Although disinfection byproducts(DBPs) in drinking water have been suggested as a cancer causing factor, the causative compounds have not yet been clarified. In this study, we used liquid chromatography quadrupole-tim...Although disinfection byproducts(DBPs) in drinking water have been suggested as a cancer causing factor, the causative compounds have not yet been clarified. In this study, we used liquid chromatography quadrupole-time-of-flight spectrometry(LC-QTOF MS) to identify the unknown disinfection byproducts(DBPs) in drinking water produced from Taihu Lake source water, which is known as a convergence point for the anthropogenic pollutants discharged from intensive industrial activities in the surrounding regions. In total, 91 formulas of DBPs were discovered through LC-QTOF MS nontarget screen, 81 of which have not yet been reported. Among the 91 molecules, 56 only contain bromine, 15 only contain chlorine and 20 DBPs have both bromine and chlorine atoms. Finally, five DBPs including 2,4,6-tribromophenol, 2,6-dibromo-4-chlorophenol, 2,6-dichloro-4-bromophenol, 4-bromo-2,6-di-tert-butylphenol and 3,6-dibromocarbazole were confirmed using standards. The former three compounds mainly formed in the predisinfection step(maximum concentration, 0.2-2.6 μg/L), while the latter two formed in the disinfection step(maximum concentration, 18.2-33.6 ng/L). In addition, 19 possible precursors of the discovered DBPs were detected, with the aromatic compounds being a major group. 2,6-di-tert-butylphenol as the precursor of 4-bromo-2,6-di-tert-butylphenol was confirmed with standard, with a concentration of 20.3 μg/L in raw water. The results of this study show that brominated DBPs which are possibly formed from industrial pollutants are relevant DBP species in drinking water produced form Taihu source water, suggesting protection of Taihu Lake source water is important to control the DBP risks.展开更多
Detection of estrogenic disrupting compounds（EDCs） in drinking waters around China has led to rising concerns about health risks associated with these compounds.There is,however,a paucity of studies on the occurrenc...Detection of estrogenic disrupting compounds（EDCs） in drinking waters around China has led to rising concerns about health risks associated with these compounds.There is,however,a paucity of studies on the occurrence and identification of the main compounds responsible for this pollution in the source waters.To fill this void,we screened estrogenic activities of 23 source water samples from six main river systems in China,using a recombinant two-hybrid yeast assay.All sample extracts induced significant estrogenic activity,with E2 equivalents（EEQ） of raw water ranging from 0.08 to 2.40 ng/L.Additionally,16 samples were selected for chemical analysis by gas chromatography-mass spectrometry.The EDCs of most concern,including estrone（E1）,17β-estradiol（E2）,17α-ethinylestradiol（EE2）,estriol（E3）,diethylstilbestrol（DES）,estradiol valerate（EV）,4-t-octylphenol（4-t-OP）,4-nonylphenols（4-NP） and bisphenol A（BPA）,were determined at concentrations of up to 2.98,1.07,2.67,4.37,2.52,1.96,89.52,280.19 and 710.65 ng/L,respectively.Causality analysis,involving comparison of EEQ values from yeast assay and chemical analysis identified E2,EE2 and 4-NP as the main responsible compounds,accounting for the whole estrogenic activities（39.74% to 96.68%）.The proposed approach using both chemical analysis and yeast assay could be used for the identification and evaluation of EDCs in source waters of China.展开更多
Odor problems in source water caused by 2-methylisoborneol(MIB) have been a common issue in China recently, posing a high risk to drinking water safety. The earthy-musty odorant MIB has an extremely low odor threshol...Odor problems in source water caused by 2-methylisoborneol(MIB) have been a common issue in China recently, posing a high risk to drinking water safety. The earthy-musty odorant MIB has an extremely low odor threshold(4–16 ng/L) and is hard to remove via conventional processes in drinking water plants(DWP), and therefore could easily provoke complaints from consumers. This compound is produced by a group of filamentous cyanobacteria, mainly belonging to Oscillatoriales. Different from the well-studied surface-blooming Microcystis, filamentous cyanobacteria have specific niche characteristics that allow them to stay at a subsurface or deep layer in the water column. The underwater bloom of these MIB producers is therefore passively determined by the underwater light availability, which is governed by the cell density of surface scum. This suggests that drinking water reservoirs with relatively low nutrient contents are not able to support surface blooms, but are a fairly good fit to the specialized ecological niche of filamentous cyanobacteria;this could explain the widespread odor problems in source water. At present, MIB is mainly treated in DWP using advanced treatment processes and/or activated carbon, but these post-treatment methods have high cost, and not able to deal with water containing high MIB concentrations.Thus, in situ control of MIB producers in source water is an effective complement and is desirable. Lowering the underwater light availability is a possible measure to control MIB producers according to their niche characteristics, which can be obtained by either changing the water level or other measures.展开更多
Municipal wastewater reclamation is becoming of increasing importance in the world to solve the problem of water scarcity. A better understanding of the molecular composition of effluent organic matter（Ef OM） in the...Municipal wastewater reclamation is becoming of increasing importance in the world to solve the problem of water scarcity. A better understanding of the molecular composition of effluent organic matter（Ef OM） in the treated effluents of municipal wastewater treatment plants（WWTPs） is crucial for ensuring the safety of water reuse. In this study, the molecular composition of Ef OM in the secondary effluent of a WWTP in Beijing and the reclaimed water further treated with a coagulation–sedimentation–ozonation process were characterized using a non-target Fourier transform ion cyclotron resonance mass spectrometry（FT-ICR MS） method and compared to that of natural organic matter（NOM） in the local source water from a reservoir. It was found that the molecular composition of Ef OM in the secondary effluent and reclaimed water was dominated by CHOS formulas, while NOM in the source water was dominated by CHO formulas. The CHO formulas of the three samples had similar origins. Anthropogenic surfactants were responsible for the CHOS formulas in Ef OM of the secondary effluent and were not well removed by the coagulation-sedimentation-ozonation treatment process adopted.展开更多
Objective To identify and determine the congener and level of microcystins in the source water of Taihu Lake. Methods Improved method of SPE combined with HPLC was employed to detect the concentration and varieties of...Objective To identify and determine the congener and level of microcystins in the source water of Taihu Lake. Methods Improved method of SPE combined with HPLC was employed to detect the concentration and varieties of microcystins in source water and bloom samples collected from Meiliang Bay, Taihu Lake. Results The contents of two predominant microcystin components, MC-RR, and MC-LR, were relatively high in samples during warm months and correlated with the phase of algae growth. The maximum concentrations of MC-RR and MC-LR in water sample reached 3.09±0.53μg/L and 2.39±0.41μg/L during the period of water bloom in September 2004, respectively. Even without waterbloom, the concentration of MC-LR in source water sample was still higher than the guideline value. Conclusion The status of microcystin pollution in this region is serious and measures to monitor and control the growth of cyanobacteria are urgently needed.展开更多
Significant iron release from cast iron pipes in water distribution systems(WDSs),which usually occurs during the source water switch period,is a great concern of water utilities because of the potential occurrence of...Significant iron release from cast iron pipes in water distribution systems(WDSs),which usually occurs during the source water switch period,is a great concern of water utilities because of the potential occurrence of"red water"and customer complaints.This study developed a new method which combined in-situ water stagnation experiments with mathematical models and numerical simulations to predict the iron release caused by source water switch.In-situ water stagnation experiments were conducted to determine the total iron accumulation in nine cast iron pipes in-service in Beijing when switching the local water to tre ated Danjiangkou Reservior water.Results showe d that the difference in the concentration increment of total iron in 24 hr(ΔCITI,24),i.e.short-term iron release,caused by source water switch was mainly dependent on the difference in the key quality parameters(pH,hardness,nitrate,Larson Ratio and dissolved oxygen(DO))between the two source waters.The iron release rate(RFe)after switch,i.e.long-term iron release,was closely related to the pipe properties as well as the DO and total residual chlorine(TRC)concentrations.Mathematical models ofΔCITI,24 and RFe were developed to quantitatively reveal the relationship between iron release and the key quality parameters.The RFe model could successfully combine with EPANET-MSX,a numerical simulator of water quality for WDSs to extend the iron release modeling from pipe level to network level.The new method is applicable to predicting iron release during source water switch,thus facilitating water utilities to take preventive actions to avoid"red water".展开更多
Mobile emergency pilot water plant was used to carry out pilot study of KMnO4 pre-oxidation enhanced coagulation treating high-algae source water. Research showed that the optimal dosages of coagulant and KMnO4 in the...Mobile emergency pilot water plant was used to carry out pilot study of KMnO4 pre-oxidation enhanced coagulation treating high-algae source water. Research showed that the optimal dosages of coagulant and KMnO4 in the process were 6 and 0. 4- 0. 6 mg / L respectively. Under the dosage,removal rate of water turbidity after precipitation rose by 11% than simple coagulation,and removal rate of algae rose by 15%. Removal rates of total amount of odor and GSM by the process were respectively 73% and 59%. The removal rate of total amount of algae by KMnO4 preoxidation was 40%,and removal effect of THM precursors was obvious.展开更多
The pollution problem arising from the flushing of initial rainwater and wastewater from accidents while transporting dangerous goods to source water protection areas needs to be solved as soon as possible.Therefore,t...The pollution problem arising from the flushing of initial rainwater and wastewater from accidents while transporting dangerous goods to source water protection areas needs to be solved as soon as possible.Therefore,the design of corresponding environmental protection measures should be considered in the engineering design stage.It is necessary to analyze the specific work in combination with engineering examples.Under this background,this paper first briefly expounds the precautions in accident risk analysis and the design of tank capacity and tank body.Finally,by analyzing actual cases,this paper systematically studies the design strategy of emergency pool in source water protection area,hoping to provide new development ideas for the upgrading of relevant work.展开更多
[Objective] The study aimed to discuss the application of a stereo constructed wetland to the treatment of slightly polluted source water. [Method] In this study, a new stereo constructed wetland mode was put forward,...[Objective] The study aimed to discuss the application of a stereo constructed wetland to the treatment of slightly polluted source water. [Method] In this study, a new stereo constructed wetland mode was put forward, and a pilot project of water ecological purification in Xinsheng River, the diversion channel of Shijiuyang Waterwork in Jiaxing City, were analyzed. Afterwards, the impact factors of water purification by the technology were discussed from water quality and quantity, season and climate, species configuration, management and maintenance. [Result] Under three different hydraulic loading conditions, the pilot project effectively improved water SD and DO level, and reduced SS, CODCr, NH3-N, TN and TP significantly in summer and autumn, so that effluent water quality reached surface water standard at Grade III. [Conclusion] The stereo constructed wetland mode composed of constructed wetland and underwater forest used to treat slightly polluted source water is feasible and has a good promotion prospect.展开更多
Precipitation isotopes(δ^(18)O and δ^(2)H)are closely related to meteorological conditions for precipitation generation and the initial state of water vapor source areas,and are essential to the study of the regiona...Precipitation isotopes(δ^(18)O and δ^(2)H)are closely related to meteorological conditions for precipitation generation and the initial state of water vapor source areas,and are essential to the study of the regional hydrological cycle.The deuterium excess(d-excess)indicates deviation in isotope fractionation during evaporation and can trace water vapor sources.This study analyzed 443 precipitation samples collected from the Gannan Plateau,China in 2022 to assess precipitation isotope variations and their driving factors.Water vapor sources were evaluated using the Hybrid Single-Particle Lagrangian Integrated Trajectory(HYSPLIT),Concentration Weighted Trajectory(CWT),and Potential Source Contribution Factor(PSCF)models.Results showed that precipitation isotope values showed significant spatial and temporal variations on the Gannan Plateau.Temporally,precipitation isotope values peaked in June(when evaporation dominated)and minimized in March(depletion effect of air masses in the westerly wind belt).Spatially,the isotope values showed a distribution pattern of"high in the east and low in the west",which was mainly regulated by the differences in altitude and local meteorological conditions.Compared with the global meteoric water line(GMWL)with equation of δ^(2)H=8.00δ^(18)O+10.00,the slope and intercept of local meteoric water line(LMWL)for precipitation on the Gannan Plateau were smaller(7.49 and 7.63,respectively),reflecting the existence of a stronger secondary evaporation effect under the clouds in the region.The sources of water vapor on the Gannan Plateau showed significant seasonality and spatial heterogeneity.Specifically,the westerly belt and monsoon were the main water vapor transport paths at each sampling point,with Central Asian continental water vapor dominating in spring(53.49%),Indian Ocean water vapor dominating in summer(52.53%),Atlantic Ocean water vapor dominating in autumn(46.74%),and Atlantic Ocean and Mediterranean Sea water vapor dominating in winter(42.30%and 33.68%,respectively).Changes in the intensity of convective activity and Outgoing Longwave Radiation(OLR)affected the enrichment of isotopic values,which exhibited the same change trends as δ^(18)O.During the precipitation process,the δ^(18)O value first decreased and then increased.During the initial and final stages of precipitation process,precipitation was mainly influenced by continental air masses,while during the middle stage,it was controlled by marine air masses.The systematic research on precipitation isotopes and water vapor sources is important for climate change research and extreme precipitation prediction on the Gannan Plateau and other similar areas.展开更多
Groundwater overextraction and contamination by heavy metals such as cadmium and arsenic have resultedin ecological degradation and increased risks of renal disease,particularly in water-scarce regions.To address thes...Groundwater overextraction and contamination by heavy metals such as cadmium and arsenic have resultedin ecological degradation and increased risks of renal disease,particularly in water-scarce regions.To address thesechallenges,this review aimed to evaluate the ecological potential of dew water harvesting as a sustainable and safealternative water source.Literature published between 2000 and 2024 was systematically searched in PubMed,Scopus,Web of Science,and Google Scholar using the terms“dew water,”“atmospheric water harvesting,”“groundwaterpollution,”“heavy metals,”“ecosystem restoration,”and“sustainable water systems.”Studies were included if theyfocused on dew water quality,ecological functions,or health-related outcomes,while non-English publications,conference abstracts without full text,and studies not directly addressing dew water were excluded.A total of 46 studiesand 7 official guidelines met the eligibility criteria.Findings indicate that natural dew water generally exhibits a neutralpH(6.5–8.5),negligible concentrations of heavy metals,and relatively high dissolved oxygen content(~9 mg/L).Casestudies from Morocco,Israel,China,and India illustrate its contributions to soil moisture retention,plant survival,biodiversity support,and microclimate regulation.Moreover,dew water produced through the Systemized Dew Process(SDP)consistently complied with WHO(2024)standards for drinking water,showing contaminant levels belowdetection thresholds.In conclusion,dew water harvesting represents a low-impact,climate-resilient,and safe alternativethat mitigates exposure to nephrotoxic pollutants,reduces reliance on overexploited groundwater,and enhances longtermecological restoration and water security in degraded and water-scarce environments.展开更多
Pharmaceuticals and personal care products(PPCPs)are receiving attention as emerging pollutants due to their extensive applications and persistent emissions.The Qiantang River Basin,a representative region in eastern ...Pharmaceuticals and personal care products(PPCPs)are receiving attention as emerging pollutants due to their extensive applications and persistent emissions.The Qiantang River Basin,a representative region in eastern China that relies on surface water for drinking purposes,experiences the movement and accumulation of PPCPs in its water and sediment,which can directly affect the safety of drinking water in the basin.This study focuses on the Qiantang River Basin’s surface water,sediment,and drinking water to determine the occurrence and potential risks of 31 PPCPs.It aims to address whether PPCPs in the environment could migrate and accumulate,thereby affecting human health.The findings indicated that PPCPs are ubiquitous in various environmental media,with surface and pore water showing distinct spatial distribution characteristics,specifically,concentrations escalated with urban scale expansion,indicating that domestic sewage discharge is the primary source of PPCP input.Bisphenol A(BPA),ketoprofen(KTP),and diethyltoluamide(DEET)were the primary contaminants.The movement of PPCPs within the surface water-sediment-pore water system was affected by various circumstances.Substances like Sulfamethoxazole(SMX)(RQ>103)and KTP(RQ=22.3)present in surface water and sediment pose significant ecological concerns,and KTP and atrazine(ATZ)(0.6<RQ<2.1)also pose a high risk in drinking water.This study performed an extensive analysis of the distribution and risks associated with typical PPCPs in the Qiantang River Basin,offering a scientific foundation and theoretical support for research on the environmental behavior of PPCPs in this area and the development of targeted pollution control strategies.展开更多
The Danjiangkou reservoir was selected to provide the source water for the middle routes of the South to North Water Transfer Project, which has provoked many environmental concerns. To date, investigations of water c...The Danjiangkou reservoir was selected to provide the source water for the middle routes of the South to North Water Transfer Project, which has provoked many environmental concerns. To date, investigations of water contamination of the source water of the Danjiangkou reservoir with organic micro-pollutants have been limited. This study was conducted to identify and rank organic contaminants that pose risks in the Danjiangkou reservoir. To this end, the Chemical Hazard Evaluation and Manage- ment Strategies （CHEMS-1） approach was adapted to integrate the deconvolution technology of qualitative identifying contaminants for site-specific environmental matrices. The samples were screened for the presence of 1093 contaminants using deconvolution technologies and the hazard values of the identified contaminants were calculated using the adapted CHEMS-1 approach accord- ing to their hazardous properties and occurrence in source water. The results showed that 46 contaminants from 1093 targets were present in Danjiangkou water, 23 of which appeared at frequencies higher than 50%, and 15 of which were identified as priorities. Over half （53%） of the high- ranked contaminants were polycyclic aromatic hydrocar- bons （PAHs）, with chrysene ranked highest on the list. Health risk assessment of the top-ranked PAHs was conducted and revealed that cancer risks of PAHs detected in the source water of Danjiangkou to different populations ranged from 10-7 to 104, indicating a low cancer risk to consumers. The results of this study indicated that the adapted CHEMS-1 approach was feasible for site-specific screening of organic contaminants to identify and rank potential priority pollutants.展开更多
Since the ammonia in the effluent of the tradi-tional water purification process could not meet the supply demand,the advanced treatment of a high concentration of NH4+-N micro-polluted source water by biological acti...Since the ammonia in the effluent of the tradi-tional water purification process could not meet the supply demand,the advanced treatment of a high concentration of NH4+-N micro-polluted source water by biological activated carbon filter(BACF)was tested.The filter was operated in the downflow manner and the results showed that the remov-ing rate of NH_(4)^(+)-N was related to the influent concentration of NH_(4)^(+)-N.Its removing rate could be higher than 95%when influent concentration was under 1.0 mg/L.It could also decrease with the increasing influent concentration when the NH_(4)^(+)-N concentration was in the range from 1.5 to 4.9 mg/L and the dissolved oxygen(DO)in the influent was under 10 mg/L,and the minimum removing rate could be 30%.The key factor of restricting nitrification in BACF was the influent DO.When the influent NH_(4)^(+)-N concentration was high,the DO in water was almost depleted entirely by the nitrifying and hetetrophic bacteria in the depth of 0.4 m filter and the filter layer was divided into aerobic and anoxic zones.The nitrification and degradation of organic matters existed in the aerobic zone,while the denitrification occurred in the anoxic zone.Due to the limited carbon source,the denitrifica-tion could not be carried out properly,which led to the accu-mulation of the denitrification intermediates such as NO_(2)^(−).In addition to the denitrification bacteria,the nitrification and the heterotrophic bacteria existed in the anoxic zone.展开更多
This study investigates the suitability of statistical techniques for evaluating the fluoride content and the groundwater quality from Robles Department(RD)and Banda Department(BD)in Santiago del Estero(Argentina).For...This study investigates the suitability of statistical techniques for evaluating the fluoride content and the groundwater quality from Robles Department(RD)and Banda Department(BD)in Santiago del Estero(Argentina).For the original statistical study,evaluation of nine parameters(fluoride,pH,conductivity,atmospheric and water temperature,total dissolved solids,chloride,hardness,and alkalinity)of 110 collected underground water samples from 23 dispersed rural areas was proposed.Groundwater samples were obtained by sampling taken from wells at different depths.Fluoride levels were determined by a standard colorimetric method in two seasonal periods,the dry(from April to September)and rainy(from October to March)period.The analytical results obtained for physicochemical parameters such as pH,total dissolved solids(TDS),and temperature does not reveal any notable difference between the rainy and dry seasons studied.In both seasons,the atmospheric temperature average was 22℃.With respect to fluoride content,approximately 50%of the analysed groundwater samples exceeded the limit established by current legislation(1.0 mg/L),obtaining concentration levels in the range of 0.01-2.80 mg/L.This study demonstrates the usefulness of the univariate statistical method(quartiles calculation,interquartile range IQR),multivariate principal component analysis(PCA),and cluster analysis to establish a better understanding of the state of the contamination of the waters in the region studied.展开更多
Heavy metal pollution in agricultural water resources is very serious in re- cent years, resulting in large losses of the agricultural economy and endangering human life and health. Due to the advantages of low cost, ...Heavy metal pollution in agricultural water resources is very serious in re- cent years, resulting in large losses of the agricultural economy and endangering human life and health. Due to the advantages of low cost, high efficiency and less secondary pollution, microbial ramediation technology is widely used in the treatment of heavy metal pollution in agricultural water resources. At present, with the progress of modern biotechnology, microbial remediation of heavy metals in agricul- tural water resources has grown rapidly. The sources and status quo of heavy met- al pollution in agricultural water resources at home and aboard, and the principles of microbial remediation of heavy metals pollution in agricultural water resources were reviewed in this paper, as well as the several common microbial remediation technology of heavy metals in agricultural water resources. Additionally, the further research work of heavy metal contaminated agricultural water resources by microbial ramediation were prospected.展开更多
The characteristics of ammonia in drinking water sources in China were evaluated during 2005-2009. The spatial distribution and seasonal changes of ammonia in different types of drinking water sources of 22 provinces,...The characteristics of ammonia in drinking water sources in China were evaluated during 2005-2009. The spatial distribution and seasonal changes of ammonia in different types of drinking water sources of 22 provinces, 5 autonomous regions and 4 municipalities were investigated. The levels of ammonia in drinking water sources follow the order of fiver 〉 lake/reservoir 〉 groundwater. The levels of ammonia concentration in river sources gradually decreased from 2005 to 2008, while no obvious change was observed in the lakes/reservoirs and groundwater drinking water sources. The proportion of the type of drinking water sources is different in different regions. In river drinking water sources, the ammonia level was varied in different regions and changed seasonally. The highest value and wide range of annual ammonia was found in South East region, while the lowest value was found in Southwest region. In lake/reservoir drinking water sources, the ammonia levels were not varied obviously in different regions. In underground drinking water sources, the ammonia levels were varied obviously in different regions due to the geological permeability and the natural features of regions. In the drinking water sources with higher ammonia levels, there are enterprises and wastewater drainages in the protected areas of the drinking water sources.展开更多
The nitrogen （N） pollution status of the 12 most important rivers in Changshu, Taihu Lake region was investigated. Water samples were collected from depths of 0.5-1.0 m with the aid of the global positioning system ...The nitrogen （N） pollution status of the 12 most important rivers in Changshu, Taihu Lake region was investigated. Water samples were collected from depths of 0.5-1.0 m with the aid of the global positioning system （GPS）. The seasonal variations in the concentrations of different N components in the rivers were measured. Using tension-free monolith lysimeters and ^15N-labeled fertilizer, field experiments were carried out in this region to determine variations of iSN abundance of NO3^- in the leachate during the rice and wheat growing seasons, respectively. Results showed that the main source of N pollution of surface waters in the Taihu Lake region was not the N fertilizer applied in the farmland but the urban domestic sewage and rural human and animal excreta directly discharged into the water bodies without treatment. Atmospheric dry and wet N deposition was another evident source of N pollutant of the surface waters. In conclusion, it would not be correct to attribute the N applied to farmlands as the source of N pollution of the surface waters in this region.展开更多
[Objective] To study the characteristics and effects of inorganic nitrogen in east water-source and inflow rivers of Chaohu Lake. [Method] The speciation and distribution characteristics of dissolvable inorganic nitro...[Objective] To study the characteristics and effects of inorganic nitrogen in east water-source and inflow rivers of Chaohu Lake. [Method] The speciation and distribution characteristics of dissolvable inorganic nitrogen （DIN） in east water-source and inflow rivers of Chaohu Lake were investigated, and their effects on water qual- ity were examined. [Result] The concentrations of NH3-N and NO2--N were the high in flood season, and low in non-flood season, while the concentration of NO3--N pre- sented the opposite trend; the concentration of NO3--N was the highest in Shuangqiao estuary, where the pollution was the worst. DIN in Zhegao estuary and Xiaozhegao estuary was mainly caused by domestic sewage and industrial wastewaters; surface runoff and pollution from ships contribute the most to the DIN content in Shuangqiao estuary. [Conclusion] This study provided basic data and theoretical basis for the control and management of eutrophication in Chaohu Lake.展开更多
An embedded reservoir that provides an efficient nutrient removal system protects drinking water.However,embedded reservoirs are rarely used in eutrophic shallow lakes because of their undetermined nutrient retention ...An embedded reservoir that provides an efficient nutrient removal system protects drinking water.However,embedded reservoirs are rarely used in eutrophic shallow lakes because of their undetermined nutrient retention efficiency and unknown effects by the phytoplankton community.In this study,we aim to investigate the nutrient retention and algae succession in an embedded reservoir and adjacent wetland from April 2017 to September 2018 in the eastern part of Lake Taihu,China.More than 40%of total phosphorus(TP)and 45%of particulate phosphorous entering the reservoir were retained semiannually,and the highest TP removal efficiency was achieved in the reservoir during autumn with an average value of 53.3%±9.9%.The overall nitrogen retention efficiency(21.7%±37.8%)was lower than that of TP(41.8%±27.8%).Similar trends were obtained in the wetland area.An important pathway for phosphorus removal is through particulate matter retention.Our study revealed that nutrient retention mechanisms in the reservoir were primarily via macrophyte absorption,particulate substance sedimentation,and prolonged water residence time.Consequently,the phytoplankton biomass(Chl-a)in the reservoir decreased(from 48.0 to 25.2μg/L)and water transparency improved,due to the decreased P level and transformation of the phytoplankton group into simple structures with good ecological status.Therefore,the combination of embedded reservoir and constructed wetland ecosystem can be used successfully to protect surface water.The results will be advantageous to groups seeking to preserve drinking water sources.展开更多
基金This work was supported by Major Science and Technology Program for Water Pollution Control and Treatment(No.2017ZX07502003)the National Key R&D Program of China(No.2018YFE0204101).
文摘Although disinfection byproducts(DBPs) in drinking water have been suggested as a cancer causing factor, the causative compounds have not yet been clarified. In this study, we used liquid chromatography quadrupole-time-of-flight spectrometry(LC-QTOF MS) to identify the unknown disinfection byproducts(DBPs) in drinking water produced from Taihu Lake source water, which is known as a convergence point for the anthropogenic pollutants discharged from intensive industrial activities in the surrounding regions. In total, 91 formulas of DBPs were discovered through LC-QTOF MS nontarget screen, 81 of which have not yet been reported. Among the 91 molecules, 56 only contain bromine, 15 only contain chlorine and 20 DBPs have both bromine and chlorine atoms. Finally, five DBPs including 2,4,6-tribromophenol, 2,6-dibromo-4-chlorophenol, 2,6-dichloro-4-bromophenol, 4-bromo-2,6-di-tert-butylphenol and 3,6-dibromocarbazole were confirmed using standards. The former three compounds mainly formed in the predisinfection step(maximum concentration, 0.2-2.6 μg/L), while the latter two formed in the disinfection step(maximum concentration, 18.2-33.6 ng/L). In addition, 19 possible precursors of the discovered DBPs were detected, with the aromatic compounds being a major group. 2,6-di-tert-butylphenol as the precursor of 4-bromo-2,6-di-tert-butylphenol was confirmed with standard, with a concentration of 20.3 μg/L in raw water. The results of this study show that brominated DBPs which are possibly formed from industrial pollutants are relevant DBP species in drinking water produced form Taihu source water, suggesting protection of Taihu Lake source water is important to control the DBP risks.
基金supported by the Chinese Academy of Sciences (No. KZCX1-YW-06-02)the National Basic Research Program of China (No. 2007CB407304)the Ministry of Environmental Protection of the People’sRepublic of China (No. 200909040)
文摘Detection of estrogenic disrupting compounds（EDCs） in drinking waters around China has led to rising concerns about health risks associated with these compounds.There is,however,a paucity of studies on the occurrence and identification of the main compounds responsible for this pollution in the source waters.To fill this void,we screened estrogenic activities of 23 source water samples from six main river systems in China,using a recombinant two-hybrid yeast assay.All sample extracts induced significant estrogenic activity,with E2 equivalents（EEQ） of raw water ranging from 0.08 to 2.40 ng/L.Additionally,16 samples were selected for chemical analysis by gas chromatography-mass spectrometry.The EDCs of most concern,including estrone（E1）,17β-estradiol（E2）,17α-ethinylestradiol（EE2）,estriol（E3）,diethylstilbestrol（DES）,estradiol valerate（EV）,4-t-octylphenol（4-t-OP）,4-nonylphenols（4-NP） and bisphenol A（BPA）,were determined at concentrations of up to 2.98,1.07,2.67,4.37,2.52,1.96,89.52,280.19 and 710.65 ng/L,respectively.Causality analysis,involving comparison of EEQ values from yeast assay and chemical analysis identified E2,EE2 and 4-NP as the main responsible compounds,accounting for the whole estrogenic activities（39.74% to 96.68%）.The proposed approach using both chemical analysis and yeast assay could be used for the identification and evaluation of EDCs in source waters of China.
基金supported by the National Natural Science Foundation of China(Nos.51878649,52030002)the National Key R&D Program of China(No.2018YFE0204100)+1 种基金the Youth Innovation Promotion Association CAS。
文摘Odor problems in source water caused by 2-methylisoborneol(MIB) have been a common issue in China recently, posing a high risk to drinking water safety. The earthy-musty odorant MIB has an extremely low odor threshold(4–16 ng/L) and is hard to remove via conventional processes in drinking water plants(DWP), and therefore could easily provoke complaints from consumers. This compound is produced by a group of filamentous cyanobacteria, mainly belonging to Oscillatoriales. Different from the well-studied surface-blooming Microcystis, filamentous cyanobacteria have specific niche characteristics that allow them to stay at a subsurface or deep layer in the water column. The underwater bloom of these MIB producers is therefore passively determined by the underwater light availability, which is governed by the cell density of surface scum. This suggests that drinking water reservoirs with relatively low nutrient contents are not able to support surface blooms, but are a fairly good fit to the specialized ecological niche of filamentous cyanobacteria;this could explain the widespread odor problems in source water. At present, MIB is mainly treated in DWP using advanced treatment processes and/or activated carbon, but these post-treatment methods have high cost, and not able to deal with water containing high MIB concentrations.Thus, in situ control of MIB producers in source water is an effective complement and is desirable. Lowering the underwater light availability is a possible measure to control MIB producers according to their niche characteristics, which can be obtained by either changing the water level or other measures.
基金supported by the National Natural Science Foundation of China(Nos.21377150 and 51578530)
文摘Municipal wastewater reclamation is becoming of increasing importance in the world to solve the problem of water scarcity. A better understanding of the molecular composition of effluent organic matter（Ef OM） in the treated effluents of municipal wastewater treatment plants（WWTPs） is crucial for ensuring the safety of water reuse. In this study, the molecular composition of Ef OM in the secondary effluent of a WWTP in Beijing and the reclaimed water further treated with a coagulation–sedimentation–ozonation process were characterized using a non-target Fourier transform ion cyclotron resonance mass spectrometry（FT-ICR MS） method and compared to that of natural organic matter（NOM） in the local source water from a reservoir. It was found that the molecular composition of Ef OM in the secondary effluent and reclaimed water was dominated by CHOS formulas, while NOM in the source water was dominated by CHO formulas. The CHO formulas of the three samples had similar origins. Anthropogenic surfactants were responsible for the CHOS formulas in Ef OM of the secondary effluent and were not well removed by the coagulation-sedimentation-ozonation treatment process adopted.
基金This work was supported by Hi-Tech Research and Development Program (863 program) of China (No. 2002AA302304) and National Natural Science Foundation of China (No. 60121101).
文摘Objective To identify and determine the congener and level of microcystins in the source water of Taihu Lake. Methods Improved method of SPE combined with HPLC was employed to detect the concentration and varieties of microcystins in source water and bloom samples collected from Meiliang Bay, Taihu Lake. Results The contents of two predominant microcystin components, MC-RR, and MC-LR, were relatively high in samples during warm months and correlated with the phase of algae growth. The maximum concentrations of MC-RR and MC-LR in water sample reached 3.09±0.53μg/L and 2.39±0.41μg/L during the period of water bloom in September 2004, respectively. Even without waterbloom, the concentration of MC-LR in source water sample was still higher than the guideline value. Conclusion The status of microcystin pollution in this region is serious and measures to monitor and control the growth of cyanobacteria are urgently needed.
基金supported by the Ministry of Science and Technology of China(Nos.2018YFE0204103,2017ZX07108002)the Youth Innovation Promotion Association,Chinese Academy of Sciences(No.2019043)。
文摘Significant iron release from cast iron pipes in water distribution systems(WDSs),which usually occurs during the source water switch period,is a great concern of water utilities because of the potential occurrence of"red water"and customer complaints.This study developed a new method which combined in-situ water stagnation experiments with mathematical models and numerical simulations to predict the iron release caused by source water switch.In-situ water stagnation experiments were conducted to determine the total iron accumulation in nine cast iron pipes in-service in Beijing when switching the local water to tre ated Danjiangkou Reservior water.Results showe d that the difference in the concentration increment of total iron in 24 hr(ΔCITI,24),i.e.short-term iron release,caused by source water switch was mainly dependent on the difference in the key quality parameters(pH,hardness,nitrate,Larson Ratio and dissolved oxygen(DO))between the two source waters.The iron release rate(RFe)after switch,i.e.long-term iron release,was closely related to the pipe properties as well as the DO and total residual chlorine(TRC)concentrations.Mathematical models ofΔCITI,24 and RFe were developed to quantitatively reveal the relationship between iron release and the key quality parameters.The RFe model could successfully combine with EPANET-MSX,a numerical simulator of water quality for WDSs to extend the iron release modeling from pipe level to network level.The new method is applicable to predicting iron release during source water switch,thus facilitating water utilities to take preventive actions to avoid"red water".
基金Supported by Major Science and Technology Program for Water Control and Treatment,China(2012ZX07404-003)Taishan Scholar Post Project,China(ts200640025)
文摘Mobile emergency pilot water plant was used to carry out pilot study of KMnO4 pre-oxidation enhanced coagulation treating high-algae source water. Research showed that the optimal dosages of coagulant and KMnO4 in the process were 6 and 0. 4- 0. 6 mg / L respectively. Under the dosage,removal rate of water turbidity after precipitation rose by 11% than simple coagulation,and removal rate of algae rose by 15%. Removal rates of total amount of odor and GSM by the process were respectively 73% and 59%. The removal rate of total amount of algae by KMnO4 preoxidation was 40%,and removal effect of THM precursors was obvious.
文摘The pollution problem arising from the flushing of initial rainwater and wastewater from accidents while transporting dangerous goods to source water protection areas needs to be solved as soon as possible.Therefore,the design of corresponding environmental protection measures should be considered in the engineering design stage.It is necessary to analyze the specific work in combination with engineering examples.Under this background,this paper first briefly expounds the precautions in accident risk analysis and the design of tank capacity and tank body.Finally,by analyzing actual cases,this paper systematically studies the design strategy of emergency pool in source water protection area,hoping to provide new development ideas for the upgrading of relevant work.
基金Supported by National Science and Technology Project of Water Pollution Control and Management(2008ZX07421-001)
文摘[Objective] The study aimed to discuss the application of a stereo constructed wetland to the treatment of slightly polluted source water. [Method] In this study, a new stereo constructed wetland mode was put forward, and a pilot project of water ecological purification in Xinsheng River, the diversion channel of Shijiuyang Waterwork in Jiaxing City, were analyzed. Afterwards, the impact factors of water purification by the technology were discussed from water quality and quantity, season and climate, species configuration, management and maintenance. [Result] Under three different hydraulic loading conditions, the pilot project effectively improved water SD and DO level, and reduced SS, CODCr, NH3-N, TN and TP significantly in summer and autumn, so that effluent water quality reached surface water standard at Grade III. [Conclusion] The stereo constructed wetland mode composed of constructed wetland and underwater forest used to treat slightly polluted source water is feasible and has a good promotion prospect.
基金supported by the National Natural Science Foundation of China(42161007)the Innovation Foundation of Higher Education Institutions of Gansu Province(2021B-081)the Foundation for Distinguished Young Scholars of Gansu Province(20JR10RA112).
文摘Precipitation isotopes(δ^(18)O and δ^(2)H)are closely related to meteorological conditions for precipitation generation and the initial state of water vapor source areas,and are essential to the study of the regional hydrological cycle.The deuterium excess(d-excess)indicates deviation in isotope fractionation during evaporation and can trace water vapor sources.This study analyzed 443 precipitation samples collected from the Gannan Plateau,China in 2022 to assess precipitation isotope variations and their driving factors.Water vapor sources were evaluated using the Hybrid Single-Particle Lagrangian Integrated Trajectory(HYSPLIT),Concentration Weighted Trajectory(CWT),and Potential Source Contribution Factor(PSCF)models.Results showed that precipitation isotope values showed significant spatial and temporal variations on the Gannan Plateau.Temporally,precipitation isotope values peaked in June(when evaporation dominated)and minimized in March(depletion effect of air masses in the westerly wind belt).Spatially,the isotope values showed a distribution pattern of"high in the east and low in the west",which was mainly regulated by the differences in altitude and local meteorological conditions.Compared with the global meteoric water line(GMWL)with equation of δ^(2)H=8.00δ^(18)O+10.00,the slope and intercept of local meteoric water line(LMWL)for precipitation on the Gannan Plateau were smaller(7.49 and 7.63,respectively),reflecting the existence of a stronger secondary evaporation effect under the clouds in the region.The sources of water vapor on the Gannan Plateau showed significant seasonality and spatial heterogeneity.Specifically,the westerly belt and monsoon were the main water vapor transport paths at each sampling point,with Central Asian continental water vapor dominating in spring(53.49%),Indian Ocean water vapor dominating in summer(52.53%),Atlantic Ocean water vapor dominating in autumn(46.74%),and Atlantic Ocean and Mediterranean Sea water vapor dominating in winter(42.30%and 33.68%,respectively).Changes in the intensity of convective activity and Outgoing Longwave Radiation(OLR)affected the enrichment of isotopic values,which exhibited the same change trends as δ^(18)O.During the precipitation process,the δ^(18)O value first decreased and then increased.During the initial and final stages of precipitation process,precipitation was mainly influenced by continental air masses,while during the middle stage,it was controlled by marine air masses.The systematic research on precipitation isotopes and water vapor sources is important for climate change research and extreme precipitation prediction on the Gannan Plateau and other similar areas.
文摘Groundwater overextraction and contamination by heavy metals such as cadmium and arsenic have resultedin ecological degradation and increased risks of renal disease,particularly in water-scarce regions.To address thesechallenges,this review aimed to evaluate the ecological potential of dew water harvesting as a sustainable and safealternative water source.Literature published between 2000 and 2024 was systematically searched in PubMed,Scopus,Web of Science,and Google Scholar using the terms“dew water,”“atmospheric water harvesting,”“groundwaterpollution,”“heavy metals,”“ecosystem restoration,”and“sustainable water systems.”Studies were included if theyfocused on dew water quality,ecological functions,or health-related outcomes,while non-English publications,conference abstracts without full text,and studies not directly addressing dew water were excluded.A total of 46 studiesand 7 official guidelines met the eligibility criteria.Findings indicate that natural dew water generally exhibits a neutralpH(6.5–8.5),negligible concentrations of heavy metals,and relatively high dissolved oxygen content(~9 mg/L).Casestudies from Morocco,Israel,China,and India illustrate its contributions to soil moisture retention,plant survival,biodiversity support,and microclimate regulation.Moreover,dew water produced through the Systemized Dew Process(SDP)consistently complied with WHO(2024)standards for drinking water,showing contaminant levels belowdetection thresholds.In conclusion,dew water harvesting represents a low-impact,climate-resilient,and safe alternativethat mitigates exposure to nephrotoxic pollutants,reduces reliance on overexploited groundwater,and enhances longtermecological restoration and water security in degraded and water-scarce environments.
基金jointly supported by the Open Research Fund of State Environmental Protection Key Laboratory of Drinking Water Source Protection,Chinese Research Academy of Environmental Sciences(2022YYSYKFYB07)the Fundamental Research Funds for the Central Publicinterest Scientific Institution(2022YSKY-07)the China Geological Survey Project(DD20211414).
文摘Pharmaceuticals and personal care products(PPCPs)are receiving attention as emerging pollutants due to their extensive applications and persistent emissions.The Qiantang River Basin,a representative region in eastern China that relies on surface water for drinking purposes,experiences the movement and accumulation of PPCPs in its water and sediment,which can directly affect the safety of drinking water in the basin.This study focuses on the Qiantang River Basin’s surface water,sediment,and drinking water to determine the occurrence and potential risks of 31 PPCPs.It aims to address whether PPCPs in the environment could migrate and accumulate,thereby affecting human health.The findings indicated that PPCPs are ubiquitous in various environmental media,with surface and pore water showing distinct spatial distribution characteristics,specifically,concentrations escalated with urban scale expansion,indicating that domestic sewage discharge is the primary source of PPCP input.Bisphenol A(BPA),ketoprofen(KTP),and diethyltoluamide(DEET)were the primary contaminants.The movement of PPCPs within the surface water-sediment-pore water system was affected by various circumstances.Substances like Sulfamethoxazole(SMX)(RQ>103)and KTP(RQ=22.3)present in surface water and sediment pose significant ecological concerns,and KTP and atrazine(ATZ)(0.6<RQ<2.1)also pose a high risk in drinking water.This study performed an extensive analysis of the distribution and risks associated with typical PPCPs in the Qiantang River Basin,offering a scientific foundation and theoretical support for research on the environmental behavior of PPCPs in this area and the development of targeted pollution control strategies.
基金Acknowledgements This work was supported by the National Natural Science Foundation of China （Grant Nos. 20977102 and 21007077）, the Ministry of Water Resources＇ Special Funds for Scientific Research on Public Causes （No. 201201032） and the Environmental Protection National Commonweal Research Project （No. 200909040）.
文摘The Danjiangkou reservoir was selected to provide the source water for the middle routes of the South to North Water Transfer Project, which has provoked many environmental concerns. To date, investigations of water contamination of the source water of the Danjiangkou reservoir with organic micro-pollutants have been limited. This study was conducted to identify and rank organic contaminants that pose risks in the Danjiangkou reservoir. To this end, the Chemical Hazard Evaluation and Manage- ment Strategies （CHEMS-1） approach was adapted to integrate the deconvolution technology of qualitative identifying contaminants for site-specific environmental matrices. The samples were screened for the presence of 1093 contaminants using deconvolution technologies and the hazard values of the identified contaminants were calculated using the adapted CHEMS-1 approach accord- ing to their hazardous properties and occurrence in source water. The results showed that 46 contaminants from 1093 targets were present in Danjiangkou water, 23 of which appeared at frequencies higher than 50%, and 15 of which were identified as priorities. Over half （53%） of the high- ranked contaminants were polycyclic aromatic hydrocar- bons （PAHs）, with chrysene ranked highest on the list. Health risk assessment of the top-ranked PAHs was conducted and revealed that cancer risks of PAHs detected in the source water of Danjiangkou to different populations ranged from 10-7 to 104, indicating a low cancer risk to consumers. The results of this study indicated that the adapted CHEMS-1 approach was feasible for site-specific screening of organic contaminants to identify and rank potential priority pollutants.
文摘Since the ammonia in the effluent of the tradi-tional water purification process could not meet the supply demand,the advanced treatment of a high concentration of NH4+-N micro-polluted source water by biological activated carbon filter(BACF)was tested.The filter was operated in the downflow manner and the results showed that the remov-ing rate of NH_(4)^(+)-N was related to the influent concentration of NH_(4)^(+)-N.Its removing rate could be higher than 95%when influent concentration was under 1.0 mg/L.It could also decrease with the increasing influent concentration when the NH_(4)^(+)-N concentration was in the range from 1.5 to 4.9 mg/L and the dissolved oxygen(DO)in the influent was under 10 mg/L,and the minimum removing rate could be 30%.The key factor of restricting nitrification in BACF was the influent DO.When the influent NH_(4)^(+)-N concentration was high,the DO in water was almost depleted entirely by the nitrifying and hetetrophic bacteria in the depth of 0.4 m filter and the filter layer was divided into aerobic and anoxic zones.The nitrification and degradation of organic matters existed in the aerobic zone,while the denitrification occurred in the anoxic zone.Due to the limited carbon source,the denitrifica-tion could not be carried out properly,which led to the accu-mulation of the denitrification intermediates such as NO_(2)^(−).In addition to the denitrification bacteria,the nitrification and the heterotrophic bacteria existed in the anoxic zone.
基金partially supported by the research project"Water and Environment"by the Secretary of Science and Technology of the University National of Santiago del Estero,Argentina(UNSE)+1 种基金National University of Distance Education(UNED)(project reference:2017/CTINV-0024)by the Comunidad of Madrid and European funding from FSE and FEDER programs(project S2018/BAA-4393,AVANSECALII-CM)。
文摘This study investigates the suitability of statistical techniques for evaluating the fluoride content and the groundwater quality from Robles Department(RD)and Banda Department(BD)in Santiago del Estero(Argentina).For the original statistical study,evaluation of nine parameters(fluoride,pH,conductivity,atmospheric and water temperature,total dissolved solids,chloride,hardness,and alkalinity)of 110 collected underground water samples from 23 dispersed rural areas was proposed.Groundwater samples were obtained by sampling taken from wells at different depths.Fluoride levels were determined by a standard colorimetric method in two seasonal periods,the dry(from April to September)and rainy(from October to March)period.The analytical results obtained for physicochemical parameters such as pH,total dissolved solids(TDS),and temperature does not reveal any notable difference between the rainy and dry seasons studied.In both seasons,the atmospheric temperature average was 22℃.With respect to fluoride content,approximately 50%of the analysed groundwater samples exceeded the limit established by current legislation(1.0 mg/L),obtaining concentration levels in the range of 0.01-2.80 mg/L.This study demonstrates the usefulness of the univariate statistical method(quartiles calculation,interquartile range IQR),multivariate principal component analysis(PCA),and cluster analysis to establish a better understanding of the state of the contamination of the waters in the region studied.
文摘Heavy metal pollution in agricultural water resources is very serious in re- cent years, resulting in large losses of the agricultural economy and endangering human life and health. Due to the advantages of low cost, high efficiency and less secondary pollution, microbial ramediation technology is widely used in the treatment of heavy metal pollution in agricultural water resources. At present, with the progress of modern biotechnology, microbial remediation of heavy metals in agricul- tural water resources has grown rapidly. The sources and status quo of heavy met- al pollution in agricultural water resources at home and aboard, and the principles of microbial remediation of heavy metals pollution in agricultural water resources were reviewed in this paper, as well as the several common microbial remediation technology of heavy metals in agricultural water resources. Additionally, the further research work of heavy metal contaminated agricultural water resources by microbial ramediation were prospected.
基金supported by the Water Pollution Control and Management (No. 2009ZX07419-002-2,2009ZX07419-003)the International Science and Technology Cooperation Program of China (No.2007DFA90510)
文摘The characteristics of ammonia in drinking water sources in China were evaluated during 2005-2009. The spatial distribution and seasonal changes of ammonia in different types of drinking water sources of 22 provinces, 5 autonomous regions and 4 municipalities were investigated. The levels of ammonia in drinking water sources follow the order of fiver 〉 lake/reservoir 〉 groundwater. The levels of ammonia concentration in river sources gradually decreased from 2005 to 2008, while no obvious change was observed in the lakes/reservoirs and groundwater drinking water sources. The proportion of the type of drinking water sources is different in different regions. In river drinking water sources, the ammonia level was varied in different regions and changed seasonally. The highest value and wide range of annual ammonia was found in South East region, while the lowest value was found in Southwest region. In lake/reservoir drinking water sources, the ammonia levels were not varied obviously in different regions. In underground drinking water sources, the ammonia levels were varied obviously in different regions due to the geological permeability and the natural features of regions. In the drinking water sources with higher ammonia levels, there are enterprises and wastewater drainages in the protected areas of the drinking water sources.
基金Project supported by the State Key Laboratory of Soil and Sustainable Agriculture, Institute of Soil Science, Chinese Academy of Sciences (No. 035109)the National Natural Science Foundation of China (No. 30390080).
文摘The nitrogen （N） pollution status of the 12 most important rivers in Changshu, Taihu Lake region was investigated. Water samples were collected from depths of 0.5-1.0 m with the aid of the global positioning system （GPS）. The seasonal variations in the concentrations of different N components in the rivers were measured. Using tension-free monolith lysimeters and ^15N-labeled fertilizer, field experiments were carried out in this region to determine variations of iSN abundance of NO3^- in the leachate during the rice and wheat growing seasons, respectively. Results showed that the main source of N pollution of surface waters in the Taihu Lake region was not the N fertilizer applied in the farmland but the urban domestic sewage and rural human and animal excreta directly discharged into the water bodies without treatment. Atmospheric dry and wet N deposition was another evident source of N pollutant of the surface waters. In conclusion, it would not be correct to attribute the N applied to farmlands as the source of N pollution of the surface waters in this region.
基金Supported by the Special Fund for the Control and Management of Chaohu Lake of the National Key Technology R&D Program,China(2008ZX07103-005)the Special Fund for the Control and Management of Huaihe River of the National Key Technology R&D Program,China(2008ZX07010-004)+1 种基金National Natural Science Foundation of China(40073030,40972092,41172121)the Natural Science Foundation of Anhui Province,China(090413083)~~
文摘[Objective] To study the characteristics and effects of inorganic nitrogen in east water-source and inflow rivers of Chaohu Lake. [Method] The speciation and distribution characteristics of dissolvable inorganic nitrogen （DIN） in east water-source and inflow rivers of Chaohu Lake were investigated, and their effects on water qual- ity were examined. [Result] The concentrations of NH3-N and NO2--N were the high in flood season, and low in non-flood season, while the concentration of NO3--N pre- sented the opposite trend; the concentration of NO3--N was the highest in Shuangqiao estuary, where the pollution was the worst. DIN in Zhegao estuary and Xiaozhegao estuary was mainly caused by domestic sewage and industrial wastewaters; surface runoff and pollution from ships contribute the most to the DIN content in Shuangqiao estuary. [Conclusion] This study provided basic data and theoretical basis for the control and management of eutrophication in Chaohu Lake.
基金supported by the Bureau of Water Resource of Wujiang District(No.SZSY2018WJG032A)the Joint Innovative and Technological Research Projects from the Ministry of Science and Technology of the People’s Republic of China(No.2016YFE0115800)+1 种基金the China Major Science and Technology Program for Water Pollution Control and Treatment(No.2017ZX07205002)Shanghai Institute of Pollution Control and Ecological Security and the Key Laboratory of Yangtze River Water Environment,Ministry of Education,China
文摘An embedded reservoir that provides an efficient nutrient removal system protects drinking water.However,embedded reservoirs are rarely used in eutrophic shallow lakes because of their undetermined nutrient retention efficiency and unknown effects by the phytoplankton community.In this study,we aim to investigate the nutrient retention and algae succession in an embedded reservoir and adjacent wetland from April 2017 to September 2018 in the eastern part of Lake Taihu,China.More than 40%of total phosphorus(TP)and 45%of particulate phosphorous entering the reservoir were retained semiannually,and the highest TP removal efficiency was achieved in the reservoir during autumn with an average value of 53.3%±9.9%.The overall nitrogen retention efficiency(21.7%±37.8%)was lower than that of TP(41.8%±27.8%).Similar trends were obtained in the wetland area.An important pathway for phosphorus removal is through particulate matter retention.Our study revealed that nutrient retention mechanisms in the reservoir were primarily via macrophyte absorption,particulate substance sedimentation,and prolonged water residence time.Consequently,the phytoplankton biomass(Chl-a)in the reservoir decreased(from 48.0 to 25.2μg/L)and water transparency improved,due to the decreased P level and transformation of the phytoplankton group into simple structures with good ecological status.Therefore,the combination of embedded reservoir and constructed wetland ecosystem can be used successfully to protect surface water.The results will be advantageous to groups seeking to preserve drinking water sources.
