We demonstrate high current efficiency of a blue fluorescent organic light-emitting diode （OLED） by using the charge control layers （CCLs） based on Alq3 . The CCLs that are inserted into the emitting layers （EMLs...We demonstrate high current efficiency of a blue fluorescent organic light-emitting diode （OLED） by using the charge control layers （CCLs） based on Alq3 . The CCLs that are inserted into the emitting layers （EMLs） could impede the hole injection and facilitate the electron transport, which can improve the carrier balance and further expand the exciton generation region. The maximal current efficiency of the optimal device is 5.89 cd/A at 1.81 mA/cm2 , which is about 2.19 times higher than that of the control device （CD） without the CCL, and the maximal luminance is 19.660 cd/m2 at 12V. The device shows a good color stability though the green light emitting material Alq3 is introduced as the CCL in the EML, but it has a poor lifetime due to the formation of cationic Alq3 species.展开更多
Graphene, a well-known two-dimensional(2 D) material, has sparked broad enthusiasm in both scientific and industrial communities in these years, due to its exceptional electrical, thermal, mechanical, and versatile pr...Graphene, a well-known two-dimensional(2 D) material, has sparked broad enthusiasm in both scientific and industrial communities in these years, due to its exceptional electrical, thermal, mechanical, and versatile properties. However, many properties and applications of graphene are layer-number dependent. The preparation of high-quality graphene with controlled layer numbers is full of challenge, since the layer number varies much with the synthesis routes and relevant experimental conditions. Hence, there is an urgent need to improve the layer-number controllability of graphene preparation. Generally, graphene can be prepared by two complementary approaches: "top-down" and "bottom-up". Since they have their own advantages, the recent advances in the layer-number tunable preparation of high-quality graphene are separately studied from the two aspects in this review, especially those dedicated to single parameter. Some effective strategies are discussed in detail, mainly including 1) supercritical-CO2 assisted sonication, electrochemical exfoliation of graphite intercalation compounds, and layer-by-layer thinning with plasma or laser, for "top-down" graphene;2) chemical vapor deposition(CVD) on dual-metal substrate, ion-implantation CVD, layer-by-layer CVD, plasma-enhanced CVD, layered-double-hydroxides template-assisted CVD;and 3) graphite-enclosure assisted epitaxial growth and pulsed-magnetron-sputtering assisted physical vapor deposition for "bottom-up" graphene on various substrates. In addition, the respective advantages of graphene with different layer numbers in properties and applications are also presented. Finally, the contribution concludes with some important perspectives on the remained challenges and future perspectives.展开更多
Because of its ease of implementation,a linear PID controller is generally used to control robotic manipulators.Linear controllers cannot effectively cope with uncertainties and variations in the parameters;therefore,...Because of its ease of implementation,a linear PID controller is generally used to control robotic manipulators.Linear controllers cannot effectively cope with uncertainties and variations in the parameters;therefore,nonlinear controllers with robust performance which can cope with these are recommended.The sliding mode control(SMC)is a robust state feedback control method for nonlinear systems that,in addition having a simple design,efficiently overcomes uncertainties and disturbances in the system.It also has a very fast transient response that is desirable when controlling robotic manipulators.The most critical drawback to SMC is chattering in the control input signal.To solve this problem,in this study,SMC is used with a boundary layer(SMCBL)to eliminate the chattering and improve the performance of the system.The proposed SMCBL was compared with inverse dynamic control(IDC),a conventional nonlinear control method.The kinematic and dynamic equations of the IRB-120 robot manipulator were initially extracted completely and accurately,and then the control of the robot manipulator using SMC was evaluated.For validation,the proposed control method was implemented on a 6-DOF IRB-120 robot manipulator in the presence of uncertainties.The results were simulated,tested,and compared in the MATLAB/Simulink environment.To further validate our work,the results were tested and confirmed experimentally on an actual IRB-120 robot manipulator.展开更多
The turbulent boundary layer control on NACA 0012 airfoil with Mach number ranging from 0.3 to 0.5 by a spanwise array of dielectric barrier discharge(DBD)plasma actuators by hot-film sensor technology is investigated...The turbulent boundary layer control on NACA 0012 airfoil with Mach number ranging from 0.3 to 0.5 by a spanwise array of dielectric barrier discharge(DBD)plasma actuators by hot-film sensor technology is investigated.Due to temperature change mainly caused through heat produced along with plasma will lead to measurement error of shear stress measured by hot-film sensor,the correction method that takes account of the change measured by another sensor is used and works well.In order to achieve the value of shear stress change,we combine computational fluid dynamics computation with experiment to calibrate the hot-film sensor.To test the stability of the hot-film sensor,seven repeated measurements of shear stress at Ma=0.3 are conducted and show that confidence interval of hot-film sensor measurement is from−0.18 to 0.18 Pa and the root mean square is 0.11 Pa giving a relative error 0.5%over all Mach numbers in this experiment.The research on the turbulent boundary layer control with DBD plasma actuators demonstrates that the control makes shear stress increase by about 6%over the three Mach numbers,which is thought to be reliable through comparing it with the relative error 0.5%,and the value is hardly affected by burst frequency and excitation voltage.展开更多
The flat-plate turbulent boundary layer at Reτ=1140 is manipulated using a spanwise array of bidirectional dielectric barrier discharge(DBD)plasma actuators.Based on the features of no moving mechanical parts in the ...The flat-plate turbulent boundary layer at Reτ=1140 is manipulated using a spanwise array of bidirectional dielectric barrier discharge(DBD)plasma actuators.Based on the features of no moving mechanical parts in the DBD plasma control technology and hot-wire anemometer velocity measurements,a novel convenient method of local drag reduction(DR)measurement is proposed by measuring the single-point velocity within the linear region of the viscous sublayer.We analyze the premise of using the method,and the maximum effective measurement range of-73.1%<DR<42.2%is obtained according to the experimental environment in this work.The local drag decreases downstream of the center of two adjacent upper electrodes and increases downstream of the upper electrodes.The magnitude of the local DR increases with increasing voltage and decreases as it moves away from the actuators.For the spanwise position in between,the streamwise distribution of the local DR is very dependent on the voltage.The variable-interval time-average detection results reveal that all bursting intensities are reduced compared to the baseline,and the amount of reduction is comparable to the absolute values of the local DR.Compared with previous results,we infer that the control mechanism is that many meandering streaks are combined together into single stabilized streaks.展开更多
The visible-light-driven hydrogen evolution is extremely important,but the poor charge transfer capa-bility,a sluggish evolution rate of hydrogen,and severe photo-corrosion make photocatalytic hydrogen evolution impra...The visible-light-driven hydrogen evolution is extremely important,but the poor charge transfer capa-bility,a sluggish evolution rate of hydrogen,and severe photo-corrosion make photocatalytic hydrogen evolution impractical.In this study,we present 1D/2D ReS_(2)-CdS hybrid nanorods for photocatalytic hy-drogen evolution,comprised of a ReS_(2)nanosheet layer grown on CdS nanorods.We found that precise control of the contents of the ReS_(2)nanosheet layer allows for manipulating the electronic structure of Re in the ReS_(2)-CdS hybrid nanorods.The ReS_(2)-CdS hybrid nanorods with optimal ReS_(2)nanosheet layer content dramatically improve photocatalytic hydrogen evolution activity.Notably,photocatalytic hydro-gen evolution activity(64.93 mmol g^(−1)h^(−1))of ReS_(2)-CdS hybrid nanorods with ReS_(2)nanosheet layers(Re/Cd atomic ratio of 0.051)is approximately 136 times higher than that of pure CdS nanorods under visible light irradiation.Furthermore,intimated coupling of the ReS_(2)nanosheet layer with CdS nanorods reduced the surface trap-site of the CdS nanorods,resulting in enhanced photocatalytic stability.The de-tailed optical and electrical investigations demonstrate that the optimal ReS_(2)nanosheet layer contents in the ReS_(2)-CdS hybrid nanorods can provide improved charge transfer capability,catalytic activity,and light absorption efficiency.This study sheds light on the development of photocatalysts for highly efficient photocatalytic hydrogen evolution.展开更多
Based on the research result on the strake-wing, when the size of a strakeis not large, there is a separation zone near the leading edge of the outwing of thestrake-wing at middle angles of attack. So the idea on sepa...Based on the research result on the strake-wing, when the size of a strakeis not large, there is a separation zone near the leading edge of the outwing of thestrake-wing at middle angles of attack. So the idea on separation control by rotating acone placed near the leading edge is presented. The cone surface consists of the part ofthe wing. The effect of rotating the cone on aerodynamic characteristics of thestrake-wing is investigated. The results show that a rotating surface could play an important role in controlling the flow separation for a 3-dimensional wing. For example,the relative increment in maximum lift coefficient attains 30%. The separation zone issuppressed to a certain extent.展开更多
A layered modeling method is proposed to resolve the problems resulting from the complexity of the error model of a multi-axis motion control system. In this model, a low level layer can be used as a virtual axis by t...A layered modeling method is proposed to resolve the problems resulting from the complexity of the error model of a multi-axis motion control system. In this model, a low level layer can be used as a virtual axis by the high level layer. The first advantage of this model is that the complex error model of a four-axis motion control system can be divided into several simple layers and each layer has different coupling strength to match the real control system. The second advantage lies in the fact that the controller in each layer can be designed specifically for a certain purpose. In this research, a three-layered cross coupling scheme in a four-axis motion control system is proposed to compensate the contouring error of the motion control system. Simulation results show that the maximum contouring error is reduced from 0.208 mm to 0.022 mm and the integration of absolute error is reduced from 0.108 mm to 0.015 mm, which are respectively better than 0.027 mm and 0.037 mm by the traditional method. And in the bottom layer the proposed method also has remarkable ability to achieve high contouring accuracy.展开更多
Graphene-metal based materials have been utilized in lithium-sulfur(Li–S)batteries owing to their integrated functionalities thus far.However,their synthesis has predominantly relied on wet-chemistry routes,which lim...Graphene-metal based materials have been utilized in lithium-sulfur(Li–S)batteries owing to their integrated functionalities thus far.However,their synthesis has predominantly relied on wet-chemistry routes,which limited their practical activity in Li–S reaction systems.In this study,we introduce a chemical vapor deposition(CVD)-triggered dry-chemistry approach for the preparation of graphene-cobalt(Co)based catalysts.The versatile CVD technique provides a dry and controllable reaction environment,effectively pledging the compact and clean catalytic interfaces between graphene and Co-based components.Additionally,programmed reactions introduce defects such as vacancies and nitrogen heteroatoms into the catalysts.Notably,the graphene layer number and Co valence state can be delicately manipulated by altering the CVD reaction temperature.Specifically,few-layer graphene wrapped Co/Co_(3)O_(4)(FGr-Co/Co_(3)O_(4))prepared at 450 ℃ shows higher catalytic activity than the multi-layer graphene wrapped Co/CoO(MGr-Co/CoO)synthesized at 550 ℃,attributed to its comprehensive control of clean interface,valence distribution range and defects.Leveraging these advantages,the battery with FGr-Co/Co_(3)O_(4)shows favorable working stability with a degradation rate of only 0.08%over 500 cycles at 1.0 C.Furthermore,under an elevated sulfur loading of 6.1 mg cm^(–2),the battery harvests a remarkable areal capacity of 5.9 mA h cm^(–2)along with stable cyclic operation.展开更多
Bilayer and multilayer two-dimensional(2D)van der Waals materials,such as graphene,hexagonal boron nitride(hBN),and transition metal dichalcogenides(TMDs),possess transformative potential across electronics,photonics,...Bilayer and multilayer two-dimensional(2D)van der Waals materials,such as graphene,hexagonal boron nitride(hBN),and transition metal dichalcogenides(TMDs),possess transformative potential across electronics,photonics,and quantum technologies due to their tunable electronic band structures,exceptional electrical and optical properties,extraordinary mechanical strength,and superior barrier performance[[1],[2],[3]].Taking graphene as a representative example,the control of stacking critically governs its electronic states and device functionalities.展开更多
This work studies the turbulent drag reduction(TDR)effect of a flat plate model using a spanwise slot blowing pulsed plasma actuator(SBP-PA).Wind tunnel experiments are carried out under a Reynolds number of 1.445...This work studies the turbulent drag reduction(TDR)effect of a flat plate model using a spanwise slot blowing pulsed plasma actuator(SBP-PA).Wind tunnel experiments are carried out under a Reynolds number of 1.445×10^(4).Using a hot-wire anemometer and an electrical data acquisition system,the influences of millisecond pulsed plasma actuation with different burst frequencies and duty cycles on the microscale coherent structures near the wall of the turbulent boundary layer(TBL)are studied.The experimental results show that the SBP-PA can effectively reduce the frictional drag of the TBL.When the duty cycle exceeds 30%,the TDR rate is greater than 11%,and the optimal drag reduction rate of 13.69%is obtained at a duty cycle of 50%.Furthermore,optimizing the electrical parameters reveals that increasing the burst frequency significantly reduces the velocity distribution in the logarithmic region of the TBL.When the normalized burst frequency reaches f+=2πf_(p)d/U_(∞)=7.196,the optimal TDR effectiveness is 16.97%,indicating a resonance phenomenon between the pulsed plasma actuation and the microscale coherent structures near the wall.Therefore,reasonably selecting the electrical parameters of the plasma actuator is expected to significantly improve the TDR effect.展开更多
In fractured reservoirs characterized by low matrix permeability,fracture networks control the main fluid flow paths.However,in layered reservoirs,the vertical extension of fractures is often restricted to single laye...In fractured reservoirs characterized by low matrix permeability,fracture networks control the main fluid flow paths.However,in layered reservoirs,the vertical extension of fractures is often restricted to single layers.In this study,we explored the effect of changing marl/shale thickness on fracture extension using comprehensive field data and numerical modeling.The field data were sampled from coastal exposures of Liassic limestone-marl/shale alternations in Wales and Somerset(Bristol Channel Basin,UK).The vertical fracture traces of more than 4000 fractures were mapped in detail.Six sections were selected to represent a variety of layer thicknesses.Besides the field data also thin sections were analyzed.Numerical models of fracture extension in a two-layer limestone-marl system were based on field data and laboratory measurements of Young's moduli.The modeled principal stress magnitude σ3 along the lithological contact was used as an indication for fracture extension through marls.Field data exhibit good correlation(R^2=0.76) between fracture extension and marl thickness,the thicker the marl layer the fewer fractures propagate through.The model results show that almost no tensile stress reaches the top of the marl layer when the marls are thicker than 30 cm.For marls that are less than 20 cm,the propagation of stress is more dependent on the stiffness of the marls.The higher the contrast between limestone and marl stiffness the lower the stress that is transmitted into the marl layer.In both model experiments and field data the critical marl thickness for fracture extension is ca.15-20 cm.This quantification of critical marl thicknesses can be used to improve predictions of fracture networks and permeability in layered rocks.Up-or downsampling methods often ignore spatially continuous impermeable layers with thicknesses that are under the detection limit of seismic data.However,ignoring these layers can lead to overestimates of the overall permeability.Therefore,the understanding of how fractures propagate and terminate through impermeable layers will help to improve the characterization of conventional reservoirs.展开更多
Nature has shown us that the microstructure of the skin of fast-swimming sharks in the ocean can reduce the skin friction drag due to the well-known shark-skin effect.In the present study,the effect of shark-skin-insp...Nature has shown us that the microstructure of the skin of fast-swimming sharks in the ocean can reduce the skin friction drag due to the well-known shark-skin effect.In the present study,the effect of shark-skin-inspired riblets on coherent vortex structures in a turbulent boundary layer（TBL） is investigated.This is done by means of tomographic particle image velocimetry（TPIV） measurements in channel fl ws over an acrylic plate of drag-reducing riblets at a friction Reynolds number of 190.The turbulent fl ws over drag-reducing riblets are verifie by a planar time-resolved particle image velocimetry（TRPIV） system initially,and then the TPIV measurements are performed.Two-dimensional（2D） experimental results with a dragreduction rate of around 4.81% are clearly visible over triangle riblets with a peak-to-peak spacing s＋of 14,indicating from the drag-reducing performance that the buffer layer within the TBL has thickened;the logarithmic law region has shifted upward and the Reynolds shear stress decreased.A comparison of the spatial topological distributions of the spanwise vorticity of coherent vortex structures extracted at different wall-normal heights through the improved quadrant splitting method shows that riblets weaken the amplitudesof the spanwise vorticity when ejection（Q2） and sweep（Q4） events occur at the near wall,having the greatest effect on Q4 events in particular.The so-called quadrupole statistical model for coherent structures in the whole TBL is verified Meanwhile,their spatial conditional-averaged topological shapes and the spatial scales of quadrupole coherent vortex structures as a whole in the overlying turbulent fl w over riblets are changed,suggesting that the riblets dampen the momentum and energy exchange between the regions of near-wall and outer portion of the TBL by depressing the bursting events（Q2 and Q4）,thereby reducing the skin friction drag.展开更多
Reconfigurable photonic integrated circuits(PICs)can implement arbitrary operations and signal processing functionalities directly in the optical domain.Run-time configuration of these circuits requires an electronic ...Reconfigurable photonic integrated circuits(PICs)can implement arbitrary operations and signal processing functionalities directly in the optical domain.Run-time configuration of these circuits requires an electronic control layer to adjust the working point of their building elements and compensate for thermal drifts or degradations of the input signal.As the advancement of photonic foundries enables the fabrication of chips of increasing complexity,developing scalable electronic controllers becomes crucial for the operation of complex PICs.In this paper,we present an electronic application-specific integrated circuit(ASIC)designed for reconfiguration of PICs featuring numerous tunable elements.Each channel of the ASIC controller independently addresses one optical component of the PIC,and multiple parallel local feedback loops are operated to achieve full control.The proposed design is validated through real-time reconfiguration of a 16-channel silicon photonics adaptive universal beam coupler.Results demonstrate automatic coupling of an arbitrary input beam to a single-mode waveguide,dynamic compensation of beam wavefront distortions and successful transmission of a 50 Gbit/s signal through an optical free-space link.The low power consumption and compactness of the electronic chip provide a scalable paradigm that can be seamlessly extended to larger photonic architectures.展开更多
Our living environment is surrounded by turbulence, which is also a concern of the global energy consumption and the greenhouse gas emission, and the viscous force on the solid-liquid/solid-gas interface is an importa...Our living environment is surrounded by turbulence, which is also a concern of the global energy consumption and the greenhouse gas emission, and the viscous force on the solid-liquid/solid-gas interface is an important part of the turbulence. Reducing friction force in turbulence to the greatest extent is becoming an urgent issue to be resolved at present. In this paper, the various state-of-the-art approaches of drag-reducing and energy-saving technologies based on the boundary layer control are reviewed, focusing on the polymer drag reduction additives, the micro-morphology, the super-hydrophobic surface, the micro air bubbles, the heating wall, the vibrant flexible wall and the composite drag reduction methods. In addition, the mechanisms of different drag reductions based on the boundary layer control and the potential applications in fluid engineering are discussed. This paper aims not only to contribute to a better understanding of drag reduction mechanisms, but also to offer new perspectives to improve the current drag-reducing and energy saving technologies.展开更多
Turbulent boundary layer control(TBLC) for skin-friction drag reduction is a relatively new technology made possible through the advances in computational-simulation capabilities,which have improved the understanding ...Turbulent boundary layer control(TBLC) for skin-friction drag reduction is a relatively new technology made possible through the advances in computational-simulation capabilities,which have improved the understanding of the flow structures of turbulence.Advances in micro-electronic technology have enabled the fabrication of active device systems able to manipulating these structures.The combination of simulation,understanding and micro-actuation technologies offers new opportunities to significantly decrease drag,and by doing so,to increase fuel efficiency of future aircraft.The literature review that follows shows that the application of active control turbulent skin-friction drag reduction is considered of prime importance by industry,even though it is still at a low technology readiness level(TRL).This review presents the state of the art of different technologies oriented to the active and passive control for turbulent skin-friction drag reduction and contributes to the improvement of these technologies.展开更多
The traditional PI controller for a hybrid energy storage system(HESS)has certain drawbacks,such as difficult tuning of the controller parameters and the additional filters to allocate high-and low-frequency power flu...The traditional PI controller for a hybrid energy storage system(HESS)has certain drawbacks,such as difficult tuning of the controller parameters and the additional filters to allocate high-and low-frequency power fluctuations.This paper proposes a model predictive control(MPC)method to control three-level bidirectional DC/DC converters for grid-connections to a HESS in a DC microgrid.First,the mathematical model of a HESS consisting of a battery and ultra capacitor(UC)is established and the neutral point voltage imbalance of a three-level converter is solved by analyzing the operating modes of the converter.Secondly,for the control of the grid-connected converters,an MPC method is proposed for calculating steady-state reference values in the outer layer and the dynamic rolling optimization in the inner layer.The outer layer ensures the voltage regulation and establishes the current predictive model,while the inner layer,using the model predictive current control,makes the current follow the predictive value,thus reducing the system current ripple.This cascaded topology has two independent controllers and is free of filters to realize the high-and low-frequency power allocation for a HESS.Therefore,it allows two types of energy storage devices to independently regulate the voltage and realizes the power allocation of the battery and UC.Finally,simulation studies are conducted in PSCAD/EMTDC,and the effectiveness of the proposed HESS control strategy is verified in a case,such as a controller comparison and fault scenario.展开更多
The increasing demand for solar energy,driven by the climate crisis and carbon neutrality goals,un-derscores the critical importance of aesthetics in solar panel integration across diverse environments,such as buildin...The increasing demand for solar energy,driven by the climate crisis and carbon neutrality goals,un-derscores the critical importance of aesthetics in solar panel integration across diverse environments,such as building-integrated photovoltaics.This study addresses this need by developing angle-insensitive coloration for translucent perovskite-colored solar cells(TPCSCs)to enhance both functionality and con-sumer appeal.By engineering oxide/metal/oxide(OMO)multilayer structures,we achieved consistent col-oration regardless of the viewing angle,overcoming a major challenge in colored solar cell technology.Specifically,ZnO:Al/Ag/ZnO:Al-based OMO layers were meticulously optimized to balance visual appeal with photovoltaic efficiency.Our results demonstrate exceptional angular stability,with negligible color shifts observed even at viewing angles exceeding 60°,significantly surpassing the limitations of previ-ous designs,which exhibited sensitivity at 40°.The OMO electrodes exploited distributed Bragg reflector(DBR)properties to amplify interference effects and utilized delocalized plasmonic modes and metal-dielectric-metal(MDM)cavity resonances to achieve vibrant colors.Advanced 3-pair OMO transparent conductive electrodes(TCEs)exhibited stable,angle-insensitive blue coloration,and the resulting translu-cent perovskite solar cell achieved a record-high power conversion efficiency(PCE)of 8.25%and an av-erage transmittance of 15.23%,maintaining consistent coloration up to a 60°viewing angle.Additionally,the optoelectronic control layer(OCL)thickness was fine-tuned to precisely target specific wavelengths,enabling a versatile spectrum of colors,including blue,green,yellowish-green,orange,and peach.This pioneering approach not only ensures color fidelity but also enhances the reflectance properties of TPC-SCs.By integrating aesthetic and functional advancements,our research makes a significant contribution to the development of sustainable energy solutions for future smart cities.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 60906022 and 60676051)the Natural Science Foundation of Tianjin,China (Grant No. 10JCYBJC01100)+2 种基金the Scientific Developing Foundation of Tianjin Education Commission, China (Grant No. 2011ZD02)the Jiangsu Provincial Natural Science Development Foundation for University, China (Grant No. 09KJB140006)the Tianjin Natural Science Council (Grant No. 10SYSYJC28100)
文摘We demonstrate high current efficiency of a blue fluorescent organic light-emitting diode （OLED） by using the charge control layers （CCLs） based on Alq3 . The CCLs that are inserted into the emitting layers （EMLs） could impede the hole injection and facilitate the electron transport, which can improve the carrier balance and further expand the exciton generation region. The maximal current efficiency of the optimal device is 5.89 cd/A at 1.81 mA/cm2 , which is about 2.19 times higher than that of the control device （CD） without the CCL, and the maximal luminance is 19.660 cd/m2 at 12V. The device shows a good color stability though the green light emitting material Alq3 is introduced as the CCL in the EML, but it has a poor lifetime due to the formation of cationic Alq3 species.
基金Sponsored by the JSPS Invitational Fellow ship for Research in Japan (Grant No. L18516)the National Natural Science Foundation of China(Grant No. 51273148)
文摘Graphene, a well-known two-dimensional(2 D) material, has sparked broad enthusiasm in both scientific and industrial communities in these years, due to its exceptional electrical, thermal, mechanical, and versatile properties. However, many properties and applications of graphene are layer-number dependent. The preparation of high-quality graphene with controlled layer numbers is full of challenge, since the layer number varies much with the synthesis routes and relevant experimental conditions. Hence, there is an urgent need to improve the layer-number controllability of graphene preparation. Generally, graphene can be prepared by two complementary approaches: "top-down" and "bottom-up". Since they have their own advantages, the recent advances in the layer-number tunable preparation of high-quality graphene are separately studied from the two aspects in this review, especially those dedicated to single parameter. Some effective strategies are discussed in detail, mainly including 1) supercritical-CO2 assisted sonication, electrochemical exfoliation of graphite intercalation compounds, and layer-by-layer thinning with plasma or laser, for "top-down" graphene;2) chemical vapor deposition(CVD) on dual-metal substrate, ion-implantation CVD, layer-by-layer CVD, plasma-enhanced CVD, layered-double-hydroxides template-assisted CVD;and 3) graphite-enclosure assisted epitaxial growth and pulsed-magnetron-sputtering assisted physical vapor deposition for "bottom-up" graphene on various substrates. In addition, the respective advantages of graphene with different layer numbers in properties and applications are also presented. Finally, the contribution concludes with some important perspectives on the remained challenges and future perspectives.
文摘Because of its ease of implementation,a linear PID controller is generally used to control robotic manipulators.Linear controllers cannot effectively cope with uncertainties and variations in the parameters;therefore,nonlinear controllers with robust performance which can cope with these are recommended.The sliding mode control(SMC)is a robust state feedback control method for nonlinear systems that,in addition having a simple design,efficiently overcomes uncertainties and disturbances in the system.It also has a very fast transient response that is desirable when controlling robotic manipulators.The most critical drawback to SMC is chattering in the control input signal.To solve this problem,in this study,SMC is used with a boundary layer(SMCBL)to eliminate the chattering and improve the performance of the system.The proposed SMCBL was compared with inverse dynamic control(IDC),a conventional nonlinear control method.The kinematic and dynamic equations of the IRB-120 robot manipulator were initially extracted completely and accurately,and then the control of the robot manipulator using SMC was evaluated.For validation,the proposed control method was implemented on a 6-DOF IRB-120 robot manipulator in the presence of uncertainties.The results were simulated,tested,and compared in the MATLAB/Simulink environment.To further validate our work,the results were tested and confirmed experimentally on an actual IRB-120 robot manipulator.
基金the European Commission through the Research and Innovation action DRAGY(Drag Reduction via Turbulent Boundary Layer Flow Control)under Grant No.690623+1 种基金the Ministry of Industry and Information Technology(MIIT)of the Chinese governmentsupport received from National Natural Science Foundation of China(No.11572256).
文摘The turbulent boundary layer control on NACA 0012 airfoil with Mach number ranging from 0.3 to 0.5 by a spanwise array of dielectric barrier discharge(DBD)plasma actuators by hot-film sensor technology is investigated.Due to temperature change mainly caused through heat produced along with plasma will lead to measurement error of shear stress measured by hot-film sensor,the correction method that takes account of the change measured by another sensor is used and works well.In order to achieve the value of shear stress change,we combine computational fluid dynamics computation with experiment to calibrate the hot-film sensor.To test the stability of the hot-film sensor,seven repeated measurements of shear stress at Ma=0.3 are conducted and show that confidence interval of hot-film sensor measurement is from−0.18 to 0.18 Pa and the root mean square is 0.11 Pa giving a relative error 0.5%over all Mach numbers in this experiment.The research on the turbulent boundary layer control with DBD plasma actuators demonstrates that the control makes shear stress increase by about 6%over the three Mach numbers,which is thought to be reliable through comparing it with the relative error 0.5%,and the value is hardly affected by burst frequency and excitation voltage.
基金the financial support received from the National Science Fund for Distinguished Young Scholars(No.12102359)。
文摘The flat-plate turbulent boundary layer at Reτ=1140 is manipulated using a spanwise array of bidirectional dielectric barrier discharge(DBD)plasma actuators.Based on the features of no moving mechanical parts in the DBD plasma control technology and hot-wire anemometer velocity measurements,a novel convenient method of local drag reduction(DR)measurement is proposed by measuring the single-point velocity within the linear region of the viscous sublayer.We analyze the premise of using the method,and the maximum effective measurement range of-73.1%<DR<42.2%is obtained according to the experimental environment in this work.The local drag decreases downstream of the center of two adjacent upper electrodes and increases downstream of the upper electrodes.The magnitude of the local DR increases with increasing voltage and decreases as it moves away from the actuators.For the spanwise position in between,the streamwise distribution of the local DR is very dependent on the voltage.The variable-interval time-average detection results reveal that all bursting intensities are reduced compared to the baseline,and the amount of reduction is comparable to the absolute values of the local DR.Compared with previous results,we infer that the control mechanism is that many meandering streaks are combined together into single stabilized streaks.
基金supported by the National Re-search Foundation of Korea(Nos.NRF-2020R1C1C1008514,2019R1A6A1A11053838,and NRF-2023R1A2C1004015)the“Regional Innovation Strategy(RIS)”through the National Research Foundation of Korea(NRF)funded by the Ministry of Education(MOE)(No.2021RIS-003).
文摘The visible-light-driven hydrogen evolution is extremely important,but the poor charge transfer capa-bility,a sluggish evolution rate of hydrogen,and severe photo-corrosion make photocatalytic hydrogen evolution impractical.In this study,we present 1D/2D ReS_(2)-CdS hybrid nanorods for photocatalytic hy-drogen evolution,comprised of a ReS_(2)nanosheet layer grown on CdS nanorods.We found that precise control of the contents of the ReS_(2)nanosheet layer allows for manipulating the electronic structure of Re in the ReS_(2)-CdS hybrid nanorods.The ReS_(2)-CdS hybrid nanorods with optimal ReS_(2)nanosheet layer content dramatically improve photocatalytic hydrogen evolution activity.Notably,photocatalytic hydro-gen evolution activity(64.93 mmol g^(−1)h^(−1))of ReS_(2)-CdS hybrid nanorods with ReS_(2)nanosheet layers(Re/Cd atomic ratio of 0.051)is approximately 136 times higher than that of pure CdS nanorods under visible light irradiation.Furthermore,intimated coupling of the ReS_(2)nanosheet layer with CdS nanorods reduced the surface trap-site of the CdS nanorods,resulting in enhanced photocatalytic stability.The de-tailed optical and electrical investigations demonstrate that the optimal ReS_(2)nanosheet layer contents in the ReS_(2)-CdS hybrid nanorods can provide improved charge transfer capability,catalytic activity,and light absorption efficiency.This study sheds light on the development of photocatalysts for highly efficient photocatalytic hydrogen evolution.
文摘Based on the research result on the strake-wing, when the size of a strakeis not large, there is a separation zone near the leading edge of the outwing of thestrake-wing at middle angles of attack. So the idea on separation control by rotating acone placed near the leading edge is presented. The cone surface consists of the part ofthe wing. The effect of rotating the cone on aerodynamic characteristics of thestrake-wing is investigated. The results show that a rotating surface could play an important role in controlling the flow separation for a 3-dimensional wing. For example,the relative increment in maximum lift coefficient attains 30%. The separation zone issuppressed to a certain extent.
基金Project(51005086)supported by the National Natural Science Foundation of ChinaProject(2010MS085)supported by the Fundamental Research Funds for the Central Universities,ChinaProject(DMETKF2013008)supported by the Open Project of the State Key Laboratory of Digital Manufacturing Equipment and Technology,China
文摘A layered modeling method is proposed to resolve the problems resulting from the complexity of the error model of a multi-axis motion control system. In this model, a low level layer can be used as a virtual axis by the high level layer. The first advantage of this model is that the complex error model of a four-axis motion control system can be divided into several simple layers and each layer has different coupling strength to match the real control system. The second advantage lies in the fact that the controller in each layer can be designed specifically for a certain purpose. In this research, a three-layered cross coupling scheme in a four-axis motion control system is proposed to compensate the contouring error of the motion control system. Simulation results show that the maximum contouring error is reduced from 0.208 mm to 0.022 mm and the integration of absolute error is reduced from 0.108 mm to 0.015 mm, which are respectively better than 0.027 mm and 0.037 mm by the traditional method. And in the bottom layer the proposed method also has remarkable ability to achieve high contouring accuracy.
基金support of the National Natural Science Foundation of China(Grant No.52172239,52202038,and 52402247)the Innovative Funds Plan of Henan University of Technology(Grant No.2020ZKCJ07)the Natural Science Foundation of Shandong Province(Grant No.ZR2022QE081)。
文摘Graphene-metal based materials have been utilized in lithium-sulfur(Li–S)batteries owing to their integrated functionalities thus far.However,their synthesis has predominantly relied on wet-chemistry routes,which limited their practical activity in Li–S reaction systems.In this study,we introduce a chemical vapor deposition(CVD)-triggered dry-chemistry approach for the preparation of graphene-cobalt(Co)based catalysts.The versatile CVD technique provides a dry and controllable reaction environment,effectively pledging the compact and clean catalytic interfaces between graphene and Co-based components.Additionally,programmed reactions introduce defects such as vacancies and nitrogen heteroatoms into the catalysts.Notably,the graphene layer number and Co valence state can be delicately manipulated by altering the CVD reaction temperature.Specifically,few-layer graphene wrapped Co/Co_(3)O_(4)(FGr-Co/Co_(3)O_(4))prepared at 450 ℃ shows higher catalytic activity than the multi-layer graphene wrapped Co/CoO(MGr-Co/CoO)synthesized at 550 ℃,attributed to its comprehensive control of clean interface,valence distribution range and defects.Leveraging these advantages,the battery with FGr-Co/Co_(3)O_(4)shows favorable working stability with a degradation rate of only 0.08%over 500 cycles at 1.0 C.Furthermore,under an elevated sulfur loading of 6.1 mg cm^(–2),the battery harvests a remarkable areal capacity of 5.9 mA h cm^(–2)along with stable cyclic operation.
基金supported by the Air Force Office of Scientific Research(FA9550-22-1-0526)the US Army Corps of Engineers,ERDC grant(W912HZ-21-2-0050 and W912HZ-24-2-0027)the Rice Academy Fellowship from Rice University.
文摘Bilayer and multilayer two-dimensional(2D)van der Waals materials,such as graphene,hexagonal boron nitride(hBN),and transition metal dichalcogenides(TMDs),possess transformative potential across electronics,photonics,and quantum technologies due to their tunable electronic band structures,exceptional electrical and optical properties,extraordinary mechanical strength,and superior barrier performance[[1],[2],[3]].Taking graphene as a representative example,the control of stacking critically governs its electronic states and device functionalities.
基金supported by National Natural Science Foundation of China(Nos.61971345 and 12175177)the Foundation for Key Laboratories of National Defense Science and Technology of China(No.614220120030810).
文摘This work studies the turbulent drag reduction(TDR)effect of a flat plate model using a spanwise slot blowing pulsed plasma actuator(SBP-PA).Wind tunnel experiments are carried out under a Reynolds number of 1.445×10^(4).Using a hot-wire anemometer and an electrical data acquisition system,the influences of millisecond pulsed plasma actuation with different burst frequencies and duty cycles on the microscale coherent structures near the wall of the turbulent boundary layer(TBL)are studied.The experimental results show that the SBP-PA can effectively reduce the frictional drag of the TBL.When the duty cycle exceeds 30%,the TDR rate is greater than 11%,and the optimal drag reduction rate of 13.69%is obtained at a duty cycle of 50%.Furthermore,optimizing the electrical parameters reveals that increasing the burst frequency significantly reduces the velocity distribution in the logarithmic region of the TBL.When the normalized burst frequency reaches f+=2πf_(p)d/U_(∞)=7.196,the optimal TDR effectiveness is 16.97%,indicating a resonance phenomenon between the pulsed plasma actuation and the microscale coherent structures near the wall.Therefore,reasonably selecting the electrical parameters of the plasma actuator is expected to significantly improve the TDR effect.
基金supported by the Deutsche Forschungsgemeinschaft(DFG,grant PH 189/2-1)
文摘In fractured reservoirs characterized by low matrix permeability,fracture networks control the main fluid flow paths.However,in layered reservoirs,the vertical extension of fractures is often restricted to single layers.In this study,we explored the effect of changing marl/shale thickness on fracture extension using comprehensive field data and numerical modeling.The field data were sampled from coastal exposures of Liassic limestone-marl/shale alternations in Wales and Somerset(Bristol Channel Basin,UK).The vertical fracture traces of more than 4000 fractures were mapped in detail.Six sections were selected to represent a variety of layer thicknesses.Besides the field data also thin sections were analyzed.Numerical models of fracture extension in a two-layer limestone-marl system were based on field data and laboratory measurements of Young's moduli.The modeled principal stress magnitude σ3 along the lithological contact was used as an indication for fracture extension through marls.Field data exhibit good correlation(R^2=0.76) between fracture extension and marl thickness,the thicker the marl layer the fewer fractures propagate through.The model results show that almost no tensile stress reaches the top of the marl layer when the marls are thicker than 30 cm.For marls that are less than 20 cm,the propagation of stress is more dependent on the stiffness of the marls.The higher the contrast between limestone and marl stiffness the lower the stress that is transmitted into the marl layer.In both model experiments and field data the critical marl thickness for fracture extension is ca.15-20 cm.This quantification of critical marl thicknesses can be used to improve predictions of fracture networks and permeability in layered rocks.Up-or downsampling methods often ignore spatially continuous impermeable layers with thicknesses that are under the detection limit of seismic data.However,ignoring these layers can lead to overestimates of the overall permeability.Therefore,the understanding of how fractures propagate and terminate through impermeable layers will help to improve the characterization of conventional reservoirs.
基金supported by the National Natural Science Foundation of China (Grants 11332006,11272233,and 11411130150)the foundation from the China Scholarship Council (CSC) (Grant 201306250092)the Foundation Project for Outstanding Doctoral Dissertations of Tianjin University
文摘Nature has shown us that the microstructure of the skin of fast-swimming sharks in the ocean can reduce the skin friction drag due to the well-known shark-skin effect.In the present study,the effect of shark-skin-inspired riblets on coherent vortex structures in a turbulent boundary layer（TBL） is investigated.This is done by means of tomographic particle image velocimetry（TPIV） measurements in channel fl ws over an acrylic plate of drag-reducing riblets at a friction Reynolds number of 190.The turbulent fl ws over drag-reducing riblets are verifie by a planar time-resolved particle image velocimetry（TRPIV） system initially,and then the TPIV measurements are performed.Two-dimensional（2D） experimental results with a dragreduction rate of around 4.81% are clearly visible over triangle riblets with a peak-to-peak spacing s＋of 14,indicating from the drag-reducing performance that the buffer layer within the TBL has thickened;the logarithmic law region has shifted upward and the Reynolds shear stress decreased.A comparison of the spatial topological distributions of the spanwise vorticity of coherent vortex structures extracted at different wall-normal heights through the improved quadrant splitting method shows that riblets weaken the amplitudesof the spanwise vorticity when ejection（Q2） and sweep（Q4） events occur at the near wall,having the greatest effect on Q4 events in particular.The so-called quadrupole statistical model for coherent structures in the whole TBL is verified Meanwhile,their spatial conditional-averaged topological shapes and the spatial scales of quadrupole coherent vortex structures as a whole in the overlying turbulent fl w over riblets are changed,suggesting that the riblets dampen the momentum and energy exchange between the regions of near-wall and outer portion of the TBL by depressing the bursting events（Q2 and Q4）,thereby reducing the skin friction drag.
基金supported by the Italian National Recovery and Resilience Plan(NRRP)of Nex tGeneration EU,partnership on“Telecommunications of the Future”(Program“RESTART”,Structural Project“Rigoletto,”and Focused Project“HePIC”)under Grant PE00000001.We thank Polifab,the nanofabrication facility of Politecnico di Milano,for dicing and wire-bonding the chips.
文摘Reconfigurable photonic integrated circuits(PICs)can implement arbitrary operations and signal processing functionalities directly in the optical domain.Run-time configuration of these circuits requires an electronic control layer to adjust the working point of their building elements and compensate for thermal drifts or degradations of the input signal.As the advancement of photonic foundries enables the fabrication of chips of increasing complexity,developing scalable electronic controllers becomes crucial for the operation of complex PICs.In this paper,we present an electronic application-specific integrated circuit(ASIC)designed for reconfiguration of PICs featuring numerous tunable elements.Each channel of the ASIC controller independently addresses one optical component of the PIC,and multiple parallel local feedback loops are operated to achieve full control.The proposed design is validated through real-time reconfiguration of a 16-channel silicon photonics adaptive universal beam coupler.Results demonstrate automatic coupling of an arbitrary input beam to a single-mode waveguide,dynamic compensation of beam wavefront distortions and successful transmission of a 50 Gbit/s signal through an optical free-space link.The low power consumption and compactness of the electronic chip provide a scalable paradigm that can be seamlessly extended to larger photonic architectures.
文摘Our living environment is surrounded by turbulence, which is also a concern of the global energy consumption and the greenhouse gas emission, and the viscous force on the solid-liquid/solid-gas interface is an important part of the turbulence. Reducing friction force in turbulence to the greatest extent is becoming an urgent issue to be resolved at present. In this paper, the various state-of-the-art approaches of drag-reducing and energy-saving technologies based on the boundary layer control are reviewed, focusing on the polymer drag reduction additives, the micro-morphology, the super-hydrophobic surface, the micro air bubbles, the heating wall, the vibrant flexible wall and the composite drag reduction methods. In addition, the mechanisms of different drag reductions based on the boundary layer control and the potential applications in fluid engineering are discussed. This paper aims not only to contribute to a better understanding of drag reduction mechanisms, but also to offer new perspectives to improve the current drag-reducing and energy saving technologies.
基金supported by the European Commission though the Research and Innovation action DRAGY(Grant No.690623)the Ministry of Industry and Information Technology(MIIT)of the Chinese government
文摘Turbulent boundary layer control(TBLC) for skin-friction drag reduction is a relatively new technology made possible through the advances in computational-simulation capabilities,which have improved the understanding of the flow structures of turbulence.Advances in micro-electronic technology have enabled the fabrication of active device systems able to manipulating these structures.The combination of simulation,understanding and micro-actuation technologies offers new opportunities to significantly decrease drag,and by doing so,to increase fuel efficiency of future aircraft.The literature review that follows shows that the application of active control turbulent skin-friction drag reduction is considered of prime importance by industry,even though it is still at a low technology readiness level(TRL).This review presents the state of the art of different technologies oriented to the active and passive control for turbulent skin-friction drag reduction and contributes to the improvement of these technologies.
基金supported in part by the State Grid Corporation of China under Grant No.521500190017.
文摘The traditional PI controller for a hybrid energy storage system(HESS)has certain drawbacks,such as difficult tuning of the controller parameters and the additional filters to allocate high-and low-frequency power fluctuations.This paper proposes a model predictive control(MPC)method to control three-level bidirectional DC/DC converters for grid-connections to a HESS in a DC microgrid.First,the mathematical model of a HESS consisting of a battery and ultra capacitor(UC)is established and the neutral point voltage imbalance of a three-level converter is solved by analyzing the operating modes of the converter.Secondly,for the control of the grid-connected converters,an MPC method is proposed for calculating steady-state reference values in the outer layer and the dynamic rolling optimization in the inner layer.The outer layer ensures the voltage regulation and establishes the current predictive model,while the inner layer,using the model predictive current control,makes the current follow the predictive value,thus reducing the system current ripple.This cascaded topology has two independent controllers and is free of filters to realize the high-and low-frequency power allocation for a HESS.Therefore,it allows two types of energy storage devices to independently regulate the voltage and realizes the power allocation of the battery and UC.Finally,simulation studies are conducted in PSCAD/EMTDC,and the effectiveness of the proposed HESS control strategy is verified in a case,such as a controller comparison and fault scenario.
基金supported by the National Research Foundation of Korea(NRF)funded by the Korea government(MSIT)(NRF-RS-2023-00217270,RS-2023-00212744,and RS-2024-00436187)the Fundamental Research Program(PNKA390)of the Korean Institute of Materials Science(KIMS)+1 种基金the National Research Council of Science&Technology(NST)grant by the Korea govern-ment(MSIT)(No.GTL24041-000)the Energy Technology De-velopment Program of the Korean Institute of Energy Technology Evaluation and Planning(KETEP)(Grant No.RS-2023-00301944).
文摘The increasing demand for solar energy,driven by the climate crisis and carbon neutrality goals,un-derscores the critical importance of aesthetics in solar panel integration across diverse environments,such as building-integrated photovoltaics.This study addresses this need by developing angle-insensitive coloration for translucent perovskite-colored solar cells(TPCSCs)to enhance both functionality and con-sumer appeal.By engineering oxide/metal/oxide(OMO)multilayer structures,we achieved consistent col-oration regardless of the viewing angle,overcoming a major challenge in colored solar cell technology.Specifically,ZnO:Al/Ag/ZnO:Al-based OMO layers were meticulously optimized to balance visual appeal with photovoltaic efficiency.Our results demonstrate exceptional angular stability,with negligible color shifts observed even at viewing angles exceeding 60°,significantly surpassing the limitations of previ-ous designs,which exhibited sensitivity at 40°.The OMO electrodes exploited distributed Bragg reflector(DBR)properties to amplify interference effects and utilized delocalized plasmonic modes and metal-dielectric-metal(MDM)cavity resonances to achieve vibrant colors.Advanced 3-pair OMO transparent conductive electrodes(TCEs)exhibited stable,angle-insensitive blue coloration,and the resulting translu-cent perovskite solar cell achieved a record-high power conversion efficiency(PCE)of 8.25%and an av-erage transmittance of 15.23%,maintaining consistent coloration up to a 60°viewing angle.Additionally,the optoelectronic control layer(OCL)thickness was fine-tuned to precisely target specific wavelengths,enabling a versatile spectrum of colors,including blue,green,yellowish-green,orange,and peach.This pioneering approach not only ensures color fidelity but also enhances the reflectance properties of TPC-SCs.By integrating aesthetic and functional advancements,our research makes a significant contribution to the development of sustainable energy solutions for future smart cities.
