A micropump induces the flow of its surrounding fluids and is extremely promising in a variety of applications such as chemical sensing or mass transportation. However, it is still challenging to manipulate its pumpin...A micropump induces the flow of its surrounding fluids and is extremely promising in a variety of applications such as chemical sensing or mass transportation. However, it is still challenging to manipulate its pumping direction. In this stud~ we examine a binary micropump based on perovskite and poly[(2-methoxy-5-ethylhexyloxy)-1,4-phenylenevinylene] (MEHPPV). The micropump is operational under the influence of light. Light exhibits significant versatility in controlling the pumping phenomenon of the micropump. It governs the start and stop and also regulates the velocity and directions. The direction control signifies immense opportunities for the development of micropumps with unprecedented pumping behaviors and functions (such as heartbeat-like pumping, rectification, and amplification). This makes them potentially useful in various fields. Hence, it is expected that the micropump reported in the current study could act as a key step towards the further development of more sophisticated micropumps for diverse applications.展开更多
It is well known that during CO2 geological storage, density-driven convective activity can significantly accelerate the dissolution of injected CO2 into water. This action could limit the escape of supercritical CO2 ...It is well known that during CO2 geological storage, density-driven convective activity can significantly accelerate the dissolution of injected CO2 into water. This action could limit the escape of supercritical CO2 from the storage formation through vertical pathways such as fractures, faults and abandoned wells, consequently increasing permanence and security of storage. First, we investigated the effect of numerical perturbation caused by time and grid resolution and the convergence criteria on the dissolution-diffusion-convection (DDC) process. Then, using the model with appropriate spatial and temporal resolution, some uncertainty parameters investigated in our previous paper such as initial gas saturation and model boundaries, and other factors such as relative liquid permeability and porosity modification were used to examine their effects on the DDC process. Finally, we compared the effect of 2D and 3D models on the simulation of the DDC process. The above modeling results should contribute to clear understanding and accurate simulation of the DDC process, especially the onset of convective activity, and the CO2 dissolution rate during the convection-dominated stage.展开更多
基金This work is supported by the National Natural Science Foundation of China (No. 21574094), the Natural Science Foundation of Jiangsu Province (No. BK20150314) and Collaborative Innovation Center (CIC) of Suzhou Nano Science. It is also supported by the 111 Project and a Project Funded by the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD), the Fund for Excellent Creative Research Teams of Jiangsu Higher Education Institutions and the project-sponsored by SRF for ROCS, SEM,
文摘A micropump induces the flow of its surrounding fluids and is extremely promising in a variety of applications such as chemical sensing or mass transportation. However, it is still challenging to manipulate its pumping direction. In this stud~ we examine a binary micropump based on perovskite and poly[(2-methoxy-5-ethylhexyloxy)-1,4-phenylenevinylene] (MEHPPV). The micropump is operational under the influence of light. Light exhibits significant versatility in controlling the pumping phenomenon of the micropump. It governs the start and stop and also regulates the velocity and directions. The direction control signifies immense opportunities for the development of micropumps with unprecedented pumping behaviors and functions (such as heartbeat-like pumping, rectification, and amplification). This makes them potentially useful in various fields. Hence, it is expected that the micropump reported in the current study could act as a key step towards the further development of more sophisticated micropumps for diverse applications.
基金This work was supported by the National Natural Science Foundation of China (Grant No. 40872158), China Geological Survey Project (Grant Nos. 1212011220914 and 1212011220794), and Librarian's Project of National Geological Library of China (Grant No. GZ201203).
文摘It is well known that during CO2 geological storage, density-driven convective activity can significantly accelerate the dissolution of injected CO2 into water. This action could limit the escape of supercritical CO2 from the storage formation through vertical pathways such as fractures, faults and abandoned wells, consequently increasing permanence and security of storage. First, we investigated the effect of numerical perturbation caused by time and grid resolution and the convergence criteria on the dissolution-diffusion-convection (DDC) process. Then, using the model with appropriate spatial and temporal resolution, some uncertainty parameters investigated in our previous paper such as initial gas saturation and model boundaries, and other factors such as relative liquid permeability and porosity modification were used to examine their effects on the DDC process. Finally, we compared the effect of 2D and 3D models on the simulation of the DDC process. The above modeling results should contribute to clear understanding and accurate simulation of the DDC process, especially the onset of convective activity, and the CO2 dissolution rate during the convection-dominated stage.