With the development of radioactive-ion-beam facilities,many exotic phenomena have been discovered or predicted in the nuclei far from the stability line,including cluster structure,shell structure,deformed halo,and s...With the development of radioactive-ion-beam facilities,many exotic phenomena have been discovered or predicted in the nuclei far from the stability line,including cluster structure,shell structure,deformed halo,and shape decoupling effects.The study of exotic nuclear phenomena is at the frontier of nuclear physics nowadays.The covariant density functional theory(CDFT)is one of the most successful microscopic models in describing the structure of nuclei in almost the whole nuclear chart.Within the framework of CDFT,toward a proper treatment of deformation and weak binding,the deformed relativistic Hartree-Bogoliubov theory in continuum(DRHBc)has been developed.In this contribution,we review the applications and extensions of the DRHBc theory to the study of exotic nuclei.The DRHBc theory has been used to investigate the deformed halos in B,C,Ne,Na,and Mg isotopes and the theoretical descriptions are reasonably consistent with available data.A DRHBc Mass Table Collaboration has been founded,aiming at a high precision nuclear mass table with deformation and continuum effects included,which is underway.By implementing the angular momentum projection based on the DRHBc theory,the rotational excitations of deformed halos have been investigated and it is shown that the deformed halos and shape decoupling effects also exist in the low-lying rotational excitation states of deformed halo nuclei.展开更多
In 2007,China surpassed the USA to become the largest carbon emitter in the world.China has promised a 60%–65%reduction in carbon emissions per unit GDP by 2030,compared to the baseline of 2005.Therefore,it is import...In 2007,China surpassed the USA to become the largest carbon emitter in the world.China has promised a 60%–65%reduction in carbon emissions per unit GDP by 2030,compared to the baseline of 2005.Therefore,it is important to obtain accurate dynamic information on the spatial and temporal patterns of carbon emissions and carbon footprints to support formulating effective national carbon emission reduction policies.This study attempts to build a carbon emission panel data model that simulates carbon emissions in China from 2000–2013 using nighttime lighting data and carbon emission statistics data.By applying the Exploratory Spatial-Temporal Data Analysis(ESTDA)framework,this study conducted an analysis on the spatial patterns and dynamic spatial-temporal interactions of carbon footprints from 2001–2013.The improved Tapio decoupling model was adopted to investigate the levels of coupling or decoupling between the carbon emission load and economic growth in 336 prefecture-level units.The results show that,firstly,high accuracy was achieved by the model in simulating carbon emissions.Secondly,the total carbon footprints and carbon deficits across China increased with average annual growth rates of 4.82%and 5.72%,respectively.The overall carbon footprints and carbon deficits were larger in the North than that in the South.There were extremely significant spatial autocorrelation features in the carbon footprints of prefecture-level units.Thirdly,the relative lengths of the Local Indicators of Spatial Association(LISA)time paths were longer in the North than that in the South,and they increased from the coastal to the central and western regions.Lastly,the overall decoupling index was mainly a weak decoupling type,but the number of cities with this weak decoupling continued to decrease.The unsustainable development trend of China’s economic growth and carbon emission load will continue for some time.展开更多
The progress from intelligent interactions requires electronic skin(E-skin)to shift from single-functional perception to multisensory capabilities.However,the intuitive and interference-free reading of multiple sensor...The progress from intelligent interactions requires electronic skin(E-skin)to shift from single-functional perception to multisensory capabilities.However,the intuitive and interference-free reading of multiple sensory signals without involving complex algorithms is a critical challenge.Herein,we propose a flexible multisensory E-skin by developing a highly homogeneous dispersion of BaTiO_(3)nanoparticles in polydimethylsiloxane dielectric layer.The E-skin is sensitive to externally applied pressure as well as temperature and can distinguish dual synergetic stimuli by the time decoupling effect.The pressure and temperature perception was achieved in an individual device,which greatly reduced the structural complexity compared with multifunctional integrated devices.The sensitivity of E-skin for pressure detection is as high as 0.0724 kPa^(−1)and the detection range reaches as wide as 15.625-10 MPa.The sensitivity to temperature detection is as high as−1.34℃^(−1)and the detection range reaches 20-200℃.More importantly,by equipping with a multilayer neural network,the evolution from tactile perception to advanced intelligent tactile cognition is demonstrated.展开更多
The past decade has witnessed the rapid increasement in power conversion efficiency of perovskite solar cells(PSCs).However,serious ion migration hampers their operational stability.Although dopants composed of varied...The past decade has witnessed the rapid increasement in power conversion efficiency of perovskite solar cells(PSCs).However,serious ion migration hampers their operational stability.Although dopants composed of varied cations and anions are introduced into perovskite to suppress ion migration,the impact of cations or anions is not individually explored,which hinders the evaluation of different cations and further application of doping strategy.Here we report that a special group of sulfonic anions(like CF_(3)SO_(3)^(-))successfully introduce alkaline earth ions(like Ca^(2+))into perovskite lattice compared to its halide counterparts.Furthermore,with effective crystallization regulation and defect passivation of sulfonic anions,perovskite with Ca(CF_(3)SO_(3))_(2)shows reduced PbI2 residue and metallic Pb0 defects;thereby,corresponding PSCs show an enhanced PCE of 24.95%.Finally by comparing the properties of perovskite with Ca(CF_(3)SO_(3))_(2)and FACF_(3)SO_(3),we found that doped Ca^(2+)significantly suppressed halide migration with an activation energy of 1.246 eV which accounts for the improved operational stability of Ca(CF_(3)SO_(3))_(2-)doped PSCs,while no obvious impact of Ca^(2+)on trap density is observed.Combining the benefits of cations and anions,this study presents an effective method to decouple the effects of cations and anions and fabricate efficient and stable PSCs.展开更多
To explore the rotational excitation of deformed halo nuclei,the angular momentum projection(AMP)has been implemented in the deformed relativistic Hartree-Bogoliubov theory in continuum(DRHBc),in which both the mean f...To explore the rotational excitation of deformed halo nuclei,the angular momentum projection(AMP)has been implemented in the deformed relativistic Hartree-Bogoliubov theory in continuum(DRHBc),in which both the mean field and collective wave functions are expanded in terms of Dirac WoodsSaxon basis.The DRHBc+AMP approach self-consistently describes the coupling between single particle bound states and the continuum not only in the ground state but also in rotational states.The rotational modes of deformed halos in ^(42,44)Mg are investigated by studying properties of rotational states such as the excitation energy,configuration,and density distribution.Our study demonstrates that the deformed halo structure persists from the ground state in the intrinsic frame to collective states.Especially,the typical behavior of shape decoupling effects in rotating deformed halo nuclei is revealed.展开更多
Optical lattice clocks demonstrate advantages in metrology and frontier physics because of their high stability.Here,we present approaches to enhancing the stability by decoupling the noise related to the short-term a...Optical lattice clocks demonstrate advantages in metrology and frontier physics because of their high stability.Here,we present approaches to enhancing the stability by decoupling the noise related to the short-term and long-term stability.For the short-term stability,we optimize the clock laser by decoupling the frequency noise,and optimize each noise contribution individually until it is below the thermal noise limit.For the long-term stability,we introduce a method to decouple the instability caused by systematic effects.Having identified that the collision frequency shift was the main limiting factor in our systems,we thus optimized the atom number fluctuations in optical lattices.Through targeted optimization,we achieve a synchronous comparison of two clocks with an average stability of 3.2×10^(-16)/√τ and a long-term stability of 2.4×10^(-18)at 8000 s.This work provides an analytical framework for enhancing optical clock stability.展开更多
文摘With the development of radioactive-ion-beam facilities,many exotic phenomena have been discovered or predicted in the nuclei far from the stability line,including cluster structure,shell structure,deformed halo,and shape decoupling effects.The study of exotic nuclear phenomena is at the frontier of nuclear physics nowadays.The covariant density functional theory(CDFT)is one of the most successful microscopic models in describing the structure of nuclei in almost the whole nuclear chart.Within the framework of CDFT,toward a proper treatment of deformation and weak binding,the deformed relativistic Hartree-Bogoliubov theory in continuum(DRHBc)has been developed.In this contribution,we review the applications and extensions of the DRHBc theory to the study of exotic nuclei.The DRHBc theory has been used to investigate the deformed halos in B,C,Ne,Na,and Mg isotopes and the theoretical descriptions are reasonably consistent with available data.A DRHBc Mass Table Collaboration has been founded,aiming at a high precision nuclear mass table with deformation and continuum effects included,which is underway.By implementing the angular momentum projection based on the DRHBc theory,the rotational excitations of deformed halos have been investigated and it is shown that the deformed halos and shape decoupling effects also exist in the low-lying rotational excitation states of deformed halo nuclei.
基金National Natural Science Foundation of China Youth Science Foundation ProjectNo.41701170+1 种基金National Natural Science Foundation of China,No.41661025,No.42071216Fundamental Research Funds for the Central Universities,No.18LZUJBWZY068。
文摘In 2007,China surpassed the USA to become the largest carbon emitter in the world.China has promised a 60%–65%reduction in carbon emissions per unit GDP by 2030,compared to the baseline of 2005.Therefore,it is important to obtain accurate dynamic information on the spatial and temporal patterns of carbon emissions and carbon footprints to support formulating effective national carbon emission reduction policies.This study attempts to build a carbon emission panel data model that simulates carbon emissions in China from 2000–2013 using nighttime lighting data and carbon emission statistics data.By applying the Exploratory Spatial-Temporal Data Analysis(ESTDA)framework,this study conducted an analysis on the spatial patterns and dynamic spatial-temporal interactions of carbon footprints from 2001–2013.The improved Tapio decoupling model was adopted to investigate the levels of coupling or decoupling between the carbon emission load and economic growth in 336 prefecture-level units.The results show that,firstly,high accuracy was achieved by the model in simulating carbon emissions.Secondly,the total carbon footprints and carbon deficits across China increased with average annual growth rates of 4.82%and 5.72%,respectively.The overall carbon footprints and carbon deficits were larger in the North than that in the South.There were extremely significant spatial autocorrelation features in the carbon footprints of prefecture-level units.Thirdly,the relative lengths of the Local Indicators of Spatial Association(LISA)time paths were longer in the North than that in the South,and they increased from the coastal to the central and western regions.Lastly,the overall decoupling index was mainly a weak decoupling type,but the number of cities with this weak decoupling continued to decrease.The unsustainable development trend of China’s economic growth and carbon emission load will continue for some time.
基金Ningbo Scientific and Technological Innovation 2025 Major Project,Grant/Award Number:2020Z022German Research Foundation(DFG)grants,Grant/Award Numbers:MA 5144/13-1,MA 5144/28-1+6 种基金the National Natural Science Foundation of China,Grant/Award Numbers:62204246,51931011,51971233,52127803,62174165the External Cooperation Program of Chinese Academy of Sciences,Grant/Award Numbers:174433KYSB20190038,174433KYSB20200013the Instrument Developing Project of the Chinese Academy of Sciences,Grant/Award Number:YJKYYQ20200030K.C.Wong Education Foundation,Grant/Award Number:GJTD-2020-11Chinese Academy of Sciences Youth Innovation Promotion Association,Grant/Award Number:2018334Zhejiang Provincial Key R&D Program,Grant/Award Numbers:2021C01183,2022C01032the National Natural Science Foundation of Zhejiang Province of China,Grant/Award Number:LQ23F040004.
文摘The progress from intelligent interactions requires electronic skin(E-skin)to shift from single-functional perception to multisensory capabilities.However,the intuitive and interference-free reading of multiple sensory signals without involving complex algorithms is a critical challenge.Herein,we propose a flexible multisensory E-skin by developing a highly homogeneous dispersion of BaTiO_(3)nanoparticles in polydimethylsiloxane dielectric layer.The E-skin is sensitive to externally applied pressure as well as temperature and can distinguish dual synergetic stimuli by the time decoupling effect.The pressure and temperature perception was achieved in an individual device,which greatly reduced the structural complexity compared with multifunctional integrated devices.The sensitivity of E-skin for pressure detection is as high as 0.0724 kPa^(−1)and the detection range reaches as wide as 15.625-10 MPa.The sensitivity to temperature detection is as high as−1.34℃^(−1)and the detection range reaches 20-200℃.More importantly,by equipping with a multilayer neural network,the evolution from tactile perception to advanced intelligent tactile cognition is demonstrated.
基金support from the National Key Research and Development Program of China(No.2022YFE0137400)the National Natural Science Foundation of China(Grant No.62274040).
文摘The past decade has witnessed the rapid increasement in power conversion efficiency of perovskite solar cells(PSCs).However,serious ion migration hampers their operational stability.Although dopants composed of varied cations and anions are introduced into perovskite to suppress ion migration,the impact of cations or anions is not individually explored,which hinders the evaluation of different cations and further application of doping strategy.Here we report that a special group of sulfonic anions(like CF_(3)SO_(3)^(-))successfully introduce alkaline earth ions(like Ca^(2+))into perovskite lattice compared to its halide counterparts.Furthermore,with effective crystallization regulation and defect passivation of sulfonic anions,perovskite with Ca(CF_(3)SO_(3))_(2)shows reduced PbI2 residue and metallic Pb0 defects;thereby,corresponding PSCs show an enhanced PCE of 24.95%.Finally by comparing the properties of perovskite with Ca(CF_(3)SO_(3))_(2)and FACF_(3)SO_(3),we found that doped Ca^(2+)significantly suppressed halide migration with an activation energy of 1.246 eV which accounts for the improved operational stability of Ca(CF_(3)SO_(3))_(2-)doped PSCs,while no obvious impact of Ca^(2+)on trap density is observed.Combining the benefits of cations and anions,this study presents an effective method to decouple the effects of cations and anions and fabricate efficient and stable PSCs.
基金supported by the National Key R&D Program of China(2018YFA0404402)the National Natural Science Foundation of China(11525524,12070131001,12047503,11975237,and 11961141004)+1 种基金the Key Research Program of Frontier Sciences of Chinese Academy of Sciences(QYZDB-SSWSYS013)the Strategic Priority Research Program of Chinese Academy of Sciences(XDB34010000 and XDPB15)。
文摘To explore the rotational excitation of deformed halo nuclei,the angular momentum projection(AMP)has been implemented in the deformed relativistic Hartree-Bogoliubov theory in continuum(DRHBc),in which both the mean field and collective wave functions are expanded in terms of Dirac WoodsSaxon basis.The DRHBc+AMP approach self-consistently describes the coupling between single particle bound states and the continuum not only in the ground state but also in rotational states.The rotational modes of deformed halos in ^(42,44)Mg are investigated by studying properties of rotational states such as the excitation energy,configuration,and density distribution.Our study demonstrates that the deformed halo structure persists from the ground state in the intrinsic frame to collective states.Especially,the typical behavior of shape decoupling effects in rotating deformed halo nuclei is revealed.
基金supported by the Shanghai Municipal Science and Technology Major Project(No.2019SHZDZX01)the National Natural Science Foundation of China(No.11134003)+1 种基金the National Key Research and Development Program of China(Nos.2016YFA0302103,2017YFF0212003,and 2016YFB0501601)the Shanghai Excellent Academic Leaders Program(No.12XD1402400)。
文摘Optical lattice clocks demonstrate advantages in metrology and frontier physics because of their high stability.Here,we present approaches to enhancing the stability by decoupling the noise related to the short-term and long-term stability.For the short-term stability,we optimize the clock laser by decoupling the frequency noise,and optimize each noise contribution individually until it is below the thermal noise limit.For the long-term stability,we introduce a method to decouple the instability caused by systematic effects.Having identified that the collision frequency shift was the main limiting factor in our systems,we thus optimized the atom number fluctuations in optical lattices.Through targeted optimization,we achieve a synchronous comparison of two clocks with an average stability of 3.2×10^(-16)/√τ and a long-term stability of 2.4×10^(-18)at 8000 s.This work provides an analytical framework for enhancing optical clock stability.
