^(147,149)Sm are slow neutron capture(s-process)nuclides in nuclear astrophysics,whose(n,γ)cross sections are important input parameters in nucleosynthesis network calculations in the samarium(Sm)region.In addition,^...^(147,149)Sm are slow neutron capture(s-process)nuclides in nuclear astrophysics,whose(n,γ)cross sections are important input parameters in nucleosynthesis network calculations in the samarium(Sm)region.In addition,^(149)Sm is a fission product of ^(235)U with a 1%yield,and its neutron resonance parameters play a critical role in reactor neutronics.According to the available nuclear evaluation databases,a significant disagreement has been observed in the resonance peaks of the ^(147,149)Sm(n,γ)crosssectional data within the energy range of 20-300 eV.In this study,tutron capture cross section of a natural samarium target was measured at the back-streaming white neutron beamline of the China Spallation Neutron Source.The neutron capture yield was obtained,and the neutron resonance parameters for ^(147)Sm at 107.0,139.4,241.7,and 257.3 eV and ^(149)Sm at 23.2,24.6,26.1,28.0,51.5,75.2,90.9,125.3,and 248.4 eV were extracted using the SAMMY code based on R-matrix theory.For the parameters Γ_(n) and Γ_(γ) in these energies of ^(147,149)Sm,the percentages consistent with the results of the CENDL-3.2,ENDF/B-Ⅷ.0,JEFF-3.3,JENDL-4.0,and BROND-3.1 database are 27%,65%,65%,42%,and 58%,respectively.However,27% of the results were inconsistent with those of the major libraries.This work enriches experimental data of the ^(147,149)Sm neutron capture resonance and helps clarify the differences between different evaluation databases at the above energies.展开更多
By analyzing ψ(3686) data sample containing (107.7±0.6)×10^(6) events taken with the BESIII detector at the BEPCII storage ring in 2009,the χ_(c 0) resonance parameters are precisely measured using χ_(c 0...By analyzing ψ(3686) data sample containing (107.7±0.6)×10^(6) events taken with the BESIII detector at the BEPCII storage ring in 2009,the χ_(c 0) resonance parameters are precisely measured using χ_(c 0,c 2)→π^(+)π^(−)/K^(+)K^(−) events.The mass of χ_(c 0) is determined to be M (χ_(c 0))=(3415.63±0.07±0.07±0.07)MeV/c^(2),and its full width is F (χ_(c 0))=(12.52±0.12±0.13)MeV,where the first uncertainty is statistical,the second systematic,and the third for mass comes from χ_(c 2) mass uncertainty.These measurements improve the precision of χ_(c 0) mass by a factor of four and width by one order of magnitude over the previous individual measurements,and significantly boost our knowledge about the charmonium spectrum.Together with additional (345.4±2.6)×10^(6)(3686) data events taken in 2012,the decay branching fractions of χ_(c 0,c 2)→π^(+)π^(−)/K^(+)K^(−) are measured as well,with precision improved by a factor of three compared to previous measurements.These χ_(c 0) decay branching fractions provide important inputs for the study of glueballs.展开更多
The neutron total cross-sections of thulium （^169Tm） were measured in the neutron energy region from 0.01 eV to 100 eV by using the time-of-flight method at the Pohang Neutron Facility, which consists of an electron...The neutron total cross-sections of thulium （^169Tm） were measured in the neutron energy region from 0.01 eV to 100 eV by using the time-of-flight method at the Pohang Neutron Facility, which consists of an electron linac, a water-cooled tantalum target with a water moderator, and a 12 m time of flight path, Two thulium plates with different thicknesses were used for the neutron transmission measurement. The background level was determined by using a notch-filter of Co, In, and Cd sheets. The present measurement was compared with the previous ones, and a new set of resonance parameters of ^169Tm isotope was obtained from the transmission rate by using the SAMMY code, with a comparison with the recommended parameters by Mughabghab.展开更多
The neutron capture resonance parameters for 159Tb are crucial for validating nuclear models,nucleosynthesis during the neutron capture process,and nuclear technology applications.In this study,resonance analyses were...The neutron capture resonance parameters for 159Tb are crucial for validating nuclear models,nucleosynthesis during the neutron capture process,and nuclear technology applications.In this study,resonance analyses were performed for the neutron capture cross sections of 159Tb measured at the China Spallation Neutron Source(CSNS)backscattering white neutron beamline(Back-n)facility.The resonance parameters were extracted from the R-Matrix code SAMMY and fitted to the experimental capture yield up to the 1.2 keV resolved resonance region(RRR).The average resonance parameters were determined by performing statistical analysis on the set of the resonance parameters in the RRR.These results were used to fit the measured average capture cross sections using the FITACS code in the unresolved resonance region from 2 keV to 1 MeV.The contributions of partial waves l=0,1,2 to the average capture cross sections are reported.展开更多
The Earth＇s free core nutation （FCN） is a retrograde eigenrnode which is attributed to the interaction between the solid mantle and the liquid core of the rotational elliptical Earth. This mode appears as an eigenm...The Earth＇s free core nutation （FCN） is a retrograde eigenrnode which is attributed to the interaction between the solid mantle and the liquid core of the rotational elliptical Earth. This mode appears as an eigenmode of nearly diurnal free wobble （NDFW） in a terrestrial reference frame with a period of about one day （XU et al, 2001）. Therefore, the NDFW will lead to an obvious resonance enhancement in the diurnal tidal gravity observations, especially those of the tidal waves with frequencies closed to its eigenfrequency such as P1, K1, ψ1 and Ф1. The FCN resonance parameters can be retrieved accurately by high-precision tidal gravity observations, especially those recorded with the superconducting gravimeters （SG）. The Global Geodynamics Project （GGP） organized by IUGG took it as an important content for determining the FCN resonance parameters by using gravity data. However, the results are affected by many factors such as station location, background noise, the selection of the tide-generating potential tables, ocean tide models, data processing techniques and so on. In our study, the FCN parameters will be retrieved by using the SG observations at Wuhan, and the effects of the choices of various tide-generating potential tables, oceanic models and weight functions on the estimation of the FCN parameters will be discussed in detail,展开更多
The purpose of this study was to investigate the nuclear magnetic resonance （NMR） assignments of hydrolyzed products extracted from human blood plasma. The correlations between chemical, functional and structural pr...The purpose of this study was to investigate the nuclear magnetic resonance （NMR） assignments of hydrolyzed products extracted from human blood plasma. The correlations between chemical, functional and structural prop- erties of highly toxic pesticides were investigated using the PreADME analysis. We observed that toxic pesticides possessed higher molecular weight and, more hydrogen bond donors and acceptors when compared with less toxic pesticides. The occurrence of functional groups and structural properties was analyzed using ~H-NMR. The ~H- NMR spectra of the phosphomethoxy class of pesticides were characterized by methyl resonances at 3.7-3.9 ppm （8） with the coupling constants of 11-16 Hz （Je-cns）. In phosphoethoxy pesticides, the methyl resonance was about 1.4 ppm （8） with the coupling constant of 10 Hz （Je-cH2） and the methylene resonances was 4.2-4.4 ppm （8） with the coupling constant of 0.8 Hz （Jp-cH3）, respectively. Our study shows that the values of four parameters such as chemical shift, coupling constant, integration and relaxation time correlated with the concentration of toxic pesticides, and can be used to characterise the proton groups in the molecular structures of toxic pesticides.展开更多
We determine the resonant parameters of the vector statesϕ(1680)andϕ(2170)by performing a combined fit to the e+e−→ηϕcross sections from the threshold to 2.85GeV measured by the BaBar,Belle,BESIII,and CMD-3 experime...We determine the resonant parameters of the vector statesϕ(1680)andϕ(2170)by performing a combined fit to the e+e−→ηϕcross sections from the threshold to 2.85GeV measured by the BaBar,Belle,BESIII,and CMD-3 experiments.The mass(1678_(−3)^(+5)±7)MeV/c^(2) and width(156±5±9)MeV are obtained forϕ(1680),and the mass(2169±5±6)MeV/c^(2) and width(96_(−14)^(+17)±9)MeV are obtained forϕ(2170).The statistical significance ofϕ(2170)is 7.2σ.Depending on the interference betweenϕ(1680),ϕ(2170),and a non-resonantηϕamplitude in the nominal fit,we obtain four solutions andΓe+e−ϕ(1680)⋅B[ϕ(1680)→ηϕ]=(79±4±16),(127±5±12),(65_(−4)^(+5)±13)or(215_(−5)^(+8)±11)eV,andΓ_(ϕ(2170))^(e+e−)⋅B[ϕ(2170)→ηϕ]=(0.56_(−0.02)^(+0.03)±0.07),(0.36_(−0.03)^(+0.05)±0.07),(38±1±5)or(41±2±6)eV.We also search for the production of X(1750)→ηϕ,and the significance is only 2.0σ.We then determine the upper limit ofΓ_(X(1750))^(e+e−)⋅B[X(1750)→ηϕ]at the 90%confidence level.展开更多
The neutron-induced total cross-section of ^(209)Bi is crucial for the physical design and safety assessment of lead-based fast reactors, and the quality of experimental data should be improved for evaluation and appl...The neutron-induced total cross-section of ^(209)Bi is crucial for the physical design and safety assessment of lead-based fast reactors, and the quality of experimental data should be improved for evaluation and application.A recent experiment was conducted on the back-streaming white neutron beamline(Back-n) at the China Spallation Neutron Source(CSNS) using the neutron total cross-section spectrometer(NTOX). The neutron energy was determined using a fast multi-cell fission chamber and the time-of-flight technique. Two high-purity bismuth samples,6 mm and 20 mm in thickness, were chosen for neutron transmission measurements and comparisons. The neutron total cross-sections of ^(209)Bi, ranging from 0.3 e V to 20 Me V, were derived considering neutron flight time determination, flight path calibration, and background subtraction. A comparison of the experimental results with the data in the ENDF/B-VⅢ.0 library showed fair agreement, and the point-wise cross-sections were found to be consistent with existing experimental data. Special attention was given to the determination of resonance parameters, which were analyzed using the R-matrix code SAMMY and Bayesian method in the 0.5 ke V to 20 ke V energy range. The extracted resonance parameters were compared to previously reported results and evaluated data. This study is recognized as the first one where the neutron total cross-section of bismuth across such a broad energy spectrum is measured in a single measurement or experiment, and it provides valuable data for the assessment of related reaction information for evaluated libraries and the advancement of lead-bismuth-based nuclear systems.展开更多
According to the new K^＊（892）^0 and K^＊（892）^- masses reported by the BELLE experiment and the K^＊（892）^0 mass reported by the FOCUS experiment, mass splitting between neutral and charged K^＊（892） becomes ...According to the new K^＊（892）^0 and K^＊（892）^- masses reported by the BELLE experiment and the K^＊（892）^0 mass reported by the FOCUS experiment, mass splitting between neutral and charged K^＊（892） becomes very small. This is significantly different from the current world average values given by the Particle Data Group 2008. We find that there are differences between models used to fit the K^＊（892） decay invariant mass spectra in different measurements and study the model dependence in the measurement of K^＊（892） parameters. We refit the K^＊（892）^0 mass spectra of the BELLE and FOCUS experiments with the formula used by BELLE in fitting K^＊（892）^- to get new mass and width. After refitting, the K^＊（892）^0 mass of the BELLE experiment becomes 1.4 MeV/c^2 larger than the initial value and that of the FOCUS experiment is 1 MeV/c^2 smaller than the initial value. We also fit the spectra of some other experiments to extract the K^＊ （892） parameters using the BELLE K^＊ （892）^- parametrization.展开更多
We have theoretically investigated two series of cyclometalated Pt（II） complexes, a series [Pt （C, N, N） Cl] and b series [Pt （C, N, Npyrazolyl） Cl]. The geometrical and electronic structures are calculated at t...We have theoretically investigated two series of cyclometalated Pt（II） complexes, a series [Pt （C, N, N） Cl] and b series [Pt （C, N, Npyrazolyl） Cl]. The geometrical and electronic structures are calculated at the ECP60MWB//6-31G＊（H, C, Cl, N, S） basis set level using DFT method; one-photon absorption （OPA） properties are calculated by using both TDDFT and ZINDO methods and two-photon absorption （TPA） properties are obtained with the ZINDO/SOS method. The resonance integrals parameters （βsp and βd） for Pt are adjusted to -1 and -28.5 eV, respectively, to make max OPA wavelength calculated by ZINDO closest to the experimental data and TDDFT results. The calculated results indicate the molecule 2b （[Pt （Cnaphthyl, N, Npyrazolyl） Cl]） has the biggest potential as outstanding TPA materials because （i） the TPA properties of b series are more outstanding in IR wavelength range, the molecules in b series have good transparencies and possess 1-pyrazolyl-NH that is also available for another metal coordination （e.g., dimerization） and chemical interactions; （ii） when C is CnaphthyI in the C, N, N ligand of cyclometalated Pt（II） complexes, the molecules have the best conjugation effect and the best TPA properties.展开更多
基金supported by the Natural Science Foundation of Hunan Province,China(No.2025JJ60020)the National Key Research and Development Program(No.2022YFA1603300)+1 种基金National Natural Science Foundation of China(Nos.12275338 and 12388102)China Institute of Atomic Energy(No.CIAE-FWGKJT-23-0820).
文摘^(147,149)Sm are slow neutron capture(s-process)nuclides in nuclear astrophysics,whose(n,γ)cross sections are important input parameters in nucleosynthesis network calculations in the samarium(Sm)region.In addition,^(149)Sm is a fission product of ^(235)U with a 1%yield,and its neutron resonance parameters play a critical role in reactor neutronics.According to the available nuclear evaluation databases,a significant disagreement has been observed in the resonance peaks of the ^(147,149)Sm(n,γ)crosssectional data within the energy range of 20-300 eV.In this study,tutron capture cross section of a natural samarium target was measured at the back-streaming white neutron beamline of the China Spallation Neutron Source.The neutron capture yield was obtained,and the neutron resonance parameters for ^(147)Sm at 107.0,139.4,241.7,and 257.3 eV and ^(149)Sm at 23.2,24.6,26.1,28.0,51.5,75.2,90.9,125.3,and 248.4 eV were extracted using the SAMMY code based on R-matrix theory.For the parameters Γ_(n) and Γ_(γ) in these energies of ^(147,149)Sm,the percentages consistent with the results of the CENDL-3.2,ENDF/B-Ⅷ.0,JEFF-3.3,JENDL-4.0,and BROND-3.1 database are 27%,65%,65%,42%,and 58%,respectively.However,27% of the results were inconsistent with those of the major libraries.This work enriches experimental data of the ^(147,149)Sm neutron capture resonance and helps clarify the differences between different evaluation databases at the above energies.
基金Supported in part by National Key R&D Program of China(2020YFA0406300,2020YFA0406400,2023YFA1606000)National Natural Science Foundation of China(NSFC)(11635010,11735014,11935015,11935016,11935018,12025502,12035009,12035013,12061131003,12192260,12192261,12192262,12192263,12192264,12192265,12221005,12225509,12235017,12361141819)+17 种基金the Chinese Academy of Sciences(CAS)Large-Scale Scientific Facility Programthe CAS Center for Excellence in Particle Physics(CCEPP)Joint Large-Scale Scientific Facility Funds of the NSFC and CAS(U1832207)100 Talents Program of CAS(ZR2022JQ02,ZR2024QA151)supported by Shandong Provincial Natural Science Foundationsupported by the China Postdoctoral Science Foundation(2023M742100)The Institute of Nuclear and Particle Physics(INPAC)and Shanghai Key Laboratory for Particle Physics and CosmologyGerman Research Foundation DFG(FOR5327,GRK 2149)Istituto Nazionale di Fisica Nucleare,ItalyKnut and Alice Wallenberg Foundation(2021.0174,2021.0299)Ministry of Development of Turkey(DPT2006K-120470)National Research Foundation of Korea(NRF-2022R1A2C1092335)National Science and Technology fund of MongoliaNational Science Research and Innovation Fund(NSRF)via the Program Management Unit for Human Resources&Institutional Development,Research and Innovation of Thailand(B16F640076,B50G670107)Polish National Science Centre(2019/35/O/ST2/02907)Swedish Research Council(2019.04595)The Swedish Foundation for International Cooperation in Research and Higher Education(CH2018-7756)U.S.Department of Energy(DE-FG02-05ER41374)。
文摘By analyzing ψ(3686) data sample containing (107.7±0.6)×10^(6) events taken with the BESIII detector at the BEPCII storage ring in 2009,the χ_(c 0) resonance parameters are precisely measured using χ_(c 0,c 2)→π^(+)π^(−)/K^(+)K^(−) events.The mass of χ_(c 0) is determined to be M (χ_(c 0))=(3415.63±0.07±0.07±0.07)MeV/c^(2),and its full width is F (χ_(c 0))=(12.52±0.12±0.13)MeV,where the first uncertainty is statistical,the second systematic,and the third for mass comes from χ_(c 2) mass uncertainty.These measurements improve the precision of χ_(c 0) mass by a factor of four and width by one order of magnitude over the previous individual measurements,and significantly boost our knowledge about the charmonium spectrum.Together with additional (345.4±2.6)×10^(6)(3686) data events taken in 2012,the decay branching fractions of χ_(c 0,c 2)→π^(+)π^(−)/K^(+)K^(−) are measured as well,with precision improved by a factor of three compared to previous measurements.These χ_(c 0) decay branching fractions provide important inputs for the study of glueballs.
基金the staff of the Pohang Accelerator Laboratory for the excellent operation of the electron linac and their strong support
文摘The neutron total cross-sections of thulium （^169Tm） were measured in the neutron energy region from 0.01 eV to 100 eV by using the time-of-flight method at the Pohang Neutron Facility, which consists of an electron linac, a water-cooled tantalum target with a water moderator, and a 12 m time of flight path, Two thulium plates with different thicknesses were used for the neutron transmission measurement. The background level was determined by using a notch-filter of Co, In, and Cd sheets. The present measurement was compared with the previous ones, and a new set of resonance parameters of ^169Tm isotope was obtained from the transmission rate by using the SAMMY code, with a comparison with the recommended parameters by Mughabghab.
基金supported by the National Natural Science Foundation of China(Nos.12365018,U2032146,12465024)Natural Science Foundation of Inner Mongolia(Nos.2023MS01005,2024ZD23,2024FX30)the program of Innovative Research Team and Young Talents of Science and Technology in Universities of Inner Mongolia Autonomous Region(Nos.NMGIRT2217,NJYT23109)。
文摘The neutron capture resonance parameters for 159Tb are crucial for validating nuclear models,nucleosynthesis during the neutron capture process,and nuclear technology applications.In this study,resonance analyses were performed for the neutron capture cross sections of 159Tb measured at the China Spallation Neutron Source(CSNS)backscattering white neutron beamline(Back-n)facility.The resonance parameters were extracted from the R-Matrix code SAMMY and fitted to the experimental capture yield up to the 1.2 keV resolved resonance region(RRR).The average resonance parameters were determined by performing statistical analysis on the set of the resonance parameters in the RRR.These results were used to fit the measured average capture cross sections using the FITACS code in the unresolved resonance region from 2 keV to 1 MeV.The contributions of partial waves l=0,1,2 to the average capture cross sections are reported.
基金The Knowledge Innovation Project of Chinese Academy of Sciences (KZCX2-YW-133)National Natural Science Foundation of China (40574034 and 40730316).
文摘The Earth＇s free core nutation （FCN） is a retrograde eigenrnode which is attributed to the interaction between the solid mantle and the liquid core of the rotational elliptical Earth. This mode appears as an eigenmode of nearly diurnal free wobble （NDFW） in a terrestrial reference frame with a period of about one day （XU et al, 2001）. Therefore, the NDFW will lead to an obvious resonance enhancement in the diurnal tidal gravity observations, especially those of the tidal waves with frequencies closed to its eigenfrequency such as P1, K1, ψ1 and Ф1. The FCN resonance parameters can be retrieved accurately by high-precision tidal gravity observations, especially those recorded with the superconducting gravimeters （SG）. The Global Geodynamics Project （GGP） organized by IUGG took it as an important content for determining the FCN resonance parameters by using gravity data. However, the results are affected by many factors such as station location, background noise, the selection of the tide-generating potential tables, ocean tide models, data processing techniques and so on. In our study, the FCN parameters will be retrieved by using the SG observations at Wuhan, and the effects of the choices of various tide-generating potential tables, oceanic models and weight functions on the estimation of the FCN parameters will be discussed in detail,
文摘The purpose of this study was to investigate the nuclear magnetic resonance （NMR） assignments of hydrolyzed products extracted from human blood plasma. The correlations between chemical, functional and structural prop- erties of highly toxic pesticides were investigated using the PreADME analysis. We observed that toxic pesticides possessed higher molecular weight and, more hydrogen bond donors and acceptors when compared with less toxic pesticides. The occurrence of functional groups and structural properties was analyzed using ~H-NMR. The ~H- NMR spectra of the phosphomethoxy class of pesticides were characterized by methyl resonances at 3.7-3.9 ppm （8） with the coupling constants of 11-16 Hz （Je-cns）. In phosphoethoxy pesticides, the methyl resonance was about 1.4 ppm （8） with the coupling constant of 10 Hz （Je-cH2） and the methylene resonances was 4.2-4.4 ppm （8） with the coupling constant of 0.8 Hz （Jp-cH3）, respectively. Our study shows that the values of four parameters such as chemical shift, coupling constant, integration and relaxation time correlated with the concentration of toxic pesticides, and can be used to characterise the proton groups in the molecular structures of toxic pesticides.
基金Supported by the National Key R&D Program of China(2022YFA1601903)the National Natural Science Foundation of China(12175041)。
文摘We determine the resonant parameters of the vector statesϕ(1680)andϕ(2170)by performing a combined fit to the e+e−→ηϕcross sections from the threshold to 2.85GeV measured by the BaBar,Belle,BESIII,and CMD-3 experiments.The mass(1678_(−3)^(+5)±7)MeV/c^(2) and width(156±5±9)MeV are obtained forϕ(1680),and the mass(2169±5±6)MeV/c^(2) and width(96_(−14)^(+17)±9)MeV are obtained forϕ(2170).The statistical significance ofϕ(2170)is 7.2σ.Depending on the interference betweenϕ(1680),ϕ(2170),and a non-resonantηϕamplitude in the nominal fit,we obtain four solutions andΓe+e−ϕ(1680)⋅B[ϕ(1680)→ηϕ]=(79±4±16),(127±5±12),(65_(−4)^(+5)±13)or(215_(−5)^(+8)±11)eV,andΓ_(ϕ(2170))^(e+e−)⋅B[ϕ(2170)→ηϕ]=(0.56_(−0.02)^(+0.03)±0.07),(0.36_(−0.03)^(+0.05)±0.07),(38±1±5)or(41±2±6)eV.We also search for the production of X(1750)→ηϕ,and the significance is only 2.0σ.We then determine the upper limit ofΓ_(X(1750))^(e+e−)⋅B[X(1750)→ηϕ]at the 90%confidence level.
基金the National Natural Science Foundation of China(12375296)the Key Laboratory of Nuclear Data Foundation(JCKY2022201C153)+1 种基金the National Key Research and Development Plan(2022YFA1603303)the Natural Science Foundation of Hunan Province of China(2021JJ40444,2020RC3054)。
文摘The neutron-induced total cross-section of ^(209)Bi is crucial for the physical design and safety assessment of lead-based fast reactors, and the quality of experimental data should be improved for evaluation and application.A recent experiment was conducted on the back-streaming white neutron beamline(Back-n) at the China Spallation Neutron Source(CSNS) using the neutron total cross-section spectrometer(NTOX). The neutron energy was determined using a fast multi-cell fission chamber and the time-of-flight technique. Two high-purity bismuth samples,6 mm and 20 mm in thickness, were chosen for neutron transmission measurements and comparisons. The neutron total cross-sections of ^(209)Bi, ranging from 0.3 e V to 20 Me V, were derived considering neutron flight time determination, flight path calibration, and background subtraction. A comparison of the experimental results with the data in the ENDF/B-VⅢ.0 library showed fair agreement, and the point-wise cross-sections were found to be consistent with existing experimental data. Special attention was given to the determination of resonance parameters, which were analyzed using the R-matrix code SAMMY and Bayesian method in the 0.5 ke V to 20 ke V energy range. The extracted resonance parameters were compared to previously reported results and evaluated data. This study is recognized as the first one where the neutron total cross-section of bismuth across such a broad energy spectrum is measured in a single measurement or experiment, and it provides valuable data for the assessment of related reaction information for evaluated libraries and the advancement of lead-bismuth-based nuclear systems.
基金National Natural Science Foundation of China (10491303, 10825524)100 Talents Program of CAS (U-25)
文摘According to the new K^＊（892）^0 and K^＊（892）^- masses reported by the BELLE experiment and the K^＊（892）^0 mass reported by the FOCUS experiment, mass splitting between neutral and charged K^＊（892） becomes very small. This is significantly different from the current world average values given by the Particle Data Group 2008. We find that there are differences between models used to fit the K^＊（892） decay invariant mass spectra in different measurements and study the model dependence in the measurement of K^＊（892） parameters. We refit the K^＊（892）^0 mass spectra of the BELLE and FOCUS experiments with the formula used by BELLE in fitting K^＊（892）^- to get new mass and width. After refitting, the K^＊（892）^0 mass of the BELLE experiment becomes 1.4 MeV/c^2 larger than the initial value and that of the FOCUS experiment is 1 MeV/c^2 smaller than the initial value. We also fit the spectra of some other experiments to extract the K^＊ （892） parameters using the BELLE K^＊ （892）^- parametrization.
基金supported by the Youth Scholar Backbone Supporting Plan Project for General Universities of Heilongjiang Province (1155G22)China Postdoctoral Science Foundation (20100481018)+2 种基金Heilongjiang Postdoctoral Financial Assistance (LBH-Z09096)Youth Science Foundation of Harbin University of Science and Technology (2009YF020)National Natural Science Foundation of China (20973078)
文摘We have theoretically investigated two series of cyclometalated Pt（II） complexes, a series [Pt （C, N, N） Cl] and b series [Pt （C, N, Npyrazolyl） Cl]. The geometrical and electronic structures are calculated at the ECP60MWB//6-31G＊（H, C, Cl, N, S） basis set level using DFT method; one-photon absorption （OPA） properties are calculated by using both TDDFT and ZINDO methods and two-photon absorption （TPA） properties are obtained with the ZINDO/SOS method. The resonance integrals parameters （βsp and βd） for Pt are adjusted to -1 and -28.5 eV, respectively, to make max OPA wavelength calculated by ZINDO closest to the experimental data and TDDFT results. The calculated results indicate the molecule 2b （[Pt （Cnaphthyl, N, Npyrazolyl） Cl]） has the biggest potential as outstanding TPA materials because （i） the TPA properties of b series are more outstanding in IR wavelength range, the molecules in b series have good transparencies and possess 1-pyrazolyl-NH that is also available for another metal coordination （e.g., dimerization） and chemical interactions; （ii） when C is CnaphthyI in the C, N, N ligand of cyclometalated Pt（II） complexes, the molecules have the best conjugation effect and the best TPA properties.
