The kagome ferrimagnet TbMn_(6)Sn_(6),featuring a pristine Mn kagome lattice,has emerged as a candidate Chern magnet with a large intrinsic anomalous Hall effect(AHE).While chemical substitution can modulate its prope...The kagome ferrimagnet TbMn_(6)Sn_(6),featuring a pristine Mn kagome lattice,has emerged as a candidate Chern magnet with a large intrinsic anomalous Hall effect(AHE).While chemical substitution can modulate its properties,hydrostatic pressure provides a disorder-free route to manipulate electronic and magnetic interactions.Herein,we investigate the effects of hydrostatic pressure on electrical and magneto-transport in TbMn6Sn6 up to 18.3 GPa.Pressure significantly enhances hysteresis in the magnetoresistance and Hall responses,causing a concurrent monotonic coercive field increase,suggesting the enhancement of interlayer magnetic couplings in a robust c-axis ferrimagnetic order.The intrinsic anomalous Hall conductivity increases considerably from 129.5 S·cm^(−1) at ambient pressure conditions to 448.7 S·cm^(−1) at 14.0 GPa—an enhancement of 247%that is unprecedented among pressure-tuned kagome magnets.Based on density functional theory calculations,we reveal that pressure induces multiple gap openings near the Fermi level,giving rise to pronounced Berry curvature hotspots that may contribute to the AHE.Our results show that pressure can be used to enhance the intrinsic topological responses of this kagome magnet.展开更多
Droplet impact dynamics on solid surfaces,which are ubiquitously present in aerospace engineering,energy systems,agricultural production,etc.,involve complex fluid–structure interactions.Herein,we employ a single-cam...Droplet impact dynamics on solid surfaces,which are ubiquitously present in aerospace engineering,energy systems,agricultural production,etc.,involve complex fluid–structure interactions.Herein,we employ a single-camera high-speed threedimensional digital image correlation system to quantify the full-field deformations of flexible thin films during droplet impact dynamics.Experimental results revealed that the substrate flexibility not only reduces the maximum spreading diameter by 10%but also modulates rebound dynamics via energy competition between kinetic energy and surface adhesion energy,suggesting that coupled deformation of the solid–fluid interface plays an important role in the dynamic progress.We propose the structure-coupled response number(Sn),a governing dimensionless parameter unifying droplet spreading on both rigid and flexible films,validated by a universal 1/2 scaling law.A theoretical criterion for droplet rebound on hydrophobic flexible thin films is derived and experimentally demonstrated,which achieves the precise control of droplet rebound/non-rebound mode.This work bridges the theories of droplet impact dynamics on rigid and flexible substrates,offering a robust strategy to govern the droplet impact behaviors.展开更多
基金supported by the National Key R&D Program of China (Grant Nos.2023YFA1406002 and 2020YFA0308801)the National Natural Science Foundation of China (NSFC) (Grant Nos.12321004,12174025,12074041,and 12204045)+7 种基金the CAS Superconducting Research Project (Grant No.SCZX-0101)the Fundamental Research Funds for the Central Universities (Grant No.2243300003)the Innovation Program for Quantum Science and Technology (Grant No.2021ZD0302800)supported by the Synergetic Extreme Condition User Facility (SECUF)Analysis & Testing center in Beijing Institute of Technologysupport from the Beijing Institute of Technology Research Fund Program (Grant No.2023CX01027)support from the Beijing Institute of Technology Research Fund Program for Young Scholarssupport from the Beijing Institute of Technology Laboratory Research Project (Grant No.2023BITSYB07)。
文摘The kagome ferrimagnet TbMn_(6)Sn_(6),featuring a pristine Mn kagome lattice,has emerged as a candidate Chern magnet with a large intrinsic anomalous Hall effect(AHE).While chemical substitution can modulate its properties,hydrostatic pressure provides a disorder-free route to manipulate electronic and magnetic interactions.Herein,we investigate the effects of hydrostatic pressure on electrical and magneto-transport in TbMn6Sn6 up to 18.3 GPa.Pressure significantly enhances hysteresis in the magnetoresistance and Hall responses,causing a concurrent monotonic coercive field increase,suggesting the enhancement of interlayer magnetic couplings in a robust c-axis ferrimagnetic order.The intrinsic anomalous Hall conductivity increases considerably from 129.5 S·cm^(−1) at ambient pressure conditions to 448.7 S·cm^(−1) at 14.0 GPa—an enhancement of 247%that is unprecedented among pressure-tuned kagome magnets.Based on density functional theory calculations,we reveal that pressure induces multiple gap openings near the Fermi level,giving rise to pronounced Berry curvature hotspots that may contribute to the AHE.Our results show that pressure can be used to enhance the intrinsic topological responses of this kagome magnet.
基金supported by the National Key R&D Program of China(grant nos.2022YFF0503500 and 2022YFA1203200)the Guangdong Basic and Applied Basic Research Foundation(grant no.2023A1515011784)+2 种基金the National Natural Science Foundation of China(grant no.12032019)the Strategic Priority Research Program of Chinese Academy of Sciences(grant nos.XDB0620101 and XDB0620103)the Youth Innovation Promotion Association,Chinese Academy of Sciences(no.2020020).
文摘Droplet impact dynamics on solid surfaces,which are ubiquitously present in aerospace engineering,energy systems,agricultural production,etc.,involve complex fluid–structure interactions.Herein,we employ a single-camera high-speed threedimensional digital image correlation system to quantify the full-field deformations of flexible thin films during droplet impact dynamics.Experimental results revealed that the substrate flexibility not only reduces the maximum spreading diameter by 10%but also modulates rebound dynamics via energy competition between kinetic energy and surface adhesion energy,suggesting that coupled deformation of the solid–fluid interface plays an important role in the dynamic progress.We propose the structure-coupled response number(Sn),a governing dimensionless parameter unifying droplet spreading on both rigid and flexible films,validated by a universal 1/2 scaling law.A theoretical criterion for droplet rebound on hydrophobic flexible thin films is derived and experimentally demonstrated,which achieves the precise control of droplet rebound/non-rebound mode.This work bridges the theories of droplet impact dynamics on rigid and flexible substrates,offering a robust strategy to govern the droplet impact behaviors.
