The reasonable design of the composition of the composite materials is of great significance to optimized the electromagnetic(EM)wave absorption performance.Herein,the Ni/NiO@C hybrid composites with tunable Ni propor...The reasonable design of the composition of the composite materials is of great significance to optimized the electromagnetic(EM)wave absorption performance.Herein,the Ni/NiO@C hybrid composites with tunable Ni proportion were successfully synthesized through a two-step process.With the assistance of X-ray diffraction with refinement treatment,the specific proportion of Ni of as-obtained hybrid composites could be obtained.Employing controlling calcination time to adjust the Ni content of Ni/NiO@C hybrid composites,it has been found that the composite carbonized at 500℃exhibited remarkable EM wave absorption with the minimum reflection loss(RLmin)of-49.1 dB at 4.9 mm and the widest effective absorption bandwidth(EABmax)of 4.56 GHz at 2.1 mm.Moreover,by adjusting the Ni source,the optimal EM wave absorption performance could be achieved.Results illustrated that the N3PC with the Ni proportion of 13.17%showed the RLm inas low as-51.1 dB at 2.4 mm and the EABmax was 5.12 GHz at 2.7 mm.It is worth noting that this work demonstrates the relevance of the composition and EM wave absorption performance of hybrid composites,which offers a feasible reference for the absorption mechanism of absorber.展开更多
Electromagnetic wave(EMW)-absorbing materials have considerable capacity in the military field and the prevention of EMW radiation from harming human health.However,obtaining lightweight,high-performance,and broadband...Electromagnetic wave(EMW)-absorbing materials have considerable capacity in the military field and the prevention of EMW radiation from harming human health.However,obtaining lightweight,high-performance,and broadband EMW-absorbing material remains an overwhelming challenge.Creating dielectric/magnetic composites with customized structures is a strategy with great promise for the development of high-performance EMW-absorbing materials.Using layered double hydroxides as the precursors of bimetallic alloys and combining them with porous biomass-derived carbon materials is a potential way for constructing multi-interface heterostructures as efficient EMW-absorbing materials because they have synergistic losses,low costs,abundant resources,and light weights.Here,FeNi alloy nanosheet array/Lycopodium spore-derived carbon(FeNi/LSC)was prepared through a simple hydrothermal and carbonization method.FeNi/LSC presents ideal EMW-absorbing performance by benefiting from the FeNi alloy nanosheet array,sponge-like structure,capability for impedance matching,and improved dielectric/magnetic losses.As expected,FeNi/LSC exhibited the minimum reflection loss of-58.3 dB at 1.5 mm with 20wt%filler content and a widely effective absorption bandwidth of 4.92 GHz.FeNi/LSC composites with effective EMW-absorbing performance provide new insights into the customization of biomass-derived composites as high-performance and lightweight broadband EMW-absorbing materials.展开更多
For active wave absorbers in force-control mode,the optimal feedback(control)force provided by the control system depends on the hydrodynamic forces.This work investigates a piston-type wave absorber with different dr...For active wave absorbers in force-control mode,the optimal feedback(control)force provided by the control system depends on the hydrodynamic forces.This work investigates a piston-type wave absorber with different draft-to-water depth ratios,focusing on the frequency-dependent hydrodynamic coefficients,wave absorption efficiency,wave absorber displacement and velocity,and control force.Analytical results were derived based on potential flow theory,confirming that regular incident waves can be fully absorbed by the piston-type active wave absorber at any draft ratio by optimizing the control force.The results for the wave tank with a typical water depth of 3 m were studied in detail.The draft ratio has a strong influence on the hydrodynamic coefficients.At the maximum wave absorption efficiency,the displacement and velocity amplitudes are sensitive to the draft ratio in the low-frequency region,increase with decreasing draft ratio,and are independent of the mass of the wave absorber.The control force required can be extremely large for a draft ratio greater than 1/3.The control force increases significantly as the draft ratio increases.The mass of the wave absorber has a weak influence on the control force.A time-domain numerical method based on the boundary element method was developed to verify the analytical solutions.Perfect agreements between the analytical solutions and the numerical results were obtained.展开更多
基金financially supported by the National Natural Science Foundation of China(Nos.51407134,51801001 and 51801108)Natural Science Foundation of Shandong Province(No.ZR2019YQ24)+5 种基金China Postdoctoral Science Foundation(No.2016M590619,No.2016M601878)Provincial Key Research and Development Program of Shaanxi(No.2019GY-197)the Qingchuang Talents Induction Program of Shandong Higher Education Institution(Research and Innovation Team of Structural-Functional Polymer Composites)the support from The Thousand Talents PlanThe World-Class University and DisciplineThe Taishan Scholar’s Advantageous and Distinctive Discipline Program of Shandong ProvinceThe World-Class Discipline Program of Shandong Province。
文摘The reasonable design of the composition of the composite materials is of great significance to optimized the electromagnetic(EM)wave absorption performance.Herein,the Ni/NiO@C hybrid composites with tunable Ni proportion were successfully synthesized through a two-step process.With the assistance of X-ray diffraction with refinement treatment,the specific proportion of Ni of as-obtained hybrid composites could be obtained.Employing controlling calcination time to adjust the Ni content of Ni/NiO@C hybrid composites,it has been found that the composite carbonized at 500℃exhibited remarkable EM wave absorption with the minimum reflection loss(RLmin)of-49.1 dB at 4.9 mm and the widest effective absorption bandwidth(EABmax)of 4.56 GHz at 2.1 mm.Moreover,by adjusting the Ni source,the optimal EM wave absorption performance could be achieved.Results illustrated that the N3PC with the Ni proportion of 13.17%showed the RLm inas low as-51.1 dB at 2.4 mm and the EABmax was 5.12 GHz at 2.7 mm.It is worth noting that this work demonstrates the relevance of the composition and EM wave absorption performance of hybrid composites,which offers a feasible reference for the absorption mechanism of absorber.
基金financial support from the National Natural Science Foundation of China(Nos.21776026,22075034,and 22178037)the Liaoning Revitalization Talents Program,China(Nos.XLYC1902037 and XLYC2002114)the Natural Science Foundation of Liaoning Province of China(No.2021-MS-303)。
文摘Electromagnetic wave(EMW)-absorbing materials have considerable capacity in the military field and the prevention of EMW radiation from harming human health.However,obtaining lightweight,high-performance,and broadband EMW-absorbing material remains an overwhelming challenge.Creating dielectric/magnetic composites with customized structures is a strategy with great promise for the development of high-performance EMW-absorbing materials.Using layered double hydroxides as the precursors of bimetallic alloys and combining them with porous biomass-derived carbon materials is a potential way for constructing multi-interface heterostructures as efficient EMW-absorbing materials because they have synergistic losses,low costs,abundant resources,and light weights.Here,FeNi alloy nanosheet array/Lycopodium spore-derived carbon(FeNi/LSC)was prepared through a simple hydrothermal and carbonization method.FeNi/LSC presents ideal EMW-absorbing performance by benefiting from the FeNi alloy nanosheet array,sponge-like structure,capability for impedance matching,and improved dielectric/magnetic losses.As expected,FeNi/LSC exhibited the minimum reflection loss of-58.3 dB at 1.5 mm with 20wt%filler content and a widely effective absorption bandwidth of 4.92 GHz.FeNi/LSC composites with effective EMW-absorbing performance provide new insights into the customization of biomass-derived composites as high-performance and lightweight broadband EMW-absorbing materials.
文摘For active wave absorbers in force-control mode,the optimal feedback(control)force provided by the control system depends on the hydrodynamic forces.This work investigates a piston-type wave absorber with different draft-to-water depth ratios,focusing on the frequency-dependent hydrodynamic coefficients,wave absorption efficiency,wave absorber displacement and velocity,and control force.Analytical results were derived based on potential flow theory,confirming that regular incident waves can be fully absorbed by the piston-type active wave absorber at any draft ratio by optimizing the control force.The results for the wave tank with a typical water depth of 3 m were studied in detail.The draft ratio has a strong influence on the hydrodynamic coefficients.At the maximum wave absorption efficiency,the displacement and velocity amplitudes are sensitive to the draft ratio in the low-frequency region,increase with decreasing draft ratio,and are independent of the mass of the wave absorber.The control force required can be extremely large for a draft ratio greater than 1/3.The control force increases significantly as the draft ratio increases.The mass of the wave absorber has a weak influence on the control force.A time-domain numerical method based on the boundary element method was developed to verify the analytical solutions.Perfect agreements between the analytical solutions and the numerical results were obtained.