Rapid and robust identification of bacteria is crucial for environmental monitoring and clinical diagnosis.Herein,a bioinspired interface-mediated multichannel sensor array was developed based on three-coloremitting a...Rapid and robust identification of bacteria is crucial for environmental monitoring and clinical diagnosis.Herein,a bioinspired interface-mediated multichannel sensor array was developed based on three-coloremitting antimicrobial functional carbon dots(FCDs)and concanavalin A doped polydopamine nanoparticles(Con A-PDA)for identification of bacteria.In this sensor,the fluorescence intensity of the three FCDs was quenched by the Con A-PDA.Upon addition different types of bacteria,the fluorescence intensity of the three FCDs was restored or further quenched.Recur to statistical analysis methods,it is employed to accurately discriminate 10 types of bacteria(including three probiotics and seven pathogenic bacteria)in natural water samples and human urine samples.The discrimination ability of the sensor array was highly enhanced via different competing binding of the FCDs and the bacteria toward Con A-PDA.The proposed array-based method offers a rapid,high-throughput,and reliable sensing platform for pathogen diagnosis in the field of environmental monitoring and clinical diagnosis.展开更多
在万物互联的云时代,云应用程序编程接口(API)是数字经济建设和服务化软件开发的关键数字基础设施。然而,云API数量的持续增长给用户决策和推广带来挑战,设计有效的推荐方法成为亟待解决的重要问题。现有研究多利用调用偏好、搜索关键...在万物互联的云时代,云应用程序编程接口(API)是数字经济建设和服务化软件开发的关键数字基础设施。然而,云API数量的持续增长给用户决策和推广带来挑战,设计有效的推荐方法成为亟待解决的重要问题。现有研究多利用调用偏好、搜索关键词或二者结合进行建模,主要解决为给定Mashup推荐合适云API的问题,未考虑开发者对个性化高阶互补云API的实际需求。该文提出一种基于个性化张量分解的高阶互补云API推荐方法(Personalized Tensor Decomposition based High-order Complementary cloud API Recommendation,PTDHCR)。首先,将Mashup与云API之间的调用关系,以及云API与云API之间的互补关系建模为三维张量,并利用RECAL张量分解技术对这两种关系进行共同学习,以挖掘云API之间的个性化非对称互补关系。然后,考虑到不同互补关系对推荐结果的影响程度不同,构建个性化高阶互补感知网络,充分利用Mashup、查询云API以及候选云API的多模态特征,动态计算Mashup对不同查询和候选云API之间互补关系的关注程度。在此基础上,将个性化互补关系拓展到高阶,得到候选云API与查询云API集合的整体个性化互补性。最后,利用两个真实云API数据集进行实验,结果表明,相较于传统方法,PTDHCR在挖掘个性化互补关系和推荐方面具有较大的优势。展开更多
Currently,the demand for electromagnetic wave(EMW)absorbing materials with specific functions and capable of withstanding harsh environments is becoming increasingly urgent.Multi-component interface engineering is con...Currently,the demand for electromagnetic wave(EMW)absorbing materials with specific functions and capable of withstanding harsh environments is becoming increasingly urgent.Multi-component interface engineering is considered an effective means to achieve high-efficiency EMW absorption.However,interface modulation engineering has not been fully discussed and has great potential in the field of EMW absorption.In this study,multi-component tin compound fiber composites based on carbon fiber(CF)substrate were prepared by electrospinning,hydrothermal synthesis,and high-temperature thermal reduction.By utilizing the different properties of different substances,rich heterogeneous interfaces are constructed.This effectively promotes charge transfer and enhances interfacial polarization and conduction loss.The prepared SnS/SnS_(2)/SnO_(2)/CF composites with abundant heterogeneous interfaces have and exhibit excellent EMW absorption properties at a loading of 50 wt%in epoxy resin.The minimum reflection loss(RL)is−46.74 dB and the maximum effective absorption bandwidth is 5.28 GHz.Moreover,SnS/SnS_(2)/SnO_(2)/CF epoxy composite coatings exhibited long-term corrosion resistance on Q235 steel surfaces.Therefore,this study provides an effective strategy for the design of high-efficiency EMW absorbing materials in complex and harsh environments.展开更多
基金supported by National Natural Science Foundation of China(Nos.22376057,22174048,22274048,22274045,22274047,and 21904039)the Foundation of the Science&Technology Department of Hunan Province(Nos.2023JJ30394 and2023ZJ1123)。
文摘Rapid and robust identification of bacteria is crucial for environmental monitoring and clinical diagnosis.Herein,a bioinspired interface-mediated multichannel sensor array was developed based on three-coloremitting antimicrobial functional carbon dots(FCDs)and concanavalin A doped polydopamine nanoparticles(Con A-PDA)for identification of bacteria.In this sensor,the fluorescence intensity of the three FCDs was quenched by the Con A-PDA.Upon addition different types of bacteria,the fluorescence intensity of the three FCDs was restored or further quenched.Recur to statistical analysis methods,it is employed to accurately discriminate 10 types of bacteria(including three probiotics and seven pathogenic bacteria)in natural water samples and human urine samples.The discrimination ability of the sensor array was highly enhanced via different competing binding of the FCDs and the bacteria toward Con A-PDA.The proposed array-based method offers a rapid,high-throughput,and reliable sensing platform for pathogen diagnosis in the field of environmental monitoring and clinical diagnosis.
文摘在万物互联的云时代,云应用程序编程接口(API)是数字经济建设和服务化软件开发的关键数字基础设施。然而,云API数量的持续增长给用户决策和推广带来挑战,设计有效的推荐方法成为亟待解决的重要问题。现有研究多利用调用偏好、搜索关键词或二者结合进行建模,主要解决为给定Mashup推荐合适云API的问题,未考虑开发者对个性化高阶互补云API的实际需求。该文提出一种基于个性化张量分解的高阶互补云API推荐方法(Personalized Tensor Decomposition based High-order Complementary cloud API Recommendation,PTDHCR)。首先,将Mashup与云API之间的调用关系,以及云API与云API之间的互补关系建模为三维张量,并利用RECAL张量分解技术对这两种关系进行共同学习,以挖掘云API之间的个性化非对称互补关系。然后,考虑到不同互补关系对推荐结果的影响程度不同,构建个性化高阶互补感知网络,充分利用Mashup、查询云API以及候选云API的多模态特征,动态计算Mashup对不同查询和候选云API之间互补关系的关注程度。在此基础上,将个性化互补关系拓展到高阶,得到候选云API与查询云API集合的整体个性化互补性。最后,利用两个真实云API数据集进行实验,结果表明,相较于传统方法,PTDHCR在挖掘个性化互补关系和推荐方面具有较大的优势。
基金financially supported by the National Natural Science Foundation of China(No.52377026 and No.52301192)Taishan Scholars and Young Experts Program of Shandong Province(No.tsqn202103057)+4 种基金Postdoctoral Fellowship Program of CPSF under Grant Number(No.GZB20240327)Shandong Postdoctoral Science Foundation(No.SDCXZG-202400275)Qingdao Postdoctoral Application Research Project(No.QDBSH20240102023)China Postdoctoral Science Foundation(No.2024M751563)the Qingchuang Talents Induction Program of Shandong Higher Education Institution(Research and Innovation Team of Structural-Functional Polymer Composites).
文摘Currently,the demand for electromagnetic wave(EMW)absorbing materials with specific functions and capable of withstanding harsh environments is becoming increasingly urgent.Multi-component interface engineering is considered an effective means to achieve high-efficiency EMW absorption.However,interface modulation engineering has not been fully discussed and has great potential in the field of EMW absorption.In this study,multi-component tin compound fiber composites based on carbon fiber(CF)substrate were prepared by electrospinning,hydrothermal synthesis,and high-temperature thermal reduction.By utilizing the different properties of different substances,rich heterogeneous interfaces are constructed.This effectively promotes charge transfer and enhances interfacial polarization and conduction loss.The prepared SnS/SnS_(2)/SnO_(2)/CF composites with abundant heterogeneous interfaces have and exhibit excellent EMW absorption properties at a loading of 50 wt%in epoxy resin.The minimum reflection loss(RL)is−46.74 dB and the maximum effective absorption bandwidth is 5.28 GHz.Moreover,SnS/SnS_(2)/SnO_(2)/CF epoxy composite coatings exhibited long-term corrosion resistance on Q235 steel surfaces.Therefore,this study provides an effective strategy for the design of high-efficiency EMW absorbing materials in complex and harsh environments.
