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Framework-solvent interactional mechanism and effect of NMP/DMF on solvothermal synthesis of [Zn_4O(BDC)_3]_8 被引量:3
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作者 吴争平 王明雪 +4 位作者 周丽姣 尹周澜 谈进 张锦玲 陈启元 《Transactions of Nonferrous Metals Society of China》 SCIE EI CAS CSCD 2014年第11期3722-3731,共10页
In order to explore the effect mechanism of solvent on the synthesis of the metal organic framework materials, the microscopic interaction between solvent and framework and the effects of N,N-dimethyl-formamide(DMF) o... In order to explore the effect mechanism of solvent on the synthesis of the metal organic framework materials, the microscopic interaction between solvent and framework and the effects of N,N-dimethyl-formamide(DMF) or N-methyl- 2-pyrrolidone(NMP) on solvothermal synthesis of [Zn4O(BDC)3]8 were investigated through a combined DFT and experimental study. XRD and SEM showed that the absorbability of NMP in the pore of [Zn4O(BDC)3]8 was weaker than that of DMF. The thermal decomposition temperature of [Zn4O(BDC)3]8 synthesized in DMF was higher than that in NMP according to TG and FT-IR. In addition, the nitrogen sorption isotherms indicated that NMP improved gas sorption property of [Zn4O(BDC)3]8. The COSMO optimized calculations indicated that the total energy of Zn4O(BDC)3 in NMP was higher than that in DMF, and compared with non-solvent system, the charge of zinc atoms decreased and the charge value was the smallest in NMP. Furthermore, the interaction of DMF, NMP or DEF in [Zn4O(BDC)3]8 crystal model was calculated by DFT method. The results suggested that NMP should be easier to be removed from pore of materials than DMF from the point of view of energy state. It can be concluded that NMP was a favorable solvent to synthesize [Zn4O(BDC)3]8 and the microscopic mechanism was that the binding force between Zn4O(BDC)3 and NMP molecule was weaker than DMF. 展开更多
关键词 solvothermal synthesis [Zn4O(BDC)3]8 N-METHYL-2-PYRROLIDONE interactional mechanism COSMO solvation model density functional method
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A Glimpse of Interactional Strategies Used in Group Discussion in the EFL Context
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作者 林美笑 《海外英语》 2013年第3X期73-75,共3页
On the basis of literature review,this paper discusses what interactional strategies are in group discussions conducted in the EFL classroom.Two frameworks for interactional strategies are investigated to explore the ... On the basis of literature review,this paper discusses what interactional strategies are in group discussions conducted in the EFL classroom.Two frameworks for interactional strategies are investigated to explore the types of interactional strategies.This aims to shed light upon the analysis of interactional features in face-to-face communication. 展开更多
关键词 STRATEGIC COMPETENCE interactional STRATEGIES grou
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From Xu to the Development of L2 Interactional Competence: A Conversation Analytic Case Study 被引量:7
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作者 Mei YANG Xiaofei LU 《Chinese Journal of Applied Linguistics》 2021年第3期273-291,430,共20页
Dialogues are fundamentally driven by xu(C. Wang, 2016, 2017), a Chinese word meaning continuation that captures the process in which interlocutors participate in interaction through the actions of(utterance) completi... Dialogues are fundamentally driven by xu(C. Wang, 2016, 2017), a Chinese word meaning continuation that captures the process in which interlocutors participate in interaction through the actions of(utterance) completion,(content) extension, and(topic) creation(CEC). This article reports a conversation analytic case study designed to investigate how the continuation strategies of CEC are used in real-time communication to achieve mutual understanding, and thus to construct intersubjectivity(Verhagen, 2005) and promote the development of second language(L2)interactional competence. Our data consisted of audio and video recordings of a 25-minute conversation between two L2 English speakers, one expert and one novice, and a stimulated recall interview with them. Results revealed that the expert employed CEC at the early stage of interaction to maintain successful communication, and the novice gradually aligned with the expert and used CEC to achieve mutual understanding, construct intersubjectivity, and create opportunities for interaction and learning at the late stage, displaying her development of L2 interactional competence. Our findings have useful implications for theoretical and methodological development of the xu-argument studies as well as for xu-based L2 pedagogy. 展开更多
关键词 the xu-argument INTERSUBJECTIVITY interactional competence continuation strategies conversation analysis
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Interactional models for adults of two populations with maturation delays
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作者 HE Ze-rong LI Jian-quan 《Applied Mathematics(A Journal of Chinese Universities)》 SCIE CSCD 2008年第2期127-135,共9页
This paper is concerned with interactional models for adults of two species delayed by their mature periods. The existence and local stability of equilibria are discussed thoroughly for competitive systems, cooperativ... This paper is concerned with interactional models for adults of two species delayed by their mature periods. The existence and local stability of equilibria are discussed thoroughly for competitive systems, cooperative systems and predator-prey systems, respectively. For systems with interaction of competition and cooperation, it is found that the two populations are uniformly persistent if the positive equilibrium is stable. For predator-prey interaction, however, some further conditions are needed to guarantee the persistence of the systems. 展开更多
关键词 interactional models mature period equilibrium stability uniform persistence.
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A Corpus-based Study of Interactional Metadiscourse in Dissertation Abstracts
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作者 HU Xue-chen LIU Ying-liang 《Journal of Literature and Art Studies》 2022年第3期268-274,共7页
Although much previous research has examined the expression of interactional metadiscourse in different registers,little is known about the ways writers express interactional metadiscourse in part-genres such as disse... Although much previous research has examined the expression of interactional metadiscourse in different registers,little is known about the ways writers express interactional metadiscourse in part-genres such as dissertation abstracts.This study explores interactional metadiscourse in doctoral students’English dissertation abstracts in material science and applied linguistics.The analysis is based on two self-built corpora of student writing:60 dissertation abstracts in material science and 60 dissertation abstracts in applied linguistics.Using Hyland’s(2005)model of interactional metadiscourse,this study compared the employment of metadiscourse resources in the two corpora.Findings of the analysis show that the students in applied linguistics use significantly more interactional devices than their material science counterparts.For each type of interpersonal resource,namely,hedges,boosters,attitude markers,self-mentions and engagement markers,significant differences were found.The results reveal students’increasing awareness of the authorial identity in academic writing.The study has practical implications for the teaching of academic writing. 展开更多
关键词 interactional metadiscourse disciplinary differences ABSTRACTS academic writing
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MOLECULES AND NEW INTERACTIONAL STRUCTURES FOR A(2+1)-DIMENSIONAL GENERALIZED KONOPELCHENKO-DUBROVSKY-KAUP-KUPERSHMIDT EQUATION 被引量:1
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作者 李岩 姚若侠 夏亚荣 《Acta Mathematica Scientia》 SCIE CSCD 2023年第1期80-96,共17页
Soliton molecules(SMs)of the(2+1)-dimensional generalized KonopelchenkoDubrovsky-Kaup-Kupershmidt(gKDKK)equation are found by utilizing a velocity resonance ansatz to N-soliton solutions,which can transform to asymmet... Soliton molecules(SMs)of the(2+1)-dimensional generalized KonopelchenkoDubrovsky-Kaup-Kupershmidt(gKDKK)equation are found by utilizing a velocity resonance ansatz to N-soliton solutions,which can transform to asymmetric solitons upon assigning appropriate values to some parameters.Furthermore,a double-peaked lump solution can be constructed with breather degeneration approach.By applying a mixed technique of a resonance ansatz and conjugate complexes of partial parameters to multisoliton solutions,various kinds of interactional structures are constructed;There include the soliton molecule(SM),the breather molecule(BM)and the soliton-breather molecule(SBM).Graphical investigation and theoretical analysis show that the interactions composed of SM,BM and SBM are inelastic. 展开更多
关键词 (2+1)-dimensional generalized Konopelchenko-Dubrovsky-Kaup-Kupershmidt equation soliton molecules velocity resonance nonelastic interaction
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Hidden Crises and Communication: An Interactional Analysis of Hidden Crises
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作者 Annette Klarenbeek 《Journalism and Mass Communication》 2011年第3期168-184,共17页
In this paper I describe the ways in which the communication discipline can make a hidden crisis transparent. For this purpose I examine the concept of crisis entrepreneurship from a communication point of view. Using... In this paper I describe the ways in which the communication discipline can make a hidden crisis transparent. For this purpose I examine the concept of crisis entrepreneurship from a communication point of view. Using discourse analysis, I analyse the discursive practices of crisis entrepreneurs in the domain of education in the Netherlands. This paper is part of my Ph.D. project in which I examine the dilemmas encountered by crisis entrepreneurs and the interactional solutions they choose in addressing a crisis. In my Ph.D. project I have analysed how crisis entrepreneurs use discursive practices: (1) to show thefactuality of the problem. For example, the way the problem is presented is too theoretical and is not a problem in reality; (2) to present the credibility of the messenger as an authentic, legitimate spokesman. Crisis entrepreneurs may be accused of wanting to attract attention to their own cause; (3) to create the accountability for the problem and the solution. For example, crisis entrepreneurs can be accused of nursing personal grievances or of drawing attention to the issue without actively attempting to solve it. The conclusion is that a communication professional is able to recognize a problem raised by crisis entrepreneurs. Knowledge of interactional dilemmas helps communication professionals understand the potential of crisis entrepreneurs. A communication professional can therefore contribute to the recognition of crises by acknowledging that a crisis entrepreneur is someone who can have a strong hand in the public agenda, i.e., public affairs that are important to the authorities. 展开更多
关键词 hidden crisis crisis communication crisis entrepreneurs discourse analyses INTERACTION
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Schisming as an Interactional Resource for Learning at the Frontiers of Work and Vocational Training-A Secondary Publication
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作者 Laurent Filliettaz Isabelle Durand +1 位作者 Marianne Zogmal Vasiliki Markaki-Lothe 《Journal of Contemporary Educational Research》 2024年第4期346-364,共19页
This paper examines the sorts of interactional competencies and institutional demands required from students as they engage in complex forms of participation combining work and training purposes.It focuses on a series... This paper examines the sorts of interactional competencies and institutional demands required from students as they engage in complex forms of participation combining work and training purposes.It focuses on a series of empirical cases,recorded through video data and analyzed from a conversation analytic perspective,in which mentors make the decision to intervene during work sessions moderated by students.Such interventions do not interrupt the student’s activity and lead to the emergence of two distinct but not impermeable interactional spaces.This complex participation framework,known as“schisming,”contributes to overcoming practical issues within multiparty settings.Our study shows how schisming constitutes a particular sequential phenomenon where participants reorganize the interaction and co-construct a social and cognitive interactional space,thus enabling a shared understanding of the specific training context.Empirical data from the practical training of medical radiographers are used to illustrate how schisming may contribute to learning in the conditions of guided practice. 展开更多
关键词 Language and interaction Student-teacher relations and interactions Analysis of professional practice Professional education
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Effects of Cooperative Learning on Interactional Strategy Use in EFL Context:An Analysis of Chinese Students' Classroom Talks
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作者 林美笑 《Chinese Journal of Applied Linguistics》 2014年第1期49-66,129,共19页
This paper presents a study that explored the effects of cooperative learning on Chinese students' interactional strategy use in the EFL classroom. A quasi-experimental research design was adopted. The experimental c... This paper presents a study that explored the effects of cooperative learning on Chinese students' interactional strategy use in the EFL classroom. A quasi-experimental research design was adopted. The experimental class (EC) participated in cooperative learning for 30 minutes in each 90-minute session in an integrated skills course while the control class (CC) had the same course following a teacher-fronted format. Interactional data of EC and CC were collected for comparison from the pre- and post-tasks conducted at the beginning and the end of the experiment respectively. The results show that EC appeared to have made more gains in interactional strategy use than CC after the experiment. Although CC made more progress in elaboration than EC, EC produced more uptakes, used much less Chinese and made fewer message abandonments, suggesting better oral fluency in their interaction as a result of cooperative learning. 展开更多
关键词 cooperative learning interactional strategies interactive practice
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Description and Evaluation of the Emission and Atmospheric Processes Integrated and Coupled Community(EPICC)Model Version 1.0 被引量:1
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作者 EPICC Model Working Group 《Advances in Atmospheric Sciences》 2026年第4期671-694,I0001-I0006,共30页
We present a comprehensive description and benchmark evaluation of the global–regional chemical transport model called the Emission and Atmospheric Processes Integrated and Coupled Community(EPICC)model.The framework... We present a comprehensive description and benchmark evaluation of the global–regional chemical transport model called the Emission and Atmospheric Processes Integrated and Coupled Community(EPICC)model.The framework incorporates(1)grid configuration,(2)transport dynamics,(3)chemical mechanisms,(4)aerosol processes,(5)wet/dry deposition parameterizations,and(6)heterogeneous chemistry treatments associated with sulfate,nitrous acid(HONO)chemistry,and aerosol/cloud–photolysis interactions(APIs/CPIs).Openly shared with the atmospheric research community,the model facilitates integration of advanced physicochemical schemes to enhance simulation accuracy.Globally,the model demonstrates realistic representations of ozone(O_(3))and aerosol optical depth.The EPICC model generally demonstrates robust performance in simulating regional concentrations of O_(3) and PM_(2.5)(and its components)in China.It successfully captures vertical profiles of both global and regional O_(3).Notably,the model mitigates frequently reported sulfate underestimations in highly industrialized regions of China.The model accurately captures two regional severe pollution episodes observed in eastern China(January/June 2021).Sensitivity experiments highlight the critical roles of heterogeneous chemical mechanisms associated with sulfate,HONO chemistry,APIs,and CPIs in capturing PM_(2.5) and O_(3) concentrations in China.Improved sulfate mechanisms result in an increase of approximately 32.4%(2.8μg m^(−3))in simulated winter sulfate concentrations when observations exceed 10μg m^(−3).Enhanced HONO elevates winter O_(3) and PM_(2.5) by≤20 and≤10μg m^(−3),respectively.Overall,CPIs dominate over APIs in improving O_(3) and PM_(2.5) simulations across China.Locally,APIs mitigate PM_(2.5) and O_(3) discrepancies in the Sichuan Basin.Seasonal cloud–chemistry coupling explains the weaker impact of PM_(2.5) in summer. 展开更多
关键词 EPICC model PM_(2.5) O_(3) sulfate nitrous acid aerosol/cloud-photolysis interactions
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Neuronal guidance signaling in neurodegenerative diseases:Key regulators that function at neuron-glia and neuroimmune interfaces
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作者 Junichi Yuasa-Kawada Mariko Kinoshita-Kawada +6 位作者 Masaki Hiramoto Satoru Yamagishi Takayasu Mishima Shin’ichiro Yasunaga Yoshio Tsuboi Nobutaka Hattori Jane Y.Wu 《Neural Regeneration Research》 2026年第2期612-635,共24页
The nervous system processes a vast amount of information,performing computations that underlie perception,cognition,and behavior.During development,neuronal guidance genes,which encode extracellular cues,their recept... The nervous system processes a vast amount of information,performing computations that underlie perception,cognition,and behavior.During development,neuronal guidance genes,which encode extracellular cues,their receptors,and downstream signal transducers,organize neural wiring to generate the complex architecture of the nervous system.It is now evident that many of these neuroguidance cues and their receptors are active during development and are also expressed in the adult nervous system.This suggests that neuronal guidance pathways are critical not only for neural wiring but also for ongoing function and maintenance of the mature nervous system.Supporting this view,these pathways continue to regulate synaptic connectivity,plasticity,and remodeling,and overall brain homeostasis throughout adulthood.Genetic and transcriptomic analyses have further revealed many neuronal guidance genes to be associated with a wide range of neurodegenerative and neuropsychiatric disorders.Although the precise mechanisms by which aberrant neuronal guidance signaling drives the pathogenesis of these diseases remain to be clarified,emerging evidence points to several common themes,including dysfunction in neurons,microglia,astrocytes,and endothelial cells,along with dysregulation of neuron-microglia-astrocyte,neuroimmune,and neurovascular interactions.In this review,we explore recent advances in understanding the molecular and cellular mechanisms by which aberrant neuronal guidance signaling contributes to disease pathogenesis through altered cell-cell interactions.For instance,recent studies have unveiled two distinct semaphorin-plexin signaling pathways that affect microglial activation and neuroinflammation.We discuss the challenges ahead,along with the therapeutic potentials of targeting neuronal guidance pathways for treating neurodegenerative diseases.Particular focus is placed on how neuronal guidance mechanisms control neuron-glia and neuroimmune interactions and modulate microglial function under physiological and pathological conditions.Specifically,we examine the crosstalk between neuronal guidance signaling and TREM2,a master regulator of microglial function,in the context of pathogenic protein aggregates.It is well-established that age is a major risk factor for neurodegeneration.Future research should address how aging and neuronal guidance signaling interact to influence an individual’s susceptibility to various late-onset neurological diseases and how the progression of these diseases could be therapeutically blocked by targeting neuronal guidance pathways. 展开更多
关键词 amyloid-β axon guidance NEURODEGENERATION neuroimmune interactions neuroinflammation neuron-glia interactions neurovascular interactions SEMAPHORIN synaptic remodeling tau TDP-43 TREM2 Α-SYNUCLEIN
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Fractional calculus approach to RT-IN enzymatic competition in modulating HIV replication dynamics
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作者 Tushar Ghosh Oluwole Daniel Makinde +1 位作者 WANG Shu Priti Kumar Roy 《Applied Mathematics(A Journal of Chinese Universities)》 2026年第1期225-254,共30页
HIV infection continues to pose a significant global health challenge,with subSaharan Africa bearing a disproportionate burden.The replication cycle of HIV is fundamentally driven by intricate molecular interactions.T... HIV infection continues to pose a significant global health challenge,with subSaharan Africa bearing a disproportionate burden.The replication cycle of HIV is fundamentally driven by intricate molecular interactions.This study investigates the competitive biochemical interplay between reverse transcriptase(RT)and integrase(IN)enzymes,employing a fractional calculus framework to model their mutual inhibitory effects.Through the application of fixed-point theory and Picard stability analysis,the existence,uniqueness,and stability of the fractional-order system are rigorously established.The role of RT-IN enzymatic competition in influencing HIV replication dynamics is elucidated through global sensitivity analysis using Latin Hypercube Sampling.Furthermore,the model incorporates memory-dependent characteristics by examining three distinct fractional operators,namely,the Caputo,Caputo-Fabrizio,and Atangana-Baleanu operators in the Caputo sense,thereby elucidating their respective influences on system behavior.The Atangana-Baleanu operator,in particular,demonstrates an enhanced capacity to capture the complex,synergistic processes underpinning HIV progression.This research provides a critical nexus between molecular virology and applied mathematics,offering foundational insights for the advancement of more precise and targeted therapeutic strategies against HIV. 展开更多
关键词 HIV biochemical interaction physical interaction fractional calculus Sumudu transformation LHS PRCC
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From preparedness to action:Synthesising insights on robot usage in post-Earthquake search operations
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作者 Rajashekhar V S Gowdham Prabhakar 《Resilient Cities and Structures》 2026年第1期60-70,共11页
Human life is invaluable,and timely efforts are crucial to rescue individuals trapped under debris following an earthquake.To identify opportunities for improving post-earthquake search and rescue(SAR)robotics,we get ... Human life is invaluable,and timely efforts are crucial to rescue individuals trapped under debris following an earthquake.To identify opportunities for improving post-earthquake search and rescue(SAR)robotics,we get insights through four different sources:(i)A literature review of disaster robotics and victim psychology,(ii)A public survey on earthquake awareness and their view of rescue robots,(iii)Semi-structured interviews with first responders,and(iv)Responses from GenAI chatbots which were prompted to assume the role of expert rescuers.The triangulated analysis show that there are challenges in mobility,autonomy,communication,situational awareness,and human-robot collaboration.The public respondents showed high acceptance of robot-assisted rescue and prioritised survivor detection,sensing,and communication as essential functionalities of robots.The experts expressed limitations in current equipment,the need for improved victim localisation,and interest in XR-based training and robot-assisted debris handling.The GenAI chatbots highlighted structural risk assessment,multi-sensor fusion,and supervised autonomy.Therefore,this study identifies critical robot features,outlines multi-modal interaction requirements,and highlights gaps in current SAR practice.These findings offer robot design directions for developing effective,trustworthy SAR robots,which can be integrated to future response disaster-workflows. 展开更多
关键词 Robots DISASTERS Earthquake search Multi-modal interaction Human-Robot interaction
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Host-yeast interactions and its influence on health and disease
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作者 Xiao-Bing Li Chun-Hui Yang +18 位作者 Qian Li Chun-Rong Chen Yuan-Fang Hou Zhen-Jun Xi Xue-Hua Yang Yan Li Jie Wan You-Chun Lei Chao Yu Fei-Ji Sun Li Wang Yong-Sheng Liu Miao Wang Bao-Cheng Yuan Ying Peng Wei Wang Wu-Tao Xie Qin Hu Li Zhang 《Infection Advances》 2026年第2期4-16,共13页
Host-yeast interactions are fundamental drivers of human microbiome dynamics,spanning a spectrum from mutualistic symbiosis to opportunistic pathogenesis with profound implications for systemic health.This review syst... Host-yeast interactions are fundamental drivers of human microbiome dynamics,spanning a spectrum from mutualistic symbiosis to opportunistic pathogenesis with profound implications for systemic health.This review systematically elucidates the complex molecular mechanisms governing these relationships,with a specific focus on metabolic interdependence and immunomodulation.We analyze how yeast-derived metabolites,particularly short-chain fatty acids(SCFAs),modulate host glucose and lipid homeostasis via signaling pathways such as GPR41/43 and GLP-1 secretion.Furthermore,the review explores the pathophysiological role of fungal dysbiosis in chronic conditions,including obesity,diabetes,and inflammatory bowel disease(IBD),highlighting how a breakdown in host-yeast homeostasis triggers pro-inflammatory cascades.Beyond the fungal-host axis,we introduce the concept of the"mycobiome-virome-bacterial axis,"discussing how commensal yeasts synergize with beneficial bacteria like Bifidobacterium and influence viral infectivity through Interferon-mediated innate immune priming.We critically evaluate how cutting-edge technologies-including transgenic mouse models(specifically Dectin-1^(-/-)and CARD9^(-/-),metabolomics,and single-cell sequencing-have revolutionized our mechanistic understanding of these multi-kingdom dynamics.By integrating current findings,we identify critical knowledge gaps and propose high-resolution research frameworks,such as humanized organ-on-a-chip systems,to simulate intricate host-microbe interactions under physiological flow conditions.This comprehensive synthesis provides a strategic foundation for developing targeted,next-generation microbiome-based interventions to restore host-yeast balance and enhance overall human health. 展开更多
关键词 host-fungal interactions Saccharomyces cerevisiae Candida albicans gut microbiota microbial metabolomics fungal-bacterial interactions gut homeostasis microbiome therapeutics
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A survey of panel aeroelasticity in shock-dominated flow:Perspectives from fluid-structure interactions and shock wave-boundary layer interactions
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作者 Aiming SHI Yiwen HE 《Chinese Journal of Aeronautics》 2026年第1期210-229,共20页
As a multidisciplinary phenomenon,panel aeroelasticity in shock-dominated flow is featured by two primary interactions:Fluid-Structure Interactions(FSIs)and Shock-Boundary Layer Interactions(SBLIs).The former raises s... As a multidisciplinary phenomenon,panel aeroelasticity in shock-dominated flow is featured by two primary interactions:Fluid-Structure Interactions(FSIs)and Shock-Boundary Layer Interactions(SBLIs).The former raises structural concerns,and the latter is of aerodynamic interest.Thus,panel aeroelasticity in shock-dominated flow represents a vital topic for the development and optimization of supersonic vehicles and propulsion systems.This review systematically summarizes recent advances in the methodologies applied to capture structural and fluid dynamics,including theoretical models,numerical simulations,and wind tunnel experiments.The application of data-driven modal decomposition,an advanced technique to extract physically crucial features,on the topic is introduced.From the perspective of FSIs,the distinctive aeroelastic behaviors in shock-dominated flow,including hysteresis phenomena and nonlinear responses,are highlighted.From the perspective of SBLIs,the modifications in their spatial and temporal characteristics imposed by the aeroelastic responses are emphasized.Motivated by the interaction between the shock waves and structural response,different strategies have been proposed to implement aeroelastic suppression and shock control,which have the potential to enhance structural safety and aerodynamic performance in the next generation of high-speed flight vehicles. 展开更多
关键词 Aeroelasticity Fluid structure interaction Modal decomposition Shock boundary layer interactions Shock waves
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Geometric control of concurrence and quantum gate operations in triangular triple quantum dots
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作者 Junqing Li Shuo Dong Jianhua Wei 《Chinese Physics B》 2026年第2期314-321,共8页
As an important index to measure the degree of entanglement in quantum systems,concurrence plays an important role in practical research.In this paper,we study the concurrence between two qubits in triangular triple q... As an important index to measure the degree of entanglement in quantum systems,concurrence plays an important role in practical research.In this paper,we study the concurrence between two qubits in triangular triple quantum dot structure.Through calculation and simulation,it is found that concurrence is mainly affected by the interdot coupling strength t,Coulomb interactionU,temperature T,and electrode coupling G.Through comparative studies with parallel triple quantum dot structures,we demonstrate that the triangular geometry exhibits significantly enhanced concurrence under identical conditions.In addition,under the condition that concurrence exceeds 0.9,the functional relationship between t and U is obtained through simulation,which provides theoretical support for quantum dot regulation under high entanglement.Finally,we demonstrate the feasibility of implementing a three-qubit quantum gate,using the Toffoli gate as a representative example,under the condition that the triangular triple quantum dot system maintains high entanglement. 展开更多
关键词 transition coupling interaction triangular triple quantum dots quantum entanglement Coulomb interaction quantum computing
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DFT Insights into the Detection of NH_(3),AsH_(3),PH_(3),CO_(2),and CH_(4)Gases with Pristine and Monovacancy Phosphorene Sheets
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作者 Naresh Kumar Anuj Kumar Abhishek K.Mishra 《Computers, Materials & Continua》 2026年第4期517-531,共15页
Density functional theory(DFT)calculations were employed to investigate the adsorption behavior of NH_(3),AsH_(3),PH_(3),CO_(2),and CH_(4)molecules on both pristine and mono-vacancy phosphorene sheets.The pristine pho... Density functional theory(DFT)calculations were employed to investigate the adsorption behavior of NH_(3),AsH_(3),PH_(3),CO_(2),and CH_(4)molecules on both pristine and mono-vacancy phosphorene sheets.The pristine phosphorene surface showsweak physisorption with all the gasmolecules,inducing onlyminor changes in its structural and electronic properties.However,the introduction ofmono-vacancies significantly enhances the interaction strength with NH_(3),PH_(3),CO_(2),and CH_(4).These variations are attributed to substantial charge redistribution and orbital hybridization in the presence of defects.The defective phosphorene sheet also exhibits enhanced adsorption energies,along with favorable sensitivity and recovery characteristics,highlighting its potential as a promising gas sensor for NH_(3),AsH_(3),PH_(3),CO_(2),and CH_(4)at ambient conditions. 展开更多
关键词 Phosphorene VACANCY defects DFT interaction sensitivity
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Host-vip interaction mediated low-shrinkage photosensitive positioning adhesive
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作者 Zhao Liu Junjian Xie +3 位作者 Xiaoming Ren Muhammad Tahir Shixin Fa Qiuyu Zhang 《Chinese Chemical Letters》 2026年第2期501-504,共4页
As a common electronic adhesive,ultraviolet(UV)curing polyurethane acrylate adhesive has both flexibility and wear resistance of polyurethane,excellent weather resistance and optical properties of acrylate.Despite the... As a common electronic adhesive,ultraviolet(UV)curing polyurethane acrylate adhesive has both flexibility and wear resistance of polyurethane,excellent weather resistance and optical properties of acrylate.Despite the extensive applications,it is still difficult to solve the problems caused by the shrinkage of adhesive.Here,a new type of photosensitive adhesive for bonding electronic components based on supramolecular interaction was designed and synthesized.The supramolecular interaction of cyclodextrin and adamantane moieties introduced into the adhesive polymer entitles the viscosity of the adhesive to rise rapidly during use,thereby preventing adhesive loss and dislocation of electronic components.UV light could further cure the adhesive and position the electronic components.The adhesive shrunk<2%when cured by UV light,so it can be used for electronic packaging and high-resolution,defect-free lithography. 展开更多
关键词 ADHESIVE Host-vip interaction UV-CURING Low-shrinkage LITHOGRAPHY
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Defoliation accelerates the depletion of non-structural carbohydrates in Chinese pine under drought conditions
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作者 Tong Li Qingqing Fan +5 位作者 Xinyi Guo Ziying Zou Meng Wang Xiaolu Zhou Peng Li Changhui Peng 《Ecological Frontiers》 2026年第1期188-196,共9页
Drought has the potential to induce extensive defoliation in forest trees.However,the responses of non-structural carbohydrates(NSCs,including soluble sugar and starch)to the combined effects of drought and defoliatio... Drought has the potential to induce extensive defoliation in forest trees.However,the responses of non-structural carbohydrates(NSCs,including soluble sugar and starch)to the combined effects of drought and defoliation remain to be elucidated,particularly in pine trees.In this study,we investigated the interactive effects of drought and defoliation on the contents of NSCs in five organs(new and old needles,twigs,stems,as well as roots)of Chinese pine(Pinus tabuliformis)seedlings.We sampled two batches of the seedlings at 30 and 50 days,respectively.Our results showed that Chinese pine could tolerate mild drought,but severe drought significantly decreased the content of soluble sugars in all organs.Defoliation initially suppressed the photosynthetic rate and significantly reduced the soluble sugar content in all organs.However,after 50 days,this effect was substantially mitigated by the new needle growth.Starch content in twigs,stems,and roots was found to be more vulnerable to defoliation than to drought.A significant interactive effect existed between drought and defoliation on NSCs,with defoliation exacerbating the negative impact of drought on the accumulation of NSCs,especially in new needles and roots.These findings highlight the complex effects of defoliation on NSCs during drought,underscoring critical implications for the management and economic value of Chinese pine forests. 展开更多
关键词 Soluble sugar STARCH Coniferous tree Interaction ALLOCATION PHOTOSYNTHESIS
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