High harmonic generation（HHG） driven by intense frequency-comb laser fields can be dramatically enhanced via multiphoton resonance by tuning the carrier-envelope phase（CEP） shift, without increasing the driving in...High harmonic generation（HHG） driven by intense frequency-comb laser fields can be dramatically enhanced via multiphoton resonance by tuning the carrier-envelope phase（CEP） shift, without increasing the driving intensity. However,the multiphoton-resonant enhancement（MRE） factor in the realistic atomic hydrogen is much smaller than that in a twolevel system. To study the deviation, we present a theoretical investigation of the multiphoton resonance dynamics of three-level systems driven by intense frequency-comb laser fields. The many-mode Floquet theorem（MMFT） is employed to provide a nonperturbative and exact treatment of the interaction between the quantum system and the laser fields. The investigations show that the dipole interaction of a two-level system with the third level affects the multiphoton resonance dynamics and enhances the HHG spectra. It is the dipole interaction of the excited level of the two-level system with other levels that results in the smaller MRE factor in the realistic atomic system.展开更多
The frequency-comb structure in the extreme ultraviolet（XUV） and vacuum ultraviolet（VUV） regions can be realized by the high-order harmonic generation（HHG） process driven by frequency-comb fields, providing an a...The frequency-comb structure in the extreme ultraviolet（XUV） and vacuum ultraviolet（VUV） regions can be realized by the high-order harmonic generation（HHG） process driven by frequency-comb fields, providing an alternative approach for the measurement of an unknown frequency in XUV or VUV. We consider the case of two driving frequency-comb fields with the same repetition frequency and the carrier frequencies of fundamental-and third-harmonics, respectively.The many-mode Floquet theorem（MMFT） is employed to provide a nonperturbative and exact treatment of the interaction between a quantum system and the frequency-comb laser fields. Multiphoton transition paths involving both fundamentaland third-harmonic photons are opened due to the coupling of the third-harmonic frequency-comb field. The multiphoton transition paths are superpositioned when the carrier-envelope-phase shifts（CEPs） fulfill the matching condition. And the interference of the multiphoton transition paths can be controlled by tuning the relative envelope delay between the fields.We find that the quasienergy structure, as well as the multiphoton resonant high-order harmonic generation（HHG） spectra,driven by the two frequency-comb fields can be coherently controlled via the interference of multiphoton transition paths.It is also found that the spectral intensities of the generated harmonics can be modulated, and the modulation behavior is harmonic-sensitive.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11374239,21203144,and 11074199)the Doctoral Fund of Ministry of Education of China(Grant No.20120201120056)the Fundamental Research Funds for the Central Universities,China
文摘High harmonic generation（HHG） driven by intense frequency-comb laser fields can be dramatically enhanced via multiphoton resonance by tuning the carrier-envelope phase（CEP） shift, without increasing the driving intensity. However,the multiphoton-resonant enhancement（MRE） factor in the realistic atomic hydrogen is much smaller than that in a twolevel system. To study the deviation, we present a theoretical investigation of the multiphoton resonance dynamics of three-level systems driven by intense frequency-comb laser fields. The many-mode Floquet theorem（MMFT） is employed to provide a nonperturbative and exact treatment of the interaction between the quantum system and the laser fields. The investigations show that the dipole interaction of a two-level system with the third level affects the multiphoton resonance dynamics and enhances the HHG spectra. It is the dipole interaction of the excited level of the two-level system with other levels that results in the smaller MRE factor in the realistic atomic system.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11504288,11374239,11534008,and 91536115)the Fundamental Research Funds for the Central Universities,China
文摘The frequency-comb structure in the extreme ultraviolet（XUV） and vacuum ultraviolet（VUV） regions can be realized by the high-order harmonic generation（HHG） process driven by frequency-comb fields, providing an alternative approach for the measurement of an unknown frequency in XUV or VUV. We consider the case of two driving frequency-comb fields with the same repetition frequency and the carrier frequencies of fundamental-and third-harmonics, respectively.The many-mode Floquet theorem（MMFT） is employed to provide a nonperturbative and exact treatment of the interaction between a quantum system and the frequency-comb laser fields. Multiphoton transition paths involving both fundamentaland third-harmonic photons are opened due to the coupling of the third-harmonic frequency-comb field. The multiphoton transition paths are superpositioned when the carrier-envelope-phase shifts（CEPs） fulfill the matching condition. And the interference of the multiphoton transition paths can be controlled by tuning the relative envelope delay between the fields.We find that the quasienergy structure, as well as the multiphoton resonant high-order harmonic generation（HHG） spectra,driven by the two frequency-comb fields can be coherently controlled via the interference of multiphoton transition paths.It is also found that the spectral intensities of the generated harmonics can be modulated, and the modulation behavior is harmonic-sensitive.
