Experimental validation of laser intensity is particularly important for the study of fundamental physics at extremely high intensities.However,reliable diagnosis of the focal spot and peak intensity faces huge challe...Experimental validation of laser intensity is particularly important for the study of fundamental physics at extremely high intensities.However,reliable diagnosis of the focal spot and peak intensity faces huge challenges.In this work,we demonstrate for the firs time that the coherent radiation farfiel patterns from laser–foil interactions can serve as an in situ,real-time,and easy-to-implement diagnostic for an ultraintense laser focus.The laser-driven electron sheets,curved by the spatially varying laser fiel and leaving the targets at nearly the speed of light,produce doughnut-shaped patterns depending on the shapes of the focal spot and the absolute laser intensities.Assisted by particle-in-cell simulations,we can achieve measurements of the intensity and the focal spot,and provide immediate feedback to optimize the focal spots for extremely high intensity.展开更多
The illicit trafficking of special nuclear materials(SNMs)poses a grave threat to global security and necessitates the development of effective nuclear material identification methods.This study investigated a method ...The illicit trafficking of special nuclear materials(SNMs)poses a grave threat to global security and necessitates the development of effective nuclear material identification methods.This study investigated a method to isotopically identify the SNMs,including^(233,235,238)U,^(239-242)Pu,and^(232)Th,based on the detection of delayedγ-rays from photofission fragments.The delayedγ-ray spectra resulting from the photofission of SNMs irradiated by a 14 MeVγbeam with a total of 10~9 were simulated using Geant4.Three high-yield fission fragments,namely^(138)Cs,^(89)Rb,and^(94)Y,were selected as candidate fragments for SNM identification.The yield ratios of these three fragments were calculated,and the results from the different SNMs were compared.The yield ratio of^(138)Cs/^(89)Rb was used to identify most SNMs,including^(233,235,238)U,^(242)Pu,and^(232)Th,with a confidence level above 95%.To identify^(239-241)Pu with the same confidence,a higher total number of 10^(11)γbeams is required.However,although the^(94)Y/^(89)Rb ratio is suitable for elementally identifying SNMs,isotopic identification is difficult.In addition,the count rate of the delayedγabove 3 MeV can be used to rapidly detect the presence of nuclear materials.展开更多
We derive the gravitational-wave(GW)strain upper limits from resolvable supermassive black-hole binaries using the data from the Five-hundred-meter Aperture Spherical radio Telescope,in the context of the Chinese Puls...We derive the gravitational-wave(GW)strain upper limits from resolvable supermassive black-hole binaries using the data from the Five-hundred-meter Aperture Spherical radio Telescope,in the context of the Chinese Pulsar Timing Array project.We focus on circular orbits in theμHz GW frequency band between 10^(−7)and 3×10^(−6)Hz.This frequency band is higher than the traditional pulsar timing array band and is less explored.We used the data of the millisecond pulsar PSR J1713+5307 observed between 2019 August and 2021 April.A dense observation campaign was carried out in 2020 September to allow for theμHz band coverage.Our sky-averaged continuous source upper limit at the 95%confidence level at 1μHz is 1.26×10^(−12),while the same limit in the direction of the pulsar is 4.77×10^(−13).展开更多
Fast Radio Bursts(FRBs) are enigmatic millisecond-duration radio transients of extra-galactic origin, whose underlying mechanisms and progenitors remain poorly understood. FRBs are broadly classified into two categori...Fast Radio Bursts(FRBs) are enigmatic millisecond-duration radio transients of extra-galactic origin, whose underlying mechanisms and progenitors remain poorly understood. FRBs are broadly classified into two categories: repeating FRBs, which emit multiple bursts over time, and one-off FRBs, which are detected as single events. A central question in FRB research is whether these two classes share a common origin. In this study, we present observations of FRB 20240114A, a repeating FRB that entered a hyperactive phase in 2024 January. We conducted a 318 hr monitoring campaign using the Kunming 40-Meter Radio Telescope(KM40M) in the S-band(2.187–2.311 GHz), during which we detected eight radio bursts. We analyzed their properties, including dispersion measure, bandwidth, pulse width, flux, fluence, and energy. Additionally, we searched for counterparts in overlapping data from the Five-hundred-meter Aperture Spherical Telescope(FAST) in the L-band(1.0–1.5 GHz). While no bursts were temporally aligned between the two telescopes, we identified one FAST burst that arrived approximately 6 ms after one of the KM40M bursts. The absence of FAST counterparts for the KM40M bursts suggests that individual bursts from FRB 20240114A are likely narrow-band, with fractional bandwidths less than 10%. By comparing the cumulative event rates from KM40M and FAST observations, we found that the two measurements are compatible, indicating a possible flattening of the event rate at higher energies. This feature aligns with observations of one-off FRBs, supporting the hypothesis that repeating and oneoff FRBs may share a common origin.展开更多
Correction to:Nuclear Science and Techniques(2025)36:100 https://doi.org/10.1007/s41365-025-01692-6 In this article,Fig.9 appeared incorrectly and have now been corrected in the original publication.For completeness a...Correction to:Nuclear Science and Techniques(2025)36:100 https://doi.org/10.1007/s41365-025-01692-6 In this article,Fig.9 appeared incorrectly and have now been corrected in the original publication.For completeness and transparency,both correct and incorrect versions are displayed below.展开更多
High-power laser pulses interacting with targets can generate intense electromagnetic pulses(EMPs),which can disrupt physical experimental diagnostics and even damage diagnostic equipment,posing a threat to the reliab...High-power laser pulses interacting with targets can generate intense electromagnetic pulses(EMPs),which can disrupt physical experimental diagnostics and even damage diagnostic equipment,posing a threat to the reliable operation of experiments.In this study,EMPs resulting from multi-petawatt laser irradiating nitrogen gas jets were systematically analyzed and investigated.The experimental results revealed that the EMP amplitude is positively correlated with the quantity and energy of the electrons captured and accelerated by the plasma channel.These factors are reflected by parameters such as laser energy and nitrogen gas jet pressure.Additionally,we propose several potential sources of EMPs produced by laser-irradiated gas jets and separately analyzed their spatiotemporal distributions.The findings provide insight into the mechanisms of EMP generation and introduce a new approach to achieve controllable EMPs by regulating the laser energy and gas jet pressure.展开更多
Short-lived medical isotopes and their generators are typically produced in nuclear reactors and cyclotrons that require extensive facilities.However,considering the environmental concerns and economic costs of these ...Short-lived medical isotopes and their generators are typically produced in nuclear reactors and cyclotrons that require extensive facilities.However,considering the environmental concerns and economic costs of these traditional approaches,modern laser technology,which provides extremely strong electric fields within tabletop-sized areas,can serve as a potential supplementary method.Focusing specifically on the(γ,p)generation of the vital medical isotopes^(47)Sc and^(67)Cu,we used both experimental results and PIC-GEANT4 simulations to demonstrate that laser-induced photonuclear reaction is a promising method for isotope production.We developed a model capable of calculating isotope yields under various laser conditions and acceleration mechanisms.The findings revealed that a 200 TW laser can sufficiently produce diagnostic amounts of^(47)Sc and^(67)Cu,while simultaneously providing high specific activity,which is significant in medical applications for improving treatment efficacy,enhancing image resolution,and reducing side effects.展开更多
The newly built Compact Laser Plasma Accelerator-Therapy facility at Peking University will deliver 60 J/1 Hz laser pulses with 30 fs duration.Driven by this petawatt laser facility,proton beams with energy up to 200 ...The newly built Compact Laser Plasma Accelerator-Therapy facility at Peking University will deliver 60 J/1 Hz laser pulses with 30 fs duration.Driven by this petawatt laser facility,proton beams with energy up to 200 MeV are expected to be generated for tumor therapy.During high-repetition operation,both prompt radiation and residual radiation may cause safety problems.Therefore,human radiological safety assessment before commissioning is essential.In this paper,we simulate both prompt and residual radiation using the Geant4 and FLUKA Monte Carlo codes with reasonable proton and as-produced electron beam parameters.We find that the prompt radiation can be shielded well by the concrete wall of the experimental hall,but the risk from residual radiation is nonnegligible and necessitates adequate radiation cooling.On the basis of the simulation results,we discuss the constraints imposed by radiation safety considerations on the annual working time,and we propose radiation cooling strategies for different shooting modes.展开更多
Ultrashort and powerful laser interactions with a target generate intense wideband electromagnetic pulses(EMPs).In this study,we report EMPs generated by the interactions between petawatt(30 fs,1.4×10^(20) W/cm^(...Ultrashort and powerful laser interactions with a target generate intense wideband electromagnetic pulses(EMPs).In this study,we report EMPs generated by the interactions between petawatt(30 fs,1.4×10^(20) W/cm^(2))femtosecond(fs)lasers with metal flat,plastic flat,and plastic nanowire-array(NWA)targets.Detailed analyses are conducted on the EMPs in terms of their spatial distribution,time and frequency domains,radiation energy,and protection.The results indicate that EMPs from metal targets exhibit larger amplitudes at varying angles than those generated by other types of targets and are enhanced significantly for NWA targets.Using a plastic target holder and increasing the laser focal spot can significantly decrease the radiation energy of the EMPs.Moreover,the composite shielding materials indicate an effective shielding effect against EMPs.The simulation results show that the NWA targets exert a collimating effect on thermal electrons,which directly affects the distribution of EMPs.This study provides guidance for regulating EMPs by controlling the laser focal spot,target parameters,and target rod material and is beneficial for electromagnetic-shielding design.展开更多
Light olefins such as ethylene and propylene are important industrial feedstocks, having essential applications in the production of plastics, ethylbenzene, and ethylene dichloride [1]. Compared with the conventional ...Light olefins such as ethylene and propylene are important industrial feedstocks, having essential applications in the production of plastics, ethylbenzene, and ethylene dichloride [1]. Compared with the conventional route, in which alkane steam cracking (SC) at high temperature is applied to produce ethylene and propylene, the catalytic ethane/propane non-oxidative dehydrogenation (EDH/PDH) possess the advantages of high selectivity and low energy consumption. Industrially, Pt is the major component to catalyze this reaction, but it suffers from low selectivity and fast deactivation because of favorable coke formation [2].展开更多
The search for the ri_(13/2) vi_(13/2 ) band in ^(178)Ir has been conducted through the ^(152)Sm(^(31) P, 5nγ)^( 178)Ir reaction and the excitation functions, x-γ and γ-γ-t coincidence measurements. Five rotationa...The search for the ri_(13/2) vi_(13/2 ) band in ^(178)Ir has been conducted through the ^(152)Sm(^(31) P, 5nγ)^( 178)Ir reaction and the excitation functions, x-γ and γ-γ-t coincidence measurements. Five rotational bands have been newly identified. The low-spin signature inversion in the πi13/2 vi13/2 band has been confirmed by the observations of linking transitions and signature crossing at I = 25.5 h. The inversion phenomenon in rh11/2 vi_(13/2), rh9/2 vi_(13/2) and ri_(13/2) vi13/2 structures in ^(178)Ir provides a unique testing ground for different theoretical interpretations.展开更多
The observables of continuous eigenvalues are de?ned in an in?nite-dimensional ket space. The complete set of such eigenstates demands a spectrum density factor, for example, for the photons in the free space and elec...The observables of continuous eigenvalues are de?ned in an in?nite-dimensional ket space. The complete set of such eigenstates demands a spectrum density factor, for example, for the photons in the free space and electrons in the vacuum. From the derivation of the Casimir force without an arti?cial regulator we determine the explicit expression of the spectrum density factor for the photon ?eld to be an exponential function. The undetermined constant in the function is ?xed by the experimental data for the Lamb shift. With that, we predict that there exists a correction to the Casimir force.展开更多
Observing and timing a group of millisecond pulsars with high rotational stability enables the direct detection of gravitational waves(GWs).The GW signals can be identified from the spatial correlations encoded in the...Observing and timing a group of millisecond pulsars with high rotational stability enables the direct detection of gravitational waves(GWs).The GW signals can be identified from the spatial correlations encoded in the times-of-arrival of widely spaced pulsar-pairs.The Chinese Pulsar Timing Array(CPTA)is a collaboration aiming at the direct GW detection with observations carried out using Chinese radio telescopes.This short article serves as a“table of contents”for a forthcoming series of papers related to the CPTA Data Release 1(CPTA DR1)which uses observations from the Five-hundred-meter Aperture Spherical radio Telescope.Here,after summarizing the time span and accuracy of CPTA DR1,we report the key results of our statistical inference finding a correlated signal with amplitude logA_(c)=-14.4_(-2.8)^(+1.0)for spectral index in the range ofα∈[-1.8,1.5]assuming a GW background(GWB)induced quadrupolar correlation.The search for the Hellings–Downs(HD)correlation curve is also presented,where some evidence for the HD correlation has been found that a 4.6σstatistical significance is achieved using the discrete frequency method around the frequency of 14 n Hz.We expect that the future International Pulsar Timing Array data analysis and the next CPTA data release will be more sensitive to the n Hz GWB,which could verify the current results.展开更多
Relative methods, which are performed with the assistance of reference materials, are widely used in photon activation analysis(PAA). On the contrary, absolute methods, which are conducted without any reference materi...Relative methods, which are performed with the assistance of reference materials, are widely used in photon activation analysis(PAA). On the contrary, absolute methods, which are conducted without any reference material, are rarely applied due to the difficulty in obtaining photon flux. To realize absolute measurement in PAA,we retrieve photon flux in the sample via Monte Carlo simulation and raise a novel procedure—quasi-absolute method. With simulated photon flux and cross section data from existing databases, it is possible to calculate the concentration of target elements in the sample straightforwardly. A controlled experiment indicates that results from the quasi-absolute method for certain elements are nearly comparable to relative methods in practice.This technique of absolute measurement has room for improvement in the future and can serve as a validation technique for experimental data on cross sections as well.展开更多
High-spin states in the beam energies. A new and 72 γ transitions odd-odd nucleus ^128I are investigated via the ^124 Sn（^7 Li,3n）^128 I reaction at 28 and 32 Me V level scheme of 12sI is established up to high-spi...High-spin states in the beam energies. A new and 72 γ transitions odd-odd nucleus ^128I are investigated via the ^124 Sn（^7 Li,3n）^128 I reaction at 28 and 32 Me V level scheme of 12sI is established up to high-spin states at I^π = 16, including 48 levels The present level scheme is largely different from the one in a recent publication due to identification of several doublet and triplet γ transitions and their proper placements in the level scheme. The high-spin level structure exhibits no obvious collective properties and is possibly associated with two and multi-quasiparticle configurations.展开更多
基金supported by the Guangdong High Level Innovation Research Institute(Grant No.2021B0909050006)the National Grand Instrument Project(Grant No.2019YFF01014402)+1 种基金the National Natural Science Foundation of China(Grant No.12205008)support from the National Science Fund for Distinguished Young Scholars(Grant No.12225501)。
文摘Experimental validation of laser intensity is particularly important for the study of fundamental physics at extremely high intensities.However,reliable diagnosis of the focal spot and peak intensity faces huge challenges.In this work,we demonstrate for the firs time that the coherent radiation farfiel patterns from laser–foil interactions can serve as an in situ,real-time,and easy-to-implement diagnostic for an ultraintense laser focus.The laser-driven electron sheets,curved by the spatially varying laser fiel and leaving the targets at nearly the speed of light,produce doughnut-shaped patterns depending on the shapes of the focal spot and the absolute laser intensities.Assisted by particle-in-cell simulations,we can achieve measurements of the intensity and the focal spot,and provide immediate feedback to optimize the focal spots for extremely high intensity.
基金supported by the National Key Research and Development Program(No.2022YFA1603300)the National Natural Science Foundation of China(Nos.U2230133,12305266,11921006,12405282)National Grand Instrument Project(No.2019YFF01014400)。
文摘The illicit trafficking of special nuclear materials(SNMs)poses a grave threat to global security and necessitates the development of effective nuclear material identification methods.This study investigated a method to isotopically identify the SNMs,including^(233,235,238)U,^(239-242)Pu,and^(232)Th,based on the detection of delayedγ-rays from photofission fragments.The delayedγ-ray spectra resulting from the photofission of SNMs irradiated by a 14 MeVγbeam with a total of 10~9 were simulated using Geant4.Three high-yield fission fragments,namely^(138)Cs,^(89)Rb,and^(94)Y,were selected as candidate fragments for SNM identification.The yield ratios of these three fragments were calculated,and the results from the different SNMs were compared.The yield ratio of^(138)Cs/^(89)Rb was used to identify most SNMs,including^(233,235,238)U,^(242)Pu,and^(232)Th,with a confidence level above 95%.To identify^(239-241)Pu with the same confidence,a higher total number of 10^(11)γbeams is required.However,although the^(94)Y/^(89)Rb ratio is suitable for elementally identifying SNMs,isotopic identification is difficult.In addition,the count rate of the delayedγabove 3 MeV can be used to rapidly detect the presence of nuclear materials.
基金supported by the FAST Key projectsupported by the National SKA Program of China (2020SKA0120100)+4 种基金the National Natural Science Foundation of China (NSFC, Grant Nos. 12041303 and 12250410246)the CAS-MPG LEGACY projectfunding from the Max-Planck Partner Groupsupport from the XPLORER PRIZE and 20 yr long-term support from Dr. Guojun Qiaosupported by Major Science and Technology Program of Xinjiang Uygur Autonomous Region No. 2022A03013-4
文摘We derive the gravitational-wave(GW)strain upper limits from resolvable supermassive black-hole binaries using the data from the Five-hundred-meter Aperture Spherical radio Telescope,in the context of the Chinese Pulsar Timing Array project.We focus on circular orbits in theμHz GW frequency band between 10^(−7)and 3×10^(−6)Hz.This frequency band is higher than the traditional pulsar timing array band and is less explored.We used the data of the millisecond pulsar PSR J1713+5307 observed between 2019 August and 2021 April.A dense observation campaign was carried out in 2020 September to allow for theμHz band coverage.Our sky-averaged continuous source upper limit at the 95%confidence level at 1μHz is 1.26×10^(−12),while the same limit in the direction of the pulsar is 4.77×10^(−13).
基金supported by the National SKA Program of China (grant No. 2020SKA0120100)the Special Project of Foreign Science and Technology Cooperation, Yunnan Provincial Science and Technology Department (grant No. 202003AD150010)+4 种基金the National Key R&D Program of China (grant No. 2022YFC2205203)the National Natural Science Foundation of China (NSFC, grant Nos. 12073076, 12173087, 12041303, and 12063003)the CAS “Western Light Youth Project,” Yunnan Fundamental Research Projects (grant Nos. 202401AT070144 and 202505AO120021)funding from the Max-Planck Partner Groupsupport from the XPLORER PRIZE
文摘Fast Radio Bursts(FRBs) are enigmatic millisecond-duration radio transients of extra-galactic origin, whose underlying mechanisms and progenitors remain poorly understood. FRBs are broadly classified into two categories: repeating FRBs, which emit multiple bursts over time, and one-off FRBs, which are detected as single events. A central question in FRB research is whether these two classes share a common origin. In this study, we present observations of FRB 20240114A, a repeating FRB that entered a hyperactive phase in 2024 January. We conducted a 318 hr monitoring campaign using the Kunming 40-Meter Radio Telescope(KM40M) in the S-band(2.187–2.311 GHz), during which we detected eight radio bursts. We analyzed their properties, including dispersion measure, bandwidth, pulse width, flux, fluence, and energy. Additionally, we searched for counterparts in overlapping data from the Five-hundred-meter Aperture Spherical Telescope(FAST) in the L-band(1.0–1.5 GHz). While no bursts were temporally aligned between the two telescopes, we identified one FAST burst that arrived approximately 6 ms after one of the KM40M bursts. The absence of FAST counterparts for the KM40M bursts suggests that individual bursts from FRB 20240114A are likely narrow-band, with fractional bandwidths less than 10%. By comparing the cumulative event rates from KM40M and FAST observations, we found that the two measurements are compatible, indicating a possible flattening of the event rate at higher energies. This feature aligns with observations of one-off FRBs, supporting the hypothesis that repeating and oneoff FRBs may share a common origin.
文摘Correction to:Nuclear Science and Techniques(2025)36:100 https://doi.org/10.1007/s41365-025-01692-6 In this article,Fig.9 appeared incorrectly and have now been corrected in the original publication.For completeness and transparency,both correct and incorrect versions are displayed below.
基金supported by the National Grand Instrument Project(No.2019YFF01014404)the Natural Science Foundation of China(Nos.12122501,61631001,11921006,U2241281,and 11975037)the Foundation of Science and Technology on Plasma Physics Laboratory(No.6142A04220108)。
文摘High-power laser pulses interacting with targets can generate intense electromagnetic pulses(EMPs),which can disrupt physical experimental diagnostics and even damage diagnostic equipment,posing a threat to the reliable operation of experiments.In this study,EMPs resulting from multi-petawatt laser irradiating nitrogen gas jets were systematically analyzed and investigated.The experimental results revealed that the EMP amplitude is positively correlated with the quantity and energy of the electrons captured and accelerated by the plasma channel.These factors are reflected by parameters such as laser energy and nitrogen gas jet pressure.Additionally,we propose several potential sources of EMPs produced by laser-irradiated gas jets and separately analyzed their spatiotemporal distributions.The findings provide insight into the mechanisms of EMP generation and introduce a new approach to achieve controllable EMPs by regulating the laser energy and gas jet pressure.
文摘Short-lived medical isotopes and their generators are typically produced in nuclear reactors and cyclotrons that require extensive facilities.However,considering the environmental concerns and economic costs of these traditional approaches,modern laser technology,which provides extremely strong electric fields within tabletop-sized areas,can serve as a potential supplementary method.Focusing specifically on the(γ,p)generation of the vital medical isotopes^(47)Sc and^(67)Cu,we used both experimental results and PIC-GEANT4 simulations to demonstrate that laser-induced photonuclear reaction is a promising method for isotope production.We developed a model capable of calculating isotope yields under various laser conditions and acceleration mechanisms.The findings revealed that a 200 TW laser can sufficiently produce diagnostic amounts of^(47)Sc and^(67)Cu,while simultaneously providing high specific activity,which is significant in medical applications for improving treatment efficacy,enhancing image resolution,and reducing side effects.
基金supported by the National Natural Science Foundation of China(Grant No.12205008)the NSFC Innovation Group Project(Grant No.11921006)+1 种基金the National Grand Instrument Project(Grant Nos.2019YFF01014402 and 2019YFF01014403)the National Science Fund for Distinguished Young Scholars(Grant No.12225501).
文摘The newly built Compact Laser Plasma Accelerator-Therapy facility at Peking University will deliver 60 J/1 Hz laser pulses with 30 fs duration.Driven by this petawatt laser facility,proton beams with energy up to 200 MeV are expected to be generated for tumor therapy.During high-repetition operation,both prompt radiation and residual radiation may cause safety problems.Therefore,human radiological safety assessment before commissioning is essential.In this paper,we simulate both prompt and residual radiation using the Geant4 and FLUKA Monte Carlo codes with reasonable proton and as-produced electron beam parameters.We find that the prompt radiation can be shielded well by the concrete wall of the experimental hall,but the risk from residual radiation is nonnegligible and necessitates adequate radiation cooling.On the basis of the simulation results,we discuss the constraints imposed by radiation safety considerations on the annual working time,and we propose radiation cooling strategies for different shooting modes.
基金This work was supported by the National Natural Science Foundation of China(Nos.12122501,11975037,61631001,and 11921006)the National Grand Instrument Project(Nos.2019YFF01014400,2019YFF01014404)the Foundation of Science and Technology on Plasma Physics Laboratory(No.6142A04220108).
文摘Ultrashort and powerful laser interactions with a target generate intense wideband electromagnetic pulses(EMPs).In this study,we report EMPs generated by the interactions between petawatt(30 fs,1.4×10^(20) W/cm^(2))femtosecond(fs)lasers with metal flat,plastic flat,and plastic nanowire-array(NWA)targets.Detailed analyses are conducted on the EMPs in terms of their spatial distribution,time and frequency domains,radiation energy,and protection.The results indicate that EMPs from metal targets exhibit larger amplitudes at varying angles than those generated by other types of targets and are enhanced significantly for NWA targets.Using a plastic target holder and increasing the laser focal spot can significantly decrease the radiation energy of the EMPs.Moreover,the composite shielding materials indicate an effective shielding effect against EMPs.The simulation results show that the NWA targets exert a collimating effect on thermal electrons,which directly affects the distribution of EMPs.This study provides guidance for regulating EMPs by controlling the laser focal spot,target parameters,and target rod material and is beneficial for electromagnetic-shielding design.
基金supported by the U.S.Department of EnergyOffice of Science,Office of Basic Energy Sciences,Chemical Sciences,Geosciences,and Biosciences Division,Catalysis Science Program to the SUNCAT Center for Interface Science and Catalysis。
文摘Light olefins such as ethylene and propylene are important industrial feedstocks, having essential applications in the production of plastics, ethylbenzene, and ethylene dichloride [1]. Compared with the conventional route, in which alkane steam cracking (SC) at high temperature is applied to produce ethylene and propylene, the catalytic ethane/propane non-oxidative dehydrogenation (EDH/PDH) possess the advantages of high selectivity and low energy consumption. Industrially, Pt is the major component to catalyze this reaction, but it suffers from low selectivity and fast deactivation because of favorable coke formation [2].
基金Supported by the National Natural Science Foundation of China under Grant Nos.10025525 and 19605008the Japan STA Scientist Exchange Programme,the JSPS Invitation Fellowship Programme for Research in Japan under Grant No.L00515the Major State Basic Research Development Programme of China(Contract No.G2000077400).
文摘The search for the ri_(13/2) vi_(13/2 ) band in ^(178)Ir has been conducted through the ^(152)Sm(^(31) P, 5nγ)^( 178)Ir reaction and the excitation functions, x-γ and γ-γ-t coincidence measurements. Five rotational bands have been newly identified. The low-spin signature inversion in the πi13/2 vi13/2 band has been confirmed by the observations of linking transitions and signature crossing at I = 25.5 h. The inversion phenomenon in rh11/2 vi_(13/2), rh9/2 vi_(13/2) and ri_(13/2) vi13/2 structures in ^(178)Ir provides a unique testing ground for different theoretical interpretations.
基金Supported by the National Natural Science Foundation of China under Grant No.11774316the Natural Science Foundation of Zhejiang Province under Grant No.Z15A050001
文摘The observables of continuous eigenvalues are de?ned in an in?nite-dimensional ket space. The complete set of such eigenstates demands a spectrum density factor, for example, for the photons in the free space and electrons in the vacuum. From the derivation of the Casimir force without an arti?cial regulator we determine the explicit expression of the spectrum density factor for the photon ?eld to be an exponential function. The undetermined constant in the function is ?xed by the experimental data for the Lamb shift. With that, we predict that there exists a correction to the Casimir force.
基金supported by the National SKA Program of China(2020SKA0120100)the National Natural Science Foundation of China(Nos.12041303 and 12250410246)+1 种基金the CAS-MPG LEGACY projectfunding from the Max-Planck Partner Group。
文摘Observing and timing a group of millisecond pulsars with high rotational stability enables the direct detection of gravitational waves(GWs).The GW signals can be identified from the spatial correlations encoded in the times-of-arrival of widely spaced pulsar-pairs.The Chinese Pulsar Timing Array(CPTA)is a collaboration aiming at the direct GW detection with observations carried out using Chinese radio telescopes.This short article serves as a“table of contents”for a forthcoming series of papers related to the CPTA Data Release 1(CPTA DR1)which uses observations from the Five-hundred-meter Aperture Spherical radio Telescope.Here,after summarizing the time span and accuracy of CPTA DR1,we report the key results of our statistical inference finding a correlated signal with amplitude logA_(c)=-14.4_(-2.8)^(+1.0)for spectral index in the range ofα∈[-1.8,1.5]assuming a GW background(GWB)induced quadrupolar correlation.The search for the Hellings–Downs(HD)correlation curve is also presented,where some evidence for the HD correlation has been found that a 4.6σstatistical significance is achieved using the discrete frequency method around the frequency of 14 n Hz.We expect that the future International Pulsar Timing Array data analysis and the next CPTA data release will be more sensitive to the n Hz GWB,which could verify the current results.
基金Supported by the U.S.Department of Energy,Basic Energy Sciences,Office of Science(No.DE-AC02-06CH11357)
文摘Relative methods, which are performed with the assistance of reference materials, are widely used in photon activation analysis(PAA). On the contrary, absolute methods, which are conducted without any reference material, are rarely applied due to the difficulty in obtaining photon flux. To realize absolute measurement in PAA,we retrieve photon flux in the sample via Monte Carlo simulation and raise a novel procedure—quasi-absolute method. With simulated photon flux and cross section data from existing databases, it is possible to calculate the concentration of target elements in the sample straightforwardly. A controlled experiment indicates that results from the quasi-absolute method for certain elements are nearly comparable to relative methods in practice.This technique of absolute measurement has room for improvement in the future and can serve as a validation technique for experimental data on cross sections as well.
基金Supported by the National Natural Science Foundation of China under Grant Nos 10825522, 1073505010 and 10775158, JSPS Invitation Fellowship （L00515）, the National Basic Research Program of China under Grant No 2007CB815005, and the Chinese Academy of Sciences.
文摘High-spin states in the beam energies. A new and 72 γ transitions odd-odd nucleus ^128I are investigated via the ^124 Sn（^7 Li,3n）^128 I reaction at 28 and 32 Me V level scheme of 12sI is established up to high-spin states at I^π = 16, including 48 levels The present level scheme is largely different from the one in a recent publication due to identification of several doublet and triplet γ transitions and their proper placements in the level scheme. The high-spin level structure exhibits no obvious collective properties and is possibly associated with two and multi-quasiparticle configurations.
