The research on two-dimensional(2D)magnetic materials and their heterostructures is crucial in fields like spintronics,materials science,and condensed matter physics.This study uses terahertz(THz)time-domain spectrosc...The research on two-dimensional(2D)magnetic materials and their heterostructures is crucial in fields like spintronics,materials science,and condensed matter physics.This study uses terahertz(THz)time-domain spectroscopy to investigate ultrafast electron transport properties in both van der Waals Fe_(4)GeTe_(2)films and Bi_(2)Te_(3)/Fe_(4)GeTe_(2)ferromagnetic/topological heterostructures.Our results show that these heterostructures exhibit effective THz electromagnetic shielding.The complex conductivity spectra of Fe_(4)GeTe_(2)films and Bi_(2)Te_(3)/Fe_(4)GeTe_(2)heterostructures with varying Fe_(4)GeTe_(2)thicknesses are analyzed using the Drude-Smith model.We quantitatively examine how Fe_(4)GeTe_(2)layer thickness affects the direct current conductivity,plasma frequency,carrier momentum scattering time,and back-scattering coefficient.As the number of Fe_(4)GeTe_(2)layers increases,intra-layer back-scattering events for charge carriers become more frequent.This work provides THz frequency spectra for both Fe_(4)GeTe_(2)and Bi_(2)Te_(3)/Fe_(4)GeTe_(2),aiding in the design and optimization of THz modulators and detectors.展开更多
基金Project supported by the National Key Research and Development Program of China(Grant No.2023YFF0719200)the National Natural Science Foundation of China(Grant Nos.62322115,U24A20226,61988102,and 62435010)+1 种基金the 111 Project(Grant No.D18014)the Science and Technology Commission of Shanghai Municipality(Grant Nos.22JC1400200 and 21S31907400)。
文摘The research on two-dimensional(2D)magnetic materials and their heterostructures is crucial in fields like spintronics,materials science,and condensed matter physics.This study uses terahertz(THz)time-domain spectroscopy to investigate ultrafast electron transport properties in both van der Waals Fe_(4)GeTe_(2)films and Bi_(2)Te_(3)/Fe_(4)GeTe_(2)ferromagnetic/topological heterostructures.Our results show that these heterostructures exhibit effective THz electromagnetic shielding.The complex conductivity spectra of Fe_(4)GeTe_(2)films and Bi_(2)Te_(3)/Fe_(4)GeTe_(2)heterostructures with varying Fe_(4)GeTe_(2)thicknesses are analyzed using the Drude-Smith model.We quantitatively examine how Fe_(4)GeTe_(2)layer thickness affects the direct current conductivity,plasma frequency,carrier momentum scattering time,and back-scattering coefficient.As the number of Fe_(4)GeTe_(2)layers increases,intra-layer back-scattering events for charge carriers become more frequent.This work provides THz frequency spectra for both Fe_(4)GeTe_(2)and Bi_(2)Te_(3)/Fe_(4)GeTe_(2),aiding in the design and optimization of THz modulators and detectors.
