Water-soluble organic nitrogen(WSON)affects the formation,hygroscopicity,acidity of organic aerosols,and nitrogen biogeochemical cycles.However,qualitative and quantitative characterizations of WSON remain limited due...Water-soluble organic nitrogen(WSON)affects the formation,hygroscopicity,acidity of organic aerosols,and nitrogen biogeochemical cycles.However,qualitative and quantitative characterizations of WSON remain limited due to its chemical complexity.In the study,1-year field samples of particulate matter 2.5(PM_(2.5))were collected fromJune 2022 to May 2023 to analyze the WSON concentration in PM_(2.5),and correlation analysis,positive matrix factor(PMF),and potential source contribution function(PSCF)modelswere employed to elucidate WSON source apportionment and transport pathways.The results revealed that the mean WSON concentrations reached 1.98±2.64μg/m^(3) with a mean WSON to water-soluble total nitrogen(WSTN)ratio of 21%.Further,WSON concentration exhibited a seasonal variation trend,with higher values in winter and lower in summer.Five sources were identified as contributors to WSON in PM_(2.5) within the reservoir area through a comprehensive analysis including correlation analysis,PSCF and concentration weighted trajectory(CWT),and PMF analyses.These sources were agricultural,dust,combustion,traffic,and industrial sources,of which agricultural source emerged as the primary contributor(76.69%).The atmosphere in the reservoir area were primarily influenced by the transport of northeastern air masses,local agricultural activities,industrial cities along the trajectory,and coastal regions,exerting significant influences on the concentration of WSON in the reservoir area.The findings of this study addressed the research gap concerning organic nitrogen in PM_(2.5) within the reservoir area,thereby offering a theoretical foundation and data support in controlling nitrogen pollution in the Danjiangkou Reservoir area.展开更多
The South-to-North Water Diversion Project in China aims to address the imbalanced distribution of water resources between the northern and southern regions,a critical safeguard for sustainable socio-economic and ecol...The South-to-North Water Diversion Project in China aims to address the imbalanced distribution of water resources between the northern and southern regions,a critical safeguard for sustainable socio-economic and ecological development.In this study,we investigated the hydroclimatic evolution of the water source area and its driving mechanisms using the inflow runoff data at Danjiangkou Reservoir from 1954 to 2013,along with multiple gridded hydroclimatic datasets.Based on the correlations between instrumental runoff data and gridded hydroclimatic variables,we used linear regression to extend the long-term runoff record to the period of 1902-2019.Our results indicate that climate changes,dominated by regional wet-dry cycles,have significant impacts on runoff variations,while the influence of human activities remains comparatively limited.Danjiangkou Reservoir can maintain a balanced base flow,even during the operation of the water diversion project.Preliminary synoptic climatology analyses reveal that runoff variations are mainly driven by the El Niño-Southern Oscillation(ENSO)and the Pacific Walker Circulation(PWC),which affect runoff by altering large-scale ocean-to-continent water vapor processes.This study advances the field by integrating multi-source data with analytical techniques,which enhances understanding of long-term runoff changes in the Danjiangkou Reservoir and their climatic drivers,ultimately supporting sustainable water resource management.展开更多
Investigating the ecological impact of land use change in the context of the construction of national water network project is crucial,as it is imperative for achieving the sustainable development goals of the nationa...Investigating the ecological impact of land use change in the context of the construction of national water network project is crucial,as it is imperative for achieving the sustainable development goals of the national water network and guaranteeing regional ecological stability.Using the Danjiangkou Reservoir Area(DRA),China as the study area,this paper first examined the spatiotemporal dynamics of natural landscape patterns and ecosystem service values(ESV)in the DRA from 2000 to 2018 and then investigated the spatial clustering characteristics of the ESV using spatial statistical analysis tools.Finally,the patch-generating land use simulation(PLUS)model was used to simulate the natural landscape and future changes in the ESV of the DRA from 2018 to 2028 under four different development scenarios:business as usual(BAU),economic development(ED),ecological protection(EP),and shoreline protection(SP).The results show that:during 2000-2018,the construction of water facilities had a significant impact on regional land use/land cover(LULC)change,with a 24830 ha increase in watershed area.ESV exhibited an increasing trend,with a significant and growing spatial clustering effect.The transformation of farmland to water bodies led to accelerated ESV growth,while the transformation of forest land to farmland led to a decrease in the ESV.Normalized difference vegetation index(NDVI)had the strongest effect on the ESV.ESV exhibited a continuous increase from 2018 to 2028 under all the simulation scenarios.The EP scenario had the greatest increase in ESV,while the ED scenario had the smallest increase.The findings suggest that projected land use patterns under different scenarios have varied impacts on ecosystem services(ESs)and that the management and planning of the DRA should balance social,economic,ecological,and security benefits.nomic,ecological,and security benefits.展开更多
Fresh water microplastic pollution is of pressing concern globally,but its distribution and sources in reservoirs are poorly documented.Danjiangkou Reservoir is the second largest reservoir in China and is divided int...Fresh water microplastic pollution is of pressing concern globally,but its distribution and sources in reservoirs are poorly documented.Danjiangkou Reservoir is the second largest reservoir in China and is divided into the Han Reservoir and Dan Reservoir.In this work,microplastic abundances and morphological characteristics of the reservoir were investigated.The microplastic abundance of 15 main tributaries of the reservoir was also measured.The vertical distribution(in water column and sediment),horizontal distribution(in Han Reservoir and Dan Reservoir)and source of microplastics were analyzed.Microplastics accumulated in the middle layer of the reservoir,and the size and color of the microplastic particles changed from the surface to the bottom,which implies that surveys of surface water are not enough to determine the microplastic contamination for deep water reservoirs.In the surface water,the microplastic abundance in the Han Reservoir was lower than that in the Dan Reservoir(p<0.05),but microplastic abundance did not differ significantly in the intermediate and bottom water.Tributaries were one of the main sources of microplastics for Han Reservoir but not for Dan Reservoir.Agricultural cultivation in the hydro-fluctuation belt might be an important source of microplastics in the Dan Reservoir,which should be given additional attention.The results of this study can provide valuable information for developing microplastic sampling strategies in deep water reservoirs.Further studies are recommended to investigate the process through which microplastics in the hydro-fluctuation belt enter the reservoir and the sinking behavior of microplastics in the reservoir.展开更多
One of the water source areas of the South-to-North Water Diversion Project is the Danjiangkou Reservoir （DJKR）. To understand seasonal variation in phytoplankton composition, abundance and distribution in the DJKR ...One of the water source areas of the South-to-North Water Diversion Project is the Danjiangkou Reservoir （DJKR）. To understand seasonal variation in phytoplankton composition, abundance and distribution in the DJKR area before water diversion, as well as to estimate potential risks of water quality after water diversion, we conducted an investigation on phytoplankton in the DJKR from August 2008 to May 2009. The investigation included 10 sampling sites, each with four depths of 0.5, 5, 10, and 20 m. In this study, 117 taxa belonging to 76 genera were identified, consisting of diatoms （39 taxa）, green algae （47 taxa）, blue-green algae （19 taxa）, and others （12 taxa）. Annual average phytoplankton abundance was 2.01×10^6 ind./L, and the highest value was 14.72 ×10^6 ind/L （at site 3 in August 2008）. Phytoplankton abundance in front of the Danjiangkou Dam （DJKD） was higher than that of the Danjiang Reservoir Basin. Phytoplankton distribution showed a vertical declining trend from 0.5 m to 20 m at most sites in August 2008 （especially at sites of 1, 2, 4 and 10）, but no distinct pattern in other sampling months. In December 2008 and March 2009, Stephanodiseus sp. was the most abundant species, amounting to 55.23% and 72.34%, respectively. We propose that high abundance ofStephanodiscus sp. may have contributed greatly to the frequent occurrence of Stephanodiscus sp. blooms in middle-low reaches of the Hanjiang River during the early spring of 2009. In comparison with previous studies conducted from 1992 to 2006, annual average phytoplankton density, green algae and blue-green algae species, as well as major nutrient concentrations increased, while phytoplankton diversity indices declined. This indicates a gradual decline in water quality. More research should be conducted and countermeasures taken to prevent further deterioration of water quality in the DJKR.展开更多
The estimation of non-point source pollution loads into the Danjiangkou Reservoir is highly significant to environmental protection in the watershed. In order to overcome the drawbacks of traditional watershed numeric...The estimation of non-point source pollution loads into the Danjiangkou Reservoir is highly significant to environmental protection in the watershed. In order to overcome the drawbacks of traditional watershed numerical models, a base flow separation method was established coupled with a digital filtering method and a flux method. The digital filtering method has been used to separate the base flows of the Hanjiang,Tianhe, Duhe, Danjiang, Laoguan, and Qihe rivers. Based on daily discharge, base flow, and pollutant concentration data, the flux method was used to calculate the point source pollution load and non-point source pollution load. The results show that:(1) In the year 2013, the total inflow of the six rivers mentioned above accounted for 95.9% of the total inflow to the Danjiangkou Reservoir. The total pollution loads of chemical oxygen demand(CODMn) and total phosphorus(TP) from the six rivers were 58.20 103 t and 1.863 10~3 t, respectively, and the non-point source pollution loads were 39.82 10~3 t and 1.544 10~3 t, respectively, indicating that the non-point source pollution is a major factor(with a contribution rate of 68.4% for CODMnand 82.9% for TP).(2) The Hanjiang River is the most significant contributor of pollution loads to the Danjiangkou Reservoir, and its CODMnand TP contribution rates reached 79.3% and 83.2%, respectively. The Duhe River took the second place.(3) Non-point source pollution mainly occurred in the wet season in 2013, accounting for 80.8% and 90.9% of the total pollution loads of CODMnand TP, respectively. It is concluded that the emphasis of pollution control should be placed on non-point source pollution.展开更多
Nitrogen deposition is an important means of exogenous nitrogen input in reservoir water.Agricultural activities around the reservoir lead to a sharp increase in the concentration of ammonia in the atmosphere,which po...Nitrogen deposition is an important means of exogenous nitrogen input in reservoir water.Agricultural activities around the reservoir lead to a sharp increase in the concentration of ammonia in the atmosphere,which poses a threat to the reservoir water body.Clarifying the contribution of agricultural ammonia release to atmospheric NH_(x)(gaseous NH_(3)and particulate NH_(4)^(+)),in the reservoir area can provide a theoretical foundation for local reactive nitrogen control.We collected atmospheric NH_(3)and NH_(4)^(+)samples during the agricultural periods and analyzed the isotopic characteristics of atmospheric NH_(x)and the contribution rates of different ammonia sources in the Xichuan area of the Danjiangkou Reservoir.The results showed that the initialδ~(15)N values of NH_(3)(-30.0‰to–7.2‰)and particulate NH_(4)^(+)(–33‰to+4.9‰for finer and coarser particles,respectively)are different,and their contribution ratios from dissimilar ammonia sources are also different,among which NH_(4)^(+)is more susceptible to meteorological factors.However,since the atmospheric NH_(x)in the Xichuan area is mainly gaseous NH_(3),the final sources of atmospheric ammonia nitrogen source depend on gaseous NH_(3).Agricultural sources(59%-74%)were the main NH_(3)sources in this area.Among them,the fertilizer use emission was dominant;it had the highest contribution rate in summer during the agricultural period and a more prominent impact in areas with less human interference.Reasonable regulation of the application of high-ammonia releasing fertilizer,especially during the agricultural period in summer,is an effective way to reduce the threat of atmospheric ammonia to water health.展开更多
Water levels in reservoirs are generally not allowed to exceed the flood-limited water level during the flood season, which means that huge amounts of water spill in order to provide adequate storage for flood prevent...Water levels in reservoirs are generally not allowed to exceed the flood-limited water level during the flood season, which means that huge amounts of water spill in order to provide adequate storage for flood prevention and that it is difficult to fill the reservoir fully at the end of year. Early reservoir refill is an effective method for addressing the contradiction between the needs of flood control and of comprehensive utilization. This study selected the Danjiangkou Reservoir, which is the water source for the middle route of the South-North Water Diversion Project （SNWDP） in China, as a case study, and analyzed the necessity and operational feasibility of early reservoir refill. An early reservoir refill model is proposed based on the maximum average storage ratio, optimized by the progressive optimality algorithm, and the optimal scheduling schemes were obtained. Results show that the best time of refill operation for the Danjiangkou Reservoir is September 15, and the upper limit water level during September is 166 m. The proposed early refill scheme, in stages, can increase the annual average storage ratio from 77.51% to 81.99%, and decrease spilled water from 2.439 × 109 m^3 to 1.692×109 m^3, in comparison to the original design scheme. The suggested early significant comprehensive benefits, which decision-making. reservoir refill scheme can be easily operated with may provide a good reference for scheduling展开更多
Soil and water loss has been a major environmental problem in the Danjiangkou Reservoir Region.A study of 14°sloping farmland was performed on impact of different contour hedgerows on runoff,losses of soil and nu...Soil and water loss has been a major environmental problem in the Danjiangkou Reservoir Region.A study of 14°sloping farmland was performed on impact of different contour hedgerows on runoff,losses of soil and nutrients during 2008 and 2011,with five treatments and three replications.The winter wheat and summer maize were used as the test crops.Treatments consisted of four hedgerows:Amorpha(Amorpha fruticosa L.),Honeysuckle(Lonicera japonica Thunb.),Day-lily flower(Hemerocallis citrina Baroni.),and Sabaigrass(Eulaliopsis binata),and a control without hedgerow.Result showed that the runoff under the control treatment was much higher than that of hedgerows.Amorpha could reduce the runoff by 35.2%compared with the control.Soil losses in four hedgerows showed significant reduction in four years(e.g.,Amorpha:78.3%;Honeysuckle:77.1%).Nutrient losses in winter were much higher than that in summer,especially total nitrogen,total phosphorus and total potassium,even though there was an abundant precipitation in summer.Hedgerows greatly affected the soil and nutrient losses on slopping farmland compared with the control treatment,especially Amorpha treatment.The present study found that the Amorpha could be used as the hedgerow species for reducing soil and water loss in the Danjiangkou Reservoir Region.展开更多
Based on optical remote sensing,two challenges should be highlighted in research on reservoir water resources in mountainous areas:(1)the isolation of climatic influences from anthropogenic impacts during impoundment ...Based on optical remote sensing,two challenges should be highlighted in research on reservoir water resources in mountainous areas:(1)the isolation of climatic influences from anthropogenic impacts during impoundment periods,and(2)the discernment of circulation mechanisms to improve early-warning-system capabilities against extreme climate events.To address these challenges,we developed an enhanced automated water-detection framework using Landsat TOA data(1986-2023)that allowed us to analyse the spatiotemporal variations and driving factors of the water surface area of the Danjiangkou(DJK)Reservoir-China’s key source of the South to North Water Diversion.The results showed that anthropogenically induced changes in water surface area were evident through infrastructure developments,notably the increase in the height of the DJK dam(contributing 34.0%of the variance)and the construction of the Wangfuzhou Hydrojunction(contributing 51.9%of the variance).Following ensemble empirical mode decomposition and first-order difference detrending to reduce the impacts from human activity,a significantly enhanced positive(negative)correlation between autumn precipitation(potential evaporation)and water surface area was revealed;this demonstrated the climate-driven controls on reservoir dynamics at the interannual and decadal scales.Importantly,atmospheric pressure anomalies over the Tibetan Plateau and the area of the Asian polar vortex are two effective indicators of autumn precipitation anomalies for the DJK Reservoir.Our research framework has the potential to support the development of early warning systems,which have direct applications to the DJK Reservoir and,more broadly,to reservoir systems across Eurasia.展开更多
Antibiotic resistance genes (ARGs) have attracted more and more attention due to their potential exposure hazards. The Danjiangkou Reservoir (DJKR) is the source of water for the Middle Route Project under the South-t...Antibiotic resistance genes (ARGs) have attracted more and more attention due to their potential exposure hazards. The Danjiangkou Reservoir (DJKR) is the source of water for the Middle Route Project under the South-to-North Water Transfer Scheme in China. To clarify the distribution of ARGs and their influencing factors in DJKR (including Danjiang Reservoir (DR) and Hanjiang River Reservoir (HR)), we used metagenomic analysis to investigate the ARGs. The results showed that the most abundant bacteria of both parts were Proteobacteteria. Antibiotic efflux (58.2 %) and alteration of antibiotic targets (69.4 %) were the main mechanisms in DR and HR. The composition of ARG species was similar in the two parts, but the number of ARG isoforms in HR was significantly higher than that in DR. ARG Intl1 was detected in both DR and HR. Network analysis showed a significant correlation between mobile genetic elements (MGEs) and ARGs. Heavy metals also showed a significant correlation with ARGs. Interestingly, the relationship between heavy metals and ARGs were more significant than that between antibiotics and ARGs.展开更多
The Danjiangkou Reservoir is the water source for the middle route of the South-to-North Water Diversion Project in China. Thus, its water quality status is of great concern. Five water quality indicators （dissolved ...The Danjiangkou Reservoir is the water source for the middle route of the South-to-North Water Diversion Project in China. Thus, its water quality status is of great concern. Five water quality indicators （dissolved oxygen, permanganate index, ammonia nitrogen, total nitrogen, and total phosphorus）, were measured at three monitoring sites （the Danjiangkou Reservoir dam, the Hejiawan and the Jiangbei bridge）, to investigate changing trends, and spatiotemporal characteristics of water quality in the Danjiangkou Reservoir area from January 2006 to May 2012. We then applied a Bayesian statistical method to evaluate the water quality comprehensively. The normal distribution sampling method was used to calculate likelihood, and the entropy weight method was used to determine indicator weights for variables of interest in to the study. The results indicated that concentrations of all five indicators increased during the last six years. In addition, the water quality in the reservoir was worse during the wet season （from May to October）, than during the dry season （from November to April of the next year）. Overall, the probability of the water＇s belonging to quality category of type lI, according to environmental quality standards for surface water in China, was 27.7%-33.7%, larger than that of its belonging to the other four water quality types. The increasing concentrations of nutrients could result in eutrophication of the Danjiangkou Reser- voir. This method reduced the subjectivity that is commonly associated with determining indicator weights and artificial classifications, achieving more reliable results. These results indicate that it is important for the interbasin water diversion project to implement integrated water quality management in the Danjiangkou Reservoir area.展开更多
The Danjiangkou reservoir was selected to provide the source water for the middle routes of the South to North Water Transfer Project, which has provoked many environmental concerns. To date, investigations of water c...The Danjiangkou reservoir was selected to provide the source water for the middle routes of the South to North Water Transfer Project, which has provoked many environmental concerns. To date, investigations of water contamination of the source water of the Danjiangkou reservoir with organic micro-pollutants have been limited. This study was conducted to identify and rank organic contaminants that pose risks in the Danjiangkou reservoir. To this end, the Chemical Hazard Evaluation and Manage- ment Strategies （CHEMS-1） approach was adapted to integrate the deconvolution technology of qualitative identifying contaminants for site-specific environmental matrices. The samples were screened for the presence of 1093 contaminants using deconvolution technologies and the hazard values of the identified contaminants were calculated using the adapted CHEMS-1 approach accord- ing to their hazardous properties and occurrence in source water. The results showed that 46 contaminants from 1093 targets were present in Danjiangkou water, 23 of which appeared at frequencies higher than 50%, and 15 of which were identified as priorities. Over half （53%） of the high- ranked contaminants were polycyclic aromatic hydrocar- bons （PAHs）, with chrysene ranked highest on the list. Health risk assessment of the top-ranked PAHs was conducted and revealed that cancer risks of PAHs detected in the source water of Danjiangkou to different populations ranged from 10-7 to 104, indicating a low cancer risk to consumers. The results of this study indicated that the adapted CHEMS-1 approach was feasible for site-specific screening of organic contaminants to identify and rank potential priority pollutants.展开更多
Inter-basin water deal of nitrogen are great transfers containing a great threats to human health, biodiversity, and air and water quality in the recipient area. Danjiangkou Reservoir, the source reservoir for China...Inter-basin water deal of nitrogen are great transfers containing a great threats to human health, biodiversity, and air and water quality in the recipient area. Danjiangkou Reservoir, the source reservoir for China＇s South-to-North Water Diversion Middle Route Project, suffers from total nitrogen pollution and threatens the water transfer to a number of metropolises including the capital, Beijing. To locate the main source of nitrogen pollution into the reservoir, especially near the Taocha canal head, where the intake of water transfer begins, we constructed a 3-D water quality model. We then used an inflow sensitivity analysis method to analyze the sig- nificance of inflows from each tributary that may contribute to the total nitrogen pollution and affect water quality. The results indicated that the Han River was the most significant river with a sensitivity index of 0.340, followed by the Dan River with a sensitivity index of 0.089, while the Guanshan River and the Lang River were not significant, with the sensitivity indices of 0.002 and 0.001, respectively. This result implies that the concentration and amount of nitrogen inflow outweighs the geographical position of the tributary for sources of total nitrogen pollution to the Taocha canal head of the Danjiangkou Reservoir.展开更多
As the biggest inter-basin water transfer scheme in the world,the South-to-North Water Diversion Project(SNWD) was designed to alleviate the water crisis in North China.The main channel of the middle route of the SNWD...As the biggest inter-basin water transfer scheme in the world,the South-to-North Water Diversion Project(SNWD) was designed to alleviate the water crisis in North China.The main channel of the middle route of the SNWD is of great concern in terms of the drinking water quality.In this study,we tested the hypothesis that the dissolved organic matter(DOM) derived from the planktonic algae causes the rising levels of COD_(Mn) along the middle route by monitoring data on water quality(2015-2019,monthly resolution).The results showed that algal density in the main channel increased along the channel and was significantly correlated with COD_(Mn)(p <0.01).Five fluorescent components of DOM,including tyrosine-like(14.85%),tryptophan-like(22.48%),microbial byproduct-like(26.34%),fulvic acid-like(11.41%),and humic acid-like(24.92%) components,were detected.The level of tyrosine-like components increased along the channel and was significantly correlated with algal density(p<0.01),indicating that algae significantly changed the level of DOM in the channel.Algal decomposition and metabolism were found to be the main mechanisms that drive the changes in COD_(Mn).Therefore,controlling algal density would be an important measure to prevent further increase in CODMn and for the guarantee of excellent water quality.展开更多
The total capacity of Three Gorges Reservoir（TGR） and Danjiangkou Reservoir（DJR） is large and has significant seasonal fluctuations, which give rise to crustal instability. In this research, we focus on studying t...The total capacity of Three Gorges Reservoir（TGR） and Danjiangkou Reservoir（DJR） is large and has significant seasonal fluctuations, which give rise to crustal instability. In this research, we focus on studying the temporal and spatial variation of crustal deformation in Hubei Province caused by reservoir impoundment of TGR and DJR.The Digital Elevation Model, historical hydrological information, GPS monitoring data and load-induced deformation model are combined to monitor the crustal deformation. The modeled results indicate that in the trapezoidal area between the TGR and DJR, the average vertical deformations at different latitudes have different variation tendencies. The vertical deformation modulus and fluctuation amplitude are larger at the latitude of 33 N/32.5 N from 2003 to 2006 and at the latitude of 31 N/32.5 N from 2008 to 2014, while the latter are much larger than the former. Moreover, from2008 to 2014, the frequency and the intensity of seismic activities are all enhanced significantly in this region. The modeled results at the GPS sites are consistent with the vertical displacement of GPS monitoring results in trends and the waveform. It can be inferred that the seasonal deformation is elastic. The horizontal deformation components have the same variation trends with that at each GPS monitoring station,which demonstrates that the whole region is moving toward the southeast. The spatial variation of crustal deformation demonstrates that the impoundment of TGR in2003 causes significant vertical displacements, with the maximum modulus of 32 mm downward located in Xiangjiang River＇s estuary. When the water storage increases, the maximum value will become larger, and the location will move toward the upstream.Besides, the earthquakes occurred more frequently in the region with maximum deformation modulus.展开更多
As a critical water source for the central route of the South-to-North Water Diversion Project,the Danjiangkou Reservoir has consistently achieved a water quality rating of Gradell or above,thanks to its efforts to ke...As a critical water source for the central route of the South-to-North Water Diversion Project,the Danjiangkou Reservoir has consistently achieved a water quality rating of Gradell or above,thanks to its efforts to keep enhancing water qualityprotection.展开更多
基金supported by the National Natural Science Foundation of China(Nos.U23A2016,U1704241,and 42007175).
文摘Water-soluble organic nitrogen(WSON)affects the formation,hygroscopicity,acidity of organic aerosols,and nitrogen biogeochemical cycles.However,qualitative and quantitative characterizations of WSON remain limited due to its chemical complexity.In the study,1-year field samples of particulate matter 2.5(PM_(2.5))were collected fromJune 2022 to May 2023 to analyze the WSON concentration in PM_(2.5),and correlation analysis,positive matrix factor(PMF),and potential source contribution function(PSCF)modelswere employed to elucidate WSON source apportionment and transport pathways.The results revealed that the mean WSON concentrations reached 1.98±2.64μg/m^(3) with a mean WSON to water-soluble total nitrogen(WSTN)ratio of 21%.Further,WSON concentration exhibited a seasonal variation trend,with higher values in winter and lower in summer.Five sources were identified as contributors to WSON in PM_(2.5) within the reservoir area through a comprehensive analysis including correlation analysis,PSCF and concentration weighted trajectory(CWT),and PMF analyses.These sources were agricultural,dust,combustion,traffic,and industrial sources,of which agricultural source emerged as the primary contributor(76.69%).The atmosphere in the reservoir area were primarily influenced by the transport of northeastern air masses,local agricultural activities,industrial cities along the trajectory,and coastal regions,exerting significant influences on the concentration of WSON in the reservoir area.The findings of this study addressed the research gap concerning organic nitrogen in PM_(2.5) within the reservoir area,thereby offering a theoretical foundation and data support in controlling nitrogen pollution in the Danjiangkou Reservoir area.
基金supported by the National Natural Science Foundation of China(NSFC Project No.32061123008)the Innovation Training Programme for Undergraduate Students of Yunnan University(Project No.202301051).
文摘The South-to-North Water Diversion Project in China aims to address the imbalanced distribution of water resources between the northern and southern regions,a critical safeguard for sustainable socio-economic and ecological development.In this study,we investigated the hydroclimatic evolution of the water source area and its driving mechanisms using the inflow runoff data at Danjiangkou Reservoir from 1954 to 2013,along with multiple gridded hydroclimatic datasets.Based on the correlations between instrumental runoff data and gridded hydroclimatic variables,we used linear regression to extend the long-term runoff record to the period of 1902-2019.Our results indicate that climate changes,dominated by regional wet-dry cycles,have significant impacts on runoff variations,while the influence of human activities remains comparatively limited.Danjiangkou Reservoir can maintain a balanced base flow,even during the operation of the water diversion project.Preliminary synoptic climatology analyses reveal that runoff variations are mainly driven by the El Niño-Southern Oscillation(ENSO)and the Pacific Walker Circulation(PWC),which affect runoff by altering large-scale ocean-to-continent water vapor processes.This study advances the field by integrating multi-source data with analytical techniques,which enhances understanding of long-term runoff changes in the Danjiangkou Reservoir and their climatic drivers,ultimately supporting sustainable water resource management.
基金Under the auspices of National Natural Science Foundation of China(No.42371315,41901213)Natural Science Foundation of Hubei Province(No.2020CFB856)Project of Changjiang Survey,Planning,Design and Research Co.,Ltd(No.CX2022Z23)。
文摘Investigating the ecological impact of land use change in the context of the construction of national water network project is crucial,as it is imperative for achieving the sustainable development goals of the national water network and guaranteeing regional ecological stability.Using the Danjiangkou Reservoir Area(DRA),China as the study area,this paper first examined the spatiotemporal dynamics of natural landscape patterns and ecosystem service values(ESV)in the DRA from 2000 to 2018 and then investigated the spatial clustering characteristics of the ESV using spatial statistical analysis tools.Finally,the patch-generating land use simulation(PLUS)model was used to simulate the natural landscape and future changes in the ESV of the DRA from 2018 to 2028 under four different development scenarios:business as usual(BAU),economic development(ED),ecological protection(EP),and shoreline protection(SP).The results show that:during 2000-2018,the construction of water facilities had a significant impact on regional land use/land cover(LULC)change,with a 24830 ha increase in watershed area.ESV exhibited an increasing trend,with a significant and growing spatial clustering effect.The transformation of farmland to water bodies led to accelerated ESV growth,while the transformation of forest land to farmland led to a decrease in the ESV.Normalized difference vegetation index(NDVI)had the strongest effect on the ESV.ESV exhibited a continuous increase from 2018 to 2028 under all the simulation scenarios.The EP scenario had the greatest increase in ESV,while the ED scenario had the smallest increase.The findings suggest that projected land use patterns under different scenarios have varied impacts on ecosystem services(ESs)and that the management and planning of the DRA should balance social,economic,ecological,and security benefits.nomic,ecological,and security benefits.
基金supported by the Fundamental Research Funds for Central Public Welfare Research Institutes of China(Nos.CKSF2019380/SH,CKSF2017062/SH)the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDA23040303)。
文摘Fresh water microplastic pollution is of pressing concern globally,but its distribution and sources in reservoirs are poorly documented.Danjiangkou Reservoir is the second largest reservoir in China and is divided into the Han Reservoir and Dan Reservoir.In this work,microplastic abundances and morphological characteristics of the reservoir were investigated.The microplastic abundance of 15 main tributaries of the reservoir was also measured.The vertical distribution(in water column and sediment),horizontal distribution(in Han Reservoir and Dan Reservoir)and source of microplastics were analyzed.Microplastics accumulated in the middle layer of the reservoir,and the size and color of the microplastic particles changed from the surface to the bottom,which implies that surveys of surface water are not enough to determine the microplastic contamination for deep water reservoirs.In the surface water,the microplastic abundance in the Han Reservoir was lower than that in the Dan Reservoir(p<0.05),but microplastic abundance did not differ significantly in the intermediate and bottom water.Tributaries were one of the main sources of microplastics for Han Reservoir but not for Dan Reservoir.Agricultural cultivation in the hydro-fluctuation belt might be an important source of microplastics in the Dan Reservoir,which should be given additional attention.The results of this study can provide valuable information for developing microplastic sampling strategies in deep water reservoirs.Further studies are recommended to investigate the process through which microplastics in the hydro-fluctuation belt enter the reservoir and the sinking behavior of microplastics in the reservoir.
基金Supported by the National Basic Research Program of China (973 Program) (No. 2008CB418006)the Knowledge Innovation Program of Chinese Academy of Sciences (No. KZCX-YW-14-1)
文摘One of the water source areas of the South-to-North Water Diversion Project is the Danjiangkou Reservoir （DJKR）. To understand seasonal variation in phytoplankton composition, abundance and distribution in the DJKR area before water diversion, as well as to estimate potential risks of water quality after water diversion, we conducted an investigation on phytoplankton in the DJKR from August 2008 to May 2009. The investigation included 10 sampling sites, each with four depths of 0.5, 5, 10, and 20 m. In this study, 117 taxa belonging to 76 genera were identified, consisting of diatoms （39 taxa）, green algae （47 taxa）, blue-green algae （19 taxa）, and others （12 taxa）. Annual average phytoplankton abundance was 2.01×10^6 ind./L, and the highest value was 14.72 ×10^6 ind/L （at site 3 in August 2008）. Phytoplankton abundance in front of the Danjiangkou Dam （DJKD） was higher than that of the Danjiang Reservoir Basin. Phytoplankton distribution showed a vertical declining trend from 0.5 m to 20 m at most sites in August 2008 （especially at sites of 1, 2, 4 and 10）, but no distinct pattern in other sampling months. In December 2008 and March 2009, Stephanodiseus sp. was the most abundant species, amounting to 55.23% and 72.34%, respectively. We propose that high abundance ofStephanodiscus sp. may have contributed greatly to the frequent occurrence of Stephanodiscus sp. blooms in middle-low reaches of the Hanjiang River during the early spring of 2009. In comparison with previous studies conducted from 1992 to 2006, annual average phytoplankton density, green algae and blue-green algae species, as well as major nutrient concentrations increased, while phytoplankton diversity indices declined. This indicates a gradual decline in water quality. More research should be conducted and countermeasures taken to prevent further deterioration of water quality in the DJKR.
基金supported by the National Key Research and Development Program of China(Grants No.2016YFC0402204 and 2016YFC0402207)
文摘The estimation of non-point source pollution loads into the Danjiangkou Reservoir is highly significant to environmental protection in the watershed. In order to overcome the drawbacks of traditional watershed numerical models, a base flow separation method was established coupled with a digital filtering method and a flux method. The digital filtering method has been used to separate the base flows of the Hanjiang,Tianhe, Duhe, Danjiang, Laoguan, and Qihe rivers. Based on daily discharge, base flow, and pollutant concentration data, the flux method was used to calculate the point source pollution load and non-point source pollution load. The results show that:(1) In the year 2013, the total inflow of the six rivers mentioned above accounted for 95.9% of the total inflow to the Danjiangkou Reservoir. The total pollution loads of chemical oxygen demand(CODMn) and total phosphorus(TP) from the six rivers were 58.20 103 t and 1.863 10~3 t, respectively, and the non-point source pollution loads were 39.82 10~3 t and 1.544 10~3 t, respectively, indicating that the non-point source pollution is a major factor(with a contribution rate of 68.4% for CODMnand 82.9% for TP).(2) The Hanjiang River is the most significant contributor of pollution loads to the Danjiangkou Reservoir, and its CODMnand TP contribution rates reached 79.3% and 83.2%, respectively. The Duhe River took the second place.(3) Non-point source pollution mainly occurred in the wet season in 2013, accounting for 80.8% and 90.9% of the total pollution loads of CODMnand TP, respectively. It is concluded that the emphasis of pollution control should be placed on non-point source pollution.
基金supported by the National Natural Science Foundation of China (Nos.U1704241 and 42007175)the Plan for Scientific Innovation Talent of Henan Province (No.194200510010)the Science Research Funds for the Universities of Henan Province (No.NSFRF200326)。
文摘Nitrogen deposition is an important means of exogenous nitrogen input in reservoir water.Agricultural activities around the reservoir lead to a sharp increase in the concentration of ammonia in the atmosphere,which poses a threat to the reservoir water body.Clarifying the contribution of agricultural ammonia release to atmospheric NH_(x)(gaseous NH_(3)and particulate NH_(4)^(+)),in the reservoir area can provide a theoretical foundation for local reactive nitrogen control.We collected atmospheric NH_(3)and NH_(4)^(+)samples during the agricultural periods and analyzed the isotopic characteristics of atmospheric NH_(x)and the contribution rates of different ammonia sources in the Xichuan area of the Danjiangkou Reservoir.The results showed that the initialδ~(15)N values of NH_(3)(-30.0‰to–7.2‰)and particulate NH_(4)^(+)(–33‰to+4.9‰for finer and coarser particles,respectively)are different,and their contribution ratios from dissimilar ammonia sources are also different,among which NH_(4)^(+)is more susceptible to meteorological factors.However,since the atmospheric NH_(x)in the Xichuan area is mainly gaseous NH_(3),the final sources of atmospheric ammonia nitrogen source depend on gaseous NH_(3).Agricultural sources(59%-74%)were the main NH_(3)sources in this area.Among them,the fertilizer use emission was dominant;it had the highest contribution rate in summer during the agricultural period and a more prominent impact in areas with less human interference.Reasonable regulation of the application of high-ammonia releasing fertilizer,especially during the agricultural period in summer,is an effective way to reduce the threat of atmospheric ammonia to water health.
基金supported by the National Natural Science Foundation of China(Grant No.51190094)the National Key Technologies Research and Development Program of China(Grant No.2009BAC56B02)
文摘Water levels in reservoirs are generally not allowed to exceed the flood-limited water level during the flood season, which means that huge amounts of water spill in order to provide adequate storage for flood prevention and that it is difficult to fill the reservoir fully at the end of year. Early reservoir refill is an effective method for addressing the contradiction between the needs of flood control and of comprehensive utilization. This study selected the Danjiangkou Reservoir, which is the water source for the middle route of the South-North Water Diversion Project （SNWDP） in China, as a case study, and analyzed the necessity and operational feasibility of early reservoir refill. An early reservoir refill model is proposed based on the maximum average storage ratio, optimized by the progressive optimality algorithm, and the optimal scheduling schemes were obtained. Results show that the best time of refill operation for the Danjiangkou Reservoir is September 15, and the upper limit water level during September is 166 m. The proposed early refill scheme, in stages, can increase the annual average storage ratio from 77.51% to 81.99%, and decrease spilled water from 2.439 × 109 m^3 to 1.692×109 m^3, in comparison to the original design scheme. The suggested early significant comprehensive benefits, which decision-making. reservoir refill scheme can be easily operated with may provide a good reference for scheduling
文摘Soil and water loss has been a major environmental problem in the Danjiangkou Reservoir Region.A study of 14°sloping farmland was performed on impact of different contour hedgerows on runoff,losses of soil and nutrients during 2008 and 2011,with five treatments and three replications.The winter wheat and summer maize were used as the test crops.Treatments consisted of four hedgerows:Amorpha(Amorpha fruticosa L.),Honeysuckle(Lonicera japonica Thunb.),Day-lily flower(Hemerocallis citrina Baroni.),and Sabaigrass(Eulaliopsis binata),and a control without hedgerow.Result showed that the runoff under the control treatment was much higher than that of hedgerows.Amorpha could reduce the runoff by 35.2%compared with the control.Soil losses in four hedgerows showed significant reduction in four years(e.g.,Amorpha:78.3%;Honeysuckle:77.1%).Nutrient losses in winter were much higher than that in summer,especially total nitrogen,total phosphorus and total potassium,even though there was an abundant precipitation in summer.Hedgerows greatly affected the soil and nutrient losses on slopping farmland compared with the control treatment,especially Amorpha treatment.The present study found that the Amorpha could be used as the hedgerow species for reducing soil and water loss in the Danjiangkou Reservoir Region.
基金National Natural Science Foundation of China,No.41701592Natural Science Foundation of Shaanxi Province,No.2023-JC-QN-0321。
文摘Based on optical remote sensing,two challenges should be highlighted in research on reservoir water resources in mountainous areas:(1)the isolation of climatic influences from anthropogenic impacts during impoundment periods,and(2)the discernment of circulation mechanisms to improve early-warning-system capabilities against extreme climate events.To address these challenges,we developed an enhanced automated water-detection framework using Landsat TOA data(1986-2023)that allowed us to analyse the spatiotemporal variations and driving factors of the water surface area of the Danjiangkou(DJK)Reservoir-China’s key source of the South to North Water Diversion.The results showed that anthropogenically induced changes in water surface area were evident through infrastructure developments,notably the increase in the height of the DJK dam(contributing 34.0%of the variance)and the construction of the Wangfuzhou Hydrojunction(contributing 51.9%of the variance).Following ensemble empirical mode decomposition and first-order difference detrending to reduce the impacts from human activity,a significantly enhanced positive(negative)correlation between autumn precipitation(potential evaporation)and water surface area was revealed;this demonstrated the climate-driven controls on reservoir dynamics at the interannual and decadal scales.Importantly,atmospheric pressure anomalies over the Tibetan Plateau and the area of the Asian polar vortex are two effective indicators of autumn precipitation anomalies for the DJK Reservoir.Our research framework has the potential to support the development of early warning systems,which have direct applications to the DJK Reservoir and,more broadly,to reservoir systems across Eurasia.
基金supported by the National Natural Science Foundation of China(41807409)the foundation for Innovative Research Team of Hubei Provincial Department of Education(JYT2021024)Advantages Discipline Group(Public health)Project in Higher Education of Hubei Province(2021-2025).
文摘Antibiotic resistance genes (ARGs) have attracted more and more attention due to their potential exposure hazards. The Danjiangkou Reservoir (DJKR) is the source of water for the Middle Route Project under the South-to-North Water Transfer Scheme in China. To clarify the distribution of ARGs and their influencing factors in DJKR (including Danjiang Reservoir (DR) and Hanjiang River Reservoir (HR)), we used metagenomic analysis to investigate the ARGs. The results showed that the most abundant bacteria of both parts were Proteobacteteria. Antibiotic efflux (58.2 %) and alteration of antibiotic targets (69.4 %) were the main mechanisms in DR and HR. The composition of ARG species was similar in the two parts, but the number of ARG isoforms in HR was significantly higher than that in DR. ARG Intl1 was detected in both DR and HR. Network analysis showed a significant correlation between mobile genetic elements (MGEs) and ARGs. Heavy metals also showed a significant correlation with ARGs. Interestingly, the relationship between heavy metals and ARGs were more significant than that between antibiotics and ARGs.
基金Acknowledgements This study was supported by the National Science and Technology Support Program （No. 2011BAC12B02）, the National Science Foundation for Innovative Research Group （No. 51121003）, and the Outstanding Doctoral Thesis Fund of Beijing Normal University （No. 105512GK）. We are grateful to the editors and anonymous reviewers＇ careful review of this paper, whom have contributed substantially to improving the paper.
文摘The Danjiangkou Reservoir is the water source for the middle route of the South-to-North Water Diversion Project in China. Thus, its water quality status is of great concern. Five water quality indicators （dissolved oxygen, permanganate index, ammonia nitrogen, total nitrogen, and total phosphorus）, were measured at three monitoring sites （the Danjiangkou Reservoir dam, the Hejiawan and the Jiangbei bridge）, to investigate changing trends, and spatiotemporal characteristics of water quality in the Danjiangkou Reservoir area from January 2006 to May 2012. We then applied a Bayesian statistical method to evaluate the water quality comprehensively. The normal distribution sampling method was used to calculate likelihood, and the entropy weight method was used to determine indicator weights for variables of interest in to the study. The results indicated that concentrations of all five indicators increased during the last six years. In addition, the water quality in the reservoir was worse during the wet season （from May to October）, than during the dry season （from November to April of the next year）. Overall, the probability of the water＇s belonging to quality category of type lI, according to environmental quality standards for surface water in China, was 27.7%-33.7%, larger than that of its belonging to the other four water quality types. The increasing concentrations of nutrients could result in eutrophication of the Danjiangkou Reser- voir. This method reduced the subjectivity that is commonly associated with determining indicator weights and artificial classifications, achieving more reliable results. These results indicate that it is important for the interbasin water diversion project to implement integrated water quality management in the Danjiangkou Reservoir area.
基金Acknowledgements This work was supported by the National Natural Science Foundation of China （Grant Nos. 20977102 and 21007077）, the Ministry of Water Resources＇ Special Funds for Scientific Research on Public Causes （No. 201201032） and the Environmental Protection National Commonweal Research Project （No. 200909040）.
文摘The Danjiangkou reservoir was selected to provide the source water for the middle routes of the South to North Water Transfer Project, which has provoked many environmental concerns. To date, investigations of water contamination of the source water of the Danjiangkou reservoir with organic micro-pollutants have been limited. This study was conducted to identify and rank organic contaminants that pose risks in the Danjiangkou reservoir. To this end, the Chemical Hazard Evaluation and Manage- ment Strategies （CHEMS-1） approach was adapted to integrate the deconvolution technology of qualitative identifying contaminants for site-specific environmental matrices. The samples were screened for the presence of 1093 contaminants using deconvolution technologies and the hazard values of the identified contaminants were calculated using the adapted CHEMS-1 approach accord- ing to their hazardous properties and occurrence in source water. The results showed that 46 contaminants from 1093 targets were present in Danjiangkou water, 23 of which appeared at frequencies higher than 50%, and 15 of which were identified as priorities. Over half （53%） of the high- ranked contaminants were polycyclic aromatic hydrocar- bons （PAHs）, with chrysene ranked highest on the list. Health risk assessment of the top-ranked PAHs was conducted and revealed that cancer risks of PAHs detected in the source water of Danjiangkou to different populations ranged from 10-7 to 104, indicating a low cancer risk to consumers. The results of this study indicated that the adapted CHEMS-1 approach was feasible for site-specific screening of organic contaminants to identify and rank potential priority pollutants.
文摘Inter-basin water deal of nitrogen are great transfers containing a great threats to human health, biodiversity, and air and water quality in the recipient area. Danjiangkou Reservoir, the source reservoir for China＇s South-to-North Water Diversion Middle Route Project, suffers from total nitrogen pollution and threatens the water transfer to a number of metropolises including the capital, Beijing. To locate the main source of nitrogen pollution into the reservoir, especially near the Taocha canal head, where the intake of water transfer begins, we constructed a 3-D water quality model. We then used an inflow sensitivity analysis method to analyze the sig- nificance of inflows from each tributary that may contribute to the total nitrogen pollution and affect water quality. The results indicated that the Han River was the most significant river with a sensitivity index of 0.340, followed by the Dan River with a sensitivity index of 0.089, while the Guanshan River and the Lang River were not significant, with the sensitivity indices of 0.002 and 0.001, respectively. This result implies that the concentration and amount of nitrogen inflow outweighs the geographical position of the tributary for sources of total nitrogen pollution to the Taocha canal head of the Danjiangkou Reservoir.
基金This research was financially supported by the National Natural Science Foundation of China(No.U2040210)the National Key R&D Program(Nos.2019YFC0408904,2019YFC0408901).
文摘As the biggest inter-basin water transfer scheme in the world,the South-to-North Water Diversion Project(SNWD) was designed to alleviate the water crisis in North China.The main channel of the middle route of the SNWD is of great concern in terms of the drinking water quality.In this study,we tested the hypothesis that the dissolved organic matter(DOM) derived from the planktonic algae causes the rising levels of COD_(Mn) along the middle route by monitoring data on water quality(2015-2019,monthly resolution).The results showed that algal density in the main channel increased along the channel and was significantly correlated with COD_(Mn)(p <0.01).Five fluorescent components of DOM,including tyrosine-like(14.85%),tryptophan-like(22.48%),microbial byproduct-like(26.34%),fulvic acid-like(11.41%),and humic acid-like(24.92%) components,were detected.The level of tyrosine-like components increased along the channel and was significantly correlated with algal density(p<0.01),indicating that algae significantly changed the level of DOM in the channel.Algal decomposition and metabolism were found to be the main mechanisms that drive the changes in COD_(Mn).Therefore,controlling algal density would be an important measure to prevent further increase in CODMn and for the guarantee of excellent water quality.
基金supported by National 973 Project China (2013CB733302, 2013CB733305)National Natural Science Foundation of China (41174011, 41429401, 41210006, 41128003, 41021061)
文摘The total capacity of Three Gorges Reservoir（TGR） and Danjiangkou Reservoir（DJR） is large and has significant seasonal fluctuations, which give rise to crustal instability. In this research, we focus on studying the temporal and spatial variation of crustal deformation in Hubei Province caused by reservoir impoundment of TGR and DJR.The Digital Elevation Model, historical hydrological information, GPS monitoring data and load-induced deformation model are combined to monitor the crustal deformation. The modeled results indicate that in the trapezoidal area between the TGR and DJR, the average vertical deformations at different latitudes have different variation tendencies. The vertical deformation modulus and fluctuation amplitude are larger at the latitude of 33 N/32.5 N from 2003 to 2006 and at the latitude of 31 N/32.5 N from 2008 to 2014, while the latter are much larger than the former. Moreover, from2008 to 2014, the frequency and the intensity of seismic activities are all enhanced significantly in this region. The modeled results at the GPS sites are consistent with the vertical displacement of GPS monitoring results in trends and the waveform. It can be inferred that the seasonal deformation is elastic. The horizontal deformation components have the same variation trends with that at each GPS monitoring station,which demonstrates that the whole region is moving toward the southeast. The spatial variation of crustal deformation demonstrates that the impoundment of TGR in2003 causes significant vertical displacements, with the maximum modulus of 32 mm downward located in Xiangjiang River＇s estuary. When the water storage increases, the maximum value will become larger, and the location will move toward the upstream.Besides, the earthquakes occurred more frequently in the region with maximum deformation modulus.
文摘As a critical water source for the central route of the South-to-North Water Diversion Project,the Danjiangkou Reservoir has consistently achieved a water quality rating of Gradell or above,thanks to its efforts to keep enhancing water qualityprotection.
