The attosecond extreme ultraviolet(XUV) pulse pump and femtosecond infrared(IR) pulse probe scheme is commonly used to study the dynamics and attosecond transient absorption(ATA) spectra of microscopic systems. In a r...The attosecond extreme ultraviolet(XUV) pulse pump and femtosecond infrared(IR) pulse probe scheme is commonly used to study the dynamics and attosecond transient absorption(ATA) spectra of microscopic systems. In a recent report [Proc. Natl. Acad. Sci. USA 121 e2307836121(2024)], we showed that shaped XUV pulses with spectral minima can significantly alter the absorption line shape of helium's 2s2p doubly excited state within a few tens of attoseconds.However, it remains unclear if similar effects could be observed in a singly excited state. In this study, we use shaped XUV pulses to excite helium's 2p singly excited state and couple the 2p and 3d states with a delayed IR pulse. Comparing these results with those from Gaussian XUV pulses, we find that the ATA spectra for the shaped XUV pulses exhibit more pronounced changes with delay, while the changes for the Gaussian pulses are gradual. We also explain these differences through population changes and analytical models. Our findings show that shaped XUV pulses can regulate the dynamics and absorption spectra of a singly excited state.展开更多
Resonance enhancement has been increasingly employed in the emergent felntosecond stimu- lated Raman spectroscopy （FSRS） to selectively monitor molecular structure and dynamics with improved spectral and temporal re...Resonance enhancement has been increasingly employed in the emergent felntosecond stimu- lated Raman spectroscopy （FSRS） to selectively monitor molecular structure and dynamics with improved spectral and temporal resolutions and signal-to-noise ratios. Such joint eflforts by the technique- and application-oriented scientists and engineers have laid the foundation for exploiting the tunable FSRS methodology to investigate a great variety of photosensitive systems and elucidate the underlying functional mechanisms on molecular time scales. Dur- ing spectral analysis, peak line shapes remain a major concern with an intricate dependence on resonance conditions. Here, we present a comprehensive study of line shapes by tuning the Rarnan pump wavelength from red to blue side of the ground-state absorption band of the fluorescent dye rhodarnine 6G in solution. Distinct line shape patterns in Stokes and anti-Stokes FSRS as well as from the low to high-frequency modes highlight the competition between multiple third-order and higher-order nonlinear pathways, governed by difl^rent res- onance conditions achieved by Raman pump and probe pulses. In particular, the resonance condition of probe wavelength is revealed to play an important role in generating circular line shape changes through oppositely phased dispersion via hot luminescence （HL） pathways. Meanwhile, on-resonance conditions of the Rarnan pump could promote excited-state vibrational modes which are broadened and red-shifted from the coincident ground-state vibrational modes, posing challenges for spectral analysis. Certain strategies in tuning the Raman pump and probe to characteristic regions across an electronic transition band are discussed to improve the FSRS usability and versatility as a powerful structural dynamics toolset to advance chemical, physical, materials, and biological sciences.展开更多
We numerically investigate a coupled-resonator structure consisting of a stub resonator and a nanodisk resonator using a two-dimensional finite element method. Simulation results show that plasmon-induced transparency...We numerically investigate a coupled-resonator structure consisting of a stub resonator and a nanodisk resonator using a two-dimensional finite element method. Simulation results show that plasmon-induced transparency （PIT） occurs in the transmission spectra, and the sharp asymmetric Fano lines increase the sensitivity to 1.4 ×10^3 nm/RIU. We also analyze the properties of the structure with different radii of the nanodisk and the length of the tooth cavity. Moreover, we find that the PIP only happens when the staggered system is around a fixed location with different separate distances, which is not similar to the previous researches. Our model may be important to photonic-integrated circuits and the sensitivity in sensors.展开更多
We present the design and the experimental demonstration of an invisible cloak with irregular shape by using tensor transmission line（TL） metamaterials. The fabricated cloak consists of tensor TL unit cells exhibiti...We present the design and the experimental demonstration of an invisible cloak with irregular shape by using tensor transmission line（TL） metamaterials. The fabricated cloak consists of tensor TL unit cells exhibiting anisotropic effective material parameters, while the background medium consists of isotropic TL unit cells. The simulated and the measured field patterns around the cloak show a fairly good agreement, both demonstrate that the fabricated cloak can shield the cloaked interior area from electromagnetic fields without perturbing the external fields. The scattering of the cloaked perfect electric conductor（PEC） is minimized. Furthermore, the nonresonant property of the TL structure results in a relatively broad bandwidth of the realized cloak, which is clearly observed in our experiment.展开更多
The study on a miniaturized, low-voltage, wide-bandwidth, high-efficiency modified V-shaped microstrip meander-line slow-wave structure is presented. This structure is evolved from the original U-shaped microstrip mea...The study on a miniaturized, low-voltage, wide-bandwidth, high-efficiency modified V-shaped microstrip meander-line slow-wave structure is presented. This structure is evolved from the original U-shaped microstrip meander-line slow-wave structure, combining the advantages of a traditional microstrip and a rectangular helix. In this paper, simulations of the electromagnetic characteristics and the beam-wave interaction of this structure are carried out. Our study shows that when the design voltage and the current of a sheet electron beam are set to be 4700 V and 100 mA, respectively, this miniature millimeter-wave power amplifier is capable of delivering 160-W output power with a corresponding gain of 37.3 dB and a maximum interaction efficiency of 34% at 97 GHz.展开更多
钢拱桥的线形监测是桥梁健康监测系统的重要组成部分。运用三维激光扫描技术,融合随机抽样一致(random sample consensus,RANSAC)算法对传统的具有噪声的基于密度的聚类方法(density-based spatial clustering of applications with noi...钢拱桥的线形监测是桥梁健康监测系统的重要组成部分。运用三维激光扫描技术,融合随机抽样一致(random sample consensus,RANSAC)算法对传统的具有噪声的基于密度的聚类方法(density-based spatial clustering of applications with noise,DBSCAN)算法进行改进,对钢拱桥拱肋线形进行提取。三维激光点云数据具有全面性和细节体现的优势,能够完整地呈现桥梁结构的形状和变形信息,融合RANSAC的改进DBSCAN算法根据钢拱桥结构特征对聚类结果进行约束,能够很好地实现删除离散点及桥面、横撑、横联和腹杆部分的点云这一目的。根据融合RANSAC的改进DBSCAN算法提取出的点云进行关键点拟合,与人工提取结果进行对比,拱肋关键点提取误差均在毫米级,最大误差为9.2 mm,最小误差为0.1 mm,此提取方法能够更加准确有效地完成钢拱桥线形提取,使线形提取精度达到毫米级,大大降低了人力成本和时间成本,对钢拱桥的复杂结构有更好的鲁棒性,能很好地适应实际生产需求。展开更多
针对当前大部分居民地形状相似性度量方法不能兼顾居民地整体特征和局部差异的局限,提出一种基于层次骨架线的居民地形状相似性评价方法。该方法以降维为基本思想,能充分考虑待度量居民地的主体特征和细节差异。先以象征性和形态概括性...针对当前大部分居民地形状相似性度量方法不能兼顾居民地整体特征和局部差异的局限,提出一种基于层次骨架线的居民地形状相似性评价方法。该方法以降维为基本思想,能充分考虑待度量居民地的主体特征和细节差异。先以象征性和形态概括性这两个特点为依据,以某区域OSM(Open Street Map)矢量面数据为例,构建一批分别对应于3个不同构型待度量居民地目标的模板;再分别对目标和模板提取层次骨架线并建立骨架线缓冲区,进一步依据骨架线的层次特性来计算二者的主体相似度、细节相似度和综合相似度。实验结果表明,该方法能对来自不同中大比例尺地图的构型相同或接近、面积差异较大的待度量居民地和模板同时进行层次和整体相似性度量。展开更多
基金Project supported by the National Natural Science Foundation of China (Grant No. 12274230)the Funding of Nanjing University of Science and Technology (Grant No. TSXK2022D005)。
文摘The attosecond extreme ultraviolet(XUV) pulse pump and femtosecond infrared(IR) pulse probe scheme is commonly used to study the dynamics and attosecond transient absorption(ATA) spectra of microscopic systems. In a recent report [Proc. Natl. Acad. Sci. USA 121 e2307836121(2024)], we showed that shaped XUV pulses with spectral minima can significantly alter the absorption line shape of helium's 2s2p doubly excited state within a few tens of attoseconds.However, it remains unclear if similar effects could be observed in a singly excited state. In this study, we use shaped XUV pulses to excite helium's 2p singly excited state and couple the 2p and 3d states with a delayed IR pulse. Comparing these results with those from Gaussian XUV pulses, we find that the ATA spectra for the shaped XUV pulses exhibit more pronounced changes with delay, while the changes for the Gaussian pulses are gradual. We also explain these differences through population changes and analytical models. Our findings show that shaped XUV pulses can regulate the dynamics and absorption spectra of a singly excited state.
基金supported by the U.S.National Science Foundation CAREER grant(CHE-1455353)the Oregon State University(OSU) Research Equipment Reserve Fund(Spring 2014)to C.Fang(USTC9603)the Wei Family Private Foundation in supporting C.Chen(USTC 0903) during his graduate studies at OSU Chemistry
文摘Resonance enhancement has been increasingly employed in the emergent felntosecond stimu- lated Raman spectroscopy （FSRS） to selectively monitor molecular structure and dynamics with improved spectral and temporal resolutions and signal-to-noise ratios. Such joint eflforts by the technique- and application-oriented scientists and engineers have laid the foundation for exploiting the tunable FSRS methodology to investigate a great variety of photosensitive systems and elucidate the underlying functional mechanisms on molecular time scales. Dur- ing spectral analysis, peak line shapes remain a major concern with an intricate dependence on resonance conditions. Here, we present a comprehensive study of line shapes by tuning the Rarnan pump wavelength from red to blue side of the ground-state absorption band of the fluorescent dye rhodarnine 6G in solution. Distinct line shape patterns in Stokes and anti-Stokes FSRS as well as from the low to high-frequency modes highlight the competition between multiple third-order and higher-order nonlinear pathways, governed by difl^rent res- onance conditions achieved by Raman pump and probe pulses. In particular, the resonance condition of probe wavelength is revealed to play an important role in generating circular line shape changes through oppositely phased dispersion via hot luminescence （HL） pathways. Meanwhile, on-resonance conditions of the Rarnan pump could promote excited-state vibrational modes which are broadened and red-shifted from the coincident ground-state vibrational modes, posing challenges for spectral analysis. Certain strategies in tuning the Raman pump and probe to characteristic regions across an electronic transition band are discussed to improve the FSRS usability and versatility as a powerful structural dynamics toolset to advance chemical, physical, materials, and biological sciences.
基金Supported by the National Natural Science Foundation of China under Grant Nos 11374041 and 11404030the Fund of State Key Laboratory of Information Photonics and Optical Communications of Beijing University of Posts and Telecommunications of China
文摘We numerically investigate a coupled-resonator structure consisting of a stub resonator and a nanodisk resonator using a two-dimensional finite element method. Simulation results show that plasmon-induced transparency （PIT） occurs in the transmission spectra, and the sharp asymmetric Fano lines increase the sensitivity to 1.4 ×10^3 nm/RIU. We also analyze the properties of the structure with different radii of the nanodisk and the length of the tooth cavity. Moreover, we find that the PIP only happens when the staggered system is around a fixed location with different separate distances, which is not similar to the previous researches. Our model may be important to photonic-integrated circuits and the sensitivity in sensors.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11174280,60990323,and 60990320)the Knowledge Innovation Program of the Chinese Academy of Sciences(Grant No.YYYJ-1123)
文摘We present the design and the experimental demonstration of an invisible cloak with irregular shape by using tensor transmission line（TL） metamaterials. The fabricated cloak consists of tensor TL unit cells exhibiting anisotropic effective material parameters, while the background medium consists of isotropic TL unit cells. The simulated and the measured field patterns around the cloak show a fairly good agreement, both demonstrate that the fabricated cloak can shield the cloaked interior area from electromagnetic fields without perturbing the external fields. The scattering of the cloaked perfect electric conductor（PEC） is minimized. Furthermore, the nonresonant property of the TL structure results in a relatively broad bandwidth of the realized cloak, which is clearly observed in our experiment.
基金Project supported by the National Natural Science Foundation of China (Grant No. 60971038)the Fundamental Research Funds for the Central Universities (Grant No. ZYGX2009Z003)
文摘The study on a miniaturized, low-voltage, wide-bandwidth, high-efficiency modified V-shaped microstrip meander-line slow-wave structure is presented. This structure is evolved from the original U-shaped microstrip meander-line slow-wave structure, combining the advantages of a traditional microstrip and a rectangular helix. In this paper, simulations of the electromagnetic characteristics and the beam-wave interaction of this structure are carried out. Our study shows that when the design voltage and the current of a sheet electron beam are set to be 4700 V and 100 mA, respectively, this miniature millimeter-wave power amplifier is capable of delivering 160-W output power with a corresponding gain of 37.3 dB and a maximum interaction efficiency of 34% at 97 GHz.
文摘针对当前大部分居民地形状相似性度量方法不能兼顾居民地整体特征和局部差异的局限,提出一种基于层次骨架线的居民地形状相似性评价方法。该方法以降维为基本思想,能充分考虑待度量居民地的主体特征和细节差异。先以象征性和形态概括性这两个特点为依据,以某区域OSM(Open Street Map)矢量面数据为例,构建一批分别对应于3个不同构型待度量居民地目标的模板;再分别对目标和模板提取层次骨架线并建立骨架线缓冲区,进一步依据骨架线的层次特性来计算二者的主体相似度、细节相似度和综合相似度。实验结果表明,该方法能对来自不同中大比例尺地图的构型相同或接近、面积差异较大的待度量居民地和模板同时进行层次和整体相似性度量。
