In this study, the micro-and macro-physical properties, thermal structure and precipitation characteristics of cyclone eye walls and their surrounding spiral clouds were analysed with Cloud Sat and TRMM data for five ...In this study, the micro-and macro-physical properties, thermal structure and precipitation characteristics of cyclone eye walls and their surrounding spiral clouds were analysed with Cloud Sat and TRMM data for five tropical cyclones(TCs) in 2013. The results show that the ice-phase clouds of a mature TC are mainly above 5 km. With increasing altitude, the cloud droplet effective radius decreases, and the particle number concentration increases. Ice water content first increases and then decreases with increasing height. In the eye area, in addition to the well-known warm-core area, another warm core is also apparent around the eye at a height of 8 to 15 km. The horizontal distribution of precipitation is characterized by large-scale stratiform precipitation mixed with independent convective precipitation. The height of precipitation is mostly below 7.5 km, and the heavy rain is mainly below 5 km. When the peripheral convective clouds are strong enough, ice particles would be generated, thus providing conditions that are favourable for the formation of precipitation below.展开更多
Accurate observation of clouds is challenging because of the high variability and complexity of cloud types and occurrences.By using the long-term cloud data collected during the ARM program at the Southern Great Plai...Accurate observation of clouds is challenging because of the high variability and complexity of cloud types and occurrences.By using the long-term cloud data collected during the ARM program at the Southern Great Plains central facility during 2001-2010,the consistencies and differences in the macrophysical properties of clouds between radiosonde and ground-based active remote sensing are quantitatively evaluated according to six cloud types:low;mid-low(ML);high-midlow;mid;high-mid(HM);and high.A similar variability trend is exhibited by the radiosonde and surface observations for the cloud fractions of the six cloud types.However,the magnitudes of the differences between the two methods are different among the six cloud types,with the largest difference seen in the high clouds.The distribution of the cloud-base height of the ML,mid,and HM clouds agrees in both methods,whereas large differences are seen in the cloud-top height for the ML and high clouds.The cloud thickness variations generally agree between the two datasets for the six cloud types.展开更多
Cloud radiative kernels(CRK)built with radiative transfer models have been widely used to analyze the cloud radiative effect on top of atmosphere(TOA)fluxes,and it is expected that the CRKs would also be useful in the...Cloud radiative kernels(CRK)built with radiative transfer models have been widely used to analyze the cloud radiative effect on top of atmosphere(TOA)fluxes,and it is expected that the CRKs would also be useful in the analyses of surface radiative fluxes,which determines the regional surface temperature change and variability.In this study,CRKs at the surface and TOA were built using the Rapid Radiative Transfer Model(RRTM).Longwave cloud radiative effect(CRE)at the surface is primarily driven by cloud base properties,while TOA CRE is primarily decided by cloud top properties.For this reason,the standard version of surface CRK is a function of latitude,longitude,month,cloud optical thickness(τ)and cloud base pressure(CBP),and the TOA CRK is a function of latitude,longitude,month,τand cloud top pressure(CTP).Considering that the cloud property histograms provided by climate models are functions of CTP instead of CBP at present,the surface CRKs on CBP-τhistograms were converted to CTP-τfields using the statistical relationship between CTP,CBP andτobtained from collocated CloudSat and MODIS observations.For both climate model outputs and satellites observations,the climatology of surface CRE and cloud-induced surface radiative anomalies calculated with the surface CRKs and cloud property histograms are well correlated with those calculated from surface radiative fluxes.The cloud-induced surface radiative anomalies reproduced by surface CRKs and MODIS cloud property histograms are not affected by spurious trends that appear in Clouds and the Earth's Radiant Energy System(CERES)surface irradiances products.展开更多
A coupled meteorology and aerosol/chemistry model WRF-Chem （Weather Research and Forecast model coupled with Chemistry） was used to conduct a pair of simulations with present-day （PD） and preindustrial （P1） emis...A coupled meteorology and aerosol/chemistry model WRF-Chem （Weather Research and Forecast model coupled with Chemistry） was used to conduct a pair of simulations with present-day （PD） and preindustrial （P1） emissions over East Asia to examine the aerosol indirect effect on clouds. As a result of an increase in aerosols in January, the cloud droplet number increased by 650 cm-3 over the ocean and East China, 400 cm-3 over Central and Southwest China, and less than 200 cm-3 over North China. The cloud liquid water path （LWP） increased by 40-60 g m-2 over the ocean and Southeast China and 30 g m-2 over Central China; the LWP in- creased less than 5 g m-2 or decreased by 5 g m2 over North China. The effective radius （Re） decreased by more than 4 pm over Southwest, Central, and Southeast China and 2 pm over North China. In July, variations in cloud properties were more uniform; the cloud droplet number increased by approximately 250400 cm-3, the LWP increased by approximately 30-50 g m 2, and Re decreased by approximately 3 μm over most regions of China. In response to cloud property changes from PI to PD, shortwave （SW） cloud radiative m-2 over the ocean and 10 forcing strengthened by 30 W W m-2 over Southeast China, and it weakened slightly by approximately 2-10 W m-2 over Central and Southwest China in January. In July, SW cloud radiative forcing strengthened by 15 W m-2 over Southeast and North China and weakened by l0 W m-2 over Central China. The different responses of SW cloud radiative forcing in different regions was related to cloud feedbacks and natural variability.展开更多
This study investigates the cloud macro-and micro-physical characteristics in the convective and stratiform regions and their different responses to the seeding for mixed convective-stratiform clouds that occurred in ...This study investigates the cloud macro-and micro-physical characteristics in the convective and stratiform regions and their different responses to the seeding for mixed convective-stratiform clouds that occurred in Shandong province on 21 May 2018,based on the observations from the aircraft,the Suomi National Polar-Orbiting Partnership(NPP)satellite,and the high-resolution Himawari-8(H8)satellite.The aircraft observations show that convection was deeper and radar echoes were significantly enhanced with higher tops in response to seeding in the convective region.This is linked with the conversion of supercooled liquid droplets to ice crystals with released latent heat,resulting in strengthened updrafts,enhanced radar echoes,higher cloud tops,and more and larger precipitation particles.In contrast,in the stratiform cloud region,after the Silver Iodide(AgI)seeding,the radar echoes become significantly weaker at heights close to the seeding layer,with the echo tops lowered by 1.4–1.7 km.In addition,a hollow structure appears at the height of 6.2–7.8 km with a depth of about 1.6 km and a diameter of about 5.5 km,and features such as icing seeding tracks appear.These suggest that the transformation between droplets and ice particles was accelerated by the seeding in the stratiform part.The NPP and H8 satellites also show that convective activity was stronger in the convective region after seeding;while in the stratiform region,a cloud seeding track with a width of 1–3 km appears 10 km downstream of the seeding layer 15 minutes after the AgI seeding,which moves along the wind direction as width increases.展开更多
To investigate the potential effects of aerosols on the microphysical properties of warm clouds, airborne observational data collected from 2009 to 2011 in Tongliao, Inner Mongolia, China, were statistically analyzed ...To investigate the potential effects of aerosols on the microphysical properties of warm clouds, airborne observational data collected from 2009 to 2011 in Tongliao, Inner Mongolia, China, were statistically analyzed in this study. The results demonstrated that the vertical distribution of the aerosol number concentration（N_a） was similar to that of the clean rural continent. The average aerosol effective diameter（D_e） was maintained at approximately 0.4 μm at all levels. The data obtained during cloud penetrations showed that there was a progressive increase in the cloud droplet concentration（N_c） and liquid water content（LWC） from outside to inside the clouds, while the Nawas negatively related to the Ncand LWC at the same height. The fluctuation of the N_a, Ncand LWC during cloud penetration was more obvious under polluted conditions（Type 1） than under clean conditions（Type 2）. Moreover, the wet scavenging of cloud droplets had a significant impact on the accumulation mode of aerosols, especially on particles with diameters less than 0.4 μm. The minimum wet scavenging coefficient within the cloud was close to 0.02 under Type 1 conditions, while it increased to 0.1 under Type 2 conditions,which proved that the cloud wet scavenging effect under Type 1 conditions was stronger than that under Type 2 conditions.Additionally, cloud droplet spectra under Type 1 conditions were narrower, and their horizontal distributions were more homogeneous than those under Type 2 conditions.展开更多
A closed-cell marine stratocumulus case during the Aerosol and Cloud Experiments in the Eastern North Atlantic(ACE-ENA)aircraft field campaign is selected to examine the heterogeneities of cloud and drizzle microphysi...A closed-cell marine stratocumulus case during the Aerosol and Cloud Experiments in the Eastern North Atlantic(ACE-ENA)aircraft field campaign is selected to examine the heterogeneities of cloud and drizzle microphysical properties and the aerosol-cloud-precipitation interactions.The spatial and vertical variabilities of cloud and drizzle microphysics are found in two different sets of flight legs:Leg-1 and Leg-2,which are parallel and perpendicular to the cloud propagation,respectively.The cloud along Leg-2 was close to adiabatic,where cloud-droplet effective radius and liquid water content linearly increase from cloud base to cloud top with less drizzle.The cloud along Leg-1 was sub-adiabatic with lower clouddroplet number concentration and larger cloud-droplet effective,but higher drizzle droplet number concentration,larger drizzle droplet median diameter and drizzle liquid water content.The heavier drizzle frequency and intensity on Leg-1 were enhanced by the collision-coalescence processes within cloud due to strong turbulence.The sub-cloud precipitation rate on Leg-1 was significantly higher than that along Leg-2.As a result,the sub-cloud accumulation mode aerosols and CCN on Leg-1 were depleted,but the coarse model aerosols increased.This further leads to a counter-intuitive phenomenon that the CCN is less than cloud-droplet number concentration for Leg-1.The average CCN loss rates are −3.89 cm^(-3)h^(-1)and −0.77 cm^(-3)h^(-1) on Leg-1 and Leg-2,respectively.The cloud and drizzle heterogeneities inside the same stratocumulus can significantly alter the sub-cloud aerosols and CCN budget.Hence it should be treated with caution in the aircraft assessment of aerosol-cloud-precipitation interactions.展开更多
Long-term observational data indicated a decreasing trend for the amount of autumn precipitation(i.e. 54.3 mm per decade) over Mid-Eastern China, especially after the 1980s(~ 5.6% per decade). To examine the cause of ...Long-term observational data indicated a decreasing trend for the amount of autumn precipitation(i.e. 54.3 mm per decade) over Mid-Eastern China, especially after the 1980s(~ 5.6% per decade). To examine the cause of the decreasing trend, the mechanisms associated with the change of autumn precipitation were investigated from the perspective of water vapor transportation, atmospheric stability and cloud microphysics. Results show that the decrease of convective available potential energy(i.e. 12.81 J kg-1/ decade) and change of cloud microphysics, which were closely related to the increase of aerosol loading during the past twenty years, were the two primary factors responsible for the decrease of autumn precipitation. Our results showed that increased aerosol could enhance the atmospheric stability thus weaken the convection. Meanwhile, more aerosols also led to a significant decline of raindrop concentration and to a delay of raindrop formation because of smaller size of cloud droplets. Thus, increased aerosols produced by air pollution could be one of the major reasons for the decrease of autumn precipitation. Furthermore, we found that the aerosol effects on precipitation in autumn was more significant than in other seasons, partly due to relatively more stable synoptic systems in autumn. The impact of large-scale circulation dominant in autumn and the dynamic influence on precipitation was more important than the thermodynamic activity.展开更多
Based on the scattering properties of nonspherical dust aerosol, a new method is developed for retrieving dust aerosol optical depths of dusty clouds. The dusty clouds are defined as the hybrid system of dust plume an...Based on the scattering properties of nonspherical dust aerosol, a new method is developed for retrieving dust aerosol optical depths of dusty clouds. The dusty clouds are defined as the hybrid system of dust plume and cloud. The new method is based on transmittance measurements from surface-based instruments multi-filter rotating shadowband radiometer （MFRSR） and cloud parameters from lidar measurements. It uses the difference of absorption between dust aerosols and water droplets for distinguishing and estimating the optical properties of dusts and clouds, respectively. This new retrieval method is not sensitive to the retrieval error of cloud properties and the maximum absolute deviations of dust aerosol and total optical depths for thin dusty cloud retrieval algorithm are only 0.056 and 0.1, respectively, for given possible uncertainties. The retrieval error for thick dusty cloud mainly depends on lidar-based total dusty cloud properties.展开更多
Aerosols are one of the important atmospheric constituents and exert indirect impact on climate through the modification of microphysical and radiative properties of clouds that in turn perturb the precipitation patte...Aerosols are one of the important atmospheric constituents and exert indirect impact on climate through the modification of microphysical and radiative properties of clouds that in turn perturb the precipitation pattern.Thus,the long term quantification of changes in aerosol and cloud characteristics and their interactions on both temporal as well as spatial scale will provide a crucial information for the better assessment of future climate change.In present study,18 years(2003-2020)MODerate Resolution Imaging Spectro-radiometer(MODIS)derived aerosol-cloud dataset over the Northern Indian Ocean(NIO)were analysed to assess climatology and trend of aerosol,cloud characteristics and their correlation.We found a strong heterogeneity in spatio-temporal variation of aerosol and cloud parameters over the NIO that are more prominent for the coastal region.The climatological mean of aerosol loading is found high(AOD≥0.5)over the outflow region along the Indian sub-continent and low(AOD≤0.2)over the northern equatorial open ocean.The climatological mean of cloud properties shows dominance of optically thicker deep convective(CTP<600 hPa and CTT<260 K)clouds over the southern Bay of Bengal(BoB)and thinner shallow(CTP>700 hPa and CTT>273 K)over the northwestern Arabian Sea(AS).Similarly,bigger effective radii(>17µm)observed along the equatorial open ocean whereas smaller CER(<17µm)were found over Indian sub-continental coastline and western AS.Further,trend analysis reveals an increasing pattern in AOD(0.002 yr^(-1)),CER(0.051µm yr^(-1)),LWP(0.033 gm^(-2) yr^(-1))and CF(0.002 yr^(-1))while COD,CTT and CTP show negative trend in order of-0.005 yr^(-1),-0.094 K yr^(-1) and-1.160 hPa yr^(-1),respectively.We also perform similar analysis for seven sub-region of interest(R1 to R7)across the NIO and results show a decreasing pattern in AOD(-0.001 yr^(-1))at R4 against maximum mean AOD(0.44±0.03).However,coastal sub-regions R1 and R5 illustrate maximum increase in aerosol loading(>0.003 yr^(-1))suggesting a significant impact of sub-continental outflow over the regions.The spatial correlation of cloud properties with respect to AOD shows a positive slope for CER(0.14)and CF(0.48)and a negative for COD(-0.19),LWP(-0.18),CTT(-0.37),CTP(-0.41).The present study provides in-depth information about the aerosol-cloud characteristics for a long term scale over NIO and could be useful in regional aerosol-cloud interaction induced climate forcing estimation.展开更多
Fengyun-4A（FY-4A）, the first of the Chinese next-generation geostationary meteorological satellites, launched in2016, offers several advances over the FY-2： more spectral bands, faster imaging, and infrared hypersp...Fengyun-4A（FY-4A）, the first of the Chinese next-generation geostationary meteorological satellites, launched in2016, offers several advances over the FY-2： more spectral bands, faster imaging, and infrared hyperspectral measurements. To support the major objective of developing the prototypes of FY-4 science algorithms, two science product algorithm testbeds for imagers and sounders have been developed by the scientists in the FY-4 Algorithm Working Group（AWG）. Both testbeds, written in FORTRAN and C programming languages for Linux or UNIX systems, have been tested successfully by using Intel/g compilers. Some important FY-4 science products, including cloud mask, cloud properties, and temperature profiles, have been retrieved successfully through using a proxy imager, Himawari-8/Advanced Himawari Imager（AHI）, and sounder data, obtained from the Atmospheric Infra Red Sounder, thus demonstrating their robustness. In addition, in early 2016, the FY-4 AWG was developed based on the imager testbed—a near real-time processing system for Himawari-8/AHI data for use by Chinese weather forecasters.Consequently, robust and flexible science product algorithm testbeds have provided essential and productive tools for popularizing FY-4 data and developing substantial improvements in FY-4 products.展开更多
The estimation of downward surface shortwave radiation(DSSR)is important for the Earth’s energy budget and climate change studies.This review was organised from the perspectives of satellite sensors,algorithms and fu...The estimation of downward surface shortwave radiation(DSSR)is important for the Earth’s energy budget and climate change studies.This review was organised from the perspectives of satellite sensors,algorithms and future trends,retrospects and summaries of the satellite-based retrieval methods of DSSR that have been developed over the past 10 years.The shortwave radiation reaching the Earth’s surface is affected by both atmospheric and land surface parameters.In recent years,studies have given detailed considerations to the factors which affect DSSR.It is important to improve the retrieval accuracy of cloud microphysical parameters and aerosols and to reduce the uncertainties caused by complex topographies and high-albedo surfaces(such as snow-covered areas)on DSSR estimation.This review classified DSSR retrieval methods into four categories:empirical,parameterisation,look-up table and machine-learning methods,and evaluated their advantages,disadvantages and accuracy.Further efforts are needed to improve the calculation accuracy of atmospheric parameters such as cloud,haze,water vapor and other land surface parameters such as albedo of complex terrain and bright surface,organically combine machine learning and other methods,use the new-generation geostationary satellite and polar orbit satellite data to produce highresolution DSSR products,and promote the application of radiation products in hydrological and climate models.展开更多
基金Young Scientists Fund of National Natural Science Foundation of China Grant(41505013,41575017)Natural Science Foundation of Shandong Province(BS2015HZ019)
文摘In this study, the micro-and macro-physical properties, thermal structure and precipitation characteristics of cyclone eye walls and their surrounding spiral clouds were analysed with Cloud Sat and TRMM data for five tropical cyclones(TCs) in 2013. The results show that the ice-phase clouds of a mature TC are mainly above 5 km. With increasing altitude, the cloud droplet effective radius decreases, and the particle number concentration increases. Ice water content first increases and then decreases with increasing height. In the eye area, in addition to the well-known warm-core area, another warm core is also apparent around the eye at a height of 8 to 15 km. The horizontal distribution of precipitation is characterized by large-scale stratiform precipitation mixed with independent convective precipitation. The height of precipitation is mostly below 7.5 km, and the heavy rain is mainly below 5 km. When the peripheral convective clouds are strong enough, ice particles would be generated, thus providing conditions that are favourable for the formation of precipitation below.
基金supported by the National Natural Science Foundation of China[grant numbers 41275039,61327810 and91337214]
文摘Accurate observation of clouds is challenging because of the high variability and complexity of cloud types and occurrences.By using the long-term cloud data collected during the ARM program at the Southern Great Plains central facility during 2001-2010,the consistencies and differences in the macrophysical properties of clouds between radiosonde and ground-based active remote sensing are quantitatively evaluated according to six cloud types:low;mid-low(ML);high-midlow;mid;high-mid(HM);and high.A similar variability trend is exhibited by the radiosonde and surface observations for the cloud fractions of the six cloud types.However,the magnitudes of the differences between the two methods are different among the six cloud types,with the largest difference seen in the high clouds.The distribution of the cloud-base height of the ML,mid,and HM clouds agrees in both methods,whereas large differences are seen in the cloud-top height for the ML and high clouds.The cloud thickness variations generally agree between the two datasets for the six cloud types.
基金supported by the National Natural Science Foundation of China(Grant No.NSFC 41875095,42075127).
文摘Cloud radiative kernels(CRK)built with radiative transfer models have been widely used to analyze the cloud radiative effect on top of atmosphere(TOA)fluxes,and it is expected that the CRKs would also be useful in the analyses of surface radiative fluxes,which determines the regional surface temperature change and variability.In this study,CRKs at the surface and TOA were built using the Rapid Radiative Transfer Model(RRTM).Longwave cloud radiative effect(CRE)at the surface is primarily driven by cloud base properties,while TOA CRE is primarily decided by cloud top properties.For this reason,the standard version of surface CRK is a function of latitude,longitude,month,cloud optical thickness(τ)and cloud base pressure(CBP),and the TOA CRK is a function of latitude,longitude,month,τand cloud top pressure(CTP).Considering that the cloud property histograms provided by climate models are functions of CTP instead of CBP at present,the surface CRKs on CBP-τhistograms were converted to CTP-τfields using the statistical relationship between CTP,CBP andτobtained from collocated CloudSat and MODIS observations.For both climate model outputs and satellites observations,the climatology of surface CRE and cloud-induced surface radiative anomalies calculated with the surface CRKs and cloud property histograms are well correlated with those calculated from surface radiative fluxes.The cloud-induced surface radiative anomalies reproduced by surface CRKs and MODIS cloud property histograms are not affected by spurious trends that appear in Clouds and the Earth's Radiant Energy System(CERES)surface irradiances products.
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences (KZCX2-YW-Q11-04)the "Strategic Priority Research Program" of the Chinese Academy of Sciences (XDA05100502)
文摘A coupled meteorology and aerosol/chemistry model WRF-Chem （Weather Research and Forecast model coupled with Chemistry） was used to conduct a pair of simulations with present-day （PD） and preindustrial （P1） emissions over East Asia to examine the aerosol indirect effect on clouds. As a result of an increase in aerosols in January, the cloud droplet number increased by 650 cm-3 over the ocean and East China, 400 cm-3 over Central and Southwest China, and less than 200 cm-3 over North China. The cloud liquid water path （LWP） increased by 40-60 g m-2 over the ocean and Southeast China and 30 g m-2 over Central China; the LWP in- creased less than 5 g m-2 or decreased by 5 g m2 over North China. The effective radius （Re） decreased by more than 4 pm over Southwest, Central, and Southeast China and 2 pm over North China. In July, variations in cloud properties were more uniform; the cloud droplet number increased by approximately 250400 cm-3, the LWP increased by approximately 30-50 g m 2, and Re decreased by approximately 3 μm over most regions of China. In response to cloud property changes from PI to PD, shortwave （SW） cloud radiative m-2 over the ocean and 10 forcing strengthened by 30 W W m-2 over Southeast China, and it weakened slightly by approximately 2-10 W m-2 over Central and Southwest China in January. In July, SW cloud radiative forcing strengthened by 15 W m-2 over Southeast and North China and weakened by l0 W m-2 over Central China. The different responses of SW cloud radiative forcing in different regions was related to cloud feedbacks and natural variability.
基金supported by the National Key Research and Development Project(Grant No.2019YFA0606803,2016YFA0601704)the National Natural Science Foundation of China(Grant No.41925022)+1 种基金the Innovation and Development Project of China Meteorological Administration(CXFZ2022J036)the Science and Technology Development Fund of Hubei Meteorological Bureau(Grant No.2017Y06,2017Y07,2016Y06,2019Y10).
文摘This study investigates the cloud macro-and micro-physical characteristics in the convective and stratiform regions and their different responses to the seeding for mixed convective-stratiform clouds that occurred in Shandong province on 21 May 2018,based on the observations from the aircraft,the Suomi National Polar-Orbiting Partnership(NPP)satellite,and the high-resolution Himawari-8(H8)satellite.The aircraft observations show that convection was deeper and radar echoes were significantly enhanced with higher tops in response to seeding in the convective region.This is linked with the conversion of supercooled liquid droplets to ice crystals with released latent heat,resulting in strengthened updrafts,enhanced radar echoes,higher cloud tops,and more and larger precipitation particles.In contrast,in the stratiform cloud region,after the Silver Iodide(AgI)seeding,the radar echoes become significantly weaker at heights close to the seeding layer,with the echo tops lowered by 1.4–1.7 km.In addition,a hollow structure appears at the height of 6.2–7.8 km with a depth of about 1.6 km and a diameter of about 5.5 km,and features such as icing seeding tracks appear.These suggest that the transformation between droplets and ice particles was accelerated by the seeding in the stratiform part.The NPP and H8 satellites also show that convective activity was stronger in the convective region after seeding;while in the stratiform region,a cloud seeding track with a width of 1–3 km appears 10 km downstream of the seeding layer 15 minutes after the AgI seeding,which moves along the wind direction as width increases.
基金jointly supported by the Strategic Priority Research Program of the Chinese Academy of Sciences (Grant No. XDA05100304)the Chinese Natural Science Foundation (Grant No. 41005073)
文摘To investigate the potential effects of aerosols on the microphysical properties of warm clouds, airborne observational data collected from 2009 to 2011 in Tongliao, Inner Mongolia, China, were statistically analyzed in this study. The results demonstrated that the vertical distribution of the aerosol number concentration（N_a） was similar to that of the clean rural continent. The average aerosol effective diameter（D_e） was maintained at approximately 0.4 μm at all levels. The data obtained during cloud penetrations showed that there was a progressive increase in the cloud droplet concentration（N_c） and liquid water content（LWC） from outside to inside the clouds, while the Nawas negatively related to the Ncand LWC at the same height. The fluctuation of the N_a, Ncand LWC during cloud penetration was more obvious under polluted conditions（Type 1） than under clean conditions（Type 2）. Moreover, the wet scavenging of cloud droplets had a significant impact on the accumulation mode of aerosols, especially on particles with diameters less than 0.4 μm. The minimum wet scavenging coefficient within the cloud was close to 0.02 under Type 1 conditions, while it increased to 0.1 under Type 2 conditions,which proved that the cloud wet scavenging effect under Type 1 conditions was stronger than that under Type 2 conditions.Additionally, cloud droplet spectra under Type 1 conditions were narrower, and their horizontal distributions were more homogeneous than those under Type 2 conditions.
基金supported by the NSF grants AGS-2031750 and AGS-2031751supported as part of the “Enabling Aerosol-cloud interactions at GLobal convection-permitting scal ES (EAGLES)” project (74358),funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Earth System Modeling program with the subcontract to the University of Arizona
文摘A closed-cell marine stratocumulus case during the Aerosol and Cloud Experiments in the Eastern North Atlantic(ACE-ENA)aircraft field campaign is selected to examine the heterogeneities of cloud and drizzle microphysical properties and the aerosol-cloud-precipitation interactions.The spatial and vertical variabilities of cloud and drizzle microphysics are found in two different sets of flight legs:Leg-1 and Leg-2,which are parallel and perpendicular to the cloud propagation,respectively.The cloud along Leg-2 was close to adiabatic,where cloud-droplet effective radius and liquid water content linearly increase from cloud base to cloud top with less drizzle.The cloud along Leg-1 was sub-adiabatic with lower clouddroplet number concentration and larger cloud-droplet effective,but higher drizzle droplet number concentration,larger drizzle droplet median diameter and drizzle liquid water content.The heavier drizzle frequency and intensity on Leg-1 were enhanced by the collision-coalescence processes within cloud due to strong turbulence.The sub-cloud precipitation rate on Leg-1 was significantly higher than that along Leg-2.As a result,the sub-cloud accumulation mode aerosols and CCN on Leg-1 were depleted,but the coarse model aerosols increased.This further leads to a counter-intuitive phenomenon that the CCN is less than cloud-droplet number concentration for Leg-1.The average CCN loss rates are −3.89 cm^(-3)h^(-1)and −0.77 cm^(-3)h^(-1) on Leg-1 and Leg-2,respectively.The cloud and drizzle heterogeneities inside the same stratocumulus can significantly alter the sub-cloud aerosols and CCN budget.Hence it should be treated with caution in the aircraft assessment of aerosol-cloud-precipitation interactions.
基金National Basic Research Program of China(2012CB955301)
文摘Long-term observational data indicated a decreasing trend for the amount of autumn precipitation(i.e. 54.3 mm per decade) over Mid-Eastern China, especially after the 1980s(~ 5.6% per decade). To examine the cause of the decreasing trend, the mechanisms associated with the change of autumn precipitation were investigated from the perspective of water vapor transportation, atmospheric stability and cloud microphysics. Results show that the decrease of convective available potential energy(i.e. 12.81 J kg-1/ decade) and change of cloud microphysics, which were closely related to the increase of aerosol loading during the past twenty years, were the two primary factors responsible for the decrease of autumn precipitation. Our results showed that increased aerosol could enhance the atmospheric stability thus weaken the convection. Meanwhile, more aerosols also led to a significant decline of raindrop concentration and to a delay of raindrop formation because of smaller size of cloud droplets. Thus, increased aerosols produced by air pollution could be one of the major reasons for the decrease of autumn precipitation. Furthermore, we found that the aerosol effects on precipitation in autumn was more significant than in other seasons, partly due to relatively more stable synoptic systems in autumn. The impact of large-scale circulation dominant in autumn and the dynamic influence on precipitation was more important than the thermodynamic activity.
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences (No.IAP09311)the National Natural Science Foundation of China (Nos.40725015 and 40633017)
文摘Based on the scattering properties of nonspherical dust aerosol, a new method is developed for retrieving dust aerosol optical depths of dusty clouds. The dusty clouds are defined as the hybrid system of dust plume and cloud. The new method is based on transmittance measurements from surface-based instruments multi-filter rotating shadowband radiometer （MFRSR） and cloud parameters from lidar measurements. It uses the difference of absorption between dust aerosols and water droplets for distinguishing and estimating the optical properties of dusts and clouds, respectively. This new retrieval method is not sensitive to the retrieval error of cloud properties and the maximum absolute deviations of dust aerosol and total optical depths for thin dusty cloud retrieval algorithm are only 0.056 and 0.1, respectively, for given possible uncertainties. The retrieval error for thick dusty cloud mainly depends on lidar-based total dusty cloud properties.
文摘Aerosols are one of the important atmospheric constituents and exert indirect impact on climate through the modification of microphysical and radiative properties of clouds that in turn perturb the precipitation pattern.Thus,the long term quantification of changes in aerosol and cloud characteristics and their interactions on both temporal as well as spatial scale will provide a crucial information for the better assessment of future climate change.In present study,18 years(2003-2020)MODerate Resolution Imaging Spectro-radiometer(MODIS)derived aerosol-cloud dataset over the Northern Indian Ocean(NIO)were analysed to assess climatology and trend of aerosol,cloud characteristics and their correlation.We found a strong heterogeneity in spatio-temporal variation of aerosol and cloud parameters over the NIO that are more prominent for the coastal region.The climatological mean of aerosol loading is found high(AOD≥0.5)over the outflow region along the Indian sub-continent and low(AOD≤0.2)over the northern equatorial open ocean.The climatological mean of cloud properties shows dominance of optically thicker deep convective(CTP<600 hPa and CTT<260 K)clouds over the southern Bay of Bengal(BoB)and thinner shallow(CTP>700 hPa and CTT>273 K)over the northwestern Arabian Sea(AS).Similarly,bigger effective radii(>17µm)observed along the equatorial open ocean whereas smaller CER(<17µm)were found over Indian sub-continental coastline and western AS.Further,trend analysis reveals an increasing pattern in AOD(0.002 yr^(-1)),CER(0.051µm yr^(-1)),LWP(0.033 gm^(-2) yr^(-1))and CF(0.002 yr^(-1))while COD,CTT and CTP show negative trend in order of-0.005 yr^(-1),-0.094 K yr^(-1) and-1.160 hPa yr^(-1),respectively.We also perform similar analysis for seven sub-region of interest(R1 to R7)across the NIO and results show a decreasing pattern in AOD(-0.001 yr^(-1))at R4 against maximum mean AOD(0.44±0.03).However,coastal sub-regions R1 and R5 illustrate maximum increase in aerosol loading(>0.003 yr^(-1))suggesting a significant impact of sub-continental outflow over the regions.The spatial correlation of cloud properties with respect to AOD shows a positive slope for CER(0.14)and CF(0.48)and a negative for COD(-0.19),LWP(-0.18),CTT(-0.37),CTP(-0.41).The present study provides in-depth information about the aerosol-cloud characteristics for a long term scale over NIO and could be useful in regional aerosol-cloud interaction induced climate forcing estimation.
基金National Natural Science Foundation(41405035,41571348,and 41405038)China Meteorological Administration Special Public Welfare Research Fund(GYHY201406011 and GYHY201506074)
文摘Fengyun-4A（FY-4A）, the first of the Chinese next-generation geostationary meteorological satellites, launched in2016, offers several advances over the FY-2： more spectral bands, faster imaging, and infrared hyperspectral measurements. To support the major objective of developing the prototypes of FY-4 science algorithms, two science product algorithm testbeds for imagers and sounders have been developed by the scientists in the FY-4 Algorithm Working Group（AWG）. Both testbeds, written in FORTRAN and C programming languages for Linux or UNIX systems, have been tested successfully by using Intel/g compilers. Some important FY-4 science products, including cloud mask, cloud properties, and temperature profiles, have been retrieved successfully through using a proxy imager, Himawari-8/Advanced Himawari Imager（AHI）, and sounder data, obtained from the Atmospheric Infra Red Sounder, thus demonstrating their robustness. In addition, in early 2016, the FY-4 AWG was developed based on the imager testbed—a near real-time processing system for Himawari-8/AHI data for use by Chinese weather forecasters.Consequently, robust and flexible science product algorithm testbeds have provided essential and productive tools for popularizing FY-4 data and developing substantial improvements in FY-4 products.
基金supported by the Second Tibetan Plateau Scientific Expedition and Research Program(STEP)(Grant No.2019QZKK0206)the National Natural Science Foundation of China(Grant No.41771395)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDA20100300)。
文摘The estimation of downward surface shortwave radiation(DSSR)is important for the Earth’s energy budget and climate change studies.This review was organised from the perspectives of satellite sensors,algorithms and future trends,retrospects and summaries of the satellite-based retrieval methods of DSSR that have been developed over the past 10 years.The shortwave radiation reaching the Earth’s surface is affected by both atmospheric and land surface parameters.In recent years,studies have given detailed considerations to the factors which affect DSSR.It is important to improve the retrieval accuracy of cloud microphysical parameters and aerosols and to reduce the uncertainties caused by complex topographies and high-albedo surfaces(such as snow-covered areas)on DSSR estimation.This review classified DSSR retrieval methods into four categories:empirical,parameterisation,look-up table and machine-learning methods,and evaluated their advantages,disadvantages and accuracy.Further efforts are needed to improve the calculation accuracy of atmospheric parameters such as cloud,haze,water vapor and other land surface parameters such as albedo of complex terrain and bright surface,organically combine machine learning and other methods,use the new-generation geostationary satellite and polar orbit satellite data to produce highresolution DSSR products,and promote the application of radiation products in hydrological and climate models.
