1.Introduction Magnesium oxide(MgO)has attracted considerable attention in recent years due to its economic viability,excellent biocompatibil-ity,chemical stability,and non-toxic,odorless nature[1,2].These inherent pr...1.Introduction Magnesium oxide(MgO)has attracted considerable attention in recent years due to its economic viability,excellent biocompatibil-ity,chemical stability,and non-toxic,odorless nature[1,2].These inherent properties position it as a promising candidate for various applications.展开更多
PCDD/Fs have been become a serious issue because of their toxicological effects and associated adverse health implications. In this study, the gliding arc plasma was tested for treatment of polychlorinated dibenzo-p-d...PCDD/Fs have been become a serious issue because of their toxicological effects and associated adverse health implications. In this study, the gliding arc plasma was tested for treatment of polychlorinated dibenzo-p-dioxins （PCDDs） and polychlorinated dibenzofurans （PCDFs）, which was synthesized from pentachlorophenol in atmospheric condition at 350℃ with or without the catalysis of CuCl2. From the experiment, we found that the destruction efficiency of PCDD/F homologues after gliding was discharge ranged from 25% to 79%. This result demonstrates that gliding arc plasma is an effective technology to decompose PCDDs/Fs in flue gas. A plausible degradation mechanism for PCDD/Fs by gliding arc was discussed. Finally, a multistage reactor structure of gliding arc was proposed to upgrade removal efficiency for PCDD/Fs.展开更多
Wheat （Triticum aestivum） seeds were treated with atmospheric pressure gliding arc discharge plasmas to investigate the effects on water absorption, seed germination rate, seedling growth and yield in wheat. The sur...Wheat （Triticum aestivum） seeds were treated with atmospheric pressure gliding arc discharge plasmas to investigate the effects on water absorption, seed germination rate, seedling growth and yield in wheat. The surface architectures and functionalities of the seeds were found to modify due to plasma treatments. 6 rain treatment was provided 95%-100% germination rate. For the treatment duration of 3 and 9 rain the growth activity, dry matter accumulation, leaves chlorophyll contents, longest spikes, number of spikes/spikelet and total soluble protein content in shoots were improved. The grain yield of wheat was increased ,--20% by 6 min treatment with H2O/O2 plasma with respect to control.展开更多
Methane conversion has been studied using gliding arc plasma in the presence of argon.The process was conducted at atmospheric pressure and ambient temperature.The focus of this research was to develop a process of co...Methane conversion has been studied using gliding arc plasma in the presence of argon.The process was conducted at atmospheric pressure and ambient temperature.The focus of this research was to develop a process of converting methane to C2 hydrocarbons and hydrogen. The main parameters,including the CH4/Ar mole ratio,the CH4 flow rate,the input voltage,and the minimum electrode gap,were varied to investigate their effects on methane conversion rate, product distribution,energy consumption,carbon deposit,and reaction stability.The specific energy requirement（SER） was used to express the energy utilization efficiency of the process and provided a practical guidance for optimizing reaction conditions for improving energy efficiency. It was found that the carbon deposition was not conducive to methane conversion,and the gliding arc plasma discharge reached a stable state twelve minutes later.Optimum conditions for methane conversion were suggested.The maximum methane conversion rate of 43.39%was obtained under the optimum conditions.Also,C2 hydrocarbons selectivity,C2 hydrocarbons yield,H2 selectivity, H2 yield and SER were 87.20%,37.83%,81.28%,35.27%,and 2.09 MJ/mol,respectively.展开更多
A gliding arc discharge plasma and its characteristics are described. Analysis of the production principle of the plasma is presented. Some experimental results about two novel types of the gliding arc plasma generato...A gliding arc discharge plasma and its characteristics are described. Analysis of the production principle of the plasma is presented. Some experimental results about two novel types of the gliding arc plasma generator have been obtained. These types of gliding arc plasma axe potentially usable in the chemical industry and environmental engineering.展开更多
In agriculture production,plant health is threatened by pathogens parasitic on seeds;hence,it is necessary to disinfect harvested seeds before germination.In this study,a technique of gliding arc plasma treatment was ...In agriculture production,plant health is threatened by pathogens parasitic on seeds;hence,it is necessary to disinfect harvested seeds before germination.In this study,a technique of gliding arc plasma treatment was proposed and investigated.The experiment was conducted to treat Astragalus membranaceus(A.membranaceus)seeds that were artificially infected with Fusarium oxysporum(F.oxysporum).The plasma treatment duration varied from 30 s to 270 s.Direct and indirect treatments were compared to evaluate the inactivation efficiency of the F.oxysporum spores on the surface of seeds.The results indicated that the direct treatment behaved significantly better in disinfection than the indirect way.Meanwhile,experiments of the quantitative assessment of seed germination were also conducted,including the germination rate,the germination potential,and the germination index.The results showed that the inactivation efficiency increased as the plasma treatment time was extended.When the treatment time was90 s,the inactivation efficiency reached more than 98%.The plasma treatment of 270 s had a complete devitalization of F.oxysporum spores on the surface of the seeds.After the treatment of 30 s and 90 s,the seed germination parameters improved significantly.This study verified the inactivation efficacy of gliding arc discharge plasma under atmospheric pressure.The technique of gliding arc treatment shows advantages of energy saving and adaptation and has the potential to be utilized in industry.展开更多
In this work, a novel direct current （DC） atmospheric pressure rotating gliding arc （RGA） plasma reactor has been developed for plasma-assisted chemical reactions. The influence of the gas composition and the gas ...In this work, a novel direct current （DC） atmospheric pressure rotating gliding arc （RGA） plasma reactor has been developed for plasma-assisted chemical reactions. The influence of the gas composition and the gas flow rate on the arc dynamic behaviour and the formation of reactive species in the N2 and air gliding arc plasmas has been investigated by means of electrical signals, high speed photography, and optical emission spectroscopic diagnostics. Compared to conventional gliding arc reactors with knife-shaped electrodes which generally require a high flow rate （e.g., 10-20 L/min） to maintain a long arc length and reasonable plasma discharge zone, in this RGA system, a lower gas flow rate （e.g., 2 L/min） can also generate a larger effective plasma reaction zone with a longer arc length for chemical reactions. Two different motion patterns can be clearly observed in the N2 and air RGA plasmas. The time-resolved arc voltage signals show that three different arc dynamic modes, the arc restrike mode, takeover mode, and combined modes, can be clearly identified in the RGA plasmas. The occurrence of different motion and arc dynamic modes is strongly dependent on the composition of the working gas and gas flow rate.展开更多
Plasma methane (CH_4) conversion in gliding arc discharge was examined. Theresult data of experiments regarding the performance of gliding arc discharge were presented in thispaper. A simulation which is consisted som...Plasma methane (CH_4) conversion in gliding arc discharge was examined. Theresult data of experiments regarding the performance of gliding arc discharge were presented in thispaper. A simulation which is consisted some chemical kinetic mechanisms has been provided toanalyze and describe the plasma process. The effect of total gas flow rate and input frequencyrefers to power consumption have been studied to evaluate the performance of gliding arc plasmasystem and the reaction mechanism of decomposition. Experiment results indicated that the maximumconversion of CH_4 reached 50% at the total gas flow rate of 1 L/min. The plasma reaction wasoccurred at the atmospheric pressure and the main products were C (solid), hydrogen, and acetylene(C_2H_2). The plasma reaction of methane conversion was exothermic reaction which increased theproduct stream temperature around 30-50℃.展开更多
a gliding arc driven by the transverse magnetic field was ignited between the electrodes with a complicated shape at atmospheric pressure and a non-equilibrium plasma was gencrated. Under our experimental conditions, ...a gliding arc driven by the transverse magnetic field was ignited between the electrodes with a complicated shape at atmospheric pressure and a non-equilibrium plasma was gencrated. Under our experimental conditions, a phenomenon was clearly observed where the arc power decreased with the increase in arc voltage. As the arc voltage was higher than 3.375 kV, the are power acquired from the power supply decreased, and the arc plasma began to switch to a non-equilibrium phase. The existence of the non-equilibrium arc plasma was very short, about 10 ms in one gliding arc discharge cycle.展开更多
Decomposition of chlorinated hydrocarbons, CCl4 and CHCl3, in gliding plasma was examined. The effects of initial concentrations, total gas flow rates, and power consumption have been investigated. The conversion resu...Decomposition of chlorinated hydrocarbons, CCl4 and CHCl3, in gliding plasma was examined. The effects of initial concentrations, total gas flow rates, and power consumption have been investigated. The conversion result was relatively high. It reached 80% for CCl4 and 97% for CHCl3. Using atmospheric air as the carrier gas, the plasma reaction occurred at exothermic reaction and the main products were CO2, CO, and Cl2. Transformation into CCl4 was also detected for CHCl3 decomposition reaction. The conversion of CCh and CHCl3 were increased with the increasing applied frequency and decreasing total gas flow rate.展开更多
The simultaneous removal of ethyl acetate, benzene and toluene with relatively low or high initial concentration is studied using a laboratory scale gliding arc gas discharge (GA) reactor. Good decomposition efficienc...The simultaneous removal of ethyl acetate, benzene and toluene with relatively low or high initial concentration is studied using a laboratory scale gliding arc gas discharge (GA) reactor. Good decomposition efficiencies are obtained which proves that the GA is effective for the treatment of volatile organic compounds (VOCs) with either low or high concentration. A theoretical decomposition mechanism is proposed based on detection of the species in the plasma region and analysis of the decomposition by-products. This preliminary investigation reveals that the GA has potential to be applied to the treatment of exhaust air during color printing and coating works, by either direct removal or combination with activated carbon adsorption/desorption process.展开更多
A gliding arc plasma fuel atomization actuator suitable for aeroengines was designed,and a gliding arc plasma fuel spray experimental platform was built to address the fuel atomization problem in aeroengine combustion...A gliding arc plasma fuel atomization actuator suitable for aeroengines was designed,and a gliding arc plasma fuel spray experimental platform was built to address the fuel atomization problem in aeroengine combustion chambers.The spray characteristics for different airflows,fuel flows,and discharge voltages were analyzed using laser particle size analysis.The research shows that the fuel atomization effect is improved from the increased airflow.The decreased fuel flow not only reduces the injection pressure of the fuel but also changes the discharge mode of the gliding arc,which affects reductions in the discharge power and inhibits fuel atomization.Gliding arc discharges accelerate the breaking,atomization,and evaporation of fuel droplets while reducing the particle size,which increases the proportion of small droplets.Compared with the working conditions of plasma-assisted atomization without the gliding arc,the D0.5,D0.9,and average particle size of the fuel droplets are reduced by 4.7%,6.5%,and 4.1%,respectively,when the modulation voltage of the gliding arc power supply is 200 V.展开更多
The effects of feed gas flow rate and operating current on the electrical characteristics and dynamic behavior of a rotating gliding arc （RGA） plasma codriven by a magnetic field and tangential flow were investigate...The effects of feed gas flow rate and operating current on the electrical characteristics and dynamic behavior of a rotating gliding arc （RGA） plasma codriven by a magnetic field and tangential flow were investigated.The operating current has been shown to significantly affect the time-resolved voltage waveforms of the discharge,particularly at flow rate =21 min^-1.When the current was lower than 140 mA,sinusoidal waveforms with regular variation periods of 13.5-17.0 ms can be observed （flow rate =21 min^-1）.The restrike mode characterized by serial sudden drops of voltage appeared under all studied conditions.Increasing the flow rate from 8 to 121 min^-1 （at the same current） led to a shift of arc rotation mode which would then result in a significant drop of discharge voltage （around 120-200 V）.For a given flow rate,the reduction of current resulted in a nearly linear increase of voltage.展开更多
Stable combustion in an afterburner can help increase the thrust of the engine in a short time,thereby improving the maneuverability of a fighter.To improve the ignition performance of an afterburner,a twin-duct ignit...Stable combustion in an afterburner can help increase the thrust of the engine in a short time,thereby improving the maneuverability of a fighter.To improve the ignition performance of an afterburner,a twin-duct ignition platform was designed to study the performance of a gliding arc plasma igniter in close-to-real afterburner conditions.The research was carried out by a combination of experiments and simulations.The working environment of the igniter was explored through a numerical simulation.The results showed that the airflow ejected from the radiating holes formed a swirling sheath,which increased the anti-interference ability of the airflow jet.The influence of the pressure difference between the inlet and outlet of the igniter(Δp),the flow rate outside the igniter outlet(W_(2)),and the installation angle(α)on the singlecycle discharge energy(E)as well as the maximum arc length(L)were studied through experiments.Three stages were identified:the airflow breakdown stage,the arc evolution stage,and the arc fracture stage.E and L increased by 107.3%and 366.2%,respectively,withΔp increasing from 10 to 70 Torr.The relationship between L andΔp obtained by data fitting is L=3-2.47/(1+(Δp/25)^(4)).The relationship of L at differentαis L_(α=0°)>(L_(α=45°)and L_(α=135°))>L_(α=180°)>L_(α=90°).E and L decrease by 18.2%and 37.3%,respectively,whenΔp=45 Torr and W_(2) is increased from 0 to 250 l min^(-1).展开更多
Atmospheric pressure air/Ar/H_2O gliding arc discharge plasma is produced by a pulsed dc power supply. An optical emission spectroscopic（OES） diagnostic technique is used for the characterization of plasmas and for ...Atmospheric pressure air/Ar/H_2O gliding arc discharge plasma is produced by a pulsed dc power supply. An optical emission spectroscopic（OES） diagnostic technique is used for the characterization of plasmas and for identifications of OH and O radicals along with other species in the plasmas. The OES diagnostic technique reveals the excitation Tx？≈？5550–9000 K, rotational Tr？≈？1350–2700 K and gas Tg？≈？850–1600 K temperatures, and electron density n？（1.1-1.9） ′101 4 cm^（-3） e under different experimental conditions. The production and destruction of OH and O radicals are investigated as functions of applied voltage and air flow rate. Relative intensities of OH and O radicals indicate that their production rates are increased with increasing Ar content in the gas mixture and applied voltage. nereveals that the higher densities of OH and O radicals are produced in the discharge due to more effective electron impact dissociation of H_2O and O_2 molecules caused by higher kinetic energies as gained by electrons from the enhanced electric field as well as by enhanced n e.The productions of OH and O are decreasing with increasing air flow rate due to removal of Joule heat from the discharge region but enhanced air flow rate significantly modifies discharge maintenance properties. Besides, Tgsignificantly reduces with the enhanced air flow rate. This investigation reveals that Ar plays a significant role in the production of OH and O radicals.展开更多
Mutual effects between a gliding arc(GA)discharge at atmospheric pressure and a premixed CH_(4)/air flame were experimentally investigated.Effects of the flame on the GA were studied using simultaneous measurements of...Mutual effects between a gliding arc(GA)discharge at atmospheric pressure and a premixed CH_(4)/air flame were experimentally investigated.Effects of the flame on the GA were studied using simultaneous measurements of the current,the voltage,and the instantaneous images of the plasma columns.The GA in the flame has a thicker and more diffusive plasma column,and it is more frequently ignited at a smaller breakdown voltage than that in the air.The GA extension velocity and the gliding velocity in the flame are larger than those in the air.The electrode voltage drop of the GA discharge in the flame is about 160 V,whereas that in the air is about 220 V.Compared with the GA in the air,the different features of the GA in the flame can be explained by high-temperature,weakly ionized,and species-abundant environment that are generated by the premixed CH_(4)/air flame.Effects of the gliding arc discharge on the premixed flames were demonstrated using planar laser-induced fluorescence of hydroxyl radicals(OH)and formaldehyde(CH_(2)O).OH and CH_(2)O can be formed in the CH_(4)/air mixture in the presence of the GA due to kinetic effects,and the increase of OH and CH_(2)O shows the great potential of the GA for combustion enhancement.展开更多
Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether(DME).A systemic procedure was employed to determine the suitable experimental conditions.It was found tha...Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether(DME).A systemic procedure was employed to determine the suitable experimental conditions.It was found that DME conversion first increased up to the maximum and then decreased slightly with the increase of added water and air.The increase of total feed gas flow rate resulted in the decrease of DME conversion and hydrogen yield,but hydrogen energy consumption dropped down to the lowest as total feed gas flow rate increased to76 ml·min 1.Larger electrode gap and higher discharge voltage were advantageous.Electrode shape had an important effect on the conversion of DME and production of H2.Among the five electrodes,electrode 2#with valid length of 55 mm and the radian of 34 degrees of the top electrode section was the best option,which enhanced obviously the conversion of DME.展开更多
The gliding arc is an important approach to production of non-thermal plasma at atmospheric pressure, it can offer high-energy efficiency and high-electivity for chemical reactions. In this paper, the gliding arc driv...The gliding arc is an important approach to production of non-thermal plasma at atmospheric pressure, it can offer high-energy efficiency and high-electivity for chemical reactions. In this paper, the gliding arc driven by the transverse magnetic field is described and its velocity is measured by using a photo-multiplier. The mean velocity of the gliding arc increases with increasing magnetic induced-intensity, and its value varies from 7.8 m/s to 32 m/s.展开更多
In this work,a gas-solid two-phase gliding arc discharge(GS-GAD)reactor was built.Gliding arc was formed in the gap between the blade electrodes,and solid powder was deposited on the sieve plate positioned beneath the...In this work,a gas-solid two-phase gliding arc discharge(GS-GAD)reactor was built.Gliding arc was formed in the gap between the blade electrodes,and solid powder was deposited on the sieve plate positioned beneath the blade electrodes.A range of experimental parameters,including the inter-electrode spacing,gas flow rate,applied voltage,and the type of the powder,were systematically varied to elucidate the influence of solid powder matter on the dynamics of gliding arc discharge(GAD).The discharge images were captured by ICCD and digital camera to investigate the mass transfer characteristics of GS-GAD,and the electrical parameters,such as the effective values of voltage,current,and discharge power were record to reveal the discharge characteristics of GS-GAD.The results demonstrate that powder undergoes spontaneous movement towards the upper region of the gliding arc due to the influence of electric field force.Increasing the discharge voltage,decreasing relative dielectric constant of the powder and reducing the electrode-to-sieve-plate distance all contribute to a greater involvement of powder in the GAD process,subsequently resulting in an enhanced powder concentration within the GAD region.Additionally,powder located beneath the gliding arc experiences downward resistance caused by the opposing gas flow and arc.Excessive gas flow rate notably hampers the powder concentration within the discharge region,and the velocity of powder motion in the upper part of the GAD region is reduced.Under the condition of electrode-to-sieve-plate distance of 30 mm,gas flow rate of 1.5 L/min,and peak-to-peak voltage of 31 kV,the best combination of arc gliding and powder spark discharge phenomena can be achieved with the addition of Al_(2)O_(3) powder.展开更多
Highly efficient and green ammonia production is an important demand for modern agriculture.In this study,a two-step ammonia production method is developed using a gliding arc discharge in combination with Cu/Cu_(2)O ...Highly efficient and green ammonia production is an important demand for modern agriculture.In this study,a two-step ammonia production method is developed using a gliding arc discharge in combination with Cu/Cu_(2)O electrocatalysis.In this method,NO_(x)is provided by the gliding arc discharge and then electrolyzed by Cu/Cu_(2)O after alkaline absorption.The electrical characteristics,the optical characteristics and the NO_(x)production are investigated in discharges at different input voltage and the gas flow.The dependence of ammonia production through Cu/Cu_(2)O electrocatalysis on pH value and reduction potential are determined by colorimetric method.In our study,two discharge modes are observed.At high input voltage and low gas flow,the discharge is operated with a stable plasma channel which is called the steady arc gliding discharge mode(A-G mode).As lowering input voltage and raising gas flow,the plasma channel is destroyed and high frequency breakdown occurs instead,which is known as the breakdown gliding discharge mode(B-G mode).The optimal NO_(x)production of 7.34 mmol h^(-1)is obtained in the transition stage of the two discharge modes.The ammonia yield reaches0.402 mmol h^(-1)cm^(-2)at pH value of 12.7 and reduction potential of-1.0 V versus reversible hydrogen electrode(RHE).展开更多
基金financially supported by the National Natural Science Foundation of China(11475041,U21A20323)Kunlun Talent Program of Qinghai Province,Qinghai Provincial Science and Technology Project(2024-QY-203)Sci-Tech Project of Qinghai Salt Lake Industry Co.,Ltd.(E141GH01).
文摘1.Introduction Magnesium oxide(MgO)has attracted considerable attention in recent years due to its economic viability,excellent biocompatibil-ity,chemical stability,and non-toxic,odorless nature[1,2].These inherent properties position it as a promising candidate for various applications.
基金Project supported by the National Natural Science Foundation of China(No.50476058)Natural Science Foundation of Zhejiang Province(No.X506214)
文摘PCDD/Fs have been become a serious issue because of their toxicological effects and associated adverse health implications. In this study, the gliding arc plasma was tested for treatment of polychlorinated dibenzo-p-dioxins （PCDDs） and polychlorinated dibenzofurans （PCDFs）, which was synthesized from pentachlorophenol in atmospheric condition at 350℃ with or without the catalysis of CuCl2. From the experiment, we found that the destruction efficiency of PCDD/F homologues after gliding was discharge ranged from 25% to 79%. This result demonstrates that gliding arc plasma is an effective technology to decompose PCDDs/Fs in flue gas. A plausible degradation mechanism for PCDD/Fs by gliding arc was discussed. Finally, a multistage reactor structure of gliding arc was proposed to upgrade removal efficiency for PCDD/Fs.
基金Partial financial support has been provided by the Ministry of Science and Technology, Republic of Bangladesh: 39.00.0000.09.06.79.2017/2/98ESBangladesh Council for Scientific and Industrial Research (BCSIR) for providing Professor Abdullah Al-Muti Sharfuddin fellowship
文摘Wheat （Triticum aestivum） seeds were treated with atmospheric pressure gliding arc discharge plasmas to investigate the effects on water absorption, seed germination rate, seedling growth and yield in wheat. The surface architectures and functionalities of the seeds were found to modify due to plasma treatments. 6 rain treatment was provided 95%-100% germination rate. For the treatment duration of 3 and 9 rain the growth activity, dry matter accumulation, leaves chlorophyll contents, longest spikes, number of spikes/spikelet and total soluble protein content in shoots were improved. The grain yield of wheat was increased ,--20% by 6 min treatment with H2O/O2 plasma with respect to control.
基金supported by National Natural Science Foundation of China(Nos.21176175,- 20606023)
文摘Methane conversion has been studied using gliding arc plasma in the presence of argon.The process was conducted at atmospheric pressure and ambient temperature.The focus of this research was to develop a process of converting methane to C2 hydrocarbons and hydrogen. The main parameters,including the CH4/Ar mole ratio,the CH4 flow rate,the input voltage,and the minimum electrode gap,were varied to investigate their effects on methane conversion rate, product distribution,energy consumption,carbon deposit,and reaction stability.The specific energy requirement（SER） was used to express the energy utilization efficiency of the process and provided a practical guidance for optimizing reaction conditions for improving energy efficiency. It was found that the carbon deposition was not conducive to methane conversion,and the gliding arc plasma discharge reached a stable state twelve minutes later.Optimum conditions for methane conversion were suggested.The maximum methane conversion rate of 43.39%was obtained under the optimum conditions.Also,C2 hydrocarbons selectivity,C2 hydrocarbons yield,H2 selectivity, H2 yield and SER were 87.20%,37.83%,81.28%,35.27%,and 2.09 MJ/mol,respectively.
基金supported by the National Natural Science Foundation of China(Nos.90205026,10375082)
文摘A gliding arc discharge plasma and its characteristics are described. Analysis of the production principle of the plasma is presented. Some experimental results about two novel types of the gliding arc plasma generator have been obtained. These types of gliding arc plasma axe potentially usable in the chemical industry and environmental engineering.
文摘In agriculture production,plant health is threatened by pathogens parasitic on seeds;hence,it is necessary to disinfect harvested seeds before germination.In this study,a technique of gliding arc plasma treatment was proposed and investigated.The experiment was conducted to treat Astragalus membranaceus(A.membranaceus)seeds that were artificially infected with Fusarium oxysporum(F.oxysporum).The plasma treatment duration varied from 30 s to 270 s.Direct and indirect treatments were compared to evaluate the inactivation efficiency of the F.oxysporum spores on the surface of seeds.The results indicated that the direct treatment behaved significantly better in disinfection than the indirect way.Meanwhile,experiments of the quantitative assessment of seed germination were also conducted,including the germination rate,the germination potential,and the germination index.The results showed that the inactivation efficiency increased as the plasma treatment time was extended.When the treatment time was90 s,the inactivation efficiency reached more than 98%.The plasma treatment of 270 s had a complete devitalization of F.oxysporum spores on the surface of the seeds.After the treatment of 30 s and 90 s,the seed germination parameters improved significantly.This study verified the inactivation efficacy of gliding arc discharge plasma under atmospheric pressure.The technique of gliding arc treatment shows advantages of energy saving and adaptation and has the potential to be utilized in industry.
基金supported by National Natural Science Foundation of China(No.51576174)the Specialized Research Fund for the Doctoral Program of Higher Education of China(No.20120101110099)the Fundamental Research Funds for the Central Universities(No.2015FZA4011)
文摘In this work, a novel direct current （DC） atmospheric pressure rotating gliding arc （RGA） plasma reactor has been developed for plasma-assisted chemical reactions. The influence of the gas composition and the gas flow rate on the arc dynamic behaviour and the formation of reactive species in the N2 and air gliding arc plasmas has been investigated by means of electrical signals, high speed photography, and optical emission spectroscopic diagnostics. Compared to conventional gliding arc reactors with knife-shaped electrodes which generally require a high flow rate （e.g., 10-20 L/min） to maintain a long arc length and reasonable plasma discharge zone, in this RGA system, a lower gas flow rate （e.g., 2 L/min） can also generate a larger effective plasma reaction zone with a longer arc length for chemical reactions. Two different motion patterns can be clearly observed in the N2 and air RGA plasmas. The time-resolved arc voltage signals show that three different arc dynamic modes, the arc restrike mode, takeover mode, and combined modes, can be clearly identified in the RGA plasmas. The occurrence of different motion and arc dynamic modes is strongly dependent on the composition of the working gas and gas flow rate.
文摘Plasma methane (CH_4) conversion in gliding arc discharge was examined. Theresult data of experiments regarding the performance of gliding arc discharge were presented in thispaper. A simulation which is consisted some chemical kinetic mechanisms has been provided toanalyze and describe the plasma process. The effect of total gas flow rate and input frequencyrefers to power consumption have been studied to evaluate the performance of gliding arc plasmasystem and the reaction mechanism of decomposition. Experiment results indicated that the maximumconversion of CH_4 reached 50% at the total gas flow rate of 1 L/min. The plasma reaction wasoccurred at the atmospheric pressure and the main products were C (solid), hydrogen, and acetylene(C_2H_2). The plasma reaction of methane conversion was exothermic reaction which increased theproduct stream temperature around 30-50℃.
文摘a gliding arc driven by the transverse magnetic field was ignited between the electrodes with a complicated shape at atmospheric pressure and a non-equilibrium plasma was gencrated. Under our experimental conditions, a phenomenon was clearly observed where the arc power decreased with the increase in arc voltage. As the arc voltage was higher than 3.375 kV, the are power acquired from the power supply decreased, and the arc plasma began to switch to a non-equilibrium phase. The existence of the non-equilibrium arc plasma was very short, about 10 ms in one gliding arc discharge cycle.
文摘Decomposition of chlorinated hydrocarbons, CCl4 and CHCl3, in gliding plasma was examined. The effects of initial concentrations, total gas flow rates, and power consumption have been investigated. The conversion result was relatively high. It reached 80% for CCl4 and 97% for CHCl3. Using atmospheric air as the carrier gas, the plasma reaction occurred at exothermic reaction and the main products were CO2, CO, and Cl2. Transformation into CCl4 was also detected for CHCl3 decomposition reaction. The conversion of CCh and CHCl3 were increased with the increasing applied frequency and decreasing total gas flow rate.
基金Project (No. 50476058) supported by the National Natural ScienceFoundation of China
文摘The simultaneous removal of ethyl acetate, benzene and toluene with relatively low or high initial concentration is studied using a laboratory scale gliding arc gas discharge (GA) reactor. Good decomposition efficiencies are obtained which proves that the GA is effective for the treatment of volatile organic compounds (VOCs) with either low or high concentration. A theoretical decomposition mechanism is proposed based on detection of the species in the plasma region and analysis of the decomposition by-products. This preliminary investigation reveals that the GA has potential to be applied to the treatment of exhaust air during color printing and coating works, by either direct removal or combination with activated carbon adsorption/desorption process.
基金supported by National Natural Science Foundation of China(Nos.91741112 and 52276142)。
文摘A gliding arc plasma fuel atomization actuator suitable for aeroengines was designed,and a gliding arc plasma fuel spray experimental platform was built to address the fuel atomization problem in aeroengine combustion chambers.The spray characteristics for different airflows,fuel flows,and discharge voltages were analyzed using laser particle size analysis.The research shows that the fuel atomization effect is improved from the increased airflow.The decreased fuel flow not only reduces the injection pressure of the fuel but also changes the discharge mode of the gliding arc,which affects reductions in the discharge power and inhibits fuel atomization.Gliding arc discharges accelerate the breaking,atomization,and evaporation of fuel droplets while reducing the particle size,which increases the proportion of small droplets.Compared with the working conditions of plasma-assisted atomization without the gliding arc,the D0.5,D0.9,and average particle size of the fuel droplets are reduced by 4.7%,6.5%,and 4.1%,respectively,when the modulation voltage of the gliding arc power supply is 200 V.
基金supported by National Natural Science Foundation of China(51576174)
文摘The effects of feed gas flow rate and operating current on the electrical characteristics and dynamic behavior of a rotating gliding arc （RGA） plasma codriven by a magnetic field and tangential flow were investigated.The operating current has been shown to significantly affect the time-resolved voltage waveforms of the discharge,particularly at flow rate =21 min^-1.When the current was lower than 140 mA,sinusoidal waveforms with regular variation periods of 13.5-17.0 ms can be observed （flow rate =21 min^-1）.The restrike mode characterized by serial sudden drops of voltage appeared under all studied conditions.Increasing the flow rate from 8 to 121 min^-1 （at the same current） led to a shift of arc rotation mode which would then result in a significant drop of discharge voltage （around 120-200 V）.For a given flow rate,the reduction of current resulted in a nearly linear increase of voltage.
基金supported by National Science and Technology Major Project (No. 2017-Ⅲ-0007-0033)
文摘Stable combustion in an afterburner can help increase the thrust of the engine in a short time,thereby improving the maneuverability of a fighter.To improve the ignition performance of an afterburner,a twin-duct ignition platform was designed to study the performance of a gliding arc plasma igniter in close-to-real afterburner conditions.The research was carried out by a combination of experiments and simulations.The working environment of the igniter was explored through a numerical simulation.The results showed that the airflow ejected from the radiating holes formed a swirling sheath,which increased the anti-interference ability of the airflow jet.The influence of the pressure difference between the inlet and outlet of the igniter(Δp),the flow rate outside the igniter outlet(W_(2)),and the installation angle(α)on the singlecycle discharge energy(E)as well as the maximum arc length(L)were studied through experiments.Three stages were identified:the airflow breakdown stage,the arc evolution stage,and the arc fracture stage.E and L increased by 107.3%and 366.2%,respectively,withΔp increasing from 10 to 70 Torr.The relationship between L andΔp obtained by data fitting is L=3-2.47/(1+(Δp/25)^(4)).The relationship of L at differentαis L_(α=0°)>(L_(α=45°)and L_(α=135°))>L_(α=180°)>L_(α=90°).E and L decrease by 18.2%and 37.3%,respectively,whenΔp=45 Torr and W_(2) is increased from 0 to 250 l min^(-1).
基金financial support has been provided by the University Grants Commission:A-663-5/52/UGC/Eng-9/2013 and A-670-5/52/UGC/Eng-4/2013,University of Rajshahi
文摘Atmospheric pressure air/Ar/H_2O gliding arc discharge plasma is produced by a pulsed dc power supply. An optical emission spectroscopic（OES） diagnostic technique is used for the characterization of plasmas and for identifications of OH and O radicals along with other species in the plasmas. The OES diagnostic technique reveals the excitation Tx？≈？5550–9000 K, rotational Tr？≈？1350–2700 K and gas Tg？≈？850–1600 K temperatures, and electron density n？（1.1-1.9） ′101 4 cm^（-3） e under different experimental conditions. The production and destruction of OH and O radicals are investigated as functions of applied voltage and air flow rate. Relative intensities of OH and O radicals indicate that their production rates are increased with increasing Ar content in the gas mixture and applied voltage. nereveals that the higher densities of OH and O radicals are produced in the discharge due to more effective electron impact dissociation of H_2O and O_2 molecules caused by higher kinetic energies as gained by electrons from the enhanced electric field as well as by enhanced n e.The productions of OH and O are decreasing with increasing air flow rate due to removal of Joule heat from the discharge region but enhanced air flow rate significantly modifies discharge maintenance properties. Besides, Tgsignificantly reduces with the enhanced air flow rate. This investigation reveals that Ar plays a significant role in the production of OH and O radicals.
基金financially supported by National Natural Science Foundation of China(Nos.12172379,12322211,and 11925207)。
文摘Mutual effects between a gliding arc(GA)discharge at atmospheric pressure and a premixed CH_(4)/air flame were experimentally investigated.Effects of the flame on the GA were studied using simultaneous measurements of the current,the voltage,and the instantaneous images of the plasma columns.The GA in the flame has a thicker and more diffusive plasma column,and it is more frequently ignited at a smaller breakdown voltage than that in the air.The GA extension velocity and the gliding velocity in the flame are larger than those in the air.The electrode voltage drop of the GA discharge in the flame is about 160 V,whereas that in the air is about 220 V.Compared with the GA in the air,the different features of the GA in the flame can be explained by high-temperature,weakly ionized,and species-abundant environment that are generated by the premixed CH_(4)/air flame.Effects of the gliding arc discharge on the premixed flames were demonstrated using planar laser-induced fluorescence of hydroxyl radicals(OH)and formaldehyde(CH_(2)O).OH and CH_(2)O can be formed in the CH_(4)/air mixture in the presence of the GA due to kinetic effects,and the increase of OH and CH_(2)O shows the great potential of the GA for combustion enhancement.
基金Supported by the National Natural Science Foundation of China(21176175,20606023)
文摘Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether(DME).A systemic procedure was employed to determine the suitable experimental conditions.It was found that DME conversion first increased up to the maximum and then decreased slightly with the increase of added water and air.The increase of total feed gas flow rate resulted in the decrease of DME conversion and hydrogen yield,but hydrogen energy consumption dropped down to the lowest as total feed gas flow rate increased to76 ml·min 1.Larger electrode gap and higher discharge voltage were advantageous.Electrode shape had an important effect on the conversion of DME and production of H2.Among the five electrodes,electrode 2#with valid length of 55 mm and the radian of 34 degrees of the top electrode section was the best option,which enhanced obviously the conversion of DME.
文摘The gliding arc is an important approach to production of non-thermal plasma at atmospheric pressure, it can offer high-energy efficiency and high-electivity for chemical reactions. In this paper, the gliding arc driven by the transverse magnetic field is described and its velocity is measured by using a photo-multiplier. The mean velocity of the gliding arc increases with increasing magnetic induced-intensity, and its value varies from 7.8 m/s to 32 m/s.
基金supported by 173 Program of China,and National Natural Science Foundation of China(No.92271116).
文摘In this work,a gas-solid two-phase gliding arc discharge(GS-GAD)reactor was built.Gliding arc was formed in the gap between the blade electrodes,and solid powder was deposited on the sieve plate positioned beneath the blade electrodes.A range of experimental parameters,including the inter-electrode spacing,gas flow rate,applied voltage,and the type of the powder,were systematically varied to elucidate the influence of solid powder matter on the dynamics of gliding arc discharge(GAD).The discharge images were captured by ICCD and digital camera to investigate the mass transfer characteristics of GS-GAD,and the electrical parameters,such as the effective values of voltage,current,and discharge power were record to reveal the discharge characteristics of GS-GAD.The results demonstrate that powder undergoes spontaneous movement towards the upper region of the gliding arc due to the influence of electric field force.Increasing the discharge voltage,decreasing relative dielectric constant of the powder and reducing the electrode-to-sieve-plate distance all contribute to a greater involvement of powder in the GAD process,subsequently resulting in an enhanced powder concentration within the GAD region.Additionally,powder located beneath the gliding arc experiences downward resistance caused by the opposing gas flow and arc.Excessive gas flow rate notably hampers the powder concentration within the discharge region,and the velocity of powder motion in the upper part of the GAD region is reduced.Under the condition of electrode-to-sieve-plate distance of 30 mm,gas flow rate of 1.5 L/min,and peak-to-peak voltage of 31 kV,the best combination of arc gliding and powder spark discharge phenomena can be achieved with the addition of Al_(2)O_(3) powder.
文摘Highly efficient and green ammonia production is an important demand for modern agriculture.In this study,a two-step ammonia production method is developed using a gliding arc discharge in combination with Cu/Cu_(2)O electrocatalysis.In this method,NO_(x)is provided by the gliding arc discharge and then electrolyzed by Cu/Cu_(2)O after alkaline absorption.The electrical characteristics,the optical characteristics and the NO_(x)production are investigated in discharges at different input voltage and the gas flow.The dependence of ammonia production through Cu/Cu_(2)O electrocatalysis on pH value and reduction potential are determined by colorimetric method.In our study,two discharge modes are observed.At high input voltage and low gas flow,the discharge is operated with a stable plasma channel which is called the steady arc gliding discharge mode(A-G mode).As lowering input voltage and raising gas flow,the plasma channel is destroyed and high frequency breakdown occurs instead,which is known as the breakdown gliding discharge mode(B-G mode).The optimal NO_(x)production of 7.34 mmol h^(-1)is obtained in the transition stage of the two discharge modes.The ammonia yield reaches0.402 mmol h^(-1)cm^(-2)at pH value of 12.7 and reduction potential of-1.0 V versus reversible hydrogen electrode(RHE).
