The realization of controllable polarity photoresponse within a single device is a crucial advancement for simulating biological bipolar vision cells to drive the development of next-generation optoelectronic technolo...The realization of controllable polarity photoresponse within a single device is a crucial advancement for simulating biological bipolar vision cells to drive the development of next-generation optoelectronic technologies.Nevertheless,current polarity photodetectors face significant challenges in fully suppressing symmetric photocurrent cancellation and optimizing carrier transport efficiency.Here,we propose a graphene-intercalated MoS_(2)/MoTe_(2)heterojunction,featuring a tailorable built-in electric field and a high efficiency transport channel.Spatially resolved photocurrent reveals that the controllable polarity photoresponse originates from the bias-dependent equivalent built-in electric field of MoS_(2)/MLG/MoTe_(2)heterojunction.The controllable polarity photoresponse realizes a large-area uniform“heart-shaped”photocurrent region.In enhanced polarity photoresponse mode,the photodetector exhibits broadband detection capabilities from visible(638 nm)to infrared(1550 nm)light,achieving a high responsivity of 18.1 A/W and an excellent detectivity of 2.8×10^(12)Jones,as well as fast response times of 94/119μs.Furthermore,precise imaging with a resolution better than 0.5 mm was successfully demonstrated,highlighting its polarity photoresponse for practical imaging applications.This work provides a new paradigm for controllable polarity photoresponse programmed by intercalated low-dimensional material structures,paving the way for next-generation intelligent sensing chips.展开更多
基金supported by National Key R&D Program of China(No.2023YFA1608701)the National Natural Science Foundation of China(Nos.62274168,11933006,U2141240,and 62005249)+3 种基金Hangzhou Leading Innovation and Entrepreneurship Team(No.TD2020002)Open Fund of State Key Laboratory of Infrared Physics(SITP-NLIST-YB-2023-13)Natural Science Foundation of Zhejiang Province(Nos.LZ24F050006 and LQ20F050005)the Research Funds of Hangzhou Institute for Advanced Study,UCAS(Nos.B02006C019025 and B02006C021010).
文摘The realization of controllable polarity photoresponse within a single device is a crucial advancement for simulating biological bipolar vision cells to drive the development of next-generation optoelectronic technologies.Nevertheless,current polarity photodetectors face significant challenges in fully suppressing symmetric photocurrent cancellation and optimizing carrier transport efficiency.Here,we propose a graphene-intercalated MoS_(2)/MoTe_(2)heterojunction,featuring a tailorable built-in electric field and a high efficiency transport channel.Spatially resolved photocurrent reveals that the controllable polarity photoresponse originates from the bias-dependent equivalent built-in electric field of MoS_(2)/MLG/MoTe_(2)heterojunction.The controllable polarity photoresponse realizes a large-area uniform“heart-shaped”photocurrent region.In enhanced polarity photoresponse mode,the photodetector exhibits broadband detection capabilities from visible(638 nm)to infrared(1550 nm)light,achieving a high responsivity of 18.1 A/W and an excellent detectivity of 2.8×10^(12)Jones,as well as fast response times of 94/119μs.Furthermore,precise imaging with a resolution better than 0.5 mm was successfully demonstrated,highlighting its polarity photoresponse for practical imaging applications.This work provides a new paradigm for controllable polarity photoresponse programmed by intercalated low-dimensional material structures,paving the way for next-generation intelligent sensing chips.
