The development of differential electrochemical mass spectrometry (DEMS) originated in the late 20th century[1–4],with its core objective being the integration of electrochemical processes with mass spectrometric det...The development of differential electrochemical mass spectrometry (DEMS) originated in the late 20th century[1–4],with its core objective being the integration of electrochemical processes with mass spectrometric detection to enable real-time tracking of reaction intermediates and products at the electrodes [5,6].DEMS was initially employed to study electrochemical processes in aqueous solutions,such as methanol oxidation [7].Recently,with the rapid development of new energy technologies,DEMS has been widely applied in the research and development of electrocatalysis,lithium-ion,sodium-ion,and metal-air batteries[8–16].展开更多
基金supported by the Jiangsu Province Carbon Peak and Neutrality Innovation Program (Industry Tackling on Prospect and Key Technology)(BE2022031-4,BE2022002-3)the National Natural Science Foundation of China (52173173,22572087)the State Key Laboratory of Materials-Oriented Chemical Engineering (SKL-MCE-24A16)。
文摘The development of differential electrochemical mass spectrometry (DEMS) originated in the late 20th century[1–4],with its core objective being the integration of electrochemical processes with mass spectrometric detection to enable real-time tracking of reaction intermediates and products at the electrodes [5,6].DEMS was initially employed to study electrochemical processes in aqueous solutions,such as methanol oxidation [7].Recently,with the rapid development of new energy technologies,DEMS has been widely applied in the research and development of electrocatalysis,lithium-ion,sodium-ion,and metal-air batteries[8–16].