Interface engineering is thought to be one of the most effective methods to reduce the recombination of electron and holes.Especially,the introduction of interfacial chemical bonds could greatly help to promote the ch...Interface engineering is thought to be one of the most effective methods to reduce the recombination of electron and holes.Especially,the introduction of interfacial chemical bonds could greatly help to promote the charge migration and separation.Interface chemical bonds are one kind of strong interactions between adjacent phases caused by the sharing of outer electrons,which could not only optimize the inter-facial electron distribution of different phases,but also pave electron-level channels like a"bridge"for charge transfer.It plays an important role in regulating photogenerated charge transfer,reactant adsorption,and the activation energy of catalytic reactions.Research in this area is the current focus for the PEC water splitting,CO_(2)reduction,organic catalysis and photodynamic antibacterial[1-3].展开更多
基金supported by the National Natural Science Foundation of China(Nos.52172174,and 51872002)the Program of Anhui Scientific and Technical Leaders Reserve Candidates(2018RH168).
文摘Interface engineering is thought to be one of the most effective methods to reduce the recombination of electron and holes.Especially,the introduction of interfacial chemical bonds could greatly help to promote the charge migration and separation.Interface chemical bonds are one kind of strong interactions between adjacent phases caused by the sharing of outer electrons,which could not only optimize the inter-facial electron distribution of different phases,but also pave electron-level channels like a"bridge"for charge transfer.It plays an important role in regulating photogenerated charge transfer,reactant adsorption,and the activation energy of catalytic reactions.Research in this area is the current focus for the PEC water splitting,CO_(2)reduction,organic catalysis and photodynamic antibacterial[1-3].
