In this work,molybdenum disulfide quantum dots（MoS2 QDs） were firstly prepared by hydrothermal method using sodium molybdate and glutathione as precursors,and applied in ascorbic acid detection.When joining MnO2 nan...In this work,molybdenum disulfide quantum dots（MoS2 QDs） were firstly prepared by hydrothermal method using sodium molybdate and glutathione as precursors,and applied in ascorbic acid detection.When joining MnO2 nanosheets into MoS2 QDs solution,they produced an obvious fluorescence quenching,which should be due to inner filter effect（IFE）.Meanwhile,the fluorescent probe was formed,Interestingly,we found that this quenching phenomenon disappeared with the addition of ascorbic acid,In other words,the fluorescence gradually restored.This recovery phenomenon is mainly due to the reduction effect of ascorbic acid for MnO2 nanosheets.Under the optimum conditions,the limit of detection（LOD） of 39 nmol/L for ascorbic acid was achieved with a linear range of 0.33-5.00 μmol/L.The repeatability was better than 5.0% for ascorbic acid in both standard and fruit samples（n = 3）.Moreover,the as-fabricated fluorescent sensing system was successfully employed to detect the ascorbic acid levels in hawthorn and jujube with satisfactory results.展开更多
This paper proposes a simple and efficient distributed algorithm for calculating minimal dominating set in wireless sensor network. This method can avoid maintaining the connectivities between backbone hosts. Consider...This paper proposes a simple and efficient distributed algorithm for calculating minimal dominating set in wireless sensor network. This method can avoid maintaining the connectivities between backbone hosts. Considering that the hosts in mobile networks have different characteristics, this paper proposes a method of calculating minimal dominating set with weight. The nodes can be chosen to form a minimal dominating set when the network topology changes. For the host switch on/off operation, the updating algorithm was provided. The change in the status of a hostaffects only the status of hosts in the restricted vicinity. Simulation results show that the proposed method can ensure fewer dominators but with higher weight to form the minimal dominating set and the nodes can be adaptive to the changes of network topology.展开更多
Up to now,“Turn-on”fluorescence sensor exhibits promising potential toward the detection of heavy metal ions,anions,drugs,organic dyes,DNA,pesticides,and other amino acids due to their simple,quick detection,and hig...Up to now,“Turn-on”fluorescence sensor exhibits promising potential toward the detection of heavy metal ions,anions,drugs,organic dyes,DNA,pesticides,and other amino acids due to their simple,quick detection,and high sensitivity and selectivity.Herein,a novel fluorescence method of detecting Cr^(3+)in an aqueous solution was described based on the fluorescence resonance energy transfer between rhodamine B(Rh B)and gold nanoparticles(Au NPs).The fluorescence of Rh B solution could be obviously quenched(“off”state)with the presence of citrate-stabilized Au NPs.However,upon addition of Cr^(3+)to Au NPs@Rh B system,the fluorescence of Au NPs was recovered owing to the strong interaction between Cr^(3+)and the specific groups on the surface of citrate-stabilized Au NPs,which will lead to the aggregation of Au NPs(“on”state).At this point,the color of the reaction solution turned to black.Under optimal conditions,the limit of detection(LOD)for Cr^(3+)was 0.95 n M(signal-to-noise ratio,S/N=3)with a linear range of 0.164 n M to 3.270μM.Furthermore,the proposed method exhibits excellent performances,such as rapid analysis,high sensitivity,extraordinary selectivity,easy preparation,switch-on fluorescence response,and non-time consuming.展开更多
在复合功率分流混合动力系统中,通过离合器对功率分流装置与动力部件进行离合和制动,可以进一步提高动力性和经济性。传统湿式离合器为适应商用车大扭矩需求,需增加摩擦片数量和体积,导致成本上升和拖曳损失,而机械式离合器虽体积小、...在复合功率分流混合动力系统中,通过离合器对功率分流装置与动力部件进行离合和制动,可以进一步提高动力性和经济性。传统湿式离合器为适应商用车大扭矩需求,需增加摩擦片数量和体积,导致成本上升和拖曳损失,而机械式离合器虽体积小、承载扭矩大,但在超越过程中产生摩擦损失,无法满足混合动力商用车对可控方向锁止和双向非接触自由的需求。设计了一种多模非接触式可控单向离合器,可实现正向锁止、反向锁止以及双向自由三种模式,承载扭矩大同时避免了拖曳和摩擦损失。对多模非接触式可控单向离合器静态和模式切换过程进行了分析,以提高承载扭矩、减小瞬态冲击和实现轻量设计为目标建立了优化模型,提出融合带精英策略的非支配排序遗传算法(Non-dominated sorting genetic algorithmⅡ,NSGA2)、约束有序加权平均算子(Constrained ordered weighted averaging,COWA)和优劣解距离法(Technique for order preference by similarity to ideal solution,TOPSIS)的多目标优化决策方法,与初始方案相比,承载扭矩提升了23.5%、空转角减少了13.7%、关键部件体积减小了0.5%;搭载混合动力专用变速箱进行了台架试验,验证了设计方法的可行性。研究为大扭矩多模非接触式可控单向离合器的设计提供了参考。展开更多
基金financially supported by National Nature Science Foundation of China (No. 21475053)
文摘In this work,molybdenum disulfide quantum dots（MoS2 QDs） were firstly prepared by hydrothermal method using sodium molybdate and glutathione as precursors,and applied in ascorbic acid detection.When joining MnO2 nanosheets into MoS2 QDs solution,they produced an obvious fluorescence quenching,which should be due to inner filter effect（IFE）.Meanwhile,the fluorescent probe was formed,Interestingly,we found that this quenching phenomenon disappeared with the addition of ascorbic acid,In other words,the fluorescence gradually restored.This recovery phenomenon is mainly due to the reduction effect of ascorbic acid for MnO2 nanosheets.Under the optimum conditions,the limit of detection（LOD） of 39 nmol/L for ascorbic acid was achieved with a linear range of 0.33-5.00 μmol/L.The repeatability was better than 5.0% for ascorbic acid in both standard and fruit samples（n = 3）.Moreover,the as-fabricated fluorescent sensing system was successfully employed to detect the ascorbic acid levels in hawthorn and jujube with satisfactory results.
基金Supported by National Natural Science Foundation of China (No.60973141)Natural Science Foundation of Tianjin (No.09JCYBJC00300)
文摘This paper proposes a simple and efficient distributed algorithm for calculating minimal dominating set in wireless sensor network. This method can avoid maintaining the connectivities between backbone hosts. Considering that the hosts in mobile networks have different characteristics, this paper proposes a method of calculating minimal dominating set with weight. The nodes can be chosen to form a minimal dominating set when the network topology changes. For the host switch on/off operation, the updating algorithm was provided. The change in the status of a hostaffects only the status of hosts in the restricted vicinity. Simulation results show that the proposed method can ensure fewer dominators but with higher weight to form the minimal dominating set and the nodes can be adaptive to the changes of network topology.
基金supported by the Natural Science Foundation of Qinghai Province in China(No.2019-ZJ-944Q)the University-level Planning Project of Qinghai Minzu University of Qinghai Province in China(Nos.2022GH11 and 2022GH13)。
文摘Up to now,“Turn-on”fluorescence sensor exhibits promising potential toward the detection of heavy metal ions,anions,drugs,organic dyes,DNA,pesticides,and other amino acids due to their simple,quick detection,and high sensitivity and selectivity.Herein,a novel fluorescence method of detecting Cr^(3+)in an aqueous solution was described based on the fluorescence resonance energy transfer between rhodamine B(Rh B)and gold nanoparticles(Au NPs).The fluorescence of Rh B solution could be obviously quenched(“off”state)with the presence of citrate-stabilized Au NPs.However,upon addition of Cr^(3+)to Au NPs@Rh B system,the fluorescence of Au NPs was recovered owing to the strong interaction between Cr^(3+)and the specific groups on the surface of citrate-stabilized Au NPs,which will lead to the aggregation of Au NPs(“on”state).At this point,the color of the reaction solution turned to black.Under optimal conditions,the limit of detection(LOD)for Cr^(3+)was 0.95 n M(signal-to-noise ratio,S/N=3)with a linear range of 0.164 n M to 3.270μM.Furthermore,the proposed method exhibits excellent performances,such as rapid analysis,high sensitivity,extraordinary selectivity,easy preparation,switch-on fluorescence response,and non-time consuming.
文摘在复合功率分流混合动力系统中,通过离合器对功率分流装置与动力部件进行离合和制动,可以进一步提高动力性和经济性。传统湿式离合器为适应商用车大扭矩需求,需增加摩擦片数量和体积,导致成本上升和拖曳损失,而机械式离合器虽体积小、承载扭矩大,但在超越过程中产生摩擦损失,无法满足混合动力商用车对可控方向锁止和双向非接触自由的需求。设计了一种多模非接触式可控单向离合器,可实现正向锁止、反向锁止以及双向自由三种模式,承载扭矩大同时避免了拖曳和摩擦损失。对多模非接触式可控单向离合器静态和模式切换过程进行了分析,以提高承载扭矩、减小瞬态冲击和实现轻量设计为目标建立了优化模型,提出融合带精英策略的非支配排序遗传算法(Non-dominated sorting genetic algorithmⅡ,NSGA2)、约束有序加权平均算子(Constrained ordered weighted averaging,COWA)和优劣解距离法(Technique for order preference by similarity to ideal solution,TOPSIS)的多目标优化决策方法,与初始方案相比,承载扭矩提升了23.5%、空转角减少了13.7%、关键部件体积减小了0.5%;搭载混合动力专用变速箱进行了台架试验,验证了设计方法的可行性。研究为大扭矩多模非接触式可控单向离合器的设计提供了参考。
