briefly,ambient HONO was first absorbed by deionized water in a two-channel stripping ...The authors regret that in 1.2.Instruments section of the article,when describing the principle of TiH300,the original content of“Briefly,ambient HONO was first absorbed by deionized water in a two-channel stripping coil.The absorbed liquid nitrite was mixed with sulfanilamide,N-(1-naphthyl)-ethylenediamine dihydrochloride,and hydrogen chloride solution to form the azo dye derivative.”展开更多
1 Initial construction of JESTwenty years ago, research on environmental science was extended beyond its initial scope including pollution source surveys, environmental pollution monitoring, and treatment of the ＂thr...1 Initial construction of JESTwenty years ago, research on environmental science was extended beyond its initial scope including pollution source surveys, environmental pollution monitoring, and treatment of the ＂three wastes＂ （waste water, waste gas, and solid waste） to a full concern with the behavior, tendencies and harmful effects of pollutants in the environment as well as the overall understanding of the ecosystem. Environmental scientists came to realize that the solutions to environmental problems and their fields of study could no longer be restricted to a particular region or country, but needed exchanges with foreign scholars and transnational cooperation between scientists. However, at that time,展开更多
Environmental science is an interdisciplinary science developed in the process of understanding and solving ecolog-ical and environmental problems.In order to tackle these problems,environmental science research is ex...Environmental science is an interdisciplinary science developed in the process of understanding and solving ecolog-ical and environmental problems.In order to tackle these problems,environmental science research is expected to reveal the source,behavior,fate,exposure,and risks of pollutants in the environment and develop potential solutions to control pollution.It provides the scientific basis for decision-makers to establish environmental and economic poli-cies,and promote concerted efforts for the sustainable development of society.Here,we articulate the development patterns,challenges,and future research needs of environmental science in China based on literature review and expert panel discussion.Environmental science research has evolved significantly in the past decade with an increas-ing diversity of environmental pollutants and health impacts,new technologies and methods,deepening fusion of multiple disciplines,and emerging solutions for pollution control.Its future development relies on the advances in our knowledge on the fate and transport of pollutants,regional environmental processes,ecotoxicological effects,environmental exposure and health effects,environmental analysis and monitoring,source control and reduction,environmental remediation,as well as environmental risk management.For each of these fields,we summarize the significant challenges and highlight the research demands for China.Based on the status quo of China’s environmen-tal science research and future needs,we provide recommendations to promote its future development,including encouraging innovation and interdisciplinary research,providing decision support for national needs,encouraging international collaboration,and improving collaboration mechanisms.展开更多
This paper reviews the major contributions made by Norwegian scientists to Arctic environmental sciences since the 1880s. The review begins with the first International Polar Year （IPY） in 1882-83. It then considers...This paper reviews the major contributions made by Norwegian scientists to Arctic environmental sciences since the 1880s. The review begins with the first International Polar Year （IPY） in 1882-83. It then considers the 1890s to 1920s with the scientific expeditions focusing on ocean and sea ice conditions of Nansen, Amundsen and H. Sverdrup, and the mapping of the Queen Elizabeth Islands by Otto Sverdrup and colleagues. The period from 1911 to the mid-1920s also witnessed annual expeditions to Svalbard led by Adolf Hoel. The 1930s to 1945 period encompassed the Second International Polar Year when Arctic weather stations were established or maintained. The time interval post-World War II to 2000 witnessed major advances made possible by technical and organizational innovations. The establishment of the Norwegian Polar Institute in 1948 led to extensive research on the glaciers and snow cover in the Svalbard archipelago and to oceanographic and sea ice research in the Barents Sea and Arctic Ocean. Remote sensing methods began to be widely used from the 1980s. The new millennium saw the undertaking of the third IPY and a shift to multinational projects. New fields such as ocean-ice-atmosphere variability became active and there was much attention to high-latitude climate change in the context of global warming.展开更多
First of all, it is my honor to announce that Professor X. Chris Le has been appointed the Editor-in-Chief of Journal of Environmental Sciences （JES） after an international search and selection by the committee memb...First of all, it is my honor to announce that Professor X. Chris Le has been appointed the Editor-in-Chief of Journal of Environmental Sciences （JES） after an international search and selection by the committee members of the Research Center of Eco-environmental Sciences, Chinese Academy of Sciences. Professor Hongxiao Tang,展开更多
This study compares the environmental sustainability of five alternatives for the remediation of marine sediments of one of the most polluted coastal sites in Europe(Bagnoli-Coroglio bay,Mediterranean Sea),using the L...This study compares the environmental sustainability of five alternatives for the remediation of marine sediments of one of the most polluted coastal sites in Europe(Bagnoli-Coroglio bay,Mediterranean Sea),using the Life Cycle Assessment(LCA)methodology.The treatments are either in-situ or exsitu,the latter requiring an initial dredging to transport the contaminated sediments to the management site.More in detail,four ex-situ remediation technologies based on landfilling,bioremediation,electrokinetic technique and soil washing were identified.These technologies are compared to an in-situ strategy currently under validation for enhancing bioremediation of the polluted sediments of the Bagnoli-Coroglio site.Our results indicate that the disposal in landfilling site is the worst option in most categories(e.g.,650 kg CO_(2) eq./t of treated sediment,considering the nearest landfilling site),followed by the bioremediation,mainly due to the high energy demand.Electrokinetic remediation,soil washing,and innovative in-situ technology represent the most sustainable options.In particular,the new in-situ technology appears to be the least impacting in all categories(e.g.,54 kg CO_(2) eq./t of treated sediment),although it is expected to require longer treatment time(estimated up to 12 months based on its potential efficiency).It can reduce the impact on climate change more than 12 times compared to the disposal and 7 times compared to bioremediation in addition to the possibility to avoid/reduce the dredging operations and the consequent dispersion of pollutants.The results open relevant perspectives towards more eco-sustainable and costly effective actions for the reclamation of contaminated marine sediments.展开更多
In recent years,intensified land use change driven by climate change and human activities have markedly impacted the ecological environmental quality of the arid inland river basins.The implementation of forestry proj...In recent years,intensified land use change driven by climate change and human activities have markedly impacted the ecological environmental quality of the arid inland river basins.The implementation of forestry projects,coupled with continuous population growth,has increased the need for systematic assessments of ecological effects to ensure sustainable development in arid inland river basins.This study generated a 22-a(2000-2021)remote sensing ecological index(RSEI)data series for the Manas River Basin,a typical arid inland river basin in China,utilizing Moderate Resolution Imaging Spectroradiometer(MODIS)data and the Google Earth Engine(GEE)platform.We examined the spatiotemporal patterns of ecological environmental quality in the Manas River Basin through the Theil-Sen estimator,Mann-Kendall trend test,coefficient of variation(CV),and Hurst index.Furthermore,we employed the Optimal Parameter-based Geographical Detector(OPGD)method to quantify the influence of seven key drivers:elevation,slope,temperature,precipitation,gross domestic product(GDP),population density,and land use change.The key findings revealed that the basin's ecological environmental quality showed significant improvement(mean RSEI of 0.38,with a range of 0.34-0.41),with areas exhibiting good and excellent grades increasing by 16.71%,particularly in the midstream oasis region and upstream mountainous region,while areas exhibiting poor and relatively poor grades decreased by 11.52%in the downstream desert region.Spatial heterogeneity of ecological environmental quality was pronounced,with 32.23%of the areas showing localized degradation,the midstream oasis region exhibiting sustainable recovery potential(Hurst index>0.50),and only 36.67%of the areas maintaining stable and highly stable conditions(primarily in the upstream mountainous region).The OPGD analysis revealed that temperature(q-value=0.496-0.780),land use change(q-value=0.705-0.782),and elevation(q-value=0.245-0.637)were dominant factors,with the influence of land use change increasing during 2000-2020.Strong interaction effects emerged between land use change and temperature(q-value>0.705)and between land use change and elevation(q-value=0.751 in 2020),highlighting intensified human-nature coupling.These findings provide vital perspectives for ecosystem management in arid inland river basins under both climate and anthropogenic pressures.展开更多
Iron and steel industry is one of the main sources of air pollution emissions in China.The sintering process is an important link in the blast furnace ironmaking process,but it is also accompanied by a large number of...Iron and steel industry is one of the main sources of air pollution emissions in China.The sintering process is an important link in the blast furnace ironmaking process,but it is also accompanied by a large number of pollutants.Under the background of ultra-low emissions,iron and steel enterprises urgently need to upgrade their existing processes to address the existing process in practical application problems.In this study,a steel group in Gansu Province was taken as an example.By comparing and analyzing the pollutant emission characteristics before and after the ultra-low emission retrofit,the collaborative control effect of the combined process on SO_(2),NO_(x),particulate matter,and dioxins after the new retrofit was systematically evaluated.The results show that after the retrofit,the concentrations of particulate matter,SO_(2) and NO_(x) have dropped to near-zero levels,and the dioxin removal efficiency has reached 98.87%,with all indicators being better than the national ultra-low emission standards.The study confirms that the optimal combination of multi-pollutant collaborative treatment technologies is the key to achieving efficient emission reduction,among which selective catalytic reduction technology has a particularly significant synergistic removal effect on NO_(x) and dioxins.This study provides an important technical reference and practical basis for the ultra-low emission retrofit of the steel industry,and has important guiding significance for promoting the green retrofit of the industry.Its ultra-low emission retrofit is of great significance for achieving green and low-carbon development.展开更多
The Gansu-Qinghai contiguous region of the upper Yellow River is located in the transition zone between the Loess Plateau and the Qinghai-Tibet Plateau,characterized by fragile ecosystems and high sensitivity to clima...The Gansu-Qinghai contiguous region of the upper Yellow River is located in the transition zone between the Loess Plateau and the Qinghai-Tibet Plateau,characterized by fragile ecosystems and high sensitivity to climate change.As a critical ecological security barrier and water conservation area,it faces persistent tensions between development demands and ecological protection.Quantitative assessments of how production-living-ecological space(PLES)evolution affects ecological and environmental quality(EEQ)under long-term,multi-scenario conditions remain limited in such vulnerable regions.Understanding PLES-EEQ relationships is essential for optimizing territorial spatial planning and maintaining ecological security in the Yellow River basin.This study utilized land use data from 2000 to 2020 and the FLUS model to simulate PLES evolution from 2030 to 2060 under SSP1,SSP2,and SSP5 scenarios.The analytical framework integrated artificial neural networks and cellular automata with Shared Socioeconomic Pathways to project spatial configurations and assess EEQ in 2035.Living space expanded across all three scenarios while ecological space decreased.Production space increased by 125 km^(2) under SSP5 but declined in other scenarios.The EEQ index in 2035 showed improvements relative to the baseline value(0.4130)in 2020.Medium-to-high quality areas were primarily grassland and forest,whereas low-quality areas consisted mainly of unused land concentrated in the central and western regions.This study reveals a nonlinear relationship between ecological space quantity and quality,showing that structural optimization can enhance EEQ despite area reduction.The findings suggest that strengthening ecological protection redlines and restraining urban expansion are essential for territorial spatial optimization in ecologically fragile regions.展开更多
Anammox bacteria in constructed wetlands(CWs)play pivotal role in sustainable nitrogen transformation,yet existing studies lack comprehensive analysis of environmental gradients and microbial interactions,both key fac...Anammox bacteria in constructed wetlands(CWs)play pivotal role in sustainable nitrogen transformation,yet existing studies lack comprehensive analysis of environmental gradients and microbial interactions,both key factors in anammox bacteria enrichment.This study investigated the mechanisms driving anammox bacteria enrichment in lab-scale simulated CWs treating high-nitrogen wastewater,focusing on bacterial community re-sponses across wetland layers with various strategies,including continuous up-flow influent,nitrogen loading increase,effluent recirculation,intermittent influent,and anammox bacteria inoculation.Results showed that total relative and absolute abundances of anammox bacteria ranged from 0.77%to 12.50%and from 0.13 to 6.46×10^(7) copies/g,respectively.Dissolved oxygen and pH had significant positive correlations with the absolute abundance of anammox bacteria,while organic matter and nitrate negatively impacted their relative abundance.Permutational multivariate analysis of variance indicated that spatial heterogeneity explained more variation in anammox bacteria abundance(43.44%)compared to operational strategies(8.58%).In terms of microbial interactions,60 dominant species exhibited potential correlations with anammox bacteria,comprising 170 interactions(105 positive and 65 negative),which suggested that anammox bacteria generally foster cooperative relationships with dominant bacteria.Notably,significant interspecies interactions were observed between Candidatus Kuenenia(dominant anammox bacteria in CWs)and species within the genera Chitinivibrio-nia and Anaerolineaceae,suggesting that microbial interactions primarily manifest as indirect facilitative effects rather than direct mutualistic relationships.Given that the Normalized Stochasticity Ratio in CWs were<50%,this study inferred that environmental gradients have greater influence on anammox bacteria than microbial interactions.展开更多
Oil-fired construction machinery(OCM)is a major source of urban air pollutants and CO_(2) emissions,and elec-trification is a crucial pathway for improving air quality and achieving China’s dual carbon goals;however,...Oil-fired construction machinery(OCM)is a major source of urban air pollutants and CO_(2) emissions,and elec-trification is a crucial pathway for improving air quality and achieving China’s dual carbon goals;however,its feasibility has not been fully explored.This study uses data envelopment analysis and the analytic hierarchy process to establish a development potential index,covering technical efficiency,economic cost,application sce-narios,and charging time and range,with an empirical analysis conducted in Beijing.The findings indicated the high feasibility of replacing OCM with electric alternatives,especially within the low-power range.Based on 2023 registered coding dat1,it is projected that by 2030,electrification could reduce regional average con-centrations of CO,NO_(x),PM_(2.5) and VOCs by 12.2%to 56.4%and reduce CO_(2) by 11.7%to 56.9%.Owing to economic considerations,small-and medium-sized machinery are particularly feasible for electrification.Key recommendations include prioritizing the electrification of forklifts,lifting platforms,and small-sized machinery in high-emission areas,particularly in central urban districts.Policies such as carbon taxes,carbon markets,and performance grading systems are suggested to incentivize electrification,along with expanding high-emission restriction zones and improving energy infrastructure to support widespread electrification.展开更多
Understanding Cd contamination in the soil-rice ecosystem and the underlying its threshold and interaction effects is crucial for controlling Cd pollution and ensuring food safety.Although the quantitative relationshi...Understanding Cd contamination in the soil-rice ecosystem and the underlying its threshold and interaction effects is crucial for controlling Cd pollution and ensuring food safety.Although the quantitative relationships between Cd and environmental variables have been extensively studied,the threshold and interaction effects of multi-source environmental variables remain largely unexplored.This study employs a combination of random forest analysis and a human health risk model to investigate the effects of variables on Cd levels in rice grains,with the goal of quantifying their contributions and elucidating their relationships.The results indicated that the 15 selected variables collectively explained 47.36%of the variation in Cd content,with the top three variables being soil pH,distance from industrial park,and soil Zn.The majority of variables exhibited threshold effects on Cd levels in rice grains.By visualizing the interaction between Soil pH,distance from industrial park,and soil Zn with Cd levels in rice,we demonstrate the threshold effects of them on Cd level in rice grains,thereby providing further insight into the variation observed.Furthermore,oral intake of rice has been identified as the primary route of human exposure,significantly contributing to overall exposure pathways.Understanding these interactions is crucial for gaining insights into the underlying processes driving Cd pollution and fostering sustainable development within the industry.Our findings underscore the crucial need to consider multiple environmental variables and their interactions when managing heavy metals(HMs)contamination and mitigating health risks.展开更多
Despite intensive research on solar-driven photocatalytic overall water splitting(POWS),the overall efficiencies remain insufficient to meet commercial standards.As a central challenge in realizing this technology mai...Despite intensive research on solar-driven photocatalytic overall water splitting(POWS),the overall efficiencies remain insufficient to meet commercial standards.As a central challenge in realizing this technology mainly lies in the precise tuning and rational designing of highly efficient materials and photocatalytic systems,which is paramount for its unlocking scalable,practical applications.However,novel materials fabrication and advanced photocatalytic systems are essential for overcoming intrinsic limitations of conventional catalysts by enabling this green technology to resolve global energy crisis.Therefore,this review critically explores the engineering developments in POWS process and novel photocatalyst designing,via shifting from simple bandgap engineering to more advanced charge carrier dynamics control via utilizing one/two-step photocatalytic excitation system,surface phase junctions i.e.,Z-scheme and S-scheme heterojunctions,surface modification,morphological tuning,and the role of co-catalysts,to control sluggish kinetics,promote oxygen evolution reaction(OER)and suppress undesirable H2/O2,backward reaction with superior visible light absorption capacity to produce remarkable energy production.Moreover,we critically discuss the recent trend of POWS from a materials discovery phase to demanding engineering and mechanistic optimization phase with viable economic viability,which requires bridging the gap between excellent lab-scale performance to stringent stability,cost,and high efficiency demands of industrial-scale solar fuel production.In addition,the currents challenges and future directions are also enclosed in detail for sustainable energy production.展开更多
Exploring hydroclimatic variability and its driving mechanisms during the Holocene is essential for comprehending both historical and prospective responses of water resources to climatic shifts in Arid Central Asia(AC...Exploring hydroclimatic variability and its driving mechanisms during the Holocene is essential for comprehending both historical and prospective responses of water resources to climatic shifts in Arid Central Asia(ACA)region.However,debate persists regarding whether dryland lakes in this region exhibited aridification or humidification during the Holocene.Lopnur serves as the terminal lake of Tarim rivers during the Holocene,which offers an ideal natural laboratory to address the questions.In this study,a high-resolution chronological framework was established through precise radiocarbon dating.Multi-proxy analyses,including geochemical composition,grain size distributions,MS,LOI,and C/N ratios were conducted from a lacustrine profile in the core area of“Great ear”in the southern part of Lopnur catchment.These analyses enabled the reconstruction of hydrological dynamics and facilitated the disentanglement of independent signals linked to climate variability,runoff fluctuations,and lake-level changes.The results demonstrate that the MidHolocene(7800–4000 cal yr B.P.)was characterized by cold and humid conditions,resulting in elevated surface runoff and lake level.The Late Holocene(4000–1300 cal yr B.P.)experienced intensified aridification,characterized by reduced runoff and declining lake level.These evidences suggested a climatic regime of a distinctive alternation between“cold-wet”and“warm-dry”climatic regimes during the Mid-to-Late Holocene.Compared with the previous studies from adjacent regions,we speculate that the hydroclimatic evolution of Lopnur catchment possibly influenced by a complex interplay of large spatial scale forcings,including variations in annual insolation,greenhouse gas concentrations,and ice sheets,as well as the localized controls such as topographic features,vegetation cover,and cloud-radiative feedbacks.Our findings enhance the understanding of past climatic complexity and provide valuable insights for future water resource management strategies in drylands.展开更多
This study investigates the facies development and sedimentology of the Late Permian Chhidru Formation,a mixed carbonate-siliciclastic unit exposed in the Western Salt Range,Potwar Basin,Pakistan.The formation is subd...This study investigates the facies development and sedimentology of the Late Permian Chhidru Formation,a mixed carbonate-siliciclastic unit exposed in the Western Salt Range,Potwar Basin,Pakistan.The formation is subdivided into four lithological units reflecting lateral variability,with thicknesses and lithologies ranging from fossiliferous sandy limestone to interbedded limestone and sandstone.These successions record a depositional shift from a carbonate platform to mixed carbonate-clastic,and ultimately,clastic-dominated environments.Lithostratigraphy suggests deposition on the underlying Wargal Limestone carbonates during a Late Permian sea-level fall on the northwest Indian margin of Gondwana.Similar Permian successions with identical lithological characteristics are documented in the Persian Gulf(Dalan Formation),Arabian Platform(Khuff Formation),and Iran(Nesen and Hambust formations).Petrographic analysis reveals deposition in the distal middle to proximal inner shelf settings of a carbonate-siliciclastic mixed,unrimmed platform.Based on identified foraminiferal assemblages,the Chhidru Formation's age is estimated to range from the late Wuchiapingian to Changhsingian stages of the Lopingian epoch.展开更多
Understanding spatial patterns of plant species diversity and the factors(e.g.,climate and human)that drive these patterns is essential for biodiversity conservation.We used data from 1700.1-ha forest plots in the She...Understanding spatial patterns of plant species diversity and the factors(e.g.,climate and human)that drive these patterns is essential for biodiversity conservation.We used data from 1700.1-ha forest plots in the Shettihalli tropical forest landscape of the Western Ghats biodiversity hotspot,India,to analyse tree community composition and the drivers of α-diversity(Shannon)andβ-diversity(LCBD).Compositional patterns were visualized using Non-Metric Multidimensional Scaling(NMDS),and hybrid feature selection with structural equation modeling(SEM)was employed to evaluate the direct and indirect effects of environmental variables on diversity.NMDS identified four distinct forest types in the Shettihalli landscape:semi-evergreen,dry deciduous,moist deciduous,and plantation forests,each with distinct plant composition.Shannon diversity and ecological uniqueness was significantly higher in semi-evergreen forest than in deciduous forest plots.The SEMs explained about 79%and 39–45%of the variation in α-diversity andβ-diversity.Our analysis indicated that current diversity patterns result from multiple processes,with structure,disturbance,and edaphic parameters exerting the strongest direct and indirect effects onα-diversity.β-diversity,in contrast,was largely influenced by climate,topography,stand structure,and edaphic factors.Overall,our findings indicate that various factors(e.g.,climate,topography,and human disturbance)interact to shape tree diversity patterns in tropical forests.These findings will help develop unique conservation and management strategies for distinct forest types in tropical forest ecosystems.展开更多
The integration of machine learning(ML)into geohazard assessment has successfully instigated a paradigm shift,leading to the production of models that possess a level of predictive accuracy previously considered unatt...The integration of machine learning(ML)into geohazard assessment has successfully instigated a paradigm shift,leading to the production of models that possess a level of predictive accuracy previously considered unattainable.However,the black-box nature of these systems presents a significant barrier,hindering their operational adoption,regulatory approval,and full scientific validation.This paper provides a systematic review and synthesis of the emerging field of explainable artificial intelligence(XAI)as applied to geohazard science(GeoXAI),a domain that aims to resolve the long-standing trade-off between model performance and interpretability.A rigorous synthesis of 87 foundational studies is used to map the intellectual and methodological contours of this rapidly expanding field.The analysis reveals that current research efforts are concentrated predominantly on landslide and flood assessment.Methodologically,tree-based ensembles and deep learning models dominate the literature,with SHapley Additive exPlanations(SHAP)frequently adopted as the principal post-hoc explanation technique.More importantly,the review further documents how the role of XAI has shifted:rather than being used solely as a tool for interpreting models after training,it is increasingly integrated into the modeling cycle itself.Recent applications include its use in feature selection,adaptive sampling strategies,and model evaluation.The evidence also shows that GeoXAI extends beyond producing feature rankings.It reveals nonlinear thresholds and interaction effects that generate deeper mechanistic insights into hazard processes and mechanisms.Nevertheless,several key challenges remain unresolved within the field.These persistent issues are especially pronounced when considering the crucial necessity for interpretation stability,the demanding scholarly task of reliably distinguishing correlation from causation,and the development of appropriate methods for the treatment of complex spatio-temporal dynamics.展开更多
基金supported by the National Natural Science Foundation of China(Nos.42077299,and U21A20290)the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDB0750400)the Ordos Key Research and Development Program(No.YF20240037).
文摘Persistent toxic substances(PTS)represent a paramount environmental issue in the 21st century.Understanding the concentrations and forms of PTS in the environment is crucial for accurately assessing their environmental health impacts.This article presents a concise overview of the components of PTS,pertinent environmental regulations,and conventional detection methodologies.Additionally,we offer an in-depth review of the principles,development,and practical applications of surface-enhanced Raman scattering(SERS)in environmental monitoring,emphasizing the advancements in detecting trace amounts of PTS in complex environmental matrices.Recent progress in enhancing SERS sensitivity,improving selectivity,and practical implementations are detailed,showcasing innovative materials and methods.Integrating SERS with advanced algorithms are highlighted as pivotal areas for future research.
文摘The authors regret that in 1.2.Instruments section of the article,when describing the principle of TiH300,the original content of“Briefly,ambient HONO was first absorbed by deionized water in a two-channel stripping coil.The absorbed liquid nitrite was mixed with sulfanilamide,N-(1-naphthyl)-ethylenediamine dihydrochloride,and hydrogen chloride solution to form the azo dye derivative.”
基金JES is financially supported by the National Nature Science Foundation of China (No.21024806,21224005)the Publishing Foundation of Chinese Academy of Sciences (the year of 2009,2010,2011)
文摘1 Initial construction of JESTwenty years ago, research on environmental science was extended beyond its initial scope including pollution source surveys, environmental pollution monitoring, and treatment of the ＂three wastes＂ （waste water, waste gas, and solid waste） to a full concern with the behavior, tendencies and harmful effects of pollutants in the environment as well as the overall understanding of the ecosystem. Environmental scientists came to realize that the solutions to environmental problems and their fields of study could no longer be restricted to a particular region or country, but needed exchanges with foreign scholars and transnational cooperation between scientists. However, at that time,
基金This work was supported by the National Natural Science Foundation of China(Grant No.L1924041)Research Project on the Discipline Development Strategy of Academic Divisions of the Chinese Academy of Sciences(Grant No.XK2019DXC006).
文摘Environmental science is an interdisciplinary science developed in the process of understanding and solving ecolog-ical and environmental problems.In order to tackle these problems,environmental science research is expected to reveal the source,behavior,fate,exposure,and risks of pollutants in the environment and develop potential solutions to control pollution.It provides the scientific basis for decision-makers to establish environmental and economic poli-cies,and promote concerted efforts for the sustainable development of society.Here,we articulate the development patterns,challenges,and future research needs of environmental science in China based on literature review and expert panel discussion.Environmental science research has evolved significantly in the past decade with an increas-ing diversity of environmental pollutants and health impacts,new technologies and methods,deepening fusion of multiple disciplines,and emerging solutions for pollution control.Its future development relies on the advances in our knowledge on the fate and transport of pollutants,regional environmental processes,ecotoxicological effects,environmental exposure and health effects,environmental analysis and monitoring,source control and reduction,environmental remediation,as well as environmental risk management.For each of these fields,we summarize the significant challenges and highlight the research demands for China.Based on the status quo of China’s environmen-tal science research and future needs,we provide recommendations to promote its future development,including encouraging innovation and interdisciplinary research,providing decision support for national needs,encouraging international collaboration,and improving collaboration mechanisms.
文摘This paper reviews the major contributions made by Norwegian scientists to Arctic environmental sciences since the 1880s. The review begins with the first International Polar Year （IPY） in 1882-83. It then considers the 1890s to 1920s with the scientific expeditions focusing on ocean and sea ice conditions of Nansen, Amundsen and H. Sverdrup, and the mapping of the Queen Elizabeth Islands by Otto Sverdrup and colleagues. The period from 1911 to the mid-1920s also witnessed annual expeditions to Svalbard led by Adolf Hoel. The 1930s to 1945 period encompassed the Second International Polar Year when Arctic weather stations were established or maintained. The time interval post-World War II to 2000 witnessed major advances made possible by technical and organizational innovations. The establishment of the Norwegian Polar Institute in 1948 led to extensive research on the glaciers and snow cover in the Svalbard archipelago and to oceanographic and sea ice research in the Barents Sea and Arctic Ocean. Remote sensing methods began to be widely used from the 1980s. The new millennium saw the undertaking of the third IPY and a shift to multinational projects. New fields such as ocean-ice-atmosphere variability became active and there was much attention to high-latitude climate change in the context of global warming.
文摘First of all, it is my honor to announce that Professor X. Chris Le has been appointed the Editor-in-Chief of Journal of Environmental Sciences （JES） after an international search and selection by the committee members of the Research Center of Eco-environmental Sciences, Chinese Academy of Sciences. Professor Hongxiao Tang,
基金support in the literature analysis.This study has been carried out in the framework of the project funded by EU entitled“Bioremediation of contaminated sediments in coastal areas of exindustrial sites-LIFE SEDREMED”(No.LIFE20 ENV/IT/000572).
文摘This study compares the environmental sustainability of five alternatives for the remediation of marine sediments of one of the most polluted coastal sites in Europe(Bagnoli-Coroglio bay,Mediterranean Sea),using the Life Cycle Assessment(LCA)methodology.The treatments are either in-situ or exsitu,the latter requiring an initial dredging to transport the contaminated sediments to the management site.More in detail,four ex-situ remediation technologies based on landfilling,bioremediation,electrokinetic technique and soil washing were identified.These technologies are compared to an in-situ strategy currently under validation for enhancing bioremediation of the polluted sediments of the Bagnoli-Coroglio site.Our results indicate that the disposal in landfilling site is the worst option in most categories(e.g.,650 kg CO_(2) eq./t of treated sediment,considering the nearest landfilling site),followed by the bioremediation,mainly due to the high energy demand.Electrokinetic remediation,soil washing,and innovative in-situ technology represent the most sustainable options.In particular,the new in-situ technology appears to be the least impacting in all categories(e.g.,54 kg CO_(2) eq./t of treated sediment),although it is expected to require longer treatment time(estimated up to 12 months based on its potential efficiency).It can reduce the impact on climate change more than 12 times compared to the disposal and 7 times compared to bioremediation in addition to the possibility to avoid/reduce the dredging operations and the consequent dispersion of pollutants.The results open relevant perspectives towards more eco-sustainable and costly effective actions for the reclamation of contaminated marine sediments.
基金supported by the National Natural Science Foundation of China(32360084).
文摘In recent years,intensified land use change driven by climate change and human activities have markedly impacted the ecological environmental quality of the arid inland river basins.The implementation of forestry projects,coupled with continuous population growth,has increased the need for systematic assessments of ecological effects to ensure sustainable development in arid inland river basins.This study generated a 22-a(2000-2021)remote sensing ecological index(RSEI)data series for the Manas River Basin,a typical arid inland river basin in China,utilizing Moderate Resolution Imaging Spectroradiometer(MODIS)data and the Google Earth Engine(GEE)platform.We examined the spatiotemporal patterns of ecological environmental quality in the Manas River Basin through the Theil-Sen estimator,Mann-Kendall trend test,coefficient of variation(CV),and Hurst index.Furthermore,we employed the Optimal Parameter-based Geographical Detector(OPGD)method to quantify the influence of seven key drivers:elevation,slope,temperature,precipitation,gross domestic product(GDP),population density,and land use change.The key findings revealed that the basin's ecological environmental quality showed significant improvement(mean RSEI of 0.38,with a range of 0.34-0.41),with areas exhibiting good and excellent grades increasing by 16.71%,particularly in the midstream oasis region and upstream mountainous region,while areas exhibiting poor and relatively poor grades decreased by 11.52%in the downstream desert region.Spatial heterogeneity of ecological environmental quality was pronounced,with 32.23%of the areas showing localized degradation,the midstream oasis region exhibiting sustainable recovery potential(Hurst index>0.50),and only 36.67%of the areas maintaining stable and highly stable conditions(primarily in the upstream mountainous region).The OPGD analysis revealed that temperature(q-value=0.496-0.780),land use change(q-value=0.705-0.782),and elevation(q-value=0.245-0.637)were dominant factors,with the influence of land use change increasing during 2000-2020.Strong interaction effects emerged between land use change and temperature(q-value>0.705)and between land use change and elevation(q-value=0.751 in 2020),highlighting intensified human-nature coupling.These findings provide vital perspectives for ecosystem management in arid inland river basins under both climate and anthropogenic pressures.
基金supported by the Key Research and Development Program of Gansu Province(22YF7FA070)the National Natural Science Foundation of China(22406076,22466026)the Basic Research Project of Yunnan Province(202301BE070001-017,202401CF070139,202401AS070085)。
文摘Iron and steel industry is one of the main sources of air pollution emissions in China.The sintering process is an important link in the blast furnace ironmaking process,but it is also accompanied by a large number of pollutants.Under the background of ultra-low emissions,iron and steel enterprises urgently need to upgrade their existing processes to address the existing process in practical application problems.In this study,a steel group in Gansu Province was taken as an example.By comparing and analyzing the pollutant emission characteristics before and after the ultra-low emission retrofit,the collaborative control effect of the combined process on SO_(2),NO_(x),particulate matter,and dioxins after the new retrofit was systematically evaluated.The results show that after the retrofit,the concentrations of particulate matter,SO_(2) and NO_(x) have dropped to near-zero levels,and the dioxin removal efficiency has reached 98.87%,with all indicators being better than the national ultra-low emission standards.The study confirms that the optimal combination of multi-pollutant collaborative treatment technologies is the key to achieving efficient emission reduction,among which selective catalytic reduction technology has a particularly significant synergistic removal effect on NO_(x) and dioxins.This study provides an important technical reference and practical basis for the ultra-low emission retrofit of the steel industry,and has important guiding significance for promoting the green retrofit of the industry.Its ultra-low emission retrofit is of great significance for achieving green and low-carbon development.
基金funded by the National Natural Science Foundation of China(Grant No.42461038 and No.42161043).
文摘The Gansu-Qinghai contiguous region of the upper Yellow River is located in the transition zone between the Loess Plateau and the Qinghai-Tibet Plateau,characterized by fragile ecosystems and high sensitivity to climate change.As a critical ecological security barrier and water conservation area,it faces persistent tensions between development demands and ecological protection.Quantitative assessments of how production-living-ecological space(PLES)evolution affects ecological and environmental quality(EEQ)under long-term,multi-scenario conditions remain limited in such vulnerable regions.Understanding PLES-EEQ relationships is essential for optimizing territorial spatial planning and maintaining ecological security in the Yellow River basin.This study utilized land use data from 2000 to 2020 and the FLUS model to simulate PLES evolution from 2030 to 2060 under SSP1,SSP2,and SSP5 scenarios.The analytical framework integrated artificial neural networks and cellular automata with Shared Socioeconomic Pathways to project spatial configurations and assess EEQ in 2035.Living space expanded across all three scenarios while ecological space decreased.Production space increased by 125 km^(2) under SSP5 but declined in other scenarios.The EEQ index in 2035 showed improvements relative to the baseline value(0.4130)in 2020.Medium-to-high quality areas were primarily grassland and forest,whereas low-quality areas consisted mainly of unused land concentrated in the central and western regions.This study reveals a nonlinear relationship between ecological space quantity and quality,showing that structural optimization can enhance EEQ despite area reduction.The findings suggest that strengthening ecological protection redlines and restraining urban expansion are essential for territorial spatial optimization in ecologically fragile regions.
基金supported by Natural Science Foundation of Xiamen,China(No.3502Z20227232)the STS Project of Fujian-CAS(No.2023T3018)Bureau of International Cooperation,Chinese Academy of Sciences(No.322GJHZ2022035MI).
文摘Anammox bacteria in constructed wetlands(CWs)play pivotal role in sustainable nitrogen transformation,yet existing studies lack comprehensive analysis of environmental gradients and microbial interactions,both key factors in anammox bacteria enrichment.This study investigated the mechanisms driving anammox bacteria enrichment in lab-scale simulated CWs treating high-nitrogen wastewater,focusing on bacterial community re-sponses across wetland layers with various strategies,including continuous up-flow influent,nitrogen loading increase,effluent recirculation,intermittent influent,and anammox bacteria inoculation.Results showed that total relative and absolute abundances of anammox bacteria ranged from 0.77%to 12.50%and from 0.13 to 6.46×10^(7) copies/g,respectively.Dissolved oxygen and pH had significant positive correlations with the absolute abundance of anammox bacteria,while organic matter and nitrate negatively impacted their relative abundance.Permutational multivariate analysis of variance indicated that spatial heterogeneity explained more variation in anammox bacteria abundance(43.44%)compared to operational strategies(8.58%).In terms of microbial interactions,60 dominant species exhibited potential correlations with anammox bacteria,comprising 170 interactions(105 positive and 65 negative),which suggested that anammox bacteria generally foster cooperative relationships with dominant bacteria.Notably,significant interspecies interactions were observed between Candidatus Kuenenia(dominant anammox bacteria in CWs)and species within the genera Chitinivibrio-nia and Anaerolineaceae,suggesting that microbial interactions primarily manifest as indirect facilitative effects rather than direct mutualistic relationships.Given that the Normalized Stochasticity Ratio in CWs were<50%,this study inferred that environmental gradients have greater influence on anammox bacteria than microbial interactions.
基金supported by the National Science and Technology Major Project of the Ministry of Science and Technology of China(No.2024ZD1200200).
文摘Oil-fired construction machinery(OCM)is a major source of urban air pollutants and CO_(2) emissions,and elec-trification is a crucial pathway for improving air quality and achieving China’s dual carbon goals;however,its feasibility has not been fully explored.This study uses data envelopment analysis and the analytic hierarchy process to establish a development potential index,covering technical efficiency,economic cost,application sce-narios,and charging time and range,with an empirical analysis conducted in Beijing.The findings indicated the high feasibility of replacing OCM with electric alternatives,especially within the low-power range.Based on 2023 registered coding dat1,it is projected that by 2030,electrification could reduce regional average con-centrations of CO,NO_(x),PM_(2.5) and VOCs by 12.2%to 56.4%and reduce CO_(2) by 11.7%to 56.9%.Owing to economic considerations,small-and medium-sized machinery are particularly feasible for electrification.Key recommendations include prioritizing the electrification of forklifts,lifting platforms,and small-sized machinery in high-emission areas,particularly in central urban districts.Policies such as carbon taxes,carbon markets,and performance grading systems are suggested to incentivize electrification,along with expanding high-emission restriction zones and improving energy infrastructure to support widespread electrification.
基金supported by the GDAS’Project of Science and Technology Development(No.2022GDASZH-2022010104-2)Guangdong Major Project of Basic and Applied Basic Research(No.2023B0303000006).
文摘Understanding Cd contamination in the soil-rice ecosystem and the underlying its threshold and interaction effects is crucial for controlling Cd pollution and ensuring food safety.Although the quantitative relationships between Cd and environmental variables have been extensively studied,the threshold and interaction effects of multi-source environmental variables remain largely unexplored.This study employs a combination of random forest analysis and a human health risk model to investigate the effects of variables on Cd levels in rice grains,with the goal of quantifying their contributions and elucidating their relationships.The results indicated that the 15 selected variables collectively explained 47.36%of the variation in Cd content,with the top three variables being soil pH,distance from industrial park,and soil Zn.The majority of variables exhibited threshold effects on Cd levels in rice grains.By visualizing the interaction between Soil pH,distance from industrial park,and soil Zn with Cd levels in rice,we demonstrate the threshold effects of them on Cd level in rice grains,thereby providing further insight into the variation observed.Furthermore,oral intake of rice has been identified as the primary route of human exposure,significantly contributing to overall exposure pathways.Understanding these interactions is crucial for gaining insights into the underlying processes driving Cd pollution and fostering sustainable development within the industry.Our findings underscore the crucial need to consider multiple environmental variables and their interactions when managing heavy metals(HMs)contamination and mitigating health risks.
基金the Taizhou University,Zhejiang,China for funding(No.T20250101215)the Deanship of research and Graduate Studies at King Khalid University for funding this work through Large Research Project(R.G.P.2/398/46).
文摘Despite intensive research on solar-driven photocatalytic overall water splitting(POWS),the overall efficiencies remain insufficient to meet commercial standards.As a central challenge in realizing this technology mainly lies in the precise tuning and rational designing of highly efficient materials and photocatalytic systems,which is paramount for its unlocking scalable,practical applications.However,novel materials fabrication and advanced photocatalytic systems are essential for overcoming intrinsic limitations of conventional catalysts by enabling this green technology to resolve global energy crisis.Therefore,this review critically explores the engineering developments in POWS process and novel photocatalyst designing,via shifting from simple bandgap engineering to more advanced charge carrier dynamics control via utilizing one/two-step photocatalytic excitation system,surface phase junctions i.e.,Z-scheme and S-scheme heterojunctions,surface modification,morphological tuning,and the role of co-catalysts,to control sluggish kinetics,promote oxygen evolution reaction(OER)and suppress undesirable H2/O2,backward reaction with superior visible light absorption capacity to produce remarkable energy production.Moreover,we critically discuss the recent trend of POWS from a materials discovery phase to demanding engineering and mechanistic optimization phase with viable economic viability,which requires bridging the gap between excellent lab-scale performance to stringent stability,cost,and high efficiency demands of industrial-scale solar fuel production.In addition,the currents challenges and future directions are also enclosed in detail for sustainable energy production.
基金supported by the National Natural Science Foundation of China(No.42001084)the Major Science and Technology Projects of Xinjiang Uygur Autonomous Region(Nos.2022A03009-2,2022A03009)the Third Xinjiang Scientific Expedition Program(No.2022xjkk1303)。
文摘Exploring hydroclimatic variability and its driving mechanisms during the Holocene is essential for comprehending both historical and prospective responses of water resources to climatic shifts in Arid Central Asia(ACA)region.However,debate persists regarding whether dryland lakes in this region exhibited aridification or humidification during the Holocene.Lopnur serves as the terminal lake of Tarim rivers during the Holocene,which offers an ideal natural laboratory to address the questions.In this study,a high-resolution chronological framework was established through precise radiocarbon dating.Multi-proxy analyses,including geochemical composition,grain size distributions,MS,LOI,and C/N ratios were conducted from a lacustrine profile in the core area of“Great ear”in the southern part of Lopnur catchment.These analyses enabled the reconstruction of hydrological dynamics and facilitated the disentanglement of independent signals linked to climate variability,runoff fluctuations,and lake-level changes.The results demonstrate that the MidHolocene(7800–4000 cal yr B.P.)was characterized by cold and humid conditions,resulting in elevated surface runoff and lake level.The Late Holocene(4000–1300 cal yr B.P.)experienced intensified aridification,characterized by reduced runoff and declining lake level.These evidences suggested a climatic regime of a distinctive alternation between“cold-wet”and“warm-dry”climatic regimes during the Mid-to-Late Holocene.Compared with the previous studies from adjacent regions,we speculate that the hydroclimatic evolution of Lopnur catchment possibly influenced by a complex interplay of large spatial scale forcings,including variations in annual insolation,greenhouse gas concentrations,and ice sheets,as well as the localized controls such as topographic features,vegetation cover,and cloud-radiative feedbacks.Our findings enhance the understanding of past climatic complexity and provide valuable insights for future water resource management strategies in drylands.
基金Dr.Stergios D.Zarkogiannis would like to acknowledge UK Research and Innovation Grant(SODIOM)EP/Y004221/1 in supporting the research reported here.
文摘This study investigates the facies development and sedimentology of the Late Permian Chhidru Formation,a mixed carbonate-siliciclastic unit exposed in the Western Salt Range,Potwar Basin,Pakistan.The formation is subdivided into four lithological units reflecting lateral variability,with thicknesses and lithologies ranging from fossiliferous sandy limestone to interbedded limestone and sandstone.These successions record a depositional shift from a carbonate platform to mixed carbonate-clastic,and ultimately,clastic-dominated environments.Lithostratigraphy suggests deposition on the underlying Wargal Limestone carbonates during a Late Permian sea-level fall on the northwest Indian margin of Gondwana.Similar Permian successions with identical lithological characteristics are documented in the Persian Gulf(Dalan Formation),Arabian Platform(Khuff Formation),and Iran(Nesen and Hambust formations).Petrographic analysis reveals deposition in the distal middle to proximal inner shelf settings of a carbonate-siliciclastic mixed,unrimmed platform.Based on identified foraminiferal assemblages,the Chhidru Formation's age is estimated to range from the late Wuchiapingian to Changhsingian stages of the Lopingian epoch.
基金supported by the Department of Biotechnology,Ministry of Science and Technology,Govt.India,under grant No.BT/Coord.Ⅱ/10/02/2016/22.03.2018the Indian Council of Social Science Research,New Delhi,India,for providing a short-term doctoral fellowship(RFD/Short-Term/2022-23/ENV/ST/66)。
文摘Understanding spatial patterns of plant species diversity and the factors(e.g.,climate and human)that drive these patterns is essential for biodiversity conservation.We used data from 1700.1-ha forest plots in the Shettihalli tropical forest landscape of the Western Ghats biodiversity hotspot,India,to analyse tree community composition and the drivers of α-diversity(Shannon)andβ-diversity(LCBD).Compositional patterns were visualized using Non-Metric Multidimensional Scaling(NMDS),and hybrid feature selection with structural equation modeling(SEM)was employed to evaluate the direct and indirect effects of environmental variables on diversity.NMDS identified four distinct forest types in the Shettihalli landscape:semi-evergreen,dry deciduous,moist deciduous,and plantation forests,each with distinct plant composition.Shannon diversity and ecological uniqueness was significantly higher in semi-evergreen forest than in deciduous forest plots.The SEMs explained about 79%and 39–45%of the variation in α-diversity andβ-diversity.Our analysis indicated that current diversity patterns result from multiple processes,with structure,disturbance,and edaphic parameters exerting the strongest direct and indirect effects onα-diversity.β-diversity,in contrast,was largely influenced by climate,topography,stand structure,and edaphic factors.Overall,our findings indicate that various factors(e.g.,climate,topography,and human disturbance)interact to shape tree diversity patterns in tropical forests.These findings will help develop unique conservation and management strategies for distinct forest types in tropical forest ecosystems.
文摘The integration of machine learning(ML)into geohazard assessment has successfully instigated a paradigm shift,leading to the production of models that possess a level of predictive accuracy previously considered unattainable.However,the black-box nature of these systems presents a significant barrier,hindering their operational adoption,regulatory approval,and full scientific validation.This paper provides a systematic review and synthesis of the emerging field of explainable artificial intelligence(XAI)as applied to geohazard science(GeoXAI),a domain that aims to resolve the long-standing trade-off between model performance and interpretability.A rigorous synthesis of 87 foundational studies is used to map the intellectual and methodological contours of this rapidly expanding field.The analysis reveals that current research efforts are concentrated predominantly on landslide and flood assessment.Methodologically,tree-based ensembles and deep learning models dominate the literature,with SHapley Additive exPlanations(SHAP)frequently adopted as the principal post-hoc explanation technique.More importantly,the review further documents how the role of XAI has shifted:rather than being used solely as a tool for interpreting models after training,it is increasingly integrated into the modeling cycle itself.Recent applications include its use in feature selection,adaptive sampling strategies,and model evaluation.The evidence also shows that GeoXAI extends beyond producing feature rankings.It reveals nonlinear thresholds and interaction effects that generate deeper mechanistic insights into hazard processes and mechanisms.Nevertheless,several key challenges remain unresolved within the field.These persistent issues are especially pronounced when considering the crucial necessity for interpretation stability,the demanding scholarly task of reliably distinguishing correlation from causation,and the development of appropriate methods for the treatment of complex spatio-temporal dynamics.
