Failure prediction plays an important role for many tasks such as optimal resource management in large-scale system. However, accurately failure number prediction of repairable large-scale long-running computing (RLL...Failure prediction plays an important role for many tasks such as optimal resource management in large-scale system. However, accurately failure number prediction of repairable large-scale long-running computing (RLLC) is a challenge because of the reparability and large-scale. To address the challenge, a general Bayesian serial revision prediction method based on Bootstrap approach and moving average approach is put forward, which can make an accurately prediction for the failure number. To demonstrate the performance gains of our method, extensive experiments on the data of Los Alamos National Laboratory (LANL) cluster is implemented, which is a typical RLLC system. And experimental results show that the prediction accuracy of our method is 80.2 %, and it is a greatly improvement with 4 % compared with some typical methods. Finally, the managerial implications of the models are discussed.展开更多
The efficient chiral Ru 3(CO) 12 systems were prepared in situ from Ru 3(CO) 12 and various chiral diimino-or diamino-diphosphine tetradentate ligands. The systems have been used for the asymmetric transfer hy...The efficient chiral Ru 3(CO) 12 systems were prepared in situ from Ru 3(CO) 12 and various chiral diimino-or diamino-diphosphine tetradentate ligands. The systems have been used for the asymmetric transfer hydrogenation of propiophenone in 2-propanol, leading to 1-phenyl-1-propanol in a 98% yield and 96% e.e. The IR study suggests that the carbonyl hydride anion [HRu 3(CO) 11]- most probably exists as a principal species under the reaction conditions. The high chiral efficiency may be due to the synergetic effect produced by the neighboring ruthenium atoms and a special chiral micro-environment involving the polydentate ligand and the Ru 3 framework.展开更多
The percolation fields constructed around the elements of a cluster system in the phase spaces of properties are studied.It is shown that such neighborhoods significantly increase the number of structure parameters of...The percolation fields constructed around the elements of a cluster system in the phase spaces of properties are studied.It is shown that such neighborhoods significantly increase the number of structure parameters of the system under study,expanding the possibilities of analytical description.To study the structure and properties of such systems in the proposed model,a three-dimensional continuum percolation problem with interacting elements is solved.The dependences of the structure and properties of clusters on the parameters of the generation processes of the cluster system are studied,and analytical dependences are obtained.展开更多
The influence of water on protein conformation was investigated by simulating the molecular dynamics of a model protein lysozyme in different water systems.The lysozyme-water system with TIP3P water model and lysozyme...The influence of water on protein conformation was investigated by simulating the molecular dynamics of a model protein lysozyme in different water systems.The lysozyme-water system with TIP3P water model and lysozyme-water cluster system with six-ring water model were evaluated.In addition,the radial distribution function of solvent around lysozyme was calculated.It is found that the distribution of water molecules around lysozyme is similar to that of water clusters.The analyses of dihedral angles and disulfide bonds of lysozyme show that the conformation of lysozyme is severely damaged in the lysozyme-water cluster system compared with that in the lysozyme-water system.This difference can be attributed to the formation of larger number of intermolecular hydrogen bonds between lysozyme and water cluster.It is in agreement with the analysis that water clusters can change the degree of denaturation in the process of heat denaturation of lysozyme.展开更多
An approach for web server cluster(WSC)reliability and degradation process analysis is proposed.The reliability process is modeled as a non-homogeneous Markov process(NHMH)composed of several non-homogeneous Poisson p...An approach for web server cluster(WSC)reliability and degradation process analysis is proposed.The reliability process is modeled as a non-homogeneous Markov process(NHMH)composed of several non-homogeneous Poisson processes(NHPPs).The arrival rate of each NHPP corresponds to the system software failure rate which is expressed using Cox s proportional hazards model(PHM)in terms of the cumulative and instantaneous load of the software.The cumulative load refers to software cumulative execution time,and the instantaneous load denotes the rate that the users requests arrive at a server.The result of reliability analysis is a time-varying reliability and degradation process over the WSC lifetime.Finally,the evaluation experiment shows the effectiveness of the proposed approach.展开更多
This work reports the structural feature and internal motion of one novel hyperbranching cluster system in dilution solution.The cluster system is composed of HB-PS_(300)-g-Pt BA_(45) hypergraft copolymer chains with ...This work reports the structural feature and internal motion of one novel hyperbranching cluster system in dilution solution.The cluster system is composed of HB-PS_(300)-g-Pt BA_(45) hypergraft copolymer chains with uniform subchain,high molar mass and low polydispersity(M_(w)=1.73×106 g/mol and<M_(w)/M_(n)>≈1.07),where HB-PS and Pt BA represent hyperbranched polystyrene core and poly(tert-butyl polyacrylate)graft,respectively.In the selective solvent of PS blocks(cyclohexane,T_(θ)=34.5℃),the aggregation kinetics and structural feature are found to be precisely tunable for assembled clusters by the aggregation temperature(11℃<T<17℃)and time(0 h<t<24 h).An interesting structural evolution kinetics is observed,namely,the fractal dimension(d_(f))of clusters is found to first increases and then decreases with t,eventually,it reaches a plateau value of d_(f)≈3.0,corresponds to a uniform spherical structure.By using dynamic light scattering(DLS)to monitor the number and strength of relaxation modes inΓ(q)withΓbeing the decay rate and q being the scattering vector,it is quantitatively revealed that the relaxation,intensity contribution and mode origin of internal motions of clusters are neither similar with previously reported cluster systems with high polydispersity,nor with the classical linear chain systems.In particular,in the broad range of 2.0<qR_(h)<6.0,we have observed that the reduced first cumulant[Γ^(*)=Γ(q)/(q^(3)k_(B)T/η_(0))]does not display an asymptotic behavior.Whereas,a better asymptotic behavior is observed by plottingΓ(q)/q^(4) versus qRh.For the first time,our observation provides direct evidence supporting that,for hyperbranching cluster system with low polydispersity and high local chain segment density,the hydrodynamic interaction is greatly weakened due to the enhanced hydrodynamic shielding effect.展开更多
We present metal abundance properties of 144 globular clusters associated with M81. These globulars represent the largest globular cluster sample in M81 till now. Our main results are: the distribution of metalliciti...We present metal abundance properties of 144 globular clusters associated with M81. These globulars represent the largest globular cluster sample in M81 till now. Our main results are: the distribution of metallicities is bimodal, with metallicity peaks at [Fe/H] -1.51 and -0.58, and the metal-poor globular clusters tend to be less spatially concentrated than the metal-rich ones; the metal-rich globular clusters in M81 do not demonstrate a centrally concentrated spatial distribution like the metalrich ones in M31 do; like our Galaxy and M31, the globular clusters in M81 have a small radial metallicity gradient. These results are consistent with those obtained from a small sample of M81 globular clusters. In addition, this paper shows that there is evidence that a strong rotation of the M81 globular cluster system around the minor axis exists, and that rotation is present in the metal-rich globular cluster subsample, but the metal-poor globular cluster subsample shows no evidence of rotation. The most significant difference between the rotation of the metal-rich and metal-poor globular clusters occurs at intermediate projected galactocentric radii. Our results confirm the conclusion of Schroder et al. that M81's metal-rich globular clusters at intermediate projected radii are associated with a thick disk of M81.展开更多
A significant portion of Landslide Early Warning Systems (LEWS) relies on the definition of operational thresholds and the monitoring of cumulative rainfall for alert issuance. These thresholds can be obtained in vari...A significant portion of Landslide Early Warning Systems (LEWS) relies on the definition of operational thresholds and the monitoring of cumulative rainfall for alert issuance. These thresholds can be obtained in various ways, but most often they are based on previous landslide data. This approach introduces several limitations. For instance, there is a requirement for the location to have been previously monitored in some way to have this type of information recorded. Another significant limitation is the need for information regarding the location and timing of incidents. Despite the current ease of obtaining location information (GPS, drone images, etc.), the timing of the event remains challenging to ascertain for a considerable portion of landslide data. Concerning rainfall monitoring, there are multiple ways to consider it, for instance, examining accumulations over various intervals (1 h, 6 h, 24 h, 72 h), as well as in the calculation of effective rainfall, which represents the precipitation that actually infiltrates the soil. However, in the vast majority of cases, both the thresholds and the rain monitoring approach are defined manually and subjectively, relying on the operators’ experience. This makes the process labor-intensive and time-consuming, hindering the establishment of a truly standardized and rapidly scalable methodology on a large scale. In this work, we propose a Landslides Early Warning System (LEWS) based on the concept of rainfall half-life and the determination of thresholds using Cluster Analysis and data inversion. The system is designed to be applied in extensive monitoring networks, such as the one utilized by Cemaden, Brazil’s National Center for Monitoring and Early Warning of Natural Disasters.展开更多
Absolute proper motions and radial velocities of 202 open clusters in the solar neighborhood, which can be used as tracers of the Galactic disk, are used to investigate the kinematics of the Galaxy in the solar vicini...Absolute proper motions and radial velocities of 202 open clusters in the solar neighborhood, which can be used as tracers of the Galactic disk, are used to investigate the kinematics of the Galaxy in the solar vicinity, including the mean heliocentric velocity components (u1, u2, u3) of the open cluster system, the characteristic velocity dispersions (σ1,σ2,σ3), Oort constants (A, B) and the large-scale radial motion parameters (C, D) of the Galaxy. The results derived from the observational data of proper motions and radial velocities of a subgroup of 117 thin disk young open clusters by means of a maximum likelihood algorithm are: (u1,u2,u3) = (-16.1 ± 1.0,-7.9 ±1.4,-10.4±1.5) km·s^-1, (σ1,σ2,σ3) = (17.0±0.7, 12.2±0.9, 8.0±1.3) km·S^-1, (A, B) = (14.8±1.0, - 13.0±2.7) km·s^-1 kpc^-1, and (C, D) = (1.5 ± 0.7, -1.2 ±1.5) km·s^-1 kpc^-1. A discussion on the results and comparisons with what was obtained by other authors is given.展开更多
Shared nothing spatial database cluster system provides high availability since a replicated node can continue service even if any node in cluster system was crashed. However if the failed node wouldn’t be recovered ...Shared nothing spatial database cluster system provides high availability since a replicated node can continue service even if any node in cluster system was crashed. However if the failed node wouldn’t be recovered quickly, whole system performance will decrease since the other nodes must process the queries which the failed node may be processed. Therefore the recovery of cluster system is very important to provide the stable service. In most previous proposed techniques, external logs should be recorded in all nodes even if the failed node does not exist. So update transactions are processed slowly. Also recovery time of the failed node increases since a single storage for all database is used to record external logs in each node. Therefore we propose a parallel recovery method for recovering the failed node quickly.展开更多
In this study,the effects of laser fields that can be achieved in the near future on cluster penetration probability and half-life are quantitatively investigated.The calculation results show that extreme laser fields...In this study,the effects of laser fields that can be achieved in the near future on cluster penetration probability and half-life are quantitatively investigated.The calculation results show that extreme laser fields can slightly change the cluster-decay half-life by affecting the penetration probability within a narrow range.Subsequently,we discuss the correlation between the change rate of the penetration probability and the tunneling path.The results indicate that for different parent nuclei emitting the same cluster,nuclei with longer tunneling paths are more easily affected by the laser fields.The shell effect on this correlation is also observed.In addition,the impact of laser fields on the penetration probability in any direction is investigated.展开更多
Various factors,including weak tie-lines into the electric power system(EPS)networks,can lead to low-frequency oscillations(LFOs),which are considered an instant,non-threatening situation,but slow-acting and poisonous...Various factors,including weak tie-lines into the electric power system(EPS)networks,can lead to low-frequency oscillations(LFOs),which are considered an instant,non-threatening situation,but slow-acting and poisonous.Considering the challenge mentioned,this article proposes a clustering-based machine learning(ML)framework to enhance the stability of EPS networks by suppressing LFOs through real-time tuning of key power system stabilizer(PSS)parameters.To validate the proposed strategy,two distinct EPS networks are selected:the single-machine infinite-bus(SMIB)with a single-stage PSS and the unified power flow controller(UPFC)coordinated SMIB with a double-stage PSS.To generate data under various loading conditions for both networks,an efficient but offline meta-heuristic algorithm,namely the grey wolf optimizer(GWO),is used,with the loading conditions as inputs and the key PSS parameters as outputs.The generated loading conditions are then clustered using the fuzzy k-means(FKM)clustering method.Finally,the group method of data handling(GMDH)and long short-term memory(LSTM)ML models are developed for clustered data to predict PSS key parameters in real time for any loading condition.A few well-known statistical performance indices(SPI)are considered for validation and robustness of the training and testing procedure of the developed FKM-GMDH and FKM-LSTM models based on the prediction of PSS parameters.The performance of the ML models is also evaluated using three stability indices(i.e.,minimum damping ratio,eigenvalues,and time-domain simulations)after optimally tuned PSS with real-time estimated parameters under changing operating conditions.Besides,the outputs of the offline(GWO-based)metaheuristic model,proposed real-time(FKM-GMDH and FKM-LSTM)machine learning models,and previously reported literature models are compared.According to the results,the proposed methodology outperforms the others in enhancing the stability of the selected EPS networks by damping out the observed unwanted LFOs under various loading conditions.展开更多
For multi-vehicle networks,Cooperative Positioning(CP)technique has become a promising way to enhance vehicle positioning accuracy.Especially,the CP performance could be further improved by introducing Sensor-Rich Veh...For multi-vehicle networks,Cooperative Positioning(CP)technique has become a promising way to enhance vehicle positioning accuracy.Especially,the CP performance could be further improved by introducing Sensor-Rich Vehicles(SRVs)into CP networks,which is called SRV-aided CP.However,the CP system may split into several sub-clusters that cannot be connected with each other in dense urban environments,in which the sub-clusters with few SRVs will suffer from degradation of CP performance.Since Unmanned Aerial Vehicles(UAVs)have been widely used to aid vehicular communications,we intend to utilize UAVs to assist sub-clusters in CP.In this paper,a UAV-aided CP network is constructed to fully utilize information from SRVs.First,the inter-node connection structure among the UAV and vehicles is designed to share available information from SRVs.After that,the clustering optimization strategy is proposed,in which the UAV cooperates with the high-precision sub-cluster to obtain available information from SRVs,and then broadcasts this positioning-related information to other low-precision sub-clusters.Finally,the Locally-Centralized Factor Graph Optimization(LC-FGO)algorithm is designed to fuse positioning information from cooperators.Simulation results indicate that the positioning accuracy of the CP system could be improved by fully utilizing positioning-related information from SRVs.展开更多
Noncohesive particle clusters are identified and tracked in turbulent flows to determine the breakdown and time evolution of cluster statistics and their implications for interscale mass transfer,which has connections...Noncohesive particle clusters are identified and tracked in turbulent flows to determine the breakdown and time evolution of cluster statistics and their implications for interscale mass transfer,which has connections to the classical turbulent energy cascade and its mass cascade counterpart running in parallel.In particular,the formation and dynamics of sediment and larvae clusters are of interest to coral larvae settlement in coastal regions and particularly the resilience of green-gray coastal protection solutions.Analogous cluster behavior is relevant to cloud microphysics and precipitation initiation,radiation transport and light transmission through colloids and suspensions,heat and mass transfer in particle-laden flows,and viral and pollutant transmission.Following a comparison between various clustering techniques,we adopt a density-based cluster identification algorithm based on its simplicity and efficiency,where particles are clustered based on the number of neighboring particles in their individual spheres of influence.We establish parallels with lattice-based percolation theory,as evident in the power-law scaling of the cluster size distribution near the percolation threshold.The degree of discontinuity of the phase transition associated with this percolation threshold is observed to broaden with larger Stokes numbers and thereby large-scale clustering.The sensitivity of our findings to the employed clustering algorithm is discussed.A novel cluster tracking algorithm is deployed to determine the interscale transfer rate along the particle-number phase-space dimension via accounting of cluster breakup and merger events,extending previous work on the bubble breakup cascade beneath surface breaking waves.Our findings shed light on the interaction between particle clusters and their carrier turbulent flows,with an eye toward transport models incorporating cluster characteristics and dynamics.展开更多
Biomass is a renewable energy source helps reduce greenhouse gas emissions.However,combustion and reaction efficiency of biomass are significantly affected by their flow behavior.In this study,the flow characteristics...Biomass is a renewable energy source helps reduce greenhouse gas emissions.However,combustion and reaction efficiency of biomass are significantly affected by their flow behavior.In this study,the flow characteristics of wet elongated biomass particles in a lifting tube were experimentally investigated.Particle Tracking Velocimetry(PTV)was used to explore the particle area and velocity distribution under different gas-to-particle mass ratios(GPMR)and initial moisture contents(IMC).A homogeneity coefficient was also formulated to quantify the flow homogeneity of the particle population.The calculated range for the homogeneity coefficientαis 4.43-6.40,with smaller values indicating better flow homogeneity.Moreover,the factors affecting the fragmentation of larger particle clusters were analyzed with respect to the suspension process,the process of being carried out by the airflow,and the fragmentation process.The results indicated that the flow homogeneity of the particle population was better in the two sets of conditions when IMC was 28.7% and GPMR was 10 and when IMC was 32.5% and GPMR was 9.The homogeneity coefficient α was 4.43 and 4.79.In addition,the degree of fragmentation of larger particle clusters is mainly affected by the IMC.展开更多
Music recommendation systems are essential due to the vast amount of music available on streaming platforms,which can overwhelm users trying to find new tracks that match their preferences.These systems analyze users...Music recommendation systems are essential due to the vast amount of music available on streaming platforms,which can overwhelm users trying to find new tracks that match their preferences.These systems analyze users’emotional responses,listening habits,and personal preferences to provide personalized suggestions.A significant challenge they face is the“cold start”problem,where new users have no past interactions to guide recommendations.To improve user experience,these systems aimto effectively recommendmusic even to such users by considering their listening behavior and music popularity.This paper introduces a novel music recommendation system that combines order clustering and a convolutional neural network,utilizing user comments and rankings as input.Initially,the system organizes users into clusters based on semantic similarity,followed by the utilization of their rating similarities as input for the convolutional neural network.This network then predicts ratings for unreviewed music by users.Additionally,the system analyses user music listening behaviour and music popularity.Music popularity can help to address cold start users as well.Finally,the proposed method recommends unreviewed music based on predicted high rankings and popularity,taking into account each user’s music listening habits.The proposed method combines predicted high rankings and popularity by first selecting popular unreviewedmusic that themodel predicts to have the highest ratings for each user.Among these,the most popular tracks are prioritized,defined by metrics such as frequency of listening across users.The number of recommended tracks is aligned with each user’s typical listening rate.The experimental findings demonstrate that the new method outperformed other classification techniques and prior recommendation systems,yielding a mean absolute error(MAE)rate and rootmean square error(RMSE)rate of approximately 0.0017,a hit rate of 82.45%,an average normalized discounted cumulative gain(nDCG)of 82.3%,and a prediction accuracy of new ratings at 99.388%.展开更多
Transient stability assessment(TSA)based on artificial intelligence typically has two distinct model management approaches:a unified management approach for all faulted lines and a separate management approach for eac...Transient stability assessment(TSA)based on artificial intelligence typically has two distinct model management approaches:a unified management approach for all faulted lines and a separate management approach for each faulted line.To address the shortcomings of the aforementioned approaches,namely accuracy,training time,and model management complexity,a multi-model management approach for power system TSA based on multi-moment feature clustering has been proposed.First,the steady-state and transient features present under fault conditions were obtained through a transient simulation of line faults.The input sample set was then constructed using the aforementioned multi-moment electrical features and the embedded faulty line numbers.Subsequently,K-means clustering was conducted on each line based on the similarity of their electrical features,employing t-SNE dimensionality reduction.The PSO-CNN model was trained separately for each cluster to generate several independent TSA models.Finally,a model effectiveness evaluation system consisting of five metrics was established,and the effect of the sample imbalance ratio on the model effectiveness was investigated.The model effectiveness was evaluated using the IEEE 39-bus system algorithm.The results showed that the multi-model management strategy based on multi-moment feature clustering can effectively combine the two advantages of superior evaluation performance and streamlined model management by fully extracting system features.Moreover,this approach allows for more flexible adjustments to line topology changes.展开更多
With the continuous expansion of the power system scale and the increasing complexity of operational mode,the interaction between transmission and distribution systems is becoming more and more significant,placing hig...With the continuous expansion of the power system scale and the increasing complexity of operational mode,the interaction between transmission and distribution systems is becoming more and more significant,placing higher requirements on the accuracy and efficiency of the power system state estimation to address the challenge of balancing computational efficiency and estimation accuracy in traditional coupled transmission and distribution state estimation methods,this paper proposes a collaborative state estimation method based on distribution systems state clustering and load model parameter identification.To resolve the scalability issue of coupled transmission and distribution power systems,clustering is first carried out based on the distribution system states.As the data and models of the transmission system and distribution systems are not shared.For the transmission system,equating the power transmitted from the transmission system to the distribution system is the same as equating the distribution system.Further,the power transmitted from the transmission system to different types of distribution systems is equivalent to different polynomial equivalent load models.Then,a parameter identification method is proposed to obtain the parameters of the equivalent load model.Finally,a transmission and distribution collaborative state estimation model is constructed based on the equivalent load model.The results of the numerical analysis show that compared with the traditional master-slave splitting method,the proposed method significantly enhances computational efficiency while maintaining high estimation accuracy.展开更多
The distillation process is an important chemical process,and the application of data-driven modelling approach has the potential to reduce model complexity compared to mechanistic modelling,thus improving the efficie...The distillation process is an important chemical process,and the application of data-driven modelling approach has the potential to reduce model complexity compared to mechanistic modelling,thus improving the efficiency of process optimization or monitoring studies.However,the distillation process is highly nonlinear and has multiple uncertainty perturbation intervals,which brings challenges to accurate data-driven modelling of distillation processes.This paper proposes a systematic data-driven modelling framework to solve these problems.Firstly,data segment variance was introduced into the K-means algorithm to form K-means data interval(KMDI)clustering in order to cluster the data into perturbed and steady state intervals for steady-state data extraction.Secondly,maximal information coefficient(MIC)was employed to calculate the nonlinear correlation between variables for removing redundant features.Finally,extreme gradient boosting(XGBoost)was integrated as the basic learner into adaptive boosting(AdaBoost)with the error threshold(ET)set to improve weights update strategy to construct the new integrated learning algorithm,XGBoost-AdaBoost-ET.The superiority of the proposed framework is verified by applying this data-driven modelling framework to a real industrial process of propylene distillation.展开更多
Under hydrothermal and solvothermal conditions,two novel cobalt-based complexes,{[Co_(2)(CIA)(OH)(1,4-dtb)]·3.2H_(2)O}n(HU23)and{[Co_(2)(CIA)(OH)(1,4-dib)]·3.5H2O·DMF}n(HU24),were successfully construct...Under hydrothermal and solvothermal conditions,two novel cobalt-based complexes,{[Co_(2)(CIA)(OH)(1,4-dtb)]·3.2H_(2)O}n(HU23)and{[Co_(2)(CIA)(OH)(1,4-dib)]·3.5H2O·DMF}n(HU24),were successfully constructed by coordinatively assembling the semi-rigid multidentate ligand 5-(1-carboxyethoxy)isophthalic acid(H₃CIA)with the Nheterocyclic ligands 1,4-di(4H-1,2,4-triazol-4-yl)benzene(1,4-dtb)and 1,4-di(1H-imidazol-1-yl)benzene(1,4-dib),respectively,around Co^(2+)ions.Single-crystal X-ray diffraction analysis revealed that in both complexes HU23 and HU24,the CIA^(3-)anions adopt aκ^(7)-coordination mode,bridging six Co^(2+)ions via their five carboxylate oxygen atoms and one ether oxygen atom.This linkage forms tetranuclear[Co4(μ3-OH)2]^(6+)units.These Co-oxo cluster units were interconnected by CIA^(3-)anions to assemble into 2D kgd-type structures featuring a 3,6-connected topology.The 2D layers were further connected by 1,4-dtb and 1,4-dib,resulting in 3D pillar-layered frameworks for HU23 and HU24.Notably,despite the similar configurations of 1,4-dtb and 1,4-dib,differences in their coordination spatial orientations lead to topological divergence in the 3D frameworks of HU23 and HU24.Topological analysis indicates that the frameworks of HU23 and HU24 can be simplified into a 3,10-connected net(point symbol:(4^(10).6^(3).8^(2))(4^(3))_(2))and a 3,8-connected tfz-d net(point symbol:(4^(3))_(2)((4^(6).6^(18).8^(4)))),respectively.This structural differentiation confirms the precise regulatory role of ligands on the topology of metal-organic frameworks.Moreover,the ultraviolet-visible absorption spectra confirmed that HU23 and HU24 have strong absorption capabilities for ultraviolet and visible light.According to the Kubelka-Munk method,their bandwidths were 2.15 and 2.08 eV,respectively,which are consistent with those of typical semiconductor materials.Variable-temperature magnetic susceptibility measurements(2-300 K)revealed significant antiferromagnetic coupling in both complexes,with their effective magnetic moments decreasing markedly as the temperature lowered.CCDC:2457554,HU23;2457553,HU24.展开更多
基金supported by the National Natural Science Foundationof China (60701006 60804054 71071158)
文摘Failure prediction plays an important role for many tasks such as optimal resource management in large-scale system. However, accurately failure number prediction of repairable large-scale long-running computing (RLLC) is a challenge because of the reparability and large-scale. To address the challenge, a general Bayesian serial revision prediction method based on Bootstrap approach and moving average approach is put forward, which can make an accurately prediction for the failure number. To demonstrate the performance gains of our method, extensive experiments on the data of Los Alamos National Laboratory (LANL) cluster is implemented, which is a typical RLLC system. And experimental results show that the prediction accuracy of our method is 80.2 %, and it is a greatly improvement with 4 % compared with some typical methods. Finally, the managerial implications of the models are discussed.
基金Supported by the National Natural Science Foundation of China(No.2 0 0 730 34,2 0 3730 5 6,2 0 1710 37),Fujian Provinceand Technology Comm ission(No.2 0 0 2 F0 16 ) and Xiamen Science and Technology Com mission(No.35 0 2 Z2 0 0 2 10 4 4 )
文摘The efficient chiral Ru 3(CO) 12 systems were prepared in situ from Ru 3(CO) 12 and various chiral diimino-or diamino-diphosphine tetradentate ligands. The systems have been used for the asymmetric transfer hydrogenation of propiophenone in 2-propanol, leading to 1-phenyl-1-propanol in a 98% yield and 96% e.e. The IR study suggests that the carbonyl hydride anion [HRu 3(CO) 11]- most probably exists as a principal species under the reaction conditions. The high chiral efficiency may be due to the synergetic effect produced by the neighboring ruthenium atoms and a special chiral micro-environment involving the polydentate ligand and the Ru 3 framework.
文摘The percolation fields constructed around the elements of a cluster system in the phase spaces of properties are studied.It is shown that such neighborhoods significantly increase the number of structure parameters of the system under study,expanding the possibilities of analytical description.To study the structure and properties of such systems in the proposed model,a three-dimensional continuum percolation problem with interacting elements is solved.The dependences of the structure and properties of clusters on the parameters of the generation processes of the cluster system are studied,and analytical dependences are obtained.
基金Supported by National Natural Science Foundation of China (No. 20676094)
文摘The influence of water on protein conformation was investigated by simulating the molecular dynamics of a model protein lysozyme in different water systems.The lysozyme-water system with TIP3P water model and lysozyme-water cluster system with six-ring water model were evaluated.In addition,the radial distribution function of solvent around lysozyme was calculated.It is found that the distribution of water molecules around lysozyme is similar to that of water clusters.The analyses of dihedral angles and disulfide bonds of lysozyme show that the conformation of lysozyme is severely damaged in the lysozyme-water cluster system compared with that in the lysozyme-water system.This difference can be attributed to the formation of larger number of intermolecular hydrogen bonds between lysozyme and water cluster.It is in agreement with the analysis that water clusters can change the degree of denaturation in the process of heat denaturation of lysozyme.
基金The National Natural Science Foundation of China(No.61402333,61402242)the National Science Foundation of Tianjin(No.15JCQNJC00400)
文摘An approach for web server cluster(WSC)reliability and degradation process analysis is proposed.The reliability process is modeled as a non-homogeneous Markov process(NHMH)composed of several non-homogeneous Poisson processes(NHPPs).The arrival rate of each NHPP corresponds to the system software failure rate which is expressed using Cox s proportional hazards model(PHM)in terms of the cumulative and instantaneous load of the software.The cumulative load refers to software cumulative execution time,and the instantaneous load denotes the rate that the users requests arrive at a server.The result of reliability analysis is a time-varying reliability and degradation process over the WSC lifetime.Finally,the evaluation experiment shows the effectiveness of the proposed approach.
基金financially supported by the National Natural Science Foundation of China(No.21973088)Shenzhen Science and Technology Program(Nos.RCYX20210706092101012 and ZDSYS20210623100800001)。
文摘This work reports the structural feature and internal motion of one novel hyperbranching cluster system in dilution solution.The cluster system is composed of HB-PS_(300)-g-Pt BA_(45) hypergraft copolymer chains with uniform subchain,high molar mass and low polydispersity(M_(w)=1.73×106 g/mol and<M_(w)/M_(n)>≈1.07),where HB-PS and Pt BA represent hyperbranched polystyrene core and poly(tert-butyl polyacrylate)graft,respectively.In the selective solvent of PS blocks(cyclohexane,T_(θ)=34.5℃),the aggregation kinetics and structural feature are found to be precisely tunable for assembled clusters by the aggregation temperature(11℃<T<17℃)and time(0 h<t<24 h).An interesting structural evolution kinetics is observed,namely,the fractal dimension(d_(f))of clusters is found to first increases and then decreases with t,eventually,it reaches a plateau value of d_(f)≈3.0,corresponds to a uniform spherical structure.By using dynamic light scattering(DLS)to monitor the number and strength of relaxation modes inΓ(q)withΓbeing the decay rate and q being the scattering vector,it is quantitatively revealed that the relaxation,intensity contribution and mode origin of internal motions of clusters are neither similar with previously reported cluster systems with high polydispersity,nor with the classical linear chain systems.In particular,in the broad range of 2.0<qR_(h)<6.0,we have observed that the reduced first cumulant[Γ^(*)=Γ(q)/(q^(3)k_(B)T/η_(0))]does not display an asymptotic behavior.Whereas,a better asymptotic behavior is observed by plottingΓ(q)/q^(4) versus qRh.For the first time,our observation provides direct evidence supporting that,for hyperbranching cluster system with low polydispersity and high local chain segment density,the hydrodynamic interaction is greatly weakened due to the enhanced hydrodynamic shielding effect.
基金supported by the National Natural Science Foundation of China (Grant Nos. 10873016, 10633020, 10803007,11003021, 11173016 and 11073032)the National Basic Research Program of China (973 Program, 2007CB815403)
文摘We present metal abundance properties of 144 globular clusters associated with M81. These globulars represent the largest globular cluster sample in M81 till now. Our main results are: the distribution of metallicities is bimodal, with metallicity peaks at [Fe/H] -1.51 and -0.58, and the metal-poor globular clusters tend to be less spatially concentrated than the metal-rich ones; the metal-rich globular clusters in M81 do not demonstrate a centrally concentrated spatial distribution like the metalrich ones in M31 do; like our Galaxy and M31, the globular clusters in M81 have a small radial metallicity gradient. These results are consistent with those obtained from a small sample of M81 globular clusters. In addition, this paper shows that there is evidence that a strong rotation of the M81 globular cluster system around the minor axis exists, and that rotation is present in the metal-rich globular cluster subsample, but the metal-poor globular cluster subsample shows no evidence of rotation. The most significant difference between the rotation of the metal-rich and metal-poor globular clusters occurs at intermediate projected galactocentric radii. Our results confirm the conclusion of Schroder et al. that M81's metal-rich globular clusters at intermediate projected radii are associated with a thick disk of M81.
文摘A significant portion of Landslide Early Warning Systems (LEWS) relies on the definition of operational thresholds and the monitoring of cumulative rainfall for alert issuance. These thresholds can be obtained in various ways, but most often they are based on previous landslide data. This approach introduces several limitations. For instance, there is a requirement for the location to have been previously monitored in some way to have this type of information recorded. Another significant limitation is the need for information regarding the location and timing of incidents. Despite the current ease of obtaining location information (GPS, drone images, etc.), the timing of the event remains challenging to ascertain for a considerable portion of landslide data. Concerning rainfall monitoring, there are multiple ways to consider it, for instance, examining accumulations over various intervals (1 h, 6 h, 24 h, 72 h), as well as in the calculation of effective rainfall, which represents the precipitation that actually infiltrates the soil. However, in the vast majority of cases, both the thresholds and the rain monitoring approach are defined manually and subjectively, relying on the operators’ experience. This makes the process labor-intensive and time-consuming, hindering the establishment of a truly standardized and rapidly scalable methodology on a large scale. In this work, we propose a Landslides Early Warning System (LEWS) based on the concept of rainfall half-life and the determination of thresholds using Cluster Analysis and data inversion. The system is designed to be applied in extensive monitoring networks, such as the one utilized by Cemaden, Brazil’s National Center for Monitoring and Early Warning of Natural Disasters.
基金Supported by the National Natural Science Foundation of China.
文摘Absolute proper motions and radial velocities of 202 open clusters in the solar neighborhood, which can be used as tracers of the Galactic disk, are used to investigate the kinematics of the Galaxy in the solar vicinity, including the mean heliocentric velocity components (u1, u2, u3) of the open cluster system, the characteristic velocity dispersions (σ1,σ2,σ3), Oort constants (A, B) and the large-scale radial motion parameters (C, D) of the Galaxy. The results derived from the observational data of proper motions and radial velocities of a subgroup of 117 thin disk young open clusters by means of a maximum likelihood algorithm are: (u1,u2,u3) = (-16.1 ± 1.0,-7.9 ±1.4,-10.4±1.5) km·s^-1, (σ1,σ2,σ3) = (17.0±0.7, 12.2±0.9, 8.0±1.3) km·S^-1, (A, B) = (14.8±1.0, - 13.0±2.7) km·s^-1 kpc^-1, and (C, D) = (1.5 ± 0.7, -1.2 ±1.5) km·s^-1 kpc^-1. A discussion on the results and comparisons with what was obtained by other authors is given.
基金This work is supported by University IT Research Center Project
文摘Shared nothing spatial database cluster system provides high availability since a replicated node can continue service even if any node in cluster system was crashed. However if the failed node wouldn’t be recovered quickly, whole system performance will decrease since the other nodes must process the queries which the failed node may be processed. Therefore the recovery of cluster system is very important to provide the stable service. In most previous proposed techniques, external logs should be recorded in all nodes even if the failed node does not exist. So update transactions are processed slowly. Also recovery time of the failed node increases since a single storage for all database is used to record external logs in each node. Therefore we propose a parallel recovery method for recovering the failed node quickly.
基金supported in part by the National Natural Science Foundation of China(Nos.12175100 and 11975132)the Construct Program of the Key Discipline in Hunan Province+5 种基金the Research Foundation of Education Bureau of Hunan Province,China(Nos.21B0402,18A237,22A0305)the Natural Science Foundation of Hunan Province,China(No.2018JJ2321)the Innovation Group of Nuclear and Particle Physics in USCthe Shandong Province Natural Science Foundation,China(No.ZR2022JQ04)the Opening Project of Cooperative Innovation Center for Nuclear Fuel Cycle Technology and Equipment,University of South China(No.2019KFZ10)the Hunan Provincial Innovation Foundation for Postgraduate(No.CX20251453)。
文摘In this study,the effects of laser fields that can be achieved in the near future on cluster penetration probability and half-life are quantitatively investigated.The calculation results show that extreme laser fields can slightly change the cluster-decay half-life by affecting the penetration probability within a narrow range.Subsequently,we discuss the correlation between the change rate of the penetration probability and the tunneling path.The results indicate that for different parent nuclei emitting the same cluster,nuclei with longer tunneling paths are more easily affected by the laser fields.The shell effect on this correlation is also observed.In addition,the impact of laser fields on the penetration probability in any direction is investigated.
基金supported by the Deanship of Research at the King Fahd University of Petroleum&Minerals,Dhahran,31261,Saudi Arabia,under Project No.EC241001.
文摘Various factors,including weak tie-lines into the electric power system(EPS)networks,can lead to low-frequency oscillations(LFOs),which are considered an instant,non-threatening situation,but slow-acting and poisonous.Considering the challenge mentioned,this article proposes a clustering-based machine learning(ML)framework to enhance the stability of EPS networks by suppressing LFOs through real-time tuning of key power system stabilizer(PSS)parameters.To validate the proposed strategy,two distinct EPS networks are selected:the single-machine infinite-bus(SMIB)with a single-stage PSS and the unified power flow controller(UPFC)coordinated SMIB with a double-stage PSS.To generate data under various loading conditions for both networks,an efficient but offline meta-heuristic algorithm,namely the grey wolf optimizer(GWO),is used,with the loading conditions as inputs and the key PSS parameters as outputs.The generated loading conditions are then clustered using the fuzzy k-means(FKM)clustering method.Finally,the group method of data handling(GMDH)and long short-term memory(LSTM)ML models are developed for clustered data to predict PSS key parameters in real time for any loading condition.A few well-known statistical performance indices(SPI)are considered for validation and robustness of the training and testing procedure of the developed FKM-GMDH and FKM-LSTM models based on the prediction of PSS parameters.The performance of the ML models is also evaluated using three stability indices(i.e.,minimum damping ratio,eigenvalues,and time-domain simulations)after optimally tuned PSS with real-time estimated parameters under changing operating conditions.Besides,the outputs of the offline(GWO-based)metaheuristic model,proposed real-time(FKM-GMDH and FKM-LSTM)machine learning models,and previously reported literature models are compared.According to the results,the proposed methodology outperforms the others in enhancing the stability of the selected EPS networks by damping out the observed unwanted LFOs under various loading conditions.
基金supported by the National Natural Science Foundation of China(No.62271399)the National Key Research and Development Program of China(No.2022YFB1807102)。
文摘For multi-vehicle networks,Cooperative Positioning(CP)technique has become a promising way to enhance vehicle positioning accuracy.Especially,the CP performance could be further improved by introducing Sensor-Rich Vehicles(SRVs)into CP networks,which is called SRV-aided CP.However,the CP system may split into several sub-clusters that cannot be connected with each other in dense urban environments,in which the sub-clusters with few SRVs will suffer from degradation of CP performance.Since Unmanned Aerial Vehicles(UAVs)have been widely used to aid vehicular communications,we intend to utilize UAVs to assist sub-clusters in CP.In this paper,a UAV-aided CP network is constructed to fully utilize information from SRVs.First,the inter-node connection structure among the UAV and vehicles is designed to share available information from SRVs.After that,the clustering optimization strategy is proposed,in which the UAV cooperates with the high-precision sub-cluster to obtain available information from SRVs,and then broadcasts this positioning-related information to other low-precision sub-clusters.Finally,the Locally-Centralized Factor Graph Optimization(LC-FGO)algorithm is designed to fuse positioning information from cooperators.Simulation results indicate that the positioning accuracy of the CP system could be improved by fully utilizing positioning-related information from SRVs.
文摘Noncohesive particle clusters are identified and tracked in turbulent flows to determine the breakdown and time evolution of cluster statistics and their implications for interscale mass transfer,which has connections to the classical turbulent energy cascade and its mass cascade counterpart running in parallel.In particular,the formation and dynamics of sediment and larvae clusters are of interest to coral larvae settlement in coastal regions and particularly the resilience of green-gray coastal protection solutions.Analogous cluster behavior is relevant to cloud microphysics and precipitation initiation,radiation transport and light transmission through colloids and suspensions,heat and mass transfer in particle-laden flows,and viral and pollutant transmission.Following a comparison between various clustering techniques,we adopt a density-based cluster identification algorithm based on its simplicity and efficiency,where particles are clustered based on the number of neighboring particles in their individual spheres of influence.We establish parallels with lattice-based percolation theory,as evident in the power-law scaling of the cluster size distribution near the percolation threshold.The degree of discontinuity of the phase transition associated with this percolation threshold is observed to broaden with larger Stokes numbers and thereby large-scale clustering.The sensitivity of our findings to the employed clustering algorithm is discussed.A novel cluster tracking algorithm is deployed to determine the interscale transfer rate along the particle-number phase-space dimension via accounting of cluster breakup and merger events,extending previous work on the bubble breakup cascade beneath surface breaking waves.Our findings shed light on the interaction between particle clusters and their carrier turbulent flows,with an eye toward transport models incorporating cluster characteristics and dynamics.
基金thefinancial support of the National Natural Science Foundation of China(grant No.51906092)Postgraduate Research&Practice Innovation Program of Jiangsu Province(grant No.SJCX23_2219).
文摘Biomass is a renewable energy source helps reduce greenhouse gas emissions.However,combustion and reaction efficiency of biomass are significantly affected by their flow behavior.In this study,the flow characteristics of wet elongated biomass particles in a lifting tube were experimentally investigated.Particle Tracking Velocimetry(PTV)was used to explore the particle area and velocity distribution under different gas-to-particle mass ratios(GPMR)and initial moisture contents(IMC).A homogeneity coefficient was also formulated to quantify the flow homogeneity of the particle population.The calculated range for the homogeneity coefficientαis 4.43-6.40,with smaller values indicating better flow homogeneity.Moreover,the factors affecting the fragmentation of larger particle clusters were analyzed with respect to the suspension process,the process of being carried out by the airflow,and the fragmentation process.The results indicated that the flow homogeneity of the particle population was better in the two sets of conditions when IMC was 28.7% and GPMR was 10 and when IMC was 32.5% and GPMR was 9.The homogeneity coefficient α was 4.43 and 4.79.In addition,the degree of fragmentation of larger particle clusters is mainly affected by the IMC.
基金funded by the National Nature Sciences Foundation of China with Grant No.42250410321。
文摘Music recommendation systems are essential due to the vast amount of music available on streaming platforms,which can overwhelm users trying to find new tracks that match their preferences.These systems analyze users’emotional responses,listening habits,and personal preferences to provide personalized suggestions.A significant challenge they face is the“cold start”problem,where new users have no past interactions to guide recommendations.To improve user experience,these systems aimto effectively recommendmusic even to such users by considering their listening behavior and music popularity.This paper introduces a novel music recommendation system that combines order clustering and a convolutional neural network,utilizing user comments and rankings as input.Initially,the system organizes users into clusters based on semantic similarity,followed by the utilization of their rating similarities as input for the convolutional neural network.This network then predicts ratings for unreviewed music by users.Additionally,the system analyses user music listening behaviour and music popularity.Music popularity can help to address cold start users as well.Finally,the proposed method recommends unreviewed music based on predicted high rankings and popularity,taking into account each user’s music listening habits.The proposed method combines predicted high rankings and popularity by first selecting popular unreviewedmusic that themodel predicts to have the highest ratings for each user.Among these,the most popular tracks are prioritized,defined by metrics such as frequency of listening across users.The number of recommended tracks is aligned with each user’s typical listening rate.The experimental findings demonstrate that the new method outperformed other classification techniques and prior recommendation systems,yielding a mean absolute error(MAE)rate and rootmean square error(RMSE)rate of approximately 0.0017,a hit rate of 82.45%,an average normalized discounted cumulative gain(nDCG)of 82.3%,and a prediction accuracy of new ratings at 99.388%.
基金supported by the Science and Technology Project of SGCC(5100-202199558A-0-5-ZN).
文摘Transient stability assessment(TSA)based on artificial intelligence typically has two distinct model management approaches:a unified management approach for all faulted lines and a separate management approach for each faulted line.To address the shortcomings of the aforementioned approaches,namely accuracy,training time,and model management complexity,a multi-model management approach for power system TSA based on multi-moment feature clustering has been proposed.First,the steady-state and transient features present under fault conditions were obtained through a transient simulation of line faults.The input sample set was then constructed using the aforementioned multi-moment electrical features and the embedded faulty line numbers.Subsequently,K-means clustering was conducted on each line based on the similarity of their electrical features,employing t-SNE dimensionality reduction.The PSO-CNN model was trained separately for each cluster to generate several independent TSA models.Finally,a model effectiveness evaluation system consisting of five metrics was established,and the effect of the sample imbalance ratio on the model effectiveness was investigated.The model effectiveness was evaluated using the IEEE 39-bus system algorithm.The results showed that the multi-model management strategy based on multi-moment feature clustering can effectively combine the two advantages of superior evaluation performance and streamlined model management by fully extracting system features.Moreover,this approach allows for more flexible adjustments to line topology changes.
基金State Grid Jiangsu Electric Power Co.,Ltd.Technology Project(J2023121).
文摘With the continuous expansion of the power system scale and the increasing complexity of operational mode,the interaction between transmission and distribution systems is becoming more and more significant,placing higher requirements on the accuracy and efficiency of the power system state estimation to address the challenge of balancing computational efficiency and estimation accuracy in traditional coupled transmission and distribution state estimation methods,this paper proposes a collaborative state estimation method based on distribution systems state clustering and load model parameter identification.To resolve the scalability issue of coupled transmission and distribution power systems,clustering is first carried out based on the distribution system states.As the data and models of the transmission system and distribution systems are not shared.For the transmission system,equating the power transmitted from the transmission system to the distribution system is the same as equating the distribution system.Further,the power transmitted from the transmission system to different types of distribution systems is equivalent to different polynomial equivalent load models.Then,a parameter identification method is proposed to obtain the parameters of the equivalent load model.Finally,a transmission and distribution collaborative state estimation model is constructed based on the equivalent load model.The results of the numerical analysis show that compared with the traditional master-slave splitting method,the proposed method significantly enhances computational efficiency while maintaining high estimation accuracy.
基金supported by the National Key Research and Development Program of China(2023YFB3307801)the National Natural Science Foundation of China(62394343,62373155,62073142)+3 种基金Major Science and Technology Project of Xinjiang(No.2022A01006-4)the Programme of Introducing Talents of Discipline to Universities(the 111 Project)under Grant B17017the Fundamental Research Funds for the Central Universities,Science Foundation of China University of Petroleum,Beijing(No.2462024YJRC011)the Open Research Project of the State Key Laboratory of Industrial Control Technology,China(Grant No.ICT2024B70).
文摘The distillation process is an important chemical process,and the application of data-driven modelling approach has the potential to reduce model complexity compared to mechanistic modelling,thus improving the efficiency of process optimization or monitoring studies.However,the distillation process is highly nonlinear and has multiple uncertainty perturbation intervals,which brings challenges to accurate data-driven modelling of distillation processes.This paper proposes a systematic data-driven modelling framework to solve these problems.Firstly,data segment variance was introduced into the K-means algorithm to form K-means data interval(KMDI)clustering in order to cluster the data into perturbed and steady state intervals for steady-state data extraction.Secondly,maximal information coefficient(MIC)was employed to calculate the nonlinear correlation between variables for removing redundant features.Finally,extreme gradient boosting(XGBoost)was integrated as the basic learner into adaptive boosting(AdaBoost)with the error threshold(ET)set to improve weights update strategy to construct the new integrated learning algorithm,XGBoost-AdaBoost-ET.The superiority of the proposed framework is verified by applying this data-driven modelling framework to a real industrial process of propylene distillation.
文摘Under hydrothermal and solvothermal conditions,two novel cobalt-based complexes,{[Co_(2)(CIA)(OH)(1,4-dtb)]·3.2H_(2)O}n(HU23)and{[Co_(2)(CIA)(OH)(1,4-dib)]·3.5H2O·DMF}n(HU24),were successfully constructed by coordinatively assembling the semi-rigid multidentate ligand 5-(1-carboxyethoxy)isophthalic acid(H₃CIA)with the Nheterocyclic ligands 1,4-di(4H-1,2,4-triazol-4-yl)benzene(1,4-dtb)and 1,4-di(1H-imidazol-1-yl)benzene(1,4-dib),respectively,around Co^(2+)ions.Single-crystal X-ray diffraction analysis revealed that in both complexes HU23 and HU24,the CIA^(3-)anions adopt aκ^(7)-coordination mode,bridging six Co^(2+)ions via their five carboxylate oxygen atoms and one ether oxygen atom.This linkage forms tetranuclear[Co4(μ3-OH)2]^(6+)units.These Co-oxo cluster units were interconnected by CIA^(3-)anions to assemble into 2D kgd-type structures featuring a 3,6-connected topology.The 2D layers were further connected by 1,4-dtb and 1,4-dib,resulting in 3D pillar-layered frameworks for HU23 and HU24.Notably,despite the similar configurations of 1,4-dtb and 1,4-dib,differences in their coordination spatial orientations lead to topological divergence in the 3D frameworks of HU23 and HU24.Topological analysis indicates that the frameworks of HU23 and HU24 can be simplified into a 3,10-connected net(point symbol:(4^(10).6^(3).8^(2))(4^(3))_(2))and a 3,8-connected tfz-d net(point symbol:(4^(3))_(2)((4^(6).6^(18).8^(4)))),respectively.This structural differentiation confirms the precise regulatory role of ligands on the topology of metal-organic frameworks.Moreover,the ultraviolet-visible absorption spectra confirmed that HU23 and HU24 have strong absorption capabilities for ultraviolet and visible light.According to the Kubelka-Munk method,their bandwidths were 2.15 and 2.08 eV,respectively,which are consistent with those of typical semiconductor materials.Variable-temperature magnetic susceptibility measurements(2-300 K)revealed significant antiferromagnetic coupling in both complexes,with their effective magnetic moments decreasing markedly as the temperature lowered.CCDC:2457554,HU23;2457553,HU24.