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Analysis of atmospheric pollutant characteristics and regional transport in coastal area along the East China Sea
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作者 Yangzhou Wu Dantong Liu +5 位作者 Honghui Xu Meng Shan Siyuan Li Ping Tian Kang Hu Junfeng Wang 《Journal of Environmental Sciences》 2025年第10期225-238,共14页
PM_(2.5) and black carbon(BC)are important air pollutants impacting radiation balance,air quality,health,and ecosystems.Ozone(O_(3))levels are increasing despite decreases in other pollutants,posing a challenge for po... PM_(2.5) and black carbon(BC)are important air pollutants impacting radiation balance,air quality,health,and ecosystems.Ozone(O_(3))levels are increasing despite decreases in other pollutants,posing a challenge for pollution control,especially in coastal cities like Zhoushan,where the monsoonal climate can exacerbate PM_(2.5) and ozone pollution.This study conducted continuous online measurements of major atmospheric pollutants in Zhoushan,Zhejiang Province,in 2020.The results indicate that the highest contribution from local air masses in Zhoushan is observed in spring,accounting for 17.7%,while the greatest average contribution from northern Zhejiang Province,Jiangsu Province,and Shanghai occurs in winter,at 18.5%.Pollutant concentrationswere seasonally variable,with PM_(2.5),BC,and sulfur dioxide concentrations 56.6%,36%,and 58.2%higher in the cold season compared to the warm season.The O_(3) in spring is approximately 50%higher than that in summer.Ship emissions significantly contributed to BC,nitrogen oxides(NO_(x)),and carbon monoxide in Zhoushan.In spring,PM_(2.5) sources included photochemical processes and northern air mass transport,while in winter,PM_(2.5) was due to regional transport.The inhibitory effect of PM_(2.5) on O_(3) formation in the Zhoushan area is relatively weak.Reducing NO_(x) emissions may increase O_(3),emphasizing the need for volatile organic compounds monitoring and regional control measures to improve air quality and ensure sustainable development in Zhoushan. 展开更多
关键词 Coastal city PM_(2.5) OZONE Black carbon Ship emission Seasonal variation
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Interannual modulation of summer precipitation over North China by the coupled tropical Pacific-Atlantic SST Dipole Mode
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作者 Yanjin Mao Xiaorui Niu +3 位作者 Ping Li Xianchun Chen Libin Huang Xin Tan 《Atmospheric and Oceanic Science Letters》 2026年第1期1-6,共6页
Using multi-source reanalysis data,this study examines the relationship between the tropical Pacific-Atlantic SST Dipole Mode(TPA-DM)and summer precipitation in North China(NCSP)on the interannual timescale during the... Using multi-source reanalysis data,this study examines the relationship between the tropical Pacific-Atlantic SST Dipole Mode(TPA-DM)and summer precipitation in North China(NCSP)on the interannual timescale during the period of 1979-2022.The results show that the TPA-DM,the dominant pattern of interannual variability in the tropical Pacific and Atlantic regions,exhibits a significant negative correlation with NCSP.The positive phase of TPA-DM induces subsidence over the Maritime Continent through a zonal circulation pattern,which initiates a Pacific-Japan-like wave train along the East Asian coast.The circulation anomalies lead to moisture deficits and convergence subsidence over North China,leading to below-normal rainfall.Further analysis reveals that cooler SST in the Southern Tropical Atlantic facilitates the persistence of the TPA-DM by stimulating the anomalous Walker circulation associated with wind-evaporation-SST-convection feedback. 展开更多
关键词 Coupled tropical Pacific-Atlantic SST mode Precipitation ENSO Atmospheric teleconnection
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Performance of a Reconfigured Atmospheric General Circulation Model at Low Resolution 被引量:17
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作者 闻新宇 周天军 +3 位作者 王绍武 王斌 万慧 李建 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2007年第4期712-728,共17页
Paleoclimate simulations usually require model runs over a very long time. The fast integration version of a state-of-the-art general circulation model (GCM), which shares the same physical and dynamical processes b... Paleoclimate simulations usually require model runs over a very long time. The fast integration version of a state-of-the-art general circulation model (GCM), which shares the same physical and dynamical processes but with reduced horizontal resolution and increased time step, is usually developed. In this study, we configure a fast version of an atmospheric GCM (AGCM), the Grid Atmospheric Model of IAP/LASG (Institute of Atmospheric Physics/State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics), at low resolution (GAMIL-L, hereafter), and compare the simulation results with the NCEP/NCAR reanalysis and other data to examine its performance. GAMIL-L, which is derived from the original GAMIL, is a finite difference AGCM with 72 × 40 grids in longitude and latitude and 26 vertical levels. To validate the simulated climatology and variability, two runs were achieved. One was a 60-year control run with fixed climatological monthly sea surface temperature (SST) forcing, and the other was a 50-yr (1950-2000) integration with observational time-varying monthly SST forcing. Comparisons between these two cases and the reanalysis, including intra-seasonal and inter-annual variability are also presented. In addition, the differences between GAMIL-L and the original version of GAMIL are also investigated.The results show that GAMIL-L can capture most of the large-scale dynamical features of the atmosphere, especially in the tropics and mid latitudes, although a few deficiencies exist, such as the underestimated Hadley cell and thereby the weak strength of the Asia summer monsoon. However, the simulated mean states over high latitudes, especially over the polar regions, are not acceptable. Apart from dynamics, the thermodynamic features mainly depend upon the physical parameterization schemes. Since the physical package of GAMIL-L is exactly the same as the original high-resolution version of GAMIL, in which the NCAR Community Atmosphere Model (CAM2) physical package was used, there are only small differences between them in the precipitation and temperature fields. Because our goal is to develop a fast-running AGCM and employ it in the coupled climate system model of IAP/LASG for paleoclimate studies such as ENSO and Australia-Asia monsoon, particular attention has been paid to the model performances in the tropics. More model validations, such as those ran for the Southern Oscillation and South Asia monsoon, indicate that GAMIL-L is reasonably competent and valuable in this regard. 展开更多
关键词 GCM GAMIL-L ATMOSPHERE model validation
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RELATIONSHIP BETWEEN THE 30 TO 60 DAY OSCILLATION OF ATMOSPHERIC HEAT SOURCE AND THE DROUGHT AND FLOOD EVENTS IN JUNE IN THE SOUTH OF CHINA 被引量:2
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作者 高斯 简茂球 乔云亭 《Journal of Tropical Meteorology》 SCIE 2012年第3期332-340,共9页
Based on the NCEP/NCAR reanalysis data and the observed precipitation data in the south of China from 1958 to 2000,the impact of 30 to 60 day oscillation of atmospheric heat sources on the drought and flood events in ... Based on the NCEP/NCAR reanalysis data and the observed precipitation data in the south of China from 1958 to 2000,the impact of 30 to 60 day oscillation of atmospheric heat sources on the drought and flood events in June in the south of China is discussed.During the flood(drought) events,there exists an anomalous low-frequency anticyclone(cyclone) at the low level of the troposphere over the South China Sea and the northwestern Pacific,accompanied with anomalous low-frequency heat sinks(heat sources),while there exists an anomalous low-frequency cyclone(anticyclone) with anomalous heat sources(sinks) over the area from the south of China to the south of Japan.On average,the phase evolution of the low-frequency in drought events is 7 to 11 days ahead of that in flood events in May to June in the south of China.In flood events,low-frequency heat sources and cyclones are propagated northward from the southern South China Sea,northwestward from the warm pool of the western Pacific and westward from the northwestern Pacific around 140°E,which have very important impact on the abundant rainfall in June in the south of China.However,in drought events,the northward propagations of the low-frequency heat sources and cyclones from the South China Sea and its vicinity are rather late compared with those in flood events,and there is no obvious westward propagation of the heat sources from the northwestern Pacific.The timing of the low-frequency heat source propagation has remarkable impact on the June rainfall in the south of China. 展开更多
关键词 CLIMATOLOGY statistical feature atmospheric heat source 30-60 day oscillation flood and drought the south of China
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Atmospheric fine particles in a typical coastal port of Yangtze River Delta 被引量:4
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作者 Qi Yuan Xiaomi Teng +10 位作者 Shaoxuan Tu Binxin Feng Zhiyu Wu Hang Xiao Qiuliang Cai Yinxiao Zhang Qiuhan Lin Zhaoce Liu Mengmeng He Xiaokun Ding Weijun Li 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2020年第12期62-70,共9页
In recent decades, coastal ports have experienced rapid development and become an important economic and ecological hub in China. Atmospheric particle is a research hotspot in atmospheric environmental sciences in inl... In recent decades, coastal ports have experienced rapid development and become an important economic and ecological hub in China. Atmospheric particle is a research hotspot in atmospheric environmental sciences in inland regions. However, few studies on the atmospheric particle were conducted in coastal port areas in China, which indeed suffers atmospheric particle pollution. Lack of the physicochemical characteristics of fine particles serves as an obstacle toward the accurate control for air pollution in the coastal port area in China. Here, a field observation was conducted in an important coastal port city in Yangtze River Delta from March 6 to March 19, 2019. The average PM2.5 concentration was 63.7 ±27.8 μg/m^3 and NO3^-, SO4^2-, NH4^+, and organic matter accounted for ?60% of PM 2.5. Fe was the most abundant trace metal element and V as the ship emission indicator was detected. Transmission electron microscopy images showed that SK-rich, soot, Fe, SK-soot and SK-Fe were the major individual particles in the coastal port. V and soluble Fe were detected in sulfate coating of SK-Fe particles. We found that anthropogenic emissions, marine sea salt, and secondary atmosphere process were the major sources of fine particles. Backward trajectory analysis indicated that the dominant air masses were marine air mass, inland air mass from northern Zhejiang and inland-marine mixed air mass from Shandong and Shanghai during the sampling period. The findings can help us better understand the physicochemical properties of atmospheric fine particles in the coastal port of Eastern China. 展开更多
关键词 Coastal port Water-soluble ion Organic matter Trace metal Individual particle
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STUDY ON THE VISIBILITY REDUCTION CAUSED BY ATMOSPHERIC HAZE IN GUANGZHOU AREA
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作者 吴兑 邓雪娇 +3 位作者 毕雪岩 李菲 谭浩波 廖国莲 《Journal of Tropical Meteorology》 SCIE 2007年第1期17-20,共4页
Using the non-hydrostatic meso-scale model MM5v3, dense fog that occurred from March 7 to March 8, 2001 over the Mts. Nanling area was studied. With integrated field experiments and observations, the occurrence, devel... Using the non-hydrostatic meso-scale model MM5v3, dense fog that occurred from March 7 to March 8, 2001 over the Mts. Nanling area was studied. With integrated field experiments and observations, the occurrence, development and lift mechanism of fog were analyzed. The results indicate that before the coming of stratiform clouds, southerly warm and wet air ascended along mountainside and cooling condensation formed mountain fog. Then fog was formed by the stratiform on cloud-contacting mountaintop. A front inversion layer accelerated the development and extended the duration of the lower cloud and fog. The intensity, occurrence time, mass content and the variation of temperature and relative humidity of the fog agreed with those of the observation. It showed that the meso-scale model has the potential to forecast mountain fog. 展开更多
关键词 FOG mountain area numerical study observation data
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The asymmetry of air temperature:A new potential method to predict precipitation frequency
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作者 Yinan Xie Fenghua Xie 《Atmospheric and Oceanic Science Letters》 2025年第4期1-6,共6页
There is a significant bias in the precipitation frequency(PF)obtained from numerical model simulations.In this study,the authors use the temperature asymmetry(TA)as an indirect indicator to predict PF.The empirical o... There is a significant bias in the precipitation frequency(PF)obtained from numerical model simulations.In this study,the authors use the temperature asymmetry(TA)as an indirect indicator to predict PF.The empirical orthogonal function method is used to analyze the spatiotemporal correlation of TA and PF at interannual and interdecadal time scales.Furthermore,the authors explore using the TA to improve PF prediction in CMIP6 models.Results show that(1)on an interannual time scale,PF and TA show good spatial and temporal correlations;(2)PF and TA exhibit similar modal transitions on interdecadal time scales;and(3)using TA as an indirect indicator can significantly improve the prediction of PF.The TA may be an indirect method for improving precipitation predictions. 展开更多
关键词 Temperature asymmetry Precipitation frequency Empirical orthogonal function CMIP6
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Biophysical Impacts of Global Deforestation on Near-Surface Air Temperature in China: Results from Land Use Model Intercomparison Project Simulations
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作者 Yue SUI Miao WEI Bo LIU 《Advances in Atmospheric Sciences》 2025年第6期1141-1155,共15页
Global deforestation has been recognized as an important factor influencing climate change over the past century.However, uncertainties remain regarding its biophysical impacts on temperature across China. Utilizing m... Global deforestation has been recognized as an important factor influencing climate change over the past century.However, uncertainties remain regarding its biophysical impacts on temperature across China. Utilizing monthly data from eight global climate models of the Land Use Model Intercomparison Project, a multimodel comparison was conducted to quantitatively analyze the biophysical impacts of global deforestation on near-surface air temperature in China, using a surface energy balance decomposition method. Results show a 38%(29% to 45%) reduction in forest cover in China(ensemble mean and range across eight models) relative to pre-industrial levels, and an annual cooling of 0.6 K(0.05 to1.4 K) accompanied by global deforestation. Notably, surface albedo causes a cooling effect of 0.6 K(0.2 to 2.0 K), while surface latent and sensible heat fluxes partially offset this cooling by 0.2 K(-0.2 to 0.5 K) and 0.2 K(-0.04 to 0.6 K),respectively. These effects are more pronounced in winter and spring in deforested regions. Furthermore, the separation of atmospheric feedbacks under clear-sky and cloudy conditions show that the cloud radiative effect only accounts for 0.1 K(-0.1 to 0.4 K), while the clear-sky surface downward radiation is a significant cooling factor, contributing up to-0.5 K(-1.2 to 0.004 K), particularly in summer. However, the consistency of these models in simulating the impact of surface latent heat flux and albedo on surface temperature in China in response to deforestation is somewhat poor, highlighting the need to improve these related processes. 展开更多
关键词 global deforestation CMIP6 models China surface temperature biophysical impacts water vapor
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Impact of deforestation on precipitation extremes in China based on land use model intercomparison project models
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作者 Tianliang Gao Yue Sui +2 位作者 Bo Liu Yuxuan Peng Wenxuan Qiao 《Atmospheric and Oceanic Science Letters》 2025年第5期8-15,共8页
Deforestation has a significant influence on the hydrological cycle.Understanding the impact of deforestation on precipitation extremes is crucial for addressing global environmental challenges.This study investigates... Deforestation has a significant influence on the hydrological cycle.Understanding the impact of deforestation on precipitation extremes is crucial for addressing global environmental challenges.This study investigates the impact of deforestation on precipitation extremes(R95p index,which represents the total amount of precipitation exceeding the 95th percentile of the reference period)in China,using outputs from three earth system models(CanESM5,IPSL-CM6A-LR,and MIROC-ES2L).All models,along with their multimodel mean,indicate a general decrease in R95p in Northeast China and southern China,and changes in Northwest China and the Tibetan Plateau are minimal.In contrast,the responses are model-dependent in the Huanghuai and Jianghuai regions.The overall nationwide multimodel mean suggests an annual R95p decrease of 10.7 mm,with individual model variations ranging from-28.0 to 2.0 mm.Further analysis using precipitation extremes scaling reveals a high spatial correlation with direct precipitation extremes changes on both annual and seasonal scales,albeit with slightly smaller magnitudes.Decomposing the response into dynamic and thermodynamic scaling,the authors find that dynamic contributions predominantly drive the changes in precipitation extremes on both annual and seasonal scales.The authors findings highlight the substantial role of dynamic processes in modulating the response of precipitation extremes to deforestation in China. 展开更多
关键词 DEFORESTATION China Precipitation extremes Precipitation extremes scaling DYNAMICS
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Source apportionment of black carbon using an advanced Aethalometer model in a typical industrial city of China
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作者 Xingxing Fan Sihang Ye +7 位作者 Huang Zheng Bin Han Guotao Zhang Zhensen Zheng Xueyan Zhao Shaofei Kong Xiaoli Wang Wen Yang 《Journal of Environmental Sciences》 2025年第5期42-53,共12页
Black carbon(BC)aerosol can lead to adverse health effects and drive climate change;therefore,the characteristic research and identification of BC sources are essential for lowering emissions.In this study,equivalent ... Black carbon(BC)aerosol can lead to adverse health effects and drive climate change;therefore,the characteristic research and identification of BC sources are essential for lowering emissions.In this study,equivalent black carbon(eBC)measurement was performed using a seven-wavelength Aethalometer(AE33)at an urban site in a typical industrial city(Zibo)of Northern China for the first time.The monitoring was performed from February 2021 to January 2022.The mass absorption cross-section(MAC)of AE33 was optimised using the online elemental carbon(EC)data,and eBC was corrected using the MAC.The corrected annual BC concentration was 1.72±1.18μg/m^(3).The diurnal variation of BC depicted a bimodal distribution.Furthermore,the BC concentration on weekends was 18%lower than on weekdays.The diurnal variation and weekend effect reflect the critical contributions of traffic emission to BC concentration.The source apportionment of BC was calculated by a constraining Aethalometer model,which restricted theÅngstrom exponent using the online potassium ions.The results revealed that BC was not significantly affected by biomass burning(BC_(bb))in Zibo.The relative contribution of BC_(bb)was higher in winter than in other seasons.The daily morning peak of BC was primarily influenced by traffic sources,whereas the contribution of biomass burning increased after 17:00 in the evening peak.Our findings suggest that it is more important to control fossil fuel sources for BC emission reduction in Zibo,while it is necessary to strengthen the control of biomass combustion sources in winter. 展开更多
关键词 Black carbon(BC) AETHALOMETER AbsorptionÅngstrom exponent(AAE) Aethalometer model Fossil fuels Biomass burning Source apportionment
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PM_(2.5)-bound metallic elements in village and urban airs in North China during wintertime:Concentration,morphology,mixing state,and size distribution
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作者 Yinxiao Zhang Jian Zhang +3 位作者 Xiaotong Jiang Yuanyuan Wang Xiaokun Ding Weijun Li 《Journal of Environmental Sciences》 2025年第12期724-734,共11页
Atmospheric metal pollution is a significant environmental issue in China.Understanding the microscopic characteristics of metallic elements are crucial for investigating their sources and health effects,but this info... Atmospheric metal pollution is a significant environmental issue in China.Understanding the microscopic characteristics of metallic elements are crucial for investigating their sources and health effects,but this information is still limited.In this study,transmission electron microscopy(TEM)combined with bulk analysis method were employed to investigate the microscopic characteristics and mass concentrations of atmospheric metallic elements at a village site and an urban site located in North China Plain during wintertime.Our results reveal that the total mass concentrations of 16 metallic elements(including nine toxic heavy metallic elements)in PM_(2.5)were 3439.18±1101.24 ng/m^(3)(1129.6±376.85 ng/m^(3))at the village site and 3555.1±916.71 ng/m^(3)(1295.26±446.39 ng/m^(3))at urban site,accounting for 2.23%and 2.76%of PM_(2.5),respectively.We found that K,Ca,and Fe were the dominant elements,constituting over 75%of total metal mass.TEM analysis indicates that these metallic elements were mainly enriched in six types of individual particles,including K-rich,mineral,fly ash,Fe-rich,Zn-rich,and Pb-rich particles.Mineral particles were predominant in all individual metal particles at urban site,while K-rich particles became the dominant metal particles influenced by residential biomass burning at village site.Moreover,we found toxic metal particles(Fe-rich,Zn-rich,Pb-rich,and fly ash)presented smaller mean sizes(243 nm)in village air compared to urban air(337 nm),suggesting that metal particles in village air might pose a higher health risk to the residents.These results emphasize that atmospheric metal pollution in the village areas need more attentions in the future. 展开更多
关键词 Metallic elements Individual particles Village air Mass concentration Microscopic characteristics
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The characterization of ambient levoglucosan in Beijing during summertime:Dynamic variation and source contributions under strong cooking influences
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作者 Jun Wang Weiwei Hu +17 位作者 Tianle Pan Yingkun Wang Wei Chen Tingting Feng Yiyu Cai Zi Tao Wenhui Zhao Zhaoce Liu Jingxiong Liu Shaofei Kong Jipeng Qi Xiaoxiao Zhang Yuwen Peng Yuan Liu Shan Huang Bin Yuan Min Shao Xinming Wang 《Journal of Environmental Sciences》 2025年第9期205-220,共16页
Particulate levoglucosan is an important tracer for biomass burning emission in ambient air.However,recent studies question its reliability as a biomass burning tracer in Chinesemega cities due to important contributi... Particulate levoglucosan is an important tracer for biomass burning emission in ambient air.However,recent studies question its reliability as a biomass burning tracer in Chinesemega cities due to important contribution from potential non-biomass burning sources,such as cooking.To address this,we examined the dynamic variation and sources of levoglucosan using a chemical ionization mass spectrometer and other advanced instruments during Beijing’s summer of 2021.The average mass concentration of levoglucosan and its isomer(C_(6)H_(10)O_(5))was 0.025±0.014μg/m^(3),constituting 0.55%±0.32%of total organic carbon(OC)in this campaign.Despite cooking emissions contributing significantly to the organic aerosol(OA,20%),levoglucosan and its isomers correlated more strongly with biomass-burning related tracers(R>0.6),black carbon(R=0.72)and less so with cooking-related sources(R=0.3).This indicates that levoglucosan is primarily dominated by biomass-burning emissions rather than cooking in Beijing’s urban areas during summertime.The diurnal variation of levoglucosan concentrations highlighted the importance of daytime and nocturnal biomass burning emissions during polluted periods in Beijing.Using levoglucosan as a tracer to quantify the biomass burning OC(BBOC),we found good agreement on the time series of BBOC between the tracermethod and other independent source apportionmentmethod.This reaffirms the reliability of levoglucosan as a biomass burning tracer.Biomass burning contributed an average of 7%-8%to OC,highlighting its significant impact on Beijing’s summer air quality.Our study enhances understanding of biomass burning influences on ambient aerosol in typical urban areas. 展开更多
关键词 LEVOGLUCOSAN Biomass burning Tracer method COOKING Chemical ionization mass spectrometer(CIMS) Online measurement
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南京冬季重污染过程中黑碳气溶胶的混合态及粒径分布 被引量:9
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作者 蒋磊 汤莉莉 +5 位作者 潘良宝 刘丹彤 花艳 张运江 周宏仓 崔玉航 《环境科学》 EI CAS CSCD 北大核心 2017年第1期13-21,共9页
2013年12月,我国中东部地区暴发持续性重污染过程.本研究利用单颗粒黑碳光度计(SP2),分析这次过程中黑碳气溶胶(BC)的质量浓度、混合态以及粒径分布特征.结果表明,观测期间南京BC质量浓度在1.01~14.05μg·m-3之间,平均为4.39μg... 2013年12月,我国中东部地区暴发持续性重污染过程.本研究利用单颗粒黑碳光度计(SP2),分析这次过程中黑碳气溶胶(BC)的质量浓度、混合态以及粒径分布特征.结果表明,观测期间南京BC质量浓度在1.01~14.05μg·m-3之间,平均为4.39μg·m-3,污染较重时呈现夜间高白天低的日变化特征,污染较轻时则为早晚双峰型;用相对包裹层厚度(Dp/Dc)表示BC混合态特征,污染较轻时日变化为凌晨及午后较高,早晚出行高峰期较低,说明在凌晨及午后BC的老化程度较深,早晚机动车排放高峰时段BC多为近地源排放的新鲜粒子.污染较重时Dp/Dc日变化相对平缓,区域性污染特征更为明显并在高相对湿度下体现出气-固转化的过程;BC质量和数谱的粒径分布均为单峰型,数谱峰值粒径在污染较轻时分布在91 nm左右,污染较重时为100 nm,不同污染程度下质量谱峰值粒径均为210 nm,通过对比全球范围的观测结果可以体现出BC一次源的区域性差异.本研究对深入认识长三角地区大气BC污染特征,具有重要的参考价值. 展开更多
关键词 黑碳 南京 单颗粒黑碳光度计(SP2) 混合态 粒径分布
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Preliminary Results of 4-D Water Vapor Tomography in the Troposphere Using GPS 被引量:11
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作者 毕研盟 毛节泰 李成才 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2006年第4期551-560,共10页
Slant-path water vapor amounts (SWV) from a station to all the GPS (Global Positioning System) satellites in view can be estimated by using a ground-based GPS receiver. In this paper, a tomographic method was util... Slant-path water vapor amounts (SWV) from a station to all the GPS (Global Positioning System) satellites in view can be estimated by using a ground-based GPS receiver. In this paper, a tomographic method was utilized to retrieve the local horizontal and vertical structure of water vapor over a local GPS receiver network using SWV amounts as observables in the tomography. The method of obtaining SWV using ground-based GPS is described first, and then the theory of tomography using GPS is presented. A water vapor tomography experiment was made using a small GPS network in the Beijing region. The tomographic results were analyzed in two ways: (1) a pure GPS method, i.e., only using GPS observables as input to the tomography, (2) combining GPS observables with vertical constraints or a priori information, which come from average radiosonde measurements over three days. It is shown that the vertical structure of water vapor is well resolved with a priori information. Comparisons of profiles between radiosondes and GPS show that the RMS error of the tomography is about 1-2 mm. It is demonstrated that the tomography can monitor the evolution of tropospheric water vapor in space and time. The vertical resolution of the tomography is tested with layer thicknesses of 600 m, 800 m and 1000 m. Comparisons with radiosondes show that the result from a resolution of 800 m is slightly better than results from the other two resolutions in the experiment. Water vapor amounts recreated from the tomography field agree well with precipitable water vapor (PWV) calculated using GPS delays. Hourly tomographic results are also shown using the resolution of 800 m. Water vapor characteristics under the background of heavy rainfall development are analyzed using these tomographic results. The water vapor spatio-temporal structures derived from the GPS network show a great potential in the investigation of weather disasters. 展开更多
关键词 GPS slant path water vapor TOMOGRAPHY
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Abrupt Climate Change around 4 ka BP:Role of the Thermohaline Circulation as Indicated by a GCM Experiment 被引量:19
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作者 王绍武 周天军 +3 位作者 蔡静宁 朱锦红 谢志辉 龚道溢 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2004年第2期291-295,共5页
A great deal of palaeoenvironmental and palaeoclimatic evidence suggests that a predominant temperature drop and an aridiflcation occurred at ca. 4.0 ka BP. Palaeoclimate studies in China support this dedution. The co... A great deal of palaeoenvironmental and palaeoclimatic evidence suggests that a predominant temperature drop and an aridiflcation occurred at ca. 4.0 ka BP. Palaeoclimate studies in China support this dedution. The collapse of ancient civilizations at ca. 4.0 ka BP in the Nile Valley and Mesopotamia has been attributed to climate-induced aridification. A widespread alternation of the ancient cultures was also found in China at ca. 4.0 ka BP in concert with the collapse of the civilizations in the Old World. Palaeoclimatic studies indicate that the abrupt climate change at 4.0 ka BP is one of the realizations of the cold phase in millennial scale climate oscillations, which may be related to the modulation of the Thermohaline Circulation (THC) over the Atlantic Ocean. Therefore, this study conducts a numerical experiment of a GCM with SST forcing to simulate the impact of the weakening of the THC. Results show a drop in temperature from North Europe, the northern middle East Asia, and northern East Asia and a significant reduction of precipitation in East Africa, the Middle East, the Indian Peninsula, and the Yellow River Valley. This seems to support the idea that coldness and aridification at ca. 4.0 ka BP was caused by the weakening of the THC. 展开更多
关键词 abrupt climate change 4 ka BP thermohaline circulation collapse of ancient civilization
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Morphology,composition,and sources of individual aerosol particles at a regional background site of the YRD,China 被引量:7
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作者 Liang Xu A.P.Lingaswamy +5 位作者 Yinxiao Zhang Lei Liu Yuanyuan Wang Jian Zhang Qianli Ma Weijun Li 《Journal of Environmental Sciences》 SCIE EI CAS CSCD 2019年第3期354-362,共9页
Aerosol samples were collected at Lin'an, a background site of Yangtze River Delta(YRD).Morphology, size, composition, and mixing state of individual aerosol particles were characterized by transmission electron m... Aerosol samples were collected at Lin'an, a background site of Yangtze River Delta(YRD).Morphology, size, composition, and mixing state of individual aerosol particles were characterized by transmission electron microscopy(TEM) coupled with energy dispersive X-ray spectroscopy(EDS), and the soluble ions of PM_(1.0) were studied by aerosol mass spectrometer(AMS). The daily average AMS mass concentrations of sulfate, nitrate, and ammonium were about 5.8, 8.6, and 5.6 μg/m^3, respectively. Individual aerosol particles were classified into seven types: S-rich, K-rich, organic matter(OM), soot, fly ash, metal, and mineral. S-rich particles were dominant in all size bins, and 51%(by number) of S-rich particles were internally mixed with other particles. The fraction of organic coating particles was 13.7% in morning, 25.2% in afternoon, and 11% in evening, suggesting that the strong photochemical process during afternoon produced more secondary organic aerosols(SOA) on the surface of inorganic particles. Fly ash and metal particles were abundant during the day, suggesting the influence of emissions from coal-fired power plants and steel plants. The results indicate that the intense industrial emissions in the YRD significantly transported to the background areas. PM_(2.5) concentration may be lower in background air than in urban air but complex mixing state of aerosol particles indicates that the long-range transported particles substantially influenced the background air quality. 展开更多
关键词 REGIONAL BACKGROUND air Transmission electron microscopy INDIVIDUAL AEROSOL particles MIXING state YANGTZE River Delta
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Monthly Changes in the Influence of the Arctic Oscillation on Surface Air Temperature over China 被引量:4
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作者 黄嘉佑 谭本馗 +1 位作者 所玲玲 胡永云 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2007年第5期799-807,共9页
Partial Least Squares Regression (PLSR) is used to study monthly changes in the influence of the Arctic Oscillation (AO) on spring, summer and autumn air temperature over China with the January 500 hPa geopotentia... Partial Least Squares Regression (PLSR) is used to study monthly changes in the influence of the Arctic Oscillation (AO) on spring, summer and autumn air temperature over China with the January 500 hPa geopotential height data from 1951 to 2004 and monthly temperature data from January to November at 160 stations in China. Several AO indices have been defined with the 500-hPa geopotential data and the index defined as the first principal component of the normalized geopotential data is best to be used to study the influence of the AO on SAT (surface air temperature) in China. There are three modes through which the AO in winter influences SAT in China. The influence of the AO on SAT in China changes monthly and is stronger in spring and summer than in autumn. The main influenced regions are Northeast China and the Changjiang River drainage area. 展开更多
关键词 arctic oscillation temperature field monthly changes partial least squares regression
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On the Decadal and Interdecadal Variability in the Pacific Ocean 被引量:7
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作者 杨海军 张琼 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2003年第2期173-184,共12页
The Pacific decadal and interdecadal oscillation (PDO) has been extensively explored in recent decades because of its profound impact on global climate systems. It is a long-lived ENSO-like pattern of Pacific climate ... The Pacific decadal and interdecadal oscillation (PDO) has been extensively explored in recent decades because of its profound impact on global climate systems. It is a long-lived ENSO-like pattern of Pacific climate variability with a period of 10-30 years. The general picture is that the anomalously warm (cool) SSTs in the central North Pacific are always accompanied by the anomalously cool (warm) SSTs along the west coast of America and in the central east tropical Pacific with comparable amplitude. In general, there are two classes of opinions on the origin of this low-frequency climate variability, one thinking that it results from deterministically coupled modes of the Pacific ocean-atmosphere system, and the other, from stochastic atmospheric forcing. The deterministic origin emphasizes that the internal physical processes in an air-sea system can provide a positive feedback mechanism to amplify an initial perturbation, and a negative feedback mechanism to reverse the phase of oscillation. The dynamic evolution of ocean circulation determines the timescale of the oscillation. The stochastic origin, however, emphasizes that because the atmospheric activities can be thought as having no preferred timescale and are associated with an essentially white noise spectrum, tne ocean response can manifest a red peak in a certain low frequency range with a decadal to interdecadal timescale. In this paper, the authors try to systematically understand the state of the art of observational, theoretical and numerical studies on the PDO and hope to provide a useful background reference for current research. 展开更多
关键词 climate system Pacific decadal oscillation deterministic origin stochastic origin
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A Study of the Extratropical Transformation of Typhoon Winnie (1997) 被引量:5
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作者 朱佩君 郑永光 +1 位作者 张春喜 陶祖钰 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2005年第5期730-740,共11页
The complicated evolutive process of how a tropical cyclone transforms into an extratropical cyclone is still an unresolved issue to date, especially one which arises in a weakly baroclinic environment. Typhoon Winnie... The complicated evolutive process of how a tropical cyclone transforms into an extratropical cyclone is still an unresolved issue to date, especially one which arises in a weakly baroclinic environment. Typhoon Winnie (1997) is studied during its extratropical transformation stage of extratropical transition (ET) with observational data and numerical simulations. Results show that Winnie experienced its extratropical transformation to the south of the subtropical high without intrusion of the mid-latitude baroclinic zone. This is significantly different from previous studies. Analyses reveal that the cold air, which appeared in the north edge of Winnie circulation, resulted from the precipitation drag and cooling effect of latent heat absorption associated with the intense precipitation there. The cooling only happened below 3 km and the greatest cooling was below 1 km. With the cold air and its advection by the circulation of Winnie, a front was formed in the lower troposphere. The front above is related not only to the cooling in the lower level but also to the warming effect of latent heat release in the middle-upper levels. The different temperature variation in the vertical caused the temperature gradient over Winnie and resulted in the baroclinicity. 展开更多
关键词 extratropical transformation TYPHOON latent heat FRONT
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Role of the 10–20-Day Oscillation in Sustained Rainstorms over Hainan,China in October 2010 被引量:6
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作者 QIAO Yunting ZHANG Chunhua JIAN Maoqiu 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2015年第3期363-374,共12页
Hainan,an island province of China in the northern South China Sea,experienced two sustained rainstorms in October 2010,which were the most severe autumn rainstorms of the past 60 years.From August to October 2010,the... Hainan,an island province of China in the northern South China Sea,experienced two sustained rainstorms in October 2010,which were the most severe autumn rainstorms of the past 60 years.From August to October 2010,the most dominant signal of Hainan rainfall was the 10-20-day oscillation.This paper examines the roles of the 10-20-day oscillation in the convective activity and atmospheric circulation during the rainstorms of October 2010 over Hainan.During both rainstorms,Hainan was near the center of convective activity and under the influence of a lower-troposphere cyclonic circulation.The convective center was initiated in the west-central tropical Indian Ocean several days prior to the rainstorm in Hainan.The convective center first propagated eastward to the maritime continent,accompanied by the cyclonic circulation,and then moved northward to the northern South China Sea and South China,causing the rainstorms over Hainan.In addition,the westward propagation of convection from the tropical western Pacific to the southern South China Sea,as well as the propagation farther northward,intensified the convective activity over the northern South China Sea and South China during the first rainstorm. 展开更多
关键词 convective activity propagation characteristics tropical Indian Ocean western Pacific
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