This study investigates the performance boundaries of ramjet and scramjet engines fueled by boronbased propellant through full-scale engine modeling and three-dimensional computational fluid dynamics simulations.Resul...This study investigates the performance boundaries of ramjet and scramjet engines fueled by boronbased propellant through full-scale engine modeling and three-dimensional computational fluid dynamics simulations.Results show that the performance boundary between ramjets and scramjets occurs near Mach 7.Specifically,at Mach 6,the ramjet exhibits a 1290 m/s higher specific impulse than the scramjet;however,at Mach 7,their performance becomes comparable.The ramjet's higher static temperature promotes boron particle vaporization and B_(2)O_(2) dissociation,limiting the total temperature increase,unlike in scramjets.The boron vapor mass fraction significantly impacts this temperature difference,with ramjets exhibiting values 8.5 and 3.9 times higher than scramjets at Mach 6 and Mach 7,respectively.Despite lower total temperatures,ramjets achieve more efficient boron combustion due to the combined effects of higher pressures and longer particle residence times.These findings offer valuable insights for engine designers in selecting ramjet or scramjet configurations for boron-fueled propulsion systems.展开更多
Probiotics can regulate the body’s immune system through both non-specific and specific immunity,thereby regulating host health.In terms of non-specific immune regulation,probiotics can activate the intrinsic immune ...Probiotics can regulate the body’s immune system through both non-specific and specific immunity,thereby regulating host health.In terms of non-specific immune regulation,probiotics can activate the intrinsic immune system,regulate the mucosal barrier function,and play an immune role by influencing the activity of intrinsic immune cells such as macrophages,dendritic cells and natural killer cells,as well as their differentiation and maturation;in terms of specific immune regulation,probiotics play a role in regulating the immunoglobulin level and the maturation of B cells.Probiotics can also regulate T-cell differentiation according to the condition of the body,thus regulating specific immunity.Many studies have focused on the role of probiotics in metabolism and nutrition,and the mechanisms involved in the immunomodulatory role of probiotics have only been partially described.This review summarises the role of common probiotics such as Lactobacillus plantarum and Lactobacillus rhamnosus in immunomodulation as well as their mechanisms,describing the currently known mechanisms of immunomodulation by probiotics in improving the host immune system.A deeper understanding of probiotics and their specific mechanisms of action will facilitate the use of probiotics for immunomodulation in clinical medicine,functional foods,and other areas.This will also contribute to the development and research of engineered probiotics,next-generation probiotics,and other new functional probiotics with immunomodulatory effects.展开更多
Stem cell proliferation is tightly regulated in developing and adult tissues through the coordinated action of cell-intrinsic and extracellular signals.Although many extracellular cues were identified,the cell-intrins...Stem cell proliferation is tightly regulated in developing and adult tissues through the coordinated action of cell-intrinsic and extracellular signals.Although many extracellular cues were identified,the cell-intrinsic mechanisms underlying the decision of a stem cell to proliferate,enter a dormant quiescent state or differentiate into a specific cell type remains incompletely understood.展开更多
The establishment of plantations has become a critical approach for reducing greenhouse gas emissions,particularly in fragile environments with carbon sequestration potential.In karst areas,plantations based on fastgr...The establishment of plantations has become a critical approach for reducing greenhouse gas emissions,particularly in fragile environments with carbon sequestration potential.In karst areas,plantations based on fastgrowing afforestation species made significant contributions to enhancing carbon sequestration.However,the impact of understory vegetation on carbon accumulation remains unclear.Especially,the carbon accumulation associated with litter produced during the replacement of understory species receives insufficient attention,which leads to the neglect of the carbon sequestration potential in plantations of karst areas.Leaf is a crucial organ that links the litter production.To explore how leaf traits adapt to competitive environments and drive litter carbon accumulation during understory species replacement,this study observed leaf traits and litter carbon content changes in three types of plantations in the Liujiang River Basin,a typical karst area.A total of 37 sampling plots were selected for field investigation over a twoyear period.Leaf traits,species diversity,vegetation coverage,and litter carbon characteristics in understory vegetation were measured.Variance analysis,allometric equations,and path analysis were used for data analysis.The results showed that most understory species adopted a biomass conservation strategy under high-coverage conditions(>44.27%)and expanded competitive leaf area under low-coverage conditions(<44.27%).However,Bidens pilosa and Miscanthus floridulus exhibited strong competitiveness during understory species replacement.They showed an expansion of competitive leaf area under high-coverage conditions.This competitive strategy reduced species diversity and community specific leaf area.But the rapid expansion of Bidens pilosa and Miscanthus floridulus increased understory vegetation coverage,and their increased specific leaf area facilitated leaf shedding,resulting in significant litter weight accumulation(P<0.05),thereby enhancing litter carbon content per unit area.These competitive strategies were key driving factors for the increase in litter carbon content per square meter,which reached a maximum of 49.6% higher than that in natural grasslands.And the maximum increase in litter carbon accumulation derived from understory vegetation reached 3.37 times from 2023 to 2024 in plantations.In the understory vegetation of plantations,the competitive strategies reflected by leaf adaptation of key competitive species are critical factors influencing litter carbon accumulation.Future research could deeply explore the carbon sequestration effects resulting from the dynamic changes in competition within the understory vegetation of plantations.展开更多
The specific surface area(S S)and pore size(D)exhibit an inherent trade-off in the microscale design of bone implants:larger pores typically correlate with reduced surface area and vice versa.This relationship has att...The specific surface area(S S)and pore size(D)exhibit an inherent trade-off in the microscale design of bone implants:larger pores typically correlate with reduced surface area and vice versa.This relationship has attracted notable attention because of its critical role in the regulation of cell adhesion and osteogenesis.However,it remains largely unclear how S S and D affect the generated bone tissue and dynamically change during long-term osteogenesis.Herein,by applying rigorous geometric mapping to minimal surfaces,we constructed precisely partitioned and layer-by-layer thickened tissue models to simulate osteogenesis across different temporal scales and thereby track the dynamic evolution of geometric characteristics,permeability,and mechanobiological tissue differentiation.The high-S S samples were found to facilitate the rapid formation of new bone tissue in the early stages.However,their smaller pores tended to cause occlusions,hindering further tissue development.In contrast,low-S S samples showed slower bone regeneration,but their larger pores provided adequate physical space for tissue regeneration and mass transport,ultimately promoting bone formation in the long term.Mechanobiological regulation suggests that fibrous tissue formation inhibits additional bone formation,establishing a dynamic equilibrium between osteogenesis and pore space to sustain nutrient/waste exchange throughout the regenerative process.Overall,smaller pores are preferable in implants for minimally loaded osteoplasty procedures focused on early-stage bone consolidation,whereas larger pores are preferable in dynamically loaded implants requiring prolonged mechanical stability.展开更多
In wireless sensor networks,ensuring communication security via specific emitter identification(SEI)is crucial.However,existing SEI methods are limited to closed-set scenarios and lack the ability to detect unknown de...In wireless sensor networks,ensuring communication security via specific emitter identification(SEI)is crucial.However,existing SEI methods are limited to closed-set scenarios and lack the ability to detect unknown devices and perform classincremental training.This study proposes a class-incremental open-set SEI approach.The open-set SEI model calculates radiofrequency fingerprints(RFFs)prototypes for known signals and employs a self-attention mechanism to enhance their discriminability.Detection thresholds are set through Gaussian fitting for each class.For class-incremental learning,the algorithm freezes the parameters of the previously trained model to initialize the new model.It designs specific losses:the RFFs extraction distribution difference loss and the prototype transformation distribution difference loss,which force the new model to retain old knowledge while learning new knowledge.The training loss enables learning of new class RFFs.Experimental results demonstrate that the open-set SEI model achieves state-of-theart performance and strong noise robustness.Moreover,the class-incremental learning algorithm effectively enables the model to retain old device RFFs knowledge,acquire new device RFFs knowledge,and detect unknown devices simultaneously.展开更多
A surface pyrolysis and gas-phase combustion of the Ammonium Perchlorate(AP)/Hydroxy Terminated Polybutadiene(HTPB)composite propellant reaction kinetic mechanism with five-step chemical reaction is adopted.The effect...A surface pyrolysis and gas-phase combustion of the Ammonium Perchlorate(AP)/Hydroxy Terminated Polybutadiene(HTPB)composite propellant reaction kinetic mechanism with five-step chemical reaction is adopted.The effects of helium injection on the burning rate and combustion of AP/HTPB propellant are analyzed in details,and the characteristics of motor performance are obtained.The numerical simulation results demonstrate that helium injection enhances the combustion chamber pressure,thereby increasing the burning rate of propellant.However,the primary combustion reaction of the AP/HTPB propellant takes place within a thin layer on the burning surface,so the low-temperature helium has minimal impact on the gasphase combustion.Ultimately,the helium not only elevates the nozzle exit velocity,resulting in specific impulse gain,but also reduces the exhaust plume temperature.With an increase of helium mass flow rate,the area of the velocity increase zone at the nozzle exit continuously decreases,but the average velocity in the motor exit continuously increases.Overall,when the helium flow rate is 2.5 kg/s,the specific impulse can reach 10.5%.Reducing the helium injection hole diameter enhances mixing of helium and combustion gas and expands the velocity increase zone,thereby maximizing the exit velocity gain in average velocity at the nozzle exit.When the injection hole diameter is reduced from 100 mm to 20 mm,the specific impulse gain increases from 3.1%to 10.6%.Furthermore,increasing helium injection temperature greatly boosts the velocity of the mixed gas with the same helium mass fraction ultimately improving specific impulse.展开更多
Dear Editor,Social anxiety disorder(SAD)is a prevalent psychiatric disorder,characterized by persistent and excessive fear of social situations in which the individual may be scrutinized by others[1].Typically emergin...Dear Editor,Social anxiety disorder(SAD)is a prevalent psychiatric disorder,characterized by persistent and excessive fear of social situations in which the individual may be scrutinized by others[1].Typically emerging in late childhood or adolescence with potential lifelong persistence,SAD significantly impairs interpersonal relationships,educational attainment,and occupational performance[2].Furthermore,SAD demonstrates high comorbidity rates with other mental disorders,including anxiety disorders,substanceuse disorder,and major depressive disorder[3].Current therapeutic interventions remain limited,with suboptimal response to existing psychological and pharmacological treatments in many patients,while the pathological mechanisms underlying SAD continue to elude comprehensive understanding[4].Establishing appropriate animal models is essential to investigating SAD's neural mechanisms and pathological underpinnings and developing effective therapeutic interventions.展开更多
Hierarchical porous MgO is a promising adsorbent for dye removal because of its large Brunauer-Emmett-Teller specific surface area(SBET)and abundant low-coordinated oxygen anions(LCO)sites.As hierarchical porous MgO p...Hierarchical porous MgO is a promising adsorbent for dye removal because of its large Brunauer-Emmett-Teller specific surface area(SBET)and abundant low-coordinated oxygen anions(LCO)sites.As hierarchical porous MgO particles with large SBET values are typically prepared by complicated procedures under harsh conditions,such as high temperatures and high pressures,their large-scale production is impractical.Consequently,the preparation of hierarchical porous MgO with a large SBET value under mild conditions is highly desirable.In this study,a morphology transition engineering strategy is introduced to change the morphology of simple MgO microspheres to an embroidered ball-shaped with a larger SBET value via hydrolysis and calcination without using surfactants as sacrificial templates.During hydrolysis,numerous Mg(OH)_(2)sheets form and attach to the MgO surface,thus increasing the SBET value of the newly obtained MgO that forms by calcination(denoted as NM-x,where x is the hydrolysis time in hours).The sizes of the crystalline sheets were tuned by controlling the hydrolysis time.NM-12 exhibited the highest density of small-sized sheets on its surface and the largest SBET value of 180.17 m^(2)g^(-1),which was 3.51 times that of the MgO precursor(51.89 m^(2)g^(-1)).However,NM-24(134.07 m^(2)g^(-1))had a higher adsorption efficiency for Congo red(CR)than NM-12,despite having a smaller SBET value,which indicates that other factors are involved.NM-24 exhibited a lower probability of exposed(200)and(220)facets which were verified to repulse CR molecules by molecular dynamics simulations,and a greater number of LCO sites,which contributed to adsorption.Thus,this study introduces a facile method for preparing hierarchical porous MgO and examines the effects of LCO sites and exposed facet probabilities on its adsorption properties.展开更多
Coconut(Cocos nucifera L.),a major oil and fruit crop of the Arecaceae family,is extensively cultivated across the Asia—Pacific region.Despite its agricultural importance,genome assembly in coconut remains challengin...Coconut(Cocos nucifera L.),a major oil and fruit crop of the Arecaceae family,is extensively cultivated across the Asia—Pacific region.Despite its agricultural importance,genome assembly in coconut remains challenging due to its large genome size and high proportion of repetitive sequences.Allele-specific expression(ASE)plays a key role in regulating plant development and evolution,yet research on ASE in coconut is limited(Shao et al.,2019;Li et al.,2021;Zhang et al.,2021;Hu et al.,2022).Among phenotypic traits,fruit color is especially important as an indicator of maturity,guiding harvest timing and post-harvest processes(Kapoor et al.,2022).While prior studies have explored various coconut traits such as salt tolerance,fiber content,and plant height(Wang et al.,2021;Yang et al.,2021),investigations into ASE and fruit color remain scarce.展开更多
Prostate-specific membrane antigen(PSMA)is a surface membrane antigen that is highly overexpressed in prostate cancer,with heterogenous expression throughout the natural history of the disease.This has generated signi...Prostate-specific membrane antigen(PSMA)is a surface membrane antigen that is highly overexpressed in prostate cancer,with heterogenous expression throughout the natural history of the disease.This has generated significant interest as a potential biomarker for use in early diagnosis and treatment of prostate cancer.We reviewed the literature surrounding PSMA and its current clinical applications in diagnosing and managing early prostate cancer that is confined to the prostate and local lymph nodes.A search on PubMed,Medline,and Web of Science was performed using the following keywords:“PSMA”,“Prostate Specific Membrane Antigen”,“Prostate cancer”,“Biomarker”,“Diagnosis”.We considered all available articles relevant to the topic of PSMA as a biomarker in early prostate cancer when developing this narrative review.Key articles assessing the biology of PSMA,as well as its use as a potential diagnostic and therapeutic target in early prostate cancer,were assessed.The role of PSMA PET as a potential diagnostic and risk stratification tool was assessed.The current use of antibody-drug conjugates and radioligand therapy targeting PSMA was assessed,along with any current evidence to support their use in early prostate cancer.PSMA is heavily expressed throughout the early stages of prostate cancer,and this has significant therapeutic implications.There is a growing body of evidence that shows PSMA PET can play a role in the diagnosis,risk stratification,and prognostication of localised prostate cancer.PSMA-targeted therapies such as Lu-177 currently do not have any proven benefit in treating early prostate cancer;however,this remains an area of ongoing research.展开更多
Alzheimer’s disease(AD)is the most common form of dementia.In addition to the lack of effective treatments,there are limitations in diagnostic capabilities.The complexity of AD itself,together with a variety of other...Alzheimer’s disease(AD)is the most common form of dementia.In addition to the lack of effective treatments,there are limitations in diagnostic capabilities.The complexity of AD itself,together with a variety of other diseases often observed in a patient’s history in addition to their AD diagnosis,make deciphering the molecular mechanisms that underlie AD,even more important.Large datasets of single-cell RNA sequencing,single-nucleus RNA-sequencing(snRNA-seq),and spatial transcriptomics(ST)have become essential in guiding and supporting new investigations into the cellular and regional susceptibility of AD.However,with unique technology,software,and larger databases emerging;a lack of integration of these data can contribute to ineffective use of valuable knowledge.Importantly,there was no specialized database that concentrates on ST in AD that offers comprehensive differential analyses under various conditions,such as sex-specific,region-specific,and comparisons between AD and control groups until the new Single-cell and Spatial RNA-seq databasE for Alzheimer’s Disease(ssREAD)database(Wang et al.,2024)was introduced to meet the scientific community’s growing demand for comprehensive,integrated,and accessible data analysis.展开更多
Deep brain sti mulation(DBS)is a neuromodulation tool that involves the delivery of electrical impulses to specific brain regions through implanted electrodes.The principle behind DBS is to modulate dysfunctional neur...Deep brain sti mulation(DBS)is a neuromodulation tool that involves the delivery of electrical impulses to specific brain regions through implanted electrodes.The principle behind DBS is to modulate dysfunctional neural circuits without the need for permanent structural alterations to the brain.Initially developed as a treatment for movement disorders such as Parkinson's disease(PD),DBS has expanded to encompass various neurological and psychiatric disorders.展开更多
Despite the superior advantages of specific emitter identification in extracting emitter features from in-phase and quadrature(I/Q)signals,challenges persist due to signal-type confusion and background noise interfere...Despite the superior advantages of specific emitter identification in extracting emitter features from in-phase and quadrature(I/Q)signals,challenges persist due to signal-type confusion and background noise interference.To address those limitations,this paper proposes a multi-channel contrast prediction coding and complex-valued residuals network(MCPC-MCVResNet)framework.This model employs contrast prediction techniques to directly extract discriminative features from electromagnetic signal sequences,effectively capturing both amplitude and phase information within I/Q data.A core innovation of this approach is the sphere space softmax(SS-softmax)loss,which optimizes intra-class clustering density of while establishing well-defined boundaries between distinct emitters.The SS-softmax mechanism significantly enhances the model's capacity to discern subtle variations among radiation emitters.Experimental results demonstrate superior identification accuracy,rapid convergence,and exceptional robustness in low signal-to-noise ratio environments.展开更多
Supercapacitors are gaining popularity due to their high cycling stability,power density,and fast charge and discharge rates.Researchers are ex-ploring electrode materials,electrolytes,and separat-ors for cost-effecti...Supercapacitors are gaining popularity due to their high cycling stability,power density,and fast charge and discharge rates.Researchers are ex-ploring electrode materials,electrolytes,and separat-ors for cost-effective energy storage systems.Ad-vances in materials science have led to the develop-ment of hybrid nanomaterials,such as combining fil-amentous carbon forms with inorganic nanoparticles,to create new charge and energy transfer processes.Notable materials for electrochemical energy-stor-age applications include MXenes,2D transition met-al carbides,and nitrides,carbon black,carbon aerogels,activated carbon,carbon nanotubes,conducting polymers,carbon fibers,and nanofibers,and graphene,because of their thermal,electrical,and mechanical properties.Carbon materials mixed with conducting polymers,ceramics,metal oxides,transition metal oxides,metal hydroxides,transition metal sulfides,trans-ition metal dichalcogenide,metal sulfides,carbides,nitrides,and biomass materials have received widespread attention due to their remarkable performance,eco-friendliness,cost-effectiveness,and renewability.This article explores the development of carbon-based hybrid materials for future supercapacitors,including electric double-layer capacitors,pseudocapacitors,and hy-brid supercapacitors.It investigates the difficulties that influence structural design,manufacturing(electrospinning,hydro-thermal/solvothermal,template-assisted synthesis,electrodeposition,electrospray,3D printing)techniques and the latest car-bon-based hybrid materials research offer practical solutions for producing high-performance,next-generation supercapacitors.展开更多
The microstructural evolution,phase stability,and mechanical properties of Al-Li-Mg-Ti-M(M=Zn,Zr,V)lightweight high-entropy alloys(LW-HEAs)were investigated.The LW-HEAs with three components,Al_(20)Li_(20)Mg_(10)-Ti_(...The microstructural evolution,phase stability,and mechanical properties of Al-Li-Mg-Ti-M(M=Zn,Zr,V)lightweight high-entropy alloys(LW-HEAs)were investigated.The LW-HEAs with three components,Al_(20)Li_(20)Mg_(10)-Ti_(40)Zn_(10)(#Zn),Al_(20)Li_(20)Mg_(10)Ti_(30)Zr_(20)(#Zr),and Al_(20)Li_(20)Mg_(10)Ti_(30)V_(20)(#V),were designed according to the thermo-dynamic design criteria of HEA,and prepared via a combination process of mechanical alloying and cold-press sintering.The effects of alloy composition and sintering temperature on the microstructure and mechanical properties of the LW-HEAs were studied.The results show that the as-milled Al-Li-Mg-Ti-M(M=Zn,Zr,V)LW-HEAs form a simple structure with HCP-type solid solution as the primary phase,a dual-HCP type solid solution phase,and a BCC phase,respectively.After cold-press sintering,the#Zn and#V alloys undergo obvious phase transformation;while the#Zr alloy with dual-HCP phases exhibits the best phase stability during heat treatment.The#V-750°C alloy demonstrates the maximum hardness and specific strength of HV 595.2 and 625 MPa∙cm3/g,respectively,under the combined effect of solid solution strengthening of BCC phase and precipitation strengthening ofβ-AlTi_(3).Moreover,the#Zr-650°C,#Zr-750°C,and#Zn-650°C alloys are expected to have excellent plasticity.展开更多
Fully implanted brain-computer interfaces(BCIs)are preferred as they eliminate signal degradation caused by interference and absorption in external tissues,a common issue in non-fully implanted systems.To optimize the...Fully implanted brain-computer interfaces(BCIs)are preferred as they eliminate signal degradation caused by interference and absorption in external tissues,a common issue in non-fully implanted systems.To optimize the design of electroencephalography electrodes in fully implanted BCI systems,this study investigates the penetration and absorption characteristics of microwave signals in human brain tissue at different frequencies.Electromagnetic simulations are used to analyze the power density distribution and specific absorption rate(SAR)of signals at various frequen-cies.The results indicate that lower-frequency signals offer advantages in terms of power density and attenuation coeffi-cients.However,SAR-normalized analysis,which considers both power density and electromagnetic radiation hazards,shows that higher-frequency signals perform better at superficial to intermediate depths.Specifically,at a depth of 2 mm beneath the cortex,the power density of a 6.5 GHz signal is 247.83%higher than that of a 0.4 GHz signal.At a depth of 5 mm,the power density of a 3.5 GHz signal exceeds that of a 0.4 GHz signal by 224.16%.The findings suggest that 6.5 GHz is optimal for electrodes at a depth of 2 mm,3.5 GHz for 5 mm,2.45 GHz for depths of 15-20 mm,and 1.8 GHz for 25 mm.展开更多
The ACF adsorbent with high Cu loading was treated with dielectric barrier discharge plasma to mitigate the negative effects of high Cu loading and enhance PH_(3)and H_(2)S adsorption and oxidation.Bruno-Emmett-Taylor...The ACF adsorbent with high Cu loading was treated with dielectric barrier discharge plasma to mitigate the negative effects of high Cu loading and enhance PH_(3)and H_(2)S adsorption and oxidation.Bruno-Emmett-Taylor(BET)result showed that the specific surface area of the adsorbent after air plasma modification was almost three times that before modification.X-ray photoelectron spectroscopy(XPS)findings revealed that the amino group was added to the adsorbent's surface,increasing lattice oxygen and chemisorbed oxygen.The adsorbent's large specific surface area,excellent surface active oxygen,and abundance of basic groups facilitate PH_(3)and H_(2)S adsorption and oxidation.The scanning electron microscopy showed that air plasma modification exposed more active components and uniformly dispersed them on the surface of adsorbent,thereby improving the adsorption performance.Activity evaluation results showed that the adsorbent has the best ability to capture PH_(3)and H_(2)S after being modified by air plasma at 4 kV voltage for 10 min.The adsorbent's breakthrough ability at high space velocity(WHSV:60,000 h^(−1))is 190 mg P/g and 146 mg S/g,respectively,which is 74%and 60%greater than that before modification.This is a great improvement over previous studies.In addition,the possible mechanism of adsorbent deactivation was proposed.展开更多
Aqueous zinc-ion batteries(AZIBs)are gaining attention owing to their affordability,high safety,and high energy density,making them a promising solution for large-scale energy storage.However,their performance is hamp...Aqueous zinc-ion batteries(AZIBs)are gaining attention owing to their affordability,high safety,and high energy density,making them a promising solution for large-scale energy storage.However,their performance is hampered by the instability of both the anode-electrolyte interface and the cathode-electrolyte interface.The use of sodium gluconate(SG),an organic sodium salt with multiple hydroxyl groups,as an electrolyte additive is suggested.Experimental and theoretical analyses demonstrate that Na^(+)from SG can intercalate and deintercalate within the associated V_(2)O_(5) cathode during in situ electrochemical processes.This action supports the layered structure of V_(2)O_(5),prevents structural collapse and phase transitions,and enhances Zn^(2+)diffusion kinetics.Additionally,the gluconate anion disrupts the original Zn^(2+)solvation structure,mitigates water-induced side reactions,and suppresses Zn dendrite growth.The synchronous regulation of both the V_(2)O_(5) cathode and Zn anode by the SG additive leads to considerable performance improvements.Zn‖Zn symmetric batteries demonstrate a cycle life exceeding 2800 h at 0.5 mA cm^(-2)and 1 mAh cm^(-2).In Zn‖V_(2)O_(5) full batteries,a high specific capacity of 288.92 mAh g^(-1)and capacity retention of 82.29%are maintained over 1000 cycles at a current density of 2 A g^(-1).This multifunctional additive strategy offers a new pathway for the practical application of AZIBs.展开更多
The present study monitored bacterial succession,physicochemical properties,and volatile organic compounds(VOCs)changes in smoked chicken legs with modified atmosphere packaging(MAP,60% CO_(2) and 40%N_(2))during a 25...The present study monitored bacterial succession,physicochemical properties,and volatile organic compounds(VOCs)changes in smoked chicken legs with modified atmosphere packaging(MAP,60% CO_(2) and 40%N_(2))during a 25-day storage period at 4℃.After 15 days of storage,S erratia proteamaculans and Pseudomonas fragi became the predominant bacteria.Furthermore,physicochemical properties changed significantly,as evidenced by an increase in thiobarbituric acid reactive substances and b*(yellowness)value,and a decrease in hardness.A total of 65 VOCs were identified during storage.Correlation between bacterial succession and quality indicators(including VOCs and physicochemical properties)allowed the identification of 26 core dominant bacteria,including S.proteamaculans,Psychrobacter alimentarius,Pseudomonas putida,and Pseudomonas poae,which were positively related to spoilage VOCs(e.g.,1-octen-3-ol,1-pentanol,and 3-methyl-1-butanol)and could be defined as specific spoilage organisms(SSOs).The results of this study provide a systematic approach to predict SSOs in smoked chicken legs during storage,which can also provide a basis for product safety.展开更多
基金funded by the National Natural Science Foundation of China(Grant No.U21B2086)。
文摘This study investigates the performance boundaries of ramjet and scramjet engines fueled by boronbased propellant through full-scale engine modeling and three-dimensional computational fluid dynamics simulations.Results show that the performance boundary between ramjets and scramjets occurs near Mach 7.Specifically,at Mach 6,the ramjet exhibits a 1290 m/s higher specific impulse than the scramjet;however,at Mach 7,their performance becomes comparable.The ramjet's higher static temperature promotes boron particle vaporization and B_(2)O_(2) dissociation,limiting the total temperature increase,unlike in scramjets.The boron vapor mass fraction significantly impacts this temperature difference,with ramjets exhibiting values 8.5 and 3.9 times higher than scramjets at Mach 6 and Mach 7,respectively.Despite lower total temperatures,ramjets achieve more efficient boron combustion due to the combined effects of higher pressures and longer particle residence times.These findings offer valuable insights for engine designers in selecting ramjet or scramjet configurations for boron-fueled propulsion systems.
基金funded by Ausnutria-kabrita Research Fund(RS2022-14).
文摘Probiotics can regulate the body’s immune system through both non-specific and specific immunity,thereby regulating host health.In terms of non-specific immune regulation,probiotics can activate the intrinsic immune system,regulate the mucosal barrier function,and play an immune role by influencing the activity of intrinsic immune cells such as macrophages,dendritic cells and natural killer cells,as well as their differentiation and maturation;in terms of specific immune regulation,probiotics play a role in regulating the immunoglobulin level and the maturation of B cells.Probiotics can also regulate T-cell differentiation according to the condition of the body,thus regulating specific immunity.Many studies have focused on the role of probiotics in metabolism and nutrition,and the mechanisms involved in the immunomodulatory role of probiotics have only been partially described.This review summarises the role of common probiotics such as Lactobacillus plantarum and Lactobacillus rhamnosus in immunomodulation as well as their mechanisms,describing the currently known mechanisms of immunomodulation by probiotics in improving the host immune system.A deeper understanding of probiotics and their specific mechanisms of action will facilitate the use of probiotics for immunomodulation in clinical medicine,functional foods,and other areas.This will also contribute to the development and research of engineered probiotics,next-generation probiotics,and other new functional probiotics with immunomodulatory effects.
基金supported by the Argentine Agency for the Promotion of Science and Technology ANPCyT(PICT2019-1472 to GP,PICT2019-4597 to FL,PICT2020-1524 to GP,and PICT2021-00627 to FL)supported by an Independent Career Position from CONICETsupported by a postdoctoral fellowship from ANPCyT。
文摘Stem cell proliferation is tightly regulated in developing and adult tissues through the coordinated action of cell-intrinsic and extracellular signals.Although many extracellular cues were identified,the cell-intrinsic mechanisms underlying the decision of a stem cell to proliferate,enter a dormant quiescent state or differentiate into a specific cell type remains incompletely understood.
基金supported by the Scientific Research Foundation supported by Yunnan Agricultural University(A3012024035044)International Cooperation and Exchange of the National Natural Science Foundation of China(No.42361144885).
文摘The establishment of plantations has become a critical approach for reducing greenhouse gas emissions,particularly in fragile environments with carbon sequestration potential.In karst areas,plantations based on fastgrowing afforestation species made significant contributions to enhancing carbon sequestration.However,the impact of understory vegetation on carbon accumulation remains unclear.Especially,the carbon accumulation associated with litter produced during the replacement of understory species receives insufficient attention,which leads to the neglect of the carbon sequestration potential in plantations of karst areas.Leaf is a crucial organ that links the litter production.To explore how leaf traits adapt to competitive environments and drive litter carbon accumulation during understory species replacement,this study observed leaf traits and litter carbon content changes in three types of plantations in the Liujiang River Basin,a typical karst area.A total of 37 sampling plots were selected for field investigation over a twoyear period.Leaf traits,species diversity,vegetation coverage,and litter carbon characteristics in understory vegetation were measured.Variance analysis,allometric equations,and path analysis were used for data analysis.The results showed that most understory species adopted a biomass conservation strategy under high-coverage conditions(>44.27%)and expanded competitive leaf area under low-coverage conditions(<44.27%).However,Bidens pilosa and Miscanthus floridulus exhibited strong competitiveness during understory species replacement.They showed an expansion of competitive leaf area under high-coverage conditions.This competitive strategy reduced species diversity and community specific leaf area.But the rapid expansion of Bidens pilosa and Miscanthus floridulus increased understory vegetation coverage,and their increased specific leaf area facilitated leaf shedding,resulting in significant litter weight accumulation(P<0.05),thereby enhancing litter carbon content per unit area.These competitive strategies were key driving factors for the increase in litter carbon content per square meter,which reached a maximum of 49.6% higher than that in natural grasslands.And the maximum increase in litter carbon accumulation derived from understory vegetation reached 3.37 times from 2023 to 2024 in plantations.In the understory vegetation of plantations,the competitive strategies reflected by leaf adaptation of key competitive species are critical factors influencing litter carbon accumulation.Future research could deeply explore the carbon sequestration effects resulting from the dynamic changes in competition within the understory vegetation of plantations.
基金financial support from the National Natural Science Foundation of China(No.52035012)the Guangdong Basic and Applied Basic Research Foundation(No.2025A1515012203)。
文摘The specific surface area(S S)and pore size(D)exhibit an inherent trade-off in the microscale design of bone implants:larger pores typically correlate with reduced surface area and vice versa.This relationship has attracted notable attention because of its critical role in the regulation of cell adhesion and osteogenesis.However,it remains largely unclear how S S and D affect the generated bone tissue and dynamically change during long-term osteogenesis.Herein,by applying rigorous geometric mapping to minimal surfaces,we constructed precisely partitioned and layer-by-layer thickened tissue models to simulate osteogenesis across different temporal scales and thereby track the dynamic evolution of geometric characteristics,permeability,and mechanobiological tissue differentiation.The high-S S samples were found to facilitate the rapid formation of new bone tissue in the early stages.However,their smaller pores tended to cause occlusions,hindering further tissue development.In contrast,low-S S samples showed slower bone regeneration,but their larger pores provided adequate physical space for tissue regeneration and mass transport,ultimately promoting bone formation in the long term.Mechanobiological regulation suggests that fibrous tissue formation inhibits additional bone formation,establishing a dynamic equilibrium between osteogenesis and pore space to sustain nutrient/waste exchange throughout the regenerative process.Overall,smaller pores are preferable in implants for minimally loaded osteoplasty procedures focused on early-stage bone consolidation,whereas larger pores are preferable in dynamically loaded implants requiring prolonged mechanical stability.
基金supported by the National Natural Science Foundation of China(62371465)Taishan Scholar Project of Shandong Province(ts201511020)。
文摘In wireless sensor networks,ensuring communication security via specific emitter identification(SEI)is crucial.However,existing SEI methods are limited to closed-set scenarios and lack the ability to detect unknown devices and perform classincremental training.This study proposes a class-incremental open-set SEI approach.The open-set SEI model calculates radiofrequency fingerprints(RFFs)prototypes for known signals and employs a self-attention mechanism to enhance their discriminability.Detection thresholds are set through Gaussian fitting for each class.For class-incremental learning,the algorithm freezes the parameters of the previously trained model to initialize the new model.It designs specific losses:the RFFs extraction distribution difference loss and the prototype transformation distribution difference loss,which force the new model to retain old knowledge while learning new knowledge.The training loss enables learning of new class RFFs.Experimental results demonstrate that the open-set SEI model achieves state-of-theart performance and strong noise robustness.Moreover,the class-incremental learning algorithm effectively enables the model to retain old device RFFs knowledge,acquire new device RFFs knowledge,and detect unknown devices simultaneously.
基金co-supported by the Fundamental Research Funds for Central Universities,China(No.3072024XX0206)the Natural Science Foundation of Heilongjiang Province,China(No.LH2024E069)。
文摘A surface pyrolysis and gas-phase combustion of the Ammonium Perchlorate(AP)/Hydroxy Terminated Polybutadiene(HTPB)composite propellant reaction kinetic mechanism with five-step chemical reaction is adopted.The effects of helium injection on the burning rate and combustion of AP/HTPB propellant are analyzed in details,and the characteristics of motor performance are obtained.The numerical simulation results demonstrate that helium injection enhances the combustion chamber pressure,thereby increasing the burning rate of propellant.However,the primary combustion reaction of the AP/HTPB propellant takes place within a thin layer on the burning surface,so the low-temperature helium has minimal impact on the gasphase combustion.Ultimately,the helium not only elevates the nozzle exit velocity,resulting in specific impulse gain,but also reduces the exhaust plume temperature.With an increase of helium mass flow rate,the area of the velocity increase zone at the nozzle exit continuously decreases,but the average velocity in the motor exit continuously increases.Overall,when the helium flow rate is 2.5 kg/s,the specific impulse can reach 10.5%.Reducing the helium injection hole diameter enhances mixing of helium and combustion gas and expands the velocity increase zone,thereby maximizing the exit velocity gain in average velocity at the nozzle exit.When the injection hole diameter is reduced from 100 mm to 20 mm,the specific impulse gain increases from 3.1%to 10.6%.Furthermore,increasing helium injection temperature greatly boosts the velocity of the mixed gas with the same helium mass fraction ultimately improving specific impulse.
基金the support of the research platform provided by Professor Zhi-Ying Wu’s research group at the Nanhu Brain-computer Interface Institutesupported by grants from the National Natural Science Foundation of China(32200822).
文摘Dear Editor,Social anxiety disorder(SAD)is a prevalent psychiatric disorder,characterized by persistent and excessive fear of social situations in which the individual may be scrutinized by others[1].Typically emerging in late childhood or adolescence with potential lifelong persistence,SAD significantly impairs interpersonal relationships,educational attainment,and occupational performance[2].Furthermore,SAD demonstrates high comorbidity rates with other mental disorders,including anxiety disorders,substanceuse disorder,and major depressive disorder[3].Current therapeutic interventions remain limited,with suboptimal response to existing psychological and pharmacological treatments in many patients,while the pathological mechanisms underlying SAD continue to elude comprehensive understanding[4].Establishing appropriate animal models is essential to investigating SAD's neural mechanisms and pathological underpinnings and developing effective therapeutic interventions.
基金supported by the National Natural Science Foundation of China(U22A20434)supported by the foundation from Qinghai Science and Technology Department(2023-ZJ-745).
文摘Hierarchical porous MgO is a promising adsorbent for dye removal because of its large Brunauer-Emmett-Teller specific surface area(SBET)and abundant low-coordinated oxygen anions(LCO)sites.As hierarchical porous MgO particles with large SBET values are typically prepared by complicated procedures under harsh conditions,such as high temperatures and high pressures,their large-scale production is impractical.Consequently,the preparation of hierarchical porous MgO with a large SBET value under mild conditions is highly desirable.In this study,a morphology transition engineering strategy is introduced to change the morphology of simple MgO microspheres to an embroidered ball-shaped with a larger SBET value via hydrolysis and calcination without using surfactants as sacrificial templates.During hydrolysis,numerous Mg(OH)_(2)sheets form and attach to the MgO surface,thus increasing the SBET value of the newly obtained MgO that forms by calcination(denoted as NM-x,where x is the hydrolysis time in hours).The sizes of the crystalline sheets were tuned by controlling the hydrolysis time.NM-12 exhibited the highest density of small-sized sheets on its surface and the largest SBET value of 180.17 m^(2)g^(-1),which was 3.51 times that of the MgO precursor(51.89 m^(2)g^(-1)).However,NM-24(134.07 m^(2)g^(-1))had a higher adsorption efficiency for Congo red(CR)than NM-12,despite having a smaller SBET value,which indicates that other factors are involved.NM-24 exhibited a lower probability of exposed(200)and(220)facets which were verified to repulse CR molecules by molecular dynamics simulations,and a greater number of LCO sites,which contributed to adsorption.Thus,this study introduces a facile method for preparing hierarchical porous MgO and examines the effects of LCO sites and exposed facet probabilities on its adsorption properties.
基金supported by Central Public-interest Scientific Institution Basal Research Fund(CATAS-Nos.1630152023007,1630152023011,1630152023012,1630152023013)the National Natural Science Foundation of China(Grant No.32071805).
文摘Coconut(Cocos nucifera L.),a major oil and fruit crop of the Arecaceae family,is extensively cultivated across the Asia—Pacific region.Despite its agricultural importance,genome assembly in coconut remains challenging due to its large genome size and high proportion of repetitive sequences.Allele-specific expression(ASE)plays a key role in regulating plant development and evolution,yet research on ASE in coconut is limited(Shao et al.,2019;Li et al.,2021;Zhang et al.,2021;Hu et al.,2022).Among phenotypic traits,fruit color is especially important as an indicator of maturity,guiding harvest timing and post-harvest processes(Kapoor et al.,2022).While prior studies have explored various coconut traits such as salt tolerance,fiber content,and plant height(Wang et al.,2021;Yang et al.,2021),investigations into ASE and fruit color remain scarce.
文摘Prostate-specific membrane antigen(PSMA)is a surface membrane antigen that is highly overexpressed in prostate cancer,with heterogenous expression throughout the natural history of the disease.This has generated significant interest as a potential biomarker for use in early diagnosis and treatment of prostate cancer.We reviewed the literature surrounding PSMA and its current clinical applications in diagnosing and managing early prostate cancer that is confined to the prostate and local lymph nodes.A search on PubMed,Medline,and Web of Science was performed using the following keywords:“PSMA”,“Prostate Specific Membrane Antigen”,“Prostate cancer”,“Biomarker”,“Diagnosis”.We considered all available articles relevant to the topic of PSMA as a biomarker in early prostate cancer when developing this narrative review.Key articles assessing the biology of PSMA,as well as its use as a potential diagnostic and therapeutic target in early prostate cancer,were assessed.The role of PSMA PET as a potential diagnostic and risk stratification tool was assessed.The current use of antibody-drug conjugates and radioligand therapy targeting PSMA was assessed,along with any current evidence to support their use in early prostate cancer.PSMA is heavily expressed throughout the early stages of prostate cancer,and this has significant therapeutic implications.There is a growing body of evidence that shows PSMA PET can play a role in the diagnosis,risk stratification,and prognostication of localised prostate cancer.PSMA-targeted therapies such as Lu-177 currently do not have any proven benefit in treating early prostate cancer;however,this remains an area of ongoing research.
文摘Alzheimer’s disease(AD)is the most common form of dementia.In addition to the lack of effective treatments,there are limitations in diagnostic capabilities.The complexity of AD itself,together with a variety of other diseases often observed in a patient’s history in addition to their AD diagnosis,make deciphering the molecular mechanisms that underlie AD,even more important.Large datasets of single-cell RNA sequencing,single-nucleus RNA-sequencing(snRNA-seq),and spatial transcriptomics(ST)have become essential in guiding and supporting new investigations into the cellular and regional susceptibility of AD.However,with unique technology,software,and larger databases emerging;a lack of integration of these data can contribute to ineffective use of valuable knowledge.Importantly,there was no specialized database that concentrates on ST in AD that offers comprehensive differential analyses under various conditions,such as sex-specific,region-specific,and comparisons between AD and control groups until the new Single-cell and Spatial RNA-seq databasE for Alzheimer’s Disease(ssREAD)database(Wang et al.,2024)was introduced to meet the scientific community’s growing demand for comprehensive,integrated,and accessible data analysis.
文摘Deep brain sti mulation(DBS)is a neuromodulation tool that involves the delivery of electrical impulses to specific brain regions through implanted electrodes.The principle behind DBS is to modulate dysfunctional neural circuits without the need for permanent structural alterations to the brain.Initially developed as a treatment for movement disorders such as Parkinson's disease(PD),DBS has expanded to encompass various neurological and psychiatric disorders.
基金supported by the National Natural Science Foundation of China(62201602)。
文摘Despite the superior advantages of specific emitter identification in extracting emitter features from in-phase and quadrature(I/Q)signals,challenges persist due to signal-type confusion and background noise interference.To address those limitations,this paper proposes a multi-channel contrast prediction coding and complex-valued residuals network(MCPC-MCVResNet)framework.This model employs contrast prediction techniques to directly extract discriminative features from electromagnetic signal sequences,effectively capturing both amplitude and phase information within I/Q data.A core innovation of this approach is the sphere space softmax(SS-softmax)loss,which optimizes intra-class clustering density of while establishing well-defined boundaries between distinct emitters.The SS-softmax mechanism significantly enhances the model's capacity to discern subtle variations among radiation emitters.Experimental results demonstrate superior identification accuracy,rapid convergence,and exceptional robustness in low signal-to-noise ratio environments.
文摘Supercapacitors are gaining popularity due to their high cycling stability,power density,and fast charge and discharge rates.Researchers are ex-ploring electrode materials,electrolytes,and separat-ors for cost-effective energy storage systems.Ad-vances in materials science have led to the develop-ment of hybrid nanomaterials,such as combining fil-amentous carbon forms with inorganic nanoparticles,to create new charge and energy transfer processes.Notable materials for electrochemical energy-stor-age applications include MXenes,2D transition met-al carbides,and nitrides,carbon black,carbon aerogels,activated carbon,carbon nanotubes,conducting polymers,carbon fibers,and nanofibers,and graphene,because of their thermal,electrical,and mechanical properties.Carbon materials mixed with conducting polymers,ceramics,metal oxides,transition metal oxides,metal hydroxides,transition metal sulfides,trans-ition metal dichalcogenide,metal sulfides,carbides,nitrides,and biomass materials have received widespread attention due to their remarkable performance,eco-friendliness,cost-effectiveness,and renewability.This article explores the development of carbon-based hybrid materials for future supercapacitors,including electric double-layer capacitors,pseudocapacitors,and hy-brid supercapacitors.It investigates the difficulties that influence structural design,manufacturing(electrospinning,hydro-thermal/solvothermal,template-assisted synthesis,electrodeposition,electrospray,3D printing)techniques and the latest car-bon-based hybrid materials research offer practical solutions for producing high-performance,next-generation supercapacitors.
基金financially supported by China Aeronautical Science Foundation (No.2023Z0530Q9002)the Program for Chongqing Talents,China (No.cstc2024ycjh-bgzxm0066)。
文摘The microstructural evolution,phase stability,and mechanical properties of Al-Li-Mg-Ti-M(M=Zn,Zr,V)lightweight high-entropy alloys(LW-HEAs)were investigated.The LW-HEAs with three components,Al_(20)Li_(20)Mg_(10)-Ti_(40)Zn_(10)(#Zn),Al_(20)Li_(20)Mg_(10)Ti_(30)Zr_(20)(#Zr),and Al_(20)Li_(20)Mg_(10)Ti_(30)V_(20)(#V),were designed according to the thermo-dynamic design criteria of HEA,and prepared via a combination process of mechanical alloying and cold-press sintering.The effects of alloy composition and sintering temperature on the microstructure and mechanical properties of the LW-HEAs were studied.The results show that the as-milled Al-Li-Mg-Ti-M(M=Zn,Zr,V)LW-HEAs form a simple structure with HCP-type solid solution as the primary phase,a dual-HCP type solid solution phase,and a BCC phase,respectively.After cold-press sintering,the#Zn and#V alloys undergo obvious phase transformation;while the#Zr alloy with dual-HCP phases exhibits the best phase stability during heat treatment.The#V-750°C alloy demonstrates the maximum hardness and specific strength of HV 595.2 and 625 MPa∙cm3/g,respectively,under the combined effect of solid solution strengthening of BCC phase and precipitation strengthening ofβ-AlTi_(3).Moreover,the#Zr-650°C,#Zr-750°C,and#Zn-650°C alloys are expected to have excellent plasticity.
基金The Open Project of State Key Laboratory of Smart Grid Protection and Operation Control in 2022(No.SGNR0000KJJS2302150).
文摘Fully implanted brain-computer interfaces(BCIs)are preferred as they eliminate signal degradation caused by interference and absorption in external tissues,a common issue in non-fully implanted systems.To optimize the design of electroencephalography electrodes in fully implanted BCI systems,this study investigates the penetration and absorption characteristics of microwave signals in human brain tissue at different frequencies.Electromagnetic simulations are used to analyze the power density distribution and specific absorption rate(SAR)of signals at various frequen-cies.The results indicate that lower-frequency signals offer advantages in terms of power density and attenuation coeffi-cients.However,SAR-normalized analysis,which considers both power density and electromagnetic radiation hazards,shows that higher-frequency signals perform better at superficial to intermediate depths.Specifically,at a depth of 2 mm beneath the cortex,the power density of a 6.5 GHz signal is 247.83%higher than that of a 0.4 GHz signal.At a depth of 5 mm,the power density of a 3.5 GHz signal exceeds that of a 0.4 GHz signal by 224.16%.The findings suggest that 6.5 GHz is optimal for electrodes at a depth of 2 mm,3.5 GHz for 5 mm,2.45 GHz for depths of 15-20 mm,and 1.8 GHz for 25 mm.
基金supported by Yunnan Major Scientific and Technological Projects(No.202202AG050005)Yunnan Fundamental Research Projects(No.202101BE070001-001).
文摘The ACF adsorbent with high Cu loading was treated with dielectric barrier discharge plasma to mitigate the negative effects of high Cu loading and enhance PH_(3)and H_(2)S adsorption and oxidation.Bruno-Emmett-Taylor(BET)result showed that the specific surface area of the adsorbent after air plasma modification was almost three times that before modification.X-ray photoelectron spectroscopy(XPS)findings revealed that the amino group was added to the adsorbent's surface,increasing lattice oxygen and chemisorbed oxygen.The adsorbent's large specific surface area,excellent surface active oxygen,and abundance of basic groups facilitate PH_(3)and H_(2)S adsorption and oxidation.The scanning electron microscopy showed that air plasma modification exposed more active components and uniformly dispersed them on the surface of adsorbent,thereby improving the adsorption performance.Activity evaluation results showed that the adsorbent has the best ability to capture PH_(3)and H_(2)S after being modified by air plasma at 4 kV voltage for 10 min.The adsorbent's breakthrough ability at high space velocity(WHSV:60,000 h^(−1))is 190 mg P/g and 146 mg S/g,respectively,which is 74%and 60%greater than that before modification.This is a great improvement over previous studies.In addition,the possible mechanism of adsorbent deactivation was proposed.
基金supported by the Battery Energy Storage Testing Center of Chongqing through their provision of testing support and technical assistance。
文摘Aqueous zinc-ion batteries(AZIBs)are gaining attention owing to their affordability,high safety,and high energy density,making them a promising solution for large-scale energy storage.However,their performance is hampered by the instability of both the anode-electrolyte interface and the cathode-electrolyte interface.The use of sodium gluconate(SG),an organic sodium salt with multiple hydroxyl groups,as an electrolyte additive is suggested.Experimental and theoretical analyses demonstrate that Na^(+)from SG can intercalate and deintercalate within the associated V_(2)O_(5) cathode during in situ electrochemical processes.This action supports the layered structure of V_(2)O_(5),prevents structural collapse and phase transitions,and enhances Zn^(2+)diffusion kinetics.Additionally,the gluconate anion disrupts the original Zn^(2+)solvation structure,mitigates water-induced side reactions,and suppresses Zn dendrite growth.The synchronous regulation of both the V_(2)O_(5) cathode and Zn anode by the SG additive leads to considerable performance improvements.Zn‖Zn symmetric batteries demonstrate a cycle life exceeding 2800 h at 0.5 mA cm^(-2)and 1 mAh cm^(-2).In Zn‖V_(2)O_(5) full batteries,a high specific capacity of 288.92 mAh g^(-1)and capacity retention of 82.29%are maintained over 1000 cycles at a current density of 2 A g^(-1).This multifunctional additive strategy offers a new pathway for the practical application of AZIBs.
基金funded by the National Natural Science Foundation of China(U22A20547)the Major Science and Technology Projects of Heilongjiang Province(2021ZX12B05 and 2020ZX07B02)。
文摘The present study monitored bacterial succession,physicochemical properties,and volatile organic compounds(VOCs)changes in smoked chicken legs with modified atmosphere packaging(MAP,60% CO_(2) and 40%N_(2))during a 25-day storage period at 4℃.After 15 days of storage,S erratia proteamaculans and Pseudomonas fragi became the predominant bacteria.Furthermore,physicochemical properties changed significantly,as evidenced by an increase in thiobarbituric acid reactive substances and b*(yellowness)value,and a decrease in hardness.A total of 65 VOCs were identified during storage.Correlation between bacterial succession and quality indicators(including VOCs and physicochemical properties)allowed the identification of 26 core dominant bacteria,including S.proteamaculans,Psychrobacter alimentarius,Pseudomonas putida,and Pseudomonas poae,which were positively related to spoilage VOCs(e.g.,1-octen-3-ol,1-pentanol,and 3-methyl-1-butanol)and could be defined as specific spoilage organisms(SSOs).The results of this study provide a systematic approach to predict SSOs in smoked chicken legs during storage,which can also provide a basis for product safety.
