The Cretaceous is a typical period for studying the greenhouse climate and the earth system interactions, and the world’s most extensive terrestrial strata are mainly in East Asia, especially in China. Continental se...The Cretaceous is a typical period for studying the greenhouse climate and the earth system interactions, and the world’s most extensive terrestrial strata are mainly in East Asia, especially in China. Continental sediments can effectively reflect the paleo-climate change, but the previous studies of the Late Cretaceous paleo-climate, based on the combined characteristics of continental climate-sensitive sediments, were barely found in China. To obtain the Late Cretaceous paleo-climate characteristics of China, the distribution characteristics of different continental climate-sensitive sediment types in the early, middle and Late Cretaceous in China were studied in detail. According to the distribution and combination characteristics and types of continental climate-sensitive sediments, seven climate types can be divided: 1) warm-humid and warm-dry climate;2) hot and dry climate;3) hot-dry and arid climate;4) hot-dry and semiarid climate;5) hot-dry and hot-wet climate;6) hot-dry and warm-humid climate;7) hot-dry and warm-dry climate. The results show that in the early Late Cretaceous, the hot and dry climate was the most widespread, followed by warm-humid and warm-dry climate, but the climate was drier than the paleo-climate of the previous study of Early Cretaceous. Hot and dry climate zone became wider in the Coniacian and Maastrichtian;furthermore, it covered Xinjiang to the east of China from east to west after the Santonian Period. The hot-dry and semiarid climate zone was nearly latitudinally distributed from the northwest to the southeast and it shows a further increase in aridification. Global geological events, paleogeographic features and regional tectonic evolution had significant impacts on the paleoclimate of China in the Late Cretaceous, such as global eruptive events of volcanoes led to the temperature increase in China in the early Late Cretaceous;coastal mountain ranges in southeastern China led to the drying of the Late Cretaceous climate in southern China;Xuefeng Mountains, Wuling Mountains, Nanling Mountains and Tai-hang Mountains were the dividing line between the hot and dry climate zone and hot-dry and arid climate zone in the early Late Cretaceous, and Altun Mountains were the dividing line between the southeastern section of the hot and dry climate zone in western China in the middle Late Cretaceous.展开更多
Fluoroquinolones(FQs)have the propensity to accumulate in sediments once introduction into aquatic envi-ronments,thereby posing potential threats to benthic organisms,yet the ecotoxicity of sediment-associated FQs rem...Fluoroquinolones(FQs)have the propensity to accumulate in sediments once introduction into aquatic envi-ronments,thereby posing potential threats to benthic organisms,yet the ecotoxicity of sediment-associated FQs remains unclear.In this study,the toxicokinetics and responses of multiple biomarkers in Bellamya aeruginosa,exposed to the three commonly used FQs(norfloxacin,NOR;ciprofloxacin,CIP;levofloxacin,LEVO)at envi-ronmentally relevant concentrations were investigated under sediment exposure scenario.The results revealed that FQs were effectively ingested by B.aeruginosa from sediments,CIP showing the highest bioaccumulation(180.59μg/kg),followed by NOR(74.49μg/kg)and LEVO(36.02μg/kg).CIP exhibiting a highest uptake rate constant(Ks)(4.64 g/(g·day))and the lowest elimination rate constant(K_(e))(0.05 g/(g·day)).The descending order of biological half-life is as follows:CIP(13.62 days),LEVO(8.14 days),and NOR(6.83 days).NOR induced the activity of superoxide dismutase,catalase,and glutathione-S-transferase while CIP and LEVO depressed their activities and increased malondialdehyde content,indicating a more pronounced oxidative damage to B.aerug-inosa caused by CIP and LEVO than NOR.Furthermore,all three FQs were found to induce DNA damage and elevate acetylcholinesterase activity,suggesting distinct genotoxic and neurotoxic effects.Interestingly,despite its low bioaccumulation potential,LEVO exhibited high toxicity towards B.aeruginosa.These findings enhance our understanding of the ecotoxicity of FQs in sediments,providing further evidence of their potential ecological risks.展开更多
With the legislative development,the organic and inorganic composition separation has become the primary requirement for sewer sediment disposal,however the relevant technology has been rarely reported and the driving...With the legislative development,the organic and inorganic composition separation has become the primary requirement for sewer sediment disposal,however the relevant technology has been rarely reported and the driving mechanism was still unclear.In this study,direct disintegration of biopolymers and indirect broken of connection point were investigated on the hydrolysis and component separation.Three typical sewer sediment treatment approaches,i.e.,alkaline,thermal and cation exchange treatments were proposed,which represented the hydrolysis-driving forces of chemical hydrolysis,physical hydrolysis and innovative cation bridging break-age.The results showed that the organic and inorganic separation rates of sewer sediment driven by alkaline,thermal and cation exchange treatments reached 21.26%,23.80%,and 19.56%-48.0%,respectively,compared to 4.43%in control.The secondary structure of proteins was disrupted,transitioning from𝛼α-helix to𝛽β-turn and random coil.Meanwhile,much biopolymers were released from solid to the liquid phase.From thermody-namic perspective,sewer sediment deposition was controlled by short-range interfacial interactions described by extended Derjaguin-Landau-Verwey-Overbeek theory.Additionally,the separation of organic and inorganic components was positively correlated with the thermodynamic parameters(Corr=0.87),highlighted the robust-ness of various driving forces.And the flocculation energy barriers were 2.40(alkaline),1.60 times(thermal),and 4.02–4.97 times(cation exchange)compared to control group.The findings revealed the contrition differ-ence of direct disintegration of gelatinous biopolymers and indirect breakage of composition connection sites in sediment composition separation,filling the critical gaps in understanding the specific mechanisms of sediment biopolymer disintegration and intermolecular connection breakage.展开更多
This study compares the environmental sustainability of five alternatives for the remediation of marine sediments of one of the most polluted coastal sites in Europe(Bagnoli-Coroglio bay,Mediterranean Sea),using the L...This study compares the environmental sustainability of five alternatives for the remediation of marine sediments of one of the most polluted coastal sites in Europe(Bagnoli-Coroglio bay,Mediterranean Sea),using the Life Cycle Assessment(LCA)methodology.The treatments are either in-situ or exsitu,the latter requiring an initial dredging to transport the contaminated sediments to the management site.More in detail,four ex-situ remediation technologies based on landfilling,bioremediation,electrokinetic technique and soil washing were identified.These technologies are compared to an in-situ strategy currently under validation for enhancing bioremediation of the polluted sediments of the Bagnoli-Coroglio site.Our results indicate that the disposal in landfilling site is the worst option in most categories(e.g.,650 kg CO_(2) eq./t of treated sediment,considering the nearest landfilling site),followed by the bioremediation,mainly due to the high energy demand.Electrokinetic remediation,soil washing,and innovative in-situ technology represent the most sustainable options.In particular,the new in-situ technology appears to be the least impacting in all categories(e.g.,54 kg CO_(2) eq./t of treated sediment),although it is expected to require longer treatment time(estimated up to 12 months based on its potential efficiency).It can reduce the impact on climate change more than 12 times compared to the disposal and 7 times compared to bioremediation in addition to the possibility to avoid/reduce the dredging operations and the consequent dispersion of pollutants.The results open relevant perspectives towards more eco-sustainable and costly effective actions for the reclamation of contaminated marine sediments.展开更多
China’s lakes are plagued by cadmium(Cd)pollution.Dissolved organic matter(DOM)significantly regulates Cd(II)transport properties at the sediment-water interface.Understanding the effects of different DOM components ...China’s lakes are plagued by cadmium(Cd)pollution.Dissolved organic matter(DOM)significantly regulates Cd(II)transport properties at the sediment-water interface.Understanding the effects of different DOM components on the transportation properties of Cd(II)at the sediment-water interface is essential.In this study,typical DOM from different sources was selected to study Cd(II)mobility at the sediment-water interface.Results showed that terrestrial-derived DOM(fulvic acids,FA)and autochthonous-derived DOM(α-amylase,B1)inhibit Cd(II)sequestration by sediments(42.5%and 5.8%,respectively),while anthropogenic-derived DOM(sodium dodecyl benzene sulfonate,SDBS)increased the Cd(II)adsorption capacity by sediments by 2.8%.Fluorescence quenching coupling with parallel factor analysis(EEM-PARAFAC)was used to characterize different DOM components.The results showed that FA contains three kinds of components(C1,C3:protein-like components,C2:humic-like components);SDBS contains two kinds of components(C1,C2:protein-like components);B1 contains three kinds of components(C1,C2:protein-like components,C3:humic-like components).Three complex reaction modelswere used to characterize the ability of Cd(II)complex with DOM,and it was found that the humic-like component could hardly be complex with Cd(II).Accordingly,humic-like components compete for Cd(II)adsorption sites on the sediment surface and inhibit Cd(II)adsorption fromsediments.Fourier transform infrared spectroscopy(FTIR)of the sediment surface before and after Cd(II)addition was analyzed and proved the competitive adsorption theory.This study provides a better understanding of the Cd(II)mobilization behavior at the sediment-water interface and indicates that the input of humic-like DOM will increase the bioavailability of Cd.展开更多
Obtaining high-quality 10000-meter-deep seafloor sediment samples is the prerequisite and foundation for conducting deep-sea geological and environmental scientific research.The bottom structure of the deep seafloor i...Obtaining high-quality 10000-meter-deep seafloor sediment samples is the prerequisite and foundation for conducting deep-sea geological and environmental scientific research.The bottom structure of the deep seafloor is complex,and the physical and mechanical properties and disturbance resistance of sediments of different lithologies vary greatly,so the sediment sampler inevitably disturbs the sediments during the sampling process and affects the quality of the sediment samples.A new type of deep-sea sediment pressure retaining sampler is introduced,the force state and elastic–plastic state of the sampler destroying sediments are analyzed,the radial disturbance model of sediment coring based on the spherical cavity expansion theory is established,and the radius of sediments undergoing plastic deformation around the spherical holes is used as an index for evaluating the radial disturbance of sediments.The distribution of stress and strain fields in the sediments during the expansion of the spherical cavity and the influencing factors of the radius of the radially disturbed region(plastic region)are analyzed using an arithmetic example,and the influence law is analyzed.A sediment disturbance experimental platform was built indoors to simulate the sediment coring process.The radial stress field and pore water pressure of the sediment during the coring process were monitored by sensors arranged inside the sediment,and the results of indoor tests verified the correctness of the perturbation theory model.The sampler was carried aboard the deep-sea manned submersible FENDOUZHE and conducted on-site tests at depths of 9298.4 and 9142.8 m in the Kuril-Kamchatka Trench.Pressure-preserved sediment samples were retrieved,with preservation rates of 94.21%and 92.02%,respectively,which are much higher than the current technical indicator of 80%of pressure-holding ratio for deep-sea sediments.The retrieved sediments have obvious stratification characteristics and little disturbance.展开更多
The spatiotemporal characterization of plume sedimentation and microorganisms is critical for developing plume ecological monitoring model.To address the limitations of traditional methods in obtaining high-quality se...The spatiotemporal characterization of plume sedimentation and microorganisms is critical for developing plume ecological monitoring model.To address the limitations of traditional methods in obtaining high-quality sediment,a novel sampling system with 6000 m operational capability and three-month endurance was developed.It is equipped with three sediment samplers,a set of formaldehyde preservation solution injection devices.The system is controlled by a low-power,timing-triggered controllers.To investigate low-disturbance rheological mechanisms,gap controlled rheological tests were conducted to optimize the structural design of the sampling and sealing assembly.Stress-controlled shear rheological tests were employed to investigate the mechanisms governing yield stress in sediments under varying temperature conditions and boundary roughness.Additionally,the coupled Eulerian-Lagrangian(CEL)method and sediment rheological constitutive models were employed to simulate tube-soil interaction dynamics and sediment disturbance.The radial heterogeneity of sediment disturbance and friction variation of the sampling tube were revealed.The tube was completely“plugged”at a penetration depth of 261 mm,providing critical data support to the penetration depth parameters.The deep-sea pressure test and South China Sea field trials demonstrated the system’s capability to collect and preserve quantitative time-series sediment samples with high fidelity.展开更多
Fine-grained sediments are widely distributed and constitute the most abundant component in sedi-mentary systems,thus the research on their genesis and distribution is of great significance.In recent years,fine-graine...Fine-grained sediments are widely distributed and constitute the most abundant component in sedi-mentary systems,thus the research on their genesis and distribution is of great significance.In recent years,fine-grained sediment gravity-flows(FGSGF)have been recognized as an important transportation and depositional mechanism for accumulating thick successions of fine-grained sediments.Through a comprehensive review and synthesis of global research on FGSGF deposition,the characteristics,depositional mechanisms,and distribution patterns of fine-grained sediment gravity-flow deposits(FGSGFD)are discussed,and future research prospects are clarified.In addition to the traditionally recognized low-density turbidity current and muddy debris flow,wave-enhanced gravity flow,low-density muddy hyperpycnal flow,and hypopycnal plumes can all form widely distributed FGSGFD.At the same time,the evolution of FGSGF during transportation can result in transitional and hybrid gravity-flow deposits.The combination of multiple triggering mechanisms promotes the widespread develop-ment of FGSGFD,without temporal and spatial limitations.Different types and concentrations of clay minerals,organic matters,and organo-clay complexes are the keys to controlling the flow transformation of FGSGF from low-concentration turbidity currents to high-concentration muddy debris flows.Further study is needed on the interaction mechanism of FGSGF caused by different initiations,the evolution of FGSGF with the effect of organic-inorganic synergy,and the controlling factors of the distribution pat-terns of FGSGFD.The study of FGSGFD can shed some new light on the formation of widely developed thin-bedded siltstones within shales.At the same time,these insights may broaden the exploration scope of shale oil and gas,which have important geological significances for unconventional shale oil and gas.展开更多
Sediment particles,as one of the key components of drip irrigation technology,significantly affect the service life of emitters and restrict the popularization of drip irrigation technology.Hence,two types of patch dr...Sediment particles,as one of the key components of drip irrigation technology,significantly affect the service life of emitters and restrict the popularization of drip irrigation technology.Hence,two types of patch drip irrigation emitters,focusing on the anti-clogging performance through the experiment,were investigated.The dynamic variations in the clogging characteristics of emitters,specifically were subjected to statistical analysis.The movement mechanism of emitter clogging and discharging sediment was studied.The effects of emitter structure and position factors on emitter clogging were analyzed.The results show that the pressure-compensated emitter exhibits superior anti-clogging perfor-mance,with a service life that is 227.8%greater than that of the labyrinth channel emitter.A single structural factor cannot completely evaluate the anti-clogging performance of emitters.All factors causing emitter clogging should be considered comprehensively.Emitters contain sensitive sediment prone to clogging,however,significant blockage occurs primarily when the sediment content is elevated.The discharge of sediment,denoted as V90,from the emitter is affected by the accumulative effect of clogged sediment.These results may offer valuable insights for the application and advancement of drip irrigation technology.展开更多
This study evaluates the dynamics of trace metals impacts on the ecosystems of the Bartlett Pond, a small shallow wetland pond located in Laredo, Texas by analyzing sediment samples taken from four quadrants of the po...This study evaluates the dynamics of trace metals impacts on the ecosystems of the Bartlett Pond, a small shallow wetland pond located in Laredo, Texas by analyzing sediment samples taken from four quadrants of the pond. The concentrations of trace elements in sediment samples are highest for iron (Fe), followed by chromium (Cr), then lead (Pb), with lower concentration of antimony (Sb), cobalt (Co), arsenic (As), cadmium (Cd), and the lowest concentration being thallium (Tl) within Bartlett Pond. The sediment quality of the pond is acceptable for organisms and the environment as trace element concentrations (e.g. As, Cd, Cr, and Pb) are within the probable effect concentration (PEC) of National Ocean and Atmospheric Administration (NOAA) guidelines although the PEC values for Co, Fe, Sb and Tl are not given. Bivariate and multivariate correlation analysis shows that most trace elements exhibit a strong positive correlation among them indicating the same anthropogenic sources and biogeochemical processes control these trace elements concentrations within the pond. We provided a comprehensive snapshot of trace element concentrations in sediments through descriptive analysis, laying the foundation for future environmental risk assessments. Correlation analysis of eight trace elements helped identify relationships, offering insights into pollution sources and potential health impacts. Additionally, univariate and multivariate predictive analyses generated numerous models, extending beyond the interpretation of partial and full regression coefficients. We also included graphical analyses of trace element variations, which are critical for understanding environmental processes and geochemical patterns. These findings advance our understanding about trace metals dynamics in sediments and may be a valuable reference for ecosystems and environmental management of different landscapes.展开更多
Under the background of global climate change, anthropogenic processes have profoundly altered the sources and transport mechanisms of coastal sediments. While previous research has primarily focused on large river de...Under the background of global climate change, anthropogenic processes have profoundly altered the sources and transport mechanisms of coastal sediments. While previous research has primarily focused on large river delta coasts,the responses of the widely distributed small bays dominated by ocean dynamics, has received comparatively less attention. To address this gap, this study examines the Weihai Bay, located in the northeast of Shandong Peninsula,China. By integrating total organic carbon isotope tracers(δ^(13)C and C/N) with sediment transport modeling, we systematically analyze the spatiotemporal patterns of surface sediment grain size inside and outside the bay, along with their responses to natural and human-induced drivers. Our findings reveal that the sedimentary environment of Weihai Bay is governed by the combined effects of tidal currents, ocean currents, wave activity, and sediment supply. Tidal dynamics dominate the hydrodynamic conditions within the bay, while ocean currents predominate offshore. Surface sediments in the bay are primarily composed of silt, originating from sediments carried by the Yellow Sea Warm Current. These sediments enter the bay through the southern bay mouth under tidal forcing, are redistributed counterclockwise by residual tidal currents, and eventually exit via the northern bay mouth. Coarser sediments in specific areas are primarily controlled by strong wave action and terrestrial inputs. Between 1988 and 2023, Weihai Bay sediments have undergone a noticeable coarsening trend, primarily driven by anthropogenic modifications to sediment supply and hydrodynamic regimes. Coastal reclamation, shoreline modification, and infrastructure development have intensified coarse-grained terrestrial sediment input. Concurrently, shoreline advancement has reduced wave dissipation, enhancing nearshore hydrodynamics and accelerating sediment coarsening. This study highlights the sensitivity of small bay sedimentary environments to anthropogenic forcing, advancing our understanding of the coupled human-marine sediment system and providing a scientific basis for coastal sediment evolution under the dual influences of climate change and human activity.展开更多
Based on recent advancements in shale oil exploration within the Ordos Basin,this study presents a comprehensive investigation of the paleoenvironment,lithofacies assemblages and distribution,depositional mechanisms,a...Based on recent advancements in shale oil exploration within the Ordos Basin,this study presents a comprehensive investigation of the paleoenvironment,lithofacies assemblages and distribution,depositional mechanisms,and reservoir characteristics of shale oil of fine-grained sediment deposition in continental freshwater lacustrine basins,with a focus on the Chang 7_(3) sub-member of Triassic Yanchang Formation.The research integrates a variety of exploration data,including field outcrops,drilling,logging,core samples,geochemical analyses,and flume simulation.The study indicates that:(1)The paleoenvironment of the Chang 7_(3) deposition is characterized by a warm and humid climate,frequent monsoon events,and a large water depth of freshwater lacustrine basin.The paleogeomorphology exhibits an asymmetrical pattern,with steep slopes in the southwest and gentle slopes in the northeast,which can be subdivided into microgeomorphological units,including depressions and ridges in lakebed,as well as ancient channels.(2)The Chang 7_(3) sub-member is characterized by a diverse array of fine-grained sediments,including very fine sandstone,siltstone,mudstone and tuff.These sediments are primarily distributed in thin interbedded and laminated arrangements vertically.The overall grain size of the sandstone predominantly falls below 62.5μm,with individual layer thicknesses of 0.05–0.64 m.The deposits contain intact plant fragments and display various sedimentary structure,such as wavy bedding,inverse-to-normal grading sequence,and climbing ripple bedding,which indicating a depositional origin associated with density flows.(3)Flume simulation experiments have successfully replicated the transport processes and sedimentary characteristics associated with density flows.The initial phase is characterized by a density-velocity differential,resulting in a thicker,coarser sediment layer at the flow front,while the upper layers are thinner and finer in grain size.During the mid-phase,sliding water effects cause the fluid front to rise and facilitate rapid forward transport.This process generates multiple“new fronts”,enabling the long-distance transport of fine-grained sandstones,such as siltstone and argillaceous siltstone,into the center of the lake basin.(4)A sedimentary model primarily controlled by hyperpynal flows was established for the southwestern part of the basin,highlighting that the frequent occurrence of flood events and the steep slope topography in this area are primary controlling factors for the development of hyperpynal flows.(5)Sandstone and mudstone in the Chang 7_(3) sub-member exhibit micro-and nano-scale pore-throat systems,shale oil is present in various lithologies,while the content of movable oil varies considerably,with sandstone exhibiting the highest content of movable oil.(6)The fine-grained sediment complexes formed by multiple episodes of sandstones and mudstones associated with density flow in the Chang 7_(3) formation exhibit characteristics of“overall oil-bearing with differential storage capacity”.The combination of mudstone with low total organic carbon content(TOC)and siltstone is identified as the most favorable exploration target at present.展开更多
The Malacca Strait(MS)is a vital conduit for the exchange of water and sediment between the Indian Ocean and the Pacific Ocean,serving as a critical‘gateway'for sediment transport.Here,we present the geochemical ...The Malacca Strait(MS)is a vital conduit for the exchange of water and sediment between the Indian Ocean and the Pacific Ocean,serving as a critical‘gateway'for sediment transport.Here,we present the geochemical characteristics of surface sediments in the MS to elucidate the relationship between terrestrial material inputs and modern oceanic dynamic transport processes in the strait.The results reveal that the MS can be divided into three distinct geochemical provinces.ProvinceⅠ,located in the central region of the strait,is characterized by residual deposits.The preservation of these residual deposits can be attributed to the restricted sediment supply and the relatively weaker modern sedimentary hydrodynamic conditions.ProvinceⅡ,situated to the north of ProvinceⅠ,exhibits provenance differences between its southern and northern regions.The northern region is primarily supplied by sediments originating from the eastern shelf of the Andaman Sea,whereas sediments derived from Sumatra and the Sunda Shelf are predominantly deposited in the southern part of ProvinceⅡ.ProvinceⅢextends along the western coast of the Malaysian Peninsula,with sediments primarily sourced from the Malaysian Peninsula and the Sunda Shelf,while contributions from Sumatra and the eastern shelf of the Andaman Sea are negligible.River sediments from the Malaysian Peninsula and Sumatra are transported northwestward along their respective coasts by prevailing currents,which also facilitate the transportation of Sunda Shelf sediments within the strait,while sediments from the eastern shelf of the Andaman Sea are delivered to the MS via southward coastal currents during the southwest monsoon period.The southward currents and well-developed eddies potentially impede the northward transport of sediments from the Sunda Shelf and restrict the distribution of Andaman Sea sediments within the strait.This study substantially enhances the understanding of source-to-sink processes in the Indo-Pacific region.展开更多
Organic phosphorus(OP)constitutes an important fraction of total phosphorus in lake sediments,with its mobility being influenced by mineralization and transformation of organic carbon(OC).OP and OC co-exist in various...Organic phosphorus(OP)constitutes an important fraction of total phosphorus in lake sediments,with its mobility being influenced by mineralization and transformation of organic carbon(OC).OP and OC co-exist in various forms in the environment,thus a thorough investigation on the impact of OC fractions on the release of OP in sediments should be comprehensively carried out.This study determined the chemical forms of OP and OC in the sediments over four seasons in Lake Taihu and found temporal and spatial variations in their concentrations.The concentration of total OP and total OC ranged from 133 to 348 mg/kg and 4.77 to 21.19 mg/kg,respectively.Correlation between chemical fractions of OP and OC also revealed that Na OH-extracted OP,and fulvic acid-bound and humic acid-bound OP were positively correlated with humic-OC and hot hydrolysis-OC.These results suggest that the algal-derived OC degradation and mineralization may enhance OP mineralization,converting stable or moderately active OP into active forms or inorganic phosphorus under cyanobacterial bloom.This study provides insight and guiding support for investigating the impact of organic matter components on the transformation of OP after cyanobacterial degradation in eutrophic lakes.展开更多
Mangrove wetlands are a vital component of the blue carbon ecosystem,which is of great significance to coastal ecosystems and the global carbon balance.However,mangrove forests worldwide face a combination of natural ...Mangrove wetlands are a vital component of the blue carbon ecosystem,which is of great significance to coastal ecosystems and the global carbon balance.However,mangrove forests worldwide face a combination of natural and anthropogenic threats.This study employs highresolution sedimentology,geochemistry,and pollen analysis to reveal the sedimentary evolution and vegetation succession in the mangrove wetland of Dongzhai Harbor,Hainan Island.By utilizing multiple proxies,including^(14)C chronology,δ^(13)C,C/N,and the chemical index of alteration(CIA),we identified three distinct stages in the sedimentary records spanning from the Late Pleistocene to the modern age.Prior to the last glaciation,during the Late Pleistocene,the study area exhibited marine carbonate facies,with an abundance of marine-derived organic matter.During the low sea-level stage of the last glaciation,the strata in the core location were exposed.Following the last glaciation,the study area gradually transitioned into intertidal settings in response to fluctuating sea levels.Since the Middle Holocene or even earlier,sedimentary organic matter continued to accumulate as terrestrial C3 vegetation and mangrove forests established,persisted,and developed.This period witnessed the formation of the current estuarine environment.Simultaneously,the pioneering mangrove species,probably represented by Avicennia,might be initially established,followed by Rhizophora,Bruguiera and Ceriops communities,ultimately being replaced by Kandelia obovata to date.These findings not only fill the gap in the study of paleo-mangroves in China but also contribute valuable knowledge to the global reconstruction of paleo-mangroves,providing crucial reference for the conservation of mangroves and prediction of their responses in the context of climate change.展开更多
To explore the relationship of microplastic pollution in different media in marine environment,microplastics in the surface seawater and sediments of Laizhou Bay,Bohai Sea,North China,were studied.Seawater samples wer...To explore the relationship of microplastic pollution in different media in marine environment,microplastics in the surface seawater and sediments of Laizhou Bay,Bohai Sea,North China,were studied.Seawater samples were collected using a pre-concentrator equipped with a 20-μm mesh size sieve,and sediment samples were collected by a box sampler.The shape,color,size,and type of microplastics were obtained by a stereomicroscope and a Fourier transform infrared spectrometer(ATR-μ-FT-IR).Results show that the abundance of microplastics in the surface seawater of Laizhou Bay was 858.3±573.2 items/m~3,and that of microplastics in sediments was 151.0±77.4 items/kg dry weight(d.w.)The microplastics in seawater and sediments were mainly fibrous.Meanwhile,the microplastics in seawater were mainly transparent,and those in sediments were transparent and blue.The highest proportion of microplastics in seawater was rayon(77.48%),followed by polyethylene terephthalate(PET,13.17%).The highest proportion of microplastics in sediments was rayon(73.66%),followed by PET(8.90%).The size of microplastics in 1000-2000μm accounted for the largest proportion of 28.54%in seawater,while that in 500-1000μm took 27.93%in sediment.Microplastics in seawater and sediment showed medium-level pollution.In seawater,microplastic abundance was higher in offshore and nearshore areas of Weifang.In sediment,microplastic abundance was higher in offshore and nearshore areas of Dongying.The results of the principal component analysis(PCA)indicated that microplastics in sediment exhibited greater stability compared to those in seawater.The microplastics in seawater and sediment show a positive correlation in terms of shape and plastic type,while exhibiting a negative correlation in terms of color.Overall,microplastics in sediments were smaller in size,and those in seawater and sediments had consistent size distribution characteristics in space.展开更多
Understanding the sedimentation and simultaneous consolidation behavior of xanthan gum(XG)-biopolymer-treated soils remains a significant research gap in developing environmentally friendly ground-improvement techniqu...Understanding the sedimentation and simultaneous consolidation behavior of xanthan gum(XG)-biopolymer-treated soils remains a significant research gap in developing environmentally friendly ground-improvement techniques for geotechnical applications.This study addresses this gap by conducting laboratory experiments on kaolinite suspensions with varying XG-to-kaolinite mass ratios(mb/ms).The results showed that the XG treatment modified the sedimentation patterns by promoting larger floc formation and accelerated settling.Additionally,the XG treatment enhanced the shear stiffness and shear strength,particularly at shallow depths.At mb/ms ratios less than 1%,the volume compression was reduced by the XG;the coefficient of compressibility decreased by 49%at 1%mb/ms,and the consolidation was accelerated,as indicated by a 387%increase in the hydraulic conductivity at 0.5%mb/ms under the vertical effective stress of 40 kPa.Contrastingly,at mb/ms ratios greater than 1%,viscous XG hydrogels clogged pores,resulting in a 45%reduction in the coefficient of consolidation at 2%mb/ms under a vertical effective stress of 15 kPa and a 35%decrease in the hydraulic conductivity at 2%mb/ms under a vertical effective stress of 40 kPa.These findings underscore the potential of XG treatment in improving the sedimentation and consolidation processes,highlighting its applicability in geotechnical projects,such as dredging,landfilling,and artificial island construction.展开更多
The contamination and accumulation of microplastics(MPs)in mangrove ecosystems have become an increasing concern due to their potential ecological risks.This study investigated and analyzed the abundance of MPs in sed...The contamination and accumulation of microplastics(MPs)in mangrove ecosystems have become an increasing concern due to their potential ecological risks.This study investigated and analyzed the abundance of MPs in sediments,water,and benthos of mangrove areas(MA)and adjacent non-vegetated areas(NA)in Qinglan Bay.Results showed that the abundance of MPs in MA was significantly higher than in adjacent NA[sediment:(4.39±2.20)items/50 g dry weight(dw)vs.(4.10±2.71)items/50 g dw;water:(11.79±7.61)items/L vs.(10.61±5.93)items/L;benthos:(4.94±5.27)items/individual vs.(3.5±0.71)items/individual].The primary components identified in sediments and benthos were rayon and cellulose,while polyethylene(PE)and polypropylene(PP)dominated in water.Smaller MPs(<1000μm)accounted for 44%,43%,and 61%of the MPs in sediments,water,and benthos,respectively,indicating that smaller MPs are more likely to be ingested or captured by benthic organisms.Additionally,MPsenrichment was calculated in benthos[enrichment index(EI)=1.41],water(EI=1.11),and sediments(EI=1.09),confirming that the unique ecological environment of the MA leads to different distribution and accumulation characteristics of MPs compared to the NA.The ecological risk assessment revealed low MPs pollution levels in sediments and water,but higher risks were observed for polychaetes and bivalves.展开更多
Plastic pollution and microplastics in sediments are a growing concern for marine ecosystems worldwide.We examined the vertical distribution and properties of microplastics in beach sediments of Xuwen Coral Reef Natio...Plastic pollution and microplastics in sediments are a growing concern for marine ecosystems worldwide.We examined the vertical distribution and properties of microplastics in beach sediments of Xuwen Coral Reef National Nature Reserve,in Leizhou Peninsula,Zhanjiang,China.Sediment samples were taken in seven locations at 5-cm intervals from the surface to a depth of 30 cm.The vertical distribution of microplastic particles ranged from 0 to 1340 particles per kg on average of 119.05particles per kg.The most prevalent material was fibers(76%),followed by film(12%),fragments(11.2%),and foam(0.8%).The microplastics in size of 1-2 mm constituted the largest percentage(40%)of the total,followed by those in size of<1 mm(26.4%),2-3 mm(21.2%),3-4 mm(9.6%),and 4-5 mm(2.81%).Site S1 observed maximum sizes between 1 and 2 mm,S2 reported higher availability of microplastics with sizes ranging from 0.3 to 1 mm.Six different types of polymers were identified in the investigation,and mostly were polyethylene(PE)and polypropylene(PP).In general,the observation of microplastics in deeper sediments indicates that they have the ability to last for prolonged periods in the marine environment,which may present long-term hazards to benthic creatures.In conclusion,the discovery of microplastics in deep layers of coastal sediments highlights the necessity of minimizing plastic waste and enhancing management strategies to safeguard marine environments.展开更多
The arsenic(As)release from sediments in great lakes is affected by various factors.In this study,the characteristics of As release fromsediments was investigated,and the As sources and sinks with the strengths in sed...The arsenic(As)release from sediments in great lakes is affected by various factors.In this study,the characteristics of As release fromsediments was investigated,and the As sources and sinks with the strengths in sediments from different areas(grass-type,algae-type,and grass-algae alternation areas)in great shallow lakes(Taihu Lake,China)were analyzed,and the influence of P competition in the process of As release was also studied.The results showed that changing trend of the values of equilibrium As concentration in sediments were consistent with the regional changes(0 to 28.12μg/L),and the sediments from algaetype areas had the higher values.The sediments from western lake and northwest lake bay were a strong As and a weak P source,and the north lake bay had the opposite trend of these two regions.Intense P source competition with As from the sediments occurred in algae-type areas.The grass-type areas had strong As and P retention capacities,indicating a sink role of sediment with high As and P sorption capacities.The degree of As and P saturation had similar trend in sediments,and the grass-type areas had the higher values,18.3%-21.4%and 15.31%-20.34%,respectively.Contribution analysis results showed that most of As release contribution was from the bottom(30-50 cm)sediments,and the surface(0-10 cm)sediments from algae-type areas contributed more to the overlying water than other region.展开更多
基金A project funded by National Natural Science Foundation of China(41572093)Central Young College Teachers Fund Project (3142020002)Supported by the Fundamental Research Funds for the Central Universities(3142021004)。
文摘The Cretaceous is a typical period for studying the greenhouse climate and the earth system interactions, and the world’s most extensive terrestrial strata are mainly in East Asia, especially in China. Continental sediments can effectively reflect the paleo-climate change, but the previous studies of the Late Cretaceous paleo-climate, based on the combined characteristics of continental climate-sensitive sediments, were barely found in China. To obtain the Late Cretaceous paleo-climate characteristics of China, the distribution characteristics of different continental climate-sensitive sediment types in the early, middle and Late Cretaceous in China were studied in detail. According to the distribution and combination characteristics and types of continental climate-sensitive sediments, seven climate types can be divided: 1) warm-humid and warm-dry climate;2) hot and dry climate;3) hot-dry and arid climate;4) hot-dry and semiarid climate;5) hot-dry and hot-wet climate;6) hot-dry and warm-humid climate;7) hot-dry and warm-dry climate. The results show that in the early Late Cretaceous, the hot and dry climate was the most widespread, followed by warm-humid and warm-dry climate, but the climate was drier than the paleo-climate of the previous study of Early Cretaceous. Hot and dry climate zone became wider in the Coniacian and Maastrichtian;furthermore, it covered Xinjiang to the east of China from east to west after the Santonian Period. The hot-dry and semiarid climate zone was nearly latitudinally distributed from the northwest to the southeast and it shows a further increase in aridification. Global geological events, paleogeographic features and regional tectonic evolution had significant impacts on the paleoclimate of China in the Late Cretaceous, such as global eruptive events of volcanoes led to the temperature increase in China in the early Late Cretaceous;coastal mountain ranges in southeastern China led to the drying of the Late Cretaceous climate in southern China;Xuefeng Mountains, Wuling Mountains, Nanling Mountains and Tai-hang Mountains were the dividing line between the hot and dry climate zone and hot-dry and arid climate zone in the early Late Cretaceous, and Altun Mountains were the dividing line between the southeastern section of the hot and dry climate zone in western China in the middle Late Cretaceous.
基金supported by the Hunan Provincial Natural Science Foundation of China(Nos.2023JJ40518 and 2023JJ30490)the Scientific Research Foundation of Hunan Provincial Education Department(Nos.21B0511 and 22A0384)the Research Funding Project of Jishou University for talent introduction.
文摘Fluoroquinolones(FQs)have the propensity to accumulate in sediments once introduction into aquatic envi-ronments,thereby posing potential threats to benthic organisms,yet the ecotoxicity of sediment-associated FQs remains unclear.In this study,the toxicokinetics and responses of multiple biomarkers in Bellamya aeruginosa,exposed to the three commonly used FQs(norfloxacin,NOR;ciprofloxacin,CIP;levofloxacin,LEVO)at envi-ronmentally relevant concentrations were investigated under sediment exposure scenario.The results revealed that FQs were effectively ingested by B.aeruginosa from sediments,CIP showing the highest bioaccumulation(180.59μg/kg),followed by NOR(74.49μg/kg)and LEVO(36.02μg/kg).CIP exhibiting a highest uptake rate constant(Ks)(4.64 g/(g·day))and the lowest elimination rate constant(K_(e))(0.05 g/(g·day)).The descending order of biological half-life is as follows:CIP(13.62 days),LEVO(8.14 days),and NOR(6.83 days).NOR induced the activity of superoxide dismutase,catalase,and glutathione-S-transferase while CIP and LEVO depressed their activities and increased malondialdehyde content,indicating a more pronounced oxidative damage to B.aerug-inosa caused by CIP and LEVO than NOR.Furthermore,all three FQs were found to induce DNA damage and elevate acetylcholinesterase activity,suggesting distinct genotoxic and neurotoxic effects.Interestingly,despite its low bioaccumulation potential,LEVO exhibited high toxicity towards B.aeruginosa.These findings enhance our understanding of the ecotoxicity of FQs in sediments,providing further evidence of their potential ecological risks.
基金supported by Shaanxi Key Research and Development Program(No.2024SF-YBXM-546)the National Natural Science Foundation of China(No.52470161)the State Key Laboratory of Pollution Control and Resource Reuse Foundation(No.PCRRF21007).
文摘With the legislative development,the organic and inorganic composition separation has become the primary requirement for sewer sediment disposal,however the relevant technology has been rarely reported and the driving mechanism was still unclear.In this study,direct disintegration of biopolymers and indirect broken of connection point were investigated on the hydrolysis and component separation.Three typical sewer sediment treatment approaches,i.e.,alkaline,thermal and cation exchange treatments were proposed,which represented the hydrolysis-driving forces of chemical hydrolysis,physical hydrolysis and innovative cation bridging break-age.The results showed that the organic and inorganic separation rates of sewer sediment driven by alkaline,thermal and cation exchange treatments reached 21.26%,23.80%,and 19.56%-48.0%,respectively,compared to 4.43%in control.The secondary structure of proteins was disrupted,transitioning from𝛼α-helix to𝛽β-turn and random coil.Meanwhile,much biopolymers were released from solid to the liquid phase.From thermody-namic perspective,sewer sediment deposition was controlled by short-range interfacial interactions described by extended Derjaguin-Landau-Verwey-Overbeek theory.Additionally,the separation of organic and inorganic components was positively correlated with the thermodynamic parameters(Corr=0.87),highlighted the robust-ness of various driving forces.And the flocculation energy barriers were 2.40(alkaline),1.60 times(thermal),and 4.02–4.97 times(cation exchange)compared to control group.The findings revealed the contrition differ-ence of direct disintegration of gelatinous biopolymers and indirect breakage of composition connection sites in sediment composition separation,filling the critical gaps in understanding the specific mechanisms of sediment biopolymer disintegration and intermolecular connection breakage.
基金support in the literature analysis.This study has been carried out in the framework of the project funded by EU entitled“Bioremediation of contaminated sediments in coastal areas of exindustrial sites-LIFE SEDREMED”(No.LIFE20 ENV/IT/000572).
文摘This study compares the environmental sustainability of five alternatives for the remediation of marine sediments of one of the most polluted coastal sites in Europe(Bagnoli-Coroglio bay,Mediterranean Sea),using the Life Cycle Assessment(LCA)methodology.The treatments are either in-situ or exsitu,the latter requiring an initial dredging to transport the contaminated sediments to the management site.More in detail,four ex-situ remediation technologies based on landfilling,bioremediation,electrokinetic technique and soil washing were identified.These technologies are compared to an in-situ strategy currently under validation for enhancing bioremediation of the polluted sediments of the Bagnoli-Coroglio site.Our results indicate that the disposal in landfilling site is the worst option in most categories(e.g.,650 kg CO_(2) eq./t of treated sediment,considering the nearest landfilling site),followed by the bioremediation,mainly due to the high energy demand.Electrokinetic remediation,soil washing,and innovative in-situ technology represent the most sustainable options.In particular,the new in-situ technology appears to be the least impacting in all categories(e.g.,54 kg CO_(2) eq./t of treated sediment),although it is expected to require longer treatment time(estimated up to 12 months based on its potential efficiency).It can reduce the impact on climate change more than 12 times compared to the disposal and 7 times compared to bioremediation in addition to the possibility to avoid/reduce the dredging operations and the consequent dispersion of pollutants.The results open relevant perspectives towards more eco-sustainable and costly effective actions for the reclamation of contaminated marine sediments.
基金supported by the National Natural Science Foundation of China(Nos.42307524,and 51879103).
文摘China’s lakes are plagued by cadmium(Cd)pollution.Dissolved organic matter(DOM)significantly regulates Cd(II)transport properties at the sediment-water interface.Understanding the effects of different DOM components on the transportation properties of Cd(II)at the sediment-water interface is essential.In this study,typical DOM from different sources was selected to study Cd(II)mobility at the sediment-water interface.Results showed that terrestrial-derived DOM(fulvic acids,FA)and autochthonous-derived DOM(α-amylase,B1)inhibit Cd(II)sequestration by sediments(42.5%and 5.8%,respectively),while anthropogenic-derived DOM(sodium dodecyl benzene sulfonate,SDBS)increased the Cd(II)adsorption capacity by sediments by 2.8%.Fluorescence quenching coupling with parallel factor analysis(EEM-PARAFAC)was used to characterize different DOM components.The results showed that FA contains three kinds of components(C1,C3:protein-like components,C2:humic-like components);SDBS contains two kinds of components(C1,C2:protein-like components);B1 contains three kinds of components(C1,C2:protein-like components,C3:humic-like components).Three complex reaction modelswere used to characterize the ability of Cd(II)complex with DOM,and it was found that the humic-like component could hardly be complex with Cd(II).Accordingly,humic-like components compete for Cd(II)adsorption sites on the sediment surface and inhibit Cd(II)adsorption fromsediments.Fourier transform infrared spectroscopy(FTIR)of the sediment surface before and after Cd(II)addition was analyzed and proved the competitive adsorption theory.This study provides a better understanding of the Cd(II)mobilization behavior at the sediment-water interface and indicates that the input of humic-like DOM will increase the bioavailability of Cd.
基金supported by the National Key Research and Development Program of China(Nos.2023YFC2809304 and 2022YFC2805904).
文摘Obtaining high-quality 10000-meter-deep seafloor sediment samples is the prerequisite and foundation for conducting deep-sea geological and environmental scientific research.The bottom structure of the deep seafloor is complex,and the physical and mechanical properties and disturbance resistance of sediments of different lithologies vary greatly,so the sediment sampler inevitably disturbs the sediments during the sampling process and affects the quality of the sediment samples.A new type of deep-sea sediment pressure retaining sampler is introduced,the force state and elastic–plastic state of the sampler destroying sediments are analyzed,the radial disturbance model of sediment coring based on the spherical cavity expansion theory is established,and the radius of sediments undergoing plastic deformation around the spherical holes is used as an index for evaluating the radial disturbance of sediments.The distribution of stress and strain fields in the sediments during the expansion of the spherical cavity and the influencing factors of the radius of the radially disturbed region(plastic region)are analyzed using an arithmetic example,and the influence law is analyzed.A sediment disturbance experimental platform was built indoors to simulate the sediment coring process.The radial stress field and pore water pressure of the sediment during the coring process were monitored by sensors arranged inside the sediment,and the results of indoor tests verified the correctness of the perturbation theory model.The sampler was carried aboard the deep-sea manned submersible FENDOUZHE and conducted on-site tests at depths of 9298.4 and 9142.8 m in the Kuril-Kamchatka Trench.Pressure-preserved sediment samples were retrieved,with preservation rates of 94.21%and 92.02%,respectively,which are much higher than the current technical indicator of 80%of pressure-holding ratio for deep-sea sediments.The retrieved sediments have obvious stratification characteristics and little disturbance.
基金supported by the National Key R&D Program of China(No.2022YFC2803900)the National Natural Science Foundation of China(No.42276191)Zhejiang University Students Science and Technology Innovation Activity Plan(New Talent Plan)(No.2024R401185).
文摘The spatiotemporal characterization of plume sedimentation and microorganisms is critical for developing plume ecological monitoring model.To address the limitations of traditional methods in obtaining high-quality sediment,a novel sampling system with 6000 m operational capability and three-month endurance was developed.It is equipped with three sediment samplers,a set of formaldehyde preservation solution injection devices.The system is controlled by a low-power,timing-triggered controllers.To investigate low-disturbance rheological mechanisms,gap controlled rheological tests were conducted to optimize the structural design of the sampling and sealing assembly.Stress-controlled shear rheological tests were employed to investigate the mechanisms governing yield stress in sediments under varying temperature conditions and boundary roughness.Additionally,the coupled Eulerian-Lagrangian(CEL)method and sediment rheological constitutive models were employed to simulate tube-soil interaction dynamics and sediment disturbance.The radial heterogeneity of sediment disturbance and friction variation of the sampling tube were revealed.The tube was completely“plugged”at a penetration depth of 261 mm,providing critical data support to the penetration depth parameters.The deep-sea pressure test and South China Sea field trials demonstrated the system’s capability to collect and preserve quantitative time-series sediment samples with high fidelity.
基金supported by National Natural Science Foundation of China(Grant Nos.42072126,42372139)the Natural Science Foundation of Sichuan Province(Grant Nos.2022NSFSC0990).
文摘Fine-grained sediments are widely distributed and constitute the most abundant component in sedi-mentary systems,thus the research on their genesis and distribution is of great significance.In recent years,fine-grained sediment gravity-flows(FGSGF)have been recognized as an important transportation and depositional mechanism for accumulating thick successions of fine-grained sediments.Through a comprehensive review and synthesis of global research on FGSGF deposition,the characteristics,depositional mechanisms,and distribution patterns of fine-grained sediment gravity-flow deposits(FGSGFD)are discussed,and future research prospects are clarified.In addition to the traditionally recognized low-density turbidity current and muddy debris flow,wave-enhanced gravity flow,low-density muddy hyperpycnal flow,and hypopycnal plumes can all form widely distributed FGSGFD.At the same time,the evolution of FGSGF during transportation can result in transitional and hybrid gravity-flow deposits.The combination of multiple triggering mechanisms promotes the widespread develop-ment of FGSGFD,without temporal and spatial limitations.Different types and concentrations of clay minerals,organic matters,and organo-clay complexes are the keys to controlling the flow transformation of FGSGF from low-concentration turbidity currents to high-concentration muddy debris flows.Further study is needed on the interaction mechanism of FGSGF caused by different initiations,the evolution of FGSGF with the effect of organic-inorganic synergy,and the controlling factors of the distribution pat-terns of FGSGFD.The study of FGSGFD can shed some new light on the formation of widely developed thin-bedded siltstones within shales.At the same time,these insights may broaden the exploration scope of shale oil and gas,which have important geological significances for unconventional shale oil and gas.
基金National Natural Science Foundation of China(52269011,52469008)。
文摘Sediment particles,as one of the key components of drip irrigation technology,significantly affect the service life of emitters and restrict the popularization of drip irrigation technology.Hence,two types of patch drip irrigation emitters,focusing on the anti-clogging performance through the experiment,were investigated.The dynamic variations in the clogging characteristics of emitters,specifically were subjected to statistical analysis.The movement mechanism of emitter clogging and discharging sediment was studied.The effects of emitter structure and position factors on emitter clogging were analyzed.The results show that the pressure-compensated emitter exhibits superior anti-clogging perfor-mance,with a service life that is 227.8%greater than that of the labyrinth channel emitter.A single structural factor cannot completely evaluate the anti-clogging performance of emitters.All factors causing emitter clogging should be considered comprehensively.Emitters contain sensitive sediment prone to clogging,however,significant blockage occurs primarily when the sediment content is elevated.The discharge of sediment,denoted as V90,from the emitter is affected by the accumulative effect of clogged sediment.These results may offer valuable insights for the application and advancement of drip irrigation technology.
文摘This study evaluates the dynamics of trace metals impacts on the ecosystems of the Bartlett Pond, a small shallow wetland pond located in Laredo, Texas by analyzing sediment samples taken from four quadrants of the pond. The concentrations of trace elements in sediment samples are highest for iron (Fe), followed by chromium (Cr), then lead (Pb), with lower concentration of antimony (Sb), cobalt (Co), arsenic (As), cadmium (Cd), and the lowest concentration being thallium (Tl) within Bartlett Pond. The sediment quality of the pond is acceptable for organisms and the environment as trace element concentrations (e.g. As, Cd, Cr, and Pb) are within the probable effect concentration (PEC) of National Ocean and Atmospheric Administration (NOAA) guidelines although the PEC values for Co, Fe, Sb and Tl are not given. Bivariate and multivariate correlation analysis shows that most trace elements exhibit a strong positive correlation among them indicating the same anthropogenic sources and biogeochemical processes control these trace elements concentrations within the pond. We provided a comprehensive snapshot of trace element concentrations in sediments through descriptive analysis, laying the foundation for future environmental risk assessments. Correlation analysis of eight trace elements helped identify relationships, offering insights into pollution sources and potential health impacts. Additionally, univariate and multivariate predictive analyses generated numerous models, extending beyond the interpretation of partial and full regression coefficients. We also included graphical analyses of trace element variations, which are critical for understanding environmental processes and geochemical patterns. These findings advance our understanding about trace metals dynamics in sediments and may be a valuable reference for ecosystems and environmental management of different landscapes.
基金The Fund of National Archaeological Talent Promotion Program of China under contract No.2024-269“2024 Shandong Weihai Underwater Archaeological Survey” program by National Center for Archaeology under contract No. 20243160A0965+2 种基金Fujian Provincial Science and Technology Planning Projects under contract No. 2022L3001Provincial Natural Science Foundation of Fujian under contract No. 2023J01020MEL Internal Program of Xiamen University under contract No. MELRI2303。
文摘Under the background of global climate change, anthropogenic processes have profoundly altered the sources and transport mechanisms of coastal sediments. While previous research has primarily focused on large river delta coasts,the responses of the widely distributed small bays dominated by ocean dynamics, has received comparatively less attention. To address this gap, this study examines the Weihai Bay, located in the northeast of Shandong Peninsula,China. By integrating total organic carbon isotope tracers(δ^(13)C and C/N) with sediment transport modeling, we systematically analyze the spatiotemporal patterns of surface sediment grain size inside and outside the bay, along with their responses to natural and human-induced drivers. Our findings reveal that the sedimentary environment of Weihai Bay is governed by the combined effects of tidal currents, ocean currents, wave activity, and sediment supply. Tidal dynamics dominate the hydrodynamic conditions within the bay, while ocean currents predominate offshore. Surface sediments in the bay are primarily composed of silt, originating from sediments carried by the Yellow Sea Warm Current. These sediments enter the bay through the southern bay mouth under tidal forcing, are redistributed counterclockwise by residual tidal currents, and eventually exit via the northern bay mouth. Coarser sediments in specific areas are primarily controlled by strong wave action and terrestrial inputs. Between 1988 and 2023, Weihai Bay sediments have undergone a noticeable coarsening trend, primarily driven by anthropogenic modifications to sediment supply and hydrodynamic regimes. Coastal reclamation, shoreline modification, and infrastructure development have intensified coarse-grained terrestrial sediment input. Concurrently, shoreline advancement has reduced wave dissipation, enhancing nearshore hydrodynamics and accelerating sediment coarsening. This study highlights the sensitivity of small bay sedimentary environments to anthropogenic forcing, advancing our understanding of the coupled human-marine sediment system and providing a scientific basis for coastal sediment evolution under the dual influences of climate change and human activity.
基金Supported by the CNPC Major Science and Technology Project(2021DJ1806).
文摘Based on recent advancements in shale oil exploration within the Ordos Basin,this study presents a comprehensive investigation of the paleoenvironment,lithofacies assemblages and distribution,depositional mechanisms,and reservoir characteristics of shale oil of fine-grained sediment deposition in continental freshwater lacustrine basins,with a focus on the Chang 7_(3) sub-member of Triassic Yanchang Formation.The research integrates a variety of exploration data,including field outcrops,drilling,logging,core samples,geochemical analyses,and flume simulation.The study indicates that:(1)The paleoenvironment of the Chang 7_(3) deposition is characterized by a warm and humid climate,frequent monsoon events,and a large water depth of freshwater lacustrine basin.The paleogeomorphology exhibits an asymmetrical pattern,with steep slopes in the southwest and gentle slopes in the northeast,which can be subdivided into microgeomorphological units,including depressions and ridges in lakebed,as well as ancient channels.(2)The Chang 7_(3) sub-member is characterized by a diverse array of fine-grained sediments,including very fine sandstone,siltstone,mudstone and tuff.These sediments are primarily distributed in thin interbedded and laminated arrangements vertically.The overall grain size of the sandstone predominantly falls below 62.5μm,with individual layer thicknesses of 0.05–0.64 m.The deposits contain intact plant fragments and display various sedimentary structure,such as wavy bedding,inverse-to-normal grading sequence,and climbing ripple bedding,which indicating a depositional origin associated with density flows.(3)Flume simulation experiments have successfully replicated the transport processes and sedimentary characteristics associated with density flows.The initial phase is characterized by a density-velocity differential,resulting in a thicker,coarser sediment layer at the flow front,while the upper layers are thinner and finer in grain size.During the mid-phase,sliding water effects cause the fluid front to rise and facilitate rapid forward transport.This process generates multiple“new fronts”,enabling the long-distance transport of fine-grained sandstones,such as siltstone and argillaceous siltstone,into the center of the lake basin.(4)A sedimentary model primarily controlled by hyperpynal flows was established for the southwestern part of the basin,highlighting that the frequent occurrence of flood events and the steep slope topography in this area are primary controlling factors for the development of hyperpynal flows.(5)Sandstone and mudstone in the Chang 7_(3) sub-member exhibit micro-and nano-scale pore-throat systems,shale oil is present in various lithologies,while the content of movable oil varies considerably,with sandstone exhibiting the highest content of movable oil.(6)The fine-grained sediment complexes formed by multiple episodes of sandstones and mudstones associated with density flow in the Chang 7_(3) formation exhibit characteristics of“overall oil-bearing with differential storage capacity”.The combination of mudstone with low total organic carbon content(TOC)and siltstone is identified as the most favorable exploration target at present.
基金the National Natural Science Foundation of China(Nos.42206076,42476078)the National Program on Global Change and Air-Sea Interaction(No.GASI-02-SCSCJB01)the China-Malaysia Cooperation Project‘Effect on variability of seasonal monsoon on sedimentary process in Peninsular Malaysia waters’。
文摘The Malacca Strait(MS)is a vital conduit for the exchange of water and sediment between the Indian Ocean and the Pacific Ocean,serving as a critical‘gateway'for sediment transport.Here,we present the geochemical characteristics of surface sediments in the MS to elucidate the relationship between terrestrial material inputs and modern oceanic dynamic transport processes in the strait.The results reveal that the MS can be divided into three distinct geochemical provinces.ProvinceⅠ,located in the central region of the strait,is characterized by residual deposits.The preservation of these residual deposits can be attributed to the restricted sediment supply and the relatively weaker modern sedimentary hydrodynamic conditions.ProvinceⅡ,situated to the north of ProvinceⅠ,exhibits provenance differences between its southern and northern regions.The northern region is primarily supplied by sediments originating from the eastern shelf of the Andaman Sea,whereas sediments derived from Sumatra and the Sunda Shelf are predominantly deposited in the southern part of ProvinceⅡ.ProvinceⅢextends along the western coast of the Malaysian Peninsula,with sediments primarily sourced from the Malaysian Peninsula and the Sunda Shelf,while contributions from Sumatra and the eastern shelf of the Andaman Sea are negligible.River sediments from the Malaysian Peninsula and Sumatra are transported northwestward along their respective coasts by prevailing currents,which also facilitate the transportation of Sunda Shelf sediments within the strait,while sediments from the eastern shelf of the Andaman Sea are delivered to the MS via southward coastal currents during the southwest monsoon period.The southward currents and well-developed eddies potentially impede the northward transport of sediments from the Sunda Shelf and restrict the distribution of Andaman Sea sediments within the strait.This study substantially enhances the understanding of source-to-sink processes in the Indo-Pacific region.
基金supported by the Project of Ecological and Environmental Protection Integration Research Institute in Yangtze River Delta(No.ZX2023SZY118)the Special Basic Research Service for the Central Level Public Welfare Research Institute(No.GYZX230409)+1 种基金the National Natural Science Foundation of China(No.42407557)the Belt and Road Special Foundation of the National Key Laboratory of Water Disaster Prevention,China(No.2023491611)。
文摘Organic phosphorus(OP)constitutes an important fraction of total phosphorus in lake sediments,with its mobility being influenced by mineralization and transformation of organic carbon(OC).OP and OC co-exist in various forms in the environment,thus a thorough investigation on the impact of OC fractions on the release of OP in sediments should be comprehensively carried out.This study determined the chemical forms of OP and OC in the sediments over four seasons in Lake Taihu and found temporal and spatial variations in their concentrations.The concentration of total OP and total OC ranged from 133 to 348 mg/kg and 4.77 to 21.19 mg/kg,respectively.Correlation between chemical fractions of OP and OC also revealed that Na OH-extracted OP,and fulvic acid-bound and humic acid-bound OP were positively correlated with humic-OC and hot hydrolysis-OC.These results suggest that the algal-derived OC degradation and mineralization may enhance OP mineralization,converting stable or moderately active OP into active forms or inorganic phosphorus under cyanobacterial bloom.This study provides insight and guiding support for investigating the impact of organic matter components on the transformation of OP after cyanobacterial degradation in eutrophic lakes.
基金financially supported by the National Natural Science Foundation of China(No.U2244225)the Fundamental Research Funds for the Central Universities,China University of Geosciences and China Geological Survey(No.DD20211391)。
文摘Mangrove wetlands are a vital component of the blue carbon ecosystem,which is of great significance to coastal ecosystems and the global carbon balance.However,mangrove forests worldwide face a combination of natural and anthropogenic threats.This study employs highresolution sedimentology,geochemistry,and pollen analysis to reveal the sedimentary evolution and vegetation succession in the mangrove wetland of Dongzhai Harbor,Hainan Island.By utilizing multiple proxies,including^(14)C chronology,δ^(13)C,C/N,and the chemical index of alteration(CIA),we identified three distinct stages in the sedimentary records spanning from the Late Pleistocene to the modern age.Prior to the last glaciation,during the Late Pleistocene,the study area exhibited marine carbonate facies,with an abundance of marine-derived organic matter.During the low sea-level stage of the last glaciation,the strata in the core location were exposed.Following the last glaciation,the study area gradually transitioned into intertidal settings in response to fluctuating sea levels.Since the Middle Holocene or even earlier,sedimentary organic matter continued to accumulate as terrestrial C3 vegetation and mangrove forests established,persisted,and developed.This period witnessed the formation of the current estuarine environment.Simultaneously,the pioneering mangrove species,probably represented by Avicennia,might be initially established,followed by Rhizophora,Bruguiera and Ceriops communities,ultimately being replaced by Kandelia obovata to date.These findings not only fill the gap in the study of paleo-mangroves in China but also contribute valuable knowledge to the global reconstruction of paleo-mangroves,providing crucial reference for the conservation of mangroves and prediction of their responses in the context of climate change.
基金the Laoshan Laboratory(No.LSKJ202203901)the Natural Science Foundation of Shandong Province,China(No.ZR2021MD079)+1 种基金the APEC Cooperation Fund(No.WJ1323001)the Asian Cooperation Fund(Nos.WJ1223001,WJ0923015)。
文摘To explore the relationship of microplastic pollution in different media in marine environment,microplastics in the surface seawater and sediments of Laizhou Bay,Bohai Sea,North China,were studied.Seawater samples were collected using a pre-concentrator equipped with a 20-μm mesh size sieve,and sediment samples were collected by a box sampler.The shape,color,size,and type of microplastics were obtained by a stereomicroscope and a Fourier transform infrared spectrometer(ATR-μ-FT-IR).Results show that the abundance of microplastics in the surface seawater of Laizhou Bay was 858.3±573.2 items/m~3,and that of microplastics in sediments was 151.0±77.4 items/kg dry weight(d.w.)The microplastics in seawater and sediments were mainly fibrous.Meanwhile,the microplastics in seawater were mainly transparent,and those in sediments were transparent and blue.The highest proportion of microplastics in seawater was rayon(77.48%),followed by polyethylene terephthalate(PET,13.17%).The highest proportion of microplastics in sediments was rayon(73.66%),followed by PET(8.90%).The size of microplastics in 1000-2000μm accounted for the largest proportion of 28.54%in seawater,while that in 500-1000μm took 27.93%in sediment.Microplastics in seawater and sediment showed medium-level pollution.In seawater,microplastic abundance was higher in offshore and nearshore areas of Weifang.In sediment,microplastic abundance was higher in offshore and nearshore areas of Dongying.The results of the principal component analysis(PCA)indicated that microplastics in sediment exhibited greater stability compared to those in seawater.The microplastics in seawater and sediment show a positive correlation in terms of shape and plastic type,while exhibiting a negative correlation in terms of color.Overall,microplastics in sediments were smaller in size,and those in seawater and sediments had consistent size distribution characteristics in space.
基金supported by the National Research Foundation of Korea(NRF)grant funded by the Korean government(MSIT)(Grant No.2022R1A2C2091517).
文摘Understanding the sedimentation and simultaneous consolidation behavior of xanthan gum(XG)-biopolymer-treated soils remains a significant research gap in developing environmentally friendly ground-improvement techniques for geotechnical applications.This study addresses this gap by conducting laboratory experiments on kaolinite suspensions with varying XG-to-kaolinite mass ratios(mb/ms).The results showed that the XG treatment modified the sedimentation patterns by promoting larger floc formation and accelerated settling.Additionally,the XG treatment enhanced the shear stiffness and shear strength,particularly at shallow depths.At mb/ms ratios less than 1%,the volume compression was reduced by the XG;the coefficient of compressibility decreased by 49%at 1%mb/ms,and the consolidation was accelerated,as indicated by a 387%increase in the hydraulic conductivity at 0.5%mb/ms under the vertical effective stress of 40 kPa.Contrastingly,at mb/ms ratios greater than 1%,viscous XG hydrogels clogged pores,resulting in a 45%reduction in the coefficient of consolidation at 2%mb/ms under a vertical effective stress of 15 kPa and a 35%decrease in the hydraulic conductivity at 2%mb/ms under a vertical effective stress of 40 kPa.These findings underscore the potential of XG treatment in improving the sedimentation and consolidation processes,highlighting its applicability in geotechnical projects,such as dredging,landfilling,and artificial island construction.
基金The Natural Science Foundation of China under contract Nos 41806130 and 42407149the National Science Foundation for Post-doctoral Scientists of China under contract No.2024M750629+2 种基金the Natural Science Foundation of Guangdong Province under contract No.2018A0303130063the Marine Ecological Survey and Evaluation in Guangdong Province under contract No.0877-23GZTP01F179the Project of the Marine Geological Survey Program of China Geological Survey under contract Nos DD20230460,DD20242792,DD20211394,and DD20190308.
文摘The contamination and accumulation of microplastics(MPs)in mangrove ecosystems have become an increasing concern due to their potential ecological risks.This study investigated and analyzed the abundance of MPs in sediments,water,and benthos of mangrove areas(MA)and adjacent non-vegetated areas(NA)in Qinglan Bay.Results showed that the abundance of MPs in MA was significantly higher than in adjacent NA[sediment:(4.39±2.20)items/50 g dry weight(dw)vs.(4.10±2.71)items/50 g dw;water:(11.79±7.61)items/L vs.(10.61±5.93)items/L;benthos:(4.94±5.27)items/individual vs.(3.5±0.71)items/individual].The primary components identified in sediments and benthos were rayon and cellulose,while polyethylene(PE)and polypropylene(PP)dominated in water.Smaller MPs(<1000μm)accounted for 44%,43%,and 61%of the MPs in sediments,water,and benthos,respectively,indicating that smaller MPs are more likely to be ingested or captured by benthic organisms.Additionally,MPsenrichment was calculated in benthos[enrichment index(EI)=1.41],water(EI=1.11),and sediments(EI=1.09),confirming that the unique ecological environment of the MA leads to different distribution and accumulation characteristics of MPs compared to the NA.The ecological risk assessment revealed low MPs pollution levels in sediments and water,but higher risks were observed for polychaetes and bivalves.
基金Supported by the Southern Marine Science and Engineering Guangdong Laboratory、Zhanjiang(No.ZJW-2019-08)APN、CRRP2019-09MYOnodera、Shinichi Onodera、and the SCS Scholar Grant(No.002029002008/2019)。
文摘Plastic pollution and microplastics in sediments are a growing concern for marine ecosystems worldwide.We examined the vertical distribution and properties of microplastics in beach sediments of Xuwen Coral Reef National Nature Reserve,in Leizhou Peninsula,Zhanjiang,China.Sediment samples were taken in seven locations at 5-cm intervals from the surface to a depth of 30 cm.The vertical distribution of microplastic particles ranged from 0 to 1340 particles per kg on average of 119.05particles per kg.The most prevalent material was fibers(76%),followed by film(12%),fragments(11.2%),and foam(0.8%).The microplastics in size of 1-2 mm constituted the largest percentage(40%)of the total,followed by those in size of<1 mm(26.4%),2-3 mm(21.2%),3-4 mm(9.6%),and 4-5 mm(2.81%).Site S1 observed maximum sizes between 1 and 2 mm,S2 reported higher availability of microplastics with sizes ranging from 0.3 to 1 mm.Six different types of polymers were identified in the investigation,and mostly were polyethylene(PE)and polypropylene(PP).In general,the observation of microplastics in deeper sediments indicates that they have the ability to last for prolonged periods in the marine environment,which may present long-term hazards to benthic creatures.In conclusion,the discovery of microplastics in deep layers of coastal sediments highlights the necessity of minimizing plastic waste and enhancing management strategies to safeguard marine environments.
基金supported by the National Natural Science Foundation(Nos.52000024 and 41907335)the Natural Science Foundation of Shanghai(No.23ZR1400700).
文摘The arsenic(As)release from sediments in great lakes is affected by various factors.In this study,the characteristics of As release fromsediments was investigated,and the As sources and sinks with the strengths in sediments from different areas(grass-type,algae-type,and grass-algae alternation areas)in great shallow lakes(Taihu Lake,China)were analyzed,and the influence of P competition in the process of As release was also studied.The results showed that changing trend of the values of equilibrium As concentration in sediments were consistent with the regional changes(0 to 28.12μg/L),and the sediments from algaetype areas had the higher values.The sediments from western lake and northwest lake bay were a strong As and a weak P source,and the north lake bay had the opposite trend of these two regions.Intense P source competition with As from the sediments occurred in algae-type areas.The grass-type areas had strong As and P retention capacities,indicating a sink role of sediment with high As and P sorption capacities.The degree of As and P saturation had similar trend in sediments,and the grass-type areas had the higher values,18.3%-21.4%and 15.31%-20.34%,respectively.Contribution analysis results showed that most of As release contribution was from the bottom(30-50 cm)sediments,and the surface(0-10 cm)sediments from algae-type areas contributed more to the overlying water than other region.
