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Evaporable luminescent lanthanide complexes based on novel tridentate ligand 被引量:2
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作者 魏晨 姚肖男 +7 位作者 孙博勋 蔡泽伦 赵子丰 陈明星 卫慧波 刘志伟 卞祖强 黄春辉 《Journal of Rare Earths》 SCIE EI CAS CSCD 2017年第1期7-14,共8页
A novel tridentate ligand N-(6-(diphenylphosphoryl)pyridin-2-yl)-2,2,2-trifluoroacetamide (DPPOPFA) was designed and synthesized. Crystal structure of the ligand revealed the "keto" form of ligand in solid sta... A novel tridentate ligand N-(6-(diphenylphosphoryl)pyridin-2-yl)-2,2,2-trifluoroacetamide (DPPOPFA) was designed and synthesized. Crystal structure of the ligand revealed the "keto" form of ligand in solid state other than the "enor' one, and it was also found that two kinds of molecules with different conformations were connected by hydrogen bonding between amide N-H and phos- phoryl P=O. This ionic ligand was used to coordinate a variety of lanthanide ions, forming neutral 3:1 complexes. Absolute overall quantum yields of these complexes in solid states were 36% for Eu(III), 29% for Tb(III) and 3% for Dy(III) with lifetimes of 1.1, 1.1 and 0.087 ms, respectively. The complexes had excellent thermal stability and did not decompose till 370 ℃. And they could subli- mate in vacuum (1 ×10^-4 Pa) at 330℃ due to the weak molecular interaction. 展开更多
关键词 luminescent complex LANTHANIDE TRIDENTATE evaporable rare earths
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Radiative Coupled Evaporation Cooling Hydrogel for Above-Ambient Heat Dissipation and Flame Retardancy
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作者 Qin Ye Yimou Huang +4 位作者 Baojian Yao Zhuo Chen Changming Shi Brian WSheldon Meijie Chen 《Nano-Micro Letters》 2026年第2期368-382,共15页
By combining the merits of radiative cooling(RC)and evaporation cooling(EC),radiative coupled evaporative cooling(REC)has attracted considerable attention for sub-ambient cooling purposes.However,for outdoor devices,t... By combining the merits of radiative cooling(RC)and evaporation cooling(EC),radiative coupled evaporative cooling(REC)has attracted considerable attention for sub-ambient cooling purposes.However,for outdoor devices,the interior heating power would increase the working temperature and fire risk,which would suppress their above-ambient heat dissipation capabilities and passive water cycle properties.In this work,we introduced a REC design based on an all-in-one photonic hydrogel for above-ambient heat dissipation and flame retardancy.Unlike conventional design RC film for heat dissipation with limited cooling power and fire risk,REC hydrogel can greatly improve the heat dissipation performance in the daytime with a high workload,indicating a 12.0℃lower temperature than the RC film under the same conditions in the outdoor experiment.In the nighttime with a low workload,RC-assisted adsorption can improve atmospheric water harvesting to ensure EC in the daytime.In addition,our REC hydrogel significantly enhanced flame retardancy by absorbing heat without a corresponding temperature rise,thus mitigating fire risks.Thus,our design shows a promising solution for the thermal management of outdoor devices,delivering outstanding performance in both heat dissipation and flame retardancy. 展开更多
关键词 Radiative cooling Evaporation cooling Heat dissipation Photonic hydrogel Flame retardancy
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Nature-Inspired Upward Hanging Evaporator with Photothermal 3D Spacer Fabric for Zero-Liquid-Discharge Desalination
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作者 Ye Peng Yang Shao +3 位作者 Longqing Zheng Haoxuan Li Meifang Zhu Zhigang Chen 《Nano-Micro Letters》 2026年第1期545-561,共17页
While desalination is a key solution for global freshwater scarcity,its implementation faces environmental challenges due to concentrated brine byproducts mainly disposed of via coastal discharge systems.Solar interfa... While desalination is a key solution for global freshwater scarcity,its implementation faces environmental challenges due to concentrated brine byproducts mainly disposed of via coastal discharge systems.Solar interfacial evaporation offers sustainable management potential,yet inevitable salt nucleation at evaporation interfaces degrades photothermal conversion and operational stability via light scattering and pathway blockage.Inspired by the mangrove leaf,we propose a photothermal 3D polydopamine and polypyrrole polymerized spacer fabric(PPSF)-based upward hanging model evaporation configuration with a reverse water feeding mechanism.This design enables zero-liquiddischarge(ZLD)desalination through phase-separation crystallization.The interconnected porous architecture and the rough surface of the PPSF enable superior water transport,achieving excellent solar-absorbing efficiency of 97.8%.By adjusting the tilt angle(θ),the evaporator separates the evaporation and salt crystallization zones via controlled capillary-driven brine transport,minimizing heat dissipation from brine discharge.At an optimal tilt angle of 52°,the evaporator reaches an evaporation rate of 2.81 kg m^(−2) h^(−1) with minimal heat loss(0.366 W)under 1-sun illumination while treating a 7 wt%waste brine solution.Furthermore,it sustains an evaporation rate of 2.71 kg m^(−2) h^(−1) over 72 h while ensuring efficient salt recovery.These results highlight a scalable,energy-efficient approach for sustainable ZLD desalination. 展开更多
关键词 DESALINATION Solar interfacial evaporation Biomimetic design Zero liquid discharge Thermal management
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Preparation of Co/S co-doped carbon catalysts for excellent methylene blue degradation 被引量:3
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作者 Haixu Li Haobo He +7 位作者 Tiannan Jiang Yunfei Du Zhichen Wu Liang Xu Xinjie Wang Xiaoguang Liu Wanhua Yu Wendong Xue 《International Journal of Minerals,Metallurgy and Materials》 SCIE EI CAS 2025年第1期169-181,共13页
S and Co co-doped carbon catalysts were prepared via pyrolysis of MOF-71 and thiourea mixtures at 800℃at a mass ratio of MOF-71 to thiourea of 1:0.1 to effectively activate peroxymonosulfate(PMS)for methylene blue(MB... S and Co co-doped carbon catalysts were prepared via pyrolysis of MOF-71 and thiourea mixtures at 800℃at a mass ratio of MOF-71 to thiourea of 1:0.1 to effectively activate peroxymonosulfate(PMS)for methylene blue(MB)degradation.The effects of two different mixing routes were identified on the MB degradation performance.Particularly,the catalyst obtained by the alcohol solvent evaporation(MOF-AEP)mixing route could degrade 95.60%MB(50 mg/L)within 4 min(degradation rate:K=0.78 min^(-1)),which was faster than that derived from the direct grinding method(MOF-DGP,80.97%,K=0.39 min^(-1)).X-ray photoelectron spectroscopy revealed that the Co-S content of MOF-AEP(43.39at%)was less than that of MOF-DGP(54.73at%),and the proportion of C-S-C in MOF-AEP(13.56at%)was higher than that of MOF-DGP(10.67at%).Density functional theory calculations revealed that the adsorption energy of Co for PMS was -2.94 eV when sulfur was doped as C-S-C on the carbon skeleton,which was higher than that when sulfur was doped next to cobalt in the form of Co-S bond(-2.86 eV).Thus,the C-S-C sites might provide more contributions to activate PMS compared with Co-S.Furthermore,the degradation parameters,including pH and MOF-AEP dosage,were investigated.Finally,radical quenching experiments and electron paramagnetic resonance(EPR)measurements revealed that ^(1)O_(2)might be the primary catalytic species,whereas·O~(2-)might be the secondary one in degrading MB. 展开更多
关键词 advanced oxidation process alcohol solvent evaporation hydrogen bond S and Co co-doped carbon catalysts wastewater remediation
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An overview of photothermal materials for solar-driven interfacial evaporation 被引量:2
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作者 Yiming Fang Huimin Gao +4 位作者 Kaiting Cheng Liang Bai Zhengtong Li Yadong Zhao Xingtao Xu 《Chinese Chemical Letters》 2025年第3期6-15,共10页
The utilization of solar-driven interfacial evaporation technology is highly important in addressing the energy crisis and water scarcity,primarily because of its affordability and minimal energy usage.Enhancing the p... The utilization of solar-driven interfacial evaporation technology is highly important in addressing the energy crisis and water scarcity,primarily because of its affordability and minimal energy usage.Enhancing the performance of solar energy evaporation and minimizing material degradation during application can be achieved through the design of novel photothermal materials.In solar interfacial evaporation,photothermal materials exhibit a wide range of additional characteristics,but a systematic overview is lacking.This paper encompasses an examination of various categories and principles pertaining to photothermal materials,as well as the structural design considerations for salt-resistant materials.Additionally,we discuss the versatile uses of this appealing technology in different sectors related to energy and the environment.Furthermore,potential solutions to enhance the durability of photothermal materials are also highlighted,such as the rational design of micro/nano-structures,the use of adhesives,the addition of anti-corrosion coatings,and the preparation of self-healing surfaces.The objective of this review is to offer a viable resolution for the logical creation of high-performance photothermal substances,presenting a guide for the forthcoming advancement of solar evaporation technology. 展开更多
关键词 Solar-driven interfacial evaporation Desalination Wastewater treatment Photothermal material SALT-RESISTANCE Durability
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Warming-Induced Increase in Flooding in the Taklimakan Desert 被引量:1
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作者 Yanan Su Xin Wang +5 位作者 Xiangjun Luo Shengqian Chen Yaqi Chen Fan Yang Jiaqiang Lei Fahu Chen 《Journal of Earth Science》 2025年第3期1351-1354,共4页
The Taklimakan Desert,located in the heart of central Asia,covers approximately 330000 km^(2),making it China's largest desert and the world's second-largest shifting desert(Dong et al.,2024).With an average a... The Taklimakan Desert,located in the heart of central Asia,covers approximately 330000 km^(2),making it China's largest desert and the world's second-largest shifting desert(Dong et al.,2024).With an average annual precipitation of less than 100 mm and evaporation rates ranging from 2000 to 3000 mm(Yang et al.,2020),it is recognized as one of the driest regions on Earth,often referred to as the“sea of death”. 展开更多
关键词 evaporation rates warming induced dry region evaporation precipitation Taklimakan Desert shifting desert FLOODING
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Diagnostics of temperature and blue-shifted velocity using soft X-ray spectra from the Macao Science Satellite-1 被引量:2
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作者 JianPing Li Xu Yang +6 位作者 Dong Li JinHua Shen Lei Yang Ya Wang LianSheng Li YongQiang Shi HaiSheng Ji 《Earth and Planetary Physics》 2025年第3期740-751,共12页
Using the new soft X-ray data from the Macao Science Satellite-1,we studied a solar flare that occurred on 22 June 2023.We found that the centroids of the Ca(around 3.9 keV)and Fe(around 6.7 keV)line features exhibit ... Using the new soft X-ray data from the Macao Science Satellite-1,we studied a solar flare that occurred on 22 June 2023.We found that the centroids of the Ca(around 3.9 keV)and Fe(around 6.7 keV)line features exhibit a rapid shift toward higher energy channels during the flare's rising phase,followed by a gradual decrease during the decay phase.Through precise energy calibration,the centroids are determined with high accuracy.Temperature and velocity are then self-consistently derived by comparing the centroids with those calculated from the synthesized line features using the latest CHIANTI atomic database(ver.10.1).The calculated maximum velocity reaches up to 710±60 km s-1,which significantly exceeds the previously reported values.Our results suggest that the entire shift of soft X-ray lines may occur during the process of chromospheric evaporation. 展开更多
关键词 Macao Science Satellite-1 solar flares soft X-ray lines chromospheric evaporation
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Effects of pressure oscillations on impinging-jet atomization and spray combustion in liquid rocket engines 被引量:1
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作者 Zhili PENG Bo ZHONG +1 位作者 Xiaodong CHEN Longfei LI 《Chinese Journal of Aeronautics》 2025年第4期25-43,共19页
Combustion dynamics are a critical factor in determining the performance and reliabilityof a chemical propulsion engine.The underlying processes include liquid atomization,evaporation,mixing,and chemical reactions.Thi... Combustion dynamics are a critical factor in determining the performance and reliabilityof a chemical propulsion engine.The underlying processes include liquid atomization,evaporation,mixing,and chemical reactions.This paper presents a high-fidelity numerical study of liquidatomization and spray combustion under high-pressure conditions,emphasizing the effects of pres-sure oscillations on the flow evolution and combustion dynamics.The theoretical framework isbased on the three-dimensional conservation equations for multiphase flows and turbulent combus-tion.The numerical solution is achieved using a coupling method of volume-of-fluid and Lagran-gian particle tracking.The Zhuang-Kadota-Sutton(ZKS)high-pressure evaporation model andthe eddy breakup-Arrhenius combustion model are employed.Simulations are conducted for amodel combustion chamber with impinging-jet injectors using liquid oxygen and kerosene as pro-pellants.Both conditions with and without inlet and outlet pressure oscillations are considered.Thefindings reveal that pressure oscillations amplify flow fluctuations and can be characterized usingkey physical parameters such as droplet evaporation,chemical reaction,and chamber pressure.The spectral analysis uncovers the axial variations of the dominant and secondary frequenciesand their amplitudes in terms of the characteristic physical quantities.This research helps establisha methodology for exploring the coupling effect of liquid atomization and spray combustion.It alsoprovides practical insights into their responses to pressure oscillations during the occurrence ofcombustion instability.This information can be used to enhance the design and operation ofliquid-fueled propulsion engines. 展开更多
关键词 Liquid atomization Spray combustion Pressure oscillations High-pressure evaporation Combustion instability
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Enhancing wastewater treatment efficiency with stereoscopic hydrogel evaporators and renewable energy integration for sustainability
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作者 unxiao Wang Yue Tian +3 位作者 Yonghang Yu Liang Wang Guangmiao Qu Shengyang Yang 《Chinese Journal of Chemical Engineering》 2025年第4期38-46,共9页
Enhancing wastewater treatment efficiency through innovative technologies is paramount in addressing global environmental challenges.This study explores utilizing stereoscopic hydrogel evaporators combined with renewa... Enhancing wastewater treatment efficiency through innovative technologies is paramount in addressing global environmental challenges.This study explores utilizing stereoscopic hydrogel evaporators combined with renewable energy sources to optimize wastewater treatment processes.A cross-linked super absorbent polymer(SAP)hydrogel was synthesized using acrylic acid and 2-hydroxyethyl methacrylate monomers and integrated with a light-absorbing carbon membrane to form a solar-assisted evaporator(MSAP).The MSAP achieved a high evaporation rate of 3.08 kg m^(-2)·h^(-1)and a photothermal conversion efficiency of 94.27%.It demonstrated excellent removal efficiency for dye-polluted wastewater,significantly reducing concentrations of pollutants.The MSAP maintained high performance in outdoor conditions,showcasing its potential for real-world applications.This approach,incorporating both solar and wind energy,significantly boosts water evaporation rates and presents a promising,eco-friendly solution for sustainable wastewater treatment within the circular development framework. 展开更多
关键词 Stereoscopic hydrogel evaporator EVAPORATION Solar energy Waste water SUSTAINABILITY
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Experimental Study on Hepatotoxicity of Hemsleya sphaerocarpa Fractions in Normal Mice
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作者 Fajin LU Xiaoyi HUANG +8 位作者 Yanbing WEI Shuai HUANG Junchen WEI Zukang DENG Aipeng LI Lixin SUN Suoyi HUANG Lixiang LU Ran CHEN 《Medicinal Plant》 2025年第3期22-25,35,共5页
[Objectives]To investigate the effects of various extract fractions of Hemsleya sphaerocarpa and their mechanisms of action on hepatotoxicity in normal experimental mice and to provide a scientific foundation for the ... [Objectives]To investigate the effects of various extract fractions of Hemsleya sphaerocarpa and their mechanisms of action on hepatotoxicity in normal experimental mice and to provide a scientific foundation for the clinical application of H.sphaerocarpa.[Methods]The extracts were separated by vacuum rotary evaporation into aqueous,n-butanol,petroleum ether,and ethyl acetate fractions.The resulting extracts from various fractions were subsequently formulated into 10%drug solutions using a normal saline solution.These solutions were administered intragastrically to mice at a dosage of 0.1 mL/10 g once daily.After 14 d of intragastric administration,various indices were assessed,and serum samples were collected from the ocular region of the mice for analysis.[Results]15 g of the aqueous fraction,20 g of the n-butanol fraction,30 g of the petroleum ether fraction,and 20 g of the ethyl acetate fraction were obtained through the vacuum rotary evaporation method.After 14 d of intragastric administration,the serum biochemical indices of the mice were assessed.It was observed that alanine aminotransferase(ALT)levels significantly increased in the mice of experimental group.This finding suggests that the ethyl acetate,petroleum ether,and n-butanol extracts of H.sphaerocarpa may contribute to liver injury in the subjects.After 14 d of drug withdrawal,the ALT level in the ethyl acetate group exhibited a significant decrease,but remained elevated compared to those in the normal saline group.In contrast,the ALT levels in the n-butanol and petroleum ether groups also demonstrated a significant reduction and were marginally lower than those observed in the normal saline group.Furthermore,the body weights of the mice in both the petroleum ether and n-butanol groups did not show any significant changes throughout the duration of drug administration.[Conclusions]The liver injury in mice induced by the ethyl acetate extract of H.sphaerocarpa is characterized as the most severe and challenging to self-heal. 展开更多
关键词 Hemsleya sphaerocarpa EXTRACT VACUUM ROTARY EVAPORATION HEPATOTOXICITY
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Experimental and model research on the evaporation of loess-like sulfate saline soil considering the influence of initial salt content
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作者 ZHANG Yabin CHOU Yaling +2 位作者 ZHAO Dong WANG Lijie ZHANG Peng 《Journal of Arid Land》 2025年第7期912-932,共21页
Intense evaporation in areas with loess-like sulfate saline soils has resulted in significant ecological challenges that include water shortages and soil salinization.Investigating evaporation rate in loess-like sulfa... Intense evaporation in areas with loess-like sulfate saline soils has resulted in significant ecological challenges that include water shortages and soil salinization.Investigating evaporation rate in loess-like sulfate saline soils under varying salt contents carries crucial implications for understanding regional water loss processes,predicting soil salinization advancement,and formulating effective ecological management strategies.Therefore,this study sampled the loess-like sulfate saline soil that is widely distributed in western China as experimental materials and investigated the impact of different initial salt contents(0.00%,0.50%,1.50%,3.00%,and 5.00%)on the evaporation rate,water content,and temperature of soil.The results showed that the evaporation rate decreased with increasing initial salt content.After a salt accumulation layer formed on the soil surface,the water content of the surface soil fluctuated.An increase in the initial salt content resulted in a corresponding increase in the surface temperature.Considering the evaporation characteristics of loess-like sulfate saline soil and the impact of an anomalous increase in surface soil water content on soil surface resistance,this study proposed a modified evaporation model on the basis of Fujimaki's evaporation model of saline soil by introducing a correction coefficientβto modify the soil surface resistance.A comparison of the calculated evaporation rates before and after the modification with the measured evaporation rates revealed a significant improvement in the calculation accuracy of the modified model,indicating that the modified model is capable of more accurately simulating the evaporation rate of sulfate saline soil with different initial salt contents.This paper proposes an effective method for calculating the evaporation rate of loess-like sulfate saline soils,providing a theoretical basis for evaporation research in saline soil. 展开更多
关键词 loess-like sulfate saline soil evaporation rate salt accumulation layer salt crystallization evaporation model soil surface resistance air resistance
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Laser melting,evaporation,and fragmentation of nanoparticles:Experiments,modeling,and applications
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作者 Victor K.Pustovalov 《Nanotechnology and Precision Engineering》 2025年第2期146-191,共46页
This review examines the processes of laser heating,melting,evaporation,fragmentation,and breakdown of metal nanoparticles,as well as the dependences and values of the threshold laser parameters that initiate these pr... This review examines the processes of laser heating,melting,evaporation,fragmentation,and breakdown of metal nanoparticles,as well as the dependences and values of the threshold laser parameters that initiate these processes.Literature results are analyzed from experimental studies of these processes with gold,silver,and other nanoparticles,including laser surface melting and evaporation of nanoparticles and Coulomb fragmentation of nanoparticles by ultrashort laser pulses.A theoretical model and description of the thermal mechanisms of mentioned processes with metal(solid)nanoparticles in a liquid(solid)medium,initiated by the action of laser pulses with the threshold fluences,are presented.Comparison of the obtained results with experimental data confirms the accuracy of the model and makes it possible to use them to evaluate the parameters of laser thermal processing of nanoparticles.Applications of the processes include the laser melting,reshaping,and fragmentation of nanoparticles,the formation of nanostructures and nanonetworks,the laser processing of nanoparticles located on substrates,and their cladding on surfaces in various laser nanotechnologies.The use of laser ignition,combustion,and incandescence of nanoparticles is discussed,as is the use of nanoparticle-triggered laser breakdown for spectroscopy.These laser processes are used in photothermal nanotechnologies,nanoenergy,laser processing of nanoparticles,nonlinear optical devices,high-temperature material science,etc.In general,this review presents a modern picture of the state of laser technology and high-temperature processes with nanoparticles and their applications,being focused on the latest publications with an emphasis on recent results from 2021-2024. 展开更多
关键词 Laser HEATING MELTING EVAPORATION FRAGMENTATION NANOPARTICLE MODELING
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A Bionic Ripple Bamboo Based Solar Interface Evaporator for High Efficiency Seawater Desalination
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作者 Juan Li Hao Yao +3 位作者 Jieyao Su Nongchao Tan Tian Zhou Lei Shi 《Journal of Bionic Engineering》 2025年第6期3095-3107,共13页
The solar interfacial evaporation has a broad application prospect in the fields of steam generation and seawater desalination to deal with the global shortage of fresh-water resources.Bamboo is a great material for s... The solar interfacial evaporation has a broad application prospect in the fields of steam generation and seawater desalination to deal with the global shortage of fresh-water resources.Bamboo is a great material for solar interface evaporators because of its low thermal conductivity and inherent micro-channel porous structure.In this paper,a novel bamboo-based solar interface evaporator with a bionic ripple wave surface structure has been proposed.The subsequent evaporation experiments have been conducted to investigate the salt resistance,stability and water absorption of the bionic ripple bamboo based solar interface evaporator.The results have exhibited that the bamboo's water absorption has been enhanced after carbonization modification.Besides,it should be pointed out that this bamboo-based evaporator’s evaporation rate has dropped during the prolonged simulated seawater evaporation experiment,yet it remained fairly consistent at approximately 1.626 kg·m^(-2)·h^(-1).The appearance for this experimental phenomenon is the decrease of the floatability of the evaporator constricted by the stored water body absorbed by the evaporator and the deposition of NaCl crystals at the photothermal interface.Besides,compared with the plate-structure evaporator,the salt deposition in the evaporator equipped with the bionic ripple wave surface structure is greatly improved.In regard to its advantages in low cost,environmental friendliness,good salt tolerance and high evaporation rate,the bamboo-based solar interface evaporator with a bionic ripple wave surface structure can provide a potential solution to the global problem of fresh-water shortage. 展开更多
关键词 Photothermal interface evaporation BAMBOO-BASED Ripple structure Evaporation rate
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Development of a capillary bundle evaporation advanced mathematical modeling for 1,2-propylene glycol-glycerin mixtures in porous media
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作者 Bingbing Li Jiantong Li +3 位作者 Side Ren Shuo Gu Zhanjian Liu Liyan Liu 《Chinese Journal of Chemical Engineering》 2025年第4期261-273,共13页
Porous liquid-conducting micro-heat exchangers have garnered considerable attention for their role in efficient heat dissipation in small electronic devices.This demand highlights the need for advanced mathematical mo... Porous liquid-conducting micro-heat exchangers have garnered considerable attention for their role in efficient heat dissipation in small electronic devices.This demand highlights the need for advanced mathematical models to optimize the selection of mixed heat exchange media and equipment design.A capillary bundle evaporation model for porous liquid-conducting media was developed based on the conjugate mass transfer evaporation rate prediction model of a single capillary tube,supplemented by mercury injection experimental data.Theoretical and experimental comparisons were conducted using 1,2-propanediol-glycerol(PG-VG)mixtures at molar ratios of 1:9,3:7,5:5,and 7:3 at 120,150,and 180℃.The Jouyban-Acree model was implemented to enhance the evaporation rate predictions.For the 7:3 PG-VG mixture at 180℃under the experimental conditions of the thermal medium,the model's error reduced from 16.75%to 10.84%post-correction.Overall,the mean relative error decreased from 11.76%to 5.98%after correction. 展开更多
关键词 Evaporation in porous media Capillary bundle model 1 2-propylene glycol-glycerin Evaporation rate
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Efficient Preparation of Fermionic Superfluids in an Optical Dipole Trap through Reinforcement Learning
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作者 Yueyang Min Ziliang Li +4 位作者 Yi Zhong Jia-An Xuan Jian Lin Lei Feng Xiaopeng Li 《Chinese Physics Letters》 2025年第10期53-61,共9页
We demonstrate a reinforcement learning(RL)-based control framework for optimizing evaporative cooling in the preparation of strongly interacting degenerate Fermi gases of 6Li.Using a Soft Actor-Critic(SAC)algorithm,t... We demonstrate a reinforcement learning(RL)-based control framework for optimizing evaporative cooling in the preparation of strongly interacting degenerate Fermi gases of 6Li.Using a Soft Actor-Critic(SAC)algorithm,the system autonomously explores a high-dimensional parameter space to learn optimal cooling trajectories.Compared to conventional exponential ramps,our method achieves up to 130%improvement in atomic density within 0.5 second,revealing non-trivial control strategies that balance fast evaporation and thermalization.While our current optimization focuses on the evaporation stage,future integration of other cooling stages,such as gray molasses cooling,could further extend RL to the full preparation pipeline.Our result highlights the promise of RL as a general tool for closed-loop quantum control and automated calibration in complex atomic physics experiments. 展开更多
关键词 soft actor critic evaporative cooling optimizing evaporative cooling atomic density fermionic superfluids reinforcement learning exponential rampsour strongly interacting degenerate fermi gases
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Smoothed Particle Hydrodynamics(SPH)Simulations of Drop Evaporation:A Comprehensive Overview of Methods and Applications
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作者 Leonardo Di G.Sigalotti Carlos A.Vargas 《Computer Modeling in Engineering & Sciences》 2025年第3期2281-2337,共57页
The evaporation ofmicrometer and millimeter liquid drops,involving a liquid-to-vapor phase transition accompanied by mass and energy transfer through the liquid-vapor interface,is encountered in many natural and indus... The evaporation ofmicrometer and millimeter liquid drops,involving a liquid-to-vapor phase transition accompanied by mass and energy transfer through the liquid-vapor interface,is encountered in many natural and industrial processes as well as in numerous engineering applications.Therefore,understanding and predicting the dynamics of evaporating flows have become of primary importance.Recent efforts have been addressed using the method of Smoothed Particle Hydrodynamics(SPH),which has proven to be very efficient in correctly handling the intrinsic complexity introduced by the multiscale nature of the evaporation process.This paper aims to provide an overview of published work on SPH-based simulations related to the evaporation of drops suspended in static and convective environments and impacting on heated solid surfaces.After a brief theoretical account of the main ingredients necessary for the modeling of drop evaporation,the fundamental aspects of SPH are revisited along with the various existing formulations that have been implemented to address the challenges imposed by the physics of evaporating flows.In the following sections,the paper summarizes the results of SPH-based simulations of drop evaporation and ends with a few comments on the limitations of the current state-of-the-art SPHsimulations and future lines of research. 展开更多
关键词 Drop evaporation surface tension heat and mass transfer phase separation smoothed particle hydrodynamics(SPH) boiling evaporation explosive vaporization droplet/wall interaction
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Biomass-based 3D solar interface evaporators integrating efficient evaporation and power generation
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作者 Chen Zhang Sijie Zhuang +2 位作者 Lei Dai Zhu Long Zhibin He 《Journal of Energy Chemistry》 2025年第11期873-883,I0020,共12页
Global freshwater scarcity and energy shortages demand integrated solutions.To overcome limitations of traditional solar evaporators,such as salt accumulation,thermal dissipation,and material scalability issues,this s... Global freshwater scarcity and energy shortages demand integrated solutions.To overcome limitations of traditional solar evaporators,such as salt accumulation,thermal dissipation,and material scalability issues,this study presents a biomass-derived three-dimensional(3D)aerogel-based dual-function solar evaporator that simultaneously achieves ultra-high freshwater production and continuous electricity generation.By ingeniously integrating a superhydrophobic inner layer for thermal insulation and buoyancy with a hydrophilic photothermal outer layer for rapid water transport and solar absorption,our design overcomes the trade-offs between evaporation efficiency,salt resistance,and energy loss.The evaporator exhibits exceptional dual performance:an evaporation rate of 3.87 kg m^(-2)h-1(1 sun)and a sustained open-circuit voltage of 222.6 mV,surpassing most reported systems.This synergy originates from ion gradient-driven streaming potentials enabled by selective Na^(+) transport through–COOH/C–OH functionalized microchannels,as verified by molecular dynamics simulations.Crucially,the fabrication process utilizes low-cost biomass materials and scalable techniques,demonstrating significant potential for commercialization.This work not only provides a mechanistic understanding of ion-selective transport in dual-function evaporators but also establishes a paradigm for sustainable co-production of clean water and renewable energy,addressing two pressing global challenges through a single and scalable platform. 展开更多
关键词 DESALINATION Solar evaporators AEROGEL Biomass materials CO-PRODUCTION
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Drainage-induced arch hydrogel-based interfacial evaporator drives long-term stable solar evaporation
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作者 Zexiang Zhao Junqi Li +7 位作者 Fan Wang Puxin Tan Lu Wang Bo Wang Jingjing Jin Xiaoxue Wang Wenhe Zhang Chengbing Wang 《Journal of Energy Chemistry》 2025年第5期540-550,共11页
Hydrogel has developed into a very important platform in solar interface evaporator.However,the current hydrogel evaporators are usually three-dimensional evaporators,which will consume a lot of raw materials.Thus,a n... Hydrogel has developed into a very important platform in solar interface evaporator.However,the current hydrogel evaporators are usually three-dimensional evaporators,which will consume a lot of raw materials.Thus,a new two-dimensional hydrogel evaporator is urgently needed to alleviate this problem.Here,a double layer hydrogel evaporator was designed by twice vacuum filtration.Furthermore,through the arched design and the introduction of concentrated brine drainage system,the hydrogel evaporator has enhanced water transportation and tailored water transportation path.Such a unique drainage evaporation system greatly improves the stability of the evaporator.Thereby,a good balance is established between photothermal conversion and water supply,and solar energy is utilized efficiently.It can remain stable in continuous evaporation for up to 12 h with an excellent evaporation rate of 2.70 kg m^(-2)h^(-1)under 1 sun irradiation.Meanwhile,the drainage system realized the 1.8×10^(-10)mol m^(-2)s^(-1)diffusion flux of concentrated brine.Through one-time freeze-drying preparation,an arch-shaped drainage evaporator was used to prepare an evaporation area of more than 20 cm^(2).With the self-made condensate collecting device in outdoor environment,the fresh water yield reaches 7.5 L m^(-2)d^(-1).This provides a new scheme for building a new hydrogel evaporator and solving the fresh water crisis. 展开更多
关键词 Solar evaporation Drainage system Arch hydrogel SALT-TOLERANT ALGINATE
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Occurrence of flash drought in reservoirs in the semi-arid area of the CearáState,Brazil
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作者 Suellen Teixeira Nobre GONÇALVES Francisco das Chagas VASCONCELOS JÚNIOR +2 位作者 Cleiton da Silva SILVEIRA JoséMicael Ferreira da COSTA Antonio Duarte MARCOS JUNIOR 《Journal of Arid Land》 2025年第7期865-887,共23页
Precipitation is scarce in semi-arid areas,which results in serious drought.Occurrence of flash drought is quite often in these areas,and flash drought may also cause significant disasters.However,monitoring flash dro... Precipitation is scarce in semi-arid areas,which results in serious drought.Occurrence of flash drought is quite often in these areas,and flash drought may also cause significant disasters.However,monitoring flash drought is still weak and remains a challenge.This study aims to identify,evaluate,and monitor flash drought events that occurred from 1961 to 2020 in reservoirs of the CearáState,Brazil.The Christian's method,standardized precipitation index(SPI),standardized precipitation evapotranspiration index(SPEI),and evaporative demand drought index(EDDI)were used to assess the severity and persistence of flash drought.Moreover,analyses conducted in 2001,2008,2011,2012,2016,and 2020revealed the complexity and interaction of flash drought with environmental and meteorological factors.The results indicated that in dry years such as 2001,2012,and 2016,drought indices pointed to the intensification of drought conditions,with impacts on major reservoirs in the area,such as Banabuiú,Castanh?o,and Orós.Low precipitation,associated with high evaporative demand,intensified water stress,reducing water availability for the population and local ecosystems.In wet years such as 2008,2011,and 2020,SPEI and EDDI indicated higher moisture levels and drought relief,favoring the recovery of reservoirs.It was also observed that most flash drought episodes evolved into conventional droughts,highlighting their persistence and potential long-term impact.Moreover,the months of May and November presented a higher frequency of flash drought during the wet and dry periods,respectively,negatively impacting most of the studied reservoirs.These findings underscore the need for effective drought monitoring and mitigation strategies to reduce its impacts on agriculture and water resources in the semi-arid area.Early detection and analysis of flash drought are important for improving water resource management and for continuous adaptation to changing drought conditions. 展开更多
关键词 water resources evaporative demand drought indices monitoring PRECIPITATION
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