Continuous dynamic experiment was conducted for the treatment of low-concentration organic waste gas with xylene as a representative, using micro-nano bubble and peroxymonosulfate working in synergy. The degradation r...Continuous dynamic experiment was conducted for the treatment of low-concentration organic waste gas with xylene as a representative, using micro-nano bubble and peroxymonosulfate working in synergy. The degradation rule of xylene under different conditions such as the ORP value of the spray liquid, pH value of the spray liquid, liquid-gas ratio of the spray liquid, residence time of xylene, and initial concentration of xylene was investigated. The results showed that at a low concentration, the pH value of the spray liquid had little effect on the degradation rate of xylene. The degradation rate of xylene rose with the increase of the ORP value of the spray liquid, the liquid-gas ratio of the spray liquid, the residence time of xylene, and the initial concentration of xylene.展开更多
With the continuous deepening of rural revitalization strategy and the increasingly strict sewage discharge standards,rural domestic sewage treatment technology is facing higher challenges and requirements.The combine...With the continuous deepening of rural revitalization strategy and the increasingly strict sewage discharge standards,rural domestic sewage treatment technology is facing higher challenges and requirements.The combined process of micro-electrolysis+micro-nano bubbles coupled with peroxymonosulfate was constructed in this study,and the treatment effect and application value of this technology were explored with the actual rural domestic sewage as the treatment object.The experimental results showed that under the conditions of HRT of 120 min,PMS dosage of 0.15 mmol/L,pH=7,MBs air intake of 15 ml/min,current intensity of 15 A,and Fe/C mass ratio of 1:1,the removal rates of COD,ammonia nitrogen and total phosphorus can reach 88.55%,77.18%and 74.67%,respectively.Under the condition that the pH value of sewage was not adjusted,the non-biochemical simultaneous decarbonization,denitrification and phosphorus removal of rural domestic sewage can be achieved by micro-electrolysis and micro-nano bubbles coupled with peroxymonosulfate.The concentrations of effluent COD,ammonia nitrogen and total phosphorus met the requirements of the first level standard of the Discharge Standard of Water Pollutants for Rural Domestic Sewage Treatment Facilities(DB45T2413-2021).And the comprehensive operating cost was about 1.15 yuan/m 3.展开更多
The activation of oxygen by ferrous(Fe^(2+))to generate·OH for contaminants degradation was inhibited due to the low utilization of oxygen,thus limiting its application in the practical environment.In this study,...The activation of oxygen by ferrous(Fe^(2+))to generate·OH for contaminants degradation was inhibited due to the low utilization of oxygen,thus limiting its application in the practical environment.In this study,with the superior oxygenation capacity of micro-nano bubbles(MNBs)and the stronger O_(2) activation capacity of Fe^(2+)-oxalate complexes,the MNBs/Fe^(2+)/oxalate(Ox)system was constructed with 4,4′-sulfonyldiphenol(BPS)as the main target emerging contaminants(ECs),and to investigate the enhancement contribution and reinforcement mechanism of the involvement of MNBs to the removal efficiency of ECs in the Fe^(2+)/Ox system.It was shown that the MNBs/Fe^(2+)/Ox system could effectively degrade four structurally diverse ECs.In this case,with BPS as the main target contaminant,adding MNBs could increase the BPS removal efficiency by about 35%.In the MNBs/Fe^(2+)/Ox system,the degradation rate of BPS depended on the concentration of Fe^(Ⅱ)(Ox)_(2)^(2-),while the extent of degradation was mainly governed by Fe^(Ⅱ)(Ox)_(2)^(2-)and Fe^(Ⅱ)(Ox)^(0).EPR and probe experiments showed that the reactive oxygen species(ROS)produced by the system and the iron hydroxide complexes produced by Fe^(3+)hydrolysis contributed to the degradation of BPS by oxidation and coagulation,respectively.In particular,·OH and O_(2)^(·-)were the main reactive oxygen species produced by this system.Moreover,the involvement of MNBs significantly increased the formation of ROS and iron hydroxide complexes in the Fe^(2+)/Ox system.The oxygenation process of MNBs used in this study enhanced the contaminants degradation performance of the Fe^(2+)/O_(x) system and has broadened the application scope of MNBs.展开更多
In this study,the dynamic characteristics of microscale floating bubbles near the vertical wall are studied.This occurrence is common in industrial and natural phenomena.Although many studies have been conducted on mi...In this study,the dynamic characteristics of microscale floating bubbles near the vertical wall are studied.This occurrence is common in industrial and natural phenomena.Although many studies have been conducted on microscale bubbles,few studies investigate floating bubbles with very small Reynolds number(Re)near the wall,which is the main research goal of this study.Therefore,this study establishes a model for the ascent of small-scale bubbles near a vertical wall using the interFoam solver in OpenFOAM.This study investigates the influences of diverse viscosity parameters,varying distances from the wall,and different gas flow rates on the terminal velocity,deformation,and motion trajectory of bubbles.The results reveal that as liquid viscosity increases,the Re of bubbles gradually decreases and reaches a minimum of 0.012,which is similar to the Re of micrometer-sized bubbles in water.The characteristics of the wall-induced force in the longitudinal direction are closely related to the changes in liquid viscosity.Under low-viscosity conditions,the induced lift is the principal form of action,whereas under high-viscosity conditions,it is primarily manifested as induced drag.展开更多
Cleaning a surface using a solution containing a large number of micro to nano scale bubbles has significant advantage regarding environmental protection.This review first briefly introduces the cleaning mechanism of ...Cleaning a surface using a solution containing a large number of micro to nano scale bubbles has significant advantage regarding environmental protection.This review first briefly introduces the cleaning mechanism of micro-nano bubbles(MNBs),including physical and chemical effects.Then the applications of MNBs in cleaning of metal parts,precision parts,cultural relics or food are introduced.After that,coupled cleaning method of ultrasound and bubbles is introduced.Finally,the characterization methods for the cleaning effect are introduced,which mainly focuses on the changes of physico-chemical properties(mass or cleaning area,infiltration,colony number and light scattering intensity)of the cleaned parts or that(like conductivity)of the solvent.It is believed that MNBs technology will be applied in a broader range of surface cleaning applications.展开更多
The material loss caused by bubble collapse during the micro-nano bubbles auxiliary chemical mechanical polishing(CMP)process cannot be ignored.In this study,the material removal mechanism of cavitation in the polishi...The material loss caused by bubble collapse during the micro-nano bubbles auxiliary chemical mechanical polishing(CMP)process cannot be ignored.In this study,the material removal mechanism of cavitation in the polishing process was investigated in detail.Based on the mixed lubrication or thin film lubrication,bubble-wafer plastic deformation,spherical indentation theory,Johnson-Cook(J-C)constitutive model,and the assumption of periodic distribution of pad asperities,a new model suitable for micro-nano bubble auxiliary material removal in CMP was developed.The model integrates many parameters,including the reactant concentration,wafer hardness,polishing pad roughness,strain hardening,strain rate,micro-jet radius,and bubble radius.The model reflects the influence of active bubbles on material removal.A new and simple chemical reaction method was used to form a controllable number of micro-nano bubbles during the polishing process to assist in polishing silicon oxide wafers.The experimental results show that micro-nano bubbles can greatly increase the material removal rate(MRR)by about 400%and result in a lower surface roughness of 0.17 nm.The experimental results are consistent with the established model.In the process of verifying the model,a better understanding of the material removal mechanism involved in micro-nano bubbles in CMP was obtained.展开更多
This paper highlights the crucial role of Indonesia’s GNSS receiver network in advancing Equatorial Plasma Bubble(EPB)studies in Southeast and East Asia,as ionospheric irregularities within EPB can disrupt GNSS signa...This paper highlights the crucial role of Indonesia’s GNSS receiver network in advancing Equatorial Plasma Bubble(EPB)studies in Southeast and East Asia,as ionospheric irregularities within EPB can disrupt GNSS signals and degrade positioning accuracy.Managed by the Indonesian Geospatial Information Agency(BIG),the Indonesia Continuously Operating Reference Station(Ina-CORS)network comprises over 300 GNSS receivers spanning equatorial to southern low-latitude regions.Ina-CORS is uniquely situated to monitor EPB generation,zonal drift,and dissipation across Southeast Asia.We provide a practical tool for EPB research,by sharing two-dimensional rate of Total Electron Content(TEC)change index(ROTI)derived from this network.We generate ROTI maps with a 10-minute resolution,and samples from May 2024 are publicly available for further scientific research.Two preliminary findings from the ROTI maps of Ina-CORS are noteworthy.First,the Ina-CORS ROTI maps reveal that the irregularities within a broader EPB structure persist longer,increasing the potential for these irregularities to migrate farther eastward.Second,we demonstrate that combined ROTI maps from Ina-CORS and GNSS receivers in East Asia and Australia can be used to monitor the development of ionospheric irregularities in Southeast and East Asia.We have demonstrated the combined ROTI maps to capture the development of ionospheric irregularities in the Southeast/East Asian sector during the G5 Geomagnetic Storm on May 11,2024.We observed simultaneous ionospheric irregularities in Japan and Australia,respectively propagating northwestward and southwestward,before midnight,whereas Southeast Asia’s equatorial and low-latitude regions exhibited irregularities post-midnight.By sharing ROTI maps from Indonesia and integrating them with regional GNSS networks,researchers can conduct comprehensive EPB studies,enhancing the understanding of EPB behavior across Southeast and East Asia and contributing significantly to ionospheric research.展开更多
Bubbles play crucial roles in various fields,including naval and ocean engineering,chemical engineering,and biochemical engineering.Numerous theoretical analyses,numerical simulations,and experimental studies have bee...Bubbles play crucial roles in various fields,including naval and ocean engineering,chemical engineering,and biochemical engineering.Numerous theoretical analyses,numerical simulations,and experimental studies have been conducted to reveal the mysteries of bubble motion and its mechanisms.These efforts have significantly advanced research in bubble dynamics,where theoretical study is an efficient method for bubble motion prediction.Since Lord Rayleigh introduced the theoretical model of single-bubble motion in incompressible fluid in 1917,theoretical studies have been pivotal in understanding bubble dynamics.This study provides a comprehensive review of the development and applicability of theoretical studies in bubble dynamics using typical theoretical bubble models across different periods as a focal point and an overview of bubble theory applications in underwater explosion,marine cavitation,and seismic exploration.This study aims to serve as a reference and catalyst for further advancements in theoretical analysis and practical applications of bubble theory across marine fields.展开更多
Unlike conventional spherical charges,a shaped charge generates not only a strong shock wave and a pulsating bubble,but also a high strain rate metal jet and a ballistic wave during the underwater explosion.They show ...Unlike conventional spherical charges,a shaped charge generates not only a strong shock wave and a pulsating bubble,but also a high strain rate metal jet and a ballistic wave during the underwater explosion.They show significant characteristic differences and couple each other.This paper designs and conducts experiments with shaped charges to analyze the complicated process.The effects of liner angle and weight of shaped charge on the characteristics of metal jets,waves,and bubbles are discussed.It is found that in underwater explosions,the shaped charge generates the metal jet accompanied by the ballistic wave.Then,the shock wave propagates and superimposes with the ballistic wave,and the generated bubble pulsates periodically.It is revealed that the maximum head velocity of the metal jet versus the liner angle a and length-to-diameter ratio k of the shaped charge follows the laws of 1/(α/180°)^(0.55)andλ^(0.16),respectively.The head shape and velocity of the metal jet determine the curvature and propagation speed of the initial ballistic wave,thus impacting the superposition time and region with the shock wave.Our findings also reveal that the metal jet carries away some explosion products,which hinders the bubble development,causing an inward depression of the bubble wall near the metal jet.Therefore,the maximum bubble radius and pulsation period are 5.2%and 3.9%smaller than the spherical charge with the same weight.In addition,the uneven axial energy distribution of the shaped charge leads to an oblique bubble jet formation.展开更多
To analyze the impact of bubbles on the mechanical behavior of glasses,by controlling the refining time,we prepared three borosilicate glasses with the same composition and different porosity.By the analysis software ...To analyze the impact of bubbles on the mechanical behavior of glasses,by controlling the refining time,we prepared three borosilicate glasses with the same composition and different porosity.By the analysis software integrated within the optical microscope,the diameter and number of the bubbles on the surface of three borosilicate glasses were quantified.From the hardness and crack initiation resistance(CR),we built the relationship between the porosity and the mechanical performance of these borosilicate glasses.展开更多
During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a rest...During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a restrictive link,closely associated with viscosity and the thickness of liquid slag.In contrast to two-dimensional surface observation,three-dimensional(3D)analysis method can offer a more intuitive,accurate,and comprehensive information.Therefore,this study employs a 3D X-ray microscope(3D-XRM)to obtained spatial distribution and 3D morphological characteristics of residual bubbles in mold flux under different basicity of liquid slag,different temperatures,and different holding times.The results indicate that as basicity of slag increases from 0.52 to 1.03,temperature increases from 1423 to 1573 K,the viscosity of slag decreases,the floating rate of bubbles increases.In addition,when holding time increases from 10 to 30 s,the bubbles floating distance increases,and the volume fraction and average equivalent sphere diameter of the bubbles solidified in the mold flux gradually decreases.In one word,increasing the basicity,temperature,and holding time leading to an increase in the removal rate of bubbles especially for the large.These findings of bubbles escape behavior provide valuable insights into optimizing low basicity mold flux for high-Mn high-Al steels.展开更多
In this paper,the failure caused by HRAM loads which were generated by high-speed projectile penetration,and protection technology of the fluid-filled structure were explored.A bubble was preset on the projectile traj...In this paper,the failure caused by HRAM loads which were generated by high-speed projectile penetration,and protection technology of the fluid-filled structure were explored.A bubble was preset on the projectile trajectory in a fluid-filled structure.Based on the reflection and transmission phenomena of pressure waves at the gas-liquid interface and the compressibility characteristics of gases,a numerical analysis was conducted on the influence of preset bubble on projectile penetration and structural failure characteristics.The results indicate that the secondary water-entry impact phenomenon occurs when a preset bubble exists on the projectile trajectory,leading to the secondary water entry impact loads.The rarefaction waves reflected on the surface of the preset bubble cause the attenuation ratio of the initial impact pressure peak to reach 68.8%and the total specific impulse attenuation ratio to reach 48.6%.Furthermore,the larger the bubble,the faster the projectile,and the more obvious the attenuation effect.Moreover,due to the compressibility of the bubble,the global deformation attenuation ratio of the front and rear walls can reach over 80%.However,the larger the bubble size,the faster the projectile velocity,the smaller the local deformation attenuation effect of the rear wall,and the more severe the failure at the perforation of the rear wall.展开更多
In nature,cavitation bubbles typically appear in clusters,engaging in interactions that create a variety of dynamicmotion patterns.To better understand the behavior ofmultiple bubble collapses and the mechanisms of in...In nature,cavitation bubbles typically appear in clusters,engaging in interactions that create a variety of dynamicmotion patterns.To better understand the behavior ofmultiple bubble collapses and the mechanisms of interbubble interaction,this study employs molecular dynamics simulation combined with a coarse-grained force field.By focusing on collapsemorphology,local density,and pressure,it elucidates how the number and arrangement of bubbles influence the collapse process.The mechanisms behind inter-bubble interactions are also considered.The findings indicate that the collapse speed of unbounded bubbles located in lateral regions is greater than that of the bubbles in the center.Moreover,it is shown that asymmetrical bubble distributions lead to a shorter collapse time overall.展开更多
The gas-liquid countercurrent flow pattern is complex and the bubble migration velocity is difficult to predict in the process of bullheading well killing.The experiment on bubble migration in gas-liquid countercurren...The gas-liquid countercurrent flow pattern is complex and the bubble migration velocity is difficult to predict in the process of bullheading well killing.The experiment on bubble migration in gas-liquid countercurrent flow in annulus is carried out under different working conditions to reveal how the wellbore inclination angle,liquid phase property and countercurrent liquid velocity affect the bubble deformation and bubble migration trajectory/velocity,and to establish a bubble migration velocity prediction model.The bubbles in the countercurrent flow mainly migrate in two modes:free rising of isolated bubbles,and interactive rising of multiple bubbles.The bubbles migrate by an S-shaped trajectory in the countercurrent flow.With the increase of countercurrent liquid velocity,the lateral oscillation of bubbles is intensified.The increases of wellbore inclination angle,liquid density and liquid viscosity make the bubble migration trajectory gradually to be linear.The bubble is generally ellipsoidal during its rising.The wellbore inclination angle has little effect on the degree of bubble deformation.The bubbles are ellipsoidal during rising,with little influence of wellbore inclination angle on bubble deformation.With the increase of liquid viscosity and density,the aspect ratio of the bubble decreases.As the wellbore inclination angle increases,the bubble migration velocity gradually decreases.As the liquid viscosity increases,the bubble migration velocity decreases.As the liquid density increases,the bubble migration velocity increases slightly.The established bubble migration velocity prediction model yields errors within±15%,and demonstrates broad applicability across a wide range of operating conditions.展开更多
Bubbles within an elastic shell,which undergo ultrasound-driven oscillation to treat tumors and soft tissues,are frequently treated as viscoelastic media.Therefore,studying the dynamic behavior of bubbles wrapped in a...Bubbles within an elastic shell,which undergo ultrasound-driven oscillation to treat tumors and soft tissues,are frequently treated as viscoelastic media.Therefore,studying the dynamic behavior of bubbles wrapped in a viscoelastic medium while considering an elastic shell can provide theoretical support for ultrasound biotherapy.Bubbles are always in the form of clusters.Therefore,a model of spherical bubble clusters in a liquid cavity wrapped by an elastic shell was constructed,the coupled oscillation equations of bubbles were obtained by taking into account the dynamic effects of the elastic shell and the viscoelastic media outside the cavity,and the oscillation behaviors of the bubbles were analyzed.Acoustic waves at 1.5 MHz could cause bubbles with a radius of 1μm to resonate.Increasing the number of bubbles increased the suppressing effect of bubble oscillation caused by bubble interaction.The bubble cluster oscillation caused the elastic shell to oscillate and be stressed,and the stress trend was the inverse of the bubble oscillation trend with maximal tensile and compressive stresses.Bubbles with an equilibrium radius of 2μm exhibited the lowest inertial cavitation threshold,making inertial cavitation more likely under high-frequency acoustic excitation.The inertial cavitation threshold of bubbles was heavily influenced by the acoustic wave frequency,bubble number density,and bubble cluster radius.The nonspherical oscillation stability of bubbles was primarily affected by the driving acoustic pressure amplitude and frequency,bubble initial radius,bubble number density,and bubble cluster radius.The acoustic frequency and amplitude exhibited a synergistic effect,with a minimum unstable driving acoustic pressure threshold of approximately 0.13 MPa.The initial radius within the elastic shell affected the minimum unstable driving acoustic pressure threshold.展开更多
Bubble column reactors fitted with tube bundles(BCR TB)belong to common heat transfer equipment in the field of chemical engineering,yet the complicated thermal-hydraulics performance of BCR TB has not been deeply rev...Bubble column reactors fitted with tube bundles(BCR TB)belong to common heat transfer equipment in the field of chemical engineering,yet the complicated thermal-hydraulics performance of BCR TB has not been deeply revealed.To fill this gap,the present study proposes a novel variable bubble size modeling approach based on the Euler-Euler two-fluid framework,which is coupled with the population balance model considering comprehensive interphase forces.On the basis of verifying numerical reliability using experimental data,the mechanism of bubble swarm flow around the tube bundle and the effects of gas sparger configurations on the thermal-hydraulics performance of BCR TB are investigated.Results indicate that the entire tube bundle can be divided into three distinct zones,namely the sparger effect zone,fully developed zone and interface effect zone in view of the local mixture-to-wall heat transfer coefficient.The maximum peak value of the mixture-to-wall heat transfer coefficient always appears at 210°of heat exchange tubes.When the orifice diameter is 4 mm,the axial gradient of gas holdup is relatively large due to more intense shearing and fragmentation effects.Interestingly,the fractions of medium-sized and large-sized bubbles are not sensitive to orifice angle.Both the mixture-to-wall heat transfer coefficient and the friction factor decrease initially and then increase when the installation height increases.Under the optimized gas sparger structure configuration,the mixture-to-wall heat transfer coefficient increases by 10.23%,accompanied by the reduction of pressure drop by 8.14%,ultimately attaining a system energy conversion efficiency of 97.88%and performance evaluation criterion of 1.087.Finally,a new dimensionless and semi-theoretical Nusselt correlation incorporating a structural correction factor with an average absolute deviation of 5.15%is developed.The findings can offer useful guidance for the optimal design of BCR TB.展开更多
The internal pressure within fission gas bubbles(FGBs)in irradiated nuclear fuels drives mechanical interactions with the surrounding fuel skeleton.To investigate the micromechanical stress fields in irradiated nuclea...The internal pressure within fission gas bubbles(FGBs)in irradiated nuclear fuels drives mechanical interactions with the surrounding fuel skeleton.To investigate the micromechanical stress fields in irradiated nuclear fuels containing pressurized FGBs,a mechanical constitutive model for the equivalent solid of FGBs was developed and validated.This model was based on the modified Van der Waals equation,incorporating the effects of surface tension.Using this model,the micromechanical fields in irradiated U-10Mo fuels with randomly distributed FGBs were calculated during uniaxial tensile testing via the finite element(FE)method.The macroscopic elastic constants of the irradiated U-10Mo fuels were then derived using homogenization theory,and the influences of bubble pressure,bubble size,and porosity on these constants were examined.Results show that adjacent FGBs exhibit mechanical interactions,which leads to distinct stress concentrations in the surrounding fuel skeleton.The macroscopic elastic constants of irradiated U-10Mo fuels decrease with increasing the macroscopic porosity,which can be quantitatively described by the Mori-Tanaka model.In contrast,bubble pressure and size have negligible effects on these constants.展开更多
This study explores the combination of ultrasound technology with a detection algorithm to categorize flow regimes in bubble columns used for aeration in aquaculture.An ultrasonic velocity profiler is used to obtain t...This study explores the combination of ultrasound technology with a detection algorithm to categorize flow regimes in bubble columns used for aeration in aquaculture.An ultrasonic velocity profiler is used to obtain the standard deviation of the bubble velocity distributed throughout the column.The bubble velocity data for three known flow regimes were used to develop a probability density function(PDF)classification model.The experimental apparatus consisted of a circular tank equipped with a bubble generator and gas hold-up monitoring systems.The flow regimes of the experimental fluid were determined,and the classification was conducted via the PDF method.The results demonstrate that the classification accuracy is not lower than that of traditional machine learning methods.展开更多
基金Supported by Guigang City Science Research and Technology Development Plan Project(GUIKEJI2203014).
文摘Continuous dynamic experiment was conducted for the treatment of low-concentration organic waste gas with xylene as a representative, using micro-nano bubble and peroxymonosulfate working in synergy. The degradation rule of xylene under different conditions such as the ORP value of the spray liquid, pH value of the spray liquid, liquid-gas ratio of the spray liquid, residence time of xylene, and initial concentration of xylene was investigated. The results showed that at a low concentration, the pH value of the spray liquid had little effect on the degradation rate of xylene. The degradation rate of xylene rose with the increase of the ORP value of the spray liquid, the liquid-gas ratio of the spray liquid, the residence time of xylene, and the initial concentration of xylene.
基金Supported by Research Foundation Ability Enhancement Project for Young and Middle-aged Teachers in Guangxi Universities(2023KY2049).
文摘With the continuous deepening of rural revitalization strategy and the increasingly strict sewage discharge standards,rural domestic sewage treatment technology is facing higher challenges and requirements.The combined process of micro-electrolysis+micro-nano bubbles coupled with peroxymonosulfate was constructed in this study,and the treatment effect and application value of this technology were explored with the actual rural domestic sewage as the treatment object.The experimental results showed that under the conditions of HRT of 120 min,PMS dosage of 0.15 mmol/L,pH=7,MBs air intake of 15 ml/min,current intensity of 15 A,and Fe/C mass ratio of 1:1,the removal rates of COD,ammonia nitrogen and total phosphorus can reach 88.55%,77.18%and 74.67%,respectively.Under the condition that the pH value of sewage was not adjusted,the non-biochemical simultaneous decarbonization,denitrification and phosphorus removal of rural domestic sewage can be achieved by micro-electrolysis and micro-nano bubbles coupled with peroxymonosulfate.The concentrations of effluent COD,ammonia nitrogen and total phosphorus met the requirements of the first level standard of the Discharge Standard of Water Pollutants for Rural Domestic Sewage Treatment Facilities(DB45T2413-2021).And the comprehensive operating cost was about 1.15 yuan/m 3.
基金financially supported by the National Natural Science Foundation of China(Nos.52470014 and 52370100)the Department of Education of Gansu Province(China):Major Cultivation Project of Scientific Research Innovation Platform in University(No.2024CXPT-14).
文摘The activation of oxygen by ferrous(Fe^(2+))to generate·OH for contaminants degradation was inhibited due to the low utilization of oxygen,thus limiting its application in the practical environment.In this study,with the superior oxygenation capacity of micro-nano bubbles(MNBs)and the stronger O_(2) activation capacity of Fe^(2+)-oxalate complexes,the MNBs/Fe^(2+)/oxalate(Ox)system was constructed with 4,4′-sulfonyldiphenol(BPS)as the main target emerging contaminants(ECs),and to investigate the enhancement contribution and reinforcement mechanism of the involvement of MNBs to the removal efficiency of ECs in the Fe^(2+)/Ox system.It was shown that the MNBs/Fe^(2+)/Ox system could effectively degrade four structurally diverse ECs.In this case,with BPS as the main target contaminant,adding MNBs could increase the BPS removal efficiency by about 35%.In the MNBs/Fe^(2+)/Ox system,the degradation rate of BPS depended on the concentration of Fe^(Ⅱ)(Ox)_(2)^(2-),while the extent of degradation was mainly governed by Fe^(Ⅱ)(Ox)_(2)^(2-)and Fe^(Ⅱ)(Ox)^(0).EPR and probe experiments showed that the reactive oxygen species(ROS)produced by the system and the iron hydroxide complexes produced by Fe^(3+)hydrolysis contributed to the degradation of BPS by oxidation and coagulation,respectively.In particular,·OH and O_(2)^(·-)were the main reactive oxygen species produced by this system.Moreover,the involvement of MNBs significantly increased the formation of ROS and iron hydroxide complexes in the Fe^(2+)/Ox system.The oxygenation process of MNBs used in this study enhanced the contaminants degradation performance of the Fe^(2+)/O_(x) system and has broadened the application scope of MNBs.
基金Supported by the National Natural Science Foundation of China(Grant No.52271319)the Jiangsu Funding Program for Excellent Postdoctoral Talent,and the Postdoctoral Fellowship Program of China Postdoctoral Science Foundation(Grant No.GZC20240618)the Natural Science Foundation of Jiangsu Province of China(BK20231525).
文摘In this study,the dynamic characteristics of microscale floating bubbles near the vertical wall are studied.This occurrence is common in industrial and natural phenomena.Although many studies have been conducted on microscale bubbles,few studies investigate floating bubbles with very small Reynolds number(Re)near the wall,which is the main research goal of this study.Therefore,this study establishes a model for the ascent of small-scale bubbles near a vertical wall using the interFoam solver in OpenFOAM.This study investigates the influences of diverse viscosity parameters,varying distances from the wall,and different gas flow rates on the terminal velocity,deformation,and motion trajectory of bubbles.The results reveal that as liquid viscosity increases,the Re of bubbles gradually decreases and reaches a minimum of 0.012,which is similar to the Re of micrometer-sized bubbles in water.The characteristics of the wall-induced force in the longitudinal direction are closely related to the changes in liquid viscosity.Under low-viscosity conditions,the induced lift is the principal form of action,whereas under high-viscosity conditions,it is primarily manifested as induced drag.
基金Financial supports from the Ministry of Science and Technology,China(No.ZK20210004)the Department of Science and Technology of Shandong Province,China(No.ZK20200026)are gratefully acknowledged.
文摘Cleaning a surface using a solution containing a large number of micro to nano scale bubbles has significant advantage regarding environmental protection.This review first briefly introduces the cleaning mechanism of micro-nano bubbles(MNBs),including physical and chemical effects.Then the applications of MNBs in cleaning of metal parts,precision parts,cultural relics or food are introduced.After that,coupled cleaning method of ultrasound and bubbles is introduced.Finally,the characterization methods for the cleaning effect are introduced,which mainly focuses on the changes of physico-chemical properties(mass or cleaning area,infiltration,colony number and light scattering intensity)of the cleaned parts or that(like conductivity)of the solvent.It is believed that MNBs technology will be applied in a broader range of surface cleaning applications.
基金supported by the National Natural Science Foundation of China(No.51975343)Science and Technology Major Project of Inner Mongolia Autonomous Region in China(No.2021ZD0028)+1 种基金Shanghai Technical Service Center for Advanced Ceramics Structure Design and Precision Manufacturing(No.20DZ2294000)the China Scholarship Council.
文摘The material loss caused by bubble collapse during the micro-nano bubbles auxiliary chemical mechanical polishing(CMP)process cannot be ignored.In this study,the material removal mechanism of cavitation in the polishing process was investigated in detail.Based on the mixed lubrication or thin film lubrication,bubble-wafer plastic deformation,spherical indentation theory,Johnson-Cook(J-C)constitutive model,and the assumption of periodic distribution of pad asperities,a new model suitable for micro-nano bubble auxiliary material removal in CMP was developed.The model integrates many parameters,including the reactant concentration,wafer hardness,polishing pad roughness,strain hardening,strain rate,micro-jet radius,and bubble radius.The model reflects the influence of active bubbles on material removal.A new and simple chemical reaction method was used to form a controllable number of micro-nano bubbles during the polishing process to assist in polishing silicon oxide wafers.The experimental results show that micro-nano bubbles can greatly increase the material removal rate(MRR)by about 400%and result in a lower surface roughness of 0.17 nm.The experimental results are consistent with the established model.In the process of verifying the model,a better understanding of the material removal mechanism involved in micro-nano bubbles in CMP was obtained.
基金JSPS KAKENHI Grant Number16H06286 supports global GNSS ionospheric maps (TEC,ROTI,and detrended TEC maps) developed by the Institute for SpaceEarth Environmental Research (ISEE) of Nagoya Universitysupport of the 2024 JASSO Follow-up Research Fellowship Program for a 90-day visiting research at the Institute for Space-Earth Environmental Research (ISEE),Nagoya University+3 种基金the support received from Telkom University under the“Skema Penelitian Terapan Periode I Tahun Anggaran 2024”the Memorandum of Understanding for Research Collaboration on Regional Ionospheric Observation (No:092/SAM3/TE-DEK/2021)the National Institute of Information and Communications Technology (NICT) International Exchange Program 2024-2025(No.2024-007)support for a one-year visiting research at Hokkaido University
文摘This paper highlights the crucial role of Indonesia’s GNSS receiver network in advancing Equatorial Plasma Bubble(EPB)studies in Southeast and East Asia,as ionospheric irregularities within EPB can disrupt GNSS signals and degrade positioning accuracy.Managed by the Indonesian Geospatial Information Agency(BIG),the Indonesia Continuously Operating Reference Station(Ina-CORS)network comprises over 300 GNSS receivers spanning equatorial to southern low-latitude regions.Ina-CORS is uniquely situated to monitor EPB generation,zonal drift,and dissipation across Southeast Asia.We provide a practical tool for EPB research,by sharing two-dimensional rate of Total Electron Content(TEC)change index(ROTI)derived from this network.We generate ROTI maps with a 10-minute resolution,and samples from May 2024 are publicly available for further scientific research.Two preliminary findings from the ROTI maps of Ina-CORS are noteworthy.First,the Ina-CORS ROTI maps reveal that the irregularities within a broader EPB structure persist longer,increasing the potential for these irregularities to migrate farther eastward.Second,we demonstrate that combined ROTI maps from Ina-CORS and GNSS receivers in East Asia and Australia can be used to monitor the development of ionospheric irregularities in Southeast and East Asia.We have demonstrated the combined ROTI maps to capture the development of ionospheric irregularities in the Southeast/East Asian sector during the G5 Geomagnetic Storm on May 11,2024.We observed simultaneous ionospheric irregularities in Japan and Australia,respectively propagating northwestward and southwestward,before midnight,whereas Southeast Asia’s equatorial and low-latitude regions exhibited irregularities post-midnight.By sharing ROTI maps from Indonesia and integrating them with regional GNSS networks,researchers can conduct comprehensive EPB studies,enhancing the understanding of EPB behavior across Southeast and East Asia and contributing significantly to ionospheric research.
文摘Bubbles play crucial roles in various fields,including naval and ocean engineering,chemical engineering,and biochemical engineering.Numerous theoretical analyses,numerical simulations,and experimental studies have been conducted to reveal the mysteries of bubble motion and its mechanisms.These efforts have significantly advanced research in bubble dynamics,where theoretical study is an efficient method for bubble motion prediction.Since Lord Rayleigh introduced the theoretical model of single-bubble motion in incompressible fluid in 1917,theoretical studies have been pivotal in understanding bubble dynamics.This study provides a comprehensive review of the development and applicability of theoretical studies in bubble dynamics using typical theoretical bubble models across different periods as a focal point and an overview of bubble theory applications in underwater explosion,marine cavitation,and seismic exploration.This study aims to serve as a reference and catalyst for further advancements in theoretical analysis and practical applications of bubble theory across marine fields.
基金funded by the National Natural Science Founda-tion of China(52071109).
文摘Unlike conventional spherical charges,a shaped charge generates not only a strong shock wave and a pulsating bubble,but also a high strain rate metal jet and a ballistic wave during the underwater explosion.They show significant characteristic differences and couple each other.This paper designs and conducts experiments with shaped charges to analyze the complicated process.The effects of liner angle and weight of shaped charge on the characteristics of metal jets,waves,and bubbles are discussed.It is found that in underwater explosions,the shaped charge generates the metal jet accompanied by the ballistic wave.Then,the shock wave propagates and superimposes with the ballistic wave,and the generated bubble pulsates periodically.It is revealed that the maximum head velocity of the metal jet versus the liner angle a and length-to-diameter ratio k of the shaped charge follows the laws of 1/(α/180°)^(0.55)andλ^(0.16),respectively.The head shape and velocity of the metal jet determine the curvature and propagation speed of the initial ballistic wave,thus impacting the superposition time and region with the shock wave.Our findings also reveal that the metal jet carries away some explosion products,which hinders the bubble development,causing an inward depression of the bubble wall near the metal jet.Therefore,the maximum bubble radius and pulsation period are 5.2%and 3.9%smaller than the spherical charge with the same weight.In addition,the uneven axial energy distribution of the shaped charge leads to an oblique bubble jet formation.
基金Funded by the National Natural Science Foundation of China(No.52172007)。
文摘To analyze the impact of bubbles on the mechanical behavior of glasses,by controlling the refining time,we prepared three borosilicate glasses with the same composition and different porosity.By the analysis software integrated within the optical microscope,the diameter and number of the bubbles on the surface of three borosilicate glasses were quantified.From the hardness and crack initiation resistance(CR),we built the relationship between the porosity and the mechanical performance of these borosilicate glasses.
基金financially supported by the National Natural Science Foundation of China(Nos.52274315 and 52374320)the Fundamental Research Funds for the Central Universities(Nos.FRF-TP-22-011A1 and FRF-DF22-16)。
文摘During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a restrictive link,closely associated with viscosity and the thickness of liquid slag.In contrast to two-dimensional surface observation,three-dimensional(3D)analysis method can offer a more intuitive,accurate,and comprehensive information.Therefore,this study employs a 3D X-ray microscope(3D-XRM)to obtained spatial distribution and 3D morphological characteristics of residual bubbles in mold flux under different basicity of liquid slag,different temperatures,and different holding times.The results indicate that as basicity of slag increases from 0.52 to 1.03,temperature increases from 1423 to 1573 K,the viscosity of slag decreases,the floating rate of bubbles increases.In addition,when holding time increases from 10 to 30 s,the bubbles floating distance increases,and the volume fraction and average equivalent sphere diameter of the bubbles solidified in the mold flux gradually decreases.In one word,increasing the basicity,temperature,and holding time leading to an increase in the removal rate of bubbles especially for the large.These findings of bubbles escape behavior provide valuable insights into optimizing low basicity mold flux for high-Mn high-Al steels.
文摘In this paper,the failure caused by HRAM loads which were generated by high-speed projectile penetration,and protection technology of the fluid-filled structure were explored.A bubble was preset on the projectile trajectory in a fluid-filled structure.Based on the reflection and transmission phenomena of pressure waves at the gas-liquid interface and the compressibility characteristics of gases,a numerical analysis was conducted on the influence of preset bubble on projectile penetration and structural failure characteristics.The results indicate that the secondary water-entry impact phenomenon occurs when a preset bubble exists on the projectile trajectory,leading to the secondary water entry impact loads.The rarefaction waves reflected on the surface of the preset bubble cause the attenuation ratio of the initial impact pressure peak to reach 68.8%and the total specific impulse attenuation ratio to reach 48.6%.Furthermore,the larger the bubble,the faster the projectile,and the more obvious the attenuation effect.Moreover,due to the compressibility of the bubble,the global deformation attenuation ratio of the front and rear walls can reach over 80%.However,the larger the bubble size,the faster the projectile velocity,the smaller the local deformation attenuation effect of the rear wall,and the more severe the failure at the perforation of the rear wall.
基金funded by the Natural Science Foundation of China[U20A20292]Shandong Province Science andTechnology SMES InnovationAbility Improvement Project[2023TSGC0005]China Postdoctoral Science Foundation[2024M752697].
文摘In nature,cavitation bubbles typically appear in clusters,engaging in interactions that create a variety of dynamicmotion patterns.To better understand the behavior ofmultiple bubble collapses and the mechanisms of interbubble interaction,this study employs molecular dynamics simulation combined with a coarse-grained force field.By focusing on collapsemorphology,local density,and pressure,it elucidates how the number and arrangement of bubbles influence the collapse process.The mechanisms behind inter-bubble interactions are also considered.The findings indicate that the collapse speed of unbounded bubbles located in lateral regions is greater than that of the bubbles in the center.Moreover,it is shown that asymmetrical bubble distributions lead to a shorter collapse time overall.
基金Supported by the National Natural Science Foundation of China(U21B2069,52274020,52288101,52274022)National Key Research and Development Program of China(2022YFC2806504)。
文摘The gas-liquid countercurrent flow pattern is complex and the bubble migration velocity is difficult to predict in the process of bullheading well killing.The experiment on bubble migration in gas-liquid countercurrent flow in annulus is carried out under different working conditions to reveal how the wellbore inclination angle,liquid phase property and countercurrent liquid velocity affect the bubble deformation and bubble migration trajectory/velocity,and to establish a bubble migration velocity prediction model.The bubbles in the countercurrent flow mainly migrate in two modes:free rising of isolated bubbles,and interactive rising of multiple bubbles.The bubbles migrate by an S-shaped trajectory in the countercurrent flow.With the increase of countercurrent liquid velocity,the lateral oscillation of bubbles is intensified.The increases of wellbore inclination angle,liquid density and liquid viscosity make the bubble migration trajectory gradually to be linear.The bubble is generally ellipsoidal during its rising.The wellbore inclination angle has little effect on the degree of bubble deformation.The bubbles are ellipsoidal during rising,with little influence of wellbore inclination angle on bubble deformation.With the increase of liquid viscosity and density,the aspect ratio of the bubble decreases.As the wellbore inclination angle increases,the bubble migration velocity gradually decreases.As the liquid viscosity increases,the bubble migration velocity decreases.As the liquid density increases,the bubble migration velocity increases slightly.The established bubble migration velocity prediction model yields errors within±15%,and demonstrates broad applicability across a wide range of operating conditions.
基金supported by the National Natural Science Foundation of China(Grant No.12374441)。
文摘Bubbles within an elastic shell,which undergo ultrasound-driven oscillation to treat tumors and soft tissues,are frequently treated as viscoelastic media.Therefore,studying the dynamic behavior of bubbles wrapped in a viscoelastic medium while considering an elastic shell can provide theoretical support for ultrasound biotherapy.Bubbles are always in the form of clusters.Therefore,a model of spherical bubble clusters in a liquid cavity wrapped by an elastic shell was constructed,the coupled oscillation equations of bubbles were obtained by taking into account the dynamic effects of the elastic shell and the viscoelastic media outside the cavity,and the oscillation behaviors of the bubbles were analyzed.Acoustic waves at 1.5 MHz could cause bubbles with a radius of 1μm to resonate.Increasing the number of bubbles increased the suppressing effect of bubble oscillation caused by bubble interaction.The bubble cluster oscillation caused the elastic shell to oscillate and be stressed,and the stress trend was the inverse of the bubble oscillation trend with maximal tensile and compressive stresses.Bubbles with an equilibrium radius of 2μm exhibited the lowest inertial cavitation threshold,making inertial cavitation more likely under high-frequency acoustic excitation.The inertial cavitation threshold of bubbles was heavily influenced by the acoustic wave frequency,bubble number density,and bubble cluster radius.The nonspherical oscillation stability of bubbles was primarily affected by the driving acoustic pressure amplitude and frequency,bubble initial radius,bubble number density,and bubble cluster radius.The acoustic frequency and amplitude exhibited a synergistic effect,with a minimum unstable driving acoustic pressure threshold of approximately 0.13 MPa.The initial radius within the elastic shell affected the minimum unstable driving acoustic pressure threshold.
基金supported by the project 2024J01421supported by Fujian Provincial Natural Science Foundation.
文摘Bubble column reactors fitted with tube bundles(BCR TB)belong to common heat transfer equipment in the field of chemical engineering,yet the complicated thermal-hydraulics performance of BCR TB has not been deeply revealed.To fill this gap,the present study proposes a novel variable bubble size modeling approach based on the Euler-Euler two-fluid framework,which is coupled with the population balance model considering comprehensive interphase forces.On the basis of verifying numerical reliability using experimental data,the mechanism of bubble swarm flow around the tube bundle and the effects of gas sparger configurations on the thermal-hydraulics performance of BCR TB are investigated.Results indicate that the entire tube bundle can be divided into three distinct zones,namely the sparger effect zone,fully developed zone and interface effect zone in view of the local mixture-to-wall heat transfer coefficient.The maximum peak value of the mixture-to-wall heat transfer coefficient always appears at 210°of heat exchange tubes.When the orifice diameter is 4 mm,the axial gradient of gas holdup is relatively large due to more intense shearing and fragmentation effects.Interestingly,the fractions of medium-sized and large-sized bubbles are not sensitive to orifice angle.Both the mixture-to-wall heat transfer coefficient and the friction factor decrease initially and then increase when the installation height increases.Under the optimized gas sparger structure configuration,the mixture-to-wall heat transfer coefficient increases by 10.23%,accompanied by the reduction of pressure drop by 8.14%,ultimately attaining a system energy conversion efficiency of 97.88%and performance evaluation criterion of 1.087.Finally,a new dimensionless and semi-theoretical Nusselt correlation incorporating a structural correction factor with an average absolute deviation of 5.15%is developed.The findings can offer useful guidance for the optimal design of BCR TB.
基金National Natural Science Foundation of China(12135008,12132005)。
文摘The internal pressure within fission gas bubbles(FGBs)in irradiated nuclear fuels drives mechanical interactions with the surrounding fuel skeleton.To investigate the micromechanical stress fields in irradiated nuclear fuels containing pressurized FGBs,a mechanical constitutive model for the equivalent solid of FGBs was developed and validated.This model was based on the modified Van der Waals equation,incorporating the effects of surface tension.Using this model,the micromechanical fields in irradiated U-10Mo fuels with randomly distributed FGBs were calculated during uniaxial tensile testing via the finite element(FE)method.The macroscopic elastic constants of the irradiated U-10Mo fuels were then derived using homogenization theory,and the influences of bubble pressure,bubble size,and porosity on these constants were examined.Results show that adjacent FGBs exhibit mechanical interactions,which leads to distinct stress concentrations in the surrounding fuel skeleton.The macroscopic elastic constants of irradiated U-10Mo fuels decrease with increasing the macroscopic porosity,which can be quantitatively described by the Mori-Tanaka model.In contrast,bubble pressure and size have negligible effects on these constants.
基金supported by the Center of Excellence on Instru-mentation Technology and Automation(CEITA),Department of Instru-mentation and Electronics Engineering,Faculty of Engineering,King Mongkut’s University of Technology North Bangkok,Thailand。
文摘This study explores the combination of ultrasound technology with a detection algorithm to categorize flow regimes in bubble columns used for aeration in aquaculture.An ultrasonic velocity profiler is used to obtain the standard deviation of the bubble velocity distributed throughout the column.The bubble velocity data for three known flow regimes were used to develop a probability density function(PDF)classification model.The experimental apparatus consisted of a circular tank equipped with a bubble generator and gas hold-up monitoring systems.The flow regimes of the experimental fluid were determined,and the classification was conducted via the PDF method.The results demonstrate that the classification accuracy is not lower than that of traditional machine learning methods.