Glucose molecules are of great significance being one of the most important molecules in metabolic chain.However,due to the small Raman scattering cross-section and weak/non-adsorption on bare metals,accurately obtain...Glucose molecules are of great significance being one of the most important molecules in metabolic chain.However,due to the small Raman scattering cross-section and weak/non-adsorption on bare metals,accurately obtaining their"fingerprint information"remains a huge obstacle.Herein,we developed a tip-enhanced Raman scattering(TERS)technique to address this challenge.Adopting an optical fiber radial vector mode internally illuminates the plasmonic fiber tip to effectively suppress the background noise while generating a strong electric-field enhanced tip hotspot.Furthermore,the tip hotspot approaching the glucose molecules was manipulated via the shear-force feedback to provide more freedom for selecting substrates.Consequently,our TERS technique achieves the visualization of all Raman modes of glucose molecules within spectral window of 400-3200 cm^(-1),which is not achievable through the far-field/surface-enhanced Raman,or the existing TERS techniques.Our TERS technique offers a powerful tool for accurately identifying Raman scattering of molecules,paving the way for biomolecular analysis.展开更多
In this study,we developed a single-beam optical trap-based surface-enhanced Raman scattering(SERS)optofluidic molecular fingerprint spectroscopy detection system.This system utilizes a single-beam optical trap to con...In this study,we developed a single-beam optical trap-based surface-enhanced Raman scattering(SERS)optofluidic molecular fingerprint spectroscopy detection system.This system utilizes a single-beam optical trap to concentrate free silver nanoparticles(AgNPs)within an optofluidic chip,significantly enhancing SERS performance.We investigated the optical field distribution characteristics within the tapered fiber using COMSOL simulation software and established a MATLAB simulation model to validate the single-beam optical trap's effectiveness in capturing AgNPs,demonstrating the theoretical feasibility of our approach.To verify the particle capture efficacy of the system,we experimentally controlled the optical trap's on-off state to manage the capture and release of particles precisely.The experimental results indicated that the Raman signal intensity in the capture state was significantly higher than in the non-capture state,confirming that the single-beam optical trap effectively enhances the SERS detection capability of the optofluidic detection system.Furthermore,we employed Raman mapping techniques to investigate the impact of the capture area on the SERS effect,revealing that the spectral intensity of molecular fingerprints in the laser-trapping region is significantly improved.We successfully detected the Raman spectrum of crystal violet at a concentration of 10^(−9)mol/L and pesticide thiram at a concentration of 10^(−5)mol/L,further demonstrating the ability of the single-beam optical trap in enhancing the molecular fingerprint spectrum identification capability of the SERS optofluidic chips.The optical trapping SERS optofluidic detection system developed in this study,as a key component of an integrated optoelectronic sensing system,holds the potential for integration with portable high-power lasers and high-performance Raman spectrometers.This integration is expected to advance highly integrated technologies and significantly enhance the overall performance and portability of optoelectronic sensing systems.展开更多
Accurate satellite data assimilation under all-sky conditions requires enhanced parameterization of scattering properties for frozen hydrometeors in clouds.This study aims to develop a nonspherical scattering look-up ...Accurate satellite data assimilation under all-sky conditions requires enhanced parameterization of scattering properties for frozen hydrometeors in clouds.This study aims to develop a nonspherical scattering look-up table that contains the optical properties of five hydrometeor types—rain,cloud water,cloud ice,graupel,and snow—for the Advanced Radiative Transfer Modeling System(ARMS)at frequencies below 220 GHz.The discrete dipole approximation(DDA)method is employed to compute the single-scattering properties of solid cloud particles,modeling these particles as aggregated roughened bullet rosettes.The bulk optical properties of the cloud layer are derived by integrating the singlescattering properties with a modified Gamma size distribution,specifically for distributions with 18 effective radii.The bulk phase function is then projected onto a series of generalized spherical functions,applying the delta-M method for truncation.The results indicate that simulations using the newly developed nonspherical scattering look-up table exhibit significant consistency with observations under deep convection conditions.In contrast,assuming spherical solid cloud particles leads to excessive scattering at mid-frequency channels and insufficient scattering at high-frequency channels.This improvement in radiative transfer simulation accuracy for cloudy conditions will better support the assimilation of allsky microwave observations into numerical weather prediction models.·Frozen cloud particles were modeled as aggregates of bullet rosettes and the optical properties at microwave range were computed by DDA.·A complete process and technical details for constructing a look-up table of ARMS are provided.·The ARMS simulations generally show agreement with observations of MWTS and MWHS under typhoon conditions using the new look-up table.展开更多
Quantitative detection of trace small-sized nanoplastics(<100 nm)remains a significant challenge in surface-enhanced Raman scattering(SERS).To tackle this issue,we developed a hydrophobic CuO@Ag nanowire substrate ...Quantitative detection of trace small-sized nanoplastics(<100 nm)remains a significant challenge in surface-enhanced Raman scattering(SERS).To tackle this issue,we developed a hydrophobic CuO@Ag nanowire substrate and introduced a multiplex-feature analysis strategy based on the coffee ring effect.This substrate not only offers high Raman enhancement but also exhibits a high probability of detection(POD),enabling rapid and accurate identification of 50 nm polystyrene nanoplastics over a broad concentration range(1–10−10 wt%).Importantly,experimental results reveal a strong correlation between the coffee ring formation and the concentration of nanoplastic dispersion.By incorporating Raman signal intensity,coffee ring diameter,and POD as combined features,we established a machine learning-based mapping between nanoplastic concentration and coffee ring characteristics,allowing precise predictions of dispersion concentration.The mean squared error of these predictions is remarkably low,ranging from 0.21 to 0.54,representing a 19 fold improvement in accuracy compared to traditional linear regression-based methods.This strategy effectively integrates SERS with wettability modification techniques,ensuring high sensitivity and fingerprinting capabilities,while addressing the limitations of Raman signal intensity in accurately reflecting concentration changes at ultra-low levels,providing a new idea for precise SERS measurements of nanoplastics.展开更多
Gas targets have been used to measure the scattering length in neutron-proton(n-p)scattering experiments.Changes in electron dynamics within the gas target have a negligible effect on the dynamics of nucleons.However,...Gas targets have been used to measure the scattering length in neutron-proton(n-p)scattering experiments.Changes in electron dynamics within the gas target have a negligible effect on the dynamics of nucleons.However,electron dynamics are sensitively related to the specific form of the n-p interaction during the scattering process.We propose a theoretical approach to explore electron dynamics and determine the parameters of the n-p interaction.This approach is based on a three-body scattering process involving a neutron,a proton and an electron.Numerical results indicate significant differences in electron dynamics with varying values of n-p interaction parameters,providing additional information beyond scattering cross-sections to accurately determine these parameters.展开更多
The mechanisms of enhancing spin-orbit torque(SOT) have attracted significant attention, particularly regarding the influence of extrinsic scattering mechanisms on SOT efficiency, as they complement intrinsic contribu...The mechanisms of enhancing spin-orbit torque(SOT) have attracted significant attention, particularly regarding the influence of extrinsic scattering mechanisms on SOT efficiency, as they complement intrinsic contributions. In multilayer systems, extrinsic interfacial scattering, along with scattering from defects or impurities inside the materials, plays a crucial role in affecting the SOT efficiency. In this study, we successfully fabricated high-quality epitaxially grown [Ir/Pt]N superlattices with an increasing number of interfaces using a magnetron sputtering system to investigate the contribution of extrinsic interfacial scattering to SOT efficiency. We measured SOT efficiency through spin-torque ferromagnetic resonance methods and determined the spin Hall angle using the spin pumping technique. Additionally, we calculated spin transparency based on the SOT efficiency and spin Hall angle. Our findings indicate that the values of SOT efficiency, spin Hall angle, and spin transparency are enhanced in the superlattice structure compared to Pt, which we attribute to the increase in interfacial scattering.This research offers an effective strategy for designing and fabricating advanced spintronic devices.展开更多
To elucidate the fracturing mechanism of deep hard rock under complex disturbance environments,this study investigates the dynamic failure behavior of pre-damaged granite subjected to multi-source dynamic disturbances...To elucidate the fracturing mechanism of deep hard rock under complex disturbance environments,this study investigates the dynamic failure behavior of pre-damaged granite subjected to multi-source dynamic disturbances.Blasting vibration monitoring was conducted in a deep-buried drill-and-blast tunnel to characterize in-situ dynamic loading conditions.Subsequently,true triaxial compression tests incorporating multi-source disturbances were performed using a self-developed wide-low-frequency true triaxial system to simulate disturbance accumulation and damage evolution in granite.The results demonstrate that combined dynamic disturbances and unloading damage significantly accelerate strength degradation and trigger shear-slip failure along preferentially oriented blast-induced fractures,with strength reductions up to 16.7%.Layered failure was observed on the free surface of pre-damaged granite under biaxial loading,indicating a disturbance-induced fracture localization mechanism.Time-stress-fracture-energy coupling fields were constructed to reveal the spatiotemporal characteristics of fracture evolution.Critical precursor frequency bands(105-150,185-225,and 300-325 kHz)were identified,which serve as diagnostic signatures of impending failure.A dynamic instability mechanism driven by multi-source disturbance superposition and pre-damage evolution was established.Furthermore,a grouting-based wave-absorption control strategy was proposed to mitigate deep dynamic disasters by attenuating disturbance amplitude and reducing excitation frequency.展开更多
The SiO_(2) inverse opal photonic crystals(PC)with a three-dimensional macroporous structure were fabricated by the sacrificial template method,followed by infiltration of a pyrene derivative,1-(pyren-8-yl)but-3-en-1-...The SiO_(2) inverse opal photonic crystals(PC)with a three-dimensional macroporous structure were fabricated by the sacrificial template method,followed by infiltration of a pyrene derivative,1-(pyren-8-yl)but-3-en-1-amine(PEA),to achieve a formaldehyde(FA)-sensitive and fluorescence-enhanced sensing film.Utilizing the specific Aza-Cope rearrangement reaction of allylamine of PEA and FA to generate a strong fluorescent product emitted at approximately 480 nm,we chose a PC whose blue band edge of stopband overlapped with the fluorescence emission wavelength.In virtue of the fluorescence enhancement property derived from slow photon effect of PC,FA was detected highly selectively and sensitively.The limit of detection(LoD)was calculated to be 1.38 nmol/L.Furthermore,the fast detection of FA(within 1 min)is realized due to the interconnected three-dimensional macroporous structure of the inverse opal PC and its high specific surface area.The prepared sensing film can be used for the detection of FA in air,aquatic products and living cells.The very close FA content in indoor air to the result from FA detector,the recovery rate of 101.5%for detecting FA in aquatic products and fast fluorescence imaging in 2 min for living cells demonstrate the reliability and accuracy of our method in practical applications.展开更多
In the heterogeneous power internet of things(IoT)environment,data signals are acquired to support different business systems to realize advanced intelligent applications,with massive,multi-source,heterogeneous and ot...In the heterogeneous power internet of things(IoT)environment,data signals are acquired to support different business systems to realize advanced intelligent applications,with massive,multi-source,heterogeneous and other characteristics.Reliable perception of information and efficient transmission of energy in multi-source heterogeneous environments are crucial issues.Compressive sensing(CS),as an effective method of signal compression and transmission,can accurately recover the original signal only by very few sampling.In this paper,we study a new method of multi-source heterogeneous data signal reconstruction of power IoT based on compressive sensing technology.Based on the traditional compressive sensing technology to directly recover multi-source heterogeneous signals,we fully use the interference subspace information to design the measurement matrix,which directly and effectively eliminates the interference while making the measurement.The measure matrix is optimized by minimizing the average cross-coherence of the matrix,and the reconstruction performance of the new method is further improved.Finally,the effectiveness of the new method with different parameter settings under different multi-source heterogeneous data signal cases is verified by using orthogonal matching pursuit(OMP)and sparsity adaptive matching pursuit(SAMP)for considering the actual environment with prior information utilization of signal sparsity and no prior information utilization of signal sparsity.展开更多
Due to the development of cloud computing and machine learning,users can upload their data to the cloud for machine learning model training.However,dishonest clouds may infer user data,resulting in user data leakage.P...Due to the development of cloud computing and machine learning,users can upload their data to the cloud for machine learning model training.However,dishonest clouds may infer user data,resulting in user data leakage.Previous schemes have achieved secure outsourced computing,but they suffer from low computational accuracy,difficult-to-handle heterogeneous distribution of data from multiple sources,and high computational cost,which result in extremely poor user experience and expensive cloud computing costs.To address the above problems,we propose amulti-precision,multi-sourced,andmulti-key outsourcing neural network training scheme.Firstly,we design a multi-precision functional encryption computation based on Euclidean division.Second,we design the outsourcing model training algorithm based on a multi-precision functional encryption with multi-sourced heterogeneity.Finally,we conduct experiments on three datasets.The results indicate that our framework achieves an accuracy improvement of 6%to 30%.Additionally,it offers a memory space optimization of 1.0×2^(24) times compared to the previous best approach.展开更多
Accurate prediction of main-engine rotational speed(RPM)is pivotal for en-ergy-efficient ship operation and compliance with emerging carbon-intensity regulations.Existing approaches either rely on computationally inte...Accurate prediction of main-engine rotational speed(RPM)is pivotal for en-ergy-efficient ship operation and compliance with emerging carbon-intensity regulations.Existing approaches either rely on computationally intensive phys-ics-based models or data-driven methods that neglect hydrodynamic con-straints and suffer from label noise in mandatory reporting data.We propose a physics-informed LightGBM framework that fuses high-resolution AIS tra-jectories,meteorological re-analyses and EU MRV logs through a temporally anchored,multi-source alignment protocol.A dual LightGBM ensemble(L1/L2)predicts RPM under laden and ballast conditions.Validation on a Panamax tanker(366 days)yields−1.52 rpm(−3%)error;ballast accuracy surpasses laden by 1.7%.展开更多
This paper deeply discusses the causes of gear howling noise,the identification and analysis of multi-source excitation,the transmission path of dynamic noise,simulation and experimental research,case analysis,optimiz...This paper deeply discusses the causes of gear howling noise,the identification and analysis of multi-source excitation,the transmission path of dynamic noise,simulation and experimental research,case analysis,optimization effect,etc.,aiming to better provide a certain guideline and reference for relevant researchers.展开更多
The quasiparticle scattering processes of the topological surface state(TSS)in three-dimensional topological insulators(TIs)have a vital effect on the many-body interactions and potential applications of topological m...The quasiparticle scattering processes of the topological surface state(TSS)in three-dimensional topological insulators(TIs)have a vital effect on the many-body interactions and potential applications of topological materials.In this study,we performed high-resolution temperature-dependent angle-resolved photoemission spectroscopy analysis of the 3D strong TI Bi_(2)Se_(3).Using an ab initio simulation,we analyzed the temperature dependence of the electronic structure and lifetime broadening of the TSS,which are closely associated with the quasiparticle scattering process,i.e.,electron–phonon coupling and spin-dependent scattering.We show that,at a low temperature(7 K),the spin-dependent electron scattering facilitates the anisotropic scattering rate of the TSS.Conversely,at room temperature(300 K),the electron–phonon coupling dominates the contribution to the scattering rate.The scattering rate increases with temperature and becomes uniform in momentum space owing to the temperature dependence of quasiparticle scattering.The quantitative study of temperature-dependent scattering rates in TSS is crucial to understanding the topological property and transport mobility of Dirac fermions for fundamental studies and potential applications.展开更多
We present experimental results on kilojoule ultraviolet laser output with 1%spectral broadening.Through stimulated rotational Raman scattering(SRRS)with signal laser injection,we achieve effective spectral broadening...We present experimental results on kilojoule ultraviolet laser output with 1%spectral broadening.Through stimulated rotational Raman scattering(SRRS)with signal laser injection,we achieve effective spectral broadening in short-range propagation,with good retention of the original near-field distribution and time waveform.Theoretical calculations show that 2%bandwidth spectral broadening can be achieved by injecting 20 kW/cm^(2) signal light at 2.2 GW/cm^(2) flux of the pump laser.In addition,high-frequency modulation in the near field can be effectively avoided through replacement of the original random noise signal light by the controllable signal light.The SRRS in the atmospheric environment excited with signal laser injection can provide wide-band light output with controllable beam quality without long-distance propagation,representing an important potential route to realization of broadband laser drivers.展开更多
Extreme ultraviolet(EUV)lithography is crucial for advancing semiconductor manufacturing;however,current EUV light sources,such as laser-produced plasma(LPP),have significant limitations,including low energy-conversio...Extreme ultraviolet(EUV)lithography is crucial for advancing semiconductor manufacturing;however,current EUV light sources,such as laser-produced plasma(LPP),have significant limitations,including low energy-conversion efficiency and debris contamination.Various schemes,including optical free-electron laser undulators,have been studied to generate coherent EUV light.However,optical undulators suffer from limited focal lengths,which pose a significant challenge to achieving a higher gain.In this study,a novel approach is proposed that employs a stretched off-axis paraboloid(sOAP)mirror,thus extending the focus distance to the centimeter range while achieving a well-controlled periodic light field.This enables high-intensity 92-eV EUV sources to exceed 1016/s,as demonstrated in the simulations.The proposed setup provides an efficient and powerful solution for advanced applications including semiconductor lithography.展开更多
The study of collision between metastable positronium(Ps)and antihydrogen(H)is crucial for precision experiments involving H.In this paper,we investigate the elastic scattering between H and Ps(2s)by combining the con...The study of collision between metastable positronium(Ps)and antihydrogen(H)is crucial for precision experiments involving H.In this paper,we investigate the elastic scattering between H and Ps(2s)by combining the confined variational method with the projection method,for scattering energies from 0.0245 eV to 0.068 eV.Our calculations provide accurate phase shifts and cross sections for the 1,3S and 1,3P symmetries.Near the binding threshold,the rapid increase in the total cross section may be attributed to the P-wave resonance effect.Additionally,we determined the S-wave scattering lengths to be 9.34 a_(0)and 5.81 a_(0)for singlet and triplet elastic scattering,respectively.展开更多
In this paper,we present some properties of scattering data for the derivative nonlinear Schrödinger equation in H^(S)(R)(s≥1/2)starting from the Lax pair.We show that the reciprocal of the transmission coeffici...In this paper,we present some properties of scattering data for the derivative nonlinear Schrödinger equation in H^(S)(R)(s≥1/2)starting from the Lax pair.We show that the reciprocal of the transmission coefficient can be expressed as the sum of some iterative integrals,and its logarithm can be written as the sum of some connected iterative integrals.We provide the asymptotic properties of the first few iterative integrals of the reciprocal of the transmission coefficient.Moreover,we provide some regularity properties of the reciprocal of the transmission coefficient related to scattering data in H^(S)(R).展开更多
Multi-source data fusion provides high-precision spatial situational awareness essential for analyzing granular urban social activities.This study used Shanghai’s catering industry as a case study,leveraging electron...Multi-source data fusion provides high-precision spatial situational awareness essential for analyzing granular urban social activities.This study used Shanghai’s catering industry as a case study,leveraging electronic reviews and consumer data sourced from third-party restaurant platforms collected in 2021.By performing weighted processing on two-dimensional point-of-interest(POI)data,clustering hotspots of high-dimensional restaurant data were identified.A hierarchical network of restaurant hotspots was constructed following the Central Place Theory(CPT)framework,while the Geo-Informatic Tupu method was employed to resolve the challenges posed by network deformation in multi-scale processes.These findings suggest the necessity of enhancing the spatial balance of Shanghai’s urban centers by moderately increasing the number and service capacity of suburban centers at the urban periphery.Such measures would contribute to a more optimized urban structure and facilitate the outward dispersion of comfort-oriented facilities such as the restaurant industry.At a finer spatial scale,the distribution of restaurant hotspots demonstrates a polycentric and symmetric spatial pattern,with a developmental trend radiating outward along the city’s ring roads.This trend can be attributed to the efforts of restaurants to establish connections with other urban functional spaces,leading to the reconfiguration of urban spaces,expansion of restaurant-dedicated land use,and the reorganization of associated commercial activities.The results validate the existence of a polycentric urban structure in Shanghai but also highlight the instability of the restaurant hotspot network during cross-scale transitions.展开更多
Taking the Ming Tombs Forest Farm in Beijing as the research object,this research applied multi-source data fusion and GIS heat-map overlay analysis techniques,systematically collected bird observation point data from...Taking the Ming Tombs Forest Farm in Beijing as the research object,this research applied multi-source data fusion and GIS heat-map overlay analysis techniques,systematically collected bird observation point data from the Global Biodiversity Information Facility(GBIF),population distribution data from the Oak Ridge National Laboratory(ORNL)in the United States,as well as information on the composition of tree species in suitable forest areas for birds and the forest geographical information of the Ming Tombs Forest Farm,which is based on literature research and field investigations.By using GIS technology,spatial processing was carried out on bird observation points and population distribution data to identify suitable bird-watching areas in different seasons.Then,according to the suitability value range,these areas were classified into different grades(from unsuitable to highly suitable).The research findings indicated that there was significant spatial heterogeneity in the bird-watching suitability of the Ming Tombs Forest Farm.The north side of the reservoir was generally a core area with high suitability in all seasons.The deep-aged broad-leaved mixed forests supported the overlapping co-existence of the ecological niches of various bird species,such as the Zosterops simplex and Urocissa erythrorhyncha.In contrast,the shallow forest-edge coniferous pure forests and mixed forests were more suitable for specialized species like Carduelis sinica.The southern urban area and the core area of the mausoleums had relatively low suitability due to ecological fragmentation or human interference.Based on these results,this paper proposed a three-level protection framework of“core area conservation—buffer zone management—isolation zone construction”and a spatio-temporal coordinated human-bird co-existence strategy.It was also suggested that the human-bird co-existence space could be optimized through measures such as constructing sound and light buffer interfaces,restoring ecological corridors,and integrating cultural heritage elements.This research provided an operational technical approach and decision-making support for the scientific planning of bird-watching sites and the coordination of ecological protection and tourism development.展开更多
This study analytically examines the ionization of atoms in strong near-circular laser fields.The classic Keldysh-Rutherford(KR)Coulomb-scattering(CS)model[Phys.Rev.Lett.121123201(2018)]successfully explained the atto...This study analytically examines the ionization of atoms in strong near-circular laser fields.The classic Keldysh-Rutherford(KR)Coulomb-scattering(CS)model[Phys.Rev.Lett.121123201(2018)]successfully explained the attoclock experimental curve for the H atom at lower laser intensities.Here,we develop a semiclassical model that includes the initial conditions related to the quantum properties of tunneling in the KR model at the beginning of the scattering process.This model is able to explain recent attoclock experimental curves over a wider range of laser and atomic parameters.Our results show the importance of system symmetry and quantum effects in attoclock measurements,suggesting the complex role of the Coulomb potential in strong-field ionization.展开更多
基金supported by National Natural Science Foundation of China(12374358,91950207)Guangdong Basic and Applied Basic Research Foundation(2024A1515010420).
文摘Glucose molecules are of great significance being one of the most important molecules in metabolic chain.However,due to the small Raman scattering cross-section and weak/non-adsorption on bare metals,accurately obtaining their"fingerprint information"remains a huge obstacle.Herein,we developed a tip-enhanced Raman scattering(TERS)technique to address this challenge.Adopting an optical fiber radial vector mode internally illuminates the plasmonic fiber tip to effectively suppress the background noise while generating a strong electric-field enhanced tip hotspot.Furthermore,the tip hotspot approaching the glucose molecules was manipulated via the shear-force feedback to provide more freedom for selecting substrates.Consequently,our TERS technique achieves the visualization of all Raman modes of glucose molecules within spectral window of 400-3200 cm^(-1),which is not achievable through the far-field/surface-enhanced Raman,or the existing TERS techniques.Our TERS technique offers a powerful tool for accurately identifying Raman scattering of molecules,paving the way for biomolecular analysis.
基金financial supports from National Natural Science Foundation of China(62175023).
文摘In this study,we developed a single-beam optical trap-based surface-enhanced Raman scattering(SERS)optofluidic molecular fingerprint spectroscopy detection system.This system utilizes a single-beam optical trap to concentrate free silver nanoparticles(AgNPs)within an optofluidic chip,significantly enhancing SERS performance.We investigated the optical field distribution characteristics within the tapered fiber using COMSOL simulation software and established a MATLAB simulation model to validate the single-beam optical trap's effectiveness in capturing AgNPs,demonstrating the theoretical feasibility of our approach.To verify the particle capture efficacy of the system,we experimentally controlled the optical trap's on-off state to manage the capture and release of particles precisely.The experimental results indicated that the Raman signal intensity in the capture state was significantly higher than in the non-capture state,confirming that the single-beam optical trap effectively enhances the SERS detection capability of the optofluidic detection system.Furthermore,we employed Raman mapping techniques to investigate the impact of the capture area on the SERS effect,revealing that the spectral intensity of molecular fingerprints in the laser-trapping region is significantly improved.We successfully detected the Raman spectrum of crystal violet at a concentration of 10^(−9)mol/L and pesticide thiram at a concentration of 10^(−5)mol/L,further demonstrating the ability of the single-beam optical trap in enhancing the molecular fingerprint spectrum identification capability of the SERS optofluidic chips.The optical trapping SERS optofluidic detection system developed in this study,as a key component of an integrated optoelectronic sensing system,holds the potential for integration with portable high-power lasers and high-performance Raman spectrometers.This integration is expected to advance highly integrated technologies and significantly enhance the overall performance and portability of optoelectronic sensing systems.
基金supported by the National Key Research and Development Program of China(Grant No.2021YFB3900400)the National Natural Science Foundation of China(Grant Nos.U2142212 and 42361074)。
文摘Accurate satellite data assimilation under all-sky conditions requires enhanced parameterization of scattering properties for frozen hydrometeors in clouds.This study aims to develop a nonspherical scattering look-up table that contains the optical properties of five hydrometeor types—rain,cloud water,cloud ice,graupel,and snow—for the Advanced Radiative Transfer Modeling System(ARMS)at frequencies below 220 GHz.The discrete dipole approximation(DDA)method is employed to compute the single-scattering properties of solid cloud particles,modeling these particles as aggregated roughened bullet rosettes.The bulk optical properties of the cloud layer are derived by integrating the singlescattering properties with a modified Gamma size distribution,specifically for distributions with 18 effective radii.The bulk phase function is then projected onto a series of generalized spherical functions,applying the delta-M method for truncation.The results indicate that simulations using the newly developed nonspherical scattering look-up table exhibit significant consistency with observations under deep convection conditions.In contrast,assuming spherical solid cloud particles leads to excessive scattering at mid-frequency channels and insufficient scattering at high-frequency channels.This improvement in radiative transfer simulation accuracy for cloudy conditions will better support the assimilation of allsky microwave observations into numerical weather prediction models.·Frozen cloud particles were modeled as aggregates of bullet rosettes and the optical properties at microwave range were computed by DDA.·A complete process and technical details for constructing a look-up table of ARMS are provided.·The ARMS simulations generally show agreement with observations of MWTS and MWHS under typhoon conditions using the new look-up table.
基金the National Natural Science Foundation of China(No.12174229 and 22375117)Natural Science Foundation of Shandong Province(No.ZR2022YQ02 and ZR2023MB149)Taishan Scholars Program of Shandong Province(No.tsqn202306152)for financial support.
文摘Quantitative detection of trace small-sized nanoplastics(<100 nm)remains a significant challenge in surface-enhanced Raman scattering(SERS).To tackle this issue,we developed a hydrophobic CuO@Ag nanowire substrate and introduced a multiplex-feature analysis strategy based on the coffee ring effect.This substrate not only offers high Raman enhancement but also exhibits a high probability of detection(POD),enabling rapid and accurate identification of 50 nm polystyrene nanoplastics over a broad concentration range(1–10−10 wt%).Importantly,experimental results reveal a strong correlation between the coffee ring formation and the concentration of nanoplastic dispersion.By incorporating Raman signal intensity,coffee ring diameter,and POD as combined features,we established a machine learning-based mapping between nanoplastic concentration and coffee ring characteristics,allowing precise predictions of dispersion concentration.The mean squared error of these predictions is remarkably low,ranging from 0.21 to 0.54,representing a 19 fold improvement in accuracy compared to traditional linear regression-based methods.This strategy effectively integrates SERS with wettability modification techniques,ensuring high sensitivity and fingerprinting capabilities,while addressing the limitations of Raman signal intensity in accurately reflecting concentration changes at ultra-low levels,providing a new idea for precise SERS measurements of nanoplastics.
基金supported by the National Natural Science Foundation of China(Grant Nos.12088101 and No.U2330401)。
文摘Gas targets have been used to measure the scattering length in neutron-proton(n-p)scattering experiments.Changes in electron dynamics within the gas target have a negligible effect on the dynamics of nucleons.However,electron dynamics are sensitively related to the specific form of the n-p interaction during the scattering process.We propose a theoretical approach to explore electron dynamics and determine the parameters of the n-p interaction.This approach is based on a three-body scattering process involving a neutron,a proton and an electron.Numerical results indicate significant differences in electron dynamics with varying values of n-p interaction parameters,providing additional information beyond scattering cross-sections to accurately determine these parameters.
基金financially supported by the Science Center of the National Science Foundation of China (Grant No. 52088101)the National Natural Science Foundation of China (Grant Nos. 52161160334, 12274437, 12174426, and 52271237)+1 种基金the Chinese Academy of Sciences (CAS) Project for Young Scientists in Basic Research No. YSBR-084the CAS Youth Interdisciplinary Team。
文摘The mechanisms of enhancing spin-orbit torque(SOT) have attracted significant attention, particularly regarding the influence of extrinsic scattering mechanisms on SOT efficiency, as they complement intrinsic contributions. In multilayer systems, extrinsic interfacial scattering, along with scattering from defects or impurities inside the materials, plays a crucial role in affecting the SOT efficiency. In this study, we successfully fabricated high-quality epitaxially grown [Ir/Pt]N superlattices with an increasing number of interfaces using a magnetron sputtering system to investigate the contribution of extrinsic interfacial scattering to SOT efficiency. We measured SOT efficiency through spin-torque ferromagnetic resonance methods and determined the spin Hall angle using the spin pumping technique. Additionally, we calculated spin transparency based on the SOT efficiency and spin Hall angle. Our findings indicate that the values of SOT efficiency, spin Hall angle, and spin transparency are enhanced in the superlattice structure compared to Pt, which we attribute to the increase in interfacial scattering.This research offers an effective strategy for designing and fabricating advanced spintronic devices.
基金supported by the National Key R&D Program of China(No.2023YFB2603602)the National Natural Science Foundation of China(Nos.52222810 and 52178383).
文摘To elucidate the fracturing mechanism of deep hard rock under complex disturbance environments,this study investigates the dynamic failure behavior of pre-damaged granite subjected to multi-source dynamic disturbances.Blasting vibration monitoring was conducted in a deep-buried drill-and-blast tunnel to characterize in-situ dynamic loading conditions.Subsequently,true triaxial compression tests incorporating multi-source disturbances were performed using a self-developed wide-low-frequency true triaxial system to simulate disturbance accumulation and damage evolution in granite.The results demonstrate that combined dynamic disturbances and unloading damage significantly accelerate strength degradation and trigger shear-slip failure along preferentially oriented blast-induced fractures,with strength reductions up to 16.7%.Layered failure was observed on the free surface of pre-damaged granite under biaxial loading,indicating a disturbance-induced fracture localization mechanism.Time-stress-fracture-energy coupling fields were constructed to reveal the spatiotemporal characteristics of fracture evolution.Critical precursor frequency bands(105-150,185-225,and 300-325 kHz)were identified,which serve as diagnostic signatures of impending failure.A dynamic instability mechanism driven by multi-source disturbance superposition and pre-damage evolution was established.Furthermore,a grouting-based wave-absorption control strategy was proposed to mitigate deep dynamic disasters by attenuating disturbance amplitude and reducing excitation frequency.
基金supported by the National Natural Science Foundation of China(21663032 and 22061041)the Open Sharing Platform for Scientific and Technological Resources of Shaanxi Province(2021PT-004)the National Innovation and Entrepreneurship Training Program for College Students of China(S202110719044)。
文摘The SiO_(2) inverse opal photonic crystals(PC)with a three-dimensional macroporous structure were fabricated by the sacrificial template method,followed by infiltration of a pyrene derivative,1-(pyren-8-yl)but-3-en-1-amine(PEA),to achieve a formaldehyde(FA)-sensitive and fluorescence-enhanced sensing film.Utilizing the specific Aza-Cope rearrangement reaction of allylamine of PEA and FA to generate a strong fluorescent product emitted at approximately 480 nm,we chose a PC whose blue band edge of stopband overlapped with the fluorescence emission wavelength.In virtue of the fluorescence enhancement property derived from slow photon effect of PC,FA was detected highly selectively and sensitively.The limit of detection(LoD)was calculated to be 1.38 nmol/L.Furthermore,the fast detection of FA(within 1 min)is realized due to the interconnected three-dimensional macroporous structure of the inverse opal PC and its high specific surface area.The prepared sensing film can be used for the detection of FA in air,aquatic products and living cells.The very close FA content in indoor air to the result from FA detector,the recovery rate of 101.5%for detecting FA in aquatic products and fast fluorescence imaging in 2 min for living cells demonstrate the reliability and accuracy of our method in practical applications.
基金supported by National Natural Science Foundation of China(12174350)Science and Technology Project of State Grid Henan Electric Power Company(5217Q0240008).
文摘In the heterogeneous power internet of things(IoT)environment,data signals are acquired to support different business systems to realize advanced intelligent applications,with massive,multi-source,heterogeneous and other characteristics.Reliable perception of information and efficient transmission of energy in multi-source heterogeneous environments are crucial issues.Compressive sensing(CS),as an effective method of signal compression and transmission,can accurately recover the original signal only by very few sampling.In this paper,we study a new method of multi-source heterogeneous data signal reconstruction of power IoT based on compressive sensing technology.Based on the traditional compressive sensing technology to directly recover multi-source heterogeneous signals,we fully use the interference subspace information to design the measurement matrix,which directly and effectively eliminates the interference while making the measurement.The measure matrix is optimized by minimizing the average cross-coherence of the matrix,and the reconstruction performance of the new method is further improved.Finally,the effectiveness of the new method with different parameter settings under different multi-source heterogeneous data signal cases is verified by using orthogonal matching pursuit(OMP)and sparsity adaptive matching pursuit(SAMP)for considering the actual environment with prior information utilization of signal sparsity and no prior information utilization of signal sparsity.
基金supported by Natural Science Foundation of China(Nos.62303126,62362008,author Z.Z,https://www.nsfc.gov.cn/,accessed on 20 December 2024)Major Scientific and Technological Special Project of Guizhou Province([2024]014)+2 种基金Guizhou Provincial Science and Technology Projects(No.ZK[2022]General149) ,author Z.Z,https://kjt.guizhou.gov.cn/,accessed on 20 December 2024)The Open Project of the Key Laboratory of Computing Power Network and Information Security,Ministry of Education under Grant 2023ZD037,author Z.Z,https://www.gzu.edu.cn/,accessed on 20 December 2024)Open Research Project of the State Key Laboratory of Industrial Control Technology,Zhejiang University,China(No.ICT2024B25),author Z.Z,https://www.gzu.edu.cn/,accessed on 20 December 2024).
文摘Due to the development of cloud computing and machine learning,users can upload their data to the cloud for machine learning model training.However,dishonest clouds may infer user data,resulting in user data leakage.Previous schemes have achieved secure outsourced computing,but they suffer from low computational accuracy,difficult-to-handle heterogeneous distribution of data from multiple sources,and high computational cost,which result in extremely poor user experience and expensive cloud computing costs.To address the above problems,we propose amulti-precision,multi-sourced,andmulti-key outsourcing neural network training scheme.Firstly,we design a multi-precision functional encryption computation based on Euclidean division.Second,we design the outsourcing model training algorithm based on a multi-precision functional encryption with multi-sourced heterogeneity.Finally,we conduct experiments on three datasets.The results indicate that our framework achieves an accuracy improvement of 6%to 30%.Additionally,it offers a memory space optimization of 1.0×2^(24) times compared to the previous best approach.
基金support from the“Ocean-going Vessel Meteorological Navigation System”project funded under the Key Core Technology Breakthrough Program for Transportation Equipment(GJ-2025-01)COSCO Shipping Group’s Third Batch of Scientific Research Projects from the 14th Five-Year Plan.
文摘Accurate prediction of main-engine rotational speed(RPM)is pivotal for en-ergy-efficient ship operation and compliance with emerging carbon-intensity regulations.Existing approaches either rely on computationally intensive phys-ics-based models or data-driven methods that neglect hydrodynamic con-straints and suffer from label noise in mandatory reporting data.We propose a physics-informed LightGBM framework that fuses high-resolution AIS tra-jectories,meteorological re-analyses and EU MRV logs through a temporally anchored,multi-source alignment protocol.A dual LightGBM ensemble(L1/L2)predicts RPM under laden and ballast conditions.Validation on a Panamax tanker(366 days)yields−1.52 rpm(−3%)error;ballast accuracy surpasses laden by 1.7%.
文摘This paper deeply discusses the causes of gear howling noise,the identification and analysis of multi-source excitation,the transmission path of dynamic noise,simulation and experimental research,case analysis,optimization effect,etc.,aiming to better provide a certain guideline and reference for relevant researchers.
基金supported by the National Key R&D Program of China(Grant No.2022YFA1604301)the Natural Science Foundation of China(Grant Nos.12334013,12204018,9205020192250306)。
文摘The quasiparticle scattering processes of the topological surface state(TSS)in three-dimensional topological insulators(TIs)have a vital effect on the many-body interactions and potential applications of topological materials.In this study,we performed high-resolution temperature-dependent angle-resolved photoemission spectroscopy analysis of the 3D strong TI Bi_(2)Se_(3).Using an ab initio simulation,we analyzed the temperature dependence of the electronic structure and lifetime broadening of the TSS,which are closely associated with the quasiparticle scattering process,i.e.,electron–phonon coupling and spin-dependent scattering.We show that,at a low temperature(7 K),the spin-dependent electron scattering facilitates the anisotropic scattering rate of the TSS.Conversely,at room temperature(300 K),the electron–phonon coupling dominates the contribution to the scattering rate.The scattering rate increases with temperature and becomes uniform in momentum space owing to the temperature dependence of quasiparticle scattering.The quantitative study of temperature-dependent scattering rates in TSS is crucial to understanding the topological property and transport mobility of Dirac fermions for fundamental studies and potential applications.
基金supported by the Presidential Foundation of CAEP(Grant No.YZJJZL2023116)the National Nature Science Foundation of China(Grant No.12275249)the Youth Talent Fund of the Laser Fusion Research Center,CAEP(Grant Nos.RCFCZ7-2024-2 and RCFPD4-2020-4).
文摘We present experimental results on kilojoule ultraviolet laser output with 1%spectral broadening.Through stimulated rotational Raman scattering(SRRS)with signal laser injection,we achieve effective spectral broadening in short-range propagation,with good retention of the original near-field distribution and time waveform.Theoretical calculations show that 2%bandwidth spectral broadening can be achieved by injecting 20 kW/cm^(2) signal light at 2.2 GW/cm^(2) flux of the pump laser.In addition,high-frequency modulation in the near field can be effectively avoided through replacement of the original random noise signal light by the controllable signal light.The SRRS in the atmospheric environment excited with signal laser injection can provide wide-band light output with controllable beam quality without long-distance propagation,representing an important potential route to realization of broadband laser drivers.
基金supported in part by the National Key R&D Program of China(No.2023YFA1606900)the National Natural Science Foundation of China(NSFC)(Nos.12235003 and 12447106).
文摘Extreme ultraviolet(EUV)lithography is crucial for advancing semiconductor manufacturing;however,current EUV light sources,such as laser-produced plasma(LPP),have significant limitations,including low energy-conversion efficiency and debris contamination.Various schemes,including optical free-electron laser undulators,have been studied to generate coherent EUV light.However,optical undulators suffer from limited focal lengths,which pose a significant challenge to achieving a higher gain.In this study,a novel approach is proposed that employs a stretched off-axis paraboloid(sOAP)mirror,thus extending the focus distance to the centimeter range while achieving a well-controlled periodic light field.This enables high-intensity 92-eV EUV sources to exceed 1016/s,as demonstrated in the simulations.The proposed setup provides an efficient and powerful solution for advanced applications including semiconductor lithography.
基金supported by the National Natural Science Foundation of China under Grant Nos.12174399,12147146 and 11934014by the Natural Science Foundation of Hainan Province under Grant No.122QN219+1 种基金through the Innovational Fund for Scientific and Technological Personnel of Hainan Provinceby the Natural Science Foundation of Shandong Provincial under Grant No.ZR2021QA046。
文摘The study of collision between metastable positronium(Ps)and antihydrogen(H)is crucial for precision experiments involving H.In this paper,we investigate the elastic scattering between H and Ps(2s)by combining the confined variational method with the projection method,for scattering energies from 0.0245 eV to 0.068 eV.Our calculations provide accurate phase shifts and cross sections for the 1,3S and 1,3P symmetries.Near the binding threshold,the rapid increase in the total cross section may be attributed to the P-wave resonance effect.Additionally,we determined the S-wave scattering lengths to be 9.34 a_(0)and 5.81 a_(0)for singlet and triplet elastic scattering,respectively.
基金W.W.was supported by the China Postdoctoral Science Foundation(Grant No.2023M741992)Z.Y.was supported by the National Natural Science Foundation of China(Grant No.11925108).
文摘In this paper,we present some properties of scattering data for the derivative nonlinear Schrödinger equation in H^(S)(R)(s≥1/2)starting from the Lax pair.We show that the reciprocal of the transmission coefficient can be expressed as the sum of some iterative integrals,and its logarithm can be written as the sum of some connected iterative integrals.We provide the asymptotic properties of the first few iterative integrals of the reciprocal of the transmission coefficient.Moreover,we provide some regularity properties of the reciprocal of the transmission coefficient related to scattering data in H^(S)(R).
基金Under the auspices of the Key Program of National Natural Science Foundation of China(No.42030409)。
文摘Multi-source data fusion provides high-precision spatial situational awareness essential for analyzing granular urban social activities.This study used Shanghai’s catering industry as a case study,leveraging electronic reviews and consumer data sourced from third-party restaurant platforms collected in 2021.By performing weighted processing on two-dimensional point-of-interest(POI)data,clustering hotspots of high-dimensional restaurant data were identified.A hierarchical network of restaurant hotspots was constructed following the Central Place Theory(CPT)framework,while the Geo-Informatic Tupu method was employed to resolve the challenges posed by network deformation in multi-scale processes.These findings suggest the necessity of enhancing the spatial balance of Shanghai’s urban centers by moderately increasing the number and service capacity of suburban centers at the urban periphery.Such measures would contribute to a more optimized urban structure and facilitate the outward dispersion of comfort-oriented facilities such as the restaurant industry.At a finer spatial scale,the distribution of restaurant hotspots demonstrates a polycentric and symmetric spatial pattern,with a developmental trend radiating outward along the city’s ring roads.This trend can be attributed to the efforts of restaurants to establish connections with other urban functional spaces,leading to the reconfiguration of urban spaces,expansion of restaurant-dedicated land use,and the reorganization of associated commercial activities.The results validate the existence of a polycentric urban structure in Shanghai but also highlight the instability of the restaurant hotspot network during cross-scale transitions.
基金Sponsored by Beijing Youth Innovation Talent Support Program for Urban Greening and Landscaping——The 2024 Special Project for Promoting High-Quality Development of Beijing’s Landscaping through Scientific and Technological Innovation(KJCXQT202410).
文摘Taking the Ming Tombs Forest Farm in Beijing as the research object,this research applied multi-source data fusion and GIS heat-map overlay analysis techniques,systematically collected bird observation point data from the Global Biodiversity Information Facility(GBIF),population distribution data from the Oak Ridge National Laboratory(ORNL)in the United States,as well as information on the composition of tree species in suitable forest areas for birds and the forest geographical information of the Ming Tombs Forest Farm,which is based on literature research and field investigations.By using GIS technology,spatial processing was carried out on bird observation points and population distribution data to identify suitable bird-watching areas in different seasons.Then,according to the suitability value range,these areas were classified into different grades(from unsuitable to highly suitable).The research findings indicated that there was significant spatial heterogeneity in the bird-watching suitability of the Ming Tombs Forest Farm.The north side of the reservoir was generally a core area with high suitability in all seasons.The deep-aged broad-leaved mixed forests supported the overlapping co-existence of the ecological niches of various bird species,such as the Zosterops simplex and Urocissa erythrorhyncha.In contrast,the shallow forest-edge coniferous pure forests and mixed forests were more suitable for specialized species like Carduelis sinica.The southern urban area and the core area of the mausoleums had relatively low suitability due to ecological fragmentation or human interference.Based on these results,this paper proposed a three-level protection framework of“core area conservation—buffer zone management—isolation zone construction”and a spatio-temporal coordinated human-bird co-existence strategy.It was also suggested that the human-bird co-existence space could be optimized through measures such as constructing sound and light buffer interfaces,restoring ecological corridors,and integrating cultural heritage elements.This research provided an operational technical approach and decision-making support for the scientific planning of bird-watching sites and the coordination of ecological protection and tourism development.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.12174239,12347165,and 12404330)Shaanxi Fundamental Science Research Project for Mathematics and Physics(Grant No.23JSY022)+2 种基金Natural Science Basic Research Program of Shaanxi(Grant No.2022JM-015)Hebei Natural Science Foundation(Grant No.A2022205002)Science and Technology Project of Hebei Education Department(Grant No.QN2022143)。
文摘This study analytically examines the ionization of atoms in strong near-circular laser fields.The classic Keldysh-Rutherford(KR)Coulomb-scattering(CS)model[Phys.Rev.Lett.121123201(2018)]successfully explained the attoclock experimental curve for the H atom at lower laser intensities.Here,we develop a semiclassical model that includes the initial conditions related to the quantum properties of tunneling in the KR model at the beginning of the scattering process.This model is able to explain recent attoclock experimental curves over a wider range of laser and atomic parameters.Our results show the importance of system symmetry and quantum effects in attoclock measurements,suggesting the complex role of the Coulomb potential in strong-field ionization.
