Timer error as well as its convention is very important for dose accuracy during irradiation. This paper determines the timer error of irradiators at Secondary Standard Dosimetry Laboratory (SSDL) in Nigeria. The irra...Timer error as well as its convention is very important for dose accuracy during irradiation. This paper determines the timer error of irradiators at Secondary Standard Dosimetry Laboratory (SSDL) in Nigeria. The irradiators are Cs-137 OB6 irradiator and X-ray irradiators at the Protection level SSDL;and Co-60 irradiator at the Therapy Level SSDL. PTW UNIDOS electrometer and LS01 Ionization chamber were used at the Protection Level to obtain doses for both Cs-137 OB6 and X-ray irradiators while an IBA farmer type ionization chamber and an IBA DOSE 1 electrometer were used at the Protection Level SSDL. Single/multiple exposure method and graphical method were used in the determination of the timer error for the three irradiators. The timer error obtained for Cs-137 OB6 irradiator was 0.48 ± 0.01 s, the timer error for the X-ray irradiator was 0.09 ± 0.01 s while the timer error obtained for GammaBeam X200 was 1.21 ± 0.04 s. It was observed that the timer error is not affected by source to detector distance. It was also observed that the timer error of Co-60 Gamma X200 irradiator is increasing with the age of the machine. Source to detector distance and field size do not contribute towards the timer error of the irradiators. The timer error of the Co-60 Gamma X200 irradiator (the only irradiator among the irradiators with a pneumatic system) increases with the age of the irradiator.展开更多
A Novel Dosimetry Method for Small Animal Irradiators Using 3D-printed Mouse Phantoms and Alanine Dosimeters.Christopher Duncan1,Chad Gunther1(1.C&C Irradiator Service,LLC,Washington,DC,20006.)Abstract:Accurate do...A Novel Dosimetry Method for Small Animal Irradiators Using 3D-printed Mouse Phantoms and Alanine Dosimeters.Christopher Duncan1,Chad Gunther1(1.C&C Irradiator Service,LLC,Washington,DC,20006.)Abstract:Accurate dosimetry is a crucial component of small animal and preclinical irradiation studies.展开更多
The effects ofγ-ray and electron irradiation on the microstructural evolution and mechanical properties of SnPb eutectic solder joints were investigated.Following electron irradiation,the SnO_(2)phase induced byγ-ra...The effects ofγ-ray and electron irradiation on the microstructural evolution and mechanical properties of SnPb eutectic solder joints were investigated.Following electron irradiation,the SnO_(2)phase induced byγ-ray irradiation transformed intoβ-Sn,and the dislocation density in theβ-Sn crystal decreased.Moreover,numerous point defect clusters formed in theβ-Sn crystal,some of which transformed into an amorphous phase,increasing the amorphous layer thickness.Meanwhile,electron irradiation likewise resulted in rotation of the(220)plane ofβ-Sn nanograins and reduction of SnO_(2)in theβ-Sn crystal.Additionally,upon exposure toγ-ray and electron irradiation,the average shear strength of the solder balls was initially increased by 10.10%,followed by a decrease of 3.53%and 4.77%,respectively.The plasticity and the dimple count on the fracture surfaces of the solder joint initially decreased but subsequently increased.展开更多
Single-crystal GaN epilayers were irradiated with heavy inert gas ions(2.3-MeV Ne^(8+),5.3-MeV Kr^(19+))to fluences ranging from 1.0×1.0^(11) to 1.0×1.0^(15)ions∕cm^(2).The strain-related damage accumulatio...Single-crystal GaN epilayers were irradiated with heavy inert gas ions(2.3-MeV Ne^(8+),5.3-MeV Kr^(19+))to fluences ranging from 1.0×1.0^(11) to 1.0×1.0^(15)ions∕cm^(2).The strain-related damage accumulation versus ion fluences was studied using highresolution X-ray diffraction(HRXRD)and ultraviolet–visible(UV–Vis)spectroscopy.The results showed that the damage accumulation was mainly dominated by nuclear energy loss.When the ion fluence was less than∼0.055 displacement per atom(dpa),the lattice expansions and lattice strains markedly increased linearly with increasing ion fluences,accompanied by a slow enhancement in the dislocation densities,distortion parameters,and Urbach energy for both ion irradiations.Above this fluence(∼0.055 dpa),the lattice strains presented a slight increase,whereas a remarkable increase was observed in the dislocation densities,distortion parameters,and Urbach energy with the ion fluences after both ion irradiations.∼0.055 dpa is the threshold ion fluence for defect evolution and lattice damage related to strain.The mechanisms underlying the damage accumulation are discussed in detail.展开更多
In this study,controllable fabrication of nickel-doped diamond-like carbon(Ni-DLC)films through laser-assisted electrochemical deposition under low-voltage conditions(5 V)is achieved.After substrate polishing,picoseco...In this study,controllable fabrication of nickel-doped diamond-like carbon(Ni-DLC)films through laser-assisted electrochemical deposition under low-voltage conditions(5 V)is achieved.After substrate polishing,picosecond laser irradiation is applied during electrodeposition to precisely control the laser energy and defocus distance during film preparation,with subsequent analysis of surface morphology,composition,and properties in correlation with growth mechanisms.Compared with conventional DLC electrodeposition,the laser-assisted technique significantly improves film quality by maintaining the deposition zone temperature at~52℃,with laser-induced micro-stirring effectively reducing cathode bubble adhesion and suppressing hydrogen evolution.Without laser assistance,the films exhibit poor adhesion,porous structure,and thickness nonuniformity,while increasing the laser energy progressively enhances densification,achieving 3.5μm thickness uniformity.Optimal performance at 8.5μJ laser energy demonstrates an improved deposition rate compared with conventional methods,a minimum corrosion current density(1.116×10^(−6)Amm^(−2)),and a stable friction coefficient(0.143),establishing a novel laser-assisted approach for controllable DLC electrodeposition.展开更多
This work presents a systematic analysis of proton-induced total ionizing dose(TID)effects in 1.2 k V silicon carbide(SiC)power devices with various edge termination structures.Three edge terminations including ring-a...This work presents a systematic analysis of proton-induced total ionizing dose(TID)effects in 1.2 k V silicon carbide(SiC)power devices with various edge termination structures.Three edge terminations including ring-assisted junction termination extension(RA-JTE),multiple floating zone JTE(MFZ-JTE),and field limiting rings(FLR)were fabricated and irradiated with45 Me V protons at fluences ranging from 1×10^(12) to 1×10^(14) cm^(-2).Experimental results,supported by TCAD simulations,show that the RA-JTE structure maintained stable breakdown performance with less than 1%variation due to its effective electric field redistribution by multiple P+rings.In contrast,MFZ-JTE and FLR exhibit breakdown voltage shifts of 6.1%and 15.2%,respectively,under the highest fluence.These results demonstrate the superior radiation tolerance of the RA-JTE structure under TID conditions and provide practical design guidance for radiation-hardened Si C power devices in space and other highradiation environments.展开更多
In this study,the dosimetric characteristics(thickness applicability,preheating time,temperature and humidity dependence,in-batch uniformity,readout reproducibility,dose linearity,self-decay,and electron energy respon...In this study,the dosimetric characteristics(thickness applicability,preheating time,temperature and humidity dependence,in-batch uniformity,readout reproducibility,dose linearity,self-decay,and electron energy response)of engineered polycarbonate films irradiated with an electron beam(0–600 kGy)were investigated using photoluminescence spectroscopy.The results show a linear relationship between photoluminescence intensity and radiation dose when the thickness of the polycarbonate film is 0.3 mm.A higher fluorescence intensity can be obtained by preheating at 60℃ for 180 min before photoluminescence spectrum analysis.As the temperature during spectral testing and the ambient humidity(during and after irradiation)increased,the photoluminescence intensity of the polycarbonate films decreased.The photoluminescence intensity deviation of the polycarbonate films produced within the same batch at 100 kGy is 2.73%.After ten times of repeated excitations and readouts,the coefficients of variation in photoluminescence intensity are less than 8.6%,and the linear correlation coefficient between photoluminescence intensity and irradiation dose is 0.965 in the dose capture range of 20–600 kGy.Within 60 days of irradiation,the photoluminescence intensity of the polycarbonate film decreased to 60%of the initial value.The response of the 0.3 mm polycarbonate films to electron beams with energies exceeding 3.5 MeV does not differ significantly.This comprehensive analysis indicates the potential of polycarbonate films as a high-radiation dose detection material.展开更多
The aerosolization and diffusion of radioactive materials caused by chemical explosions represent a typical nuclear accident scenario that poses severe radioactive hazards to human health and the environment.This stud...The aerosolization and diffusion of radioactive materials caused by chemical explosions represent a typical nuclear accident scenario that poses severe radioactive hazards to human health and the environment.This study examines the diffusion of plutonium aerosol generated by a chemical explosion within a typical representative underground facility.The state of explosion products following a single-point detonation of explosives was simulated.Subsequently,a numerical simulation of plutonium aerosol diffusion using the discrete phase model(DPM)was conducted based on the outcomes of the chemical explosion simulation.The simulation results indicate that plutonium aerosols diffuse throughout underground facilities after a chemical explosion;small particle size aerosols primarily accumulate in the upper part of the room after the accident;the concentrations of plutonium aerosol in the room and tunnel are significantly higher than those in the other areas;and the temporal variations in aerosol concentration in each area were quantified.Based on the particle concentration distribution and the effective dose computation approach,the study computes the internal irradiation dose received by personnel in seven areas over various time periods post-accident.Recommendations for emergency decision-making were derived from these calculations.These findings provide important theoretical insight and practical engineering application value for understanding the diffusion of radioactive aerosol in confined spaces following chemical explosions and for evaluating personnel radiation dose.展开更多
Under certain accident conditions in particle accelerators,high-power beam irradiation may damage vacuum pipes,magnets,and other key equipment.Therefore,machine protection for high-power accelerators is critical to en...Under certain accident conditions in particle accelerators,high-power beam irradiation may damage vacuum pipes,magnets,and other key equipment.Therefore,machine protection for high-power accelerators is critical to ensure safe operation.It is important to study radiation damage to materials to support the design and operation of machine protection systems.In the shock-wave regime,a pronounced hydrodynamic tunneling effect occurs within materials.The traditional one-way coupling simulation method results in substantial errors in this regime.Therefore,a bidirectional iterative coupling simulation method was developed.This method enables the bidirectional coupling of the Monte Carlo code FLUKA and the thermodynamic program Ansys-Autodyn.Density changes are monitored during the simulations,and the updated density is promptly fed back to FLUKA.The program remodels the target with the new density distribution to calculate the new energy deposition distribution,which is then returned to Autodyn for subsequent simulations.This iterative process continues until the entire beam has completed the energy deposition process.Compared to existing methods,this automated method significantly improves the efficiency of the coupled simulations and reduces the possibility of human error.The HRMT-12 beam irradiation experiment at CERN was used for a benchmark study,and simulations were conducted and compared using different equations of state.The results demonstrate the efficiency and accuracy of this simulation method.Compared to complex and costly beam irradiation experiments,this approach is expected to provide fast and cost-effective scientific guidance for the machine protection of high-power accelerators.Considering the severe consequences of the hydrodynamic tunneling effect,machine protection components such as beam collimators,absorbers,and dump blocks should adopt low-density materials to reduce the energy deposition density.Beam dilution may be required in beam dumping systems to avoid target damage.This method can be applied to the redundancy design of such beam dumping systems.展开更多
To address the poor mechanical performance and improve the tribological properties of self-lubricating polyphenylene sulfide/irradiation treated polytetrafluoroethylene(PPS/i-PTFE)blends,different aspect ratio carbon ...To address the poor mechanical performance and improve the tribological properties of self-lubricating polyphenylene sulfide/irradiation treated polytetrafluoroethylene(PPS/i-PTFE)blends,different aspect ratio carbon fibers(i.e.,PSCF:50,SCF:about 429)were introduced as reinforcement fillers.The results showed that the hybriding of PSCF and SCF at certain mass ratios exhibited simultaneous enhancement of mechanical and tribological performance for PPS/i-PTFE blend through the construction of synergistic lubrication and mechanical interlocking network.Specifically,the flexural strength and modulus of PPS/i-PTFE were increased by 125.6% and 389.3%,the friction coefficient and specific wear rate were decreased by 13.9% and 95%,respectively.It was worth noting that PPS composites possessed excellent integrated performance which were able to withstand sliding action under high PV(≥10 MPa·m/s)conditions,as assessed by a customized pin-on-disc tester.This work demonstrated that the formation of intact lubricating film combined with the enhanced thermal and mechanical properties were favorable for improving the tribological properties of PPS-based composites,which makes them suitable for advanced engineering applications.展开更多
High-Mach-number plasma jets have been extensively investigated in both astrophysical and laboratory contexts.In this work,we revisit the framework of magnetohydrodynamic(MHD)theory and introduce a new analytical appr...High-Mach-number plasma jets have been extensively investigated in both astrophysical and laboratory contexts.In this work,we revisit the framework of magnetohydrodynamic(MHD)theory and introduce a new analytical approach for examining plasma jets generated by intense laser-plasma interactions.Specifically,we reformulate the fundamental MHD equations to elucidate the governing factors of local plasma density evolution.Furthermore,MHD simulations of laser irradiation on planar targets demonstrate that impact pressure plays a dominant role in the propagation of high-Mach-number plasma jets.In addition,a pronounced dependence on the atomic number is identified:higher-Z materials amplify the impact pressure,suggesting that metallicity exerts a significant influence on the morphology and dynamics of astrophysical jets.展开更多
Conventional polyethylene(PE)fibers face limitations in large-scale industrial applications due to their poor thermal stability and inherent hydrophobicity,which restrict processing temperatures and dyeability,especia...Conventional polyethylene(PE)fibers face limitations in large-scale industrial applications due to their poor thermal stability and inherent hydrophobicity,which restrict processing temperatures and dyeability,especially in blended fabric production.In this research,a one-step ultraviolet(UV)irradiation technology was employed to modify medium molecular weight PE fibers through simultaneous crosslinking and grafting modifications,aiming to enhance their thermal stability and hydrophilicity.The modification employed a cost-effective,UV-initiated crosslinking system consisting of benzophenone(BP)as the photoinitiator and triallyl isocyanurate(TAIC)as the cocrosslinker.Acrylic acid(AA)was selected as the grafting monomer.These modifiers were thoroughly mixed with the PE matrix in a liquid-phase environment,and the mixture was melt-spun into fibers.The resulting fibers were then subjected to UV irradiation,which triggered the crosslinking and grafting reactions.The effects of the mass fraction of each component and irradiation parameters on modification efficacy were systematically investigated,followed by a comprehensive characterization of the modified PE fibers.The modified PE fibers achieved optimal thermal stability under the following conditions:2.0%mass fractions for both BP and TAIC,a UV irradiation intensity of 2000 mW/cm^(2),and an equivalent irradiation time of 60 s.This synergistic modification approach enables the fibers to maintain superior morphological integrity and mechanical performance when exposed to elevated temperatures ranging from 130 to 150℃.Meanwhile,an AA grafting mass fraction of 2.0%maximizes hydrophilicity with minimal impact on other properties,as evidenced by a dramatic reduction in the water contact angle(WCA)from 105.0°(hydrophobic)to 48.4°(hydrophilic).These improvements confirm the effectiveness of the modification strategy in synergistically enhancing both thermal stability and hydrophilicity of PE fibers.展开更多
The failure mechanisms and structural damage of SiC MOSFETs induced by heavy ion irradiation were demonstrated.The findings reveal three degradation modes,depending on the drain voltage.At a relatively low voltage,the...The failure mechanisms and structural damage of SiC MOSFETs induced by heavy ion irradiation were demonstrated.The findings reveal three degradation modes,depending on the drain voltage.At a relatively low voltage,the damage is triggered by the formation and activation of gate latent damage(LDs),with damage concentrated in the gate oxide.The second degradation mode involves permanent leakage current degradation,with damage progressively transitioning from the oxide to the SiC material as the drain voltage escalates.Ultimately,the device undergoes catastrophic burnout above certain voltages,characterized by the lattice temperature reaching the sublimation point of SiC,resulting in surface cavity and complete structural destruction.This paper presents a comprehensive investigation of SiC MOSFETs under heavy ion exposure,providing radiation resistance methods of SiC-based devices for aerospace applications.展开更多
Achieving uniform X-ray irradiation in indirect-drive inertial confinement fusion(ICF)is a key challenge for successful capsule implosion.Spherical hohlraums,particularly those with octahedral laser entrance holes(LEH...Achieving uniform X-ray irradiation in indirect-drive inertial confinement fusion(ICF)is a key challenge for successful capsule implosion.Spherical hohlraums,particularly those with octahedral laser entrance holes(LEHs),are an alternative to the cylindrical hohlraums currently considered for ICF at NIF(USA)and LMJ(France).These spherical hohlraums are advantageous in terms of irradiation uniformity on the fusion capsule because,owing to their octahedral symmetry,low-order asymmetries cancel out intrinsically.However,they may be less favorable from an energetic point of view,primarily owing to radiation losses through their multiple LEHs.The net balance of these advantages and disadvantages is difficult to determine,because,unlike cylindrical hohlraums,they require fully 3D modeling.To address this,a new version of the MULTI-3D simulation code has been developed.MULTI-3D is a 3D radiation-hydrodynamics code with arbitrary Langrangian-Eulerian(ALE)hydrodynamics,multigroup SN radiation transport,and ray-tracing laser deposition.Using this tool,several aspects of the behavior of spherical hohlraums have been analyzed,with special attention to phenomena inaccessible to 2D modeling.In these targets,laser beams strike the inner walls at very oblique angles,and the expansion of plasma significantly alters the locations where primary X rays are produced.Furthermore,the complex distribution of laser hot spots leads to mutual interactions,where plasma bubbles from one beam intersect the path of another.The laser-to-X-ray energy conversion efficiency has been analyzed as a function of key parameters.The symmetry on the capsule has also been evaluated,revealing nonuniformities of less than 1%.展开更多
Inertial confinement fusion(ICF)requires a constant search for the most effective materials to improve the efficiency of compression of the capsule and of laser-to-target energy transfer.Foams could provide a solution...Inertial confinement fusion(ICF)requires a constant search for the most effective materials to improve the efficiency of compression of the capsule and of laser-to-target energy transfer.Foams could provide a solution,but they require further experimental and theoretical investigation.The new 3D-printing technologies,such as two-photon polymerization,are opening a new era in the production of foams,allowing fine control of material morphology.Very few detailed studies of the interaction of foams with high-power lasers in regimes relevant for ICF have been described in the literature to date,and more investigation is needed.In this work,we present the results of an experimental campaign performed at the ABC laser facility at ENEA Centro Ricerche Frascati in which 3D-printed microstructured materials were irradiated at high power.3D simulations of the laser-target interaction performed with the FLASH code reveal that the laser is scattered by plasma density gradients and channeled into the structure when the center of the focal spot is on the through hole.The time required for the laser to completely ablate the structure given by the simulations is in good agreement with the experimental measurement.Measurements of the reflected and transmitted laser light indicate that scattering occurred during the irradiation,in accordance with the simulations.Two-plasmon decay has also been found to be active during irradiation.展开更多
Satellite remote sensing is essential for solar energy meteorology.The 14-channel Advanced Geostationary Radiation Imager of the Fengyun-4 series of satellites performs a full-disc scan over greater China every 15 min...Satellite remote sensing is essential for solar energy meteorology.The 14-channel Advanced Geostationary Radiation Imager of the Fengyun-4 series of satellites performs a full-disc scan over greater China every 15 min,providing highgranularity information that allows the retrieval of cloud properties,aerosol optical depth,and precipitable water vapor content,which can facilitate the acquisition of surface solar irradiance components through physical methods.Machinelearning methods have also shown potential in providing accurate end-to-end surface solar radiation retrievals.Albeit the physical principles of irradiance retrieval and machine-learning algorithms are fairly well known,the public service concerning disseminating the irradiance product to the energy and power industry still lacks robustness and consistency.In this perspective article,the status quo of Fengyun-4 irradiance products is first reviewed.Then,from the perspective of solar resource assessment and forecasting,three fundamental characteristics of the kind of irradiance products that are most serviceable to the solar energy sector are identified,namely,coverage,timeliness,and accessibility.Finally,an outlook on the new-generation Fengyun radiation service is put forward,and the prospective scientific and practical challenges are elaborated.展开更多
The removal of ammonia nitrogen(NH_(4)^(+)-N)and bacteria from aquaculture wastewater holds paramount ecological and production significance.In this study,Pt/RuO_(2)/g-C_(3)N_(4)photocatalysts were prepared by deposit...The removal of ammonia nitrogen(NH_(4)^(+)-N)and bacteria from aquaculture wastewater holds paramount ecological and production significance.In this study,Pt/RuO_(2)/g-C_(3)N_(4)photocatalysts were prepared by depositing Pt and RuO_(2)particles onto g-C_(3)N_(4).The physicochemical properties of photocatalysts were explored by X-ray photoelectron spectroscopy(XPS),scanning electron microscopy(SEM),X-ray diffraction(XRD),and UV–vis diffuse reflectance spectrometer(UV–vis DRS).The photocatalysts were then applied to the removal of both NH_(4)^(+)-N and bacteria from simulated mariculture wastewater.The results clarified that the removals of both NH_(4)^(+)-N and bacteria were in the sequence of g-C_(3)N_(4)<RuO_(2)/g-C_(3)N_(4)<Pt/g-C_(3)N_(4)<Pt/RuO_(2)/g-C_(3)N_(4).This magnificent photocatalytic ability of Pt/RuO_(2)/g-C_(3)N_(4)can be interpreted by the transfer of holes from g-C_(3)N_(4)to RuO_(2)to facilitate the in situ generation of HClO from Cl^(−)in wastewater,while Pt extracts photogenerated electrons for H_(2)formation to enhance the reaction.The removal of NH_(4)^(+)-N and disinfection effect were more pronounced in simulated seawater than in purewater.The removal efficiency ofNH_(4)^(+)-N increases with an increase in pH of wastewater,while the bactericidal effect was more significant under a lower pH in a pH range of 6–9.In actual seawater aquaculture wastewater,Pt/RuO_(2)/g-C_(3)N_(4)still exhibits effective removal efficiency of NH_(4)^(+)-N and bactericidal performance under sunlight.This study provides an alternative avenue for removement of NH_(4)^(+)-N and bacteria from saline waters under sunlight.展开更多
The Mg alloys with combination of high strength and excellent irradiation resistance are currently re-quired for research reactors.In this work,the novel Mg-3Mn-0.5Ca alloy with a high strength of over 300 MPa has bee...The Mg alloys with combination of high strength and excellent irradiation resistance are currently re-quired for research reactors.In this work,the novel Mg-3Mn-0.5Ca alloy with a high strength of over 300 MPa has been fabricated via co-addition of Mn and Ca elements.Moreover,the Xe ion implantation(300℃/4.5×10^(15)ions/cm^(2))is conducted for pure Mg,Mg-3Mn and Mg-3Mn-0.5Ca alloys.Microstruc-ture characterization shows that the number density of dislocation loops is comparable between Mg-3Mn and pure Mg,while the phase boundary of nano-Mn particles could act as the sink to absorb more Xe atoms,resulting in the abundant formation of Xe bubbles in the matrix of irradiated Mg-3Mn alloy.With further minor addition of Ca element,the formation of Xe bubbles and dislocation loops in Mg-3Mn-0.5Ca alloy has been obviously suppressed,and the abundant grain boundaries(GBs)due to grain refinement then act as the sink region for Xe precipitation.The limited number density of Xe bubbles leads to the extremely low swelling ratio in Mg-3Mn-0.5Ca alloy,∼0.08%.The result above suggests that the Mn and Ca co-addition could enhance the mechanical properties and irradiation tolerance of Mg alloys,si-multaneously.The present low-alloying strategy would provide a new design reference for novel nuclear materials.展开更多
Establishing Consensus with Users of Research Irradiator Devices to Facilitate Source Type Replacement Danette R.Fennesy1,Janet M.Gutiérrez1,2,Scott J.Patlovich1,Robert J.Emery1(1.The University of Texas Health S...Establishing Consensus with Users of Research Irradiator Devices to Facilitate Source Type Replacement Danette R.Fennesy1,Janet M.Gutiérrez1,2,Scott J.Patlovich1,Robert J.Emery1(1.The University of Texas Health Science Center at Houston,Environmental Health&Safety,6431 Fannin St,CYF G.102,Houston,TX,77030;2.Corresponding author)Abstract:The ability to irradiate cells,tissues,and other biological materials with high-energy photons has been an essential tool in the discovery of numerous biomedical research advancements.展开更多
On the surfaces of celestial bodies with no or thin atmospheres,such as the Moon and Mars,the solar wind irradiation process leads to the formation of hydrogen and helium enriched regions in the extraterrestrial soil ...On the surfaces of celestial bodies with no or thin atmospheres,such as the Moon and Mars,the solar wind irradiation process leads to the formation of hydrogen and helium enriched regions in the extraterrestrial soil particles.However,soil particles on the Earth with the similar composition lack such structures and properties.This discrepancy raises a key question whether there is a direct relationship between solar wind irradiation and the alterations in the structure and chemical performance of extraterrestrial materials.To address this question,this work investigates the effects of proton irradiation,simulating solar wind radiation,on the structure and photothermal catalytic properties of the classic catalyst In_(2)O_(3).It reveals that proton irradiation induces structural features in In_(2)O_(3) analogous to those characteristics of solar wind weathering observed in extraterrestrial materials.Furthermore,after proton beam irradiation with an energy of 30 keV and a dose of 3×10^(17) protons·cm^(-2),the methanol production yield of the In_(2)O_(3) catalyst increased to 2.6 times of its preirradiation level,and the methanol selectivity improved to 2.1 times of the original value.This work provides both theoretical and experimental support for the development of high-efficiency,radiation-resistant photothermal catalysts.展开更多
文摘Timer error as well as its convention is very important for dose accuracy during irradiation. This paper determines the timer error of irradiators at Secondary Standard Dosimetry Laboratory (SSDL) in Nigeria. The irradiators are Cs-137 OB6 irradiator and X-ray irradiators at the Protection level SSDL;and Co-60 irradiator at the Therapy Level SSDL. PTW UNIDOS electrometer and LS01 Ionization chamber were used at the Protection Level to obtain doses for both Cs-137 OB6 and X-ray irradiators while an IBA farmer type ionization chamber and an IBA DOSE 1 electrometer were used at the Protection Level SSDL. Single/multiple exposure method and graphical method were used in the determination of the timer error for the three irradiators. The timer error obtained for Cs-137 OB6 irradiator was 0.48 ± 0.01 s, the timer error for the X-ray irradiator was 0.09 ± 0.01 s while the timer error obtained for GammaBeam X200 was 1.21 ± 0.04 s. It was observed that the timer error is not affected by source to detector distance. It was also observed that the timer error of Co-60 Gamma X200 irradiator is increasing with the age of the machine. Source to detector distance and field size do not contribute towards the timer error of the irradiators. The timer error of the Co-60 Gamma X200 irradiator (the only irradiator among the irradiators with a pneumatic system) increases with the age of the irradiator.
文摘A Novel Dosimetry Method for Small Animal Irradiators Using 3D-printed Mouse Phantoms and Alanine Dosimeters.Christopher Duncan1,Chad Gunther1(1.C&C Irradiator Service,LLC,Washington,DC,20006.)Abstract:Accurate dosimetry is a crucial component of small animal and preclinical irradiation studies.
基金financially supported by the National Natural Science Foundation of China Young Student Basic Research Program(for Ph.D.students)(No.525B2069)the Fundamental Research Funds for the Central Universities,China(No.HIT.DZJJ.2025005)the National Key Laboratory of Precision Welding&Joining of Materials and Structures Research Project,China(No.24-Z-09)。
文摘The effects ofγ-ray and electron irradiation on the microstructural evolution and mechanical properties of SnPb eutectic solder joints were investigated.Following electron irradiation,the SnO_(2)phase induced byγ-ray irradiation transformed intoβ-Sn,and the dislocation density in theβ-Sn crystal decreased.Moreover,numerous point defect clusters formed in theβ-Sn crystal,some of which transformed into an amorphous phase,increasing the amorphous layer thickness.Meanwhile,electron irradiation likewise resulted in rotation of the(220)plane ofβ-Sn nanograins and reduction of SnO_(2)in theβ-Sn crystal.Additionally,upon exposure toγ-ray and electron irradiation,the average shear strength of the solder balls was initially increased by 10.10%,followed by a decrease of 3.53%and 4.77%,respectively.The plasticity and the dimple count on the fracture surfaces of the solder joint initially decreased but subsequently increased.
基金supported by the Program for National Natural Science Foundation of China(No.11675231)the Sichuan Science and Technology Program(Nos.2022YFG0263 and 2024NSFSC1097)the Scientific Research Starting Foundation for talents(Nos.21zx7109 and 22zx7175,24ycx1005).
文摘Single-crystal GaN epilayers were irradiated with heavy inert gas ions(2.3-MeV Ne^(8+),5.3-MeV Kr^(19+))to fluences ranging from 1.0×1.0^(11) to 1.0×1.0^(15)ions∕cm^(2).The strain-related damage accumulation versus ion fluences was studied using highresolution X-ray diffraction(HRXRD)and ultraviolet–visible(UV–Vis)spectroscopy.The results showed that the damage accumulation was mainly dominated by nuclear energy loss.When the ion fluence was less than∼0.055 displacement per atom(dpa),the lattice expansions and lattice strains markedly increased linearly with increasing ion fluences,accompanied by a slow enhancement in the dislocation densities,distortion parameters,and Urbach energy for both ion irradiations.Above this fluence(∼0.055 dpa),the lattice strains presented a slight increase,whereas a remarkable increase was observed in the dislocation densities,distortion parameters,and Urbach energy with the ion fluences after both ion irradiations.∼0.055 dpa is the threshold ion fluence for defect evolution and lattice damage related to strain.The mechanisms underlying the damage accumulation are discussed in detail.
基金supported by the National Natural Science Foundation of China(Grant Nos.52275431 and 52075227).
文摘In this study,controllable fabrication of nickel-doped diamond-like carbon(Ni-DLC)films through laser-assisted electrochemical deposition under low-voltage conditions(5 V)is achieved.After substrate polishing,picosecond laser irradiation is applied during electrodeposition to precisely control the laser energy and defocus distance during film preparation,with subsequent analysis of surface morphology,composition,and properties in correlation with growth mechanisms.Compared with conventional DLC electrodeposition,the laser-assisted technique significantly improves film quality by maintaining the deposition zone temperature at~52℃,with laser-induced micro-stirring effectively reducing cathode bubble adhesion and suppressing hydrogen evolution.Without laser assistance,the films exhibit poor adhesion,porous structure,and thickness nonuniformity,while increasing the laser energy progressively enhances densification,achieving 3.5μm thickness uniformity.Optimal performance at 8.5μJ laser energy demonstrates an improved deposition rate compared with conventional methods,a minimum corrosion current density(1.116×10^(−6)Amm^(−2)),and a stable friction coefficient(0.143),establishing a novel laser-assisted approach for controllable DLC electrodeposition.
基金supported by the IITP(Institute for Information&Communications Technology Planning&Evaluation)under the ITRC(Information Technology Research Center)support program(IITP-2025-RS-2024-00438288)grant funded by the Korea government(MSIT)+1 种基金National Research Council of Science&Technology(NST)grant by the MSIT(Aerospace Semiconductor Strategy Research Project No.GTL25051-000)supported by the IC Design Education Center(IDEC),Korea。
文摘This work presents a systematic analysis of proton-induced total ionizing dose(TID)effects in 1.2 k V silicon carbide(SiC)power devices with various edge termination structures.Three edge terminations including ring-assisted junction termination extension(RA-JTE),multiple floating zone JTE(MFZ-JTE),and field limiting rings(FLR)were fabricated and irradiated with45 Me V protons at fluences ranging from 1×10^(12) to 1×10^(14) cm^(-2).Experimental results,supported by TCAD simulations,show that the RA-JTE structure maintained stable breakdown performance with less than 1%variation due to its effective electric field redistribution by multiple P+rings.In contrast,MFZ-JTE and FLR exhibit breakdown voltage shifts of 6.1%and 15.2%,respectively,under the highest fluence.These results demonstrate the superior radiation tolerance of the RA-JTE structure under TID conditions and provide practical design guidance for radiation-hardened Si C power devices in space and other highradiation environments.
基金supported by the National Natural Science Foundation of China(No.12305385)Key Projects of Scientific Research of the Hunan Provincial Department of Education(22A0310)the Research Startup Project of University of South China(220XQD025).
文摘In this study,the dosimetric characteristics(thickness applicability,preheating time,temperature and humidity dependence,in-batch uniformity,readout reproducibility,dose linearity,self-decay,and electron energy response)of engineered polycarbonate films irradiated with an electron beam(0–600 kGy)were investigated using photoluminescence spectroscopy.The results show a linear relationship between photoluminescence intensity and radiation dose when the thickness of the polycarbonate film is 0.3 mm.A higher fluorescence intensity can be obtained by preheating at 60℃ for 180 min before photoluminescence spectrum analysis.As the temperature during spectral testing and the ambient humidity(during and after irradiation)increased,the photoluminescence intensity of the polycarbonate films decreased.The photoluminescence intensity deviation of the polycarbonate films produced within the same batch at 100 kGy is 2.73%.After ten times of repeated excitations and readouts,the coefficients of variation in photoluminescence intensity are less than 8.6%,and the linear correlation coefficient between photoluminescence intensity and irradiation dose is 0.965 in the dose capture range of 20–600 kGy.Within 60 days of irradiation,the photoluminescence intensity of the polycarbonate film decreased to 60%of the initial value.The response of the 0.3 mm polycarbonate films to electron beams with energies exceeding 3.5 MeV does not differ significantly.This comprehensive analysis indicates the potential of polycarbonate films as a high-radiation dose detection material.
文摘The aerosolization and diffusion of radioactive materials caused by chemical explosions represent a typical nuclear accident scenario that poses severe radioactive hazards to human health and the environment.This study examines the diffusion of plutonium aerosol generated by a chemical explosion within a typical representative underground facility.The state of explosion products following a single-point detonation of explosives was simulated.Subsequently,a numerical simulation of plutonium aerosol diffusion using the discrete phase model(DPM)was conducted based on the outcomes of the chemical explosion simulation.The simulation results indicate that plutonium aerosols diffuse throughout underground facilities after a chemical explosion;small particle size aerosols primarily accumulate in the upper part of the room after the accident;the concentrations of plutonium aerosol in the room and tunnel are significantly higher than those in the other areas;and the temporal variations in aerosol concentration in each area were quantified.Based on the particle concentration distribution and the effective dose computation approach,the study computes the internal irradiation dose received by personnel in seven areas over various time periods post-accident.Recommendations for emergency decision-making were derived from these calculations.These findings provide important theoretical insight and practical engineering application value for understanding the diffusion of radioactive aerosol in confined spaces following chemical explosions and for evaluating personnel radiation dose.
基金supported by the National Natural Science Foundation of China(No.12275196)。
文摘Under certain accident conditions in particle accelerators,high-power beam irradiation may damage vacuum pipes,magnets,and other key equipment.Therefore,machine protection for high-power accelerators is critical to ensure safe operation.It is important to study radiation damage to materials to support the design and operation of machine protection systems.In the shock-wave regime,a pronounced hydrodynamic tunneling effect occurs within materials.The traditional one-way coupling simulation method results in substantial errors in this regime.Therefore,a bidirectional iterative coupling simulation method was developed.This method enables the bidirectional coupling of the Monte Carlo code FLUKA and the thermodynamic program Ansys-Autodyn.Density changes are monitored during the simulations,and the updated density is promptly fed back to FLUKA.The program remodels the target with the new density distribution to calculate the new energy deposition distribution,which is then returned to Autodyn for subsequent simulations.This iterative process continues until the entire beam has completed the energy deposition process.Compared to existing methods,this automated method significantly improves the efficiency of the coupled simulations and reduces the possibility of human error.The HRMT-12 beam irradiation experiment at CERN was used for a benchmark study,and simulations were conducted and compared using different equations of state.The results demonstrate the efficiency and accuracy of this simulation method.Compared to complex and costly beam irradiation experiments,this approach is expected to provide fast and cost-effective scientific guidance for the machine protection of high-power accelerators.Considering the severe consequences of the hydrodynamic tunneling effect,machine protection components such as beam collimators,absorbers,and dump blocks should adopt low-density materials to reduce the energy deposition density.Beam dilution may be required in beam dumping systems to avoid target damage.This method can be applied to the redundancy design of such beam dumping systems.
基金financially supported by the National Natural Science Foundation of China(No.52103040)China Postdoctoral Science Foundation(No.2020M673217)the Fundamental Research Funds for the Central Universities(No.2023SCU12022)。
文摘To address the poor mechanical performance and improve the tribological properties of self-lubricating polyphenylene sulfide/irradiation treated polytetrafluoroethylene(PPS/i-PTFE)blends,different aspect ratio carbon fibers(i.e.,PSCF:50,SCF:about 429)were introduced as reinforcement fillers.The results showed that the hybriding of PSCF and SCF at certain mass ratios exhibited simultaneous enhancement of mechanical and tribological performance for PPS/i-PTFE blend through the construction of synergistic lubrication and mechanical interlocking network.Specifically,the flexural strength and modulus of PPS/i-PTFE were increased by 125.6% and 389.3%,the friction coefficient and specific wear rate were decreased by 13.9% and 95%,respectively.It was worth noting that PPS composites possessed excellent integrated performance which were able to withstand sliding action under high PV(≥10 MPa·m/s)conditions,as assessed by a customized pin-on-disc tester.This work demonstrated that the formation of intact lubricating film combined with the enhanced thermal and mechanical properties were favorable for improving the tribological properties of PPS-based composites,which makes them suitable for advanced engineering applications.
基金supported by the National Natural Science Foundation of China(Grant Nos.12325305,12175018,and 12135001)the National Key RD Program of China(Grant Nos.2022YFA1603200 and 2022YFA1603203).
文摘High-Mach-number plasma jets have been extensively investigated in both astrophysical and laboratory contexts.In this work,we revisit the framework of magnetohydrodynamic(MHD)theory and introduce a new analytical approach for examining plasma jets generated by intense laser-plasma interactions.Specifically,we reformulate the fundamental MHD equations to elucidate the governing factors of local plasma density evolution.Furthermore,MHD simulations of laser irradiation on planar targets demonstrate that impact pressure plays a dominant role in the propagation of high-Mach-number plasma jets.In addition,a pronounced dependence on the atomic number is identified:higher-Z materials amplify the impact pressure,suggesting that metallicity exerts a significant influence on the morphology and dynamics of astrophysical jets.
文摘Conventional polyethylene(PE)fibers face limitations in large-scale industrial applications due to their poor thermal stability and inherent hydrophobicity,which restrict processing temperatures and dyeability,especially in blended fabric production.In this research,a one-step ultraviolet(UV)irradiation technology was employed to modify medium molecular weight PE fibers through simultaneous crosslinking and grafting modifications,aiming to enhance their thermal stability and hydrophilicity.The modification employed a cost-effective,UV-initiated crosslinking system consisting of benzophenone(BP)as the photoinitiator and triallyl isocyanurate(TAIC)as the cocrosslinker.Acrylic acid(AA)was selected as the grafting monomer.These modifiers were thoroughly mixed with the PE matrix in a liquid-phase environment,and the mixture was melt-spun into fibers.The resulting fibers were then subjected to UV irradiation,which triggered the crosslinking and grafting reactions.The effects of the mass fraction of each component and irradiation parameters on modification efficacy were systematically investigated,followed by a comprehensive characterization of the modified PE fibers.The modified PE fibers achieved optimal thermal stability under the following conditions:2.0%mass fractions for both BP and TAIC,a UV irradiation intensity of 2000 mW/cm^(2),and an equivalent irradiation time of 60 s.This synergistic modification approach enables the fibers to maintain superior morphological integrity and mechanical performance when exposed to elevated temperatures ranging from 130 to 150℃.Meanwhile,an AA grafting mass fraction of 2.0%maximizes hydrophilicity with minimal impact on other properties,as evidenced by a dramatic reduction in the water contact angle(WCA)from 105.0°(hydrophobic)to 48.4°(hydrophilic).These improvements confirm the effectiveness of the modification strategy in synergistically enhancing both thermal stability and hydrophilicity of PE fibers.
基金Project supported by the National Key Research and Development Program of China(Grant No.2023YFA1609000)the National Natural Science Foundation of China(Grant Nos.U2341222,U2441248,12275061,and 12075069)。
文摘The failure mechanisms and structural damage of SiC MOSFETs induced by heavy ion irradiation were demonstrated.The findings reveal three degradation modes,depending on the drain voltage.At a relatively low voltage,the damage is triggered by the formation and activation of gate latent damage(LDs),with damage concentrated in the gate oxide.The second degradation mode involves permanent leakage current degradation,with damage progressively transitioning from the oxide to the SiC material as the drain voltage escalates.Ultimately,the device undergoes catastrophic burnout above certain voltages,characterized by the lattice temperature reaching the sublimation point of SiC,resulting in surface cavity and complete structural destruction.This paper presents a comprehensive investigation of SiC MOSFETs under heavy ion exposure,providing radiation resistance methods of SiC-based devices for aerospace applications.
基金supported by the Project Nos.PID2022-137339OB-C22 of the“Plan Estatal 2021-2023R”of the Spanish Government and ENR-IFE.01.CEA of EUROFUSION.
文摘Achieving uniform X-ray irradiation in indirect-drive inertial confinement fusion(ICF)is a key challenge for successful capsule implosion.Spherical hohlraums,particularly those with octahedral laser entrance holes(LEHs),are an alternative to the cylindrical hohlraums currently considered for ICF at NIF(USA)and LMJ(France).These spherical hohlraums are advantageous in terms of irradiation uniformity on the fusion capsule because,owing to their octahedral symmetry,low-order asymmetries cancel out intrinsically.However,they may be less favorable from an energetic point of view,primarily owing to radiation losses through their multiple LEHs.The net balance of these advantages and disadvantages is difficult to determine,because,unlike cylindrical hohlraums,they require fully 3D modeling.To address this,a new version of the MULTI-3D simulation code has been developed.MULTI-3D is a 3D radiation-hydrodynamics code with arbitrary Langrangian-Eulerian(ALE)hydrodynamics,multigroup SN radiation transport,and ray-tracing laser deposition.Using this tool,several aspects of the behavior of spherical hohlraums have been analyzed,with special attention to phenomena inaccessible to 2D modeling.In these targets,laser beams strike the inner walls at very oblique angles,and the expansion of plasma significantly alters the locations where primary X rays are produced.Furthermore,the complex distribution of laser hot spots leads to mutual interactions,where plasma bubbles from one beam intersect the path of another.The laser-to-X-ray energy conversion efficiency has been analyzed as a function of key parameters.The symmetry on the capsule has also been evaluated,revealing nonuniformities of less than 1%.
基金framework of the EUROfusion Consortium,funded by the European Union via the Euratom Research and Training Programme(Grant Agreement No.101052200—EUROfusion)The CRESCO-ENEAGRID High Performance Computing infrastructure is funded by ENEA+3 种基金the Italian National Agency for New Technologies,Energy and Sustainable Economic Developmentby Italian and European research programmesthe framework of the“Universities’Excellence Initiative”programme by the Ministry of Education,Science and Sports of the Republic of Lithuania under an agreement with the Research Council of Lithuania(Project No.S-A-UEI-23-6)support was received through EU LASERLAB-EUROPE JRAextension(Grant Agreement No.871124,Horizon 2020 Research and Innovation Programme).
文摘Inertial confinement fusion(ICF)requires a constant search for the most effective materials to improve the efficiency of compression of the capsule and of laser-to-target energy transfer.Foams could provide a solution,but they require further experimental and theoretical investigation.The new 3D-printing technologies,such as two-photon polymerization,are opening a new era in the production of foams,allowing fine control of material morphology.Very few detailed studies of the interaction of foams with high-power lasers in regimes relevant for ICF have been described in the literature to date,and more investigation is needed.In this work,we present the results of an experimental campaign performed at the ABC laser facility at ENEA Centro Ricerche Frascati in which 3D-printed microstructured materials were irradiated at high power.3D simulations of the laser-target interaction performed with the FLASH code reveal that the laser is scattered by plasma density gradients and channeled into the structure when the center of the focal spot is on the through hole.The time required for the laser to completely ablate the structure given by the simulations is in good agreement with the experimental measurement.Measurements of the reflected and transmitted laser light indicate that scattering occurred during the irradiation,in accordance with the simulations.Two-plasmon decay has also been found to be active during irradiation.
基金supported by the National Natural Science Foundation of China(project no.42375192)。
文摘Satellite remote sensing is essential for solar energy meteorology.The 14-channel Advanced Geostationary Radiation Imager of the Fengyun-4 series of satellites performs a full-disc scan over greater China every 15 min,providing highgranularity information that allows the retrieval of cloud properties,aerosol optical depth,and precipitable water vapor content,which can facilitate the acquisition of surface solar irradiance components through physical methods.Machinelearning methods have also shown potential in providing accurate end-to-end surface solar radiation retrievals.Albeit the physical principles of irradiance retrieval and machine-learning algorithms are fairly well known,the public service concerning disseminating the irradiance product to the energy and power industry still lacks robustness and consistency.In this perspective article,the status quo of Fengyun-4 irradiance products is first reviewed.Then,from the perspective of solar resource assessment and forecasting,three fundamental characteristics of the kind of irradiance products that are most serviceable to the solar energy sector are identified,namely,coverage,timeliness,and accessibility.Finally,an outlook on the new-generation Fengyun radiation service is put forward,and the prospective scientific and practical challenges are elaborated.
基金supported by the Science and Technology Planning Project of Fujian Province(No.2023Y4015)the Marine and Fishery Development Special Fund of Xiamen(No.23YYST064QCB36)the Natural Science Foundation of Fujian Province(No.2021J011210).
文摘The removal of ammonia nitrogen(NH_(4)^(+)-N)and bacteria from aquaculture wastewater holds paramount ecological and production significance.In this study,Pt/RuO_(2)/g-C_(3)N_(4)photocatalysts were prepared by depositing Pt and RuO_(2)particles onto g-C_(3)N_(4).The physicochemical properties of photocatalysts were explored by X-ray photoelectron spectroscopy(XPS),scanning electron microscopy(SEM),X-ray diffraction(XRD),and UV–vis diffuse reflectance spectrometer(UV–vis DRS).The photocatalysts were then applied to the removal of both NH_(4)^(+)-N and bacteria from simulated mariculture wastewater.The results clarified that the removals of both NH_(4)^(+)-N and bacteria were in the sequence of g-C_(3)N_(4)<RuO_(2)/g-C_(3)N_(4)<Pt/g-C_(3)N_(4)<Pt/RuO_(2)/g-C_(3)N_(4).This magnificent photocatalytic ability of Pt/RuO_(2)/g-C_(3)N_(4)can be interpreted by the transfer of holes from g-C_(3)N_(4)to RuO_(2)to facilitate the in situ generation of HClO from Cl^(−)in wastewater,while Pt extracts photogenerated electrons for H_(2)formation to enhance the reaction.The removal of NH_(4)^(+)-N and disinfection effect were more pronounced in simulated seawater than in purewater.The removal efficiency ofNH_(4)^(+)-N increases with an increase in pH of wastewater,while the bactericidal effect was more significant under a lower pH in a pH range of 6–9.In actual seawater aquaculture wastewater,Pt/RuO_(2)/g-C_(3)N_(4)still exhibits effective removal efficiency of NH_(4)^(+)-N and bactericidal performance under sunlight.This study provides an alternative avenue for removement of NH_(4)^(+)-N and bacteria from saline waters under sunlight.
基金the National Natural Science Foun-dation of China(Nos.U2241235,U2167213 and U2067218)the Project funded by the Science&Technology Department of Sichuan Province(No.21MZGC0400,No.2022JDJQ0021)+3 种基金the China National Nuclear Corporation(CNNC)Science Fund for Talented Young Scholars(No.CNNC-2021-31)the Funds of Science and Technol-ogy on Reactor Fuel and Materials Laboratory(No.6142A06190510)the fund from the Fundamental Research Funds for the Cen-tral Universities(No.N2202020)XingLiao Talent Plan(No.XLYC2203202).
文摘The Mg alloys with combination of high strength and excellent irradiation resistance are currently re-quired for research reactors.In this work,the novel Mg-3Mn-0.5Ca alloy with a high strength of over 300 MPa has been fabricated via co-addition of Mn and Ca elements.Moreover,the Xe ion implantation(300℃/4.5×10^(15)ions/cm^(2))is conducted for pure Mg,Mg-3Mn and Mg-3Mn-0.5Ca alloys.Microstruc-ture characterization shows that the number density of dislocation loops is comparable between Mg-3Mn and pure Mg,while the phase boundary of nano-Mn particles could act as the sink to absorb more Xe atoms,resulting in the abundant formation of Xe bubbles in the matrix of irradiated Mg-3Mn alloy.With further minor addition of Ca element,the formation of Xe bubbles and dislocation loops in Mg-3Mn-0.5Ca alloy has been obviously suppressed,and the abundant grain boundaries(GBs)due to grain refinement then act as the sink region for Xe precipitation.The limited number density of Xe bubbles leads to the extremely low swelling ratio in Mg-3Mn-0.5Ca alloy,∼0.08%.The result above suggests that the Mn and Ca co-addition could enhance the mechanical properties and irradiation tolerance of Mg alloys,si-multaneously.The present low-alloying strategy would provide a new design reference for novel nuclear materials.
文摘Establishing Consensus with Users of Research Irradiator Devices to Facilitate Source Type Replacement Danette R.Fennesy1,Janet M.Gutiérrez1,2,Scott J.Patlovich1,Robert J.Emery1(1.The University of Texas Health Science Center at Houston,Environmental Health&Safety,6431 Fannin St,CYF G.102,Houston,TX,77030;2.Corresponding author)Abstract:The ability to irradiate cells,tissues,and other biological materials with high-energy photons has been an essential tool in the discovery of numerous biomedical research advancements.
基金National Key Research and Development Program of China(2020YFA0710302)The Major Research Plan of the National Natural Science Foundation of China(91963206)+2 种基金The National Natural Science Foundation of China(52072169,51972164,51972167,22279053)The Fundamental Research Funds for the Central Universities(14380193)The Program for Guangdong Introducing Innovative and Entrepreneurial Teams(2019ZT08L101).
文摘On the surfaces of celestial bodies with no or thin atmospheres,such as the Moon and Mars,the solar wind irradiation process leads to the formation of hydrogen and helium enriched regions in the extraterrestrial soil particles.However,soil particles on the Earth with the similar composition lack such structures and properties.This discrepancy raises a key question whether there is a direct relationship between solar wind irradiation and the alterations in the structure and chemical performance of extraterrestrial materials.To address this question,this work investigates the effects of proton irradiation,simulating solar wind radiation,on the structure and photothermal catalytic properties of the classic catalyst In_(2)O_(3).It reveals that proton irradiation induces structural features in In_(2)O_(3) analogous to those characteristics of solar wind weathering observed in extraterrestrial materials.Furthermore,after proton beam irradiation with an energy of 30 keV and a dose of 3×10^(17) protons·cm^(-2),the methanol production yield of the In_(2)O_(3) catalyst increased to 2.6 times of its preirradiation level,and the methanol selectivity improved to 2.1 times of the original value.This work provides both theoretical and experimental support for the development of high-efficiency,radiation-resistant photothermal catalysts.
