We delve into the phenomenon of high-order harmonic generation within a helium atom under the influence of a plasmon-assisted shaping pulse.Our findings reveal an intriguing manipulation of the frequency peak position...We delve into the phenomenon of high-order harmonic generation within a helium atom under the influence of a plasmon-assisted shaping pulse.Our findings reveal an intriguing manipulation of the frequency peak position in the harmonic emission by adjusting the absolute phase parameter within the frequency domain of the shaping pulse.This phenomenon holds potential significance for experimental setups necessitating precisely tuned single harmonics.Notably,we observe a modulated shift in the created harmonic photon energy,spanning an impressive range of 1.2 eV.This frequency peak shift is rooted in the asymmetry exhibited by the rising and falling edges of the laser pulse,directly influencing the position of the peak frequency emission.Our study quantifies the dependence of this tuning range and the asymmetry of the laser pulse,offering valuable insights into the underlying mechanisms driving this phenomenon.Furthermore,our investigation uncovers the emergence of semi-integer order harmonics as the phase parameter is altered.We attribute this discovery to the intricate interference between harmonics generated by the primary and secondary return cores.This observation introduces an innovative approach for generating semi-integer order harmonics,thus expanding our understanding of high-order harmonic generation.Ultimately,our work contributes to the broader comprehension of complex phenomena in laser-matter interactions and provides a foundation for harnessing these effects in various applications,particularly those involving precise spectral control and the generation of unique harmonic patterns.展开更多
We theoretically investigated the properties of the high-order harmonic generation from an argon atom by bichromatic counter-rotating circularly polarized(BCCP)laser field.The harmonic emission processes have been ill...We theoretically investigated the properties of the high-order harmonic generation from an argon atom by bichromatic counter-rotating circularly polarized(BCCP)laser field.The harmonic emission processes have been illustrated by numerically solving the two-dimensional time-dependent Schr¨odinger equation of an atom in intense laser fields.It is found that with the decrease of the right-circularly polarized laser wavelength,the harmonic spectra are gradually splitting and the harmonic orders move towards the higher frequency.Meanwhile,the integer and semi-integer harmonic emission will be generated when the frequency ratios of right-and left-circularly polarized lasers are semi-integer.The emission mechanism of the semi-integer-order harmonics has been investigated by using the rules of photon absorption and emission.展开更多
基金This project was supported by the National Key Research and Development Program of China(Grant Nos.2022YFE134200 and 2019YFA0307700)the National Natural Science Foundation of China(Grant Nos.11604119,12104177,11904192,12074145,and 11704147)the Fundamental Research Funds for the Central Universities(Grant Nos.GK202207012 and QCYRCXM-2022-241).
文摘We delve into the phenomenon of high-order harmonic generation within a helium atom under the influence of a plasmon-assisted shaping pulse.Our findings reveal an intriguing manipulation of the frequency peak position in the harmonic emission by adjusting the absolute phase parameter within the frequency domain of the shaping pulse.This phenomenon holds potential significance for experimental setups necessitating precisely tuned single harmonics.Notably,we observe a modulated shift in the created harmonic photon energy,spanning an impressive range of 1.2 eV.This frequency peak shift is rooted in the asymmetry exhibited by the rising and falling edges of the laser pulse,directly influencing the position of the peak frequency emission.Our study quantifies the dependence of this tuning range and the asymmetry of the laser pulse,offering valuable insights into the underlying mechanisms driving this phenomenon.Furthermore,our investigation uncovers the emergence of semi-integer order harmonics as the phase parameter is altered.We attribute this discovery to the intricate interference between harmonics generated by the primary and secondary return cores.This observation introduces an innovative approach for generating semi-integer order harmonics,thus expanding our understanding of high-order harmonic generation.Ultimately,our work contributes to the broader comprehension of complex phenomena in laser-matter interactions and provides a foundation for harnessing these effects in various applications,particularly those involving precise spectral control and the generation of unique harmonic patterns.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61575077 and 11904122)the Natural Science Foundation of Jilin Province of China(Grant No.20180101225JC)the China Postdoctoral Science Foundation(Grant Nos.2018M641766 and 2019T120232).
文摘We theoretically investigated the properties of the high-order harmonic generation from an argon atom by bichromatic counter-rotating circularly polarized(BCCP)laser field.The harmonic emission processes have been illustrated by numerically solving the two-dimensional time-dependent Schr¨odinger equation of an atom in intense laser fields.It is found that with the decrease of the right-circularly polarized laser wavelength,the harmonic spectra are gradually splitting and the harmonic orders move towards the higher frequency.Meanwhile,the integer and semi-integer harmonic emission will be generated when the frequency ratios of right-and left-circularly polarized lasers are semi-integer.The emission mechanism of the semi-integer-order harmonics has been investigated by using the rules of photon absorption and emission.
