The important applications of quantum dot system are to implement logic operations and achieve universal quantum computing based on different quantum nonlocalities.Here,we characterize the quantum steering,Bell nonloc...The important applications of quantum dot system are to implement logic operations and achieve universal quantum computing based on different quantum nonlocalities.Here,we characterize the quantum steering,Bell nonlocality,and nonlocal advantage of quantum coherence(NAQC)of quantum dot system suffering nonunital and unital channels.The results reveal that quantum steering,Bell nonlocality,and NAQC can display the traits of dissipation,enhancement,and freezing.One can achieve the detections of quantum steering,Bell nonlocality,and NAQC of quantum dot system in different situations.Among these quantum nonlocalities,NAQC is the most fragile,and it is most easily influenced by different system parameters.Furthermore,considering quantum dot system coupling with amplitude damping channel and phase damping channel,these quantum nonlocalities degenerate with the enlargement of the channel parameters t andΓ.Remarkably,measurement reversal can effectively control and enhance quantum steering,Bell nonlocality,and NAQC of quantum dot system suffering from decoherence,especially in the scenarios of the amplitude damping channel and strong operation strength.展开更多
In the present paper, we study the effect of van Hove singularities of conduction electron on the transport of a single quantum dot system in the Kondo regime. By using both the equation-of-motion and the noncrossing ...In the present paper, we study the effect of van Hove singularities of conduction electron on the transport of a single quantum dot system in the Kondo regime. By using both the equation-of-motion and the noncrossing approximation techniques, we show that the corrections caused by these singularities are actually minor. It can be explained by observing that the singularities in the equations, which determine the electronic DOS on the dot, are integrable. Furthermore, we find that, although each line width function is divergent at van Hove singular points, the total divergence is canceled out in the final formula to calculate the current through the system. Therefore, as far as the qualitative properties of the system is concerned, these singularities can be ignored and the wide-band approximation can be safely used in calculation.展开更多
In the present paper, we shall rigorously re-establish the result of the single-particle function of a quantum dot system at finite temperature. Unlike the proof given in our previous work （Phys. Rev. B 74 195414 （2...In the present paper, we shall rigorously re-establish the result of the single-particle function of a quantum dot system at finite temperature. Unlike the proof given in our previous work （Phys. Rev. B 74 195414 （2006））, we take a different approach, which does not exploit the explicit expression of the Gibbs distribution function. Instead, we only assume that the statistical distribution function of the quantum dot system is thermodynamically stable. As a result, we are able to show clearly that the electronic structure in the quantum dot system is completely determined by its thermodynamic stability. Furthermore, the weaker requirements on the statistical distribution function also make it possible to apply the same method to the quantum dot systems in non-equilibrium states.展开更多
A parallel-coupled double quantum dot （PCDQD） system with two multi-quantum dot chains is designed. Conductance versus Fermi energy level is investigated utilizing the non-equilibrium Green＇s function approach. If ...A parallel-coupled double quantum dot （PCDQD） system with two multi-quantum dot chains is designed. Conductance versus Fermi energy level is investigated utilizing the non-equilibrium Green＇s function approach. If two quantum dots are added on each side of the PCDQD system, additional Breit Wigner and Fano resonances occur in the conductance spectra. If quantum dots are added on one side of the system, small Fano resonances can be observed in the conductance spectra. Adjusting the number of side-coupled quantum dots, the anti-resonance bands emerge at different positions, which makes the system applicable as a quantum switching device. Moreover, the I-V characteristic curve presents the step characteristic and the width of the step decreases with increasing the number of side-coupled quantum dots.展开更多
We investigate entanglement transfer from two separate cavities to the excitons in two quantum dots separately placed in the two cavities. The cavity fields and the excitons are treated as two continuous-variable （CV...We investigate entanglement transfer from two separate cavities to the excitons in two quantum dots separately placed in the two cavities. The cavity fields and the excitons are treated as two continuous-variable （CV） subsystems. The time-dependent characteristic functions in the Wigner representation for the two subsystems are analytically obtained. Under the conditions that one of the two CV subsystems is initially prepared in a two-mode squeezed vacuum state and the other in its lowest energy state, we show that the entanglement reciprocation between the cavity fields and the excitons is realizable.展开更多
In this paper, we propose a scheme to realize quantum information transfer from a double quantum dot （DQD） system to a quantized cavity field. The DQD and the cavity field are treated as a two-state charge qubit and...In this paper, we propose a scheme to realize quantum information transfer from a double quantum dot （DQD） system to a quantized cavity field. The DQD and the cavity field are treated as a two-state charge qubit and a continuous-variable system, respectively. It is shown that quantum information encoded in the two-state DQD system can be transferred to quantum states of the cavity field with a continuous-variable basis through appropriate projective measurements with respect to the DQD.展开更多
Using the innovative method of the additional Bloch vector,the electron transfer properties of a double quantum dot(DQD) system measured by a quantum point contact(QPC) in a fluctuating environment are investigated.Th...Using the innovative method of the additional Bloch vector,the electron transfer properties of a double quantum dot(DQD) system measured by a quantum point contact(QPC) in a fluctuating environment are investigated.The results show that the environmental noises in transverse and longitudinal directions play different roles in the dynamical evolution of the open quantum systems.Considering the DQD with symmetric energy level,the Fano factor exhibits a slight peak with the increase of transverse noise amplitude σ_(T),which provides a basis for distinguishing dynamical phenomena caused by different directional fluctuation noises in symmetric DQD structures by studying the detector output.In the case of asymmetric DQD,the dependence of a detector current involving the level displacement is distinct when increasing the transverse noise damping coefficient τ_(T) and the longitudinal noise damping coefficient τ_(ε) respectively.Meanwhile,the transverse noise damping coefficient τ_(T) could significantly reduce the Fano factor and enhance the stability of the quantum system compared with the longitudinal one.The Fano factors with stable values as the enhancement of noise amplitudes show different external influences from the detector measurement,and provide a numerical reference for adjusting the noise amplitudes in both transverse and longitudinal directions appropriately in a microscopic experimental process to offset the decoherence effect caused by the measurements.Finally,the research of average waiting time provides unique insights to the development of single electron transfer theory in the short-time limit.展开更多
Using the nonequilibrium Keldysh Green＇s function technique, the Fano effect of a parallel-coupled triple Rashba quantum dot system is investigated. The conductance as a function of electron energy is numerically cal...Using the nonequilibrium Keldysh Green＇s function technique, the Fano effect of a parallel-coupled triple Rashba quantum dot system is investigated. The conductance as a function of electron energy is numerically calculated. Compared with the case of a parallel-coupled double quantum dot system, two additional Fano resonance peaks occur in the conductance spectrum. By adjusting the structural parameters, the two Fano resonance peaks may change into the resoaance peaks. In addition, the influence of Rashba spin-orbit interaction on the conductance is studied.展开更多
Using the nonequilibrium Green＇s function technique,electron transport through a laterally coupled vertical triple quantum dot is investigated.The conductance as a function of electron energy is numerically calculate...Using the nonequilibrium Green＇s function technique,electron transport through a laterally coupled vertical triple quantum dot is investigated.The conductance as a function of electron energy is numerically calculated.The evolution of the conductance strongly depends on the configuration of dot levels and interdot coupling strengths.展开更多
There are some disadvantages to Nikolopoulos et al.＇s protocol [Nikolopoulos G M, Petrosyan D and Lambropoulos P 2004 Europhys. Left. 65 297] where a quantum dot system is used to realize quantum communication. To ov...There are some disadvantages to Nikolopoulos et al.＇s protocol [Nikolopoulos G M, Petrosyan D and Lambropoulos P 2004 Europhys. Left. 65 297] where a quantum dot system is used to realize quantum communication. To overcome these disadvantages, we propose a protocol that uses a quantum dot array to construct a four-qubit spin chain to realize perfect quantum state transfer （PQST）. First, we calculate the interaction relation for PQST in the spin chain. Second, we review the interaction between the quantum dots in the Heitler-London approach. Third, we present a detailed program for designing the proper parameters of a quantum dot array to realize PQST.展开更多
The presence of anticrossings induced by coupling between two states causes curvature in energy levels, yielding a nonlinearity in the quantum system. When the system is driven back and forth along the bending energy ...The presence of anticrossings induced by coupling between two states causes curvature in energy levels, yielding a nonlinearity in the quantum system. When the system is driven back and forth along the bending energy levels, subharmonic transitions and energy shifts can be observed, which would cause a significant influence as the system is applied to quantum computing. In this paper, we study a longitudinally driven singlet-triplet(ST) system in a double quantum dot(DQD)system, and illustrate the consequences of nonlinearity by driving the system close to the anticrossings. We provide a straightforward theory to quantitatively describe the energy shift and subharmonics caused by nonlinearity, and find good agreement between our theoretical result and the numerical simulation. Our results reveal the existence of nonlinearity in the vicinity of anticrossings and provide a direct way of analytically assessing its impact, which can be applied to other quantum systems without excessive labor.展开更多
Nonequilibrium electronic transports through a system hosting three quantum dots hybridized with superconductors are investigated. By tuning the relative positions of the dot levels, we illustrate the existence of Maj...Nonequilibrium electronic transports through a system hosting three quantum dots hybridized with superconductors are investigated. By tuning the relative positions of the dot levels, we illustrate the existence of Majorana fermions and show that the Majorana feimions will either survive separately on single dots or distribute themselves among different dots with tunable probabilities. As a result, different physical mechanisms appear, including local Andreev reflection（LAR）,cross Andreev reflection（CAR）, and cross resonant tunneling（CRT）. The resulting characteristics may be used to reveal the unique properties of Majorana fermions. In addition, we discuss the spin-polarized transports and find a pure spin current and a spin filter effect due to the joint effect of CRT and CAR, which is important for designing spintronic devices.展开更多
Using Keldysh nonequilibrium Green function formalism and mapping a many-body electron-phonon interaction onto a one body problem, the electron transport through a serially coupled double quantum dot system is analyze...Using Keldysh nonequilibrium Green function formalism and mapping a many-body electron-phonon interaction onto a one body problem, the electron transport through a serially coupled double quantum dot system is analyzed. The influence of the electron-phonon interaction, temperature, detuning, and interdot tunneling on the transmission coefficient and current is studied. Our results show that the electron-phonon interaction results in the appearance of the side peaks in the transmission coefficient, whose height is strongly dependent on the phonon temperature. We have also found that the inequality of the electron-phonon interaction strength in two dots gives rise to an asymmetry in the current-voltage characteristic. In addition, the temperature difference between the phonon and electron subsystems results in the reduction of the saturated current and the destruction of the step-like behavior of the current. It is also observed that the detuning can improve the magnitude of the current by compensating the mismatch of the quantum dots energy levels induced by the electron-phonon interaction.展开更多
We study the electron transport through a special quantum-dot(QD)structure composed of three QDs and two Majorana bound states(MBSs)using the nonequilibrium Green’s function technique.This QD-MBS ring structure inclu...We study the electron transport through a special quantum-dot(QD)structure composed of three QDs and two Majorana bound states(MBSs)using the nonequilibrium Green’s function technique.This QD-MBS ring structure includes two channels with the two coupled MBSs being Channel 1 and one QD being Channel 2,and three types of transport processes such as the electron transmission(ET),the Andreev reflection(AR),and the crossed Andreev reflection(CAR).By comparing the ET,AR,and CAR processes through Channels 1 and 2,we make a systematic study on the transport properties of the QD-MBS ring.It is shown that there appear two kinds of characteristic transport patterns for Channels 1 and 2,as well as the interplay between the two patterns.Of particular interest is that there exists an AR-assisted ET process in Channel 2,which is different from that in Channel 1.Thus a clear"X"pattern due to the ET and AR processes appears in the ET,AR,and CAR transmission coefficients.Moreover,we study how Channel 2 affects the three transport processes when Channel 1 is tuned in the ET and CAR regimes.It is shown that the transport properties of the ET,AR and CAR processes can be adjusted by tuning the energy level of the QD embedded in Channel 2.We believe this research should be a helpful reference for understanding the transport properties in the QD-MBS coupled systems.展开更多
Quantum dot(QD)-based fluorescent inks offer high potential due to their tunable emission and high quantum yield,but their practical application suffers from poor environmental stability,aggregation,and challenges in ...Quantum dot(QD)-based fluorescent inks offer high potential due to their tunable emission and high quantum yield,but their practical application suffers from poor environmental stability,aggregation,and challenges in scalable flexible fabrication.In this study,a high-stability fluorescent ink was developed by incorporating QDs into a polydimethylsiloxane(PDMS)colloidal matrix.High-performance patterned films were then obtained via systematic optimization of screen-printing parameters,with film quality governed by substrate type(131μm PDMS),QD concentration(1.5 mg/mL),and screen mesh count(420 mesh).The optimized films exhibit outstanding environmental and photostability,retaining 75.6% of their fluorescence intensity after immersion in deionized water and 63.8% in 75%ethanol at 25℃ for 100 minutes.Under UV irradiation(365 nm,9 W,100 min),fluorescence intensity decreases by less than 20%.Utilizing their daylight transparency and UV-excitable luminescence,various patterns including QR codes and Code 93 standard barcodes were fabricated via screen printing with high pattern fidelity and machine readability.This study presents a scalable and reliable strategy for the fabrication of flexible,high-stability fluorescent films,supporting their integration into next-generation optoelectronic devices,advanced displays,and secure anti-counterfeiting.展开更多
Near-infrared image sensors are widely used in fields such as material identification,machine vision,and autonomous driving.Lead sulfide colloidal quantum dot-based infrared photodiodes can be integrated with sil⁃icon...Near-infrared image sensors are widely used in fields such as material identification,machine vision,and autonomous driving.Lead sulfide colloidal quantum dot-based infrared photodiodes can be integrated with sil⁃icon-based readout circuits in a single step.Based on this,we propose a photodiode based on an n-i-p structure,which removes the buffer layer and further simplifies the manufacturing process of quantum dot image sensors,thus reducing manufacturing costs.Additionally,for the noise complexity in quantum dot image sensors when capturing images,traditional denoising and non-uniformity methods often do not achieve optimal denoising re⁃sults.For the noise and stripe-type non-uniformity commonly encountered in infrared quantum dot detector imag⁃es,a network architecture has been developed that incorporates multiple key modules.This network combines channel attention and spatial attention mechanisms,dynamically adjusting the importance of feature maps to en⁃hance the ability to distinguish between noise and details.Meanwhile,the residual dense feature fusion module further improves the network's ability to process complex image structures through hierarchical feature extraction and fusion.Furthermore,the pyramid pooling module effectively captures information at different scales,improv⁃ing the network's multi-scale feature representation ability.Through the collaborative effect of these modules,the network can better handle various mixed noise and image non-uniformity issues.Experimental results show that it outperforms the traditional U-Net network in denoising and image correction tasks.展开更多
Developing on-demand biomass valorization represents an ideal path to alleviate the double burden of a sustainable energy-environment future,yet exploring tunable lignin-first chemistry to accomplish multifunctional w...Developing on-demand biomass valorization represents an ideal path to alleviate the double burden of a sustainable energy-environment future,yet exploring tunable lignin-first chemistry to accomplish multifunctional water purification remains elusive.Herein,we report a versatile solvent-fractionation to construct heteroatom-doped multicolor lignin carbon quantum dots(CQDs)with the functions of bimodal pollutant sensing,metal-ionic visualization,and photocatalytic antibiotic dissociation.With the aid of oxidation cleavage and biphasic extraction,the underlying lignin features of molecular weight and functional linkages influence the quantum size and core-surface state of CQDs conferring the unique optical-structure-performance.The N,S co-doped blue-emitting CQDs via light-quenching offer the selective identification of Fe^(3+)-ions in a broad response range with an acceptable limit of detection.The addition of L-cysteine can efficiently restore the fluorescence of CQDs by forming a stable Fe^(3+)-L-cys complex.The green-emissive CQDs are facilely embedded into cellulose hydrogel to directly visualize the presence of metal-ions.A red-CQDs modified ternary ZnIn2S4(ZIS)composite is fabricated to achieve photocatalytic antibiotic removal with an efficiency of~85%.The excellent photo-generated electron and storage capabilities of CQDs improve the light-capturing,electron conduction,and charge carrier separation of ZIS.The reactive species are of importance to photocatalytic tetracycline oxidation,wherein the electron holes(h+)function as the main contributor followed by∙O_(2)^(-),1O2 and∙OH.The directly interfacial electron escaping-shuttling with the help of optimized electronic and energy-band structures is confirmed via electrochemical test and theoretical computation.We anticipate that the present work not only sheds substantial light to manipulate polychromatic lignin-based CQDs via a tailored solvent-engineering,but also presents an emerging green route of emphasizing biomass-water nexus.展开更多
Quantum dot systems emerge as promising platforms for studying nanoscale thermoelectric effects and quantum fluctuation phenomena.In this work,we investigate the thermodynamic performance of a Coulomb-blockaded quantu...Quantum dot systems emerge as promising platforms for studying nanoscale thermoelectric effects and quantum fluctuation phenomena.In this work,we investigate the thermodynamic performance of a Coulomb-blockaded quantum dot operating as a quantum heat engine using the quantum master equation approach.By incorporating full counting statistics,we analyze both average transport properties and current fluctuations in this nanoscale system.We demonstrate that electron-electron interactions significantly enhance thermoelectric performance by increasing both the output power and energy conversion efficiency.Furthermore,we show that Coulomb interactions suppress current fluctuations while preserving the validity of the thermodynamic uncertainty relation.Our results provide important insights into the interplay between quantum effects and thermodynamic principles in nanoscale heat engines.展开更多
The development of quantum materials for single-photon emission is crucial for the advancement of quantum information technology.Although significant advancements have been witnessed in recent years for single-photon ...The development of quantum materials for single-photon emission is crucial for the advancement of quantum information technology.Although significant advancements have been witnessed in recent years for single-photon sources in the near-infrared band(λ∼700–1000 nm),several challenges have yet to be addressed for ideal single-photon emission at the telecommunication band.In this study,we present a droplet-epitaxy strategy for O-band to C-band single-photon source-based semiconductor quantum dots(QDs)using metal-organic vaporphase epitaxy(MOVPE).By investigating the growth conditions of the epitaxial process,we have successfully synthesized InAs/InP QDs with narrow emission lines spanning a broad spectral range of λ∼1200–1600 nm.The morphological and optical properties of the samples were characterized using atomic force microscopy and microphotoluminescence spectroscopy.The recorded single-photon purity of a plain QD structure reaches g^((2))(0)=0.16,with a radiative recombination lifetime as short as 1.5 ns.This work provides a crucial platform for future research on integrated microcavity enhancement techniques and coupled QDs with other quantum photonics in the telecom bands,offering significant prospects for quantum network applications.展开更多
Flexible materials with perovskite quantum dots(PQDs)are widely used in the field of photonics and opto-electronics due to their unique properties.Development of new materials based on these nanoparticles,incorporated...Flexible materials with perovskite quantum dots(PQDs)are widely used in the field of photonics and opto-electronics due to their unique properties.Development of new materials based on these nanoparticles,incorporated into flexible and lightweight nonwoven fabrics,demonstrated high photoconductivity and efficient light energy conversion.In this work,we propose a method for creating a stable luminescent nonwoven material using electrospinning,in which inorganic salt precursors are used without the need for additional stabilizers.Equimolar solutions of cesium and lead(Ⅱ)bromide were mixed with a fluoroplast,resulting in a series of samples.Luminescent materials were obtained containing PQDs with a composition of CsPbBr_(3),with emission peaks ranging from 507 to 517 nm under 365-nm excitation.We have experimentally established and theoretically confirmed that the peak position is related to the size of the particles formed in the fiber during electrospinning and depends on processing time.Developed materials exhibited stable luminescent properties for up to 2.5 years,making them a promising candidate for the development of new flexible optoelectronic devices based on PQDs.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant No.12175001)the Natural Science Research Key Project of the Education Department of Anhui Province,China(Grant Nos.KJ2021A0943 and KJ2020A0527)+4 种基金the University Synergy Innovation Program of Anhui Province,China(Grant No.GXXT-2021-026)the Anhui Provincial Natural Science Foundation,China(Grant Nos.2108085MA18 and 2008085MA20)the Key Project of Program for Excellent Young Talents of Anhui University,China(Grant No.gxyqZD2019042)the Open Project of Key Laboratory of Functional Materials and Devices for Informatics of Anhui Higher Education Institutes,China(Grant No.FMDI202106)the Research Start-up Funding Project of High Level Talent of West Anhui University,China(Grant No.WGKQ2021048).
文摘The important applications of quantum dot system are to implement logic operations and achieve universal quantum computing based on different quantum nonlocalities.Here,we characterize the quantum steering,Bell nonlocality,and nonlocal advantage of quantum coherence(NAQC)of quantum dot system suffering nonunital and unital channels.The results reveal that quantum steering,Bell nonlocality,and NAQC can display the traits of dissipation,enhancement,and freezing.One can achieve the detections of quantum steering,Bell nonlocality,and NAQC of quantum dot system in different situations.Among these quantum nonlocalities,NAQC is the most fragile,and it is most easily influenced by different system parameters.Furthermore,considering quantum dot system coupling with amplitude damping channel and phase damping channel,these quantum nonlocalities degenerate with the enlargement of the channel parameters t andΓ.Remarkably,measurement reversal can effectively control and enhance quantum steering,Bell nonlocality,and NAQC of quantum dot system suffering from decoherence,especially in the scenarios of the amplitude damping channel and strong operation strength.
文摘In the present paper, we study the effect of van Hove singularities of conduction electron on the transport of a single quantum dot system in the Kondo regime. By using both the equation-of-motion and the noncrossing approximation techniques, we show that the corrections caused by these singularities are actually minor. It can be explained by observing that the singularities in the equations, which determine the electronic DOS on the dot, are integrable. Furthermore, we find that, although each line width function is divergent at van Hove singular points, the total divergence is canceled out in the final formula to calculate the current through the system. Therefore, as far as the qualitative properties of the system is concerned, these singularities can be ignored and the wide-band approximation can be safely used in calculation.
基金Project supported by the National Science Foundation of China (Grant Nos. 10874003 and 11074004)the National Basic Research Program of China (Grant No. 2009CB939901)
文摘In the present paper, we shall rigorously re-establish the result of the single-particle function of a quantum dot system at finite temperature. Unlike the proof given in our previous work （Phys. Rev. B 74 195414 （2006））, we take a different approach, which does not exploit the explicit expression of the Gibbs distribution function. Instead, we only assume that the statistical distribution function of the quantum dot system is thermodynamically stable. As a result, we are able to show clearly that the electronic structure in the quantum dot system is completely determined by its thermodynamic stability. Furthermore, the weaker requirements on the statistical distribution function also make it possible to apply the same method to the quantum dot systems in non-equilibrium states.
基金Supported by the National Natural Science Foundation of China under Grant Nos 11447132 and 11504042the Chongqing Science and Technology Commission Project under Grant Nos cstc2014jcyj A00032 and cstc2016jcyj A1158the Scientific Research Project for Advanced Talents of Yangtze Normal University under Grant No 2017KYQD09
文摘A parallel-coupled double quantum dot （PCDQD） system with two multi-quantum dot chains is designed. Conductance versus Fermi energy level is investigated utilizing the non-equilibrium Green＇s function approach. If two quantum dots are added on each side of the PCDQD system, additional Breit Wigner and Fano resonances occur in the conductance spectra. If quantum dots are added on one side of the system, small Fano resonances can be observed in the conductance spectra. Adjusting the number of side-coupled quantum dots, the anti-resonance bands emerge at different positions, which makes the system applicable as a quantum switching device. Moreover, the I-V characteristic curve presents the step characteristic and the width of the step decreases with increasing the number of side-coupled quantum dots.
基金The project supported by National Natural Science Foundation of China under Grant Nos. 10374007 and 60472021
文摘We investigate entanglement transfer from two separate cavities to the excitons in two quantum dots separately placed in the two cavities. The cavity fields and the excitons are treated as two continuous-variable （CV） subsystems. The time-dependent characteristic functions in the Wigner representation for the two subsystems are analytically obtained. Under the conditions that one of the two CV subsystems is initially prepared in a two-mode squeezed vacuum state and the other in its lowest energy state, we show that the entanglement reciprocation between the cavity fields and the excitons is realizable.
基金Supported by the National Fundamental Research Program under Grant No.2007CB925204the National Natural Science Foundation of China under Grant Nos.10775048 and 10325523the Education Committee of Hunan Province under Grant No.08W012
文摘In this paper, we propose a scheme to realize quantum information transfer from a double quantum dot （DQD） system to a quantized cavity field. The DQD and the cavity field are treated as a two-state charge qubit and a continuous-variable system, respectively. It is shown that quantum information encoded in the two-state DQD system can be transferred to quantum states of the cavity field with a continuous-variable basis through appropriate projective measurements with respect to the DQD.
基金Project supported by the Natural Science Foundation of Shandong Province,China(Grant No.ZR2014AM030)。
文摘Using the innovative method of the additional Bloch vector,the electron transfer properties of a double quantum dot(DQD) system measured by a quantum point contact(QPC) in a fluctuating environment are investigated.The results show that the environmental noises in transverse and longitudinal directions play different roles in the dynamical evolution of the open quantum systems.Considering the DQD with symmetric energy level,the Fano factor exhibits a slight peak with the increase of transverse noise amplitude σ_(T),which provides a basis for distinguishing dynamical phenomena caused by different directional fluctuation noises in symmetric DQD structures by studying the detector output.In the case of asymmetric DQD,the dependence of a detector current involving the level displacement is distinct when increasing the transverse noise damping coefficient τ_(T) and the longitudinal noise damping coefficient τ_(ε) respectively.Meanwhile,the transverse noise damping coefficient τ_(T) could significantly reduce the Fano factor and enhance the stability of the quantum system compared with the longitudinal one.The Fano factors with stable values as the enhancement of noise amplitudes show different external influences from the detector measurement,and provide a numerical reference for adjusting the noise amplitudes in both transverse and longitudinal directions appropriately in a microscopic experimental process to offset the decoherence effect caused by the measurements.Finally,the research of average waiting time provides unique insights to the development of single electron transfer theory in the short-time limit.
基金supported by the Youth Foundation of Heilongjiang Province,China(Grant No.QC2009C41)the Heilongjiang Provincial Natural Science Foundation,China(Grant No.F200939)
文摘Using the nonequilibrium Keldysh Green＇s function technique, the Fano effect of a parallel-coupled triple Rashba quantum dot system is investigated. The conductance as a function of electron energy is numerically calculated. Compared with the case of a parallel-coupled double quantum dot system, two additional Fano resonance peaks occur in the conductance spectrum. By adjusting the structural parameters, the two Fano resonance peaks may change into the resoaance peaks. In addition, the influence of Rashba spin-orbit interaction on the conductance is studied.
基金Project supported by the Youth Foundation of Heilongjiang Province,China (Grant No. QC2009C41)the Heilongjiang Provincial Natural Science Foundation,China (Grant No. F200939)
文摘Using the nonequilibrium Green＇s function technique,electron transport through a laterally coupled vertical triple quantum dot is investigated.The conductance as a function of electron energy is numerically calculated.The evolution of the conductance strongly depends on the configuration of dot levels and interdot coupling strengths.
基金supported by the Natural Science Foundation of Shaanxi Province of China (Grant No. 2009JQ8006)
文摘There are some disadvantages to Nikolopoulos et al.＇s protocol [Nikolopoulos G M, Petrosyan D and Lambropoulos P 2004 Europhys. Left. 65 297] where a quantum dot system is used to realize quantum communication. To overcome these disadvantages, we propose a protocol that uses a quantum dot array to construct a four-qubit spin chain to realize perfect quantum state transfer （PQST）. First, we calculate the interaction relation for PQST in the spin chain. Second, we review the interaction between the quantum dots in the Heitler-London approach. Third, we present a detailed program for designing the proper parameters of a quantum dot array to realize PQST.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 12074368, 92165207, 12034018 and 92265113)the Anhui Province Natural Science Foundation (Grant No. 2108085J03)。
文摘The presence of anticrossings induced by coupling between two states causes curvature in energy levels, yielding a nonlinearity in the quantum system. When the system is driven back and forth along the bending energy levels, subharmonic transitions and energy shifts can be observed, which would cause a significant influence as the system is applied to quantum computing. In this paper, we study a longitudinally driven singlet-triplet(ST) system in a double quantum dot(DQD)system, and illustrate the consequences of nonlinearity by driving the system close to the anticrossings. We provide a straightforward theory to quantitatively describe the energy shift and subharmonics caused by nonlinearity, and find good agreement between our theoretical result and the numerical simulation. Our results reveal the existence of nonlinearity in the vicinity of anticrossings and provide a direct way of analytically assessing its impact, which can be applied to other quantum systems without excessive labor.
基金supported by the New Century Excellent Talents in University of China(Grant No.NCET-10-0090)the National Natural Science Foundation of China(Grant Nos.11474106,11174088,and 11274124)+1 种基金the Program for Changjiang Scholars and Innovative Research Team in University of China(Grant No.IRT1243)the Natural Science Foundation of Guangdong Province,China(Grant No.S2012010010681)
文摘Nonequilibrium electronic transports through a system hosting three quantum dots hybridized with superconductors are investigated. By tuning the relative positions of the dot levels, we illustrate the existence of Majorana fermions and show that the Majorana feimions will either survive separately on single dots or distribute themselves among different dots with tunable probabilities. As a result, different physical mechanisms appear, including local Andreev reflection（LAR）,cross Andreev reflection（CAR）, and cross resonant tunneling（CRT）. The resulting characteristics may be used to reveal the unique properties of Majorana fermions. In addition, we discuss the spin-polarized transports and find a pure spin current and a spin filter effect due to the joint effect of CRT and CAR, which is important for designing spintronic devices.
文摘Using Keldysh nonequilibrium Green function formalism and mapping a many-body electron-phonon interaction onto a one body problem, the electron transport through a serially coupled double quantum dot system is analyzed. The influence of the electron-phonon interaction, temperature, detuning, and interdot tunneling on the transmission coefficient and current is studied. Our results show that the electron-phonon interaction results in the appearance of the side peaks in the transmission coefficient, whose height is strongly dependent on the phonon temperature. We have also found that the inequality of the electron-phonon interaction strength in two dots gives rise to an asymmetry in the current-voltage characteristic. In addition, the temperature difference between the phonon and electron subsystems results in the reduction of the saturated current and the destruction of the step-like behavior of the current. It is also observed that the detuning can improve the magnitude of the current by compensating the mismatch of the quantum dots energy levels induced by the electron-phonon interaction.
基金Supported by National Natural Science Foundation of China under Grant No.11274040the Program for New Century Excellent Talents in University under Grant No.NCET-08-0044
文摘We study the electron transport through a special quantum-dot(QD)structure composed of three QDs and two Majorana bound states(MBSs)using the nonequilibrium Green’s function technique.This QD-MBS ring structure includes two channels with the two coupled MBSs being Channel 1 and one QD being Channel 2,and three types of transport processes such as the electron transmission(ET),the Andreev reflection(AR),and the crossed Andreev reflection(CAR).By comparing the ET,AR,and CAR processes through Channels 1 and 2,we make a systematic study on the transport properties of the QD-MBS ring.It is shown that there appear two kinds of characteristic transport patterns for Channels 1 and 2,as well as the interplay between the two patterns.Of particular interest is that there exists an AR-assisted ET process in Channel 2,which is different from that in Channel 1.Thus a clear"X"pattern due to the ET and AR processes appears in the ET,AR,and CAR transmission coefficients.Moreover,we study how Channel 2 affects the three transport processes when Channel 1 is tuned in the ET and CAR regimes.It is shown that the transport properties of the ET,AR and CAR processes can be adjusted by tuning the energy level of the QD embedded in Channel 2.We believe this research should be a helpful reference for understanding the transport properties in the QD-MBS coupled systems.
文摘Quantum dot(QD)-based fluorescent inks offer high potential due to their tunable emission and high quantum yield,but their practical application suffers from poor environmental stability,aggregation,and challenges in scalable flexible fabrication.In this study,a high-stability fluorescent ink was developed by incorporating QDs into a polydimethylsiloxane(PDMS)colloidal matrix.High-performance patterned films were then obtained via systematic optimization of screen-printing parameters,with film quality governed by substrate type(131μm PDMS),QD concentration(1.5 mg/mL),and screen mesh count(420 mesh).The optimized films exhibit outstanding environmental and photostability,retaining 75.6% of their fluorescence intensity after immersion in deionized water and 63.8% in 75%ethanol at 25℃ for 100 minutes.Under UV irradiation(365 nm,9 W,100 min),fluorescence intensity decreases by less than 20%.Utilizing their daylight transparency and UV-excitable luminescence,various patterns including QR codes and Code 93 standard barcodes were fabricated via screen printing with high pattern fidelity and machine readability.This study presents a scalable and reliable strategy for the fabrication of flexible,high-stability fluorescent films,supporting their integration into next-generation optoelectronic devices,advanced displays,and secure anti-counterfeiting.
基金Supported by the National key research and development program in the 14th five year plan 2021YFA1200700)the National Natural Science Foundation of China(62535018,62431025,62561160113)the Natural Science Foundation of Shanghai(23ZR1473400).
文摘Near-infrared image sensors are widely used in fields such as material identification,machine vision,and autonomous driving.Lead sulfide colloidal quantum dot-based infrared photodiodes can be integrated with sil⁃icon-based readout circuits in a single step.Based on this,we propose a photodiode based on an n-i-p structure,which removes the buffer layer and further simplifies the manufacturing process of quantum dot image sensors,thus reducing manufacturing costs.Additionally,for the noise complexity in quantum dot image sensors when capturing images,traditional denoising and non-uniformity methods often do not achieve optimal denoising re⁃sults.For the noise and stripe-type non-uniformity commonly encountered in infrared quantum dot detector imag⁃es,a network architecture has been developed that incorporates multiple key modules.This network combines channel attention and spatial attention mechanisms,dynamically adjusting the importance of feature maps to en⁃hance the ability to distinguish between noise and details.Meanwhile,the residual dense feature fusion module further improves the network's ability to process complex image structures through hierarchical feature extraction and fusion.Furthermore,the pyramid pooling module effectively captures information at different scales,improv⁃ing the network's multi-scale feature representation ability.Through the collaborative effect of these modules,the network can better handle various mixed noise and image non-uniformity issues.Experimental results show that it outperforms the traditional U-Net network in denoising and image correction tasks.
基金the National Natural Science Foundation of China(32171728 and 22008159)Wuhan Knowledge Innovation Project(2022020801020312).
文摘Developing on-demand biomass valorization represents an ideal path to alleviate the double burden of a sustainable energy-environment future,yet exploring tunable lignin-first chemistry to accomplish multifunctional water purification remains elusive.Herein,we report a versatile solvent-fractionation to construct heteroatom-doped multicolor lignin carbon quantum dots(CQDs)with the functions of bimodal pollutant sensing,metal-ionic visualization,and photocatalytic antibiotic dissociation.With the aid of oxidation cleavage and biphasic extraction,the underlying lignin features of molecular weight and functional linkages influence the quantum size and core-surface state of CQDs conferring the unique optical-structure-performance.The N,S co-doped blue-emitting CQDs via light-quenching offer the selective identification of Fe^(3+)-ions in a broad response range with an acceptable limit of detection.The addition of L-cysteine can efficiently restore the fluorescence of CQDs by forming a stable Fe^(3+)-L-cys complex.The green-emissive CQDs are facilely embedded into cellulose hydrogel to directly visualize the presence of metal-ions.A red-CQDs modified ternary ZnIn2S4(ZIS)composite is fabricated to achieve photocatalytic antibiotic removal with an efficiency of~85%.The excellent photo-generated electron and storage capabilities of CQDs improve the light-capturing,electron conduction,and charge carrier separation of ZIS.The reactive species are of importance to photocatalytic tetracycline oxidation,wherein the electron holes(h+)function as the main contributor followed by∙O_(2)^(-),1O2 and∙OH.The directly interfacial electron escaping-shuttling with the help of optimized electronic and energy-band structures is confirmed via electrochemical test and theoretical computation.We anticipate that the present work not only sheds substantial light to manipulate polychromatic lignin-based CQDs via a tailored solvent-engineering,but also presents an emerging green route of emphasizing biomass-water nexus.
基金supported by the National Natural Science Foundation of China(Grant No.12305050)the Natural Science Foundation of Jiangsu Higher Education Institutions of China(Grant No.23KJB140017)the Zhejiang Provincial Natural Science Foundation of China(Grant No.LZ25A050001)。
文摘Quantum dot systems emerge as promising platforms for studying nanoscale thermoelectric effects and quantum fluctuation phenomena.In this work,we investigate the thermodynamic performance of a Coulomb-blockaded quantum dot operating as a quantum heat engine using the quantum master equation approach.By incorporating full counting statistics,we analyze both average transport properties and current fluctuations in this nanoscale system.We demonstrate that electron-electron interactions significantly enhance thermoelectric performance by increasing both the output power and energy conversion efficiency.Furthermore,we show that Coulomb interactions suppress current fluctuations while preserving the validity of the thermodynamic uncertainty relation.Our results provide important insights into the interplay between quantum effects and thermodynamic principles in nanoscale heat engines.
基金supported by the National Natural Science Foundation of China (Grant Nos.12494604,12393834,12393831,62274014,6223501662335015)the National Key R&D Program of China (Grant No.2024YFA1208900)。
文摘The development of quantum materials for single-photon emission is crucial for the advancement of quantum information technology.Although significant advancements have been witnessed in recent years for single-photon sources in the near-infrared band(λ∼700–1000 nm),several challenges have yet to be addressed for ideal single-photon emission at the telecommunication band.In this study,we present a droplet-epitaxy strategy for O-band to C-band single-photon source-based semiconductor quantum dots(QDs)using metal-organic vaporphase epitaxy(MOVPE).By investigating the growth conditions of the epitaxial process,we have successfully synthesized InAs/InP QDs with narrow emission lines spanning a broad spectral range of λ∼1200–1600 nm.The morphological and optical properties of the samples were characterized using atomic force microscopy and microphotoluminescence spectroscopy.The recorded single-photon purity of a plain QD structure reaches g^((2))(0)=0.16,with a radiative recombination lifetime as short as 1.5 ns.This work provides a crucial platform for future research on integrated microcavity enhancement techniques and coupled QDs with other quantum photonics in the telecom bands,offering significant prospects for quantum network applications.
基金supported by the Russian Science Foundation grant number 24-23-00481,https://rscf.ru/project/24-2300481/.
文摘Flexible materials with perovskite quantum dots(PQDs)are widely used in the field of photonics and opto-electronics due to their unique properties.Development of new materials based on these nanoparticles,incorporated into flexible and lightweight nonwoven fabrics,demonstrated high photoconductivity and efficient light energy conversion.In this work,we propose a method for creating a stable luminescent nonwoven material using electrospinning,in which inorganic salt precursors are used without the need for additional stabilizers.Equimolar solutions of cesium and lead(Ⅱ)bromide were mixed with a fluoroplast,resulting in a series of samples.Luminescent materials were obtained containing PQDs with a composition of CsPbBr_(3),with emission peaks ranging from 507 to 517 nm under 365-nm excitation.We have experimentally established and theoretically confirmed that the peak position is related to the size of the particles formed in the fiber during electrospinning and depends on processing time.Developed materials exhibited stable luminescent properties for up to 2.5 years,making them a promising candidate for the development of new flexible optoelectronic devices based on PQDs.
