Founded in September 2020,the International SparkLink Alliance(iSLA)now has approximately 1,200 members in diverse sectors including terminals,homes,vehicles,manufacturing,transportation,finance and healthcare.The iSL...Founded in September 2020,the International SparkLink Alliance(iSLA)now has approximately 1,200 members in diverse sectors including terminals,homes,vehicles,manufacturing,transportation,finance and healthcare.The iSLA has established a technical standards system for wireless short-range communication covering full-stack standards such as the end-to-end protocol system.展开更多
Geodetic observations over the past several decades identify the Tien Shan as a prominent and active intracontinental mountain belt,characterized by a meridional shortening rate of up to 20 mm/a.The region has experie...Geodetic observations over the past several decades identify the Tien Shan as a prominent and active intracontinental mountain belt,characterized by a meridional shortening rate of up to 20 mm/a.The region has experienced significant seismic events,particularly along its northern boundary,highlighting the recurrent seismic activity in the Kyrgyz Republic.The Issyk-Ata fault,stretching 120 km from west to east in the northern Tien Shan,bounds from the north a young,growing anticline demarcating the foothills of the Kyrgyz Range and the Chui depression.This region is susceptible to strong earthquakes,posing a significant threat to the Chui region and Bishkek,the capital city with over a million residents.The youngest fault in the area is the Issyk-Ata fault,traversing the southern part of Bishkek,where modern construction has obscured its features.This study integrates remote sensing,detailed fieldwork,and paleoseismological investigations to map and analyze surface ruptures,quantify vertical displacements,and assess seismic hazards along the Issyk-Ata fault.Using optically stimulated luminescence and radiocarbon dating,we determined ages for documented paleoseismic events,placing two ancient earthquakes in the Holocene.Magnitude estimates suggest seismic events with magnitudes ranging from 6.6 to 7.1.In the Dzhal area,geological and geomorphological analysis yielded a longterm fault-slip rate of 1.15 mm/a.The Issyk-Ata fault shows variable rupture behavior,with distinct segments demonstrating different seismic characteristics and histories of activity.This variability necessitates comprehensive seismic hazard modeling to better understand and mitigate potential risks in the region.展开更多
The Cenozoic source-to-sink history of the Qaidam Basin is crucial for understanding of the basin-filling architecture,mountain-building processes and even the dynamics of the Tibetan Plateau growth.However,the proven...The Cenozoic source-to-sink history of the Qaidam Basin is crucial for understanding of the basin-filling architecture,mountain-building processes and even the dynamics of the Tibetan Plateau growth.However,the provenance history of Cenozoic strata in the Qaidam Basin remains ambiguous,especially in the northern Qaidam Basin.This controversy highlights the importance of obtaining the spatial source-to-sink relationships between the Qaidam Basin and its surrounding mountain ranges.In this study,we investigated the detrital zircon U-Pb ages of modern fluvial systems draining the East Kunlun Mountain.Their detrital zircon age distributions fall into five age groups:300-190,530-360,1000-560,2000-1100 and 2650-2000 Ma.The dominant age groups are 530-360 and 300-190 Ma,which represent the successive subduction of the Proto-Tethys and PaleoTethys Oceans and the subsequent continental collisions,respectively.Combining these new detrital zircon U-Pb ages with available age datasets,we finally obtained complete detrital zircon age information for modern fluvial systems in the whole Qaidam Basin.The U-Pb age distributions of modern river sands reveal that the zircon age signature of basement rocks in the East Kunlun Mountain is significantly different from that in the South Qilian Mountain but is similar to that in the Altyn Tagh Mountain.Moreover,these zircon age observations were confirmed by the significant difference in the Nd isotopic signature of modern river sands,which reveals a significant difference between the East Kunlun Mountain and South Qilian Mountain in the formation and evolution process.展开更多
The surface of sequence boundary is a negative record. Its recognition largely depends on the physics of the sediments below and above the boundaries, or on the different sedimentary structures are synthetic marks for...The surface of sequence boundary is a negative record. Its recognition largely depends on the physics of the sediments below and above the boundaries, or on the different sedimentary structures are synthetic marks for the sedimentation and tectonic movements in the sedimentary basin. The Qiangtang Basin that is in 5000m above the sea level is located in Northern Tibet. The Lazhulung—Jinshajiang suture zone now bound it to the north and the Bangong—Nujiang suture zone to the south. Three second\|order tectonic units have been distinguished, i.e. North Qiangtang depression, Central rise and South Qiangtang depression from north to south.The Upper Permian Riejuichaka Formation is built up of mudstone and mud\|limestone, which is represented by sediments in seamarsh. The Lower Triassic Kuanglu Formation, which exhibits the structure unconformable contact with the overlying Upper Permian strata, is characterized by terrigenous clastic rocks in the lower area and is carbonate rocks in the upwarding area and the Middle Triassic Kuangnan Formation. The Upper Triassic Xiachaka Formation consisting of terrigenous clastic rocks, carbonates rocks and mixed sediments, is confined to the uplift zones. The lower Jurassic volcanic rocks are deposited in continental rift. The middle and Upper Jurassic Yangshiping Group are conformable contact and assembled by the gypsum\|bearing terrigenous clastic rock formations and carbonate rock formation. The Middle Cretaceous and the Paleocene strata is built up of the terrigenous clastic rock formations.展开更多
During the Late Mesozoic Middle Jurassic--Late Cretaceous, basin and range tectonics and associated magmatism representative of an extensional tectonic setting was widespread in southeastern China as a result of Pacif...During the Late Mesozoic Middle Jurassic--Late Cretaceous, basin and range tectonics and associated magmatism representative of an extensional tectonic setting was widespread in southeastern China as a result of Pacific Plate subduction. Basin tectonics consists of post-orogenic （Type I） and intra-continental extensional basins （Type II）. Type I basins developed in the piedmont and intraland during the Late Triassic to Early Jurassic, in which coarse-grained terrestrial clastic sediments were deposited. Type II basins formed during intra-continental crustal thinning and were characterized by the development of grabens and half-grabens. Graben basins were mainly generated during the Middle Jurassic and were associated with bimodal volcanism. Sediments in half-grabens are intercalated with rhyolitic tufts and lavas and are Early Cretaceous in age with a dominance of Late Cretaceous-Paleogene red beds. Ranges are composed of granitoids and bimodal volcanic rocks, A-type granites and dome-type metamorphic core complexes. The authors analyzed lithological, geochemical and geochronological features of the Late Mesozoic igneous rock assemblages and proposed some geodynamical constraints on forming the basin and range tectonics of South China. A comparison of the similarities and differences of basin and range tectonics between the eastern and western shores of the Pacific is made, and the geo- dynamical evolution model of the Southeast China Block during Late Mesozoic is discussed. Studied results suggest that the basin and range terrane within South China developed on a pre-Mesozoic folded belt was derived from a polyphase tectonic evolution mainly constrained by subduction of the western Pacific Plate since the Late Mesozoic, leading to formation of various magmatism in a back-arc exten- sional setting. Its geodynamic mechanism can compare with that of basin and range tectonics in the eastern shore of the Pacific. Differences of basin and range tectonics between both shores of the Pacific, such as mantle plume formation, scales of extensional and igneous rock assemblages and the age of basin and range tectonics, were caused mainly by the Yellowstone mantle plume in the eastern shore of the Pacific.展开更多
Air temperature(AT) is a subsystem of a complex climate.Long-range correlation(LRC) is an important feature of complexity.Our research attempt to evaluate AT’s complexity differences in different land-use types in th...Air temperature(AT) is a subsystem of a complex climate.Long-range correlation(LRC) is an important feature of complexity.Our research attempt to evaluate AT’s complexity differences in different land-use types in the Heihe River Basin(HRB) based on the stability and LRC.The results show the following:(1) AT’s stability presents differences in different land-use types.In agricultural land,there is no obvious variation in the trend throughout the year.Whereas in a desert,the variation in the trend is obvious: the AT is more stable in summer than it is in winter,with Ta ranges of [8,20]°C and SD of the AT residual ranges of [0.2,0.7],respectively.Additionally,in mountainous areas,when the altitude is beyond a certain value,AT’s stability changes.(2) AT’s LRC presents differences in different land-use types.In agricultural land,the long-range correlation of AT is the most persistent throughout the year,showing the smallest difference between summer and winter,with the Hs range of [0.8,1].Vegetation could be an important factor.In a desert,the long-range correlation of AT is less persistent,showing the greatest difference between summer and winter,with the Hs range of [0.54,0.96].Solar insolation could be a dominant factor.In an alpine meadow,the long-range correlation of AT is the least persistent throughout the year,presenting a smaller difference between summer and winter,with the Hs range of [0.6,0.85].Altitude could be an important factor.(3) Usually,LRC is a combination of the Ta and SD of the AT residuals.A larger Ta and smaller SD of the AT residual would be conducive to a more persistent LRC,whereas a smaller Ta and larger SD of the AT residual would limit the persistence of LRC.A larger Ta and SD of the AT residual would create persistence to a degree between those of the first two cases,as would a smaller Ta and SD of the AT residual.In addition,the last two cases might show the same LRC.展开更多
The basin-range coupling relation is a leading subject of the modern geology. In geometry, relations of this type include couplings between stretched orogenic belt and down-faulted basin, compressional orogenic belt a...The basin-range coupling relation is a leading subject of the modern geology. In geometry, relations of this type include couplings between stretched orogenic belt and down-faulted basin, compressional orogenic belt and foreland basin, strike-slip orogenic belt and strike-slip basin and so on. Fault chains are the key for these couplings and there are typical examples for all these cases. The North China down-faulted basin is coupled west with the Taihang uplift, east with the Jiao-Liao Mountains, north with the Yanshan orogenic belt and south with the Dabie orogenic belt, that is to say, the central down-faulted basin and the surrounding orogenic belts bear a coupling relation within a uniform dynamistic system. Study shows that the central down-faulted basin and the North China mantle sub-plume structure have a close relation during their formation. Owing to intensive mantle sub-plume uplifting, the bottom of the lithosphere suffered from resistance, which caused the lithosphere of the eastern North China to be heated, thinned and fault-depressed. Meanwhile, mantle rocks that were detached outwards in the shape of mushroom was dissected by surrounding ductile shearing zones, which lead to decompression and unloading to generate hypomagmas, and a series of mantle-branch structures were formed around the down-faulted basin. There is an obvious comparability among these mantle branch structures (orogenic belts), and they have basin-range coupling relations with the central down-faulted basins.展开更多
The characteristics of coal seam development,and the prospects of a favorable coal-forming area,were evaluated for the Liaohe Basin located in China.The Number 3 and Number 9 coal seam thickness series from 60 nearly ...The characteristics of coal seam development,and the prospects of a favorable coal-forming area,were evaluated for the Liaohe Basin located in China.The Number 3 and Number 9 coal seam thickness series from 60 nearly equally spaced bores in the Eastern depression of the Liaohe Basin were examined by a rescaled range analysis.The results indicate that the Hurst exponents of the Number 3 and Number 9 coal seam thickness series are 0.69 and 0.68,respectively.This suggests the presence of persistence.As the bore spacing increases the Hurst exponent of the Number 3 series gradually decreases（H changes from 0.69 to 0.52） and shifts from persistence to randomness.The Hurst exponent of the Number 9 thickness data gradually increases（H changes from 0.68 to 0.91） and always shows the characteristic of persistence.A combination of geological characteristics and the series data allow the conclusion that it is more suitable for the Number 9 coal seam to form in the Northeastern part of the Eastern depression than the Number 3 coal seam.展开更多
Studies show that the Tianshan orogenic belt was built in the late stage of the Paleozoic, as evidenced by the Permian red molasses and foreland basins, which are distributed in parallel with the Tianshan belt, indica...Studies show that the Tianshan orogenic belt was built in the late stage of the Paleozoic, as evidenced by the Permian red molasses and foreland basins, which are distributed in parallel with the Tianshan belt, indicating that an intense folding and uplifting event took place. During the Triassic, this orogenic belt was strongly eroded, and basins were further developed. Starting from the Jurassic, a within-plate regional extension occurred, forming a series of Jurassic-Paleogene extensional basins in the peneplaned Tianshan region. Since the Neogene, a collision event between the Indian and the Eurasian plates that took place on the southern side of the Tianshan belt has caused a strong intra-continental orogeny, which is characterized by thrusting and folding. Extremely thick coarse conglomerate and sandy conglomerate of the Xiyu Formation of Neogene System were accumulated unconformably on the Tianshan piedmont. Studies have revealed that the strong compression caused by the Indian-Eurasian collision had a profound influence over the orogenic belt in the hinterland, and MesozoiC-Cenozoic brittle deformed structures superposed on the ductile deformed Paleozoic rocks. The Mesozoic extensional basins were converted into Cenozoic compressional basins. The deformation in the basins is featured by step thrusts and fault-related folds. Statistics of joints show that the principal compressive stress since the Neogene is in a N-S direction. Meanwhile, owing to the underthrusting of the basin toward the orogenic belt, the Paleozoic strata were thrust on the Meso-Cenozoic rocks as tectonic slices, revealing distinct kinematic features in different geologic units. The basin-range coupling zones are characterized by intensive compression, folding and thrusting, accompanied by local sub-E-W-trending strike-slip faults. In the Tianshan region, Cenozoic thrusting is the most common basin-range coupling mode. The folding and faulting of Mesozoic sedimentary rocks, spontaneous combustion of Jurassic coal layers and formation of sintered rocks, the Cenozoic earthquakes and active faulting, and the unique mosaic pattern of basin-range framework of Xinjiang are all products of tectonism since the Neogene.展开更多
The Laramie River after flowing in a north direction through southeast Wyoming’s Laramie Basin abruptly turns in an east direction to flow across the north-to-south oriented Laramie Range in a bedrock-walled canyon a...The Laramie River after flowing in a north direction through southeast Wyoming’s Laramie Basin abruptly turns in an east direction to flow across the north-to-south oriented Laramie Range in a bedrock-walled canyon and eventually reaches the lower elevation Great Plains and southeast-oriented North Platte River. The North Laramie River, Bluegrass Creek, and North Sybille/Sybille Creek also flow from the Laramie Basin in separate bedrock-walled valleys into the Laramie Range before eventually joining the Laramie River. Bedrock-walled through valleys link the various Laramie Range stream and river crossing valleys and detailed topographic maps were used to determine how this anastomosing bedrock-walled canyon complex and the large escarpment-surrounded Goshen Hole basin (located just to the east of the anastomosing canyon complex) originated. Map evidence shows multiple streams of water must have diverged in the Laramie Basin from the north-oriented Laramie River to enter the Laramie Range before converging in or east of the Laramie Range and also shows how present day through valleys enabled diverging and converging streams of water to cross the Laramie Range. The anastomosing bedrock-walled valley complex studied here extends from north of the North Laramie River valley to south of the North Sybille/Sybille Creek valley. Large volumes of water flowing from the Laramie Basin to the Great Plains are interpreted to have eroded the anastomosing canyon complex and the “downstream” Goshen Hole escarpment-surrounded basin. Headward erosion of the north-oriented Sybille and Chugwater Creek valleys across large sheets of east-oriented water are interpreted to have left the Goshen Hole escarpment-surrounded basin as a large abandoned headcut. A water source was not determined, although a continental ice sheet that deeply eroded and warped the North American continent is considered to be a possible source.展开更多
Continent-continent collision is the most important driving mechanism for the occurrence of various geological processes in the continental lithosphere. How to recognize and determine continent-continent collision, es...Continent-continent collision is the most important driving mechanism for the occurrence of various geological processes in the continental lithosphere. How to recognize and determine continent-continent collision, especially its four-dimensional temporal-spatial evolution, is a subject that geological communities have long been concerned about and studied. Continent-continent collision is mainly manifested by strong underthrusting (subduction) of the underlying block along an intracontinental subduction zone and continuous obduction (thrusting propagation) of the overlying block along the intracontinental subduction zone, the occurrence of a basin-range tectonic framework in a direction perpendicular to the subduction zone and the flexure and disruption of the Moho. On the basis of numerical modeling, the authors discuss in detail the couplings between various amounts and rates of displacement caused by basin subsidence, mountain uplift and Moho updoming and downflexure during obduction (thrusting propagation) and subduction and the migration pattern of basin centers. They are probably indications or criteria for judgment or determination of continent-continent collision.展开更多
Resonant linear and nonlinear properties in terahertz range of 2D materials graphene and silicene placed into a bias magnetic field are investigated theoretically on the base of the quasi-classical kinetic theory. Whe...Resonant linear and nonlinear properties in terahertz range of 2D materials graphene and silicene placed into a bias magnetic field are investigated theoretically on the base of the quasi-classical kinetic theory. When the electromagnetic frequency is close to the cyclotron one, the linear conductivity increases two orders. Under the resonant frequencies nonlinearity becomes essential at low magnitudes of terahertz electric fields. In absence of a bias magnetic field the nonlinear dependences of the surface electric currents on terahertz electric field are practically the same simulated from kinetics and electron hydrodynamics with nonzero “kinetic” electron effective mass. Graphene possesses higher values of nonlinearity of the resonant conductivity, whereas in absence of a bias magnetic field, the electron nonlinearity is higher in silicene.展开更多
The Fringe Projection Profilometry(FPP)system with a single exposure time or a single projection intensity is limited by the dynamic range of the camera,which can lead to overexposure and underexposure of the image,re...The Fringe Projection Profilometry(FPP)system with a single exposure time or a single projection intensity is limited by the dynamic range of the camera,which can lead to overexposure and underexposure of the image,resulting in point cloud loss or reduced accuracy.To address this issue,unlike the pixel modulation method of projectors,we utilize the characteristics of color projectors where the intensity of the three-channel LED can be controlled independently.We propose a method for separating the projector's three-channel light intensity,combined with a color camera,to achieve single exposure and multi-intensity image acquisition.Further,the crosstalk coefficient is applied to predict the three-channel reflectance of the measured object.By integrating clustering and channel mapping,we establish a pixel-level mapping model between the projector's three-channel current and the camera's three-channel image intensity,which realizes the optimal projection current prediction and the high dynamic range(HDR)image acquisition.The proposed method allows for high-precision three-dimensional(3D)data acquisition of HDR scenes with a single exposure.The effectiveness of this method has been validated through experiments with standard planes and standard steps,showing a significant reduction in mean absolute error(44.6%)compared to existing singleexposure HDR methods.Additionally,the number of images required for acquisition is significantly reduced(by 70.8%)compared to multi-exposure fusion methods.This proposed method has great potential in various FPP-related fields.展开更多
Hydrologiska Byrans Vattenbalansavdeling(HBV) Light model was used to evaluate the performance of the model in response to climate change in the snowy and glaciated catchment area of Hunza River Basin. The study aimed...Hydrologiska Byrans Vattenbalansavdeling(HBV) Light model was used to evaluate the performance of the model in response to climate change in the snowy and glaciated catchment area of Hunza River Basin. The study aimed to understand the temporal variation of streamflow of Hunza River and its contribution to Indus River System(IRS). HBV model performed fairly well both during calibration(R2=0.87, Reff=0.85, PBIAS=-0.36) and validation(R2=0.86, Reff=0.83, PBIAS=-13.58) periods on daily time scale in the Hunza River Basin. Model performed better on monthly time scale with slightly underestimated low flows period during bothcalibration(R2=0.94, Reff=0.88, PBIAS=0.47) and validation(R2=0.92, Reff=0.85, PBIAS=15.83) periods. Simulated streamflow analysis from 1995-2010 unveiled that the average percentage contribution of snow, rain and glacier melt to the streamflow of Hunza River is about 16.5%, 19.4% and 64% respectively. In addition, the HBV-Light model performance was also evaluated for prediction of future streamflow in the Hunza River using future projected data of three General Circulation Model(GCMs) i.e. BCC-CSM1.1, CanESM2, and MIROCESM under RCP2.6, 4.5 and 8.5 and predictions were made over three time periods, 2010-2039, 2040-2069 and 2070-2099, using 1980-2010 as the control period. Overall projected climate results reveal that temperature and precipitation are the most sensitiveparameters to the streamflow of Hunza River. MIROC-ESM predicted the highest increase in the future streamflow of the Hunza River due to increase in temperature and precipitation under RCP4.5 and 8.5 scenarios from 2010-2099 while predicted slight increase in the streamflow under RCP2.6 during the start and end of the 21 th century. However, BCCCSM1.1 predicted decrease in the streamflow under RCP8.5 due to decrease in temperature and precipitation from 2010-2099. However, Can ESM2 predicted 22%-88% increase in the streamflow under RCP4.5 from 2010-2099. The results of this study could be useful for decision making and effective future strategic plans for water management and their sustainability in the region.展开更多
Analyses of the soil moisture evolution trend and the influence of different types of radiation on soil moisture are of great significance to the simulation and prediction of soil moisture.In this paper,soil moisture(...Analyses of the soil moisture evolution trend and the influence of different types of radiation on soil moisture are of great significance to the simulation and prediction of soil moisture.In this paper,soil moisture(2–60 cm) and various radiation data from 2014–2015 at the A’rou superstation were selected.The radiation data include the net radiation(NR),shortwave and longwave radiation(SR and LR).Using adaptive fractal analysis(AFA),the long-range correlation(LRC) of soil moisture and long-range cross correlation(LRCC) between moisture and three types of radiation were analyzed at different timescales and soil depths.The results show that:(1) Persistence of soil moisture and consistency between soil moisture and radiation mutate at 18-d and 6-d timescales,respectively.The timescale variation of soil moisture persistence is mainly related to the influence process of radiation on soil moisture;(2) Both the soil moisture persistence and soil moisture-radiation consistency vary substantially with soil depth.The soil depth variation of soil moisture persistence is related to the influence intensity of radiation;(3) From 2–6 day timescales,LR displays the strongest influence on soil moisture at depths of 2–10 cm through negative feedback of radiation on the soil temperature.The influence intensity decreases with depth from 2–15 cm.Therefore,the soil moisture persistence is weak and increases with depth from 2–15 cm;and(4) At more than 6 day timescales,SR and NR display a stronger influence on the soil moisture persistence at depths of 2–40 cm through positive feedback of radiation on the soil temperature,especially at depths of 2–10 cm.This influence also weakens with depth.The soil moisture persistence at depths of 2–10 cm is the weakest and increases with depth from 2–40 cm.The research results are instructive for determining timescales and soil depths related to soil water in hydrological models.展开更多
30 July–14 August 2011,Novosibirsk,Russia Numerous Neoproterozoic sedimentary basins were developed on the Siberian Craton,and the Siberian successions play an important role in the Neoproterozoic biostratigraphy,che...30 July–14 August 2011,Novosibirsk,Russia Numerous Neoproterozoic sedimentary basins were developed on the Siberian Craton,and the Siberian successions play an important role in the Neoproterozoic biostratigraphy,chemostratigraphy,basin dynamics,and petroleum exploration.To take advantage of Siberia’s rich geological and paleobiological heritages.展开更多
PLP City Range项目坐落在曼谷通罗地区一个宁静的高档社区内,是一座为尖端高尔夫模拟中心建造的创新性混合用途建筑。引人注目的建筑立面,采用曲面预制混凝土板正反向拼贴组合而成,兼具美学和功能性。这些造型独特的混凝土模块在自然...PLP City Range项目坐落在曼谷通罗地区一个宁静的高档社区内,是一座为尖端高尔夫模拟中心建造的创新性混合用途建筑。引人注目的建筑立面,采用曲面预制混凝土板正反向拼贴组合而成,兼具美学和功能性。这些造型独特的混凝土模块在自然光下形成光影交织的效果,巧妙地呼应了高尔夫运动挥杆时的优雅弧线,在视觉上呈现这项运动独特的魅力。展开更多
Vibration detection using sensors with both wide working frequency range,good sensitivity,and other good performances is a topic of great interest in fields such as inertial navigation,deep-sea fishing boat engines co...Vibration detection using sensors with both wide working frequency range,good sensitivity,and other good performances is a topic of great interest in fields such as inertial navigation,deep-sea fishing boat engines condition monitoring,seismic monitoring,attitude,and heading reference system,etc.This paper investigates two 6H-SIC MEMS diaphragms,one triangular and the other square,used in a fiber optic Fabry–Perot(FP)accelerometer in an experimental scenario.The triangular chip shows a wide working frequency range of 630 Hz–5300 Hz,a natural frequency of 44.3 k Hz,and a mechanical sensitivity of 0.154 nm/g.An optimal structure of the square chip used in a probe such as a fiber optic FP accelerometer also shows a wide working frequency range of 120 Hz–2300 Hz;a good sensitivity of 31.5 m V/g,a resonance frequency of7873 Hz,an accuracy of 0.96%F.S.,a frequency measurement error of 1.15%,and an excellent linearity of 0.9995.展开更多
Two-dimensional(2D)organic-inorganic hybrid perovskites(OIHPs)have been developed as promising candidates for photodetection,owing to their excellent semiconducting features and structural tunability.However,as an imp...Two-dimensional(2D)organic-inorganic hybrid perovskites(OIHPs)have been developed as promising candidates for photodetection,owing to their excellent semiconducting features and structural tunability.However,as an important parameter for photodetection,the photoresponsive range of 2D OIHPs is usually modulated by finite metal-halide combinations,constraining their further development.The emerging aromatic amine-based alternating-cations-interlayered(A-ACI)hybrid perovskites that exhibit excellent charge transport and additional interlayered structural designability,provide an extra solution for achieving ideal photoresponsive range.Herein,for the first time,the photoresponsive range is successfully broadened in A-ACI hybrid perovskites(NMA)_(4)(FA)_(2)Pb_(3)Br_(12)(2)remolding from(NMA)_(4)(MA)_(2)Pb_(3)Br_(12)(1)(NMA=N-methylbenzylaminium,FA=formamidinium and MA=methylammonium).Particularly,1 and 2adopt an unprecedented configuration that NMA and MA/FA are alternately arranged in the interlayer in a 4:2 manner.Importantly,2 exhibits a narrower bandgap than 1,which can be ascribed to the lowlying conduct band composed of intercalation FAπ*orbitals.Meanwhile,2 possesses a shorter interlayer distance and flatter inorganic skeleton,synergistically facilitating the wider photo-absorption range and further endowing a broadening photoresponsive range(70 nm).This research not only enriches the perovskite family but also provides insights into structure-property relationships.展开更多
文摘Founded in September 2020,the International SparkLink Alliance(iSLA)now has approximately 1,200 members in diverse sectors including terminals,homes,vehicles,manufacturing,transportation,finance and healthcare.The iSLA has established a technical standards system for wireless short-range communication covering full-stack standards such as the end-to-end protocol system.
基金financial support of the Faculty Research Grant project of the American University of Central Asia(AUCA)supported by the Ministry of Education of the Republic of Korea and the National Research Foundation of Korea(NRF-2023S1A5B5A16080131)。
文摘Geodetic observations over the past several decades identify the Tien Shan as a prominent and active intracontinental mountain belt,characterized by a meridional shortening rate of up to 20 mm/a.The region has experienced significant seismic events,particularly along its northern boundary,highlighting the recurrent seismic activity in the Kyrgyz Republic.The Issyk-Ata fault,stretching 120 km from west to east in the northern Tien Shan,bounds from the north a young,growing anticline demarcating the foothills of the Kyrgyz Range and the Chui depression.This region is susceptible to strong earthquakes,posing a significant threat to the Chui region and Bishkek,the capital city with over a million residents.The youngest fault in the area is the Issyk-Ata fault,traversing the southern part of Bishkek,where modern construction has obscured its features.This study integrates remote sensing,detailed fieldwork,and paleoseismological investigations to map and analyze surface ruptures,quantify vertical displacements,and assess seismic hazards along the Issyk-Ata fault.Using optically stimulated luminescence and radiocarbon dating,we determined ages for documented paleoseismic events,placing two ancient earthquakes in the Holocene.Magnitude estimates suggest seismic events with magnitudes ranging from 6.6 to 7.1.In the Dzhal area,geological and geomorphological analysis yielded a longterm fault-slip rate of 1.15 mm/a.The Issyk-Ata fault shows variable rupture behavior,with distinct segments demonstrating different seismic characteristics and histories of activity.This variability necessitates comprehensive seismic hazard modeling to better understand and mitigate potential risks in the region.
基金supported by the Geological Survey of China(No.DD20221645)the National Natural Science Foundation of China(Nos.42171010,42072141,41702118)。
文摘The Cenozoic source-to-sink history of the Qaidam Basin is crucial for understanding of the basin-filling architecture,mountain-building processes and even the dynamics of the Tibetan Plateau growth.However,the provenance history of Cenozoic strata in the Qaidam Basin remains ambiguous,especially in the northern Qaidam Basin.This controversy highlights the importance of obtaining the spatial source-to-sink relationships between the Qaidam Basin and its surrounding mountain ranges.In this study,we investigated the detrital zircon U-Pb ages of modern fluvial systems draining the East Kunlun Mountain.Their detrital zircon age distributions fall into five age groups:300-190,530-360,1000-560,2000-1100 and 2650-2000 Ma.The dominant age groups are 530-360 and 300-190 Ma,which represent the successive subduction of the Proto-Tethys and PaleoTethys Oceans and the subsequent continental collisions,respectively.Combining these new detrital zircon U-Pb ages with available age datasets,we finally obtained complete detrital zircon age information for modern fluvial systems in the whole Qaidam Basin.The U-Pb age distributions of modern river sands reveal that the zircon age signature of basement rocks in the East Kunlun Mountain is significantly different from that in the South Qilian Mountain but is similar to that in the Altyn Tagh Mountain.Moreover,these zircon age observations were confirmed by the significant difference in the Nd isotopic signature of modern river sands,which reveals a significant difference between the East Kunlun Mountain and South Qilian Mountain in the formation and evolution process.
文摘The surface of sequence boundary is a negative record. Its recognition largely depends on the physics of the sediments below and above the boundaries, or on the different sedimentary structures are synthetic marks for the sedimentation and tectonic movements in the sedimentary basin. The Qiangtang Basin that is in 5000m above the sea level is located in Northern Tibet. The Lazhulung—Jinshajiang suture zone now bound it to the north and the Bangong—Nujiang suture zone to the south. Three second\|order tectonic units have been distinguished, i.e. North Qiangtang depression, Central rise and South Qiangtang depression from north to south.The Upper Permian Riejuichaka Formation is built up of mudstone and mud\|limestone, which is represented by sediments in seamarsh. The Lower Triassic Kuanglu Formation, which exhibits the structure unconformable contact with the overlying Upper Permian strata, is characterized by terrigenous clastic rocks in the lower area and is carbonate rocks in the upwarding area and the Middle Triassic Kuangnan Formation. The Upper Triassic Xiachaka Formation consisting of terrigenous clastic rocks, carbonates rocks and mixed sediments, is confined to the uplift zones. The lower Jurassic volcanic rocks are deposited in continental rift. The middle and Upper Jurassic Yangshiping Group are conformable contact and assembled by the gypsum\|bearing terrigenous clastic rock formations and carbonate rock formation. The Middle Cretaceous and the Paleocene strata is built up of the terrigenous clastic rock formations.
基金funded by the National Basic Research Program of China(973 Program,No.2012CB416701)National Natural Science Foundation of China(Grant 40972132)was partly supported by the State Key Laboratory for Mineral Deposits Research of Nanjing University(No.2008-Ⅰ-01)
文摘During the Late Mesozoic Middle Jurassic--Late Cretaceous, basin and range tectonics and associated magmatism representative of an extensional tectonic setting was widespread in southeastern China as a result of Pacific Plate subduction. Basin tectonics consists of post-orogenic （Type I） and intra-continental extensional basins （Type II）. Type I basins developed in the piedmont and intraland during the Late Triassic to Early Jurassic, in which coarse-grained terrestrial clastic sediments were deposited. Type II basins formed during intra-continental crustal thinning and were characterized by the development of grabens and half-grabens. Graben basins were mainly generated during the Middle Jurassic and were associated with bimodal volcanism. Sediments in half-grabens are intercalated with rhyolitic tufts and lavas and are Early Cretaceous in age with a dominance of Late Cretaceous-Paleogene red beds. Ranges are composed of granitoids and bimodal volcanic rocks, A-type granites and dome-type metamorphic core complexes. The authors analyzed lithological, geochemical and geochronological features of the Late Mesozoic igneous rock assemblages and proposed some geodynamical constraints on forming the basin and range tectonics of South China. A comparison of the similarities and differences of basin and range tectonics between the eastern and western shores of the Pacific is made, and the geo- dynamical evolution model of the Southeast China Block during Late Mesozoic is discussed. Studied results suggest that the basin and range terrane within South China developed on a pre-Mesozoic folded belt was derived from a polyphase tectonic evolution mainly constrained by subduction of the western Pacific Plate since the Late Mesozoic, leading to formation of various magmatism in a back-arc exten- sional setting. Its geodynamic mechanism can compare with that of basin and range tectonics in the eastern shore of the Pacific. Differences of basin and range tectonics between both shores of the Pacific, such as mantle plume formation, scales of extensional and igneous rock assemblages and the age of basin and range tectonics, were caused mainly by the Yellowstone mantle plume in the eastern shore of the Pacific.
基金Strategic Priority Research Program of the Chinese Academy of Sciences,No.XDA23100303
文摘Air temperature(AT) is a subsystem of a complex climate.Long-range correlation(LRC) is an important feature of complexity.Our research attempt to evaluate AT’s complexity differences in different land-use types in the Heihe River Basin(HRB) based on the stability and LRC.The results show the following:(1) AT’s stability presents differences in different land-use types.In agricultural land,there is no obvious variation in the trend throughout the year.Whereas in a desert,the variation in the trend is obvious: the AT is more stable in summer than it is in winter,with Ta ranges of [8,20]°C and SD of the AT residual ranges of [0.2,0.7],respectively.Additionally,in mountainous areas,when the altitude is beyond a certain value,AT’s stability changes.(2) AT’s LRC presents differences in different land-use types.In agricultural land,the long-range correlation of AT is the most persistent throughout the year,showing the smallest difference between summer and winter,with the Hs range of [0.8,1].Vegetation could be an important factor.In a desert,the long-range correlation of AT is less persistent,showing the greatest difference between summer and winter,with the Hs range of [0.54,0.96].Solar insolation could be a dominant factor.In an alpine meadow,the long-range correlation of AT is the least persistent throughout the year,presenting a smaller difference between summer and winter,with the Hs range of [0.6,0.85].Altitude could be an important factor.(3) Usually,LRC is a combination of the Ta and SD of the AT residuals.A larger Ta and smaller SD of the AT residual would be conducive to a more persistent LRC,whereas a smaller Ta and larger SD of the AT residual would limit the persistence of LRC.A larger Ta and SD of the AT residual would create persistence to a degree between those of the first two cases,as would a smaller Ta and SD of the AT residual.In addition,the last two cases might show the same LRC.
基金supported by the National Natural Science Foundation of China(grants 40272088,40072073)the Knowledge Innovation Project of the Chinese Academy of Sciences(KZCX1-07)the Project of Large scale Geological Survey in China(200110200038).
文摘The basin-range coupling relation is a leading subject of the modern geology. In geometry, relations of this type include couplings between stretched orogenic belt and down-faulted basin, compressional orogenic belt and foreland basin, strike-slip orogenic belt and strike-slip basin and so on. Fault chains are the key for these couplings and there are typical examples for all these cases. The North China down-faulted basin is coupled west with the Taihang uplift, east with the Jiao-Liao Mountains, north with the Yanshan orogenic belt and south with the Dabie orogenic belt, that is to say, the central down-faulted basin and the surrounding orogenic belts bear a coupling relation within a uniform dynamistic system. Study shows that the central down-faulted basin and the North China mantle sub-plume structure have a close relation during their formation. Owing to intensive mantle sub-plume uplifting, the bottom of the lithosphere suffered from resistance, which caused the lithosphere of the eastern North China to be heated, thinned and fault-depressed. Meanwhile, mantle rocks that were detached outwards in the shape of mushroom was dissected by surrounding ductile shearing zones, which lead to decompression and unloading to generate hypomagmas, and a series of mantle-branch structures were formed around the down-faulted basin. There is an obvious comparability among these mantle branch structures (orogenic belts), and they have basin-range coupling relations with the central down-faulted basins.
基金supported by National Basic Research Program of China(No.2007CB209503)
文摘The characteristics of coal seam development,and the prospects of a favorable coal-forming area,were evaluated for the Liaohe Basin located in China.The Number 3 and Number 9 coal seam thickness series from 60 nearly equally spaced bores in the Eastern depression of the Liaohe Basin were examined by a rescaled range analysis.The results indicate that the Hurst exponents of the Number 3 and Number 9 coal seam thickness series are 0.69 and 0.68,respectively.This suggests the presence of persistence.As the bore spacing increases the Hurst exponent of the Number 3 series gradually decreases（H changes from 0.69 to 0.52） and shifts from persistence to randomness.The Hurst exponent of the Number 9 thickness data gradually increases（H changes from 0.68 to 0.91） and always shows the characteristic of persistence.A combination of geological characteristics and the series data allow the conclusion that it is more suitable for the Number 9 coal seam to form in the Northeastern part of the Eastern depression than the Number 3 coal seam.
基金supports from the National 973 Project on western China No.2001CB409804the key project of National Natural Science Foundation of China No.49832040.
文摘Studies show that the Tianshan orogenic belt was built in the late stage of the Paleozoic, as evidenced by the Permian red molasses and foreland basins, which are distributed in parallel with the Tianshan belt, indicating that an intense folding and uplifting event took place. During the Triassic, this orogenic belt was strongly eroded, and basins were further developed. Starting from the Jurassic, a within-plate regional extension occurred, forming a series of Jurassic-Paleogene extensional basins in the peneplaned Tianshan region. Since the Neogene, a collision event between the Indian and the Eurasian plates that took place on the southern side of the Tianshan belt has caused a strong intra-continental orogeny, which is characterized by thrusting and folding. Extremely thick coarse conglomerate and sandy conglomerate of the Xiyu Formation of Neogene System were accumulated unconformably on the Tianshan piedmont. Studies have revealed that the strong compression caused by the Indian-Eurasian collision had a profound influence over the orogenic belt in the hinterland, and MesozoiC-Cenozoic brittle deformed structures superposed on the ductile deformed Paleozoic rocks. The Mesozoic extensional basins were converted into Cenozoic compressional basins. The deformation in the basins is featured by step thrusts and fault-related folds. Statistics of joints show that the principal compressive stress since the Neogene is in a N-S direction. Meanwhile, owing to the underthrusting of the basin toward the orogenic belt, the Paleozoic strata were thrust on the Meso-Cenozoic rocks as tectonic slices, revealing distinct kinematic features in different geologic units. The basin-range coupling zones are characterized by intensive compression, folding and thrusting, accompanied by local sub-E-W-trending strike-slip faults. In the Tianshan region, Cenozoic thrusting is the most common basin-range coupling mode. The folding and faulting of Mesozoic sedimentary rocks, spontaneous combustion of Jurassic coal layers and formation of sintered rocks, the Cenozoic earthquakes and active faulting, and the unique mosaic pattern of basin-range framework of Xinjiang are all products of tectonism since the Neogene.
文摘The Laramie River after flowing in a north direction through southeast Wyoming’s Laramie Basin abruptly turns in an east direction to flow across the north-to-south oriented Laramie Range in a bedrock-walled canyon and eventually reaches the lower elevation Great Plains and southeast-oriented North Platte River. The North Laramie River, Bluegrass Creek, and North Sybille/Sybille Creek also flow from the Laramie Basin in separate bedrock-walled valleys into the Laramie Range before eventually joining the Laramie River. Bedrock-walled through valleys link the various Laramie Range stream and river crossing valleys and detailed topographic maps were used to determine how this anastomosing bedrock-walled canyon complex and the large escarpment-surrounded Goshen Hole basin (located just to the east of the anastomosing canyon complex) originated. Map evidence shows multiple streams of water must have diverged in the Laramie Basin from the north-oriented Laramie River to enter the Laramie Range before converging in or east of the Laramie Range and also shows how present day through valleys enabled diverging and converging streams of water to cross the Laramie Range. The anastomosing bedrock-walled valley complex studied here extends from north of the North Laramie River valley to south of the North Sybille/Sybille Creek valley. Large volumes of water flowing from the Laramie Basin to the Great Plains are interpreted to have eroded the anastomosing canyon complex and the “downstream” Goshen Hole escarpment-surrounded basin. Headward erosion of the north-oriented Sybille and Chugwater Creek valleys across large sheets of east-oriented water are interpreted to have left the Goshen Hole escarpment-surrounded basin as a large abandoned headcut. A water source was not determined, although a continental ice sheet that deeply eroded and warped the North American continent is considered to be a possible source.
基金the National Natural Science Foundation of China(grant 19972072)Project of the Open Laboratory of Continental Geodynamics of the Ministry of Land and Resources(grant 9812) Stat Project 305 rgrant 96—915—06—04).
文摘Continent-continent collision is the most important driving mechanism for the occurrence of various geological processes in the continental lithosphere. How to recognize and determine continent-continent collision, especially its four-dimensional temporal-spatial evolution, is a subject that geological communities have long been concerned about and studied. Continent-continent collision is mainly manifested by strong underthrusting (subduction) of the underlying block along an intracontinental subduction zone and continuous obduction (thrusting propagation) of the overlying block along the intracontinental subduction zone, the occurrence of a basin-range tectonic framework in a direction perpendicular to the subduction zone and the flexure and disruption of the Moho. On the basis of numerical modeling, the authors discuss in detail the couplings between various amounts and rates of displacement caused by basin subsidence, mountain uplift and Moho updoming and downflexure during obduction (thrusting propagation) and subduction and the migration pattern of basin centers. They are probably indications or criteria for judgment or determination of continent-continent collision.
文摘Resonant linear and nonlinear properties in terahertz range of 2D materials graphene and silicene placed into a bias magnetic field are investigated theoretically on the base of the quasi-classical kinetic theory. When the electromagnetic frequency is close to the cyclotron one, the linear conductivity increases two orders. Under the resonant frequencies nonlinearity becomes essential at low magnitudes of terahertz electric fields. In absence of a bias magnetic field the nonlinear dependences of the surface electric currents on terahertz electric field are practically the same simulated from kinetics and electron hydrodynamics with nonzero “kinetic” electron effective mass. Graphene possesses higher values of nonlinearity of the resonant conductivity, whereas in absence of a bias magnetic field, the electron nonlinearity is higher in silicene.
文摘The Fringe Projection Profilometry(FPP)system with a single exposure time or a single projection intensity is limited by the dynamic range of the camera,which can lead to overexposure and underexposure of the image,resulting in point cloud loss or reduced accuracy.To address this issue,unlike the pixel modulation method of projectors,we utilize the characteristics of color projectors where the intensity of the three-channel LED can be controlled independently.We propose a method for separating the projector's three-channel light intensity,combined with a color camera,to achieve single exposure and multi-intensity image acquisition.Further,the crosstalk coefficient is applied to predict the three-channel reflectance of the measured object.By integrating clustering and channel mapping,we establish a pixel-level mapping model between the projector's three-channel current and the camera's three-channel image intensity,which realizes the optimal projection current prediction and the high dynamic range(HDR)image acquisition.The proposed method allows for high-precision three-dimensional(3D)data acquisition of HDR scenes with a single exposure.The effectiveness of this method has been validated through experiments with standard planes and standard steps,showing a significant reduction in mean absolute error(44.6%)compared to existing singleexposure HDR methods.Additionally,the number of images required for acquisition is significantly reduced(by 70.8%)compared to multi-exposure fusion methods.This proposed method has great potential in various FPP-related fields.
基金the National Natural Science foundation of China(Grant Nos.41690145 and 41670158)
文摘Hydrologiska Byrans Vattenbalansavdeling(HBV) Light model was used to evaluate the performance of the model in response to climate change in the snowy and glaciated catchment area of Hunza River Basin. The study aimed to understand the temporal variation of streamflow of Hunza River and its contribution to Indus River System(IRS). HBV model performed fairly well both during calibration(R2=0.87, Reff=0.85, PBIAS=-0.36) and validation(R2=0.86, Reff=0.83, PBIAS=-13.58) periods on daily time scale in the Hunza River Basin. Model performed better on monthly time scale with slightly underestimated low flows period during bothcalibration(R2=0.94, Reff=0.88, PBIAS=0.47) and validation(R2=0.92, Reff=0.85, PBIAS=15.83) periods. Simulated streamflow analysis from 1995-2010 unveiled that the average percentage contribution of snow, rain and glacier melt to the streamflow of Hunza River is about 16.5%, 19.4% and 64% respectively. In addition, the HBV-Light model performance was also evaluated for prediction of future streamflow in the Hunza River using future projected data of three General Circulation Model(GCMs) i.e. BCC-CSM1.1, CanESM2, and MIROCESM under RCP2.6, 4.5 and 8.5 and predictions were made over three time periods, 2010-2039, 2040-2069 and 2070-2099, using 1980-2010 as the control period. Overall projected climate results reveal that temperature and precipitation are the most sensitiveparameters to the streamflow of Hunza River. MIROC-ESM predicted the highest increase in the future streamflow of the Hunza River due to increase in temperature and precipitation under RCP4.5 and 8.5 scenarios from 2010-2099 while predicted slight increase in the streamflow under RCP2.6 during the start and end of the 21 th century. However, BCCCSM1.1 predicted decrease in the streamflow under RCP8.5 due to decrease in temperature and precipitation from 2010-2099. However, Can ESM2 predicted 22%-88% increase in the streamflow under RCP4.5 from 2010-2099. The results of this study could be useful for decision making and effective future strategic plans for water management and their sustainability in the region.
基金National Key R&D Program of China,No.2017YFB0504102National Natural Science Foundation of China No.41771537
文摘Analyses of the soil moisture evolution trend and the influence of different types of radiation on soil moisture are of great significance to the simulation and prediction of soil moisture.In this paper,soil moisture(2–60 cm) and various radiation data from 2014–2015 at the A’rou superstation were selected.The radiation data include the net radiation(NR),shortwave and longwave radiation(SR and LR).Using adaptive fractal analysis(AFA),the long-range correlation(LRC) of soil moisture and long-range cross correlation(LRCC) between moisture and three types of radiation were analyzed at different timescales and soil depths.The results show that:(1) Persistence of soil moisture and consistency between soil moisture and radiation mutate at 18-d and 6-d timescales,respectively.The timescale variation of soil moisture persistence is mainly related to the influence process of radiation on soil moisture;(2) Both the soil moisture persistence and soil moisture-radiation consistency vary substantially with soil depth.The soil depth variation of soil moisture persistence is related to the influence intensity of radiation;(3) From 2–6 day timescales,LR displays the strongest influence on soil moisture at depths of 2–10 cm through negative feedback of radiation on the soil temperature.The influence intensity decreases with depth from 2–15 cm.Therefore,the soil moisture persistence is weak and increases with depth from 2–15 cm;and(4) At more than 6 day timescales,SR and NR display a stronger influence on the soil moisture persistence at depths of 2–40 cm through positive feedback of radiation on the soil temperature,especially at depths of 2–10 cm.This influence also weakens with depth.The soil moisture persistence at depths of 2–10 cm is the weakest and increases with depth from 2–40 cm.The research results are instructive for determining timescales and soil depths related to soil water in hydrological models.
文摘30 July–14 August 2011,Novosibirsk,Russia Numerous Neoproterozoic sedimentary basins were developed on the Siberian Craton,and the Siberian successions play an important role in the Neoproterozoic biostratigraphy,chemostratigraphy,basin dynamics,and petroleum exploration.To take advantage of Siberia’s rich geological and paleobiological heritages.
文摘PLP City Range项目坐落在曼谷通罗地区一个宁静的高档社区内,是一座为尖端高尔夫模拟中心建造的创新性混合用途建筑。引人注目的建筑立面,采用曲面预制混凝土板正反向拼贴组合而成,兼具美学和功能性。这些造型独特的混凝土模块在自然光下形成光影交织的效果,巧妙地呼应了高尔夫运动挥杆时的优雅弧线,在视觉上呈现这项运动独特的魅力。
基金Project supported by the National Natural Science Foundation of China(Grant No.32473216)Ningbo Youth Science and Technology Innovation Leading Talent Project(Grant No.2023QL004)。
文摘Vibration detection using sensors with both wide working frequency range,good sensitivity,and other good performances is a topic of great interest in fields such as inertial navigation,deep-sea fishing boat engines condition monitoring,seismic monitoring,attitude,and heading reference system,etc.This paper investigates two 6H-SIC MEMS diaphragms,one triangular and the other square,used in a fiber optic Fabry–Perot(FP)accelerometer in an experimental scenario.The triangular chip shows a wide working frequency range of 630 Hz–5300 Hz,a natural frequency of 44.3 k Hz,and a mechanical sensitivity of 0.154 nm/g.An optimal structure of the square chip used in a probe such as a fiber optic FP accelerometer also shows a wide working frequency range of 120 Hz–2300 Hz;a good sensitivity of 31.5 m V/g,a resonance frequency of7873 Hz,an accuracy of 0.96%F.S.,a frequency measurement error of 1.15%,and an excellent linearity of 0.9995.
基金financially supported by the National Natural Science Foundation of China(Nos.22435005,22193042,21921001,52202194,22305105,22201284)the Key Research Program of Frontier Sciences of the Chinese Academy of Sciences(No.ZDBSLY-SLH024)。
文摘Two-dimensional(2D)organic-inorganic hybrid perovskites(OIHPs)have been developed as promising candidates for photodetection,owing to their excellent semiconducting features and structural tunability.However,as an important parameter for photodetection,the photoresponsive range of 2D OIHPs is usually modulated by finite metal-halide combinations,constraining their further development.The emerging aromatic amine-based alternating-cations-interlayered(A-ACI)hybrid perovskites that exhibit excellent charge transport and additional interlayered structural designability,provide an extra solution for achieving ideal photoresponsive range.Herein,for the first time,the photoresponsive range is successfully broadened in A-ACI hybrid perovskites(NMA)_(4)(FA)_(2)Pb_(3)Br_(12)(2)remolding from(NMA)_(4)(MA)_(2)Pb_(3)Br_(12)(1)(NMA=N-methylbenzylaminium,FA=formamidinium and MA=methylammonium).Particularly,1 and 2adopt an unprecedented configuration that NMA and MA/FA are alternately arranged in the interlayer in a 4:2 manner.Importantly,2 exhibits a narrower bandgap than 1,which can be ascribed to the lowlying conduct band composed of intercalation FAπ*orbitals.Meanwhile,2 possesses a shorter interlayer distance and flatter inorganic skeleton,synergistically facilitating the wider photo-absorption range and further endowing a broadening photoresponsive range(70 nm).This research not only enriches the perovskite family but also provides insights into structure-property relationships.
