High-resolution spectroscopy unveils the fundamental physics of quantum states,molecular dynamics,and energy transfers.Ideally,a higher spectral resolution over a broader bandwidth is the prerequisite,but traditional ...High-resolution spectroscopy unveils the fundamental physics of quantum states,molecular dynamics,and energy transfers.Ideally,a higher spectral resolution over a broader bandwidth is the prerequisite,but traditional spectroscopic techniques can only partially fulfill this requirement even with a bulky system.Here we report that a multi-frequency acousto-optic phase modulation at a chip-scale of soft polydimethylsiloxane can readily support a 200-times higher 0.5-MHz spectral resolution for the frequency-comb-based spectroscopy,while co-located plasmonic nanostructures mediate the strong light-matter interaction.These results suggest the potential of polydimethylsiloxane acousto-optic phase modulation for cost-effective,compact,multifunctional chip-scale tools in diverse applications such as quantum spectroscopy,high-finesse cavity analysis,and surface plasmonic spectroscopy.展开更多
基金supported by BrainLink program funded by the Ministry of Science and ICT through the National Research Foundation of Korea(RS-2023-00236798)BK21 FOUR Program by Pusan National University Research Grant,2021+1 种基金This work was supported by the National Research Foundation(NRF)grant funded by the Korean government(RS-2024-00336583)the Korea government(MSIT)(No.RS-2024-00406152).
文摘High-resolution spectroscopy unveils the fundamental physics of quantum states,molecular dynamics,and energy transfers.Ideally,a higher spectral resolution over a broader bandwidth is the prerequisite,but traditional spectroscopic techniques can only partially fulfill this requirement even with a bulky system.Here we report that a multi-frequency acousto-optic phase modulation at a chip-scale of soft polydimethylsiloxane can readily support a 200-times higher 0.5-MHz spectral resolution for the frequency-comb-based spectroscopy,while co-located plasmonic nanostructures mediate the strong light-matter interaction.These results suggest the potential of polydimethylsiloxane acousto-optic phase modulation for cost-effective,compact,multifunctional chip-scale tools in diverse applications such as quantum spectroscopy,high-finesse cavity analysis,and surface plasmonic spectroscopy.
